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Gallium behavior and isotopic compositions in marine siliceous sediments from the southern Mariana Trench 南马里亚纳海沟海相硅质沉积物中镓的行为和同位素组成
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2025-01-18 DOI: 10.1016/j.gloplacha.2025.104704
Guohong Qin, Zixiao Guo, Qingying Du, Yadong Liu, Lanping Feng, Xi Chen, Shahab Varkouhi, Daiyong Cao, Xiaotong Peng
To further constrain the contribution of marine siliceous sediments in the subduction zones to the oceanic gallium (Ga) cycle, we investigated Ga geochemical behavior by examining the mineral, elemental and Ga isotopic compositions of siliceous sediments from the southern Mariana Trench (SMT). The results show that Ga contents vary from 15.6 to 17.6 μg/g (average = 16.7 μg/g) in the lower part of the sediment core but the lower Ga contents (2.7 to 10.9 μg/g, average = 5.9 μg/g) in the upper part. The systematic variation in geochemistry and mineralogical compositions indicates that abundant Ga in the lower part originates from volcanogenic/basaltic rocks, while the addition of biogenic SiO2 to the upper part dilutes the concentration of these source-rock components, resulting in the concomitant decreases in contents of Ga and other elements. Particularly, reverse weathering leads to an increase of Ga in the top section of the upper part by favoring an uptake of Ga in the seawater into aluminosilicates, as evidenced by the range of pH, Al/Nb, Ga/Nb, and Ga/Al variations. In contrast, δ71Ga values (relative to the Ga-IPGP standard) show a monotonous range from −0.06 to 0.05 ‰ (average = −0.01 ‰, n = 17), which is consistent with those for basalts (0.00 ± 0.05 ‰). We find that the addition of biogenic SiO2 and reverse weathering do not significantly change the Ga isotopic compositions in the SMT marine siliceous sediments. Collectively, our study highlights that marine siliceous sediments in the SMT may act as an isotopically light sink of Ga in the modern ocean via reverse weathering, and could shed new light for understanding the oceanic Ga cycles.
为了进一步确定俯冲带海相硅质沉积物对海洋镓(Ga)旋回的贡献,我们通过检测南马里亚纳海沟(SMT)硅质沉积物的矿物、元素和Ga同位素组成来研究镓的地球化学行为。结果表明:下部Ga含量变化范围为15.6 ~ 17.6 μg/g(平均为16.7 μg/g),上部Ga含量变化范围为2.7 ~ 10.9 μg/g(平均为5.9 μg/g);地球化学和矿物组成的系统变化表明,下部丰富的Ga来源于火山/玄武岩,而上部生物源SiO2的加入稀释了这些源岩组分的浓度,导致Ga等元素含量降低。特别是,逆风化作用有利于将海水中的Ga吸收到铝硅酸盐中,从而导致上部顶部Ga含量的增加,这可以从pH、Al/Nb、Ga/Nb和Ga/Al的变化范围中得到证明。δ71Ga值(相对于Ga-IPGP标准)呈现单调的- 0.06 ~ 0.05‰(平均= - 0.01‰,n = 17),与玄武岩的δ71Ga值(0.00±0.05‰)一致。研究发现,生物成因SiO2的添加和逆风化作用对SMT海相硅质沉积物的Ga同位素组成没有显著影响。总的来说,我们的研究强调SMT海相硅质沉积物可能通过反风化作用在现代海洋中充当同位素轻的Ga汇,并为理解海洋Ga旋回提供了新的思路。
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引用次数: 0
Population migration with improved productivity caused a heterogeneity pattern of Holocene vegetation succession in typical areas of the lower Yangtze region 人口迁移和生产力的提高导致长江下游典型地区全新世植被演替呈现异质性格局
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2025-01-16 DOI: 10.1016/j.gloplacha.2025.104705
Li Xiao, Xiaoyu Zhang, Jinqi Dai, Xueming Li, Ning Zhao, Shihao Liu, Jing Chen, Maotian Li, Yuanhao Sun, Haoyan Wang, Kai Li, Yan Liu, Qianli Sun
Climate fluctuations and human activities shaped vegetation dynamics during the Holocene, yet the underlying mechanisms remain elusive. Our investigation utilizes the MAT-REVEALS approach to analyze 17 fossil pollen records spanning the past 8500 years collected at three typical areas of the lower Yangtze: South Zhejiang Mountains (SZJM), Taihu Basin (THB), and Yaojiang Valley (YJV). The reconstructed vegetation in SZJM revealed a high proportion of arboreal content during 8500–2000 cal yr BP, and the vegetation succession generally followed the variation of mean annual temperature and precipitation, indicating the Asian monsoon climate dominated the vegetation change. Of note, the minor decline of the broadleaved forest at 6000–5000 cal yr BP coincided with the drop in winter temperature, indicating its role as a limiting factor for the broadleaved arboreal. A marked increase of herbs (15.6 % to 36.5 %) occurred in the coastal region of YJV at 7500–5000 cal yr BP, which was not registered in SZJM, was coeval with a surging population and the start of extensive and intensive rice farming on the newly formed alluvial plain, indicating this noticeable landscape openness was induced by anthropogenic factors. Conversely, significant anthropogenic modifications of vegetation only emerged after 5000 cal yr BP in the THB, likely linked to large immigrations of population and the establishment of the Liangzhu hierarchical state that consumed abundant arboreal resources for large-scale constructions. Since 3000–2000 cal yr BP, a widespread decline of arboreal proportion took place in all three areas, which was coeval with a sharp decline of winter temperature as well as the introduction of bronze and later iron to this region during the Spring and Autumn to Three Kingdoms period. Notably, the decline in forest cover in the SZJM region was relatively late. However, it accelerated in the recent millennium, matching the timing of new immigrants from northern China during the Tang-Song dynasties. Overall, natural vegetation changes mainly followed the pattern of monsoon rainfall and winter temperature variations. Nevertheless, the heterogeneity pattern of vegetation changes on the coast underscored the pivotal role of the spatial-temporal distribution of population and advancing technology. This study highlights the regional and local impact of climatic and anthropogenic forces on vegetation composition, providing new insights for interpreting the timing and scale of human impact on past land cover and land use changes.
在全新世期间,气候波动和人类活动塑造了植被动态,但潜在的机制仍然难以捉摸。本研究利用mat -揭示方法分析了在浙南、太湖盆地和姚江流域3个长江下游典型地区采集的17份8500年花粉化石记录。8500 ~ 2000 cal yr BP期间,长江三角洲植被的乔木含量占比较高,植被演替总体上服从年平均气温和降水的变化,表明亚洲季风气候主导了植被的变化。值得注意的是,在6000 ~ 5000 cal yr BP,阔叶林的轻微下降与冬季气温的下降相吻合,表明冬季气温对阔叶林的限制作用。7500 ~ 5000 cal yr BP期间,长江流域沿海地区草本植物显著增加(15.6% ~ 36.5%),而长江流域未记录到这一变化,这与人口激增和新形成的冲积平原开始广泛集约种植水稻同时发生,表明这种明显的景观开放是由人为因素引起的。相反,人类对THB地区植被的显著改变仅在5000 cal yr BP之后才出现,这可能与人口的大规模移民和良渚等级国家的建立有关,这些国家消耗了大量的树木资源进行大规模建设。自3000-2000 cal yr BP以来,这三个地区树木比例普遍下降,与冬季气温急剧下降以及春秋三国时期青铜和后来的铁传入该地区同时发生。值得注意的是,SZJM地区森林覆盖下降的时间相对较晚。然而,在最近的千年里,它加速了,与唐宋时期来自中国北方的新移民的时间相匹配。总体而言,自然植被变化主要遵循季风降水和冬季气温变化的格局。然而,沿海植被变化的异质性格局强调了人口时空分布和技术进步的关键作用。该研究强调了气候和人为力量对植被组成的区域和局部影响,为解释人类对过去土地覆盖和土地利用变化的影响时间和规模提供了新的见解。
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引用次数: 0
Using seasonal palaeo-flow reconstructions and artificial neural networks for daily water balance modelling: A case study from Tasmania, Australia 利用季节性古水流重建和人工神经网络进行每日水量平衡建模:以澳大利亚塔斯马尼亚州为例
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2025-01-13 DOI: 10.1016/j.gloplacha.2025.104702
Danielle C. Verdon-Kidd, Kathryn J. Allen, Luke J. Kidd, Carolyn Maxwell, Mark Willis, Patrick Baker
Robust hydroclimate risk assessment requires a thorough understanding of past climate variability, which can be achieved by supplementing short instrumental hydroclimate records with palaeoclimate data. However, long-term continuous simulation of catchments and storage modelling, essential for hydrological risk assessment, necessitates monthly or daily time series input data, while palaeoclimate records are typically available at annual or seasonal scales. Additionally, modelling operational water storages used for hydropower is complex, requiring inputs such as water extraction information, which are difficult to replicate due to their inherent variability. Based on Lake Burbury, part of Hydro Tasmania's hydroelectric scheme in southern Australia, we demonstrate a novel method through which seasonal flow reconstructions can be used for daily palaeo water balance modelling, coupled with an Artificial Neural Network (ANN) model to simulate storage extractions. We first developed two seasonal tree-ring based inflow reconstructions, an approximately 1000-year Austral summer and a 400-year Austral winter reconstruction. We then used these as a guide to bootstrap historical daily inflows and the ANN known as Long Short-Term Memory (LSTM) was trained to simulate extractions for hydroelectricity. A Source model of the Lake Burbury hydro-electric water supply system was prepared to simulate the daily surface water balance of Lake Burbury, including inflows, outflows and resultant storage levels over some 1000 years. The simulations were used to ‘stress test’ the current storage system under a broader range of climatic conditions than the instrumental period. Based on our simulation, a low flow period like that in the 18th century represents the highest risk to hydroelectricity production, while a repeat of 12-13th century conditions would be associated with the highest spill volumes and most reliable electricity production. Importantly, by extending the instrumental record, we can place contemporary trends in water availability in a longer historical context, better assess the likelihood of extreme events, and hence adjust plans to decrease the vulnerability of the hydroelectric sector (among other water users) to drought/shifts in climate. This approach requires collaboration between palaeoclimatologists, the modelling community, hydrologists and managers of natural resources and the built environment.
可靠的水文气候风险评估需要对过去的气候变率有透彻的了解,这可以通过用古气候数据补充简短的仪器水文气候记录来实现。然而,对水文风险评估至关重要的集水区和储水模型的长期连续模拟需要每月或每天的时间序列输入数据,而古气候记录通常在年或季节尺度上可用。此外,对用于水力发电的运行储水进行建模是复杂的,需要诸如取水信息等输入,由于其固有的可变性,这些信息难以复制。基于澳大利亚南部塔斯马尼亚水电计划的一部分伯伯里湖,我们展示了一种新的方法,通过季节性流量重建可以用于日常古水平衡建模,再加上人工神经网络(ANN)模型来模拟存储提取。我们首先建立了两个基于季节树木年轮的流入重建,一个是大约1000年的南方夏季,一个是400年的南方冬季。然后,我们使用这些作为引导历史每日流入的指南,并训练被称为长短期记忆(LSTM)的人工神经网络来模拟水力发电的提取。准备了一个伯伯里湖水电供水系统的源模型来模拟伯伯里湖每天的地表水平衡,包括大约1000年来的流入、流出和由此产生的储水量。这些模拟被用来对当前的储存系统进行“压力测试”,在更大范围的气候条件下进行测试。根据我们的模拟,像18世纪那样的低流量时期代表着水力发电的最高风险,而重复12-13世纪的情况将与最高的泄漏量和最可靠的电力生产有关。重要的是,通过扩展仪器记录,我们可以在更长的历史背景下,将当代的水可用性趋势,更好地评估极端事件的可能性,从而调整计划,以减少水电部门(以及其他用水方)对干旱/气候变化的脆弱性。这种方法需要古气候学家、建模界、水文学家、自然资源和建筑环境管理者之间的合作。
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引用次数: 0
Flood occurrences and characteristics in Poland (Central Europe) in the last millennium 上个千年波兰(中欧)的洪水发生和特征
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2025-01-13 DOI: 10.1016/j.gloplacha.2025.104706
Babak Ghazi, Rajmund Przybylak, Piotr Oliński, Aleksandra Pospieszyńska
In the current era of global climate change, extreme events such as flood exposure are increasing globally. Knowledge about floods during historical periods is limited worldwide, mainly due to gaps in the documentary evidence and the lack of a reliable, comprehensive database. A new comprehensive database of floods in Poland in the 11th–18th centuries was created using quality-controlled documentary evidence. In addition, a list of floods for the 19th and 20th centuries was created based on a literature review. Using all these data, the frequency, intensity, genesis, and spatial distribution of floods in Poland in the last millennium were investigated. Results revealed the occurrence of 1680 floods in Poland in the last millennium. The 18th century was the most abundant in recorded floods (356, 21 %). Floods in the period 1001–1800 were most frequent in the Silesia region (553, 43 %) and in the Oder River basin (671, 55 %). The number of floods was greatest in summer (JJA, 46 %) and the lowest in autumn (SON, 8 %). An investigation of the origin of floods indicated that rain was the main contributing factor to the occurrences of floods in Poland (44 %). The estimation of the intensity of floods showed that most of them were of extreme nature: “above-average, or supra-regional flood” (33 %) and “extraordinary” floods (70 %). Analysis of the multi-temporal trend demonstrated that, overall, for the periods of 1501–1700 and 1601–1800, positive trends were more numerous than negative trends, whereas, for 1801–2000, negative trends were slightly more numerous than positive trends.
在当前全球气候变化的时代,洪水等极端事件在全球范围内不断增加。世界范围内关于历史时期洪水的知识有限,主要是由于文献证据的缺失和缺乏可靠、全面的数据库。一个关于11 - 18世纪波兰洪水的新的综合数据库被建立起来,使用的是有质量控制的文献证据。此外,根据文献综述,还列出了19世纪和20世纪的洪水清单。利用所有这些数据,我们调查了过去一千年波兰洪水的频率、强度、成因和空间分布。结果显示,在过去的一千年里,波兰发生了1680次洪水。18世纪是有记录以来发生洪水最多的世纪(356.21%)。2001年至1800年期间,西里西亚地区(553.43%)和奥得河流域(671.55%)的洪水最为频繁。夏季洪涝次数最多(JJA, 46%),秋季最少(SON, 8%)。对洪水起源的调查表明,降雨是波兰发生洪水的主要因素(44%)。对洪水强度的估计表明,大多数洪水属于极端性质:“高于平均水平或超区域洪水”(33%)和“异常”洪水(70%)。多时段趋势分析表明,总体而言,1501-1700年和1601-1800年期间,正趋势多于负趋势,而1801-2000年期间,负趋势略多于正趋势。
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引用次数: 0
Enhanced human activities have disturbed the vegetation-climate relationship over the last millennium in the Changbai Mountains, north-east China 近一千年来,人类活动加剧扰乱了中国东北长白山地区的植被-气候关系
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2025-01-09 DOI: 10.1016/j.gloplacha.2025.104701
Lina Song, Dongmei Jie, Feng Xie, Guizai Gao, Xianyong Cao
Understanding long-term regional anthropogenic impacts on vegetation can enhance our knowledge of natural environmental development. In this study, a 140-cm-long peat core covering the last ∼2850 years collected from the Changbai Mountain range was analysed for pollen and charcoal, to reconstruct vegetation and fire history, and to investigate the intensity and effects of human activities. Results show that the forest gradually shrank as precipitation decreased before around 1000 cal yr BP, characterised by the relative changes between Pinus and broad-leaved taxa. Over the last millennium, the forest further shrank, with broad-leaved components relatively increasing and herbaceous species significantly expanding at the cost of Pinus. Human activities in the Changbai Mountains have intensified since 1500 cal yr BP, as inferred from the increase in anthropogenic pollen indicators, along with a rise in both the frequency and intensity of palaeofire. Notably, human activities via the selective felling of Pinus and facilitation of the expansion of herbaceous species have disturbed the vegetation-climate relationship and thus introduced a bias into pollen-based climate reconstructions covering the last millennium. Additionally, human activities increased the frequency and intensity of palaeofire, with a significant contribution of local fires. We highlight that in the context of enhanced anthropogenic impact on the natural vegetation, pollen-based palaeoclimate reconstructions should be approached carefully.
了解长期区域人为对植被的影响可以提高我们对自然环境发展的认识。在这项研究中,研究人员分析了长白山140厘米长的泥炭岩心,分析了过去~ 2850年的花粉和木炭,重建了植被和火灾历史,并研究了人类活动的强度和影响。结果表明:在1000 calyr BP之前,森林面积随着降水的减少而逐渐缩小,其特征是松林与阔叶类群之间的相对变化;在过去的一千年里,森林进一步缩小,阔叶成分相对增加,草本物种显著增加,以松树为代价。1500 calyr BP以来,人类活动在长白山地区有所加剧,古火发生的频率和强度均有所增加。值得注意的是,人类活动通过对松林的选择性砍伐和促进草本物种的扩张扰乱了植被-气候关系,从而引入了基于花粉的气候重建,覆盖了过去一千年。此外,人类活动增加了古火的频率和强度,其中局部火灾的贡献很大。在人类活动对自然植被影响增强的背景下,应谨慎地进行基于花粉的古气候重建。
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引用次数: 0
Westerlies migrations and volcanic records over the past 4000 years from the Azores lacustrine sequences. Exploring correlations and impacts on Western Europe 亚速尔群岛湖泊序列中过去4000年的西风迁移和火山记录。探索对西欧的相关性和影响
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2025-01-08 DOI: 10.1016/j.gloplacha.2025.104698
Alberto Sáez, Armand Hernández, Adriano Pimentel, Mariana Andrade, Roberto Bao, Pedro M. Raposeiro, Vitor Gonçalves, Mario Benavente, Sergi Pla-Rabes, Ricardo Ramalho, Santiago Giralt
The Azores region plays a crucial role as a pathway for precipitation fronts traversing the North Atlantic from west to east, driven by the prevailing westerly winds. Variations in the strength of the Azores High affect the dynamics of the North Atlantic Oscillation (NAO), leading to latitudinal shifts in the trajectory of the westerlies and jet stream current over time.
亚速尔群岛地区在盛行的西风的驱动下,作为从西向东穿越北大西洋的降水锋面的通道,发挥着至关重要的作用。亚速尔高压强度的变化影响北大西洋涛动(NAO)的动力学,导致西风带和急流的轨迹随时间的纬度变化。
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引用次数: 0
Magnetic evidence of redox transition event in the Okinawa Trough during the early-middle Holocene and its links to the Kuroshio Current evolution 全新世早中期冲绳海槽氧化还原转变事件的磁学证据及其与黑潮演化的联系
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2025-01-07 DOI: 10.1016/j.gloplacha.2025.104699
Feng Wang, Tuqin Huang, Zhongbo Wang, Weiguo Zhang, Pengyu Qiao, Haiyan Tang, Xi Mei, Ping Yin, Zhongping Lai
The Kuroshio Current significantly influences the physical, chemical, and biological properties in the western Pacific Ocean, while its strength and path in the Okinawa Trough during the Holocene remains unclear. Previous studies have not established consistent conclusions due to the multiple explanations for sediment provenance proxies, but these inconsistencies can potentially be addressed by identifying redox variability through diagenetic effects on magnetic minerals. Magnetic data (χ, SIRM, χARM, and S-ratios) obtained from cores SHDZ10 and A4 in the middle Okinawa Trough indicate an intensified reductive diagenesis effect prior to the early-middle Holocene period, whereas a contrasting trend is observed since the early-middle Holocene. Geochemical analyses (Mo, Mn, Mo/Mn, Mn/Al, TOC and TS) and Pulleniatina obliquiloculata content variations suggest that the decrease in early diagenesis since early-middle Holocene was a consequence of increased oxygenation, which is related to a strengthened Kuroshio Current and enhanced deep-water ventilation. By synthesizing the observed redox transition phenomena in nearby sediment cores (MD012403, MD012404, KX12–3, MD063–05, CSH1), we discover a coherent redox transition event during the early-middle Holocene. The occurrence ages show millennial-scale variability from south to north, which may suggest a periodic northward movement trajectory of a strengthened Kuroshio Current. This study not only provides novel insights into the reconstruction of the Kuroshio Current evolution, but also highlights the applicability of environmental magnetism methods in investigating deep-water ventilation.
黑潮对西太平洋的物理、化学和生物特性有显著影响,但其在全新世冲绳海槽的强度和路径尚不清楚。由于对沉积物物源的多种解释,以往的研究尚未得出一致的结论,但这些不一致性可以通过对磁性矿物的成岩作用确定氧化还原变异性来解决。冲绳海槽中部SHDZ10和A4岩心的磁性资料(χ、SIRM、χ arm和s比)表明,早中全新世之前还原成岩作用增强,而早中全新世以来则呈现相反的趋势。地球化学分析(Mo、Mn、Mo/Mn、Mn/Al、TOC和TS)和斜叶扁豆(Pulleniatina obliquilocata)含量变化表明,全新世早中期以来早期成岩作用减少是氧化作用增强的结果,这与黑潮增强和深水通风增强有关。综合观测到的MD012403、MD012404、KX12-3、MD063-05、CSH1等沉积物岩心的氧化还原转变现象,发现了全新世早中期前后的连续氧化还原转变事件。从南向北呈现出千禧年尺度的变化,这可能表明黑潮的周期性北移轨迹。该研究不仅为重建黑潮演化提供了新的见解,而且突出了环境磁学方法在研究深水通风中的适用性。
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引用次数: 0
Testing and improving brGMGTs-based paleotemperature estimates in peat sediments: Evidence from global surface peat samples and two well-dated Holocene peat cores in far Northwest China 基于brgmgts的泥炭沉积物古温度估算的检验与改进:来自全球地表泥炭样品和中国西北远地区两个全新世泥炭岩心的证据
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2025-01-07 DOI: 10.1016/j.gloplacha.2025.104700
Zhongwei Shen, Minghua Zhao, Tianyan Lin, Xiaoxu Qu, Haichun Guo, Jiantao Cao, Guodong Jia, Zhiguo Rao
BrGMGTs (branched glycerol monoalkyl glycerol tetraethers) are proposed as potential proxies for temperature estimation due to their constrained and consistent biological origin. However, discrepancies observed between brGMGTs-based proxies and MAAT (mean annual air temperature) have raised concerns about their applicability. Here, we analyzed surface samples from three peatlands across China, and two well-dated Holocene peat cores. We found: 1) surface peat samples showed that %brGMGTs (abundance of brGMGTs relative to brGMGTs and brGDGTs; brGDGTs: branched glycerol dialkyl glycerol tetraethers) and H-MBT (methylation degree of brGMGTs) were ineffective to represent temperature. 2) Holocene records of %brGMGTs and H-MBT were uncorrelated with MBT’5ME records (previously established as reliable temperature records) in the same cores, as well as with regional other proxy temperature records. Our data, along with the global peat dataset, indicated that brGMGTs are ineffective for temperature estimation under cold conditions (MAAT <10 °C). This ineffectiveness may be due to unfavorable temperature niches, changes in aerobic/anaerobic conditions and microbial communities. By setting a threshold (%brGMGTs >4 %), we found that H-MBT showed a higher positive correlation with MAAT (R2 = 0.50, p < 0.01, n = 26), compared to all samples (R2 = 0.47, p < 0.01, n = 72). Although this improvement in correlation is modest, it helps exclude samples with MAAT <10 °C. Our revised method for temperature estimation using brGMGTs could potentially be applied to peat sediments with MAAT ranging from 10 °C to 27 °C, enhancing their application for paleotemperature reconstruction in future research.
BrGMGTs(支链甘油单烷基甘油四醚)由于其受约束和一致的生物来源而被提出作为温度估计的潜在代理。然而,基于brgmgts的代用物与MAAT(年平均气温)之间观测到的差异引起了人们对其适用性的担忧。在这里,我们分析了来自中国三个泥炭地的地表样本,以及两个年代确定的全新世泥炭岩心。结果表明:1)表层泥炭样品中brGMGTs(相对于brGMGTs和brGMGTs的丰度)%;brGMGTs:支化甘油二烷基甘油四醚)和H-MBT (brGMGTs的甲基化程度)不能代表温度。2)全新世的% brgmgt和H-MBT记录与同一岩心的MBT’5ME记录(以前建立的可靠温度记录)以及区域其他代理温度记录不相关。我们的数据以及全球泥炭数据表明,在寒冷条件下(MAAT <10°C), brGMGTs对温度估计无效。这种无效可能是由于不利的温度生态位,好氧/厌氧条件和微生物群落的变化。通过设置阈值(%brGMGTs > 4%),我们发现H-MBT与MAAT有较高的正相关(R2 = 0.50, p <;0.01, n = 26),与所有样本相比(R2 = 0.47, p <;0.01, n = 72)。虽然这种相关性的改善是适度的,但它有助于排除MAAT <;10°C的样品。修正后的brGMGTs温度估算方法可应用于MAAT范围为10 ~ 27℃的泥炭沉积物,增强了其在未来研究中古温度重建的应用价值。
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引用次数: 0
Impact of the 1994–1997 temporary decrease in Northern Hemisphere stratospheric methane on the 1990s methane trend 1994-1997年北半球平流层甲烷暂时减少对1990年代甲烷趋势的影响
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2025-01-05 DOI: 10.1016/j.gloplacha.2025.104697
Yuanyuan Han, Shentao Li, Xinlong Tan, Wenyan Guo, Wuhu Feng, Xin Li, Feiyang Wang, Fei Xie
Methane (CH4) ranks as the second most significant anthropogenic greenhouse gas following carbon dioxide (CO2). It originates from a wide range of surface sources and subsequently enters the stratosphere through the tropical tropopause. In line with the observed positive trend in tropospheric CH4, stratospheric CH4 has shown an overall increase in the long-term trend. However, contrary to the continuous increase in tropospheric CH4, stratospheric CH4 exhibits a temporal decrease in the Northern Hemisphere middle and upper stratosphere during short-time periods. This study investigates the causes behind the decreasing trend of stratospheric CH4 in the Northern Hemisphere from 1991 to 2000. We find that the extreme decrease of stratospheric CH4 from July 1994 to May 1997 contributes to the overall decreasing trend of CH4 from 1991 to 2000. This extreme decrease is attributed to the weakened meridional component of the residual circulation. The weakened meridional component attenuates the transport of CH4-rich air from the low-latitude lower stratosphere to the mid-latitude middle and upper stratosphere, leading to the observed decrease in CH4. It is further found that the smallest SST gradient in the North Pacific and adjacent regions from 1980 to 2020 is identified as a significant factor contributing to the weakened residual circulation and the decrease in CH4. Simulations by a chemistry-climate model support the results.
甲烷(CH4)是仅次于二氧化碳(CO2)的第二大人为温室气体。它起源于广泛的地表来源,随后通过热带对流层顶进入平流层。与观测到的对流层CH4正趋势一致,平流层CH4在长期趋势上总体呈增加趋势。然而,与对流层CH4的持续增加相反,北半球平流层中上层CH4在短时间内呈现出时间上的减少。本研究探讨了1991 - 2000年北半球平流层CH4呈下降趋势的原因。1994年7月至1997年5月平流层CH4的极端减少是导致1991年至2000年CH4总体减少趋势的原因。这种极端的减少是由于剩余环流的经向成分减弱。经向分量减弱减弱了富CH4空气从低纬度平流层向中纬度平流层中上层的输送,导致观测到的CH4减少。1980 - 2020年北太平洋及邻近地区海温梯度最小是导致剩余环流减弱和CH4减少的重要因素。化学-气候模式的模拟支持了这一结果。
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引用次数: 0
Centennial to multidecadal scales variability of East Asian summer monsoon precipitation in North China during the Holocene 全新世东亚夏季风在华北地区降水的百年至几十年尺度变化
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2025-01-04 DOI: 10.1016/j.gloplacha.2025.104692
Dandan Wang, Qinghai Xu, Yuanhao Sun, Shengrui Zhang
Understanding the variability and forcing mechanisms of the East Asian summer monsoon (EASM) precipitation on different timescales is critically important given its potentially adverse influence on ecosystems and economic development in North China. We present a pollen-based, well-dated, ∼10 yr resolution quantitative precipitation reconstruction from an alpine lake in North China, which provides a detailed picture of EASM evolution during the past ∼11,860 years. Based on ensemble empirical mode decomposition (EEMD) method and spectral analysis, we have revealed the centennial to multidecadal scales variability of EASM precipitation and its possible driving mechanisms during the Holocene. Our results suggest that the mean annual precipitation (MAP) varied greatly during the Holocene, with the maximum precipitation (520 mm) occurring during 9500–5020 cal. yr BP, which was ∼20 % higher than present. On the centennial scale, EASM precipitation exhibited ∼500 yr, ∼200 yr, ∼130 yr, and ∼105 yr cycles. The amplitude of the ∼500 yr cycle varied greatly during the Holocene, being higher in the early and late Holocene and lower in the middle Holocene, which was possibly linked to changes in ocean circulation induced by freshwater influx to the North Atlantic. On the multidecadal scale, the EASM precipitation was dominated by a 70–90 yr cycle, which may be related to the solar activity cycle and ocean-atmosphere interactions at both high and low latitudes. Weaker (stronger) solar activity, combined with stronger El Niño-Southern Oscillation (ENSO) during the warm phase of the Pacific Interdecadal Oscillation (PDO) and a negative phase of the Atlantic Multidecadal Oscillation (AMO), caused lower (higher) sea surface temperatures (SSTs) in the Indo-West Pacific Warm Pool (IWPWP) region, resulted in weaker (stronger) EASM circulation and decreased (increased) precipitation in North China. Our findings provide significant enlightenment for distinguishing the contribution of natural factors to the changes in EASM precipitation under future global warming scenarios.
鉴于东亚夏季季候风降水对华北地区生态系统和经济发展的潜在不利影响,了解不同时间尺度上东亚夏季季候风降水的变率和强迫机制至关重要。我们从华北的一个高山湖泊中重建了基于花粉、年代明确、分辨率为 10 年的定量降水,详细描述了东亚夏季季候风在过去 11,860 年的演变过程。基于集合经验模式分解(EEMD)方法和频谱分析,我们揭示了全新世期间EASM降水的百年尺度到多年尺度变率及其可能的驱动机制。我们的研究结果表明,在全新世期间,平均年降水量(MAP)变化很大,最大降水量(520 毫米)出现在公元前 9500 至 5020 年期间,比现在高出 20%。在百年尺度上,EASM 降水量呈现出 500 年、200 年、130 年和 105 年的周期。在全新世期间,∼500 年周期的振幅变化很大,在全新世早期和晚期较高,而在全新世中期较低,这可能与淡水流入北大西洋引起的海洋环流变化有关。在多年代尺度上,EASM 降水量以 70-90 年为一个周期,这可能与太阳活动周期以及高纬度和低纬度的海洋-大气相互作用有关。太阳活动减弱(增强),加上太平洋年代际涛动(PDO)暖涛期厄尔尼诺-南方涛动(ENSO)增强和大西洋年代际涛动(AMO)负涛期,导致印度-西太平洋暖池(IWPWP)区域海表温度(SST)降低(升高),导致华北地区东亚-东南亚环流减弱(增强)和降水减少(增加)。我们的研究结果为区分未来全球变暖情景下自然因素对东亚大气环流降水变化的影响提供了重要启示。
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Global and Planetary Change
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