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U-series isotope constraints on the rates of aeolian-impacted basaltic weathering under tropical climate 热带气候下风成冲击玄武岩风化速率的u系列同位素约束
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-12-09 DOI: 10.1016/j.gloplacha.2024.104673
Guodong Ming, Jingyi Huang, Jiaru Sheng, Yingzeng Gong, Jiye Guo, Huimin Yu, Wenhan Cheng, Craig C. Lundstrom, Fang Huang
The chemical weathering of basalt rocks is crucial for stabilizing Earth's habitability and carbon cycle. Currently, the soil chemistry and weathering rates of basalt under significant aeolian influence are not fully understood. This study addresses this gap by investigating the U geochemistry and regolith production rates in a highly weathered basalt profile in Southern China. The εNd(0) values decrease from the bedrock sample (4.68) to the top soils (0.94), indicating aerosol input from the top. Dust accretion decrease downward and significantly affects the vertical distribution of U (R2 = 0.86), while the chemical mobilization of U is controlled by binding with Fe oxides-organic matter complexes (R2 = 0.33).
玄武岩的化学风化作用对稳定地球的宜居性和碳循环至关重要。目前,玄武岩在风成作用下的土壤化学性质和风化速率还不完全清楚。本研究通过研究中国南方高风化玄武岩剖面的U地球化学和风化层生成速率来解决这一空白。从基岩样品(4.68)到顶部土壤(0.94),εNd(0)值逐渐减小,表明气溶胶输入来自顶部。尘积向下减小,显著影响U的垂直分布(R2 = 0.86),而U的化学动员受铁氧化物-有机物配合物的结合控制(R2 = 0.33)。
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引用次数: 0
Triggering of a 2500-year coral shutdown in northern South China Sea by coupled East Asian Monsoon and El Niño–Southern Oscillation 东亚季风和厄尔尼诺Niño-Southern涛动耦合引发南海北部2500年珊瑚停摆
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-12-09 DOI: 10.1016/j.gloplacha.2024.104672
Fei Tan, Yunfeng Zhang, Guowei Fu, Qi Shi, Xiyang Zhang, Shengnan Zhou, Mingzhuang Wang, Guotao Zhang, Xiaoju Liu, Jian-xin Zhao, Hongqiang Yang
Rapid climate change is reshaping the ecological dynamics of coral reefs, posing significant challenges in understanding the long-term effects of environmental disturbances on reef development. In the current study, we conducted a chronological analysis and regional review of Holocene massive Porites corals in the northern South China Sea, revealing a unique episodic growth pattern, including a 2500-year growth hiatus. The findings suggest that this collapse was driven by the coupling of intensified East Asian winter monsoon and broader-scale El Niño–Southern Oscillation variability. Regional environmental drivers significantly influenced spatiotemporal variations in coral growth stagnation across the Pan-Pacific region. While future sea level rise and warming may benefit nearshore corals, the projected intensification of El Niño–Southern Oscillation variability could undermine the potential of the northern South China Sea as a coral refuge. Effective coral management and environmental mitigation measures are crucial to preventing further collapse of regional coral reefs.
快速的气候变化正在重塑珊瑚礁的生态动态,为了解环境干扰对珊瑚礁发展的长期影响带来了重大挑战。在目前的研究中,我们对南海北部全新世的大块珊瑚进行了年代分析和区域回顾,揭示了一种独特的偶发性生长模式,包括长达 2500 年的生长中断。研究结果表明,这种崩溃是由东亚冬季季风加强和更大范围的厄尔尼诺-南方涛动变率耦合驱动的。区域环境驱动因素极大地影响了泛太平洋地区珊瑚生长停滞的时空变化。虽然未来海平面上升和气候变暖可能有利于近岸珊瑚,但预计厄尔尼诺-南方涛动变率的加剧可能会削弱南海北部作为珊瑚避难所的潜力。有效的珊瑚管理和环境缓解措施对于防止区域珊瑚礁的进一步崩溃至关重要。
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引用次数: 0
Pacific Walker Circulation modulated millennial-scale East Asian summer monsoon rainfall variability over the past 40 kyr 太平洋沃克环流在过去40年调制了千禧年尺度东亚夏季风降雨变率
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-12-09 DOI: 10.1016/j.gloplacha.2024.104676
Yi Zhong, Yuxing Liu, Xiaojing Du, Xiaoxu Shi, Xing Xu, Zhengyao Lu, Stefanie Kaboth-Bahr, Mark J. Dekkers, Juan C. Larrasoaña, Keiji Horikawa, Chijun Sun, Liang Ning, André Bahr, Yanan Zhang, Debo Zhao, Jiabo Liu, Wenyue Xia, Jingyu Zhang, Sheng Yang, Hai Li, Xiaoyue Liang, Chenxi Hong, Zhengyang Dai, Yuanjie Li, Qingsong Liu
The millennial-scale hydroclimate variability in East Asia has been debated for a long time due to the lack of reliable precipitation records from southern China and inconsistent model simulations. Here, we reconstruct a 40-kyr rainfall record for southern China and Taiwan based on enviro-magnetic and clay mineral proxy parameters from a northern South China Sea marine sediment core. Both proxies suggest reduced East Asian Summer Monsoon (EASM) precipitation in the southern China-Taiwan region during North Atlantic cooling episodes. After integration with other EASM precipitation records and modeling results, we conclude that the spatial precipitation pattern across Southeast Asia is closely related to the strength of the Pacific Walker Circulation. This interpretation is supported by a model simulation that emphasizes the role of the Walker Circulation in transferring North Atlantic climate variability to the East Asian hydroclimate. Our findings contribute to resolving the disparities between precipitation proxies and model simulations in Southeast Asia.
由于缺乏可靠的华南降水记录以及模式模拟的不一致,东亚地区千年尺度的水文气候变异一直存在争议。在此,我们根据南海北部海相沉积岩芯的环境磁性和粘土矿物代用参数,重建了中国南部和台湾 40 年的降水记录。这两种代用参数都表明,在北大西洋降温期间,中国南部-台湾地区的东亚夏季季候风(EASM)降水量减少。结合其他东亚夏季季候风降水记录和模拟结果,我们得出结论:东南亚的降水空间模式与太平洋沃克环流的强度密切相关。这一解释得到了模型模拟的支持,模型模拟强调了沃克环流在将北大西洋气候变率传递到东亚水文气候中的作用。我们的发现有助于解决东南亚降水代用指标与模式模拟之间的差异。
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引用次数: 0
Late Miocene-early Pliocene hydroclimate evolution of the western Altiplano, northern Chile: Implications for aridification trends under warming climate conditions 智利北部Altiplano西部中新世晚期-上新世早期水文气候演化:气候变暖条件下干旱化趋势的影响
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-12-09 DOI: 10.1016/j.gloplacha.2024.104674
Carlie Mentzer, Carmala Garzione, Carlos Jaramillo, Luis Felipe Hinojosa, Jaime Escobar, Nataly Glade, Sebastian Gomez, Deepshikha Upadhyay, Aradhna Tripati, Kaustubh Thirumalai
The Miocene-Pliocene boundary (∼5.3 million years ago, Ma) represents a climate transition, where global warming resulted in a rise in sea surface temperatures from near modern values in the late Miocene, to sustained, warmer than modern values in the early Pliocene. Estimated atmospheric CO2 concentrations were within the range of anthropogenic values. Thus, this transition provides an opportunity to evaluate hydroclimate responses to warming, when the Earth system was in equilibrium with near modern atmospheric CO2 levels. Here, we utilize lacustrine carbonate stable and clumped isotope methods, and palynology, to investigate hydroclimate trends within the western Altiplano of Chile during the late Miocene and early Pliocene. The results provide observational support for a warmer and wetter-than-modern climate over these timeframes. However, increasing aridity across the Miocene-Pliocene boundary suggests a hydroclimate response to global climate forcing. Given the sensitivity of the region's climate to disturbances in tropical Pacific, ocean-atmospheric processes, we speculate that this aridification may reflect progressive weakening of the Pacific Walker Circulation, in response to global warming.
中新世-上新世边界(距今 530 万年前,Ma)是一个气候转变期,全球变暖导致海面温度从中新世晚期的接近现代温度值上升到上新世早期的持续、比现代温度值更高的温度值。估计的大气二氧化碳浓度在人为值范围之内。因此,当地球系统与接近现代的大气二氧化碳水平处于平衡状态时,这一转变为评估水文气候对变暖的反应提供了机会。在这里,我们利用湖泊碳酸盐稳定同位素和团块同位素方法以及古植物学,研究了智利西部阿尔蒂普拉诺在中新世晚期和上新世早期的水文气候趋势。研究结果为这些时期的气候比现代气候温暖湿润提供了观测支持。然而,中新世-上新世边界日益干旱的现象表明,水文气候对全球气候胁迫做出了反应。考虑到该地区气候对热带太平洋海洋-大气过程干扰的敏感性,我们推测这种干旱化可能反映了太平洋沃克环流因全球变暖而逐渐减弱。
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引用次数: 0
Sedimentary responses to climatic variations and Kuroshio intrusion into the northern South China Sea since the last deglaciation 末次冰期以来南海北部对气候变化和黑潮入侵的沉积响应
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-12-08 DOI: 10.1016/j.gloplacha.2024.104671
Chao Huang, Liyuan Wu, Jiansen Cheng, Xiaoxu Qu, Yongyi Luo, Huiling Zhang, Feng Ye, Gangjian Wei
The terrigenous sediment source-to-sink processes in marginal seas are governed by intricate interactions among climate, sea level, and ocean currents. The continental slope of the northern South China Sea (SCS) provides an excellent setting to examine these processes due to its substantial terrigenous influx and continuous sedimentation. In this study, we present a high-resolution sedimentary record from the northern SCS continental slope covering the last deglaciation. Analyses of Rare Earth Elements (REEs) and Sr–Nd isotopic compositions in the NH07 core indicate that the predominant source of terrigenous sediment was Taiwan. Grain size-standard deviation analysis identified two sensitive grain size components, with the sensitive component 2 used as a marker of the Kuroshio intrusion into the northern SCS through Luzon Strait. The intensity of the Kuroshio intrusion into the northern SCS was found to be inversely related to that of the open Pacific. The Asian monsoon and El Niño-Southern Oscillation (ENSO) significantly influenced the variability of the Kuroshio Current throughout the deglaciation period. During the interval 16, 000–11, 700 cal yr BP, variations in terrigenous influx were collectively driven by sea level changes and the intensity of the Kuroshio intrusion, while chemical weathering intensity was affected by the reworking of previously exposed shelf sediments due to sea level fluctuations. During the Holocene, however, the East Asian summer monsoon intensity became the primary factor influencing variations in terrigenous influx and chemical weathering.
边缘海的土著沉积物从源到汇过程受气候、海平面和洋流之间错综复杂的相互作用的支配。南中国海(SCS)北部的大陆坡因其大量的陆相沉积和持续的沉积作用,为研究这些过程提供了极佳的环境。在本研究中,我们展示了南中国海北部大陆坡涵盖末次脱冰期的高分辨率沉积记录。对NH07岩芯中稀土元素(REEs)和Sr-Nd同位素组成的分析表明,陆相沉积的主要来源是台湾。粒度标准偏差分析确定了两个敏感粒度分量,其中敏感分量 2 是黑潮通过吕宋海峡侵入南中国海北部的标志。研究发现,黑潮侵入南中国海北部的强度与开阔太平洋的强度成反比。亚洲季风和厄尔尼诺-南方涛动(ENSO)对黑潮在整个降冰期的变化有显著影响。在公元前16,000-11,700年期间,海平面变化和黑潮入侵强度共同驱动了土著涌入量的变化,而化学风化强度则受到海平面波动导致的先前裸露陆架沉积物再加工的影响。然而,在全新世期间,东亚夏季季风强度成为影响土著流入量和化学风化作用变化的主要因素。
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引用次数: 0
Magnetic susceptibility cyclostratigraphy of the lower Schwarzrand Subgroup in southern Namibia refines temporal calibration of late Ediacaran bilaterian radiation 纳米比亚南部下Schwarzrand亚群的磁化率旋回地层改进了晚埃迪卡拉世两侧辐射的时间定标
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-12-06 DOI: 10.1016/j.gloplacha.2024.104668
Zheng Gong, Iona Baillie, Lyle L. Nelson, Stacey H. Gerasimov, Catherine Rose, Emily F. Smith
The Nama Group in southern Namibia captures one of the best-preserved records of the last ∼10 million years of the Ediacaran Period, recording pivotal changes to Earth's biosphere and oceans. Within the Nama Group, the lower Schwarzrand Subgroup preserves early complex bilaterian trace fossils, but uncertainties surrounding the ages of their first occurrences hinder global correlation and the understanding of the rates at which critical biological changes occurred. This study presents magnetic susceptibility cyclostratigraphy of a recently acquired drill core that covers the Nudaus Formation and Nasep Member within the lower Schwarzrand Subgroup. Spectral analysis reveals a hierarchy of orbital cycles that could be responsible for the repeating depositional sequences at various length scales in the Schwarzrand Subgroup. Matching the wavelengths of the orbital cycles to their expected periodicities, we established sedimentation rates throughout the stratigraphy. Utilizing available UPb ages from correlative outcrop sections and the sedimentation rates from cyclostratigraphy, we refine the age-depth model for the lower Schwarzrand Subgroup. Our new age-depth model places tighter temporal constraints on the first appearances of complex trace fossils, thus constraining the earliest major radiation of bilaterian metazoans and contributing to a better-calibrated chronostratigraphy of the terminal Ediacaran Period.
纳米比亚南部的Nama群捕获了埃迪卡拉纪最后~ 1000万年保存最完好的记录之一,记录了地球生物圈和海洋的关键变化。在Nama群中,较低的Schwarzrand亚群保存了早期复杂的双边动物痕迹化石,但围绕它们首次出现的年龄的不确定性阻碍了全球相关性和对关键生物变化发生速度的理解。本文研究了最近获得的覆盖下Schwarzrand亚群中的Nudaus组和Nasep段的钻芯的磁化率旋回地层学。光谱分析揭示了Schwarzrand亚群中不同长度尺度的重复沉积序列的轨道旋回层次。将轨道旋回的波长与其预期的周期相匹配,我们确定了整个地层的沉积速率。利用相关露头剖面的UPb年龄和旋回地层的沉积速率,我们完善了下Schwarzrand亚群的年龄-深度模型。我们的新年龄-深度模型对复杂痕迹化石的首次出现施加了更严格的时间限制,从而限制了最早的双边后生动物的主要辐射,并有助于更好地校准埃迪卡拉末期的年代地层。
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引用次数: 0
Influence of climatic variables on biome transitions in the Colombian and Panamanian Caribbean region 气候变量对哥伦比亚和巴拿马加勒比地区生物群落转变的影响
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-12-04 DOI: 10.1016/j.gloplacha.2024.104669
Y. Nuñez-Bolaño, N. Hoyos, A. Correa-Metrio, C. Martínez, C. Pizano, J. Escobar, C. Huertas, C. Jaramillo
Disentangling the environmental determinants of tropical biomes is crucial for understanding their response to climate change. This study investigated the effect of climate and soil-related variables on biome transitions in the Caribbean region of Colombia and Panama, focusing on xerophytic forest (XF), tropical dry forest (TDF), and tropical rainforest (TRF). We analyzed the climatic variables at different time scales (daily, seasonal, and annual) and their interaction with soil properties. We performed an ordinal logistic regression to assess the combined effect of the most important variables in biome transitions. Our results showed that climate variables are major discriminators in our study region, particularly precipitation at a seasonal and annual scale. The ordinal logistic regression highlighted the significance of annual precipitation and dry-season length in biome transitions, with maximum temperature impacting TDF-TRF transitions. Soil differences, although present (e.g., higher sand content in XF), played a marginal role. Overall, our findings emphasize the dominance of climate over soil in shaping tropical biome distributions in the northern Caribbean part of South America. These findings contribute to a deeper understanding of tropical biome responses to climate change.
解开热带生物群落的环境决定因素对于理解它们对气候变化的反应至关重要。本文研究了气候和土壤相关变量对哥伦比亚和巴拿马加勒比地区生物群落转变的影响,重点研究了旱生林(XF)、热带干林(TDF)和热带雨林(TRF)。分析了不同时间尺度(日、季、年)的气候变量及其与土壤性质的相互作用。我们进行了有序逻辑回归来评估生物群落转变中最重要变量的综合影响。结果表明,气候变量是主要的判别因子,尤其是季节和年尺度上的降水。有序logistic回归结果表明,年降水量和干季长度对生物群落过渡具有显著影响,最高温度对TDF-TRF过渡具有显著影响。土壤差异虽然存在(如XF含沙量较高),但起了次要作用。总的来说,我们的研究结果强调了气候在塑造南美洲北加勒比地区热带生物群落分布方面的主导地位。这些发现有助于更深入地了解热带生物群落对气候变化的响应。
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引用次数: 0
Large ensemble simulations indicate increases in spatial compounding of droughts and hot extremes across multiple croplands in China 大集合模拟表明,中国多个农田的干旱和极端高温的空间复合增加
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-12-04 DOI: 10.1016/j.gloplacha.2024.104670
Boying Lv, Zengchao Hao, Yutong Jiang, Qian Ma, Yitong Zhang
The simultaneous occurrence of extremes (e.g., droughts) at multiple regions (usually termed as spatial compounding of extremes), such as croplands, may lead to large impacts on global food security. Recently, the concurrent droughts and hot extremes at a specific location, which are referred to as compound droughts and hot extremes (CDHEs), have garnered considerable attention due to the potentially amplified impacts of individual extremes. Though the spatial compounding of individual droughts or hot extremes has been assessed, the variability of the spatial compounding of CDHEs across multiple croplands in China has been lacking due to relatively short records or small sample sizes. In this study, we evaluated changes in the spatial compounding of CDHEs across multiple croplands in China, including Songnen Plain (SN), North China Plain (NC), and Sichuan Basin (SC), based on precipitation and temperature data from CN05.1 and large ensemble model (CESM1-CAM5). Results show that the frequency of CDHEs in each region will increase in future periods especially for the eastern SN, central NC, and northern SC (increase by more than 15 months), with more than 70 % of the 40 ensemble members showing a large increase. Projected changes of different cases of spatial compounding of CDHEs in three croplands (i.e., SN-NC, NC-SC, SN-SC, SN-NC-SC) showed increases from 1961–2010 to 2031–2080. In particular, higher increases in the spatial compounding of CDHEs in the NC-SC region are projected (from 0.58 to 3.73 months on average), with the ratio of non-zero event members increasing from 47.5 % to 95 %. These results underscore the high risk of the spatial compounding of extremes at multiple croplands in China in the future.
极端天气(如干旱)在多个区域(通常称为极端天气的空间复合)(如农田)同时发生,可能会对全球粮食安全造成巨大影响。最近,由于单个极端天气的影响可能会被放大,在特定地点同时出现的干旱和炎热极端天气(称为复合干旱和炎热极端天气(CDHEs))引起了广泛关注。虽然已经对单个干旱或高温极端天气的空间复合性进行了评估,但由于记录时间较短或样本量较小,一直缺乏对中国多个耕地的 CDHEs 空间复合性变化的研究。在本研究中,我们基于 CN05.1 和大型集合模式(CESM1-CAM5)的降水和温度数据,评估了中国松嫩平原、华北平原和四川盆地等多个耕地的 CDHEs 空间复合变化。结果表明,各地区CDHE的发生频率在未来一段时间内都将增加,尤其是四川东部、华北平原中部和四川盆地北部(增加15个月以上),在40个集合成员中超过70%的集合成员的CDHE发生频率都有较大幅度的增加。从 1961-2010 年到 2031-2080 年,三种耕地(即 SN-NC、NC-SC、SN-SC、SN-NC-SC)CDHEs 不同空间复合情况的预测变化均呈上升趋势。特别是,在 NC-SC 地区,CDHEs 的空间复合增长率预计更高(平均从 0.58 个月增至 3.73 个月),非零事件成员的比率从 47.5% 增至 95%。这些结果凸显了未来中国多耕地极端天气空间复合的高风险。
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引用次数: 0
Holocene dust activity in inland Asia driven by both the mid-latitude Westerlies and the East Asian winter monsoon 由中纬度西风带和东亚冬季风驱动的全新世亚洲内陆沙尘活动
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-12-02 DOI: 10.1016/j.gloplacha.2024.104661
Haipeng Wang, Jianhui Chen, Yuanhao Sun, Ruijin Chen, Nasetay Aydenbek, Jianbao Liu
Inland Asia is a major global source of dust and the dust transport from this region has global implications. However, the processes and forcing mechanisms of dust activity in inland Asia during the Holocene are still debated due to the lack of high-quality records with accurate dating, unambiguous dust signals, and a high resolution. Here we present a well-dated record of dust activity based on the Ti content of the sediments of Shuanghu Lake, in the southern Altai Mountains, with a ∼ 15-yr-resolution and covering the entire Holocene. This record shows a gradual decrease in dust intensity during ∼11.7–6 thousand years ago (ka), followed by a persistent increase since ∼6 ka. Frequent dust events are also evident, lasting hundreds of years, and are superimposed on the millennial-scale trend, corresponding to the nine North Atlantic Bond events. We propose that the millennial-scale trend of dust activity was primarily influenced by variations in the mid-latitude Westerlies, while the dust events on the centennial scale were driven primarily by a strengthened East Asian winter monsoon. Overall, this study provides a reliable, high-resolution record of Holocene dust activity in inland Asia, and it updates the previous view that dust activity in this region was solely controlled by the mid-latitude Westerlies or the Siberian High. Our findings contribute to an improved understanding of global dust transport with implications for predicting future dust activity in this region.
亚洲内陆是全球主要的沙尘来源,该地区的沙尘输送具有全球影响。然而,由于缺乏精确测年、明确沙尘信号和高分辨率的高质量记录,亚洲内陆全新世沙尘活动的过程和强迫机制仍然存在争议。在这里,我们根据阿尔泰山脉南部双湖沉积物的Ti含量,提供了一个精确的尘埃活动记录,具有~ 15年的分辨率,覆盖了整个全新世。该记录显示,在~ 11.7-6千年前(ka),尘埃强度逐渐下降,随后自~ 6 ka以来持续增加。频繁的沙尘事件也很明显,持续了数百年,并叠加在千年尺度的趋势上,对应于9次北大西洋Bond事件。千年尺度的沙尘活动趋势主要受中纬度西风带变化的影响,而百年尺度的沙尘活动主要受东亚冬季风增强的驱动。总体而言,本研究提供了可靠的、高分辨率的亚洲内陆全新世沙尘活动记录,更新了以往认为该地区沙尘活动仅受中纬度西风带或西伯利亚高压控制的观点。我们的发现有助于提高对全球沙尘运输的理解,并有助于预测该地区未来的沙尘活动。
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引用次数: 0
Dual carbon isotopes constrain the sources and age variations of terrestrial organic carbon in the middle Okinawa Trough since the last deglaciation 双碳同位素限制了冲绳海槽中部末次消冰期以来陆相有机碳的来源和年龄变化
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-11-29 DOI: 10.1016/j.gloplacha.2024.104660
Mengna Chen, Chenglong Su, Shuang Wang, Da-Wei Li, Hailong Zhang, Li Li, Guangxue Li, Bingyuan Xu, Jishang Xu, Meixun Zhao
The burial of terrestrial organic carbon (OC) in marine sediments is a crucial process in the global carbon cycle, as it transfers carbon from relatively active to inactive reservoirs. However, there remains a limited understanding of the spatial and temporal variations in the source and age characteristics of terrestrial OC in marine sediments, which determine its ability to serve as a contemporary carbon sink. In this study, radiocarbon isotope (14C, expressed as F14C) analysis was conducted on bulk OC from a sediment core (M063–05) collected from the middle Okinawa Trough, with core depositional ages spanning 1.5–16.1 ka. A novel mathematical approach was developed to differentiate the carbon isotope signals of terrestrial OC from those of bulk OC properties, enabling the investigation of the source, age, and burial flux of terrestrial OC in the Okinawa Trough. Our results indicate that sedimentary OC in the Okinawa Trough was predominantly composed of marine OC (average proportion, 58 %), with terrestrial OC present to a lesser extent (average proportion, 42 %). Terrestrial OC in core M063–05 was found to be primarily a mixture of terrestrial OC from the Huanghe (Yellow River) and petrogenic OC from Taiwan Island, and the apparent initial ages of terrestrial OC (AIRterrestrial) exhibited higher values of 7933–8886 yr during the mid-late Holocene compared to 3062–7677 yr during the marine transgression stage. The elevated AIRterrestrial during sea level highstand was attributed to (1) increased petrogenic OC input from Taiwan Island due to the intensified Kuroshio Current, which transports material from Taiwan northward along the Okinawa Trough, and (2) vigorous hydrodynamic processes in the continental shelves of the East China marginal seas, leading to significant aging of terrestrial OC during lateral transport. This innovative dual carbon isotope-based approach (enumeration method) elucidates the temporal variations in terrestrial OC sources and age characteristics in a typical continental slope within the western Pacific Ocean, providing a framework for investigating the sources and fate of terrestrial OC in marginal seas, especially in scenarios where potential changes in carbon isotope endmembers occur in response to climate and environmental changes.
海洋沉积物中陆相有机碳的埋藏是全球碳循环的一个重要过程,因为它将碳从相对活跃的储集层转移到不活跃的储集层。然而,对海洋沉积物中陆相OC的来源和年龄特征的时空变化的了解仍然有限,这决定了其作为当代碳汇的能力。本文对冲绳海槽中部沉积岩心(M063-05)的大块OC进行了放射性碳同位素(14C,用F14C表示)分析,岩心沉积年龄为1.5 ~ 16.1 ka。提出了一种新的区分陆相OC与块状OC特征碳同位素信号的数学方法,从而对冲绳海槽陆相OC的来源、年龄和埋藏通量进行了研究。结果表明,冲绳海槽沉积OC以海相OC为主(平均比例为58%),陆相OC较少(平均比例为42%)。M063-05岩心陆相OC主要为黄河陆相OC与台湾岩源OC的混合,其表观初始年龄(AIRterrestrial)在全新世中晚期为7933-8886 yr,高于海侵期的3062-7677 yr。海平面高水位期间AIRterrestrial升高的主要原因是:(1)黑潮强化了台湾沿冲绳海槽向北输送物质,增加了台湾岛的成岩OC输入;(2)东部边缘海大陆架剧烈的水动力过程导致陆地OC在横向输送过程中明显老化。这种创新的基于双碳同位素的方法(枚举法)阐明了西太平洋典型大陆斜坡陆相OC来源的时间变化和年龄特征,为研究边缘海陆相OC的来源和命运提供了框架,特别是在碳同位素端元可能发生变化的情况下响应气候和环境变化。
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Global and Planetary Change
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