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Two-dimensional polarized MoSSe/MoTe2 van der Waals heterostructure: A polarization-tunable optoelectronic material 二维极化MoSSe/MoTe2范德华异质结构:一种偏振可调光电材料
IF 7.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-09-06 DOI: 10.1007/s11467-023-1330-2
Fahhad Alsubaie, Munirah Muraykhan, Lei Zhang, Dongchen Qi, Ting Liao, Liangzhi Kou, Aijun Du, Cheng Tang

Two-dimensional (2D) heterostructures have shown great potential in advanced photovoltaics due to their restrained carrier recombination, prolonged exciton lifetime and improved light absorption. Herein, a 2D polarized heterostructure is constructed between Janus MoSSe and MoTe2 monolayers and is systematically investigated via first-principles calculations. Electronically, the valence band and conduction band of the MoSSe–MoTe2 (MoSeS–MoTe2) are contributed by MoTe2 and MoSSe layers, respectively, and its bandgap is 0.71 (0.03) eV. A built-in electric field pointing from MoTe2 to MoSSe layers appears at the interface of heterostructures due to the interlayer carrier redistribution. Notably, the band alignment and built-in electric field make it a direct z-scheme heterostructure, benefiting the separation of photogenerated electron-hole pairs. Besides, the electronic structure and interlayer carrier reconstruction can be readily controlled by reversing the electric polarization of the MoSSe layer. Furthermore, the light absorption of the MoSSe/MoTe2 heterostructure is also improved in comparison with the separated monolayers. Consequently, in this work, a new z-scheme polarized heterostructure with polarization-controllable optoelectronic properties is designed for highly efficient optoelectronics.

二维异质结构具有抑制载流子复合、延长激子寿命和改善光吸收等优点,在先进光伏电池中显示出巨大的潜力。本文在Janus MoSSe和MoTe2单层之间构建了二维极化异质结构,并通过第一性原理计算进行了系统的研究。MoSSe - MoTe2的价带和导带分别由MoTe2层和MoSSe层贡献,其带隙为0.71 (0.03)eV。由于层间载流子的重新分布,在异质结构界面处出现了从MoTe2指向MoSSe层的内置电场。值得注意的是,带对准和内置电场使其成为直接的z-scheme异质结构,有利于光生电子-空穴对的分离。此外,通过反转MoSSe层的电极化,可以很容易地控制电子结构和层间载流子重构。此外,与分离的单层相比,MoSSe/MoTe2异质结构的光吸收也得到了改善。因此,在本工作中,设计了一种具有偏振可控光电子特性的新型z-scheme极化异质结构,用于高效光电子学。
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引用次数: 0
Distributed exact Grover’s algorithm 分布式精确格罗弗算法
IF 7.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-08-14 DOI: 10.1007/s11467-023-1327-x
Xu Zhou, Daowen Qiu, Le Luo

Distributed quantum computation has gained extensive attention. In this paper, we consider a search problem that includes only one target item in the unordered database. After that, we propose a distributed exact Grover’s algorithm (DEGA), which decomposes the original search problem into ⌊n/2⌋ parts. Specifically, (i) our algorithm is as exact as the modified version of Grover’s algorithm by Long, which means the theoretical probability of finding the objective state is 100%; (ii) the actual depth of our circuit is 8(n mod 2) + 9, which is less than the circuit depths of the original and modified Grover’s algorithms, (1 + 8leftlfloor {{pi over 4}sqrt {{2^n}} } rightrfloor ) and (9 + 8leftlfloor {{pi over 4}sqrt {{2^n}} - {1 over 2}} rightrfloor ), respectively. It only depends on the parity of n, and it is not deepened as n increases; (iii) we provide particular situations of the DEGA on MindQuantum (a quantum software) to demonstrate the practicality and validity of our method. Since our circuit is shallower, it will be more resistant to the depolarization channel noise.

分布式量子计算得到了广泛的关注。本文考虑一个在无序数据库中只包含一个目标项的搜索问题。在此基础上,提出了一种分布式精确格罗弗算法(DEGA),该算法将原搜索问题分解为⌊n/2⌋部分。具体来说,(i)我们的算法与Long对Grover算法的改进版本一样精确,即找到目标状态的理论概率为100%; (ii) the actual depth of our circuit is 8(n mod 2) + 9, which is less than the circuit depths of the original and modified Grover’s algorithms, (1 + 8leftlfloor {{pi over 4}sqrt {{2^n}} } rightrfloor ) and (9 + 8leftlfloor {{pi over 4}sqrt {{2^n}} - {1 over 2}} rightrfloor ), respectively. It only depends on the parity of n, and it is not deepened as n increases; (iii) we provide particular situations of the DEGA on MindQuantum (a quantum software) to demonstrate the practicality and validity of our method. Since our circuit is shallower, it will be more resistant to the depolarization channel noise.
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引用次数: 1
Taiji data challenge for exploring gravitational wave universe 探索引力波宇宙的太极数据挑战
IF 7.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-08-11 DOI: 10.1007/s11467-023-1318-y
Zhixiang Ren, Tianyu Zhao, Zhoujian Cao, Zong-Kuan Guo, Wen-Biao Han, Hong-Bo Jin, Yue-Liang Wu

The direct observation of gravitational waves (GWs) opens a new window for exploring new physics from quanta to cosmos and provides a new tool for probing the evolution of universe. GWs detection in space covers a broad spectrum ranging over more than four orders of magnitude and enables us to study rich physical and astronomical phenomena. Taiji is a proposed space-based gravitational wave (GW) detection mission that will be launched in the 2030s. Taiji will be exposed to numerous overlapping and persistent GW signals buried in the foreground and background, posing various data analysis challenges. In order to empower potential scientific discoveries, the Mock Laser Interferometer Space Antenna (LISA) data challenge and the LISA data challenge (LDC) were developed. While LDC provides a baseline framework, the first LDC needs to be updated with more realistic simulations and adjusted detector responses for Taiji’s constellation. In this paper, we review the scientific objectives and the roadmap for Taiji, as well as the technical difficulties in data analysis and the data generation strategy, and present the associated data challenges. In contrast to LDC, we utilize second-order Keplerian orbit and second-generation time delay interferometry techniques. Additionally, we employ a new model for the extreme-mass-ratio inspiral waveform and stochastic GW background spectrum, which enables us to test general relativity and measure the non-Gaussianity of curvature perturbations. Furthermore, we present a comprehensive showcase of parameter estimation using a toy dataset. This showcase not only demonstrates the scientific potential of the Taiji data challenge (TDC) but also serves to validate the effectiveness of the pipeline. As the first data challenge for Taiji, we aim to build an open ground for data analysis related to Taiji sources and sciences. More details can be found on the official website (taiji-tdc.ictp-ap.org).

引力波的直接观测为探索从量子到宇宙的新物理打开了一扇新的窗口,为探索宇宙演化提供了一种新的工具。在太空中探测地球引力波覆盖了超过四个数量级的广泛光谱,使我们能够研究丰富的物理和天文现象。“太极”是一项拟议中的天基引力波探测任务,将于本世纪30年代发射。Taiji将暴露在大量重叠和持续的GW信号中,这些信号隐藏在前景和背景中,对数据分析提出了各种挑战。为了支持潜在的科学发现,开发了模拟激光干涉仪空间天线(LISA)数据挑战和LISA数据挑战(LDC)。虽然LDC提供了一个基线框架,但第一个LDC需要更新更真实的模拟,并调整探测器对太极星座的响应。本文回顾了太极的科学目标和发展路线图,以及在数据分析和数据生成策略方面的技术难点,并提出了相关的数据挑战。与LDC相比,我们利用了二阶开普勒轨道和第二代延迟干涉测量技术。此外,我们采用了一个新的模型,用于极端质量比吸气波形和随机GW背景谱,使我们能够检验广义相对论和测量曲率摄动的非高斯性。此外,我们还全面展示了使用玩具数据集进行参数估计的方法。这次展示不仅展示了Taiji数据挑战(TDC)的科学潜力,而且还有助于验证该管道的有效性。作为太极的第一个数据挑战,我们的目标是建立一个与太极来源和科学相关的数据分析的开放场所。更多细节可以在官方网站(taiji-tdc.ictp-ap.org)上找到。
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引用次数: 2
Structure and dynamics of binary Bose–Einstein condensates with vortex phase imprinting 具有涡旋相印迹的二元玻色-爱因斯坦凝聚体的结构和动力学
IF 7.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-07-26 DOI: 10.1007/s11467-023-1316-0
Jianchong Xing, Wenkai Bai, Bo Xiong, Jun-Hui Zheng, Tao Yang

The combination of multi-component Bose–Einstein condensates (BECs) and phase imprinting techniques provides an ideal platform for exploring nonlinear dynamics and investigating the quantum transport properties of superfluids. In this paper, we study abundant density structures and corresponding dynamics of phase-separated binary Bose–Einstein condensates with phase-imprinted single vortex or vortex dipole. By adjusting the ratio between the inter-species and intra-species interactions, and the locations of the phase singularities, the typical density profiles such as ball-shell structures, crescent-gibbous structures, Matryoshka-like structures, sector-sector structures and sandwich-type structures appear, and the phase diagrams are obtained. The dynamics of these structures exhibit diverse properties, including the penetration of vortex dipoles, emergence of halfvortex dipoles, co-rotation of sectors, and oscillation between sectors. The pinning effects induced by a potential defect are also discussed, which is useful for controlling and manipulating individual quantum states.

多组分玻色-爱因斯坦凝聚体(BECs)和相印迹技术的结合为探索非线性动力学和研究超流体的量子输运特性提供了理想的平台。本文研究了相印单涡旋或涡旋偶极子相分离二元玻色-爱因斯坦凝聚体的丰富密度结构和相应的动力学。通过调整种间和种内相互作用的比例以及相奇点的位置,出现了典型的球壳结构、新月形结构、套娃结构、扇区-扇区结构和三明治型结构等密度分布,并得到了相图。这些结构的动力学表现出不同的特性,包括涡旋偶极子的穿透、半涡旋偶极子的出现、扇区的共旋以及扇区之间的振荡。讨论了由潜在缺陷引起的钉住效应,这对控制和操纵单个量子态是有用的。
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引用次数: 0
High-sensitive two-dimensional PbI2 photodetector with ultrashort channel 超短通道高灵敏度二维PbI2光电探测器
IF 7.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-07-26 DOI: 10.1007/s11467-023-1323-1
Kaiyue He, Jijie Zhu, Zishun Li, Zhe Chen, Hehe Zhang, Chao Liu, Xu Zhang, Shuo Wang, Peiyi Zhao, Yu Zhou, Shizheng Zhang, Yao Yin, Xiaorui Zheng, Wei Huang, Lin Wang

Photodetectors based on two-dimensional (2D) semiconductors have attracted many research interests owing to their excellent optoelectronic characteristics and application potential for highly integrated applications. However, the unique morphology of 2D materials also restricts the further improvement of the device performance, as the carrier transport is very susceptible to intrinsic and extrinsic environment of the materials. Here, we report the highest responsivity (172 A/W) achieved so far for a PbI2-based photodetector at room temperature, which is an order of magnitude higher than previously reported. Thermal scanning probe lithography (t-SPL) was used to pattern electrodes to realize the ultrashort channel (~60 nm) in the device. The shortening of the channel length greatly reduces the probability of the photo-generated carriers being scattered during the transport process, which increases the photocurrent density and thus the responsivity. Our work shows that the combination of emerging processing technologies and 2D materials is an effective route to shrink device size and improve device performance.

基于二维半导体的光电探测器以其优异的光电特性和高集成度的应用潜力引起了人们的广泛关注。然而,二维材料的独特形态也限制了器件性能的进一步提高,因为载流子输运非常容易受到材料的内在和外在环境的影响。在这里,我们报告了迄今为止在室温下实现的基于pbi2的光电探测器的最高响应率(172 A/W),这比以前报道的要高一个数量级。利用热扫描探针光刻技术(t-SPL)对电极进行图像化,实现了器件内的超短通道(~60 nm)。通道长度的缩短大大降低了光生载流子在传输过程中散射的概率,从而提高了光电流密度,从而提高了响应率。我们的工作表明,新兴加工技术与二维材料的结合是缩小器件尺寸和提高器件性能的有效途径。
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引用次数: 0
Generation and modulation of multiple 2D bulk photovoltaic effects in space-time reversal asymmetric 2H-FeCl2 时空反转不对称2H-FeCl2中多重2D体光伏效应的产生和调制
IF 7.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-07-26 DOI: 10.1007/s11467-023-1320-4
Liang Liu, Xiaolin Li, Luping Du, Xi Zhang

The two-dimensional (2D) bulk photovoltaic effect (BPVE) is a cornerstone for future highly efficient 2D solar cells and optoelectronics. The ferromagnetic semiconductor 2H-FeCl2 is shown to realize a new type of BPVE in which spatial inversion (P), time reversal (T), and space–time reversal (PT) symmetries are broken (PT-broken). Using density functional theory and perturbation theory, we show that 2H-FeCl2 exhibits giant photocurrents, photo-spin-currents, and photo-orbital-currents under illumination by linearly polarized light. The injection-like and shift-like photocurrents coexist and propagate in different directions. The material also demonstrates substantial photoconductance, photo-spin-conductance, and photo-orbital-conductance, with magnitudes up to 4650 (nm·µA/V2), 4620 [nm·µA/V2ħ/(2e)], and 6450 (nm·µA/V2ħ/e), respectively. Furthermore, the injection-currents, shift-spin-currents, and shift-orbital-currents can be readily switched via rotating the magnetizations of 2H-FeCl2. These results demonstrate the superior performance and intriguing control of a new type of BPVE in 2H-FeCl2.

二维体光伏效应(BPVE)是未来高效二维太阳能电池和光电子技术的基石。铁磁半导体2H-FeCl2实现了空间反演(P)、时间反演(T)和时空反演(PT)对称性被打破(PT-broken)的新型BPVE。利用密度泛函理论和微扰理论,我们证明了在线偏振光照射下,2H-FeCl2表现出巨大的光电流、光自旋电流和光轨道电流。类注入光电流和类移位光电流共存,并向不同方向传播。该材料还表现出可观的光电导、光自旋电导和光轨道电导,其量级分别高达4650 (nm·µA/V2)、4620 (nm·µA/ v2h / 2e)和6450 (nm·µA/ v2h /e)。此外,注入电流、移位自旋电流和移位轨道电流可以通过旋转2H-FeCl2的磁化而容易地切换。这些结果证明了一种新型BPVE在2H-FeCl2中的优越性能和有趣的控制。
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引用次数: 0
Eigenvector-based analysis of cluster synchronization in general complex networks of coupled chaotic oscillators 基于特征向量的耦合混沌振子复杂网络簇同步分析
IF 7.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-07-26 DOI: 10.1007/s11467-023-1324-0
Huawei Fan, Ya Wang, Xingang Wang

Whereas topological symmetries have been recognized as crucially important to the exploration of synchronization patterns in complex networks of coupled dynamical oscillators, the identification of the symmetries in large-size complex networks remains as a challenge. Additionally, even though the topological symmetries of a complex network are known, it is still not clear how the system dynamics is transited among different synchronization patterns with respect to the coupling strength of the oscillators. We propose here the framework of eigenvector-based analysis to identify the synchronization patterns in the general complex networks and, incorporating the conventional method of eigenvalue-based analysis, investigate the emergence and transition of the cluster synchronization states. We are able to argue and demonstrate that, without a prior knowledge of the network symmetries, the method is able to predict not only all the cluster synchronization states observable in the network, but also the critical couplings where the states become stable and the sequence of these states in the process of synchronization transition. The efficacy and generality of the proposed method are verified by different network models of coupled chaotic oscillators, including artificial networks of perfect symmetries and empirical networks of non-perfect symmetries. The new framework paves a way to the investigation of synchronization patterns in large-size, general complex networks.

尽管拓扑对称性已经被认为对耦合动态振荡器复杂网络中同步模式的探索至关重要,但在大型复杂网络中识别对称性仍然是一个挑战。此外,尽管已知复杂网络的拓扑对称性,但仍不清楚系统动力学如何在不同的同步模式之间与振荡器的耦合强度有关。本文提出了基于特征向量的分析框架来识别一般复杂网络中的同步模式,并结合传统的基于特征值的分析方法来研究集群同步状态的产生和转变。我们能够论证并证明,在没有网络对称性先验知识的情况下,该方法不仅能够预测网络中所有可观察到的集群同步状态,而且能够预测状态变得稳定的临界耦合以及这些状态在同步过渡过程中的顺序。通过不同的耦合混沌振子网络模型,包括完全对称的人工网络和非完全对称的经验网络,验证了所提方法的有效性和通用性。新的框架为研究大规模、一般复杂网络中的同步模式铺平了道路。
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引用次数: 0
Experimental studies for nuclear chirality in China 中国核手性的实验研究
IF 7.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-07-25 DOI: 10.1007/s11467-023-1303-5
Shouyu Wang  (, ), Chen Liu  (, ), Bin Qi  (, ), Wenzheng Xu  (, ), Hui Zhang  (, )

In the last decade, chiral symmetry in atomic nuclei has attracted significant attention and become one of the hot topics in current nuclear physics frontiers. This paper provides a review of experimental studies for nuclear chirality in China. In particular, the experimental setups, chiral mass regions, lifetime measurements, and simultaneous breaking of chirality and other symmetries are discussed in detail. These studies found a new chiral mass region (A ≈ 80), extended the boundaries of the A ≈ 100 and 130 chiral mass regions, and tested the chiral geometry of 130Cs, 106Ag, 80Br and 76Br by lifetime measurements. In addition, simultaneous breaking of chirality and other symmetries have been studied in 74As, 76Br, 78Br, 80Br, 81Kr and 131Ba.

近十年来,原子核的手性对称性引起了人们的极大关注,成为当前核物理前沿研究的热点之一。本文综述了国内核手性的实验研究进展。详细讨论了实验装置、手性质量区域、寿命测量以及手性和其他对称性的同时断裂。这些研究发现了一个新的手性质量区(a≈80),扩展了a≈100和130手性质量区的边界,并通过寿命测量测试了130Cs、106Ag、80Br和76Br的手性几何形状。此外,还研究了74As、76Br、78Br、80Br、81Kr和131Ba中手性和其他对称性的同时断裂。
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引用次数: 0
Recent review of surface plasmons and plasmonic hot electron effects in metallic nanostructures 金属纳米结构中表面等离子体和等离子体热电子效应的研究进展
IF 7.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-07-19 DOI: 10.1007/s11467-023-1328-9
Hao Zhang, Mohsin Ijaz, Richard J. Blaikie

Plasmonic resonators are widely used for the manipulation of light on subwavelength scales through the near-field electromagnetic wave produced by the collective oscillation of free electrons within metallic systems, well known as the surface plasmon (SP). The non-radiative decay of the surface plasmon can excite a plasmonic hot electron. This review article systematically describes the excitation progress and basic properities of SPs and plasmonic hot electrons according to recent publications. The extraction mechanism of plasmonic hot electrons via Schottky conjunction to an adjacent semiconductor is also illustrated. Also, a calculation model of hot electron density is given, where the efficiency of hot-electron excitation, transport and extraction is discussed. We believe that plasmonic hot electrons have a huge potential in the future development of optoelectronic systems and devices.

等离子体谐振器被广泛用于操纵亚波长尺度上的光,通过近场电磁波由金属系统内自由电子的集体振荡产生,众所周知的表面等离子体(SP)。表面等离子体的非辐射衰变可以激发出等离子体热电子。本文系统地介绍了等离子体热电子和等离子体热电子的激发过程和基本性质。并说明了等离子体热电子通过肖特基连接到相邻半导体的提取机制。给出了热电子密度的计算模型,讨论了热电子的激发、输运和萃取效率。我们认为,等离子体热电子在光电系统和器件的未来发展中具有巨大的潜力。
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引用次数: 1
Dynamical-corrected nonadiabatic geometric quantum computation 动态校正非绝热几何量子计算
IF 7.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2023-07-14 DOI: 10.1007/s11467-023-1322-2
Cheng-Yun Ding, Li Chen, Li-Hua Zhang, Zheng-Yuan Xue

Recently, nonadiabatic geometric quantum computation has been received great attentions, due to its fast operation and intrinsic error resilience. However, compared with the corresponding dynamical gates, the robustness of implemented nonadiabatic geometric gates based on the conventional single-loop geometric scheme still has the same order of magnitude due to the requirement of strict multi-segment geometric controls, and the inherent geometric fault-tolerance characteristic is not fully explored. Here, we present an effective geometric scheme combined with a general dynamical-corrected technique, with which the super-robust nonadiabatic geometric quantum gates can be constructed over the conventional single-loop geometric and two-loop composite-pulse geometric strategies, in terms of resisting the systematic error, i.e., σx error. In addition, combined with the decoherence-free subspace (DFS) coding, the resulting geometric gates can also effectively suppress the σz error caused by the collective dephasing. Notably, our protocol is a general one with simple experimental setups, which can be potentially implemented in different quantum systems, such as Rydberg atoms, trapped ions and superconducting qubits. These results indicate that our scheme represents a promising way to explore large-scale fault-tolerant quantum computation.

近年来,非绝热几何量子计算以其快速的运算速度和固有的抗误差能力受到了广泛的关注。然而,与相应的动态门相比,基于传统单回路几何方案实现的非绝热几何门由于需要严格的多段几何控制,鲁棒性仍处于同一数量级,并且没有充分挖掘其固有的几何容错特性。在此,我们提出了一种有效的几何方案,结合一般的动态校正技术,在传统的单回路几何和双回路复合脉冲几何策略的基础上,构建了超鲁棒非绝热几何量子门,以抵抗系统误差,即σx误差。此外,结合无退相干子空间(DFS)编码,所得到的几何栅极还能有效地抑制由集体退相引起的σz误差。值得注意的是,我们的协议是一个具有简单实验设置的通用协议,可以潜在地在不同的量子系统中实现,例如里德伯原子,捕获离子和超导量子比特。这些结果表明,我们的方案是探索大规模容错量子计算的一种有前途的方法。
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引用次数: 0
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