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Giant anomalous transverse transport properties of Co-doped two-dimensional Fe3GaTe2 掺杂 Co 的二维 Fe3GaTe2 的巨型反常横向输运特性
IF 6.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-07-12 DOI: 10.1007/s11467-024-1424-5
Imran Khan, Jisang Hong

In spintronics, transverse anomalous transport properties have emerged as a highly promising avenue surpassing the conventional longitudinal transport behaviors. Here, we explore the transverse transport properties of monolayer and bilayer Fe3−xCoxGaTe2 (x = 0.083, 0.167, 0.250, and 0.330) systems. All the systems exhibit ferromagnetic ground states with metallic features and also have perpendicular magnetic anisotropy. Besides, the magnetic anisotropy is substantially enhanced with increasing Co-doping concentration. However, unlike magnetic anisotropy, the Curie temperature is suppressed by increasing the Co-doping concentration. For instance, the monolayer and bilayer Fe2.917Co0.083GaTe2 hold a Curie temperature of 253 K and 269 K, which decreases to 163 K and 173 K in monolayer and bilayer Fe2.67Co0.33GaTe2 systems, respectively. We find a giant anomalous Nernst conductivity (ANC) of 6.03 A/(K·m) in the monolayer Fe2.917Co0.083GaTe2 at −30 meV, and this is further enhanced to 11.30 A/(K·m) in the bilayer Fe2.917Co0.083GaTe2 at −20 meV. Moreover, the bilayer Fe2.917Co0.083GaTe2 structure has a large anomalous thermal Hall conductivity (ATHC) of −0.14 W/(K·m) at 100 K. Overall, we find that the Fe3−xCoxGaTe2 (x = 0.083, 0.167, 0.250, and 0.330) structures have better anomalous transverse transport performance than the pristine Fe3GaTe2 system and can be used for potential spintronics and spin caloritronics applications.

在自旋电子学中,横向反常输运特性已成为超越传统纵向输运行为的极有前途的途径。在这里,我们探讨了单层和双层 Fe3-xCoxGaTe2 (x = 0.083、0.167、0.250 和 0.330)系统的横向传输特性。所有系统都呈现出具有金属特征的铁磁基态,并且具有垂直磁各向异性。此外,随着钴掺杂浓度的增加,磁各向异性也大大增强。然而,与磁各向异性不同的是,居里温度会随着 Co 掺杂浓度的增加而受到抑制。例如,单层和双层 Fe2.917Co0.083GaTe2 的居里温度分别为 253 K 和 269 K,而单层和双层 Fe2.67Co0.33GaTe2 系统的居里温度则分别降至 163 K 和 173 K。我们发现单层 Fe2.917Co0.083GaTe2 在零下 30 meV 时的巨大异常 Nernst 电导率 (ANC) 为 6.03 A/(K-m),而双层 Fe2.917Co0.083GaTe2 在零下 20 meV 时的异常 Nernst 电导率 (ANC) 进一步提高到 11.30 A/(K-m)。总之,我们发现 Fe3-xCoxGaTe2(x = 0.083、0.167、0.250 和 0.330)结构比原始 Fe3GaTe2 系统具有更好的反常横向传输性能,可用于潜在的自旋电子学和自旋热电子学应用。
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引用次数: 0
Machine learning in laser-induced breakdown spectroscopy: A review 激光诱导击穿光谱学中的机器学习:综述
IF 6.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-07-12 DOI: 10.1007/s11467-024-1427-2
Zhongqi Hao, Ke Liu, Qianlin Lian, Weiran Song, Zongyu Hou, Rui Zhang, Qianqian Wang, Chen Sun, Xiangyou Li, Zhe Wang

Laser-induced breakdown spectroscopy (LIBS) is a spectroscopic analytic technique with great application potential because of its unique advantages for online/in-situ detection. However, due to the spatially inhomogeneity and drastically temporal varying nature of its emission source, the laser-induced plasma, it is difficult to find or hard to generate an appropriate spatiotemporal window for high repeatable signal collection with lower matrix effects. The quantification results of traditional physical principle based calibration model are unsatisfactory since these models were not able to compensate for complicate matrix effects as well as signal fluctuation. Machine learning is an emerging approach, which can intelligently correlated the complex LIBS spectral data with its qualitative or/and quantitative composition by establishing multivariate regression models with greater potential to reduce the impacts of signal fluctuation and matrix effects, therefore achieving relatively better qualitative and quantitative performance. In this review, the progress of machine learning application in LIBS is summarized from two main aspects: i) Pre-processing data for machine learning model, including spectral selection, variable reconstruction, and denoising to improve qualitative/quantitative performance; ii) Machine learning methods for better quantification performance with reduction of the impact of matrix effect as well as LIBS spectra fluctuations. The review also points out the issues that researchers need to address in their future research on improving the performance of LIBS analysis using machine learning algorithms, such as restrictions on training data, the disconnect between physical principles and algorithms, the low generalization ability and massive data processing ability of the model.

激光诱导击穿光谱(LIBS)是一种光谱分析技术,因其在线/原位检测的独特优势而具有巨大的应用潜力。然而,由于其发射源--激光诱导等离子体--在空间上的不均匀性和时间上的急剧变化性,很难找到或很难生成一个合适的时空窗口来采集具有较低矩阵效应的高重复性信号。基于物理原理的传统校准模型的量化结果并不令人满意,因为这些模型无法弥补复杂的矩阵效应和信号波动。机器学习是一种新兴的方法,它可以通过建立多元回归模型,智能地将复杂的 LIBS 光谱数据与其定性或/和定量组成相关联,从而获得相对更好的定性和定量性能。本综述从两个主要方面总结了机器学习在 LIBS 中的应用进展:i) 机器学习模型的数据预处理,包括光谱选择、变量重构和去噪,以提高定性/定量性能;ii) 机器学习方法可降低矩阵效应和 LIBS 光谱波动的影响,从而获得更好的定量性能。综述还指出了研究人员在利用机器学习算法提高 LIBS 分析性能的未来研究中需要解决的问题,如对训练数据的限制、物理原理与算法之间的脱节、模型的低泛化能力和海量数据处理能力等。
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引用次数: 0
Emerging single-photon detection technique for high-performance photodetector 用于高性能光电探测器的新兴单光子探测技术
IF 6.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-07-12 DOI: 10.1007/s11467-024-1428-1
Jinxiu Liu, Zhenghan Peng, Chao Tan, Lei Yang, Ruodan Xu, Zegao Wang

Single-photon detections (SPDs) represent a highly sensitive light detection technique capable of detecting individual photons at extremely low light intensity levels. This technology mainly relies on the mainstream SPDs, such as photomultiplier tubes (PMTs), avalanche photodiodes (SAPD), superconducting nanowire single-photon detectors (SNSPDs), superconducting transition-edge sensor (TES), and hybrid lead halide perovskite. However, the complexity and high manufacturing cost, coupled with the requirement of special conditions like a low-temperature environment, pose significant challenges to the wide adoption of SPDs. To address the challenges faced by SPDs, significant efforts have been devoted to enhancing their performance. In this review, we first summarize the principles and technical challenges of several SPDs. Conductors, superconductors, semiconductors, 3D bulk materials, 2D film materials, 1D nanowires, and 0D quantum dots have all been discussed for single-photon detectors. Methods such as special optical structure, waveguide integration, and strain engineering have been employed to elevate the performance of single-photon detectors. These techniques enhance light absorption and modulate the band structure of the material, thereby improving the single-photon sensitivity. By providing an overview of the current situation and future challenges of SPDs, this review aims to propose potential solutions for photon detection technology.

单光子探测器(SPD)是一种高灵敏度的光探测技术,能够在极低的光强水平下探测单个光子。该技术主要依靠主流单光子探测器,如光电倍增管(PMT)、雪崩光电二极管(SAPD)、超导纳米线单光子探测器(SNSPD)、超导过渡边传感器(TES)和混合卤化铅过氧化物。然而,SPD 的复杂性和高制造成本,以及对低温环境等特殊条件的要求,给其广泛应用带来了巨大挑战。为了应对 SPD 所面临的挑战,人们一直致力于提高其性能。在本综述中,我们首先总结了几种 SPD 的原理和技术挑战。导体、超导体、半导体、三维块体材料、二维薄膜材料、一维纳米线和零维量子点都曾被讨论用于单光子探测器。为了提高单光子探测器的性能,人们采用了特殊光学结构、波导集成和应变工程等方法。这些技术增强了材料的光吸收并调节了材料的带状结构,从而提高了单光子灵敏度。本综述概述了单光子探测器的现状和未来挑战,旨在为光子探测技术提出潜在的解决方案。
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引用次数: 0
Visualization for physics analysis improvement and applications in BESIII 改进物理分析的可视化和在 BESIII 中的应用
IF 6.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-07-04 DOI: 10.1007/s11467-024-1422-7
Zhi-Jun Li  (, ), Ming-Kuan Yuan  (, ), Yun-Xuan Song  (, ), Yan-Gu Li  (, ), Jing-Shu Li  (, ), Sheng-Sen Sun  (, ), Xiao-Long Wang  (, ), Zheng-Yun You  (, ), Ya-Jun Mao  (, )

Modern particle physics experiments usually rely on highly complex and large-scale spectrometer devices. In high energy physics experiments, visualization helps detector design, data quality monitoring, offline data processing, and has great potential for improving physics analysis. In addition to the traditional physics data analysis based on statistical methods, visualization provides unique intuitive advantages in searching for rare signal events and reducing background noises. By applying the event display tool to several physics analyses in the BESIII experiment, we demonstrate that visualization can benefit potential physics discovery and improve the signal significance. With the development of modern visualization techniques, it is expected to play a more important role in future data processing and physics analysis of particle physics experiments.

现代粒子物理实验通常依赖于高度复杂的大型光谱仪设备。在高能物理实验中,可视化有助于探测器设计、数据质量监控和离线数据处理,在改进物理分析方面具有巨大潜力。除了基于统计方法的传统物理数据分析外,可视化在搜索罕见信号事件和减少背景噪音方面具有独特的直观优势。通过将事件显示工具应用于 BESIII 实验中的多项物理分析,我们证明了可视化可以为潜在的物理发现带来益处,并提高信号的显著性。随着现代可视化技术的发展,它有望在未来粒子物理实验的数据处理和物理分析中发挥更重要的作用。
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引用次数: 0
Self-aligned TiOx-based 3D vertical memristor for a high-density synaptic array 用于高密度突触阵列的基于氧化钛的自对准三维垂直忆阻器
IF 6.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-07-03 DOI: 10.1007/s11467-024-1419-2
Subaek Lee, Juri Kim, Sungjun Kim

The emerging nonvolatile memory, three-dimensional vertical resistive random-access memory (VRRAM), inspired by the vertical NAND structure, has been proposed to replace NAND flash memory which has reached its integration limit. To improve the vertical ionic diffusion occurring in the conventional VRRAM structure, we propose a Pt/HfO2/TiO2/Ti self-aligned VRRAM with physically confined switching cells through sidewall thermal oxidation. We achieved stable bipolar switching, endurance (>104 cycles), and retention (>104 s) responses, and improved the interlayer leakage current issue through a distinctive self-aligned structure. Additionally, we elucidated the switching mechanism by analyzing current levels concerning ambient temperature. To utilize VRRAM for neuromorphic computing, the biological synaptic functions are emulated by applying pulse stimulation to the synaptic cell. The weight modulation of biological synapses is demonstrated based on potentiation, depression, spike-rate-dependent plasticity, and spike-timing-dependent plasticity. Additionally, we improve the pattern recognition rate by creating a linear conductance modulation with an incremental pulse train in pattern recognition simulations. The stable electrical characteristics and implementation of various synaptic functions demonstrate that self-aligned VRRAM is suitable for neuromorphic systems as a high-density synaptic device.

受垂直 NAND 结构的启发,新兴的非易失性存储器--三维垂直电阻式随机存取存储器(VRRAM)被提出来取代已达到集成极限的 NAND 闪存。为了改善传统 VRRAM 结构中发生的垂直离子扩散,我们提出了一种 Pt/HfO2/TiO2/Ti 自对准 VRRAM,通过侧壁热氧化实现了开关单元的物理限制。我们实现了稳定的双极开关、耐久性(104 次)和保持(104 秒)响应,并通过独特的自对准结构改善了层间漏电流问题。此外,我们还通过分析环境温度下的电流水平,阐明了开关机制。为了将 VRRAM 用于神经形态计算,我们通过对突触细胞施加脉冲刺激来模拟生物突触功能。基于电位、抑制、尖峰速率依赖性可塑性和尖峰定时依赖性可塑性,演示了生物突触的权重调制。此外,我们还通过在模式识别模拟中使用增量脉冲序列创建线性电导调制来提高模式识别率。稳定的电气特性和各种突触功能的实现表明,自对准 VRRAM 适合作为神经形态系统的高密度突触设备。
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引用次数: 0
Localized surface plasmon resonance enhanced photodetector: Physical model, enhanced mechanism and applications 局部表面等离子体共振增强型光电探测器:物理模型、增强机制和应用
IF 6.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-07-03 DOI: 10.1007/s11467-024-1413-8
Jiangtong Su, Xiaoqi Hou, Ning Dai, Yang Li

Localized surface plasmon resonance (LSPR) is an intriguing phenomenon that can break diffraction limitations and exhibit excellent light-confinement abilities, making it an attractive strategy for enhancing the light absorption capabilities of photodetectors. However, the complex mechanism behind this enhancement is still plaguing researchers, especially for hot-electron injection process, which inhibits further optimization and development. A clear guideline for basic physical model, enhancement mechanism, material selection and architectural design for LSPR photodetector are still required. This review firstly describes the mainstream understanding of fundamental physical modes of LSPR and related enhancement mechanism for LSPR photodetectors. Then, the universal strategies for tuning the LSPR frequency are introduced. Besides, the state-of-the-art progress in the development of LSPR photodetectors is briefly summarized. Finally, we highlight the remaining challenges and issues needed to be resolved in the future research.

局部表面等离子体共振(LSPR)是一种引人入胜的现象,它可以打破衍射限制,表现出卓越的光聚合能力,是增强光电探测器光吸收能力的一种极具吸引力的策略。然而,这种增强功能背后的复杂机制仍然困扰着研究人员,尤其是热电子注入过程,这阻碍了进一步的优化和开发。LSPR 光电探测器的基本物理模型、增强机制、材料选择和结构设计仍需要一个明确的指导原则。本综述首先介绍了对 LSPR 基本物理模式和 LSPR 光电探测器相关增强机制的主流认识。然后,介绍了调谐 LSPR 频率的通用策略。此外,还简要总结了 LSPR 光电探测器开发的最新进展。最后,我们强调了未来研究中仍需解决的挑战和问题。
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引用次数: 0
Generation and characterization of customized Laguerre–Gaussian beams with arbitrary profiles 具有任意剖面的定制拉盖尔-高斯光束的生成和特性分析
IF 6.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-07-01 DOI: 10.1007/s11467-024-1426-3
Chengyuan Wang, Yun Chen, Jinwen Wang, Xin Yang, Hong Gao, Fuli Li

We experimentally demonstrate the generation of customized Laguerre–Gaussian (LG) beams whose intensity maxima are localized around any desired curves. The principle is to act with appropriate algebraic functions on the angular spectra of LG beams. We characterize the propagation properties of these beams and compare them with non-diffraction caustic beams possessing the same intensity profiles. The results manifest that the customized-LG beams can maintain their profiles during propagation and suffer less energy loss than the non-diffraction caustic beams, and hence are able to propagate a longer distance. Moreover, the customized-LG beam exhibits self-healing ability when parts of their bodies are blocked. This new structure beam has potential applications in areas such as optical communication, soliton routing and steering, and optical tweezing.

我们通过实验演示了定制拉盖尔-高斯(LG)光束的生成,这些光束的强度最大值被定位在任何所需的曲线周围。其原理是用适当的代数函数作用于 LG 光束的角频谱。我们描述了这些光束的传播特性,并将它们与具有相同强度剖面的非衍射苛性光束进行了比较。结果表明,与非衍射苛性光束相比,定制 LG 光束在传播过程中能保持其轮廓,能量损失较小,因此能传播更长的距离。此外,定制 LG 光束在其部分主体受阻时还能表现出自我修复能力。这种新结构光束在光通信、孤子路由和转向以及光镊等领域具有潜在的应用前景。
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引用次数: 0
Van der Waals epitaxy of type-II band alignment CsPbI3/TMDC heterostructure for optoelectronic applications 用于光电应用的范德华外延 II 型带排列 CsPbI3/TMDC 异质结构
IF 6.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-06-24 DOI: 10.1007/s11467-024-1404-9
Chang Lu, Shunhui Zhang, Meili Chen, Haitao Chen, Mengjian Zhu, Zhengwei Zhang, Jun He, Lin Zhang, Xiaoming Yuan

Van der Waals epitaxy allows heterostructure formation without considering the lattice match requirement, thus is a promising method to form 2D/2D and 2D/3D heterojunction. Considering the unique optical properties of CsPbI3 and transition metal dichalcogenides (TMDCs), their heterostructure presents potential applications in both photonics and optoelectronics fields. Here, we demonstrate selective growth of cubic phase CsPbI3 nanofilm with thickness as thin as 4.0 nm and zigzag/armchair oriented nanowires (NWs) on monolayer WSe2. Furthermore, we show growth of CsPbI3 on both transferred WSe2 on copper grid and WSe2–based optoelectrical devices, providing a platform for structure analysis and device performance modification. Transmission electron microscopy (TEM) results reveal the epitaxial nature of cubic CsPbI3 phase. The revealed growth fundamental of CsPbI3 is universal valid for other two-dimensional substrates, offering a great advantage to fabricate CsPbI3 based van der Waals heterostructures (vdWHs). X-ray photoelectron spectroscopy (XPS) and optical characterization confirm the type-II band alignment, resulting in a fast charge transfer process and the occurrence of a broad emission peak at lower energy. The formation of WSe2/CsPbI3 heterostructure largely enhances the photocurrent from 2.38 nA to 38.59 nA. These findings are vital for bottom-up epitaxy of inorganic semiconductor on atomic thin 2D substrates for optoelectronic applications.

范德华外延可以在不考虑晶格匹配要求的情况下形成异质结构,因此是形成二维/二维和二维/三维异质结的一种很有前途的方法。考虑到 CsPbI3 和过渡金属二卤化物(TMDCs)独特的光学特性,它们的异质结构在光子学和光电子学领域都具有潜在的应用前景。在这里,我们展示了在单层 WSe2 上选择性生长厚度为 4.0 nm 的立方相 CsPbI3 纳米薄膜和人字形/臂向纳米线 (NW)。此外,我们还展示了 CsPbI3 在铜栅转印 WSe2 和基于 WSe2 的光电器件上的生长情况,为结构分析和器件性能改进提供了一个平台。透射电子显微镜(TEM)结果显示了立方 CsPbI3 相的外延性质。所揭示的 CsPbI3 生长基本原理对其他二维衬底也普遍适用,这为制造基于 CsPbI3 的范德华异质结构(vdWHs)提供了巨大优势。X 射线光电子能谱(XPS)和光学表征证实了 II 型带排列,从而产生了快速的电荷转移过程和较低能量的宽发射峰。WSe2/CsPbI3 异质结构的形成在很大程度上将光电流从 2.38 nA 提高到 38.59 nA。这些发现对于在原子薄二维衬底上自下而上地外延无机半导体以实现光电应用至关重要。
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引用次数: 0
Unidirectional propagation of water waves near ancient Luoyang Bridge 洛阳古桥附近水波的单向传播
IF 6.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-06-20 DOI: 10.1007/s11467-024-1411-x
Linkang Han, Qilin Duan, Junliang Duan, Shan Zhu, Shiming Chen, Yuhang Yin, Huanyang Chen

Metasurfaces and metagratings offer new platforms for electromagnetic wave control with significant responses. However, metasurfaces based on abrupt phase change and resonant structures suffer from the drawback of high loss and face challenges when applied in water waves. Therefore, the application of metasurfaces in water wave control is not ideal due to the limitations associated with high loss and other challenges. We have discovered that non-resonant metagratings exhibit promising effects in water wave control. Leveraging the similarity between bridges and metagratings, we have successfully developed a water wave metagrating model inspired by the ancient Luoyang Bridge in China. We conduct theoretical calculations and simulations on the metagrating and derive the equivalent anisotropic model of the metagrating. This model provides evidence that the metagrating has the capability to control water waves and achieve unidirectional surface water wave. The accuracy of our theory is strongly supported by the clear observation of the unidirectional propagation phenomenon during simulation and experiments conducted using a reduced version of the metagrating. It is the first time that the unidirectional propagation of water waves has been seen in water wave metagrating experiment. Above all, we realize the water wave metagrating experiment for the first time. By combining complex gratings with real bridges, we explore the physics embedded in the ancient building — Luoyang Bridge, which are of great significance for the water wave metagrating design and provide a new method for analyzing the effects of water waves on bridges. At the same time, this discovery also provides a new idea for ocean cargo transportation, ocean garbage cleaning, and the development and protection of ancient bridges.

元表面和元格拉特为电磁波控制提供了新的平台,可产生显著的响应。然而,基于突变相位和谐振结构的元表面具有高损耗的缺点,在水波中应用时面临挑战。因此,由于高损耗和其他挑战带来的限制,元表面在水波控制中的应用并不理想。我们发现,非共振元表面在水波控制中表现出良好的效果。我们利用桥梁和元障壁之间的相似性,成功开发了一种水波元障壁模型,其灵感来自于中国古代的洛阳桥。我们对元气淋膜进行了理论计算和模拟,并推导出元气淋膜的等效各向异性模型。该模型证明了元栅具有控制水波和实现单向表面水波的能力。在模拟和使用简化版元气发生器进行的实验中,单向传播现象被清晰观测到,这有力地证明了我们理论的准确性。水波的单向传播现象首次出现在水波元晶实验中。最重要的是,我们首次实现了水波元光栅实验。通过将复杂光栅与真实桥梁相结合,我们探索了古建筑--洛阳桥中蕴含的物理规律,这对水波元侵设计具有重要意义,并为分析水波对桥梁的影响提供了一种新方法。同时,这一发现也为海洋货物运输、海洋垃圾清理、古桥开发与保护提供了新思路。
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引用次数: 0
Vortex excites unidirectional water waves near ancient Luoyang Bridge 洛阳古桥附近的涡流激发单向水波
IF 6.5 2区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Pub Date : 2024-06-20 DOI: 10.1007/s11467-024-1421-8
Yichen Li, Xinhua Hu
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引用次数: 0
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