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Tunable near-infrared light emission from layered TiS3 nanoribbons 层状 TiS3 纳米带的可调谐近红外光发射
IF 7.5 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-02-12 DOI: 10.1007/s11467-023-1376-1
Junrong Zhang, Cheng Chen, Yanming Wang, Yang Lu, Honghong Li, Xingang Hou, Yaning Liang, Long Fang, Du Xiang, Kai Zhang, Junyong Wang

The low-dimensional light source shows promise in photonic integrated circuits. Stable layered van der Waals material that exhibits luminescence in the near-infrared optical communication waveband is an essential component in on-chip light sources. Herein, the tunable near-infrared photoluminescence (PL) of the air-stable layered titanium trisulfide (TiS3) is reported. Compared with iodine particles as a transport agent, TiS3 grown by chemical vapor transport using sulfur powder as a transport agent has fewer sulfur vacancies, which increases the luminescence intensity by an order of magnitude. The PL emission wavelength can be regulated in the near-infrared regime by thickness control. In addition, we observed an interesting anisotropic strain response of PL in layered TiS3 nanoribbon: a blue shift of PL was achieved when the uniaxial tensile strain was applied along the b-axis, while a negligible shift was observed when the strain was applied along the a-axis. Our work reveals the tunable near-infrared luminescent properties of TiS3 nanoribbons, suggesting their potential applications as near-infrared light sources in photonic integrated circuits.

低维光源在光子集成电路中大有可为。能在近红外光通信波段发光的稳定层状范德华材料是片上光源的重要组成部分。本文报告了空气稳定的层状三硫化钛(TiS3)的可调近红外光致发光(PL)。与作为传输剂的碘粒子相比,以硫磺粉为传输剂通过化学气相传输生长的 TiS3 具有更少的硫空位,从而将发光强度提高了一个数量级。通过厚度控制,可在近红外范围内调节 PL 发射波长。此外,我们还在层状 TiS3 纳米带中观察到了有趣的各向异性应变响应:当沿 b 轴施加单轴拉伸应变时,PL 会发生蓝移;而沿 a 轴施加应变时,PL 的蓝移可以忽略不计。我们的研究揭示了 TiS3 纳米带的可调近红外发光特性,这表明它们有望在光子集成电路中用作近红外光源。
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引用次数: 0
Research on the knee region of cosmic ray by using a novel type of electron–neutron detector array 利用新型电子-中子探测器阵列研究宇宙射线的膝区
IF 7.5 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-02-08 DOI: 10.1007/s11467-023-1383-2
Bing-Bing Li, Xin-Hua Ma, Shu-Wang Cui, Hao-Kun Chen, Tian-Lu Chen, Danzengluobu, Wei Gao, Hai-Bing Hu, Denis Kuleshov, Kirill Kurinov, Hu Liu, Mao-Yuan Liu, Ye Liu, Da-Yu Peng, Yao-Hui Qi, Oleg Shchegolev, Yuri Stenkin, Li-Qiao Yin, Heng-Yu Zhang, Liang-Wei Zhang

By accurately measuring composition and energy spectrum of cosmic ray, the origin problem of so called “knee” region (energy >one PeV) can be solved. However, up to the present, the results of the spectrum in the knee region obtained by several previous experiments have shown obvious differences, so they cannot give effective evidence for judging the theoretical models on the origin of the knee. Recently, the Large High Altitude Air Shower Observatory (LHAASO) has reported several major breakthroughs and important results in astro-particle physics field. Relying on its advantages of wide-sky survey, high altitude location and large area detector arrays, the research content of LHAASO experiment mainly includes ultra high-energy gamma-ray astronomy, measurement of cosmic ray spectra in the knee region, searching for dark matter and new phenomena of particle physics at higher energy. The electron and thermal neutron detector (EN-Detector) is a new scintillator detector which applies thermal neutron detection technology to measure cosmic ray extensive air shower (EAS). This technology is an extension of LHAASO. The EN-Detector Array (ENDA) can highly efficiently measure thermal neutrons generated by secondary hadrons so called “skeleton” of EAS. In this paper, we perform the optimization of ENDA configuration, and obtain expectations on the ENDA results, including thermal neutron distribution, trigger efficiency and capability of cosmic ray composition separation. The obtained real data results are consistent with those by the Monte Carlo simulation.

通过精确测量宇宙线的成分和能谱,可以解决所谓 "膝区"(能量为1PeV)的起源问题。然而,迄今为止,前几次实验所获得的 "膝区 "能谱结果存在明显差异,无法为判断 "膝区 "起源的理论模型提供有效证据。最近,大型高空气流淋浴天文台(LHAASO)在天体粒子物理领域取得了多项重大突破和重要成果。依托其宽巡天、高海拔和大面积探测器阵列的优势,LHAASO 实验的研究内容主要包括超高能伽马射线天文学、膝区宇宙线谱测量、暗物质搜索和高能粒子物理新现象等。电子和热中子探测器(EN-Detector)是一种新型闪烁体探测器,它采用热中子探测技术来测量宇宙射线大范围空气淋射(EAS)。这项技术是 LHAASO 的延伸。热中子探测器阵列(ENDA)可以高效地测量由二次强子产生的热中子,即 EAS 的 "骨架"。本文对ENDA的配置进行了优化,获得了ENDA的预期结果,包括热中子分布、触发效率和宇宙射线成分分离能力。获得的真实数据结果与蒙特卡洛模拟结果一致。
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引用次数: 0
Variational quantum algorithms for scanning the complex spectrum of non-Hermitian systems 扫描非ermitian 系统复杂频谱的变量量子算法
IF 7.5 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-02-07 DOI: 10.1007/s11467-023-1382-3
Xu-Dan Xie, Zheng-Yuan Xue, Dan-Bo Zhang

Solving non-Hermitian quantum many-body systems on a quantum computer by minimizing the variational energy is challenging as the energy can be complex. Here, we propose a variational quantum algorithm for solving the non-Hermitian Hamiltonian by minimizing a type of energy variance, where zero variance can naturally determine the eigenvalues and the associated left and right eigenstates. Moreover, the energy is set as a parameter in the cost function and can be tuned to scan the whole spectrum efficiently by using a two-step optimization scheme. Through numerical simulations, we demonstrate the algorithm for preparing the left and right eigenstates, verifying the biorthogonal relations, as well as evaluating the observables. We also investigate the impact of quantum noise on our algorithm and show that its performance can be largely improved using error mitigation techniques. Therefore, our work suggests an avenue for solving non-Hermitian quantum many-body systems with variational quantum algorithms on near-term noisy quantum computers.

在量子计算机上通过最小化变异能量求解非ermitian量子多体系统具有挑战性,因为能量可能很复杂。在这里,我们提出了一种变分量子算法,通过最小化一种能量方差来求解非ermitian Hamiltonian,其中零方差可以自然地确定特征值以及相关的左右特征状态。此外,能量被设定为成本函数中的一个参数,可以通过两步优化方案进行调整,从而高效地扫描整个频谱。通过数值模拟,我们演示了准备左、右特征状态、验证双谐调关系以及评估观测值的算法。我们还研究了量子噪声对算法的影响,并证明利用误差缓解技术可以在很大程度上提高算法的性能。因此,我们的工作为在近期噪声量子计算机上使用变分量子算法求解非赫米提量子多体系统提供了一条途径。
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引用次数: 0
Effect of ambient pressures on laser-induced breakdown spectroscopy signals 环境压力对激光诱导击穿光谱信号的影响
IF 7.5 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-02-07 DOI: 10.1007/s11467-023-1380-5
Kaifan Zhang, Weiran Song, Zongyu Hou, Zhe Wang

Laser-induced breakdown spectroscopy (LIBS) is regarded as the future superstar for analytical chemistry and widely applied in various fields. Improving the quality of LIBS signal is fundamental to achieving accurate quantification and large-scale commercialization of LIBS. To propose control methods that improve LIBS signal quality, it is essential to have a comprehensive understanding of the influence of key parameters, such as ambient gas pressure, temperature, and sample temperature on LIBS signals. To date, extensive research has been carried out. However, different researchers often yield significantly different experimental results for LIBS, preventing the formation of consistent conclusions. This greatly prevents the understanding of influencing laws of key parameters and the improvement of LIBS quantitative performance. Taking ambient gas pressure as an example, this paper compares the effects of ambient gas pressure under different optimization conditions, reveals the influence of spatiotemporal window caused by inherent characteristics of LIBS signal sources, i.e., intense temporal changes and spatial non-uniformity of laser-induced plasmas, on the impact patterns of key parameters. From the perspective of plasma spatiotemporal evolution, the paper elucidates the influence patterns of ambient gas pressure on LIBS signals, clarifying seemingly contradictory research results in the literature.

激光诱导击穿光谱(LIBS)被认为是未来分析化学的超级明星,广泛应用于各个领域。提高 LIBS 信号质量是实现精确定量和大规模商业化的基础。要提出提高 LIBS 信号质量的控制方法,必须全面了解环境气体压力、温度和样品温度等关键参数对 LIBS 信号的影响。迄今为止,已经开展了大量研究。然而,不同的研究人员对 LIBS 的实验结果往往大相径庭,无法形成一致的结论。这极大地阻碍了对关键参数影响规律的理解和 LIBS 定量性能的提高。本文以环境气体压力为例,比较了不同优化条件下环境气体压力的影响,揭示了LIBS信号源固有特性(即激光诱导等离子体的强烈时间变化和空间不均匀性)导致的时空窗口对关键参数影响规律的影响。论文从等离子体时空演变的角度,阐明了环境气体压力对 LIBS 信号的影响模式,澄清了文献中看似矛盾的研究成果。
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引用次数: 0
Generalized time-dependent generator coordinate method for induced fission dynamics 诱导裂变动力学的广义时变发电机坐标法
IF 7.5 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-02-01 DOI: 10.1007/s11467-023-1381-4
B. Li, D. Vretenar, T. Nikšić, J. Zhao, P. W. Zhao, J. Meng

The generalized time-dependent generator coordinate method (TD-GCM) is extended to include pairing correlations. The correlated GCM nuclear wave function is expressed in terms of time-dependent generator states and weight functions. The particle–hole channel of the effective interaction is determined by a Hamiltonian derived from an energy density functional, while pairing is treated dynamically in the standard BCS approximation with time-dependent pairing tensor and single-particle occupation probabilities. With the inclusion of pairing correlations, various time-dependent phenomena in open-shell nuclei can be described more realistically. The model is applied to the description of saddle-to-scission dynamics of induced fission. The generalized TD-GCM charge yields and total kinetic energy distribution for the fission of 240Pu, are compared to those obtained using the standard time-dependent density functional theory (TD-DFT) approach, and with available data.

广义随时间变化的发电机坐标法(TD-GCM)被扩展到包括配对相关性。相关 GCM 核波函数用随时间变化的发电机状态和权函数来表示。有效相互作用的粒子-空穴通道由能量密度函数导出的哈密顿确定,而配对则用标准 BCS 近似动态处理,并采用随时间变化的配对张量和单粒子占据概率。加入配对相关性后,开壳原子核中各种随时间变化的现象可以得到更真实的描述。该模型被应用于描述诱导裂变的鞍到裂变动力学。将 240Pu 裂变的广义 TD-GCM 电荷量和总动能分布与使用标准时变密度泛函理论(TD-DFT)方法获得的电荷量和总动能分布以及现有数据进行了比较。
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引用次数: 0
High performance photodetector based on few-layer MoTe2/CdS0.42Se0.58 flake heterojunction 基于少层 MoTe2/CdS0.42Se0.58 薄片异质结的高性能光电探测器
IF 7.5 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-27 DOI: 10.1007/s11467-023-1374-3
Ran Ma, Qiuhong Tan, Peizhi Yang, Yingkai Liu, Qianjin Wang

Two-dimensional (2D) transition metal dichalcogenides have been extensively studied due to their fascinating physical properties for constructing high-performance photodetectors. However, their relatively low responsivities, current on/off ratios and response speeds have hindered their widespread application. Herein, we fabricated a high-performance photodetector based on few-layer MoTe2 and CdS0.42Se0.58 flake heterojunctions. The photodetector exhibited a high responsivity of 7221 A/W, a large current on/off ratio of 1.73×104, a fast response speed of 90/120 µs, external quantum efficiency (EQE) reaching up to 1.52×106 % and detectivity (D*) reaching up to 1.67×1015 Jones. The excellent performance of the heterojunction photodetector was analyzed by a photocurrent mapping test and first-principle calculations. Notably, the visible light imaging function was successfully attained on the MoTe2/CdS0.42Se0.58 photodetectors, indicating that the device had practical imaging application prospects. Our findings provide a reference for the design of ultrahigh-performance MoTe2-based photodetectors.

二维(2D)过渡金属二钙化物因其迷人的物理特性而被广泛研究,用于构建高性能光电探测器。然而,它们相对较低的响应率、电流开/关比和响应速度阻碍了它们的广泛应用。在此,我们基于少层 MoTe2 和 CdS0.42Se0.58 薄片异质结制造了一种高性能光电探测器。该光电探测器具有 7221 A/W 的高响应率、1.73×104 的大电流开/关比、90/120 µs 的快速响应速度、1.52×106 % 的外部量子效率(EQE)和 1.67×1015 Jones 的检测率(D*)。通过光电流映射测试和第一原理计算,分析了异质结光电探测器的优异性能。值得注意的是,MoTe2/CdS0.42Se0.58 光探测器成功实现了可见光成像功能,表明该器件具有实际成像应用前景。我们的研究结果为设计基于 MoTe2 的超高性能光电探测器提供了参考。
{"title":"High performance photodetector based on few-layer MoTe2/CdS0.42Se0.58 flake heterojunction","authors":"Ran Ma, Qiuhong Tan, Peizhi Yang, Yingkai Liu, Qianjin Wang","doi":"10.1007/s11467-023-1374-3","DOIUrl":"https://doi.org/10.1007/s11467-023-1374-3","url":null,"abstract":"<p>Two-dimensional (2D) transition metal dichalcogenides have been extensively studied due to their fascinating physical properties for constructing high-performance photodetectors. However, their relatively low responsivities, current on/off ratios and response speeds have hindered their widespread application. Herein, we fabricated a high-performance photodetector based on few-layer MoTe<sub>2</sub> and CdS<sub>0.42</sub>Se<sub>0.58</sub> flake heterojunctions. The photodetector exhibited a high responsivity of 7221 A/W, a large current on/off ratio of 1.73×10<sup>4</sup>, a fast response speed of 90/120 µs, external quantum efficiency (EQE) reaching up to 1.52×10<sup>6</sup> % and detectivity (<i>D*</i>) reaching up to 1.67×10<sup>15</sup> Jones. The excellent performance of the heterojunction photodetector was analyzed by a photocurrent mapping test and first-principle calculations. Notably, the visible light imaging function was successfully attained on the MoTe<sub>2</sub>/CdS<sub>0.42</sub>Se<sub>0.58</sub> photodetectors, indicating that the device had practical imaging application prospects. Our findings provide a reference for the design of ultrahigh-performance MoTe<sub>2</sub>-based photodetectors.\u0000</p>","PeriodicalId":573,"journal":{"name":"Frontiers of Physics","volume":null,"pages":null},"PeriodicalIF":7.5,"publicationDate":"2024-01-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"139584409","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Solar manipulations of perpendicular magnetic anisotropy for flexible spintronics 太阳能操纵垂直磁各向异性以实现柔性自旋电子学
IF 7.5 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-24 DOI: 10.1007/s11467-023-1377-0
Zhexi He, Yifan Zhao, Yujing Du, Meng Zhao, Yuxuan Jiang, Ming Liu, Ziyao Zhou

Flexible electronics/spintronics attracts researchers’ attention for their application potential abroad in wearable devices, healthcare, and other areas. Those devices’ performance (speed, energy consumption) is highly dependent on manipulating information bits (spin-orientation in flexible spintronics). In this work, we established an organic photovoltaic (OPV)/ ZnO/Pt/Co/Pt heterostructure on flexible PET substrates with perpendicular magnetic anisotropy (PMA). Under sunlight illumination, the photo-electrons generated from the OPV layer transfer into the PMA heterostructure, then they reduce the PMA strength by enhancing the interfacial Rashba field accordingly. The coercive field (Hc) reduces from 800 Oe to 500 Oe at its maximum, and the magnetization can be switched up and down reversibly. The stability of sunlight control of magnetization reversal under various bending conditions is also tested for flexible spintronic applications. Lastly, the voltage output of sunlight-driven PMA is achieved in our prototype device, exhibiting an excellent angular dependence and opening a door towards solar-driven flexible spintronics with much lower energy consumption.

柔性电子学/自旋电子学因其在国外可穿戴设备、医疗保健和其他领域的应用潜力而备受研究人员关注。这些设备的性能(速度、能耗)在很大程度上取决于信息比特的操作(柔性自旋电子学中的自旋方向)。在这项工作中,我们在具有垂直磁各向异性(PMA)的柔性 PET 基底上建立了有机光伏(OPV)/ ZnO/Pt/Co/Pt 异质结构。在阳光照射下,OPV 层产生的光电子转移到 PMA 异质结构中,然后通过增强界面拉什巴场相应地降低 PMA 强度。矫顽力场(Hc)从 800 Oe 降低到最大值 500 Oe,磁化率可以上下可逆切换。此外,还测试了在各种弯曲条件下阳光控制磁化反转的稳定性,以实现灵活的自旋电子应用。最后,我们的原型装置实现了阳光驱动 PMA 的电压输出,表现出极佳的角度依赖性,为实现能耗更低的太阳能驱动柔性自旋电子学打开了一扇大门。
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引用次数: 0
Self organizing optimization and phase transition in reinforcement learning minority game system 强化学习少数民族游戏系统中的自组织优化和阶段转换
IF 7.5 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-24 DOI: 10.1007/s11467-023-1378-z
Si-Ping Zhang, Jia-Qi Dong, Hui-Yu Zhang, Yi-Xuan Lü, Jue Wang, Zi-Gang Huang

Whether the complex game system composed of a large number of artificial intelligence (AI) agents empowered with reinforcement learning can produce extremely favorable collective behaviors just through the way of agent self-exploration is a matter of practical importance. In this paper, we address this question by combining the typical theoretical model of resource allocation system, the minority game model, with reinforcement learning. Each individual participating in the game is set to have a certain degree of intelligence based on reinforcement learning algorithm. In particular, we demonstrate that as AI agents gradually becomes familiar with the unknown environment and tries to provide optimal actions to maximize payoff, the whole system continues to approach the optimal state under certain parameter combinations, herding is effectively suppressed by an oscillating collective behavior which is a self-organizing pattern without any external interference. An interesting phenomenon is that a first-order phase transition is revealed based on some numerical results in our multi-agents system with reinforcement learning. In order to further understand the dynamic behavior of agent learning, we define and analyze the conversion path of belief mode, and find that the self-organizing condensation of belief modes appeared for the given trial and error rates in the AI system. Finally, we provide a detection method for period-two oscillation collective pattern emergence based on the Kullback–Leibler divergence and give the parameter position where the period-two appears.

由大量人工智能(AI)代理组成的复杂博弈系统在强化学习的加持下,能否仅通过代理自我探索的方式产生极为有利的集体行为,是一个具有重要现实意义的问题。本文通过将资源分配系统的典型理论模型--少数人博弈模型与强化学习相结合来解决这一问题。基于强化学习算法,每个参与博弈的个体都被设定为具有一定程度的智能。我们特别证明,当人工智能代理逐渐熟悉未知环境并试图提供最优行动以获得最大回报时,整个系统会在特定参数组合下不断接近最优状态,羊群行为会被一种振荡的集体行为有效抑制,而这种振荡的集体行为是一种不受任何外部干扰的自组织模式。一个有趣的现象是,基于强化学习的多代理系统的一些数值结果显示了一阶相变。为了进一步理解代理学习的动态行为,我们定义并分析了信念模式的转换路径,发现在给定的试错率下,人工智能系统出现了信念模式的自组织凝聚。最后,我们提供了一种基于库尔贝-莱布勒发散的周期-2振荡集体模式出现的检测方法,并给出了周期-2出现的参数位置。
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引用次数: 0
Unravelling-based (auto)control of back-action in atomic Bose–Einstein condensate 原子玻色-爱因斯坦凝聚态中基于解析的反作用(自动)控制
IF 7.5 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-24 DOI: 10.1007/s11467-023-1375-2
V. A. Tomilin, L. V. Il’ichov

We present a novel feedback control method for quantum systems. Feedback does not affect the controlled system itself. Instead, it controls the unravelling of the quantum channel of interaction between the system and its environment. This interaction can be represented as a history of events. If their informational content is changed, their back-action on the system is also modified. Feedback action is trigged by the events, thus granting the system the degree of control over its own state. The efficiency of the proposed scheme is demonstrated on the example of two-mode atomic Bose-Einstein condensate, with one of its modes subject to phase-contrast imaging in a Mach–Zehnder interferometer. The histories of photocounts in the output channels of the interferometer are used for feedback. Its capabilities of state engineering are studied for different settings of the feedback loop and different numbers of events in the recorded histories.

我们提出了一种新颖的量子系统反馈控制方法。反馈不会影响受控系统本身。相反,它控制着系统与其环境之间相互作用的量子通道的解开。这种相互作用可以表示为事件的历史。如果这些事件的信息内容发生变化,它们对系统的反作用也会随之改变。反馈行动由事件触发,从而赋予系统对自身状态的控制能力。我们以双模原子玻色-爱因斯坦凝聚态为例,证明了所提方案的效率,其中一种模式在马赫-泽恩德干涉仪中进行相位对比成像。干涉仪输出通道的光计数历史用于反馈。针对反馈回路的不同设置和记录历史中事件的不同数量,对其状态工程能力进行了研究。
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引用次数: 0
Intertype superconductivity evoked by the interplay of disorder and multiple bands 无序和多带相互作用引发的类型间超导电性
IF 7.5 2区 物理与天体物理 Q1 Physics and Astronomy Pub Date : 2024-01-24 DOI: 10.1007/s11467-023-1379-y
P. M. Marychev, A. A. Shanenko, A. V. Vagov

Nonmagnetic impurity scattering is known to shift up the Ginzburg–Landau parameter κ of a superconductor. In this case, when the system is initially in type I, it can change its magnetic response, crossing the intertype domain with κ ∼ 1 between the two standard superconductivity types and arriving at type II. In the present work we demonstrate that the impact of disorder can be much more profound in the presence of the multiband structure of the charge carrier states. In particular, when the band diffusivities differ from each other, the intertype domain tends to expand significantly, including points with κ ≫ 1 that belong to deep type-II in conventional single-band superconductors. Our finding sheds light on the nontrivial disorder effect and significantly complements earlier results on the enlargement of the intertype domain in clean multiband superconductors.

众所周知,非磁性杂质散射会使超导体的金兹堡-朗道参数κ上移。在这种情况下,当系统最初处于 I 型时,它可以改变磁响应,跨越介于两种标准超导类型之间的 κ ∼ 1 型域,到达 II 型。在本研究中,我们证明了当电荷载流子态存在多带结构时,无序的影响会更加深远。特别是,当带扩散性互不相同时,类型间域往往会显著扩大,包括κ ≫ 1 的点,而这些点在传统单带超导体中属于深 II 型。我们的发现揭示了非微不足道的无序效应,并极大地补充了早先关于清洁多带超导体中类型间域扩大的结果。
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引用次数: 0
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