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Cobalt Concentration-Dependent Structural and Magnetic Transitions in Nanocrystalline Ni0.9−xZn0.1CoxFe2O4 Ferrites 纳米晶Ni0.9−xZn0.1CoxFe2O4铁氧体中钴浓度相关的结构和磁跃迁
IF 1.4 3区 物理与天体物理 Q4 PHYSICS, APPLIED Pub Date : 2025-06-01 DOI: 10.1007/s10909-025-03299-y
K. K. Palsaniya,  Anchal,  Sarita, M. S. Rulaniya, Pooja Yadav, R. K. Beniwal, Namita Kumari, P. A. Alvi, B. L. Choudhary

Nanocrystalline Ni0.9−xZn0.1CoxFe2O4 (x = 0.2, 0.4, 0.6, 0.8) ferrites were synthesized via the sol–gel method, yielding a cubic single-phase spinel structure (Fd−3m), as confirmed through Rietveld refinement. The crystallite size was observed to increase from 7 to 10 nm with higher Co substitution. Magnetic characterization revealed a pronounced dependence on Co concentration, with zero-field-cooled and field-cooled magnetization curves exhibiting bifurcation indicative of magnetic relaxation phenomena. The Ni0.5Zn0.1Co0.4Fe2O4 composition exhibited a blocking temperature of 191 K, a Curie temperature of 207 K, and a transition from ferromagnetic ordering at 5 K to superparamagnetic behavior at 300 K. Similarly, Ni0.3Zn0.1Co0.6Fe2O4 demonstrated a transition at 251 K with retained ferromagnetic ordering at 5 K. In contrast, Ni0.1Zn0.1Co0.8Fe2O4 displayed magnetic irreversibility and a paramagnetic state at 300 K. Raman spectroscopy further corroborated the inverse spinel structure, revealing characteristic vibrational modes at ~ 460 cm⁻1 and 680 cm⁻1. These findings underscore the pivotal role of Co substitution in modulating the structural and magnetic properties of Ni0.9−xZn0.1CoxFe2O4 nanocrystals, particularly their temperature-dependent magnetic phase transitions. Collectively, the results highlight the influence of Co concentration on the structural and magnetic properties of Ni0.9−xZn0.1CoxFe2O4 nanocrystals, particularly their temperature-dependent magnetic transitions.

采用溶胶-凝胶法合成了纳米晶Ni0.9−xZn0.1CoxFe2O4 (x = 0.2, 0.4, 0.6, 0.8)铁氧体,经Rietveld细化证实为立方单相尖晶石结构(Fd−3m)。随着Co取代量的增加,晶体尺寸从7 nm增加到10 nm。磁性表征显示了Co浓度的显著依赖性,零场冷却和场冷却磁化曲线出现分叉,表明存在磁弛豫现象。Ni0.5Zn0.1Co0.4Fe2O4的阻滞温度为191 K,居里温度为207 K,在5 K时从铁磁有序转变为300 K时的超顺磁行为。同样,Ni0.3Zn0.1Co0.6Fe2O4在251 K时发生转变,在5 K时保持铁磁有序。相比之下,Ni0.1Zn0.1Co0.8Fe2O4在300 K时表现出磁不可逆性和顺磁性。拉曼光谱进一步证实了尖晶石的反向结构,揭示了~ 460 cm - 1和680 cm - 1的特征振动模式。这些发现强调了Co取代在调节Ni0.9−xZn0.1CoxFe2O4纳米晶体的结构和磁性方面的关键作用,特别是它们的温度依赖的磁相变。总的来说,这些结果突出了Co浓度对Ni0.9−xZn0.1CoxFe2O4纳米晶体结构和磁性能的影响,特别是它们的温度依赖性磁跃迁。
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引用次数: 0
Magnetocaloric Effect and Thermodynamic Properties of Trapped Polarons in 2D Monolayers Transition Metal Dichalcogenides 二维单层过渡金属硫化物中捕获极化子的磁热效应和热力学性质
IF 1.4 3区 物理与天体物理 Q4 PHYSICS, APPLIED Pub Date : 2025-05-30 DOI: 10.1007/s10909-025-03298-z
J. V. Nguepnang, B. Donfack, C. M. Ekengoue, E. L. Mbieda-Posseu, F. X. Ngagoum Tchamdjeu, W. Nganfo, C. Kenfack-Sadem

We investigated the magnetocaloric effect (MCE) and thermodynamic properties of Magnetopolaron embedded in two-dimensional (2D) transition metal dichalcogenides (TMDs) under the canonical ensemble approach. From the results, we found that an increase in magnetic field considerably affects the magnetic moment alignment or brings an additional energy in 2D TMDs monolayers which is responsible for the energy exchange observed. The entropy change or MCE, which is more pronounced in the case of molybdenum and less for tungsten, affects the magnetic state of material. The combined effect of magnetic field and temperature has a great change on the magnetic state of 2D TMDs monolayer materials. The behavior of free energy obtained in the present paper can be used as a characteristic of paramagnetic materials. It comes that all 2D TMDs monolayers studied in the present manuscript present a paramagnetic aspect making them promising candidates for practical applications of magnetic refrigeration.

利用正则系综方法研究了嵌入二维(2D)过渡金属二硫化物(TMDs)中的磁极化子的磁热效应(MCE)和热力学性质。从结果来看,我们发现磁场的增加会显著影响磁矩排列或在二维tmd单层中带来额外的能量,这是所观察到的能量交换的原因。熵变(MCE)影响材料的磁性状态,钼的熵变更明显,钨的熵变较小。磁场和温度的共同作用对二维tmd单层材料的磁态有很大的影响。本文所得的自由能行为可以作为顺磁性材料的一种特性。在本论文中研究的所有二维tmd单层都呈现出顺磁性,使它们成为磁制冷实际应用的有希望的候选者。
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引用次数: 0
Surface Dilution Effects on Magnetic Properties and Compensation Phenomena of ({Fe}^{text{II}}), ({Fe}^{text{III}})) Core–Shell Ferrimagnetic Nanotubes: Monte Carlo Study 表面稀释对({Fe}^{text{II}}), ({Fe}^{text{III}}))核-壳铁磁纳米管磁性能和补偿现象的影响:蒙特卡罗研究
IF 1.4 3区 物理与天体物理 Q4 PHYSICS, APPLIED Pub Date : 2025-05-30 DOI: 10.1007/s10909-025-03305-3
Z. Elmghabar, A. Elidrysy, L. B. Drissi, S. Harir

Using Monte Carlo simulations (MCS), we investigated the magnetic properties and phase diagrams of a hexagonal ferrimagnetic Ising nanotube with a core–shell structure composed of spin-5/2 and spin-2 particles, taking surface dilution into account. Our results revealed several characteristic behaviors. Notably, the concentration of magnetic atoms has a significant influence on both the critical and compensation temperatures. For low values of the exchange interaction ({J}_{s})​, dilution has no effect on the critical temperature. However, a compensation point appears beyond a dilution threshold, observed for (xge 0.6).We also identified critical thresholds for the crystal field anisotropies ({D}_{s})​ and ({D}_{c})​. Below these thresholds, the critical temperature remains nearly constant, then gradually increases and converges toward a saturation value once the thresholds are exceeded. Furthermore, the analysis of hysteresis loops shows that the system’s magnetic response is highly influenced by dilution: the remanent magnetization increases significantly in absolute value as the concentration of magnetic atoms rises from (0.6) to(1.0).

利用蒙特卡罗模拟(Monte Carlo simulation, MCS)研究了考虑表面稀释的六方铁磁Ising纳米管的磁性和相图,该六方铁磁Ising纳米管具有自旋5/2和自旋2粒子组成的核壳结构。我们的结果揭示了几个特征行为。值得注意的是,磁性原子的浓度对临界温度和补偿温度都有显著影响。对于低交换相互作用({J}_{s})值,稀释对临界温度没有影响。然而,补偿点出现在稀释阈值之外,观察到(xge 0.6)。我们还确定了晶体场各向异性的临界阈值({D}_{s})和({D}_{c})。在这些阈值以下,临界温度几乎保持不变,一旦超过阈值,临界温度逐渐升高并收敛到饱和值。此外,对磁滞回线的分析表明,系统的磁响应受稀释的影响很大:随着磁性原子浓度从(0.6)增加到(1.0),剩余磁化强度的绝对值显著增加。
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引用次数: 0
Study on Structural and Thermodynamic Properties of Solid Nitrogen with HCP Structure by Statistical Moment Method 用统计矩法研究具有HCP结构的固体氮的结构和热力学性质
IF 1.4 3区 物理与天体物理 Q4 PHYSICS, APPLIED Pub Date : 2025-05-30 DOI: 10.1007/s10909-025-03302-6
Hoc Quang Nguyen, Linh Mai Thi Le, Yen Hai Le, Huyen Ngoc Thi Ha, Hoa Ngoc Pham, Dat Xuan Hua, Cuong Chinh Nguyen

The paper presents the analytic expressions of nearest neighbor distance between two particle, Helmholtz free energy, thermodynamic and structural quantities for hcp crystals on the basis of the statistical moment method (SMM) taking into account of vibrational motion of particles, Helmholtz free energy and thermodynamic quantities for hcp crystals on the basis of the self-consistent field method (SCFM) taking into account of molecular motion. The theoretical results are applied to calculate numerically for hcp-N2. Some numerical results are compared with experiments and other calculations.

本文给出了考虑粒子振动运动的统计矩法(SMM)和考虑分子运动的自洽场法(SCFM)的两粒子最近邻距离、hcp晶体的亥姆霍兹自由能、热力学和结构量的解析表达式。将理论结果应用于hcp-N2的数值计算。一些数值计算结果与实验和其他计算结果进行了比较。
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引用次数: 0
Thermodynamic Properties of Gapped Graphene Quantum Dots in Aharonov–Bohm Field Aharonov-Bohm场中石墨烯量子点的热力学性质
IF 1.4 3区 物理与天体物理 Q4 PHYSICS, APPLIED Pub Date : 2025-05-27 DOI: 10.1007/s10909-025-03303-5
Guichao Liu, Jie Zhang

This investigation explores the influence of temperature, radius, Aharonov–Bohm flux, and bandgap energy on the specific heat and magnetocaloric properties of graphene quantum dots. By enforcing the continuity condition of eigenspinors at the graphene quantum dots boundary, an analytical relation is derived, demonstrating the dependence of quantized energy levels on external physical parameters. The specific heat exhibits a Schottky-like anomaly, characterized by an initial rise with increasing temperature, reaching a maximum, followed by a subsequent decline. Enhanced magnetic fields induce a shift in the peak temperature while maintaining a consistent peak magnitude (~ 0.44 J/K). The magnetocaloric potential exhibits a monotonic increase with magnetic field intensity, converging to a saturation value of − 0.7 J/(kg⋅K) at elevated temperatures, where thermal fluctuations dominate. Furthermore, the magnetocaloric response demonstrates greater sensitivity to variations in bandgap energy and magnetic field strength compared to changes in the dot radius and Aharonov–Bohm flux.

本研究探讨了温度、半径、Aharonov-Bohm通量和带隙能量对石墨烯量子点比热和磁热性能的影响。通过在石墨烯量子点边界施加本征旋量的连续性条件,推导出一个解析关系,证明了量子化能级与外部物理参数的依赖关系。比热表现为肖特基异常,其特征是随着温度的升高而开始上升,达到最大值,随后下降。增强磁场会引起峰值温度的变化,同时保持恒定的峰值量级(~ 0.44 J/K)。磁热势随磁场强度单调增加,在高温下趋于饱和值- 0.7 J/(kg·K),其中热波动占主导地位。此外,与点半径和Aharonov-Bohm通量的变化相比,磁热响应对带隙能量和磁场强度的变化更敏感。
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引用次数: 0
Luminescence of Nitrogen–Neon Nanoclusters 氮-氖纳米团簇的发光特性
IF 1.4 3区 物理与天体物理 Q4 PHYSICS, APPLIED Pub Date : 2025-05-23 DOI: 10.1007/s10909-025-03304-4
Oleksandr Korostyshevskyi, Cameron Wetzel, Ivan V. Borzenets, David M. Lee, Vladimir V. Khmelenko

The decay dynamics of the (alpha)-group ((^2)(rightarrow ^4)S transition) of N atoms stabilized in the collection of (hbox {N}_2)–Ne nanoclusters were studied at a temperature of 1.3 K. The variation of the (hbox {N}_2)/Ne ratio in nanoclusters results in substantial changes in the luminescence spectra of the (alpha)-group and in the characteristic decay times for the components of these spectra. In all obtained (alpha)-group spectra, the narrow component at (lambda) = 519.9 nm was observed. The spectroscopic results provide information about the structure of the nitrogen–neon nanoclusters. At elevated temperatures ((approx) 15–36 K), enhanced oxygen (beta)-group luminescence is observed in (hbox {N}_2)–Ne nanoclusters, with a smaller intensity enhancement than those observed within pure (hbox {N}_2) and mixed (hbox {N}_2)–Kr nanoclusters. These results confirm the energy transfer mechanism, in which excited nitrogen molecules formed on the nanocluster surface transfer energy to the stabilized oxygen atoms through the chain of (hbox {N}_2) molecules in a solid matrix.

研究了(hbox {N}_2) -Ne纳米团簇中稳定的N原子(alpha) -基团((^2) D (rightarrow ^4) S跃迁)在1.3 K温度下的衰变动力学。纳米团簇中(hbox {N}_2) /Ne比的变化导致(alpha) -基团的发光光谱和这些光谱成分的特征衰减时间发生实质性变化。在所有得到的(alpha) -基团光谱中,在(lambda) = 519.9 nm处观察到窄组分。光谱结果提供了有关氮氖纳米团簇结构的信息。在高温((approx) 15-36 K)下,(hbox {N}_2) -Ne纳米团簇中的氧- (beta)基团发光增强,强度增强幅度小于纯(hbox {N}_2)和混合(hbox {N}_2) -Kr纳米团簇。这些结果证实了纳米簇表面形成的受激氮分子通过固体基质中(hbox {N}_2)分子链将能量传递给稳定氧原子的传递机制。
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引用次数: 0
Non-Monotonic Thermal Relaxation in the Nanopore Heat Exchanger for Dilution Refrigerator 稀释冰箱用纳米孔热交换器的非单调热松弛
IF 1.4 3区 物理与天体物理 Q4 PHYSICS, APPLIED Pub Date : 2025-05-22 DOI: 10.1007/s10909-025-03297-0
Azimjon A. Temurjonov, Taku Matsushita, Mitsunori Hieda, Nobuo Wada

Thermal resistance and the thermal relaxation time are important physical properties in order to cool down samples at low temperatures. In the case of a dilution refrigerator, the relation between the thermal relaxation time of working fluid in a heat exchanger and the circulation rate should be taken care of. Recently, we reported on the nanopore heat exchanger with dramatically reduced thermal resistance. Experimental results suggested that the thermal relaxation time in the sinter pad is very short (less than 1 s), while the exact value was not determined. In order to verify its relation to the circulation rate, we performed numerical simulations of the thermal relaxation time. The expected monotonic increase with decrease of temperature has been confirmed down to 50 mK. However, at lower temperatures unexpected decrease is found. This unusual behavior is considered due to relatively small thermal resistance of liquid helium compared with the thermal boundary resistance.

热阻和热松弛时间是低温冷却样品的重要物理性质。对于稀释式制冷机,应注意换热器内工质的热松弛时间与循环速率的关系。最近,我们报道了热阻显著降低的纳米孔换热器。实验结果表明,烧结垫上的热松弛时间很短(小于1 s),但没有确定确切的时间。为了验证其与循环速率的关系,我们对热松弛时间进行了数值模拟。在低至50 mK时,随温度的降低而出现了预期的单调增加,但在较低的温度下却出现了意想不到的下降。这种不寻常的行为被认为是由于与热边界阻力相比,液氦的热阻相对较小。
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引用次数: 0
The 2024 International Symposium on Quantum Fluids and Solids (QFS2024) 2024年量子流体与固体国际学术研讨会(QFS2024)
IF 1.4 3区 物理与天体物理 Q4 PHYSICS, APPLIED Pub Date : 2025-05-19 DOI: 10.1007/s10909-025-03308-0
Wei Guo, Yoonseok Lee
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引用次数: 0
Preface of "Quantum Technologies with Floating Charged Particles" 《带有浮动带电粒子的量子技术》前言
IF 1.4 3区 物理与天体物理 Q4 PHYSICS, APPLIED Pub Date : 2025-05-13 DOI: 10.1007/s10909-025-03300-8
Denis Konstantinov
{"title":"Preface of \"Quantum Technologies with Floating Charged Particles\"","authors":"Denis Konstantinov","doi":"10.1007/s10909-025-03300-8","DOIUrl":"10.1007/s10909-025-03300-8","url":null,"abstract":"","PeriodicalId":641,"journal":{"name":"Journal of Low Temperature Physics","volume":"219 5-6","pages":"227 - 229"},"PeriodicalIF":1.4,"publicationDate":"2025-05-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145165288","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Temperature-Sensitive Porous Thin-Films for Superconducting Transition-Edge Sensors 用于超导过渡边缘传感器的温度敏感多孔薄膜
IF 1.4 3区 物理与天体物理 Q4 PHYSICS, APPLIED Pub Date : 2025-05-12 DOI: 10.1007/s10909-025-03296-1
Tao Wang, SongNing Wang, YaQiang Chai, L. F. Wei

Superconducting transition-edge sensor (TES) is one of the sensitive single-photon detectors and possesses the photon-number resolving ability. Almost all of the existing sensitive radiation thermal absorption thin films for the generation of TESs are usually generated by optimizing the material components of the films. Alternatively, in this paper we experimentally demonstrated a flexible and controllable approach to generate the temperature-sensitive superconducting one-component thin film, by using the laser drilling technique. Specifically, we designed the sample by numerical simulation method, fabricated the aluminum (Al) thin film with the optimized pore parameters, and experimentally measured the temperature-dependent resistances in ultra-low thermal noise environments. The measured results indicate that, the resistances of the fabricated porous Al films are highly temperature-sensitive around their superconducting transition-edge regimes, and thus they can be utilized to make the desired TES devices. Although the work temperature of the prepared (mu)-Mux readout circuit does not match the generated TES configuration at present, we argue that the one-component porous films, demonstrated here, may provide an effective approach to make the desired TES device for the experimental implementation of infrared single-photon detection.

超导过渡边缘传感器(TES)是一种灵敏的单光子探测器,具有光子数分辨能力。现有的用于生成TESs的敏感辐射热吸收薄膜,几乎都是通过优化薄膜的材料组分来生成的。另外,在本文中,我们通过实验证明了一种灵活可控的方法,通过使用激光钻孔技术来产生温度敏感的超导单组分薄膜。具体而言,我们采用数值模拟方法设计样品,制备了具有优化孔径参数的铝(Al)薄膜,并在超低热噪声环境下实验测量了温度相关电阻。测量结果表明,制备的多孔铝膜在其超导过渡边缘区附近具有高度的温度敏感性,因此可以用来制造所需的TES器件。虽然目前制备的(mu) -Mux读出电路的工作温度与生成的TES配置不匹配,但我们认为,这里展示的单组分多孔膜可能提供了一种有效的方法来制造所需的TES器件,用于红外单光子探测的实验实现。
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引用次数: 0
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Journal of Low Temperature Physics
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