Pub Date : 2024-12-16DOI: 10.1007/s10948-024-06852-0
Xiu-Zhi Duan, Guang-Xin Wang, Li-Chun Hu, Zhang Pan
We have investigated the superconductor-insulator transition (SIT) induced by a disorder of a granular system. The effective energy gap model based on localized Cooper pairs and hopping quasiparticles has been used. The “quasi-reentrant” behavior appears when the metal volume fraction is slightly smaller than the percolation threshold. In particular, we have found the double “quasi-reentrant” behavior with the increased superconducting transition width. This result indicates that the double “quasi-reentrant” behavior should have been observed in a granular system with a large transition width. Besides, the “quasi-reentrant” behavior has been flattened when applying the magnetic field. In order to clarify the method is suitable for a granular system, the theoretical result has been compared with the experimental value of Pb(_x)(SiO(_2))(_{1-x}) granular film. It has almost no difference near the minimum value and the differences onset at lower temperatures due to the negative electroresistance effect. The “quasi-reentrant” behavior becomes unobvious due to the Copper pairs destroyed by the magnetic field.
{"title":"The Properties of “Quasi-Reentrant” Behavior in Granular System","authors":"Xiu-Zhi Duan, Guang-Xin Wang, Li-Chun Hu, Zhang Pan","doi":"10.1007/s10948-024-06852-0","DOIUrl":"10.1007/s10948-024-06852-0","url":null,"abstract":"<div><p>We have investigated the superconductor-insulator transition (SIT) induced by a disorder of a granular system. The effective energy gap model based on localized Cooper pairs and hopping quasiparticles has been used. The “quasi-reentrant” behavior appears when the metal volume fraction is slightly smaller than the percolation threshold. In particular, we have found the double “quasi-reentrant” behavior with the increased superconducting transition width. This result indicates that the double “quasi-reentrant” behavior should have been observed in a granular system with a large transition width. Besides, the “quasi-reentrant” behavior has been flattened when applying the magnetic field. In order to clarify the method is suitable for a granular system, the theoretical result has been compared with the experimental value of Pb<span>(_x)</span>(SiO<span>(_2)</span>)<span>(_{1-x})</span> granular film. It has almost no difference near the minimum value and the differences onset at lower temperatures due to the negative electroresistance effect. The “quasi-reentrant” behavior becomes unobvious due to the Copper pairs destroyed by the magnetic field.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142826303","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-16DOI: 10.1007/s10948-024-06864-w
Gourav Vaid, Atharv Sawant, Neeraj K. Rajak, D. Jaiswal-Nagar
The growth of the high-T(_c) cuprate Bi(_2)Sr(_2)CaCu(_2)O(_{8+delta }) (BSCCO-2212) superconductor is always challenging due to the contamination from alumina crucible or the intergrowth of other phases such as Bi(_2)Sr(_2)CuO(_{6+ delta }) (Bi-2201). In this work, we report the synthesis of single crystals of BSCCO-2212 with the highest reported superconducting transition temperature, T(_c), of 96.6 K, achieved using an improved self-flux technique. The as-grown crystals were characterized by scanning electron microscopy (SEM), energy-dispersive x-ray spectroscopy (EDS), and powder x-ray diffraction (p-XRD) measurements. PXRD on single crystals reveals the absence of contamination from the alumina crucible as well as the absence of the intergrowth of Bi-2201 phase. PXRD on crushed single crystals reveals minimal intergrowth of Bi-2201 and Bi-2223 phases. The physical properties were investigated by carrying out temperature-dependent magnetization and resistance measurements. Magnetization measurements revealed the T(_c) of three single crystals of BSCCO-2212 to be 93 K, 94 K, and 96.6 K, higher than the previously reported values in the range from (sim ) 90 to 93 K [1,2,3,4,5]. Such a high T(_c) and the absence of an intergrowth phase indicates a good quality of the grown crystals that can be utilized for fundamental as well as basic research.
高t (_c)铜酸铋(_2) Sr (_2) CaCu (_2) O (_{8+delta }) (BSCCO-2212)超导体的生长总是具有挑战性,因为氧化铝坩埚的污染或其他相如Bi (_2) Sr (_2) CuO (_{6+ delta }) (Bi-2201)的共同生长。在这项工作中,我们报道了利用改进的自通量技术合成BSCCO-2212单晶,其超导转变温度T (_c)为96.6 K,达到了报道的最高水平。通过扫描电子显微镜(SEM)、能量色散x射线能谱(EDS)和粉末x射线衍射(p-XRD)测量对生长晶体进行了表征。对单晶进行PXRD分析,发现没有氧化铝坩埚的污染,也没有Bi-2201相的共生。破碎单晶的PXRD分析显示,Bi-2201和Bi-2223相的共生生长极少。通过进行温度相关的磁化和电阻测量来研究其物理性质。磁化测量结果显示,BSCCO-2212的三个单晶的T (_c)分别为93 K、94 K和96.6 K,高于之前报道的(sim ) 90 ~ 93 K[1,2,3,4,5]。如此高的T (_c)和没有共生相表明生长的晶体质量好,可以用于基础研究和基础研究。
{"title":"Growth of High Quality Bi(_2)Sr(_2)CaCu(_2)O(_{8+delta }) Single Crystals with a High Critical Temperature of 96 K Using Alumina Crucible","authors":"Gourav Vaid, Atharv Sawant, Neeraj K. Rajak, D. Jaiswal-Nagar","doi":"10.1007/s10948-024-06864-w","DOIUrl":"10.1007/s10948-024-06864-w","url":null,"abstract":"<div><p>The growth of the high-T<span>(_c)</span> cuprate Bi<span>(_2)</span>Sr<span>(_2)</span>CaCu<span>(_2)</span>O<span>(_{8+delta })</span> (BSCCO-2212) superconductor is always challenging due to the contamination from alumina crucible or the intergrowth of other phases such as Bi<span>(_2)</span>Sr<span>(_2)</span>CuO<span>(_{6+ delta })</span> (Bi-2201). In this work, we report the synthesis of single crystals of BSCCO-2212 with the highest reported superconducting transition temperature, T<span>(_c)</span>, of 96.6 K, achieved using an improved self-flux technique. The as-grown crystals were characterized by scanning electron microscopy (SEM), energy-dispersive x-ray spectroscopy (EDS), and powder x-ray diffraction (p-XRD) measurements. PXRD on single crystals reveals the absence of contamination from the alumina crucible as well as the absence of the intergrowth of Bi-2201 phase. PXRD on crushed single crystals reveals minimal intergrowth of Bi-2201 and Bi-2223 phases. The physical properties were investigated by carrying out temperature-dependent magnetization and resistance measurements. Magnetization measurements revealed the T<span>(_c)</span> of three single crystals of BSCCO-2212 to be 93 K, 94 K, and 96.6 K, higher than the previously reported values in the range from <span>(sim )</span> 90 to 93 K [1,2,3,4,5]. Such a high T<span>(_c)</span> and the absence of an intergrowth phase indicates a good quality of the grown crystals that can be utilized for fundamental as well as basic research.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142826161","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-14DOI: 10.1007/s10948-024-06860-0
D. V. Seleznev, S. S. Seidov, N. G. Pugach, D. G. Bezymiannykh, S. I. Mukhin, B. G. L’vov
We consider a spin valve composed of a superconducting film (S) between two ferromagnetic insulators (FI) on two sides. In the dirty limit, the superconductor is described by Usadel equations. Appropriate boundary conditions were chosen for two S-FI interfaces, which are described via the interface parameter spin mixing angle. By numerically solving the Usadel equations, the density of states (DOS) at different spin mixing angles was obtained. It was shown previously that the critical temperature of such an FI-S-FI structure depends on the mutual alignment of the FI layers’ magnetization. We follow the evolution of DOS at the change of misalignment of ferromagnets magnetization and probe the zero bias peak creation. The DOS characteristic features may give fruitful information about triplet superconducting components creation and interplay inside the S layer.
我们考虑一个自旋阀,它由两面铁磁绝缘体(FI)之间的超导薄膜(S)组成。在脏极限下,超导体由乌萨德尔方程描述。为两个 S-FI 接口选择了适当的边界条件,通过接口参数自旋混合角来描述。通过对乌萨德尔方程进行数值求解,得到了不同自旋混合角下的状态密度(DOS)。之前的研究表明,这种 FI-S-FI 结构的临界温度取决于 FI 层磁化的相互排列。我们跟踪了铁磁体磁化错位变化时的 DOS 演变,并探究了零偏压峰的产生。DOS特征可能会提供有关三重超导成分在S层内部产生和相互作用的有用信息。
{"title":"Density of States in the Heterostructure Ferromagnetic Insulator-Superconductor-Ferromagnetic Insulator","authors":"D. V. Seleznev, S. S. Seidov, N. G. Pugach, D. G. Bezymiannykh, S. I. Mukhin, B. G. L’vov","doi":"10.1007/s10948-024-06860-0","DOIUrl":"10.1007/s10948-024-06860-0","url":null,"abstract":"<div><p>We consider a spin valve composed of a superconducting film (S) between two ferromagnetic insulators (FI) on two sides. In the dirty limit, the superconductor is described by Usadel equations. Appropriate boundary conditions were chosen for two S-FI interfaces, which are described via the interface parameter spin mixing angle. By numerically solving the Usadel equations, the density of states (DOS) at different spin mixing angles was obtained. It was shown previously that the critical temperature of such an FI-S-FI structure depends on the mutual alignment of the FI layers’ magnetization. We follow the evolution of DOS at the change of misalignment of ferromagnets magnetization and probe the zero bias peak creation. The DOS characteristic features may give fruitful information about triplet superconducting components creation and interplay inside the S layer.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142821358","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-13DOI: 10.1007/s10948-024-06887-3
D. H. Ryan
Recently, Junbao He et al. reported on magnetic ordering in the topological candidate EuZnBi(_2) (He et al. J. Supercond. Nov. Magn. 37, 579 2024) and suggested that there is a spin reorientation near 15 K, below the initial antiferromagnetic transition at T(_N)=20 K. Here we use (^{151})Eu Mössbauer spectroscopy to show that the situation is more complex. The initial ordering involves an incommensurate sinusoidally modulated structure that progressively squares up on further cooling.
最近,何俊宝等人报道了拓扑候选者EuZnBi (_2)的磁有序(He et al.)。J.超低温;Nov. Magn. 37, 579 2024),并提出在T (_N) = 20k的初始反铁磁跃迁下,在15k附近存在自旋重定向。这里我们用(^{151}) Eu Mössbauer光谱来说明情况要复杂得多。最初的排序涉及一个不相称的正弦调制结构,该结构在进一步冷却时逐渐调整。
{"title":"A (^{151})Eu Mössbauer investigation of Magnetic Ordering in the Topological Material Candidate EuZnBi(_2)","authors":"D. H. Ryan","doi":"10.1007/s10948-024-06887-3","DOIUrl":"10.1007/s10948-024-06887-3","url":null,"abstract":"<div><p>Recently, Junbao He et al. reported on magnetic ordering in the topological candidate EuZnBi<span>(_2)</span> (He et al. J. Supercond. Nov. Magn. <b>37</b>, 579 2024) and suggested that there is a spin reorientation near 15 K, below the initial antiferromagnetic transition at T<span>(_N)</span>=20 K. Here we use <span>(^{151})</span>Eu Mössbauer spectroscopy to show that the situation is more complex. The initial ordering involves an incommensurate sinusoidally modulated structure that progressively squares up on further cooling.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142811266","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
In this paper, a microscopic model of anisotropic soft magnetic composites based on three-dimensional homogeneous distribution is established with numerical calculation. The effects of the particle orientation angle and the axial diameter ratio on the equivalent permeability of composites were investigated by the finite element method, and the accuracy of the model was verified by using experimental results in comparison with the simulation results. The results show that the composites have the largest equivalent permeability of 63.944 when the particle orientation angle is 0° (particle size of 75 µm). As the insulating layer is consistent, the larger equivalent permeability of composites is obtained by the larger particle axial diameter ratio. The equivalent permeability of composites is 114.07 when the axial diameter ratio is 100, which is 89.76% larger than that of the composites with an axial diameter ratio of 5. The equivalent permeability of the specimen with the orientation angle of 0° and the particle axial diameter ratio of 42 is 48.579, and the equivalent permeability of the model under the same conditions is 47.276 in the simulation. The comparative analysis found that the simulation and experiment value only have an error of 2.68%, which is within the acceptable range and further proves the accuracy of this model.
{"title":"Influence of Particle Orientation Angle and Axial Diameter Ratio on the Magnetic Properties of Soft Magnetic Composites by Finite Element Method","authors":"Shen Wu, Zhenzhen Dong, Xiaoran Sun, Xiangkui Zhou, Jianglei Fan, Ying Li, Xin Li, Shizhong Wei","doi":"10.1007/s10948-024-06856-w","DOIUrl":"10.1007/s10948-024-06856-w","url":null,"abstract":"<div><p>In this paper, a microscopic model of anisotropic soft magnetic composites based on three-dimensional homogeneous distribution is established with numerical calculation. The effects of the particle orientation angle and the axial diameter ratio on the equivalent permeability of composites were investigated by the finite element method, and the accuracy of the model was verified by using experimental results in comparison with the simulation results. The results show that the composites have the largest equivalent permeability of 63.944 when the particle orientation angle is 0° (particle size of 75 µm). As the insulating layer is consistent, the larger equivalent permeability of composites is obtained by the larger particle axial diameter ratio. The equivalent permeability of composites is 114.07 when the axial diameter ratio is 100, which is 89.76% larger than that of the composites with an axial diameter ratio of 5. The equivalent permeability of the specimen with the orientation angle of 0° and the particle axial diameter ratio of 42 is 48.579, and the equivalent permeability of the model under the same conditions is 47.276 in the simulation. The comparative analysis found that the simulation and experiment value only have an error of 2.68%, which is within the acceptable range and further proves the accuracy of this model.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142811267","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-13DOI: 10.1007/s10948-024-06839-x
G. P. Fuentes, D. B. O. Silva, L. K. C. S. Assis, L. A. P. Gonçalves, E. Padrón-Hernández
The analysis of ferromagnetic resonance (FMR) through micromagnetic simulations is a powerful tool used to gain insight into the effects of shape on magnetization dynamics. Mathematical models incorporated into simulation programs have greatly facilitated the understanding of resulting magnetic behaviors. The present study aimed to investigate the influence of shape on the magnetization dynamics of Permalloy discs and stadium-like geometries of finite dimensions. The finite element numerical method was used to perform simulations, employing the Nmag simulator. To simulate the FMR spectra, the ringdown method was utilized, a common technique in computational micromagnetism. Resonance modes were identified using Fourier transform analysis. The novelty of this work is to demonstrate that in a film with a thickness of 50 nm and lateral dimensions less than 1000 nm, it cannot be considered as an infinite film. The results of the calculations showed that, for an in-plane field in a Py disk with these dimensions, there are resonance fields affected when the geometry is slightly stretched. This phenomenon was observed applying a field parallel to the plane of a stadium-shaped geometry. The effects of shape anisotropy remain relevant even in a 50 nm film with lateral dimensions exceeding 1000 nm. The aim of the study is to review results that are normally used for work with thin films. Assuming infinite dimensions and disregarding shape effects always requires care, since depending on the study in question, artifacts due to the shape effect may arise and be interpreted incorrectly.
{"title":"The Unexpected Shape Effects on Magnetic Properties of Films of Nanometer Thickness and Micrometer Extension","authors":"G. P. Fuentes, D. B. O. Silva, L. K. C. S. Assis, L. A. P. Gonçalves, E. Padrón-Hernández","doi":"10.1007/s10948-024-06839-x","DOIUrl":"10.1007/s10948-024-06839-x","url":null,"abstract":"<div><p>The analysis of ferromagnetic resonance (FMR) through micromagnetic simulations is a powerful tool used to gain insight into the effects of shape on magnetization dynamics. Mathematical models incorporated into simulation programs have greatly facilitated the understanding of resulting magnetic behaviors. The present study aimed to investigate the influence of shape on the magnetization dynamics of Permalloy discs and stadium-like geometries of finite dimensions. The finite element numerical method was used to perform simulations, employing the Nmag simulator. To simulate the FMR spectra, the ringdown method was utilized, a common technique in computational micromagnetism. Resonance modes were identified using Fourier transform analysis. The novelty of this work is to demonstrate that in a film with a thickness of 50 nm and lateral dimensions less than 1000 nm, it cannot be considered as an infinite film. The results of the calculations showed that, for an in-plane field in a Py disk with these dimensions, there are resonance fields affected when the geometry is slightly stretched. This phenomenon was observed applying a field parallel to the plane of a stadium-shaped geometry. The effects of shape anisotropy remain relevant even in a 50 nm film with lateral dimensions exceeding 1000 nm. The aim of the study is to review results that are normally used for work with thin films. Assuming infinite dimensions and disregarding shape effects always requires care, since depending on the study in question, artifacts due to the shape effect may arise and be interpreted incorrectly.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142811268","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-13DOI: 10.1007/s10948-024-06837-z
A. S. Lileev, J. Kargin, Y. V. Konyukhov, D. G. Zhukov, H. Sanchez Cornejo, Ji Won Seo, S. N. Holmes, J. Albino Aguiar, C. H. W. Barnes, L. De Los Santos Valladares
The influence of thermal and thermomagnetic treatment on the magnetic properties of iron—cobalt oxides compacts fabricated by powder metallurgy is studied. The influence of magnetic pulse processing (MPP) on the formation of the phase composition and magnetic properties of nanocrystalline α-Fe (50%) + Fe2O3 (50%); α-Fe (50%) + Fe2O3 (40%) + Co3O4 (10%) and α-Fe (50%) + Fe2O3 (30%) + Co3O4 (20%) pressed powder compacts during synthesis in a high-energy mill and subsequent annealing have been investigated. According to the X-ray diffraction analysis, annealing α-Fe (50%) + Fe2O3 (50%) pressed samples at 250 ℃ in air, promotes the oxidation of α-Fe and FeO to magnetite (Fe3O4). Additional annealing of the compact in vacuum at 250 ℃ increases its remnant magnetization and magnetic anisotropy. Whereas, increasing the concentration of Co3O4 oxide has no strong effect on the coercivity and residual magnetization of the compacts. Eventually, thermomagnetic treatment of the α-Fe (50%) + Fe2O3 (30%) + Co3O4 (20%) system does not improve its magnetic properties.
{"title":"The Effects of Thermomagnetic Treatment on the Magnetic Properties of Nanocrystalline Fe–O and Fe-Co–O Pressed Compacts","authors":"A. S. Lileev, J. Kargin, Y. V. Konyukhov, D. G. Zhukov, H. Sanchez Cornejo, Ji Won Seo, S. N. Holmes, J. Albino Aguiar, C. H. W. Barnes, L. De Los Santos Valladares","doi":"10.1007/s10948-024-06837-z","DOIUrl":"10.1007/s10948-024-06837-z","url":null,"abstract":"<div><p>The influence of thermal and thermomagnetic treatment on the magnetic properties of iron—cobalt oxides compacts fabricated by powder metallurgy is studied. The influence of magnetic pulse processing (MPP) on the formation of the phase composition and magnetic properties of nanocrystalline α-Fe (50%) + Fe<sub>2</sub>O<sub>3</sub> (50%); α-Fe (50%) + Fe<sub>2</sub>O<sub>3</sub> (40%) + Co<sub>3</sub>O<sub>4</sub> (10%) and α-Fe (50%) + Fe<sub>2</sub>O<sub>3</sub> (30%) + Co<sub>3</sub>O<sub>4</sub> (20%) pressed powder compacts during synthesis in a high-energy mill and subsequent annealing have been investigated. According to the X-ray diffraction analysis, annealing α-Fe (50%) + Fe<sub>2</sub>O<sub>3</sub> (50%) pressed samples at 250 ℃ in air, promotes the oxidation of α-Fe and FeO to magnetite (Fe<sub>3</sub>O<sub>4</sub>). Additional annealing of the compact in vacuum at 250 ℃ increases its remnant magnetization and magnetic anisotropy. Whereas, increasing the concentration of Co<sub>3</sub>O<sub>4</sub> oxide has no strong effect on the coercivity and residual magnetization of the compacts. Eventually, thermomagnetic treatment of the α-Fe (50%) + Fe<sub>2</sub>O<sub>3</sub> (30%) + Co<sub>3</sub>O<sub>4</sub> (20%) system does not improve its magnetic properties.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10948-024-06837-z.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142821472","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-12DOI: 10.1007/s10948-024-06863-x
Poonam Rani, Rajveer Jha, V. P. S. Awana, Yoshikazu Mizuguchi
Decomposition of superconductors sometimes becomes crucial when studying essential physical properties of the superconductors. For example, the cuprate superconductor YBa2Cu3O7-d decomposes by long-time air exposure. In this study, we investigate the aging effects on superconducting properties of BiS2-based superconductors Bi4O4S3 and LaO0.5F0.5BiS2; both were first synthesized in 2012, using their polycrystalline samples synthesized several years ago. We find that 12-year-old Bi4O4S3 samples exhibit bulk superconductivity with a slight degradation of the superconducting transition temperature (Tc) of 0.2 K. For a high-pressure-synthesized LaO0.5F0.5BiS2 sample, clear decrease in Tc is observed, which suggests that high-pressure strain is reduced by aging.
{"title":"Investigation of Aging Effects on Superconducting Properties of BiS2-based Compounds: First 12-Year Restudy","authors":"Poonam Rani, Rajveer Jha, V. P. S. Awana, Yoshikazu Mizuguchi","doi":"10.1007/s10948-024-06863-x","DOIUrl":"10.1007/s10948-024-06863-x","url":null,"abstract":"<div><p>Decomposition of superconductors sometimes becomes crucial when studying essential physical properties of the superconductors. For example, the cuprate superconductor YBa<sub>2</sub>Cu<sub>3</sub>O<sub>7-<i>d</i></sub> decomposes by long-time air exposure. In this study, we investigate the aging effects on superconducting properties of BiS<sub>2</sub>-based superconductors Bi<sub>4</sub>O<sub>4</sub>S<sub>3</sub> and LaO<sub>0.5</sub>F<sub>0.5</sub>BiS<sub>2</sub>; both were first synthesized in 2012, using their polycrystalline samples synthesized several years ago. We find that 12-year-old Bi<sub>4</sub>O<sub>4</sub>S<sub>3</sub> samples exhibit bulk superconductivity with a slight degradation of the superconducting transition temperature (<i>T</i><sub><i>c</i></sub>) of 0.2 K. For a high-pressure-synthesized LaO<sub>0.5</sub>F<sub>0.5</sub>BiS<sub>2</sub> sample, clear decrease in <i>T</i><sub><i>c</i></sub> is observed, which suggests that high-pressure strain is reduced by aging.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142811036","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-11DOI: 10.1007/s10948-024-06841-3
Elena V. Mostovshchikova, Sergey V. Naumov, Timofey N. Pavlov, Anton Stepanov
The features of the charge subsystem of the Pr0.5Nd0.5BaMn2O6 single crystal with partial A-site ordering are investigated. The manganite is a mixture of a phase with a tetragonal structure (43%) with a high degree of A-site ordering and a disordered phase with a cubic structure (57%). Anisotropy of the optical properties and electrical resistance in the crystallographic ab plane and along the c axis was found. The anisotropy manifests itself as a metal–insulator transition near T≈TC = 150 K in the ab plane and a semiconductor character of the resistance along c above and below TC. The magnetoresistance effect was revealed, which in a field of 1 T reaches 65% in the ab plane and 45% along the c axis near TC and about 40% at low temperatures.
{"title":"Anisotropy of Resistance and Magnetoresistance of Pr0.5Nd0.5BaMn2O6 Single Crystal with Partial A-Site Ordering","authors":"Elena V. Mostovshchikova, Sergey V. Naumov, Timofey N. Pavlov, Anton Stepanov","doi":"10.1007/s10948-024-06841-3","DOIUrl":"10.1007/s10948-024-06841-3","url":null,"abstract":"<div><p>The features of the charge subsystem of the Pr<sub>0.5</sub>Nd<sub>0.5</sub>BaMn<sub>2</sub>O<sub>6</sub> single crystal with partial A-site ordering are investigated. The manganite is a mixture of a phase with a tetragonal structure (43%) with a high degree of A-site ordering and a disordered phase with a cubic structure (57%). Anisotropy of the optical properties and electrical resistance in the crystallographic <i>ab</i> plane and along the <i>c</i> axis was found. The anisotropy manifests itself as a metal–insulator transition near <i>T</i>≈<i>T</i><sub>C</sub> = 150 K in the <i>ab</i> plane and a semiconductor character of the resistance along <i>c</i> above and below <i>T</i><sub>C</sub>. The magnetoresistance effect was revealed, which in a field of 1 T reaches 65% in the <i>ab</i> plane and 45% along the <i>c</i> axis near <i>T</i><sub>C</sub> and about 40% at low temperatures.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142811087","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-11DOI: 10.1007/s10948-024-06835-1
Natalia G. Zamkova, Vyacheslav S. Zhandun, Oksana N. Draganyuk
In this manuscript we study the magnetic MAOX phases (M = Mn, Cr; A = Ga, Al, X = C) obtained by the replacement of the A-layer in the parent MAX phase by the AO2 layer. The screening analysis of the magnetic and electronic properties of Mn- and Cr-based MAOX phases is performed using DFT calculations. All MAOX are thermodynamically stable. It was found that in MAOX phases Cr magnetic moments are pronounced increased in compare to corresponding MAX phase. Moreover, drastically changes in the electronic structure arise in Cr2AlO2C and Cr2GaO2C MAOX phases. The metal behavior in Cr2GaC MAX phase changes for the near to half-metallic behavior with 90% spin polarization at the Fermi energy in Cr2GaO2C MAOX phases. We have found that in Cr2AlO2C, the change in the electronic structure leads to the formation of the spin-gapless semiconductor state under slight extension in the ab plane. The obtained results make Cr2GaO2C and especially Cr2AlO2C prospective candidates for application as functional elements of electronics and spintronics.
{"title":"Magnetic Layered MAOX Phases: DFT Screening of the Magnetic and Electronic Properties","authors":"Natalia G. Zamkova, Vyacheslav S. Zhandun, Oksana N. Draganyuk","doi":"10.1007/s10948-024-06835-1","DOIUrl":"10.1007/s10948-024-06835-1","url":null,"abstract":"<div><p>In this manuscript we study the magnetic MAOX phases (M = Mn, Cr; A = Ga, Al, X = C) obtained by the replacement of the A-layer in the parent MAX phase by the AO<sub>2</sub> layer. The screening analysis of the magnetic and electronic properties of Mn- and Cr-based MAOX phases is performed using DFT calculations. All MAOX are thermodynamically stable. It was found that in MAOX phases Cr magnetic moments are pronounced increased in compare to corresponding MAX phase. Moreover, drastically changes in the electronic structure arise in Cr<sub>2</sub>AlO<sub>2</sub>C and Cr<sub>2</sub>GaO<sub>2</sub>C MAOX phases. The metal behavior in Cr<sub>2</sub>GaC MAX phase changes for the near to half-metallic behavior with 90% spin polarization at the Fermi energy in Cr<sub>2</sub>GaO<sub>2</sub>C MAOX phases. We have found that in Cr<sub>2</sub>AlO<sub>2</sub>C, the change in the electronic structure leads to the formation of the spin-gapless semiconductor state under slight extension in the ab plane. The obtained results make Cr<sub>2</sub>GaO<sub>2</sub>C and especially Cr<sub>2</sub>AlO<sub>2</sub>C prospective candidates for application as functional elements of electronics and spintronics. </p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142811089","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}