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Structure–Magnetism Correlation in 5% Fe-doped TiO₂ Nanostructures Via Mechanical Alloying 机械合金化中掺铁5% tio2纳米结构的结构磁性相关性研究
IF 1.7 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2025-11-08 DOI: 10.1007/s10948-025-07073-9
Hayette Boutarfa, Samah Adjmi, Ali Hafs, Toufik Hafs, Djamel Berdjane, Ramazan Ayaz

Nanocrystalline TiO₂ powders doped with 5 wt% Fe were synthesized by mechanical alloying (MA) with milling times ranging from 0 to 48 h, and their magnetic behavior was systematically investigated. Structural evolution was characterized by X-ray diffraction (XRD) and Rietveld refinement, while magnetic properties were assessed at room temperature using vibrating sample magnetometry (VSM). The structural analysis revealed a progressive anatase-to-rutile transformation with increasing milling time. Metallic Fe reflections, detected at the early stages, diminished as milling progressed, indicating Fe incorporation into the TiO₂ lattice. This structural evolution was accompanied by decreasing crystallite size and increasing microstrain, consistent with enhanced defect generation. Magnetic characterization demonstrated weak ferromagnetism in all samples, with saturation magnetization (Ms) increasing steadily with milling time. The enhancement of Ms is attributed to defect-mediated exchange mechanisms involving Fe substitution at Ti sites and the formation of oxygen vacancies, which act as centers for magnetic interactions. These results underline the strong correlation between structural defects and emergent ferromagnetism in Fe-doped TiO₂ nanostructures, emphasizing the potential of mechanical alloying as an efficient route for engineering dilute magnetic oxides with tunable properties.

采用机械合金化(MA)法制备了掺杂5wt % Fe的纳米tio2粉体,磨矿时间为0 ~ 48 h,并对其磁性行为进行了系统研究。通过x射线衍射(XRD)和Rietveld细化表征了结构演化,通过振动样品磁强计(VSM)在室温下评估了磁性能。结构分析表明,随着磨矿时间的延长,锐钛矿逐渐向金红石转变。在早期阶段检测到的金属铁反射随着铣削的进行而减弱,表明铁掺入了tio2晶格中。这种结构演变伴随着晶粒尺寸的减小和微应变的增加,与缺陷生成的增加相一致。磁性表征表明,所有样品的铁磁性都较弱,饱和磁化强度(Ms)随磨矿时间的增加而稳定增加。Ms的增强归因于缺陷介导的交换机制,包括在Ti位点上的铁取代和氧空位的形成,氧空位作为磁相互作用的中心。这些结果强调了铁掺杂tio2纳米结构中结构缺陷与出现铁磁性之间的强烈相关性,强调了机械合金化作为工程稀释磁性氧化物的有效途径的潜力。
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引用次数: 0
Upper Limit for Superconducting Transition Temperature in Electron – Phonon Superconductors: Very Strong Coupling 电子-声子超导体中超导转变温度的上限:强耦合
IF 1.7 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2025-11-08 DOI: 10.1007/s10948-025-07076-6
M. V. Sadovskii

We present a brief review of some recent work on the problem of highest achievable temperature of superconducting transition (T_c) in electron – phonon systems. The discovery of record – breaking values of (T_c) in quite a number of hydrides under high pressure was an impressive demonstration of capabilities of electron – phonon mechanism of Cooper pairing. This lead to an increased interest on possible limitations of Eliashberg – McMillan theory as the main theory of superconductivity in a system of electrons and phonons. We shall consider some basic conclusions following from this theory and present some remarks on the limit of very strong electron – phonon coupling. We shall discuss possible limitations on the value of the coupling constant related to possible lattice and specific heat instability and conclude that within the stable metallic phase the effective pairing constant may acquire very large values. We discuss some bounds for (T_c) derived in the strong coupling limit and propose an elementary estimate of an upper limit for (T_c), expressed via combination of fundamental physical constants. Finally we also briefly discuss some pessimistic estimates for (T_c) of metallic hydrogen obtained in “jellium” model

我们简要地回顾了最近关于电子-声子系统中超导跃迁最高可达温度(T_c)问题的一些工作。在高压下,在相当多的氢化物中发现了破纪录的(T_c)值,这是对库珀配对的电子-声子机制的一个令人印象深刻的证明。这导致了对Eliashberg - McMillan理论作为电子和声子系统中超导的主要理论的可能局限性的兴趣增加。我们将考虑由这一理论得出的一些基本结论,并对强电子-声子耦合的极限提出一些看法。我们将讨论与可能的晶格和比热不稳定性有关的耦合常数值的可能限制,并得出结论,在稳定的金属相内,有效配对常数可能获得非常大的值。我们讨论了在强耦合极限下推导出的(T_c)的一些边界,并提出了用基本物理常数组合表示的(T_c)的一个上限的初步估计。最后简要讨论了在“凝胶”模型中对(T_c)金属氢的一些悲观估计
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引用次数: 0
Critical Current Anisotropy and Vortex Pinning in NaFe0.935Co0.065As Single Crystals NaFe0.935Co0.065As单晶的临界电流各向异性和涡旋钉钉
IF 1.7 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2025-11-03 DOI: 10.1007/s10948-025-07062-y
A. Yu. Levakhova, V. A. Vlasenko, S. Yu. Gavrilkin, A. Yu. Tsvetkov, S. A. Kuzmichev, A. V. Muratov, T. E. Kuzmicheva, A. I. Shilov, E. O. Rakhmanov, I. V. Morozov

In this work, the nature of vortex pinning has been investigated in overdoped NaFe0.935Co0.065As single crystals. We obtain temperature and field dependences of the critical current density from the magnetic hysteresis loops measured for two field orientations B || ab and B || c. The obtained magnetic anisotropy is about γ ≈ 10 near Tc and drops to about γ ≈ 2 at temperatures below 12 K. Using a Dew-Hughes model, we calculate the normalized pinning force and discuss the pinning nature in NaFe0.935Co0.065As.

本文研究了超掺杂NaFe0.935Co0.065As单晶中涡旋钉钉的性质。我们从两个磁场取向B || ab和B || c测量的磁滞回线中得到了临界电流密度的温度和场依赖性,得到的磁各向异性在Tc附近约为γ≈10,在温度低于12 K时降至约γ≈2。采用Dew-Hughes模型计算归一化钉钉力,讨论了NaFe0.935Co0.065As中的钉钉性质。
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引用次数: 0
Proximity Induced Superconductivity in Antimony Telluride Single Crystal by an Interplay of Indium contacts 铟触点相互作用下碲化锑单晶的邻近感应超导性
IF 1.7 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2025-11-03 DOI: 10.1007/s10948-025-07072-w
Satyendra Singh, R. Venkatesh

To investigate the proximity and inverse proximity superconductivity (SC) in topological materials (TMs) {such as topological insulators (TIs) and topological crystalline insulators (TCIs)} by the hosting of an interface between TM/SC may be the novel strategy in the understanding of the unexplored Majorana fermions and spin-triplet superconductivity etc. [https://doi.org/10.1103/PhysRevB.81.241310, https://doi.org/10.1103/PhysRevRes.3.033008]. The TMs are known to preserve the non-trivial surface states (SS) which have emerged for exploring the exotic superconducting properties induced by the proximity effect. The observed superconductivity (proximity & inverse proximity) induced due to the mutual competition between the robust SS of TMs and sub energy gap of SCs. This strong competition between the electron–electron interaction (EEI) and cooper pairs correlation lead to proximity (inverse proximity) superconductivity if SC energy gap is dominant over EEI or vice versa (if rapidly mobile Dirac electrons break the phase coherence of cooper pairs at the interface (EEI > SC gap)) as discussed in this article. The subsequent changes discussed in the superconducting proximity with perpendicular and parallel magnetic field (M.F) makes this work very interesting due to the field dependence mechanism. The superconducting onset temperature is found to be (Tconset) ~ 4.1 K with the upper critical field (Hc2) ~ 1541 Oersted which is accordance with Ginzburg Landau Theory (GLT) observed in Sb2Te3 contacted with s-wave SC indium.

通过在拓扑材料(如拓扑绝缘体(TIs)和拓扑晶体绝缘体(tci))之间设置界面来研究拓扑材料(TMs)(如拓扑绝缘体(TIs))中的邻近和逆邻近超导性(SC)可能是理解未被探索的马约拉纳费米子和自旋三重态超导性等的新策略[https://doi.org/10.1103/PhysRevB.81.241310, https://doi.org/10.1103/PhysRevRes.3.033008]]。已知TMs可以保留非平凡表面态(SS),这是为了探索由邻近效应引起的奇异超导特性而出现的。观察到的超导性(接近&逆接近)是由于TMs的强SS和sc的亚能隙之间的相互竞争引起的。电子-电子相互作用(EEI)和铜对相关之间的这种强烈竞争导致接近(逆接近)超导性,如果SC能隙占主导地位,反之亦然(如果快速移动的狄拉克电子打破了界面上铜对的相相干性(EEI >; SC间隙)),如本文所讨论的。由于磁场的依赖机制,讨论了垂直和平行磁场下超导接近度的后续变化,使得这项工作非常有趣。发现Sb2Te3与s波SC铟接触时的超导起始温度为(Tconset) ~ 4.1 K,上临界场为(Hc2) ~ 1541 Oersted,符合Ginzburg - Landau理论(GLT)。
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引用次数: 0
Synthesis, Structure, Magnetism of Two-Dimensional Triangular Lattice Materials Ba3REB9O18 (RE = Dy, Ho, Er, Tm and Yb) 二维三角形晶格材料Ba3REB9O18 (RE = Dy, Ho, Er, Tm和Yb)的合成、结构和磁性
IF 1.7 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2025-11-01 DOI: 10.1007/s10948-025-07070-y
Wanxia Liu, Yuxia Gao, Yaning Li, Yulong Li, Weijie Ren, Xin Sun, Xiaofeng Li, Mingli Wang

The synthesis, structure, and magnetic properties of Ba3REB9O18 (RE = Dy-Yb) compounds were investigated. Rietveld Refinement of the X-ray diffraction (XRD) data confirms that all compounds crystallize in a hexagonal Ba3YB9O18-type structure with space group P63/m (No. 176) and Pearson symbol hP62. The lattice parameters a and c increase linearly with the increasing ionic radii of the RE3+ ions. RE3+ ions form two-dimensional triangular layers in the ab plane, which are separated by non-magnetic Ba/B-O polyhedra. The magnetic susceptibility measurement reveals no long-range magnetic order or spin glass behavior in any of the compounds above 2 K. The negative Curie-Weiss temperatures indicate dominant antiferromagnetic (AFM) exchange interactions between the RE3+ ions. The combination of triangular lattice and antiferromagnetic interaction suggests this family of compounds is a promising system for researching magnetic frustration.

研究了Ba3REB9O18 (RE = Dy-Yb)化合物的合成、结构和磁性能。x射线衍射(XRD)数据的Rietveld细化证实,所有化合物结晶为六边形ba3yb9o18型结构,空间群为P63/m (No. 176), Pearson符号为hP62。随着RE3+离子半径的增大,晶格参数a和c呈线性增加。RE3+离子在ab平面上形成二维三角形层,由非磁性Ba/B-O多面体隔开。磁化率测量结果表明,在2 K以上的任何化合物中都没有长程磁序或自旋玻璃行为。负居里-魏斯温度表明RE3+离子之间主要的反铁磁(AFM)交换相互作用。三角形晶格和反铁磁相互作用的结合表明,该化合物家族是研究磁挫败的一个有前途的体系。
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引用次数: 0
Sarma-Bogomol’nyi Equations in Superconductivity 超导中的Sarma-Bogomol 'nyi方程
IF 1.7 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2025-11-01 DOI: 10.1007/s10948-025-07071-x
Mia Kyler, Eugene B. Kolomeisky

Topological defects occurring in nonlinear classical field theories are described by a system of second-order differential equations. A breakthrough was made in 1976 by E. B. Bogomoln’yi who demonstrated that in several field theories these equations can be reduced to first-order provided the coupling constants take on particular values. One of the examples involved a string in the Abelian Higgs model which is equivalent to the Abrikosov flux line of the Ginzburg-Landau theory of superconductivity. In a similar vein, in the 1966 textbook Superconductivity of Metals and Alloys P. G. de Gennes explained how to reduce the second-order Ginzburg-Landau equations to first-order at a particular value of the Ginzburg-Landau parameter by a method due to G. Sarma. We analyze the two ways of arriving at the first-order Sarma-Bogomol’nyi equations and conclude that while they both rely on the same operator identity, Sarma’s method is free of the assumption that there is a topological defect. The implication is that Bogomol’nyi equations found in other field theories may be a source of a wider range of solutions beyond topological defects.

用二阶微分方程组描述了非线性经典场论中的拓扑缺陷。1976年,E. B. Bogomoln 'yi取得了突破,他证明了在一些场论中,如果耦合常数取特定值,这些方程可以简化为一阶。其中一个例子涉及阿贝尔希格斯模型中的一根弦,它相当于金兹堡-朗道超导理论中的阿布里科索夫通量线。同样,在1966年出版的《金属和合金的超导性》一书中,P. G. de Gennes解释了如何用G. Sarma提出的一种方法,将二阶金兹堡-朗道方程在金兹堡-朗道参数的特定值处降阶为一阶。我们分析了得到一阶Sarma- bogomol 'nyi方程的两种方法,并得出结论,虽然它们都依赖于相同的算子恒等式,但Sarma的方法没有假设存在拓扑缺陷。这意味着在其他场论中发现的Bogomol’nyi方程可能是超越拓扑缺陷的更广泛解的来源。
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引用次数: 0
Numerical and Theoretical Analyses of Losses in Armature Windings of Motors for Liquid Hydrogen Pumps 液氢泵电机电枢绕组损耗的数值与理论分析
IF 1.7 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2025-10-30 DOI: 10.1007/s10948-025-07069-5
Kazuhiro Kajikawa, Yuto Mametsuka, Masahiro Furukakoi, Taketsune Nakamura, Akihiro Kikuchi, Tomohito Miura

In order to develop submerged pumps to transfer liquid hydrogen, high temperature superconducting (HTS) motors to drive them as one of key components are a promising candidate with low electromagnetic loss and large specific power density per unit mass. However, since armature windings wound using HTS wires have a couple of problems such as three-phase unbalanced currents and frequency limitations, HTS wires are used only for rotor windings of the motors and metallic cables have to be applied to their armature windings. Therefore, numerical analyses to evaluate loss properties in multi-strand metal twisted cables for armature windings of HTS motors cooled at liquid hydrogen temperature are carried out by means of a two-dimensional finite element method. On the basis of a clarified physical mechanism of losses generated in the windings arranged within a slot of armature iron core, the obtained numerical results are also reproduced with theoretical expressions of the Joule loss for an alternating transport current and the eddy-current loss for an externally applied AC magnetic field. The influences of losses on the frequency and number of strands in metal twisted cables are investigated quantitatively.

高温超导电机作为驱动液氢泵的关键部件之一,具有电磁损耗小、单位质量比功率密度大等优点,是开发液氢泵的理想选择。然而,由于使用高温超导导线缠绕的电枢绕组有一些问题,如三相不平衡电流和频率限制,高温超导导线仅用于电机的转子绕组,金属电缆必须应用于其电枢绕组。为此,采用二维有限元法对液氢温度下高温超导电机电枢绕组用多股金属绞线的损耗特性进行了数值分析。在阐明电枢铁芯槽内绕组产生损耗的物理机理的基础上,用交流输运电流的焦耳损耗和外加交流磁场的涡流损耗的理论表达式再现了所得到的数值结果。定量研究了损耗对金属绞合电缆的频率和股数的影响。
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引用次数: 0
Flux Pinning and Vortex Dynamics in (Y0.5Gd0.5)Ba2Cu3O7-δ Superconducting Film with High-Density BaZrO3 Columnar Defects 高密度BaZrO3柱状缺陷(Y0.5Gd0.5)Ba2Cu3O7-δ超导膜的磁通钉钉和涡流动力学
IF 1.7 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2025-10-23 DOI: 10.1007/s10948-025-07061-z
Qingbin Tang, Lubin Wang, Qiankun Lei, He Lin, Xiaolei Yi, Fangtao Li, Chunlei Wang, Yushan Wang, Dongliang Wang, Benhai Yu

The vortex dynamics for a high-performance BaZrO3 doped (Y0.5Gd0.5)Ba2Cu3O7-δ superconducting films are investigated by a dynamic magnetization-relaxation method. The superconducting films have dense columnar defects with density ~ 1.1×1011 cm−2. The dynamic relaxation rates exhibit a complex temperature dependence, indicating the presence of multiple magnetic vortex phase transitions and complex vortex-vortex interactions. Based on the experimental data, a vortex phase diagram has been constructed, which shows a large vortex elastic motion region suggesting strong flux pinning and potential applications of the REBCO films. There seems to be a vortex slush region under magnetic fields less than 2 T within the temperature range from 10 to 25 K. The investigation on the vortex pinning mechanisms indicates that δl-pinning takes the key role for the vortex motion in the present REBCO films. Based on the present results, it is believed that introducing strong δTc-pinning into REBCO superconducting films is the key to further improving their performance at high temperatures and strong magnetic fields.

采用动态磁化弛豫方法研究了高性能掺杂(Y0.5Gd0.5)Ba2Cu3O7-δ BaZrO3超导薄膜的涡旋动力学。超导薄膜具有致密的柱状缺陷,其密度为~ 1.1×1011 cm−2。动态弛豫率表现出复杂的温度依赖关系,表明存在多重磁涡相变和复杂的涡-涡相互作用。在实验数据的基础上,建立了旋涡相图,显示出一个大的涡弹性运动区域,表明REBCO薄膜具有较强的通量钉住作用和潜在的应用前景。在10 ~ 25 K的温度范围内,在小于2 T的磁场下,似乎存在一个涡滑区。对涡旋钉钉机理的研究表明,δl钉钉对目前REBCO薄膜的涡旋运动起着关键作用。基于目前的研究结果,认为在REBCO超导薄膜中引入强δ tc钉钉是进一步提高其高温强磁场性能的关键。
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引用次数: 0
Tunneling Conductance in Superconducting Junctions with p-wave Unconventional Magnets Breaking Time-reversal Symmetry p波非常规磁体破坏时间反转对称超导结的隧穿电导
IF 1.7 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2025-10-23 DOI: 10.1007/s10948-025-07064-w
Yuri Fukaya, Keiji Yada, Yukio Tanaka

A new type of magnet called p-wave unconventional magnet is proposed, stimulated by the discovery of altermagnet. We study the tunneling conductance of p-wave unconventional magnet/superconductor junctions by adopting the effective Hamiltonian of p-wave unconventional magnets with time-reversal symmetry breaking, suggested (Hellenes et al. P-wave magnets, http://arxiv.org/abs/2309.016072024). The tunneling conductance shows an asymmetric behavior with respect to bias voltage in the helical p-wave superconductor junctions. It is caused by the missing of helical edge states contributing to the charge conductance owing to the momentum-dependent spin-split feature of the Fermi surface in p-wave unconventional magnets. In chiral d and p-wave superconductor junctions, the resulting spin-resolved tunneling conductance takes a different value for spin sectors due to the time-reversal symmetry breaking in superconductors. Our results qualitatively reproduce the results based on the simplified Hamiltonian (Maeda et al. J. Phys. Soc. Jpn. 93, 114703 2024), where only the odd function of the exchange coupling of p-wave unconventional magnets is taken into account, which gives the shift of the Fermi surface and preserves the time-reversal symmetry similar to the spin-orbit coupling.

在交替磁体发现的刺激下,提出了一种新型的p波非常规磁体。我们采用Hellenes等人提出的具有时间反转对称性破缺的p波非常规磁体的有效哈密顿量来研究p波非常规磁体/超导体结的隧穿电导。p波磁体,http://arxiv.org/abs/2309.016072024)。在螺旋p波超导结中,隧穿电导率与偏置电压呈不对称关系。这是由于p波非常规磁体中费米表面的动量依赖自旋分裂特征导致的有助于电荷电导的螺旋边缘态的缺失造成的。在手性d波和p波超导结中,由于超导体中的时间反转对称性破缺,导致自旋分辨隧穿电导率在自旋扇区中具有不同的值。我们的结果定性地再现了基于简化哈密顿量的结果(Maeda et al.)。期刊。Soc。(Jpn. 93, 114703 2024),其中只考虑p波非常规磁体交换耦合的奇函数,该函数给出了费米表面的位移,并保持了类似自旋-轨道耦合的时间反转对称性。
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引用次数: 0
Nonreciprocal Anderson Localization in Disordered Magnetophotonic Crystals: Interplay of Birefringence and Thickness Disorder 无序磁光子晶体中的非互反安德森局域化:双折射和厚度无序的相互作用
IF 1.7 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2025-10-22 DOI: 10.1007/s10948-025-07059-7
Mehrnaz Sarabandi, Mojtaba Golshani, Mehdi Zamani

In this paper, we investigate the interplay between disorder-induced localization and magneto-optical (MO) effects in one-dimensional magnetophotonic crystals (MPCs) composed of alternating Ce:YIG and GGG layers with randomized thicknesses. Using the transfer matrix method, we analyze the localization length and MO responses across polar, longitudinal, and transverse magnetic geometries for wavelengths inside and outside the photonic band gap (PBG). Our results reveal that disorder strength critically modulates localization: while it enhances transmission at PBG edges (consistent with), it suppresses MO effects in longitudinal/transverse geometries, contrasting with the polar case where nonreciprocal localization emerges for circular polarizations. Notably, in the polar geometry, disorder amplifies Faraday rotation. These findings align with recent studies on disorder-enhanced MO responses while demonstrating the tunability of localization via magnetic and structural parameters. The work provides design principles for disordered MPCs in applications such as optical isolation, sensors, and tuneable filters.

在本文中,我们研究了由随机厚度的Ce:YIG和GGG交替层组成的一维磁光子晶体(MPCs)中无序诱导定位和磁光(MO)效应之间的相互作用。利用传递矩阵方法,我们分析了光子带隙(PBG)内外波长在极性、纵向和横向磁几何上的定位长度和MO响应。我们的研究结果表明,无序强度对局域化起着关键的调节作用:虽然它增强了PBG边缘的传输(与)一致,但它抑制了纵向/横向几何中的MO效应,这与圆极化中出现非互反局域化的极性情况形成了对比。值得注意的是,在极几何中,无序放大了法拉第旋转。这些发现与最近关于无序增强MO响应的研究一致,同时证明了通过磁性和结构参数定位的可调性。这项工作为光学隔离、传感器和可调谐滤波器等应用中的无序mpc提供了设计原则。
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引用次数: 0
期刊
Journal of Superconductivity and Novel Magnetism
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