Pub Date : 2024-12-21DOI: 10.1007/s10948-024-06838-y
S. Idrissi, A. Jabar, L. Bahmad
The Fullerene C18 is one of the most active types of nanostructures used as an active ingredient in several applications. This study used Monte Carlo simulations to investigate the magnetic properties of mixed 3/2 and 2 in the fullerene C18 systems. We first perform a theoretical analysis of the ground state phase diagrams. Indeed, we only present and analyze more stable configurations among all possible configurations. Second, calculations were performed to determine how the compound's magnetic properties changed when various physical parameters were altered. In addition, we provide studies of the magnetic behavior of the system at reduced temperature, reduced crystal fields, reduced exchange coupling interactions, and reduced external magnetic fields. Finally, we study and discuss the critical lowering temperature of fullerene C18. To conclude this study, we examined the different hysteresis loops when varying the values of the different physical parameters.
{"title":"Magnetism and Critical Behavior of the Fullerene C18 Studied by Monte Carlo simulations","authors":"S. Idrissi, A. Jabar, L. Bahmad","doi":"10.1007/s10948-024-06838-y","DOIUrl":"10.1007/s10948-024-06838-y","url":null,"abstract":"<div><p>The Fullerene C18 is one of the most active types of nanostructures used as an active ingredient in several applications. This study used Monte Carlo simulations to investigate the magnetic properties of mixed 3/2 and 2 in the fullerene C18 systems. We first perform a theoretical analysis of the ground state phase diagrams. Indeed, we only present and analyze more stable configurations among all possible configurations. Second, calculations were performed to determine how the compound's magnetic properties changed when various physical parameters were altered. In addition, we provide studies of the magnetic behavior of the system at reduced temperature, reduced crystal fields, reduced exchange coupling interactions, and reduced external magnetic fields. Finally, we study and discuss the critical lowering temperature of fullerene C18. To conclude this study, we examined the different hysteresis loops when varying the values of the different physical parameters.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142859671","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-20DOI: 10.1007/s10948-024-06844-0
Anastasiya Lebedeva, František Herman
We study the energy gap within the Dynes superconductor theory. This model generalizes the Bardeen-Cooper-Schrieffer (BCS) approach by including the pair-breaking scattering, introducing the tunneling in-gap states up to a Fermi level. We analytically solve the energy gap equation in various limit cases. The solution provides simple tools for further studies, compared to more complex numerics, and highlights the basic characteristics of the theory. First, in the critical limit of pair-breaking scattering, we derive an analytical form of zero-temperature gap to transition temperature ratio. Next, we derive the dependence of the energy gap close to critical temperature and look at its behavior for general and critical pair-breaking scattering rate. Furthermore, we compare our result with the numerical solution of the gap equation assuming general temperature. We show the range of temperatures, for which the analytical approximation is valid. In the end, we provide the approximative formula of the gap, assuming general pair-breaking scattering, emphasizing its exact behavior close to transition temperature.
{"title":"Detailed Analysis of the Superconducting Gap with Dynes Pair-Breaking Scattering","authors":"Anastasiya Lebedeva, František Herman","doi":"10.1007/s10948-024-06844-0","DOIUrl":"10.1007/s10948-024-06844-0","url":null,"abstract":"<div><p>We study the energy gap within the Dynes superconductor theory. This model generalizes the Bardeen-Cooper-Schrieffer (BCS) approach by including the pair-breaking scattering, introducing the tunneling in-gap states up to a Fermi level. We analytically solve the energy gap equation in various limit cases. The solution provides simple tools for further studies, compared to more complex numerics, and highlights the basic characteristics of the theory. First, in the critical limit of pair-breaking scattering, we derive an analytical form of zero-temperature gap to transition temperature ratio. Next, we derive the dependence of the energy gap close to critical temperature and look at its behavior for general and critical pair-breaking scattering rate. Furthermore, we compare our result with the numerical solution of the gap equation assuming general temperature. We show the range of temperatures, for which the analytical approximation is valid. In the end, we provide the approximative formula of the gap, assuming general pair-breaking scattering, emphasizing its exact behavior close to transition temperature.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10948-024-06844-0.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142859549","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-19DOI: 10.1007/s10948-024-06879-3
Alexander C. Mark, Russell J. Hemley
Recent reports of superconductivity in the vicinity of room temperature have been the subject of discussion by the community. Specifically, features in the resistance-temperature (R-T) relations have raised questions. We show that many of these features can arise from previously unaccounted-for dynamic effects associated with the AC transport techniques often used in high-pressure experiments. These dynamic AC effects can cause the apparent resistance (( R_{apparent} )) to diverge from the DC resistance (( R_{DC} )), sharpen measured superconducting transitions, and produce other features in the measured R-T response. We also show that utilizing the full output of phase-sensitive transport measurements provides a valuable probe of superconducting samples in difficult-to-measure systems.
{"title":"On the Lineshapes of Temperature-Dependent Transport Measurements of Superconductors Under Pressure","authors":"Alexander C. Mark, Russell J. Hemley","doi":"10.1007/s10948-024-06879-3","DOIUrl":"10.1007/s10948-024-06879-3","url":null,"abstract":"<div><p>Recent reports of superconductivity in the vicinity of room temperature have been the subject of discussion by the community. Specifically, features in the resistance-temperature (<i>R</i>-<i>T</i>) relations have raised questions. We show that many of these features can arise from previously unaccounted-for dynamic effects associated with the AC transport techniques often used in high-pressure experiments. These dynamic AC effects can cause the apparent resistance (<span>( R_{apparent} )</span>) to diverge from the DC resistance (<span>( R_{DC} )</span>), sharpen measured superconducting transitions, and produce other features in the measured <i>R</i>-<i>T</i> response. We also show that utilizing the full output of phase-sensitive transport measurements provides a valuable probe of superconducting samples in difficult-to-measure systems.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142844745","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-18DOI: 10.1007/s10948-024-06888-2
H. Y. Dai, Z. H. Zu, Y. K. Chu, R. J. Cui, Z. D. Han
As magnetic refrigerants, first-order transition (FOT) and second-order transition (SOT) materials possess distinct advantages and disadvantages. If the phase transition can be tuned to the critical point between FOT and SOT, it may be possible to combine the benefits of both, thereby achieving an outstanding magnetocaloric effect. Here, we demonstrated this approach through phase transition engineering in Er(Co1-xMnx)2 alloys. When x ≤ 0.06, the magnetic phase transition of the samples was FOT, exhibiting a significant magnetic entropy change. However, at x = 0.08, the samples underwent a SOT from ferromagnetic to paramagnetic, leading to a substantial reduction in the magnetocaloric effect. At the critical point of the FOT/SOT border with x = 0.06, the sample exhibited a large magnetic entropy change along with negligible magnetic hysteresis. This work demonstrates that the critical point between FOT and SOT is an effective means of achieving an excellent magnetocaloric effect.
{"title":"Effect of Phase Transition Type on the Magnetocaloric Effect and Magnetic Hysteresis in Er(Co1-xMnx)2 Laves Alloys","authors":"H. Y. Dai, Z. H. Zu, Y. K. Chu, R. J. Cui, Z. D. Han","doi":"10.1007/s10948-024-06888-2","DOIUrl":"10.1007/s10948-024-06888-2","url":null,"abstract":"<div><p>As magnetic refrigerants, first-order transition (FOT) and second-order transition (SOT) materials possess distinct advantages and disadvantages. If the phase transition can be tuned to the critical point between FOT and SOT, it may be possible to combine the benefits of both, thereby achieving an outstanding magnetocaloric effect. Here, we demonstrated this approach through phase transition engineering in Er(Co<sub>1-x</sub>Mn<sub>x</sub>)<sub>2</sub> alloys. When <i>x</i> ≤ 0.06, the magnetic phase transition of the samples was FOT, exhibiting a significant magnetic entropy change. However, at <i>x</i> = 0.08, the samples underwent a SOT from ferromagnetic to paramagnetic, leading to a substantial reduction in the magnetocaloric effect. At the critical point of the FOT/SOT border with <i>x</i> = 0.06, the sample exhibited a large magnetic entropy change along with negligible magnetic hysteresis. This work demonstrates that the critical point between FOT and SOT is an effective means of achieving an excellent magnetocaloric effect.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142844831","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-18DOI: 10.1007/s10948-024-06873-9
Pinkesh Kumar Mishra, Swapnil Bhuktare
In pursuing energy-efficient and high-performance nonvolatile magnetic memory devices, this study explores voltage-induced techniques, specifically voltage-controlled magnetic anisotropy (VCMA), as an alternative to current-induced methods, which suffer from Ohmic loss. The perpendicular magnetic anisotropy (PMA) nanomagnet, known for its superior stability and scalability compared to in-plane variants, VCMA switching in PMA system requires an in-plane symmetry breaking field, which limits its practicality for on-chip applications. We investigate field-free VCMA switching utilizing strain from a piezoelectric layer and an exchange bias from an antiferromagnetic material. Using macro-spin simulations based on the Landau-Lifshitz-Gilbert equation, we systematically analyze how the VCMA effect, strain-induced magnetoelastic effect, exchange bias, oxide and free layer thicknesses, and damping constant affect the switching performance of the device. The write error rate (WER) drops drastically from 0.2 (without stress) to ({10}^{-6}) (100 MPa stress), showcasing the effectiveness of our approach. We also find that the damping constant, especially in the 0.01–0.05 range, plays a crucial role in further optimizing the switching performance of the device. This study offers new insights for enhancing magnetic memory technology.
{"title":"Strain and Exchange Bias-Enabled Field-Free Voltage-Controlled Magnetic Anisotropy Switching","authors":"Pinkesh Kumar Mishra, Swapnil Bhuktare","doi":"10.1007/s10948-024-06873-9","DOIUrl":"10.1007/s10948-024-06873-9","url":null,"abstract":"<div><p>In pursuing energy-efficient and high-performance nonvolatile magnetic memory devices, this study explores voltage-induced techniques, specifically voltage-controlled magnetic anisotropy (VCMA), as an alternative to current-induced methods, which suffer from Ohmic loss. The perpendicular magnetic anisotropy (PMA) nanomagnet, known for its superior stability and scalability compared to in-plane variants, VCMA switching in PMA system requires an in-plane symmetry breaking field, which limits its practicality for on-chip applications. We investigate field-free VCMA switching utilizing strain from a piezoelectric layer and an exchange bias from an antiferromagnetic material. Using macro-spin simulations based on the Landau-Lifshitz-Gilbert equation, we systematically analyze how the VCMA effect, strain-induced magnetoelastic effect, exchange bias, oxide and free layer thicknesses, and damping constant affect the switching performance of the device. The write error rate (WER) drops drastically from 0.2 (without stress) to <span>({10}^{-6})</span> (100 MPa stress), showcasing the effectiveness of our approach. We also find that the damping constant, especially in the 0.01–0.05 range, plays a crucial role in further optimizing the switching performance of the device. This study offers new insights for enhancing magnetic memory technology.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142844832","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-18DOI: 10.1007/s10948-024-06872-w
Doyel Rakshit, Ajay Kumar Ghosh
Superfluid phase stiffness (SPS) in the presence of two co-existing and mutually exclusive superconducting and magnetic ordering has been studied in (i) the pure EBCO and (ii) a composite system of nanoparticles of Sn and EBCO superconductors. SPS has been extracted in two different methods by using (i) nonlinear current–voltage (IV) characteristics and (ii) magnetization (M) as a function of the applied magnetic field (H). Variations of the SPS with temperature (T) are found to be different in transport and magnetic methods. A possible reason of the difference has been discussed. The nature of the variation of the SPS in the presence of nanoparticles of Sn has been explored in terms of the distribution of the bound vortex–anti-vortex pairs within the framework of the BKT transition.
{"title":"Low Temperature Variation of Superfluid Phase Stiffness in the Presence of Two Mutually Exclusive Orderings","authors":"Doyel Rakshit, Ajay Kumar Ghosh","doi":"10.1007/s10948-024-06872-w","DOIUrl":"10.1007/s10948-024-06872-w","url":null,"abstract":"<div><p>Superfluid phase stiffness (SPS) in the presence of two co-existing and mutually exclusive superconducting and magnetic ordering has been studied in (i) the pure EBCO and (ii) a composite system of nanoparticles of Sn and EBCO superconductors. SPS has been extracted in two different methods by using (i) nonlinear current–voltage (<i>IV</i>) characteristics and (ii) magnetization (<i>M</i>) as a function of the applied magnetic field (<i>H</i>). Variations of the SPS with temperature (<i>T</i>) are found to be different in transport and magnetic methods. A possible reason of the difference has been discussed. The nature of the variation of the SPS in the presence of nanoparticles of Sn has been explored in terms of the distribution of the bound vortex–anti-vortex pairs within the framework of the BKT transition.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142844927","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-17DOI: 10.1007/s10948-024-06857-9
Milad Arman, Farzad Shahri, Reza Gholamipour, Sajad Sohrabi
This work attempted to study the effects of the solidification behavior on the magnetic and magnetocaloric properties of stoichiometric Ni50Mn34In16 Heusler alloy. In this respect, the samples with two different diameters of 2 mm (D2 sample) and 8 mm (D8 sample) were prepared by suction casting technique. X-ray diffraction (XRD), field emission scanning electron microscopy (FE-SEM), and magnetic force microscopy (MFM) were employed to identify the structure, microstructure, and magnetic domain distribution of the samples. Also, phase transformation behavior was characterized using differential scanning calorimetry (DSC) across a temperature range of 200–350 K. Thermo-magnetic properties of samples were evaluated using SQUID Quantum Design MPMS®3 during heating and cooling at the temperature range of 175–350 K at the constant magnetic field of 2 T. Moreover, the magnetic and magnetocaloric properties of the samples were analyzed using the cryostat-equipped VSM around the magnetic phase transition temperature under a magnetic field up to 1.75 T. Based on the results obtained, it is shown that an increase in the sample diameter leads to an increase in the Curie temperature. Furthermore, it was concluded that the magnetocaloric properties such as magnetic entropy change ((Delta {S}_{text{M}})), adiabatic temperature change ((Delta {T}_{text{ad}})), and refrigerant capacity ((RC)) parameters improved with an increase in the sample diameter through the microstructural refinement and enhancing the atomic ordering. Specifically, the maximum values of the (Delta {S}_{text{M}}), (RC), and (Delta {T}_{text{ad}}) for the D8 sample are estimated to be 3.04 J/kg K, 109.83 J/kg, and 0.94 K, respectively.
{"title":"Effect of the Solidification Rate on the Magnetic and Magnetocaloric Properties of NiMnIn Heusler Alloy: Second-Order Magnetic Transition","authors":"Milad Arman, Farzad Shahri, Reza Gholamipour, Sajad Sohrabi","doi":"10.1007/s10948-024-06857-9","DOIUrl":"10.1007/s10948-024-06857-9","url":null,"abstract":"<div><p>This work attempted to study the effects of the solidification behavior on the magnetic and magnetocaloric properties of stoichiometric Ni<sub>50</sub>Mn<sub>34</sub>In<sub>16</sub> Heusler alloy. In this respect, the samples with two different diameters of 2 mm (D2 sample) and 8 mm (D8 sample) were prepared by suction casting technique. X-ray diffraction (XRD), field emission scanning electron microscopy (FE-SEM), and magnetic force microscopy (MFM) were employed to identify the structure, microstructure, and magnetic domain distribution of the samples. Also, phase transformation behavior was characterized using differential scanning calorimetry (DSC) across a temperature range of 200–350 K. Thermo-magnetic properties of samples were evaluated using SQUID Quantum Design MPMS®3 during heating and cooling at the temperature range of 175–350 K at the constant magnetic field of 2 T. Moreover, the magnetic and magnetocaloric properties of the samples were analyzed using the cryostat-equipped VSM around the magnetic phase transition temperature under a magnetic field up to 1.75 T. Based on the results obtained, it is shown that an increase in the sample diameter leads to an increase in the Curie temperature. Furthermore, it was concluded that the magnetocaloric properties such as magnetic entropy change (<span>(Delta {S}_{text{M}})</span>), adiabatic temperature change (<span>(Delta {T}_{text{ad}})</span>), and refrigerant capacity (<span>(RC)</span>) parameters improved with an increase in the sample diameter through the microstructural refinement and enhancing the atomic ordering. Specifically, the maximum values of the <span>(Delta {S}_{text{M}})</span>, <span>(RC)</span>, and <span>(Delta {T}_{text{ad}})</span> for the D8 sample are estimated to be 3.04 J/kg K, 109.83 J/kg, and 0.94 K, respectively.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142845092","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-17DOI: 10.1007/s10948-024-06870-y
Satya Narayana Murthy V
Underwater wireless communication is an exciting and demanding technology, where communication for longer distances with less noise is essential. The widely used underwater communications, such as communication by acoustic waves, and terrestrial waves, such as optical and radiofrequency waves, have limitations. Communication by magnetic induction appears to be an alternative technique, which needs an improvement in long-distance communication. Storing the data digitally and sending the higher current pulses to the transmitter coil will generate stronger magnetic pulses. The digital magnetic pulses can transfer the data to longer distances, increasing the transfer rate.
{"title":"A New Methodology for the Development of Underwater Magnetic Pulse Wireless Communication","authors":"Satya Narayana Murthy V","doi":"10.1007/s10948-024-06870-y","DOIUrl":"10.1007/s10948-024-06870-y","url":null,"abstract":"<div><p>Underwater wireless communication is an exciting and demanding technology, where communication for longer distances with less noise is essential. The widely used underwater communications, such as communication by acoustic waves, and terrestrial waves, such as optical and radiofrequency waves, have limitations. Communication by magnetic induction appears to be an alternative technique, which needs an improvement in long-distance communication. Storing the data digitally and sending the higher current pulses to the transmitter coil will generate stronger magnetic pulses. The digital magnetic pulses can transfer the data to longer distances, increasing the transfer rate.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142826124","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-17DOI: 10.1007/s10948-024-06853-z
A. Jabar, S. Idrissi, L. Bahmad
This paper studies the nano-diamond structure, commonly known as the ultra-dispersed diamond (UDD) structure. This diamond-decorated system is formed with the mixed spins S = 2 and σ = 3/2. This study uses the Monte Carlo simulations (MCS) under the Metropolis algorithm. We envisaged both the first nearest-neighbor interactions and the second nearest-neighbor interactions. For simplicity, we used the reduced crystal and external magnetic field. When fixing the other physical parameters, we inspected the temperature effect on the phase diagrams of the studied system. Also, we illustrated the thermal behavior of the magnetic entropy changes of the studied system for several reduced external magnetic field values. In addition, we presented the relative cooling power (RCP) as a function of the reduced external magnetic field of the (UDD) system. The effect of the reduced crystal field on the magnetizations of the diamond-decorated system has been investigated. To complete this study, we presented and discussed the magnetic hysteresis cycle of the studied diamond-decorated system.
本文研究了纳米金刚石的结构,俗称超分散金刚石(UDD)结构。该菱形装饰体系由S = 2和σ = 3/2混合自旋形成。本研究采用Metropolis算法下的蒙特卡洛模拟(Monte Carlo simulations, MCS)。我们设想了第一个最近邻相互作用和第二个最近邻相互作用。为简单起见,我们使用了简化后的晶体和外加磁场。在确定其他物理参数时,考察了温度对所研究体系相图的影响。此外,我们还说明了在几个减小的外磁场值下,所研究系统的磁熵变化的热行为。此外,我们给出了相对冷却功率(RCP)作为(UDD)系统减少的外部磁场的函数。研究了还原晶体场对金刚石装饰体系磁化性能的影响。为了完成这项研究,我们提出并讨论了所研究的钻石装饰系统的磁滞循环。
{"title":"Physical Impacts of Magnetic Impurities in a Diamond-decorated System by Monte Carlo Simulations","authors":"A. Jabar, S. Idrissi, L. Bahmad","doi":"10.1007/s10948-024-06853-z","DOIUrl":"10.1007/s10948-024-06853-z","url":null,"abstract":"<div><p>This paper studies the nano-diamond structure, commonly known as the ultra-dispersed diamond (UDD) structure. This diamond-decorated system is formed with the mixed spins S = 2 and σ = 3/2. This study uses the Monte Carlo simulations (MCS) under the Metropolis algorithm. We envisaged both the first nearest-neighbor interactions and the second nearest-neighbor interactions. For simplicity, we used the reduced crystal and external magnetic field. When fixing the other physical parameters, we inspected the temperature effect on the phase diagrams of the studied system. Also, we illustrated the thermal behavior of the magnetic entropy changes of the studied system for several reduced external magnetic field values. In addition, we presented the relative cooling power (RCP) as a function of the reduced external magnetic field of the (UDD) system. The effect of the reduced crystal field on the magnetizations of the diamond-decorated system has been investigated. To complete this study, we presented and discussed the magnetic hysteresis cycle of the studied diamond-decorated system.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142844911","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-12-17DOI: 10.1007/s10948-024-06880-w
Akshaya A., Shailesh Kalal, K. Saravanan, Sunil Ojha, Jochen Stahn, Mukul Gupta
Tetra metal nitrides (M4N; M = Cr, Fe, Co, Mn, Ni) are a promising spintronic material with an anti-perovskite structure and fascinating magnetic characteristics due to a magneto-volume effect. Though a fully stochiometric Mn4N or Fe4N has been achieved, the lattice parameter (LP) of Co4N was always been found to be significantly lower than the anticipated theoretical values, indicating a sub-stochiometric Co4N phase. The formation enthalpy of Co4N is slightly positive resulting in unfavorable thermodynamical conditions and significant out-diffusion of N from Co4N. In this work, we present a comparative study of undoped and Pd-doped Co4N thin films synthesized using a reactive nitrogen sputtering. The structural, composition, and magnetic properties have been studied by combining x-ray diffraction, Rutherford backscattering, energy-dispersive x-ray spectroscopy, secondary ion mass spectroscopy, vibrating sample magnetometer, magneto-optical Kerr effect, and polarized neutron reflectivity measurements. It was found that Pd doping of about 5 at.% results in a significant enhancement in the LP of Co4N signifying a higher amount of N retention without adversely affecting the growth and magnetic properties. It is further suggested that the amount of Pd doping may further be increased to realize a fully stoichiometric Co4N.
{"title":"Study of Structural and Magnetic Properties of Pd-Doped Co4N Thin Films","authors":"Akshaya A., Shailesh Kalal, K. Saravanan, Sunil Ojha, Jochen Stahn, Mukul Gupta","doi":"10.1007/s10948-024-06880-w","DOIUrl":"10.1007/s10948-024-06880-w","url":null,"abstract":"<div><p>Tetra metal nitrides (M<sub>4</sub>N; M = Cr, Fe, Co, Mn, Ni) are a promising spintronic material with an anti-perovskite structure and fascinating magnetic characteristics due to a magneto-volume effect. Though a fully stochiometric Mn<sub>4</sub>N or Fe<sub>4</sub>N has been achieved, the lattice parameter (LP) of Co<sub>4</sub>N was always been found to be significantly lower than the anticipated theoretical values, indicating a sub-stochiometric Co<sub>4</sub>N phase. The formation enthalpy of Co<sub>4</sub>N is slightly positive resulting in unfavorable thermodynamical conditions and significant out-diffusion of N from Co<sub>4</sub>N. In this work, we present a comparative study of undoped and Pd-doped Co<sub>4</sub>N thin films synthesized using a reactive nitrogen sputtering. The structural, composition, and magnetic properties have been studied by combining x-ray diffraction, Rutherford backscattering, energy-dispersive x-ray spectroscopy, secondary ion mass spectroscopy, vibrating sample magnetometer, magneto-optical Kerr effect, and polarized neutron reflectivity measurements. It was found that Pd doping of about 5 at.% results in a significant enhancement in the LP of Co<sub>4</sub>N signifying a higher amount of N retention without adversely affecting the growth and magnetic properties. It is further suggested that the amount of Pd doping may further be increased to realize a fully stoichiometric Co<sub>4</sub>N.</p></div>","PeriodicalId":669,"journal":{"name":"Journal of Superconductivity and Novel Magnetism","volume":"38 1","pages":""},"PeriodicalIF":1.6,"publicationDate":"2024-12-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142826122","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}