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Magnetism and Critical Behavior of the Fullerene C18 Studied by Monte Carlo simulations 用蒙特卡罗模拟研究富勒烯C18的磁性和临界行为
IF 1.6 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-12-21 DOI: 10.1007/s10948-024-06838-y
S. Idrissi, A. Jabar, L. Bahmad

The Fullerene C18 is one of the most active types of nanostructures used as an active ingredient in several applications. This study used Monte Carlo simulations to investigate the magnetic properties of mixed 3/2 and 2 in the fullerene C18 systems. We first perform a theoretical analysis of the ground state phase diagrams. Indeed, we only present and analyze more stable configurations among all possible configurations. Second, calculations were performed to determine how the compound's magnetic properties changed when various physical parameters were altered. In addition, we provide studies of the magnetic behavior of the system at reduced temperature, reduced crystal fields, reduced exchange coupling interactions, and reduced external magnetic fields. Finally, we study and discuss the critical lowering temperature of fullerene C18. To conclude this study, we examined the different hysteresis loops when varying the values of the different physical parameters.

富勒烯 C18 是最活跃的纳米结构类型之一,在多种应用中用作活性成分。本研究使用蒙特卡罗模拟来研究富勒烯 C18 系统中混合 3/2 和 2 的磁性。我们首先对基态相图进行了理论分析。事实上,我们只提出并分析了所有可能构型中较为稳定的构型。其次,我们进行了计算,以确定当各种物理参数发生变化时,化合物的磁性如何变化。此外,我们还研究了该体系在温度降低、晶体场降低、交换耦合相互作用降低和外部磁场降低时的磁性行为。最后,我们研究并讨论了富勒烯 C18 的临界降低温度。最后,我们研究并讨论了富勒烯 C18 的临界降低温度。在本研究的最后,我们研究了改变不同物理参数值时的不同磁滞环。
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引用次数: 0
Detailed Analysis of the Superconducting Gap with Dynes Pair-Breaking Scattering 超导间隙与Dynes破对散射的详细分析
IF 1.6 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-12-20 DOI: 10.1007/s10948-024-06844-0
Anastasiya Lebedeva, František Herman

We study the energy gap within the Dynes superconductor theory. This model generalizes the Bardeen-Cooper-Schrieffer (BCS) approach by including the pair-breaking scattering, introducing the tunneling in-gap states up to a Fermi level. We analytically solve the energy gap equation in various limit cases. The solution provides simple tools for further studies, compared to more complex numerics, and highlights the basic characteristics of the theory. First, in the critical limit of pair-breaking scattering, we derive an analytical form of zero-temperature gap to transition temperature ratio. Next, we derive the dependence of the energy gap close to critical temperature and look at its behavior for general and critical pair-breaking scattering rate. Furthermore, we compare our result with the numerical solution of the gap equation assuming general temperature. We show the range of temperatures, for which the analytical approximation is valid. In the end, we provide the approximative formula of the gap, assuming general pair-breaking scattering, emphasizing its exact behavior close to transition temperature.

我们研究了戴纳斯超导体理论中的能隙。该模型将巴丁-库珀-施里弗(BCS)方法概括为包括对破散射,引入了费米级以下的隧穿隙内态。我们对各种极限情况下的能隙方程进行了分析求解。与更复杂的数值计算相比,这种解法为进一步研究提供了简单的工具,并突出了该理论的基本特征。首先,在对破散射的临界极限中,我们导出了零温能隙与转变温度比的解析形式。接下来,我们推导了接近临界温度时的能隙依赖性,并研究了它在一般和临界对破散射率下的行为。此外,我们还将我们的结果与假设一般温度下的能隙方程数值解进行了比较。我们展示了分析近似有效的温度范围。最后,我们提供了假定一般对破散射的间隙近似公式,强调了其接近过渡温度的精确行为。
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引用次数: 0
On the Lineshapes of Temperature-Dependent Transport Measurements of Superconductors Under Pressure 论压力下超导体随温度变化的传输测量线形
IF 1.6 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-12-19 DOI: 10.1007/s10948-024-06879-3
Alexander C. Mark, Russell J. Hemley

Recent reports of superconductivity in the vicinity of room temperature have been the subject of discussion by the community. Specifically, features in the resistance-temperature (R-T) relations have raised questions. We show that many of these features can arise from previously unaccounted-for dynamic effects associated with the AC transport techniques often used in high-pressure experiments. These dynamic AC effects can cause the apparent resistance (( R_{apparent} )) to diverge from the DC resistance (( R_{DC} )), sharpen measured superconducting transitions, and produce other features in the measured R-T response. We also show that utilizing the full output of phase-sensitive transport measurements provides a valuable probe of superconducting samples in difficult-to-measure systems.

最近关于室温附近超导性的报道一直是科学界讨论的主题。具体来说,电阻-温度(R-T)关系的特征提出了问题。我们表明,许多这些特征可能源于以前未解释的与高压实验中经常使用的交流输运技术相关的动态效应。这些动态交流效应可能导致表观电阻(( R_{apparent} ))偏离直流电阻(( R_{DC} )),使测量到的超导跃迁变得尖锐,并在测量到的R-T响应中产生其他特征。我们还表明,利用相敏输运测量的全部输出,在难以测量的系统中为超导样品提供了有价值的探针。
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引用次数: 0
Effect of Phase Transition Type on the Magnetocaloric Effect and Magnetic Hysteresis in Er(Co1-xMnx)2 Laves Alloys 相变类型对Er(Co1-xMnx)2合金磁热效应和磁滞的影响
IF 1.6 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-12-18 DOI: 10.1007/s10948-024-06888-2
H. Y. Dai, Z. H. Zu, Y. K. Chu, R. J. Cui, Z. D. Han

As magnetic refrigerants, first-order transition (FOT) and second-order transition (SOT) materials possess distinct advantages and disadvantages. If the phase transition can be tuned to the critical point between FOT and SOT, it may be possible to combine the benefits of both, thereby achieving an outstanding magnetocaloric effect. Here, we demonstrated this approach through phase transition engineering in Er(Co1-xMnx)2 alloys. When x ≤ 0.06, the magnetic phase transition of the samples was FOT, exhibiting a significant magnetic entropy change. However, at x = 0.08, the samples underwent a SOT from ferromagnetic to paramagnetic, leading to a substantial reduction in the magnetocaloric effect. At the critical point of the FOT/SOT border with x = 0.06, the sample exhibited a large magnetic entropy change along with negligible magnetic hysteresis. This work demonstrates that the critical point between FOT and SOT is an effective means of achieving an excellent magnetocaloric effect.

作为磁性制冷剂,一阶过渡(FOT)和二阶过渡(SOT)材料各有优缺点。如果相变可以调整到FOT和SOT之间的临界点,就有可能将两者的优点结合起来,从而实现出色的磁热效应。在这里,我们通过Er(Co1-xMnx)2合金的相变工程证明了这种方法。当x≤0.06时,样品的磁相变为FOT,表现出明显的磁熵变化。然而,当x = 0.08时,样品经历了从铁磁性到顺磁性的SOT,导致磁热效应大幅降低。在FOT/SOT边界x = 0.06的临界点处,样品表现出较大的磁熵变化,磁滞可以忽略不计。这项工作表明,在FOT和SOT之间的临界点是实现优异磁热效应的有效手段。
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引用次数: 0
Strain and Exchange Bias-Enabled Field-Free Voltage-Controlled Magnetic Anisotropy Switching 应变和交换偏置使能无场电压控制磁各向异性开关
IF 1.6 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-12-18 DOI: 10.1007/s10948-024-06873-9
Pinkesh Kumar Mishra, Swapnil Bhuktare

In pursuing energy-efficient and high-performance nonvolatile magnetic memory devices, this study explores voltage-induced techniques, specifically voltage-controlled magnetic anisotropy (VCMA), as an alternative to current-induced methods, which suffer from Ohmic loss. The perpendicular magnetic anisotropy (PMA) nanomagnet, known for its superior stability and scalability compared to in-plane variants, VCMA switching in PMA system requires an in-plane symmetry breaking field, which limits its practicality for on-chip applications. We investigate field-free VCMA switching utilizing strain from a piezoelectric layer and an exchange bias from an antiferromagnetic material. Using macro-spin simulations based on the Landau-Lifshitz-Gilbert equation, we systematically analyze how the VCMA effect, strain-induced magnetoelastic effect, exchange bias, oxide and free layer thicknesses, and damping constant affect the switching performance of the device. The write error rate (WER) drops drastically from 0.2 (without stress) to ({10}^{-6}) (100 MPa stress), showcasing the effectiveness of our approach. We also find that the damping constant, especially in the 0.01–0.05 range, plays a crucial role in further optimizing the switching performance of the device. This study offers new insights for enhancing magnetic memory technology.

为了追求高能效和高性能的非易失性磁存储器件,本研究探索了电压感应技术,特别是电压控制磁各向异性(VCMA),作为电流感应方法的替代方法,因为电流感应方法存在欧姆损耗。垂直磁各向异性(PMA)纳米磁体以其优越的稳定性和可扩展性而闻名,但PMA系统中的VCMA开关需要一个面内对称破缺场,这限制了其在片上应用的实用性。我们利用压电层的应变和反铁磁材料的交换偏置来研究无场VCMA开关。采用基于Landau-Lifshitz-Gilbert方程的宏观自旋模拟,系统分析了VCMA效应、应变磁弹性效应、交换偏置、氧化层和自由层厚度以及阻尼常数对器件开关性能的影响。写入错误率(WER)从0.2(无压力)急剧下降到({10}^{-6}) (100 MPa压力),显示了我们的方法的有效性。我们还发现,阻尼常数,特别是在0.01-0.05范围内,对进一步优化器件的开关性能起着至关重要的作用。本研究为增强磁记忆技术提供了新的思路。
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引用次数: 0
Low Temperature Variation of Superfluid Phase Stiffness in the Presence of Two Mutually Exclusive Orderings 存在两种互斥排序时超流体相刚性的低温变化
IF 1.6 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-12-18 DOI: 10.1007/s10948-024-06872-w
Doyel Rakshit, Ajay Kumar Ghosh

Superfluid phase stiffness (SPS) in the presence of two co-existing and mutually exclusive superconducting and magnetic ordering has been studied in (i) the pure EBCO and (ii) a composite system of nanoparticles of Sn and EBCO superconductors. SPS has been extracted in two different methods by using (i) nonlinear current–voltage (IV) characteristics and (ii) magnetization (M) as a function of the applied magnetic field (H). Variations of the SPS with temperature (T) are found to be different in transport and magnetic methods. A possible reason of the difference has been discussed. The nature of the variation of the SPS in the presence of nanoparticles of Sn has been explored in terms of the distribution of the bound vortex–anti-vortex pairs within the framework of the BKT transition.

研究了 (i) 纯 EBCO 和 (ii) 锡和 EBCO 超导纳米粒子复合系统中存在两种共存且互斥的超导和磁有序情况下的超流体相刚度(SPS)。通过使用 (i) 非线性电流-电压 (IV) 特性和 (ii) 磁化 (M) 作为外加磁场 (H) 的函数,用两种不同的方法提取了 SPS。发现在传输和磁性方法中,SPS 随温度 (T) 的变化是不同的。我们讨论了造成这种差异的可能原因。根据 BKT 转变框架内束缚涡旋-反涡旋对的分布情况,探讨了存在纳米锡粒子时 SPS 变化的性质。
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引用次数: 0
Effect of the Solidification Rate on the Magnetic and Magnetocaloric Properties of NiMnIn Heusler Alloy: Second-Order Magnetic Transition 凝固速率对NiMnIn Heusler合金磁性和磁热性能的影响:二阶磁转变
IF 1.6 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-12-17 DOI: 10.1007/s10948-024-06857-9
Milad Arman, Farzad Shahri, Reza Gholamipour, Sajad Sohrabi

This work attempted to study the effects of the solidification behavior on the magnetic and magnetocaloric properties of stoichiometric Ni50Mn34In16 Heusler alloy. In this respect, the samples with two different diameters of 2 mm (D2 sample) and 8 mm (D8 sample) were prepared by suction casting technique. X-ray diffraction (XRD), field emission scanning electron microscopy (FE-SEM), and magnetic force microscopy (MFM) were employed to identify the structure, microstructure, and magnetic domain distribution of the samples. Also, phase transformation behavior was characterized using differential scanning calorimetry (DSC) across a temperature range of 200–350 K. Thermo-magnetic properties of samples were evaluated using SQUID Quantum Design MPMS®3 during heating and cooling at the temperature range of 175–350 K at the constant magnetic field of 2 T. Moreover, the magnetic and magnetocaloric properties of the samples were analyzed using the cryostat-equipped VSM around the magnetic phase transition temperature under a magnetic field up to 1.75 T. Based on the results obtained, it is shown that an increase in the sample diameter leads to an increase in the Curie temperature. Furthermore, it was concluded that the magnetocaloric properties such as magnetic entropy change ((Delta {S}_{text{M}})), adiabatic temperature change ((Delta {T}_{text{ad}})), and refrigerant capacity ((RC)) parameters improved with an increase in the sample diameter through the microstructural refinement and enhancing the atomic ordering. Specifically, the maximum values of the (Delta {S}_{text{M}}), (RC), and (Delta {T}_{text{ad}}) for the D8 sample are estimated to be 3.04 J/kg K, 109.83 J/kg, and 0.94 K, respectively.

本工作试图研究凝固行为对Ni50Mn34In16 Heusler合金磁性和磁热性能的影响。为此,采用吸铸技术制备了2 mm (D2样品)和8 mm (D8样品)两种不同直径的样品。采用x射线衍射(XRD)、场发射扫描电镜(FE-SEM)和磁力显微镜(MFM)对样品的结构、微观结构和磁畴分布进行了表征。此外,用差示扫描量热法(DSC)在200-350 K的温度范围内表征了相变行为。利用SQUID Quantum Design MPMS®3在175-350 K的恒定磁场2 t下加热和冷却样品的热磁性能,并在1.75 t的磁场下,使用配备低温恒温器的VSM分析样品在磁相变温度附近的磁性和磁热性。结果表明,试样直径的增大会导致居里温度的升高。结果表明,随着样品直径的增大,材料的磁熵变化((Delta {S}_{text{M}}))、绝热温度变化((Delta {T}_{text{ad}}))和制冷剂容量((RC))等磁热性能均得到改善。具体来说,D8样品的(Delta {S}_{text{M}})、(RC)和(Delta {T}_{text{ad}})的最大值估计分别为3.04 J/kg K、109.83 J/kg和0.94 K。
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引用次数: 0
A New Methodology for the Development of Underwater Magnetic Pulse Wireless Communication 开发水下磁脉冲无线通信的新方法
IF 1.6 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-12-17 DOI: 10.1007/s10948-024-06870-y
Satya Narayana Murthy V

Underwater wireless communication is an exciting and demanding technology, where communication for longer distances with less noise is essential. The widely used underwater communications, such as communication by acoustic waves, and terrestrial waves, such as optical and radiofrequency waves, have limitations. Communication by magnetic induction appears to be an alternative technique, which needs an improvement in long-distance communication. Storing the data digitally and sending the higher current pulses to the transmitter coil will generate stronger magnetic pulses. The digital magnetic pulses can transfer the data to longer distances, increasing the transfer rate.

水下无线通信是一项令人兴奋且要求极高的技术,在这种技术中,必须以较小的噪音进行较远距离的通信。目前广泛使用的水下通信(如声波通信)和地面通信(如光波和射频波)都有其局限性。磁感应通信似乎是一种替代技术,但在长距离通信方面需要改进。以数字方式存储数据并向发射线圈发送较大的电流脉冲,将产生较强的磁脉冲。数字磁脉冲可以将数据传输到更远的距离,从而提高传输速率。
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引用次数: 0
Physical Impacts of Magnetic Impurities in a Diamond-decorated System by Monte Carlo Simulations 磁性杂质在钻石装饰系统中的物理影响的蒙特卡罗模拟
IF 1.6 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-12-17 DOI: 10.1007/s10948-024-06853-z
A. Jabar, S. Idrissi, L. Bahmad

This paper studies the nano-diamond structure, commonly known as the ultra-dispersed diamond (UDD) structure. This diamond-decorated system is formed with the mixed spins S = 2 and σ = 3/2. This study uses the Monte Carlo simulations (MCS) under the Metropolis algorithm. We envisaged both the first nearest-neighbor interactions and the second nearest-neighbor interactions. For simplicity, we used the reduced crystal and external magnetic field. When fixing the other physical parameters, we inspected the temperature effect on the phase diagrams of the studied system. Also, we illustrated the thermal behavior of the magnetic entropy changes of the studied system for several reduced external magnetic field values. In addition, we presented the relative cooling power (RCP) as a function of the reduced external magnetic field of the (UDD) system. The effect of the reduced crystal field on the magnetizations of the diamond-decorated system has been investigated. To complete this study, we presented and discussed the magnetic hysteresis cycle of the studied diamond-decorated system.

本文研究了纳米金刚石的结构,俗称超分散金刚石(UDD)结构。该菱形装饰体系由S = 2和σ = 3/2混合自旋形成。本研究采用Metropolis算法下的蒙特卡洛模拟(Monte Carlo simulations, MCS)。我们设想了第一个最近邻相互作用和第二个最近邻相互作用。为简单起见,我们使用了简化后的晶体和外加磁场。在确定其他物理参数时,考察了温度对所研究体系相图的影响。此外,我们还说明了在几个减小的外磁场值下,所研究系统的磁熵变化的热行为。此外,我们给出了相对冷却功率(RCP)作为(UDD)系统减少的外部磁场的函数。研究了还原晶体场对金刚石装饰体系磁化性能的影响。为了完成这项研究,我们提出并讨论了所研究的钻石装饰系统的磁滞循环。
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引用次数: 0
Study of Structural and Magnetic Properties of Pd-Doped Co4N Thin Films 掺钯Co4N薄膜的结构和磁性能研究
IF 1.6 4区 物理与天体物理 Q3 PHYSICS, APPLIED Pub Date : 2024-12-17 DOI: 10.1007/s10948-024-06880-w
Akshaya A., Shailesh Kalal, K. Saravanan, Sunil Ojha, Jochen Stahn, Mukul Gupta

Tetra metal nitrides (M4N; M = Cr, Fe, Co, Mn, Ni) are a promising spintronic material with an anti-perovskite structure and fascinating magnetic characteristics due to a magneto-volume effect. Though a fully stochiometric Mn4N or Fe4N has been achieved, the lattice parameter (LP) of Co4N was always been found to be significantly lower than the anticipated theoretical values, indicating a sub-stochiometric Co4N phase. The formation enthalpy of Co4N is slightly positive resulting in unfavorable thermodynamical conditions and significant out-diffusion of N from Co4N. In this work, we present a comparative study of undoped and Pd-doped Co4N thin films synthesized using a reactive nitrogen sputtering. The structural, composition, and magnetic properties have been studied by combining x-ray diffraction, Rutherford backscattering, energy-dispersive x-ray spectroscopy, secondary ion mass spectroscopy, vibrating sample magnetometer, magneto-optical Kerr effect, and polarized neutron reflectivity measurements. It was found that Pd doping of about 5 at.% results in a significant enhancement in the LP of Co4N signifying a higher amount of N retention without adversely affecting the growth and magnetic properties. It is further suggested that the amount of Pd doping may further be increased to realize a fully stoichiometric Co4N.

四金属氮化物(M4N;M = Cr, Fe, Co, Mn, Ni)是一种很有前途的自旋电子材料,具有反钙钛矿结构和由于磁体积效应而具有迷人的磁性。虽然已经获得了完全化学计量的Mn4N或Fe4N,但Co4N的晶格参数(LP)总是被发现明显低于预期的理论值,表明Co4N是一个亚化学计量的相。Co4N的生成焓略为正,导致了不利的热力学条件和N从Co4N向外扩散。在这项工作中,我们提出了用反应氮溅射合成未掺杂和掺pd的Co4N薄膜的比较研究。结合x射线衍射、卢瑟福后向散射、能量色散x射线光谱学、二次离子质谱学、振动样品磁强计、磁光克尔效应和偏振中子反射率测量,研究了其结构、组成和磁性能。结果表明,Pd掺杂量约为5at。%导致Co4N的LP显著增强,这表明在不影响生长和磁性能的情况下,N的保留量更高。进一步表明,可以进一步增加钯的掺杂量,以实现完全化学计量的Co4N。
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引用次数: 0
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Journal of Superconductivity and Novel Magnetism
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