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Sub-100 fs Kerr-lens Mode-locked femtosecond Yb:CaYAlO4 Laser at GHz repetition rate 100秒以下的克尔透镜锁模飞秒Yb:CaYAlO4激光器,重复频率为GHz
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20222297
Zheng Li, Tian Wenlong, Ma Junyi, Yu Yang, Xu Xiao-Dong, Han Hainian, Wei Zhiyi, Zhu Jiangfeng
Femtosecond lasers with GHz repetition rate play an important role in scientific and industrial applications, such as spectroscopy, optical frequency combs and GHz-Burst pulse trains for micro-machining in the ablation-cooled regime. Kerr-lens Mode-locked (KLM) technique and passively modelocking based on Semiconductor Saturable Absorber Mirror (SESAM) are the primary methods to generate GHz femtosecond all-solid-state lasers (ASSLs). Kerr-lens mode-locked Ti:Sapphire lasers have made a significant progress benefitting from the high-power green pump lasers, repetition rate up to 10 GHz has been obtained with an average power of 1.2 W. In the early 21st century, ytterbium ion (Yb3+) doped laser crystals and ceramics with emission wavelengths near 1 μm gained attention due to their high conversion efficiency and broad gain-bandwidth. Combining with the customized SESAM and high-power multimode fiber-coupled laser diodes (LD), GHz Yb-doped ASSLs with watt-level average power may be easily attained and have made rapid progress. However, GHz KLM lasers have strict requirements for the cavity design and pump sources. For satisfying mode matching and enhancing the soft aperture effect within the gain medium, a high-brightness pump source with excellent beam quality (M2~1) is desired, such as the single-mode fiber coupled LD, however, the maximum pump power of which is only~1 W. As a result, the average power of GHz KLM femtosecond lasers is typically restricted to few tens of milliwatts, which limits the further applications. In this work, we reported the first GHz high-power KLM Yb:CaYAlO4 laser by using a high-power single-mode fiber laser instead of the low-power single-mode fiber coupled LDs as the pump source. On the basis of ABCD matrices, a simple four-mirror bow-tie ring cavity was built such that the laser mode can match well with the focused pump spot in the crystal. At the pump power of 8 W, stable unidirectional KLM was achieved, the laser had an average power of 2.1 W with a pulse duration of 88 fs and a repetition rate of 1.8 GHz, corresponding to a peak power of 11.57 kW. The high peak power and extremely short pulse duration are crucial for coherent octave-spanning supercontinuum generation. The powerful GHz KLM laser with sub-100 fs pulse duration provides an attractive source for optical frequency combs and micro-machining applications.
重复频率为GHz的飞秒激光器在科学和工业应用中发挥着重要作用,如光谱学、光学频率梳和用于烧蚀冷却条件下微加工的GHz脉冲串。克尔透镜锁模技术(KLM)和基于半导体可饱和吸收镜(SESAM)的被动锁模技术是产生GHz飞秒全固态激光器(ASSLs)的主要方法。克尔透镜锁模Ti:蓝宝石激光器得益于高功率绿色泵浦激光器取得了重大进展,重复频率高达10 GHz,平均功率为1.2 W。21世纪初,发射波长接近1 μm的掺镱激光晶体和陶瓷因其高转换效率和宽增益带宽而备受关注。结合定制化SESAM和大功率多模光纤耦合激光二极管(LD),可以很容易地获得平均功率为瓦级的GHz掺镱assl,并取得了快速进展。然而,GHz KLM激光器对腔体设计和泵浦源有严格的要求。为了满足模式匹配和增强增益介质内的软孔径效应,需要具有优良光束质量(M2~1)的高亮度泵浦源,如单模光纤耦合LD,但其最大泵浦功率仅为~1 W。因此,GHz KLM飞秒激光器的平均功率通常限制在几十毫瓦,这限制了进一步的应用。本文报道了用高功率单模光纤激光器代替低功率单模光纤耦合ld作为泵浦源的首个GHz高功率KLM Yb:CaYAlO4激光器。在ABCD矩阵的基础上,建立了一个简单的四镜领结环腔,使激光模式与晶体中的聚焦泵浦光斑匹配良好。当泵浦功率为8 W时,实现了稳定的单向KLM,激光平均功率为2.1 W,脉冲持续时间为88 fs,重复频率为1.8 GHz,峰值功率为11.57 kW。高峰值功率和极短脉冲持续时间是产生相干跨八度超连续谱的关键。强大的GHz KLM激光器,脉冲持续时间低于100 fs,为光学频率梳和微加工应用提供了有吸引力的光源。
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引用次数: 0
Lattice Boltzmann simulation and analysis of two-dimensional trapezoidal cavity flow based on GPU 基于GPU的二维梯形空腔流动晶格玻尔兹曼模拟与分析
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230430
Chen Bai-Hui, Shi Bao-Chang, Wang Lei, Chai Zhen-Hua
In this study, we utilize the lattice Boltzmann method to investigate the flow behavior in a two-dimensional trapezoidal cavity, which is under two-sided driving on the upper and lower walls. Our calculations have been accelerated through GPU-CUDA software. We have conducted an analysis of the flow field mode using proper orthogonal decomposition. The effects of various parameters such as Reynolds number (Re) and driving direction on the flow characteristics are examined through numerical simulations. The results show that:(1) for the upper wall drive (T1a), the flow field remains stable within the range of Re from 1000 to 8000. However, when Re=8500, the flow field becomes periodic yet unstable. The velocity phase diagram at the monitoring point is a smooth circle, and the energy of the first two modes has dominated the energy of the whole field. Once Re exceeds 10000, the velocity phase diagram turns irregular and the flow field becomes aperiodic and unsteady. (2) As for the lower wall drive (T1b), the flow is stable within Re 1000-8000, yet when Re=11500, the flow field becomes periodic yet unsteady. The energy of the first three modes appears relatively large. When Re is greater than 12500, the flow field becomes aperiodic and unsteady. At this time, the phase diagram exhibits a smooth circle, with the energy of the first two modes almost entirely dominating the entire energy. (3) For the case of upper and lower walls moving in the same direction with the same speed (T2a), the flow field remains stable when Re changes from 1000 to 10000. When Re is between 12500 to 15000, the flow becomes periodic yet unstable. The velocity phase diagram continues to be a smooth circle, with the first two modes still occupying a large portion of the energy. Once Re surpasses 20000, the energy proportion of the first three modes significantly decreases, and the flow becomes aperiodic and unsteady. (4) For the case in which the upper and lower walls are driven in opposite directions with the same velocity (T2b), the flow field remains stable within Re changes from 1000 to 5000. When Re=6000, the energy of the first mode accounts for 86%, and the flow field becomes periodic yet unstable. When Re surpasses 8000, the energy proportion of the first three modes decreases significantly, and the flow field becomes aperiodic and unsteady.
本文利用晶格玻尔兹曼方法研究了上下壁面双向驱动下二维梯形腔内的流动行为。我们的计算已经通过GPU-CUDA软件加速。我们用适当的正交分解法对流场模式进行了分析。通过数值模拟研究了雷诺数、驱动方向等参数对流动特性的影响。结果表明:(1)对于上壁面传动(T1a),流场在Re为1000 ~ 8000的范围内保持稳定;而当Re=8500时,流场变得周期性但不稳定。测点处的速度相图呈光滑圆形,前两种模式的能量占整个场能量的主导地位。当Re超过10000时,速度相图变得不规则,流场变得非周期性和非定常。(2)下壁面传动(T1b)在Re 1000 ~ 8000范围内流动稳定,而当Re=11500时,流场变得周期性但不稳定。前三种模态的能量显得比较大。当Re大于12500时,流场变得非周期性和非定常。此时,相图呈现出一个光滑的圆,前两个模态的能量几乎完全支配了整个能量。(3)上下壁面以相同速度同向运动(T2a)时,Re从1000变化到10000时,流场保持稳定。当Re在12500 ~ 15000之间时,流变得周期性但不稳定。速度相图仍然是一个光滑的圆,前两个模态仍然占据很大一部分能量。一旦Re超过20000,前三阶模态的能量占比显著降低,流动变得非周期性和非定常。(4)上下壁面以相同速度反向驱动(T2b)时,流场在Re从1000到5000的变化范围内保持稳定。当Re=6000时,第一模态能量占86%,流场变得周期性但不稳定。当Re超过8000时,前三阶模态的能量比例显著降低,流场变得非周期性和非定常。
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引用次数: 0
Quantitative study on isotope effect of rubidium clusters 铷团簇同位素效应的定量研究
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230778
Di Shu-Hong, Zhang Yang, Yang Hui-Jing, Cui Nai-Zhong, Li Yan-Kun, Liu Hui-Yuan, Li Ling-Li, Shi Feng-Liang, Jia Yu-Xuan
Because of the difficulty in measuring the cluster isotope displacement and identifying its causes, the resonance dissociation spectra, the moment shift and Zeeman energy shift of isotope cluster 87,85Rbn(n=1,2, 3,..., 13) are obtained by the combination of optical magnetic resonance and thermal dissociation techniques in this study. The quantitative calculation is carried out based on the conceptual model of the giant atom, and the results are in strict agreement with the measured results, which shows that rubidium clusters can be analyzed as giant-like atoms. Furthermore, 5s electron shell level structure of the rubidium cluster 87,85Rbn(n=1,2, 3,..., 92) is calculated using Zeeman level interval model. It is found that the main order and step distance of the 5s electron shell structure are similar to those of 3s single electron shell structure of sodium cluster in spherical symmetric. It is confirmed that the structure of the 5s electron shell of the rubidium cluster is determined by the largest energy gap of total Zeeman levels and the characteristic peaks of odd and even alternating and anomalous magnetic moments of special numbers such as n=2 are caused by the intrinsic properties of electrons and molecular structures. It is also found that 87Rbn and 85Rbn level shell structure is strictly consistent with the ratio of 3/2 magnitude relationship, and there are abnormal differences in spectral center frequency and broadening, which may be directly related to the 85,87Rb nuclide on the closed surface of the core-shell.
由于团簇同位素位移的测量和原因难以确定,同位素团簇87,85rbn (n= 1,2,3,…)的共振解离谱、矩移和塞曼能量移, 13)是本研究结合光磁共振和热解离技术得到的。根据巨原子概念模型进行了定量计算,结果与实测结果吻合较好,表明铷团簇可以作为类巨原子来分析。此外,铷原子团簇87,85rbn (n= 1,2,3,…)的5s电子壳层结构, 92),采用Zeeman水平区间模型计算。发现在球对称情况下,钠团簇的5s电子壳层结构的主序和阶距与3s单电子壳层结构相似。证实了铷原子团簇的5s电子壳层结构是由总塞曼能级的最大能隙决定的,而n=2等特殊数的奇偶交变磁矩和异常磁矩的特征峰是由电子和分子结构的固有性质引起的。还发现87Rbn和85Rbn能级壳层结构严格符合3/2量级的比值关系,且谱中心频率和展宽存在异常差异,这可能与核壳层封闭表面上的85、87Rb核素有直接关系。
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引用次数: 0
Brownian dynamics simulation of electrical properties of KcsA potassium ion channel KcsA钾离子通道电性能的布朗动力学模拟
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230118
Gao Ming-Zhu, Liu Chun-Liang, Wang Hong-Guang, Li Yong-Dong, Lin Shu, Zhai Yong-Gui
As a regulator of cation activity in living cells, KcsA (K+ Conduction and Selectivity Architecture) potassium channel plays an important role in the depolarization and repolarization of nerve cell action potential. In this paper, Brownian Dynamics (BD) method is used to simulate the electrical characteristics of the actual KcsA potassium channel systematically. The PMF of ions in the channel under electrostatic field, the current-voltage characteristic curve of symmetric solution and asymmetric solution, the ion concentration distribution curve in the axial direction of the channel, and the conduction-concentration curve are obtained. The results showed that the SF region of KcsA potassium ion channel blocked the passage of Cl- basically, showing a special selection characteristic of the passage of K+; Its current-voltage curve basically presents a linear distribution, and the conductivity-concentration curve presents a trend of first increasing and then flattening. The basic law is consistent with the experimental phenomenon. In addition, the influence of the specific intensity THz field on the channel K+ current is also simulated and analyzed. Compared with the electrostatic field of the same amplitude, the selected 0.6/1.2/5THz terahertz field can reduce the PMF by affecting the interaction potential energy between ion pairs, thereby increasing the K+ current. The research in this paper not only deepens the understanding of the regularity of KcsA potassium ion channels, but also provides a new idea for the study of other types of ion channels and the influence of terahertz field on the characteristics of ion channels.
KcsA (K+ Conduction and Selectivity Architecture)钾离子通道作为活细胞中阳离子活性的调节剂,在神经细胞动作电位的去极化和复极化过程中起着重要作用。本文采用布朗动力学方法系统地模拟了实际KcsA钾通道的电特性。得到了静电场作用下通道内离子的PMF、对称溶液和非对称溶液的电流-电压特性曲线、通道轴向离子浓度分布曲线和电导-浓度曲线。结果表明:KcsA钾离子通道的SF区基本阻断Cl-的通过,对K+的通过表现出特殊的选择特性;其电流-电压曲线基本呈线性分布,电导率-浓度曲线呈先升高后趋于平缓的趋势。该基本定律与实验现象是一致的。此外,还模拟分析了比强太赫兹场对通道K+电流的影响。与相同振幅的静电场相比,选择0.6/1.2/5THz太赫兹场可以通过影响离子对之间的相互作用势能来降低PMF,从而增加K+电流。本文的研究不仅加深了对KcsA钾离子通道的规律性的认识,而且为研究其他类型的离子通道以及太赫兹场对离子通道特性的影响提供了新的思路。
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引用次数: 0
Design and Fabrication of 940 nm VCSEL Single-emitter Device 940nm VCSEL单发射极器件的设计与制造
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230297
Pan Zhi-Peng, Li Wei, Lv Jia-Gang, Nie Yu-Wei, Zhong Li, Liu Su-ping, Ma Xiao-Yu
As the key part of Vertical Cavity Surface Emitting Laser (VCSEL), active region will seriously affect the threshold and efficiency of the device. To obtain appropriate laser wavelength and material gain, the In0.18Ga0.82As strain compensated quantum well is optimized design. The relationship between the lasing wavelength of multiple quantum wells (MQWs) and the thickness is calculated. Take into account the influence between the active region temperature and the lasing wavelength, the thickness of the quantum well is chose as 6 nm, the quantum barrier thickness is chose as 8 nm, corresponding to the lasing wavelength of 929 nm. The material gain characteristics of the MQWs under different temperature are simulated by Rsoft. The material gain exceeds 3300 /cm at 300 K, and the temperature drift coefficient of the peak wavelength is 0.3 nm/K. In this paper, Al0.09Ga0.91As and Al0.89Ga0.11As are selected as high and low refractive index materials of Distributed Braagg Reflector (DBR), and 20 nm graded layer is inserted between two types of materials. The influence of the graded layer thickness of DBR on the valence band barrier and reflection spectrum is calculated and analyzed. The increase of graded layer thickness can lead to the decrease of band barrier peak and the decrease of reflection spectrum bandwidth. The reflection spectrum and phase spectrum of P-DBR and N-DBR are calculated by the transmission matrix mode (TMM), the reflectance of DBR is over 99% and the phase shift is zero at 940 nm. The optical field distribution of the whole VCSEL structure is simulated, in which the standing wave peak overlaps with the active region, and the maximum gain can be obtained. Based on the finite element method (FEM), the effect of oxidation confined layer on the injection current is simulated. The current in the active region is effectively limited to the position corresponding to the oxidation confined hole, and its current density is stronger and more uniform. The optical field distribution in different modes of PC-VCSEL is simulated, different modes have different resonant wavelengths. The quality factor Q in different modes of VCSEL and Photonic Crystal-Vertical Cavity Surface Emitting Laser (PC-VCSEL) is calculated, Q of the fundamental mode is higher than higher transverse mode. It is demonstrated that the photonic crystal air hole structure can realize the output of basic transverse mode by increasing the loss of high order transverse mode. VCSEL and PC-VCSEL with oxidation hole size of 22 μm are successfully fabricated, in which the photonic crystal period is 5 μm, the air pore diameter is 2.5 μm and the etching depth is 2 μm. Under continuous current test, the maximum slope efficiency of VCSEL is 0.66 mW/mA, the output power is 9.3 mW at 22 mA, and the lasing wavelength is 948.64 nm at 20 mA injection current. Multiple wavelengths and large spectrum width is observed in the spectrum of VSCEL, which is an obvious multi-transverse mode. The maxi
有源区作为垂直腔面发射激光器(VCSEL)的关键部分,将严重影响器件的阈值和效率。为了获得合适的激光波长和材料增益,对In0.18Ga0.82As应变补偿量子阱进行了优化设计。计算了多量子阱的激光波长与厚度的关系。考虑到活性区温度和激光波长的影响,选择量子阱厚度为6 nm,量子势垒厚度为8 nm,对应激光波长为929 nm。利用Rsoft软件模拟了不同温度下mqw的材料增益特性。材料在300 K时的增益超过3300 /cm,峰值波长的温度漂移系数为0.3 nm/K。本文选择Al0.09Ga0.91As和Al0.89Ga0.11As作为分布式bragg反射器(DBR)的高、低折射率材料,并在两种材料之间插入20 nm的渐变层。计算分析了DBR渐变层厚对价带势垒和反射谱的影响。梯度层厚度的增加会导致能带势垒峰的减小和反射光谱带宽的减小。采用透射矩阵模式(TMM)计算了P-DBR和N-DBR的反射光谱和相谱,DBR的反射率大于99%,在940 nm处相移为零。模拟了整个VCSEL结构的光场分布,其中驻波峰与有源区重叠,可以获得最大增益。基于有限元法,模拟了氧化约束层对注射电流的影响。有源区的电流被有效地限制在氧化限制孔对应的位置,其电流密度更强、更均匀。模拟了PC-VCSEL在不同模式下的光场分布,不同模式下有不同的谐振波长。计算了VCSEL和光子晶体垂直腔面发射激光器(PC-VCSEL)不同模式下的品质因子Q,基模的Q高于高横模的Q。结果表明,光子晶体气穴结构可以通过增加高阶横模的损耗来实现基本横模的输出。成功制备了氧化孔尺寸为22 μm的VCSEL和PC-VCSEL,其中光子晶体周期为5 μm,空气孔径为2.5 μm,蚀刻深度为2 μm。在连续电流测试下,VCSEL的最大斜率效率为0.66 mW/mA,在22 mA时输出功率为9.3 mW,在20 mA注入电流下,激光波长为948.64 nm。VSCEL光谱具有多波长、大谱宽的特点,具有明显的多横向模式。PC-VCSEL的最大基模横模输出达到2.55 mW,侧模抑制比(SMSR)大于25 dB,谱宽小于0.2 nm,说明光子晶体空气孔对横模有较强的控制作用,在17 mA时激光波长为946.4 nm。
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引用次数: 0
First-principles calculations on O-atom diffusion on fluorinated graphene 氟化石墨烯上o原子扩散的第一性原理计算
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20221630
Hailin Yang, Qili Chen, Xing Gu, Ning Lin
Fluorination of graphene is one of the most effective methods to improve the corrosion protection of graphene coatings. In this paper, the diffusion and penetration behaviors of O atoms on fully fluorinated graphene (CF) and partially fluorinated graphene (C4F) were investigated using the NEB transition state search method. The effects of F atoms on the corrosion resistance of fluorinated graphene films were analyzed either. The results show that the adsorption of F atoms can effectively inhibit the diffusion of O atoms on graphene. On C4F, the F atoms are distributed in a para-top position, which greatly increases the surface diffusion energy barrier of O atoms. Moreover, it is difficult for the adsorbed O atoms to diffuse to different sp2 C rings through the obstruction of F atoms. The energy barrier of the horizontal diffusion of O atoms even reaches 2.69 eV in CF. And with the increase of F atoms, the stable structure of graphene is gradually destroyed, the barrier ability of C-atom layer for penetration behaviors of O atoms is greatly reduced. Furthermore, the interfacial adhesion work of pure graphene, CF and C4F films with Cu(111) surfaces were calculated, as well as the electronic structures of the composite interface using first-principles calculations. The interfacial adhesion work of the Cu/G, Cu/C4F and Cu/CF interfaces are 2.626J/m2、3.529J/m2and 3.559J/m2, respectively. The calculations show that the bonding of C4F and C4F with Cu substrate are more strong than pure graphene with Cu substrate, and the interfacial adhesion work increase with increasing of F atom adsorption concentration. The calculation of the density of states also conform stronger interaction between Cu and C atoms of the Cu/C4F interface than that of the Cu/CF interface. Bader charge analysis show increased charge transfer at both the Cu/C4F and Cu/CF interfaces comparing with the Cu/G interface, and Cu/C4F interface has more charge transfer, in which Cu-C bonds are formed.
石墨烯氟化是提高石墨烯涂层防腐性能的最有效方法之一。本文采用NEB过渡态搜索方法研究了O原子在全氟化石墨烯(CF)和部分氟化石墨烯(C4F)上的扩散和渗透行为。分析了F原子对氟化石墨烯薄膜耐腐蚀性能的影响。结果表明,F原子的吸附能有效抑制O原子在石墨烯上的扩散。在C4F上,F原子呈顶状分布,极大地提高了O原子的表面扩散能垒。此外,由于F原子的阻挡,吸附的O原子很难扩散到不同的sp2 C环上。在CF中,O原子水平扩散的能垒甚至达到2.69 eV,并且随着F原子的增加,石墨烯的稳定结构逐渐被破坏,c原子层对O原子穿透行为的势垒能力大大降低。此外,利用第一性原理计算计算了纯石墨烯、CF和C4F薄膜与Cu(111)表面的界面粘附功,以及复合界面的电子结构。Cu/G、Cu/C4F和Cu/CF界面的界面粘附功分别为2.626J/m2、3.529J/m2和3.559J/m2。计算表明,C4F和C4F与Cu衬底的结合比纯石墨烯与Cu衬底的结合更强,界面粘附功随着F原子吸附浓度的增加而增加。态密度的计算也证实Cu/C4F界面中Cu和C原子之间的相互作用强于Cu/CF界面。Bader电荷分析表明,Cu/C4F和Cu/CF界面的电荷转移均比Cu/G界面增加,Cu/C4F界面的电荷转移更多,并形成Cu- c键。
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引用次数: 0
Physical origins of complex interference structures in harmonic emission from molecular ions stretched to large internuclear distances 伸展到大核间距离的分子离子谐波发射中复杂干涉结构的物理起源
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20222410
Weiyan Li, Na Liu, Shang Wang
High-order harmonic generation (HHG) from the molecular ions stretched to large internuclear distances is studied numerically and analytically in this work. We focus on the fine structure of the HHG spectrum related to the contribution of short electron trajectory. In our numerically solving the time-dependent Schrodinger equation (TDSE), we use a trajectory-dependent filtering procedure to separate the short-trajectory contribution from other contributions of long trajectory and multiple returns. Our TDSE results reveal that the short-trajectory HHG spectra of molecular ion with larger internuclear distance show some complex interference structures characterized by some remarkable dips, and that the position of the dip is sensitive to the laser parameters. With a developed model arising from strong-field approximation (SFA), we are able to identify the physical origins of the complex interference structures. In this model considered is the charge-resonance effect which induces the strong coupling between the ground state and the first excited state of the molecular ion at large internuclear distance. In this model, the well-known effect of two-center interference occurs in the form of the canonical momentum instead of the momentum related to the instantaneous velocity of the electron in the general SFA. It is shown that some dips in TDSE results arise from two-center interference of the electronic wave between these two atomic cores of the molecule in the ionization process, while others come from that in the recombination process. These ionization and recombination dips alternately appear in the HHG spectra from the formed complex interference structures. The main differences between the interference effects in the ionization process and the recombination process are twofold. Firstly, in the ionization process, the destructive two-center interference strongly suppresses the forming of the continuum wavepacket, while in the recombination process, the recombination of the rescattering electron with other bound eigenstates with small weights can also contribute to HHG bedsides the recombination of the ground state with the first excited state with large weights. As a result, in TDSE results, the ionization dips are deeper and more remarkable than the recombination ones. Secondly, in the recombination process, the Coulomb acceleration remarkably changes the de Broglie wavelength of the rescattering electron and therefore changes the position of the interference-induced dip. While in the ionization process, the Coulomb potential plays a small role in the interference effect. As a result, the interference dips in the ionization process and the recombination process differ from each other.
本文用数值方法和解析方法研究了分子离子伸展到较大核间距离时产生的高次谐波。我们重点研究了与短电子轨迹贡献有关的HHG谱的精细结构。在我们的数值求解时变薛定谔方程(TDSE)时,我们使用了一个轨迹相关的滤波过程,将短轨迹的贡献与长轨迹和多重回报的其他贡献分离开来。我们的TDSE结果表明,较大核间距的分子离子的短轨迹HHG光谱表现出复杂的干涉结构,其特征是一些显著的倾角,并且倾角的位置对激光参数敏感。利用由强场近似(SFA)产生的成熟模型,我们能够识别复杂干涉结构的物理起源。在该模型中考虑了电荷共振效应,该效应在较大的核间距离上引起分子离子的基态和第一激发态之间的强耦合。在这个模型中,众所周知的双中心干涉效应以正则动量的形式出现,而不是一般SFA中与电子瞬时速度相关的动量。结果表明,TDSE的一些下降是由于电离过程中分子两个原子核之间的电子波的双中心干涉,而另一些则是由于复合过程中的电子波的双中心干涉。这些电离和复合倾角交替出现在形成的复杂干涉结构的HHG光谱中。电离过程中的干扰效应与复合过程中的干扰效应的主要区别有两个方面。首先,在电离过程中,破坏性双中心干涉强烈地抑制了连续波包的形成,而在复合过程中,重散射电子与其他小质量束缚本征态的复合也有助于HHG的形成,同时基态与大质量第一激发态的复合也有助于HHG的形成。结果表明,在TDSE结果中,电离下降比复合下降更深、更显著。其次,在复合过程中,库仑加速度显著改变了重散射电子的德布罗意波长,从而改变了干涉诱导倾角的位置。而在电离过程中,库仑势对干涉效应的影响很小。因此,电离过程和复合过程中的干涉幅度不同。
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引用次数: 0
Dependence of retrieval efficiency on the waist ratio of read beam and anti-Stokes photon modes in cavity-enhanced quantum memory 腔增强量子存储中读光束和反stokes光子模式腰比对检索效率的影响
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230966
Fan Wen-Xin, Wang Min-Jie, Jiao Hao-Le, Lu Jia-Jin, Liu Hai-Long, Yang Zhi-Fang, Xi Meng-Qi, Li Shu-Jing, Wang Hai
Quantum communication holds promise for absolutely secure information transmission. However, the direct transmission distance of quantum states is limited by the no-cloning theorem and transmission loss. To overcome these problems, Duan et al. proposed a promising quantum repeater scheme, DLCZ protocol (for Duan, Lukin, Cirac, and Zoller, in 2001), in which linear optics and atomic ensembles are used to combine entanglement generation and quantum memory into a single node. A quantum memory with highly retrieval efficiency is beneficial to increase the rate of entanglement swapping, achieving high-speed entanglement distribution. Up to now, high-efficiency quantum memories have been realized using high-optical-depth atomic ensembles or by coupling atomic ensembles with a medium-finesse optical cavity. However, the effect of the waist ratio of read beam and anti-Stokes photon modes on intrinsic retrieval efficiency has not been studied in detail. Here, we study the dependence of intrinsic retrieval efficiency on the waist ratio of read beam and anti-Stokes photon modes in cavity-enhanced quantum memory.In this work, a 87Rb atomic ensemble, that is placed at the center of a passively stabilized polarization interferometer (BD1,2), is used as quantum memory. Firstly, the ensemble is captured through magneto-optical trapping (MOT) and prepared to the Zeeman sub-level of ground state $|5{S_{1/2}},F = 1,m = 0rangle$. Then, a weak write pulse, with frequency red-detuned from the $|5{S_{1/2}},F = 1,m = 0rangle$$ to |5{P_{1/2}},F' = 1,m = 1rangle $ transition by 110 MHz, illuminates the atoms and induces spontaneous Raman scattering out a Stokes photon. In this regime of weak excitation, the detection of a Stokes photon heralds the storage of a single spin wave $|5{S_{1/2}},F = 1,m = 0rangle$$ leftrightarrow |5{S_{1/2}},F = 2,m = 0rangle $ ($|5{S_{1/2}},F = 1,m = 0rangle$$leftrightarrow |5{S_{1/2}},F = 2,m = 2rangle $) distributed among the whole ensemble. After a programmable delay, a read pulse, red-detuned from the $|5{S_{1/2}},F = 2,m = 0rangle to |5{P_{1/2}},F' = 2,m = - 1rangle $ transition by 110MHz, transfer this spin wave into an anti-Stokes photon. We detect the Stokes photons and anti-Stokes photons with polarization ${sigma ^ + }$, which means all the spin-wave are stored in a magnetic-field-insensitive state to reduce the decoherence caused by the stray magnetic fields. In order to increase the intrinsic retrieval efficiency, the atomic ensemble is placed in a ring cavity. The cavity length is 4 m, the finesse is measured to be ~15, and the escape efficiency of ring cavity is 52.9%. Both Stokes and anti-Stokes photon qubits are required to resonate with the ring cavity. To meet this requirement, a cavity-locking beam is injected into the cavity to stabilize the cavity length using a Pound-Drever-Hall locking scheme. Finally, we fixed the Stokes (anti-Stokes) photon modes waist and changed the waist ratio by changing the write beam (read beam)
量子通信有望实现绝对安全的信息传输。然而,量子态的直接传输距离受到不可克隆定理和传输损耗的限制。为了克服这些问题,Duan等人提出了一种很有前途的量子中继器方案,DLCZ协议(为Duan、Lukin、Cirac和Zoller于2001年提出),其中使用线性光学和原子系综将纠缠产生和量子存储结合到单个节点中。具有高检索效率的量子存储器有利于提高纠缠交换速率,实现高速纠缠分配。到目前为止,高效量子存储主要是利用高光深原子系综或将原子系综与中等精细度的光腔耦合实现的。然而,读光束和反斯托克斯光子模式腰比对本征检索效率的影响尚未得到详细的研究。本文研究了腔增强量子存储中读光束和反stokes光子模式腰比对本征检索效率的影响。在这项工作中,放置在被动稳定偏振干涉仪(BD1,2)中心的87Rb原子系综被用作量子存储器。首先,通过磁光捕获(MOT)捕获该系综,并将其制备到基态的塞曼亚能级$|5{S_{1/2}},F = 1,m = 0rangle$。然后,一个频率从$|5{S_{1/2}},F = 1,m = 0rangle$$ to |5{P_{1/2}},F' = 1,m = 1rangle $跃迁红失调谐110兆赫兹的弱写入脉冲,照亮原子并诱导自发拉曼散射出一个斯托克斯光子。在这种弱激发状态下,斯托克斯光子的探测预示着单个自旋波$|5{S_{1/2}},F = 1,m = 0rangle$$ leftrightarrow |5{S_{1/2}},F = 2,m = 0rangle $ ($|5{S_{1/2}},F = 1,m = 0rangle$$leftrightarrow |5{S_{1/2}},F = 2,m = 2rangle $)分布在整个系综中的存储。经过可编程延迟后,读取脉冲,从$|5{S_{1/2}},F = 2,m = 0rangle to |5{P_{1/2}},F' = 2,m = - 1rangle $跃迁红失调谐110MHz,将该自旋波转换为反斯托克斯光子。我们检测到Stokes光子和反Stokes光子的极化${sigma ^ + }$,这意味着所有的自旋波都以磁场不敏感的状态存储,以减少杂散磁场引起的退相干。为了提高本征检索效率,原子系综被放置在环形腔中。环形腔长度为4 m,精密度为15,环形腔的逃逸效率为52.9%. Both Stokes and anti-Stokes photon qubits are required to resonate with the ring cavity. To meet this requirement, a cavity-locking beam is injected into the cavity to stabilize the cavity length using a Pound-Drever-Hall locking scheme. Finally, we fixed the Stokes (anti-Stokes) photon modes waist and changed the waist ratio by changing the write beam (read beam) waist.The experiment result show that when the waist ratio of read beam and anti-Stokes photon modes is 3, the intrinsic retrieval efficiency is up to 68.9±1.6% and normalized cross-correlation function g(2) reaches 26.5±1.9. We built a theoretical model, the intrinsic retrieval efficiency increases with the rise of the waist ratio, which show that the intrinsic retrieval efficiency is up to the peak when the waist ratio is 3, and the intrinsic retrieval efficiency tends to be stable when the waist ratio continues to increase. The experiment agrees with the theory. In the future, we will improve the intrinsic retrieval efficiency by enhance the fineness of the optical cavity with optimizing the cavity parameters.
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引用次数: 0
The Study of Photon Acceleration Driven by the Near-forward Scattering in the Intense Laser Under-dense Plasma Interaction 强激光低密度等离子体相互作用中近前向散射驱动光子加速的研究
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20222014
Yue Dong-Ning, Dong Quan-Li, Chen Min, Zhao Yao, Geng Pan-Fei, Yuan Xiao-hui, Sheng Zheng-Ming, Zhang Jie
The mechanism of photon acceleration driven by the near-forward scattering (NFS) in intense laser under-dense plasma interaction has been studied by particle-in-cell (PIC) simulation. This mechanism utilizes tunneling ionization effect to stimulate electron plasma waves when the intense laser pulse propagates in under-dense plasmas. The electron plasma density is inhomogeneous both in longitudinal and transverse direction. In longitudinal direction, a steep ionized electron density front is generated by incident laser ionizing the helium gas. Around the ionization front, the incident laser interacts with electron plasma waves and generates the first kind of NFS waves. The frequency of NFS waves increases compared to the laser frequency. This is the first characteristic peak in the frequency spectrum. In transverse direction, the electron plasma waves have different phase velocities which makes the incident laser pulse undergoes NFS process and upshifts its frequency. This is the second characteristic peak in the frequency spectrum. Due to that the electron density inhomogeneity is much larger than the electron density perturbation of electron plasma wave, the scattering model and dispersion relationships, which are based on perturbation theory like the stimulated Raman scattering, are no longer applicable in this case. Our further study shows that the incident laser, electron density plasma waves and NFS waves still satisfy the energy conservation and momentum conservation which leads to the three-waves matching conditions of NFS process for inhomogeneous electron density. This can explain the appearance of two characteristic peaks in the frequency spectrum and their growth in the wave-vector space. This study has significant reference for the spectrum evolution when the intense laser pulse propagates in under-dense plasmas.
采用粒子池(PIC)模拟研究了强激光低密度等离子体相互作用中近前向散射(NFS)驱动光子加速的机理。该机制利用隧道电离效应刺激强激光脉冲在低密度等离子体中传播时产生的电子等离子体波。电子等离子体密度在纵向和横向上都是不均匀的。在纵向上,入射激光电离氦气产生一个陡峭的电离电子密度锋。在电离锋附近,入射激光与电子等离子体波相互作用,产生第一类NFS波。NFS波的频率相对于激光频率增大。这是频谱中的第一个特征峰。在横向上,电子等离子体波具有不同的相速度,使入射激光脉冲发生NFS过程,使其频率上升。这是频谱中的第二个特征峰。由于电子密度的不均匀性远大于电子等离子体波的电子密度摄动,基于受激拉曼散射等摄动理论的散射模型和色散关系在这种情况下不再适用。进一步的研究表明,入射激光、电子密度等离子体波和NFS波仍然满足能量守恒和动量守恒,这导致了非均匀电子密度的NFS过程的三波匹配条件。这可以解释频谱中两个特征峰的出现及其在波矢量空间中的增长。该研究对强激光脉冲在低密度等离子体中传播时的光谱演化具有重要的参考意义。
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引用次数: 0
Electron-spin polarization effect in Rashba spin-orbit coupling modulated single-layered semiconductor nanostructure Rashba自旋轨道耦合调制单层半导体纳米结构中的电子自旋极化效应
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20221381
He Ya-Ping, Chen Ming-Xia, Pan Jie-Feng, Li Dong, Lin Gang-Jun, Huang Xin-Hong
Nanothick semiconductors can grow orderly along a desired direction with the help of modern materials growth technology such as molecular beam epitaxy, which allows researchers to fabricate the so-called layered semiconductor nanostructure (LSN) in experiments. Due to the broken structure inversion symmetry by the layered form in the LSN, the electron spins interact tightly with its momentums, in literatures referred to as the spin-orbit coupling (SOC) effect, which can be modulated well by the interfacial confining electric field or the stain engineering. These significant SOC effects can effectively eliminate the spin degeneracy of the electrons in semiconductor materials, induce the spin splitting phenomenon at the zero magnetic field and generate the electron-spin polarization in the semiconductors. In recent years, the spin-polarized transport for electrons in the LSN has attracted a lot of research interests, thanks to itself scientific importance and potential applications as spin polarized sources in the research field of semiconductor spintronics. Adopting the theoretical analysis combined with the numerical calculation, we investigate the spin-polarized transport induced by the Rashba-type SOC effect for electrons in a single-layered semiconductor nanostructure (SLSN)-InSb. The research objective is to explore the new way for generating and manipulating spin current in semiconductor materials without any magnetic field, and focus on developing new electron-spin filter for semiconductor spintronics device applications. The improved transfer matrix method (ITMM) is exploited to exactly solve Schrödinger equation for an electron in the SLSN-InSb device, which allows us to calculate the spin-dependent transmission coefficient and the spin polarization ratio. Due to a strong Rashba-type SOC, a considerable electron-spin polarization effect appears in the SLSN-InSb device. Because of the effective potential experienced by the electrons in the SLSN-InSb device, the spin polarization ratio is associated with the electron energy and the in-plane wave vector. In particular, the spin polarization ratio can be manipulated effectively by an externally-applied electric field or the semiconductor-layer thickness, owing to the dependence of the effective potential felt by the electrons in the SLSN-InSb device on the electric field or the layer thickness. Therefore, such a SLSN-InSb device can serve as a controllable electron-spin filter as a manipulable spin-polarized source for the research area of semiconductor spintronics.
在分子束外延等现代材料生长技术的帮助下,纳米厚半导体可以沿着期望的方向有序生长,这使得研究人员可以在实验中制造出所谓的分层半导体纳米结构(LSN)。由于层状结构破坏了LSN的结构反演对称性,电子自旋与动量紧密相互作用,在文献中称为自旋-轨道耦合(SOC)效应,这种效应可以通过界面约束电场或染色工程进行调制。这些显著的SOC效应可以有效消除半导体材料中电子的自旋简并,在零磁场下诱导自旋分裂现象,在半导体中产生电子-自旋极化。近年来,LSN中电子的自旋极化输运由于其科学重要性和作为自旋极化源在半导体自旋电子学研究领域的潜在应用,引起了人们的广泛关注。采用理论分析与数值计算相结合的方法,研究了单层半导体纳米结构(SLSN)-InSb中rashba型SOC效应对电子的自旋极化输运。研究目标是探索在半导体材料中无磁场产生和控制自旋电流的新方法,并重点开发用于半导体自旋电子器件的新型电子自旋滤波器。利用改进的传递矩阵法(ITMM)精确求解了SLSN-InSb器件中电子的Schrödinger方程,从而计算出自旋相关透射系数和自旋极化比。由于具有较强的rashba型SOC, SLSN-InSb器件中出现了相当大的电子自旋极化效应。由于SLSN-InSb器件中电子所经历的有效电位,自旋极化比与电子能量和面内波矢量有关。特别是,由于SLSN-InSb器件中电子感受到的有效电位依赖于电场或半导体层厚度,因此可以通过外加电场或半导体层厚度有效地控制自旋极化比。因此,这种SLSN-InSb器件可以作为半导体自旋电子学研究领域的可控电子自旋滤波器和可操纵自旋极化源。
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引用次数: 1
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