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A study on the thermoelectric properties of acene molecular junctions 丙烯酸分子结的热电性质研究
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230354
Xie Zhong-Xiang, 周五星, Yu Xia, Jia Pin-Zhen, Chen Xue-Kun, Deng Yuan-Xiang, Zhang Yong, Zhou Wu-Xing
By using non-equilibrium Green's function method, we investigate the thermoelectric properties of the molecular junctions based on acene-linked graphene nanoribbons. In this paper, effects of the length of the acene molecule, the contact position between the acene molecule and graphene nanoribbon electrodes on the thermoelectric parameters is mainly considered. It is found that the phonon contribution is dominant in the thermal conductance corresponding to the maximum of the thermoelectric figure of merit (ZTmax). As the length of the acene molecules increases, the phonon thermal conductance decreases monotonically, and eventually becomes almost independent of the acene molecules’ length. When the acene molecules are in contact with the middle (upper) part of the left (right) electrode of graphene nanoribbons, the corresponding ZTmax is highest. However, when the acene molecules are in contact with the middle (middle) part of the left (right) electrode of graphene nanoribbons, the corresponding ZTmax is lowest. When the temperature increases, ZTmax has an monotonously increasing tendency, regardless of the contact position. With the increase of the length of the acene molecules, the chemical potential corresponding to ZTmax becomes closer to the intrinsic Fermi level. The above findings may provide the valuable reference for the future design of thermoelectric devices based on the acene molecular junctions.
利用非平衡格林函数方法,研究了烯链石墨烯纳米带分子结的热电性质。本文主要考虑了烯分子的长度、烯分子与石墨烯纳米带电极的接触位置对热电参数的影响。发现声子的贡献在热电优值(ZTmax)最大值对应的热导率中占主导地位。随着酰基分子长度的增加,声子热导率单调减小,最终几乎与酰基分子长度无关。当烯分子与石墨烯纳米带左(右)电极的中(上)部分接触时,对应的ZTmax最大。然而,当烯分子与石墨烯纳米带左(右)电极的中间(中)部分接触时,对应的ZTmax最小。当温度升高时,无论接触位置如何,ZTmax都有单调增加的趋势。随着烯类分子长度的增加,ZTmax对应的化学势更接近于本征费米能级。以上研究结果可为今后基于分子结的热电器件的设计提供有价值的参考。
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引用次数: 1
Dissipation-Induced Recurrence of Non-Hermitian Edge Burst 非厄米边爆发的耗散诱导递推
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230338
Ren Cui-Cui, Yin Xiang-Guo
In quantum mechanics, the Hermitian Hamiltonian is generally used to describe the ideal closed quantum system, but in reality, the physical system is closely related to the environment, and the open quantum system coupled to the environment can be described by the equivalent non-Hermitian Hamiltonian to a certain extent. Among them, the dissipation intensity is closely related to the dynamic properties of non-Hermitian quantum systems. Therefore, it is of great practical significance to study how dissipation affects particle loss. In this paper, the dynamic law related to dissipation intensity in one-dimensional non-Hermitian systems under open boundary conditions is studied, and it is found that dissipation can induce the recurrence of edge burst. After the time-dependent evolution of the particles in the one-dimensional non-Hermitian dissipative lattice system with open boundary conditions, there is an edge burst in the system, that is, there is a large probability of particle loss at the edge, and the edge burst disappears after increasing the intensity of intracellular transition. It is found that if the dissipation intensity is increased or decreased, the edge burst will reappear. This kind of reappearance is different from the original edge burst, which is mainly manifested in the loss probability distribution of particles from the edge distribution to the volume distribution, which is due to the different probability of particle motion direction in the two cases. Under the re-induced edge burst, the particles move from the initial position to the left and right directions, and the left side rebounds after reaching the boundary, forming a more obvious loss probability at the edge and gradually decreasing to the body area. In the original edge burst, the probability of particles only moving to the left is larger, and the 'trapped' is completely dissipated at the edge, forming a distribution with an independent loss peak at the edge, the movement to the left is due to due to the non-Hermitian skin effect. The deeper reason for different movement directions is related to the defect of non-Hermitian system far from parity-time symmetry breaking. Under the parameter near the parity-time symmetry breaking defect, the loss probability of the particle is unilateral distribution, and the loss probability of the particle moving to both sides is bilateral distribution when it is far away. This is the description of the dissipation-induced edge burst recurrence phenomenon and its characteristics. In addition, this paper also studies the influence of impurity barrier on the probability distribution of particle loss in non-Hermitian dynamics. The results show that placing a small barrier on the non-dissipative A-site can obviously hinder the particle motion, and when the barrier increases to a certain height, its influence on the particle motion tends to be unchanged. And the barrier at the dissipative B lattice has little effect on the dynamics.
在量子力学中,厄米哈密顿量一般用来描述理想的封闭量子系统,但在现实中,物理系统与环境密切相关,与环境耦合的开放量子系统在一定程度上可以用等效的非厄米哈密顿量来描述。其中,耗散强度与非厄米量子系统的动力学性质密切相关。因此,研究耗散对颗粒损耗的影响具有重要的现实意义。本文研究了开放边界条件下一维非厄米系统耗散强度的动力学规律,发现耗散可以引起边缘突发的重复发生。在开放边界条件下的一维非厄米耗散晶格系统中,粒子经过随时间的演化后,系统中存在边缘爆裂现象,即粒子在边缘处有较大的损失概率,增加胞内跃迁强度后,边缘爆裂现象消失。研究发现,增大或减小耗散强度,都会重新出现边缘爆裂。这种再现与原始边缘爆发不同,主要表现在粒子从边缘分布到体积分布的损失概率分布上,这是由于两种情况下粒子运动方向的概率不同造成的。在再次诱导的边缘爆裂下,粒子从初始位置向左右方向移动,左侧到达边界后反弹,在边缘处形成更明显的损失概率,并逐渐减小到体面积。在原始边缘爆发中,粒子只向左移动的概率更大,“被困”的粒子在边缘完全耗散,在边缘形成一个具有独立损耗峰的分布,向左移动是由于非厄米集肤效应。运动方向不同的深层原因与非厄米系统远离奇偶时间对称性破缺的缺陷有关。参数在奇偶时间对称性破缺缺陷附近时,粒子的损失概率为单侧分布,粒子向两侧移动时的损失概率为双侧分布。这是对耗散引起的边缘爆发重现现象及其特征的描述。此外,本文还研究了杂质势垒对非厄米动力学中粒子损失概率分布的影响。结果表明,在非耗散a位上放置一个小的势垒可以明显阻碍粒子的运动,当势垒增加到一定高度时,对粒子运动的影响趋于不变。耗散B晶格的势垒对动力学的影响很小。
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引用次数: 0
Soliton Solutions of the Spin-Orbit Coupled Binary Bose-Einstein Condensate System 自旋-轨道耦合二元玻色-爱因斯坦凝聚系统的孤子解
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20222319
Li Xin-Yue, Qi Juan-Juan, Zhao Dun, Liu Wu-ming
In a quantum system with spin, spin-orbit coupling is manifested by linking the spin angular momentum of a particle with its orbital angular momentum, which leads to many exotic phenomena. The experimental realization of synthetic spin-orbit coupling effects in ultra-cold atomic systems provides a completely new platform for exploring quantum simulations. In a spinor Bose-Einstein condensate, the spin-orbit coupling can change the properties of the system significantly, which offers a great opportunity to investigate the influence of spin-orbit coupling to the quantum state at the macroscopic level. As typical states of macroscopic quantum effects, solitons in spin-orbit coupled Bose-Einstein condensates can be manipulated by spin-orbit coupling directly, this makes the study on spin-orbit coupled Bose-Einstein condensates become one of the hottest topics in the research of ultracold atomic physics in recent years. This paper investigates exact vector soliton solutions of the Gross-Pitaevskii equation for the one-dimensional spin-orbit coupled binary Bose-Einstein condensates, which has four parameters μ,δ,α and β, where μ denotes the strength of the spin-orbit coupling, δ is the detuning parameter,α and β are the parameters of the self-and cross-interaction, respectively. For the case β=α, by a direct ansatz, two kinds of stripe solitons, namely, the oscillating dark-dark solitons are obtained; meanwhile, a transformation is presented such that from the solutions of the integrable Manakov system, one can get soliton solutions for the spin-orbit coupled Gross-Pitaevskii equation. For the case β=3α, a bright-W type soliton for α>0 and a kink-antikink type soliton for α<0 are presented. It is found that the relation between μ and δ can affect the states of the solitons. Based on these solutions, the corresponding dynamics and the impact of the spin-orbit coupling effects on the quantum magnetization and spin-polarized domains are discussed. Our results show that spin-orbit coupling can result in rich kinds of soliton states in the two-component Bose gases, including the stripe solitons as well as the classical non-stripe solitons, and various kinds of multi-solitons. Furthermore, spin-orbit coupling has remarkable influence on the behaviors of quantum magnetization. In the experiments of Bose-Einstein condensates, there have been many different methods to observe the soliton states of the population distribution, the magnetic solitons, and the spin domains, so our results provide some possible options for the related experiments.
在有自旋的量子系统中,粒子的自旋角动量与其轨道角动量相联系,表现为自旋-轨道耦合,从而导致许多奇异现象。超冷原子系统合成自旋轨道耦合效应的实验实现为探索量子模拟提供了一个全新的平台。在旋量玻色-爱因斯坦凝聚体中,自旋-轨道耦合可以显著地改变系统的性质,这为在宏观水平上研究自旋-轨道耦合对量子态的影响提供了很好的机会。自旋-轨道耦合玻色-爱因斯坦凝聚体中的孤子作为宏观量子效应的典型状态,可以通过自旋-轨道耦合直接操纵,这使得自旋-轨道耦合玻色-爱因斯坦凝聚体的研究成为近年来超冷原子物理研究的热点之一。本文研究了一维自旋-轨道耦合二元玻色-爱因斯坦凝聚体的Gross-Pitaevskii方程的精确矢量孤子解,该凝聚体具有四个参数μ、δ、α和β,其中μ表示自旋-轨道耦合强度,δ表示失谐参数,α和β分别表示自旋-轨道耦合和相互作用的参数。对于β=α的情况,通过直接解析得到两种条纹孤子,即振荡的暗-暗孤子;同时,给出了由可积Manakov系统的解得到自旋-轨道耦合Gross-Pitaevskii方程的孤子解的变换。在β=3α的情况下,得到了α>0的亮w型孤子和α<0的扭结-反扭结型孤子。发现μ和δ之间的关系会影响孤子的态。在此基础上,讨论了相应的动力学以及自旋轨道耦合效应对量子磁化和自旋极化畴的影响。结果表明,自旋轨道耦合可以在双组分玻色气体中产生丰富的孤子态,包括条纹孤子、经典非条纹孤子和各种多孤子。此外,自旋-轨道耦合对量子磁化行为有显著影响。在玻色-爱因斯坦凝聚体的实验中,已经有许多不同的方法来观察种群分布、磁孤子和自旋域的孤子态,因此我们的结果为相关实验提供了一些可能的选择。
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引用次数: 0
Research progress on the laser system of the cold atomic clock in China Space Station 中国空间站冷原子钟激光系统研究进展
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230412
Liu Yun, Wang Wen-Hai, He De-Jing, Zhou Yong-Zhuang, Shen Yong, Zou Hong-Xin
The first space optical clock (SOC) in the world developed in China, which is composed by five subsystems, including an optical unit, a physics unit, an electronic control unit, a space optical frequency comb, and an ultrastable laser, has been successfully launched with the Mengtian space laboratory into the China Space Station (CSS). Compact and stable lasers are key elements for the operation of the SOC. The optical unit consists of 5 lasers at 461 nm, 679 nm, 689 nm, 707nm, and 813 nm. With a synchronous-tuning-like scheme, high quality external cavity diode lasers (ECDL) have been developed as the seeds. The linewidth of the lasers is suppressed to the order of 100 kHz, and the mode-hop-free tuning range reaches 20 GHz, which meet the requirements of the SOC. With careful mechanical and thermal design, the stability of the lasers against vibration and temperature fluctuation has been sufficiently promoted to confront the challenge of rocket launching. While the power from the ECDL is sufficient for 679 nm and 707 nm repump lasers, additional injection lock is utilized for the 461 nm and 689 nm lasers to amplify the power of the seeds to more than 600 mW, so that efficient first and second stage Doppler cooling can be achieved. To generate an optical lattice with deep enough potential well, over 800 mW 813 nm lasers is required. Therefore, a semiconductor tapered amplifier is adopted to amplify the seed to more than 2 W, so as to cope with various losses of the coupling optics. The wavelength and output power of the 5 lasers are monitored and feedback-controlled by the electronic control unit. All the modules are designed and manufactured as orbital replaceable units, which can be easily replaced by astronauts in case failure occurs. Now the lasers are all turned on and operates normally in CSS. More data of the SOC will be obtained in the near future. At present stage, according to our evaluation, the continuous operation time of the SOC is limited by the injection locked lasers, which are relatively vulnerable to mode hopping. Hopefully this problem can be solved by improving the laser diode manufacturing technology, or developing fiber lasers with compact frequency conversion modules.
由光学单元、物理单元、电子控制单元、空间光频梳和超稳激光器等5个子系统组成的世界首个空间光时钟(SOC)已随蒙田空间实验室成功发射进入中国空间站。紧凑和稳定的激光器是SOC运行的关键要素。光单元由461 nm、679 nm、689 nm、707nm和813 nm波长的5个激光器组成。利用类似同步调谐的方案,高质量的外腔二极管激光器(ECDL)作为种子被开发出来。该激光器的线宽被抑制到100 kHz数量级,无跳模调谐范围达到20 GHz,满足SOC的要求。通过精心的机械和热设计,充分提高了激光器对振动和温度波动的稳定性,以应对火箭发射的挑战。虽然ECDL的功率足以用于679 nm和707 nm的再泵激光器,但额外的注入锁用于461 nm和689 nm激光器,将种子的功率放大到600 mW以上,因此可以实现高效的第一和第二阶段多普勒冷却。为了产生具有足够深的势阱的光学晶格,需要超过800 mW的813 nm激光器。因此,采用半导体锥形放大器将种子放大到2w以上,以应对耦合光学器件的各种损耗。电子控制单元对5种激光器的波长和输出功率进行监测和反馈控制。所有的模块都被设计和制造为轨道可更换单元,如果发生故障,宇航员可以很容易地更换。现在激光器全部打开并在CSS中正常运行。更多的SOC数据将在不久的将来获得。现阶段,根据我们的评估,SOC的连续工作时间受到注入锁定激光器的限制,这些激光器相对容易受到模式跳变的影响。希望通过改进激光二极管制造技术,或开发具有紧凑变频模块的光纤激光器来解决这一问题。
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引用次数: 0
Compact broadband bandpass filter with wide stopband based on halberd-shaped spoof surface plasmon polariton 基于戟形欺骗表面等离子激元极化子的紧凑型宽阻带带通滤波器
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20222291
Shu-Peng Sun, Yongzhi Cheng, Hui Luo, Fu Chen, Xiangcheng Li
In this paper, a compact broadband bandpass filter with wide out-of-band rejection characteristics based on halberd-shaped spoof surface plasmon polariton (SSPP) is proposed. The filtering structure is achieved by etching a periodic halberd-shaped groove at the bottom of the substrate and a microstrip-to-slot line transition with a crescent-shaped patch at the top. Compared with the traditional dumbbell-shaped SSPP, the halberd-shaped SSPP has good slow-wave property, and the designed bandpass filter based on halberd-shaped SSPP can achieve a more compact size. The upper cutoff frequency and lower cutoff frequency of the passband can be adjusted by regulating the SSPP structure and the transition structure from microstrip-to-slot line, respectively. The simulation results show that the center frequency of broadband bandpass filter is 2.85 GHz, with the relative bandwidth of 130%, and the return loss in the passband is better than –10 dB, and the extreme strong out-of-band rejection of –40 dB from 5.6 GHz to 20 GHz. The size of the broadband bandpass filter is compact, only 1.08λg×0.39λg, where λg is the wavelength at the center frequency. In order to verify the effectiveness of the wideband bandpass filter, the traditional printed circuit board technology is used to fabricate the wideband bandpass filter. The measurement results are in good agreement with the simulation results, verifying the feasibility of the design. The proposed broadband bandpass filter shows promising prospects for developing SSPP functional devices and circuits at microwave frequencies.
提出了一种基于戟形欺骗表面等离子激元(SSPP)的窄带带通滤波器,具有宽带外抑制特性。该滤波结构是通过在衬底底部蚀刻周期性戟形凹槽和在顶部蚀刻具有月牙形贴片的微带到槽线过渡来实现的。与传统的哑铃形SSPP相比,戟形SSPP具有良好的慢波性能,基于戟形SSPP设计的带通滤波器可以实现更紧凑的尺寸。通带的上截止频率和下截止频率可以分别通过调节SSPP结构和微带到槽线的过渡结构来调节。仿真结果表明,该宽带带通滤波器的中心频率为2.85 GHz,相对带宽为130%,在5.6 GHz ~ 20 GHz范围内回波损耗优于-10 dB,带外抑制极强,为-40 dB。宽带带通滤波器尺寸紧凑,只有1.08λg×0.39λg,其中λg为中心频率处的波长。为了验证宽带带通滤波器的有效性,采用传统的印刷电路板技术制作宽带带通滤波器。测量结果与仿真结果吻合较好,验证了设计的可行性。所提出的宽带带通滤波器在开发微波频率的SSPP功能器件和电路方面具有良好的前景。
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引用次数: 1
A simple DGTD method with the impedance boundary condition 具有阻抗边界条件的简单DGTD方法
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20222104
Yang Qian, Wei Bing, Li Linqian, Deng Haochuan
Large-size conductive targets or coated targets are difficult issues in computational electromagnetics. In general, such targets can be classified as multi-scale problems. Multi-scale problems usually consume a large number of computational resources. Researchers are devoted to seeking fast methods for these problems. When the skin depth is less than the size of a conductive target, the tangential components of the electric and magnetic fields over the surface of the target can be correlated by the surface impedance Ẑ. Ẑ is usually a complex function of the frequency, and it can be used to formulate an impedance boundary condition (IBC) to describe iterative equations in time domain methods to avoid the volumetric discretization of the target to improve computational efficiency. This condition is commonly known as the surface impedance boundary condition (SIBC). Similarly, for a conductor with thickness on the order or less than the skin depth, it also has high resource requirements if the target is straightforward volumetric discretization. The transmission impedance boundary condition (TIBC) can be applied to replace a coated object to reduce resource requirements. Thus, volumetric discretization is not required. There are few studies on the IBC scheme in the DGTD method. P. Li discussed the IBC scheme in DGTD, which involves complex matrix operations in the processing of IBC. In the DGTD method, numerical flux is used to transmit data between neighboring elements, and the key to the IBC scheme in DGTD is how to handle numerical flux. We hope to propose a DGTD method with a simple form and matrix-free IBC scheme. The key in dealing with IBC in DGTD is numerical flux. Unlike the literature, the impedance ẐR is not approximated by rational functions in our study. A specfic function ẐR obtained after the derivation in this paper is approximated by rational functions in the Laplace domain using the vector-fitting (VF) method, and its time-domain iteration scheme is given. This approach avoids matrix operations. The TIBC and SIBC processing schemes are given in section 4. The proposed method's advantage is that the upwind flux's standard coefficients are retained, and the complex frequency-time conversion problem is implemented by the vector-fitting method. The one-dimensional and three-dimensional examples also show the accuracy and effectiveness of our work in this paper.
大尺寸导电目标或涂覆目标是计算电磁学中的难题。一般来说,这类目标可以归类为多尺度问题。多尺度问题通常会消耗大量的计算资源。研究人员致力于寻找解决这些问题的快速方法。当蒙皮深度小于导电目标的尺寸时,可以通过表面阻抗Ẑ来关联目标表面上电场和磁场的切向分量。Ẑ通常是频率的复函数,在时域方法中可以用它来建立阻抗边界条件(IBC)来描述迭代方程,避免了目标的体积离散化,提高了计算效率。这种条件通常被称为表面阻抗边界条件(SIBC)。同样,对于厚度为或小于蒙皮深度的导体,如果目标是直接的体积离散化,它也有很高的资源要求。传输阻抗边界条件(TIBC)可用于代替被涂覆物体,以减少资源需求。因此,不需要体积离散化。对于DGTD方法中IBC方案的研究很少。李鹏讨论了DGTD中的IBC方案,其中IBC的处理涉及复杂的矩阵运算。在DGTD方法中,采用数值通量在相邻单元之间进行数据传输,而DGTD中IBC方案的关键是如何处理数值通量。我们希望提出一种具有简单形式和无矩阵IBC方案的DGTD方法。在DGTD中处理IBC的关键是数值通量。与文献不同的是,在我们的研究中,阻抗ẐR不是用有理函数近似的。用向量拟合(vector-fitting, VF)方法在拉普拉斯域中用有理函数逼近了本文推导得到的一个特定函数ẐR,并给出了它的时域迭代格式。这种方法避免了矩阵运算。第4节给出了TIBC和SIBC处理方案。该方法的优点是保留了迎风通量的标准系数,并采用矢量拟合方法实现了复频率-时间转换问题。一维和三维的算例也证明了本文工作的准确性和有效性。
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引用次数: 0
Dual-channel structured illumination super-resolution quantitative FRET imaging 双通道结构照明超分辨率定量FRET成像
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20230853
ZEWEI LUO, GE WU, ZHI CHEN, CHINAN DANG, RONG WAN, Tao Yang, ZHENGFEI ZHUANG, AND TONGSHENG CHEN
The Structured Illumination (SI)-based Super Resolution Fluorescence Resonance Energy Transfer (SR-FRET) imaging technique, known as SISR-FRET, enables the investigation of molecular structures and functions in cellular organelles by resolving sub-diffraction FRET signals within living cells. FRET microscopy offers unique advantages for quantitatively detecting dynamic interactions and spatial distribution of biomolecules within living cells. The spatial resolution of conventional FRET microscopy is limited by the diffraction limit, and it can only capture the average behavior of these events within the resolution limits of conventional fluorescence microscopy. SISR-FRET performs sequential linear reconstruction of the three-channel SIM images followed by FRET quantitative analysis using a common localization mask-based filtering approach. This two-step process ensures the fidelity of the reconstructed SR-FRET signals while effectively removing false-positive FRET signals caused by SIM artifacts. However, the slow imaging speed resulting from the switching of excitation-emission channels in SISR-FRET imaging limits its application in fast imaging scenarios. To address this issue, this study proposes a dual-channel structured illumination super-resolution quantitative FRET imaging system and method. By incorporating a FRET dual-channel imaging and registration module into the imaging pathway, spatial switching and channel multiplexing of the SISR-FRET excitation-emission channels are achieved. Combining the image reconstruction algorithm with channel sub-pixel registration correction, the dual-channel SISR-FRET technique enhances the temporal resolution by 3.5 times while preserving the quantitative super-resolution FRET analysis. Experimental results were obtained using a multi-color SIM system to perform super-resolution imaging of living cells expressing mitochondria outer membrane FRET standard plasmids. These experiments validate the improved spatial and temporal resolution of dual-channel SISR-FRET and the fidelity of FRET quantification analysis. In summary, this research presents a novel dual-channel structured illumination super-resolution FRET imaging system and methodology. It overcomes the limitations of slow imaging speed in SISR-FRET by enabling spatial switching and channel multiplexing of excitation-emission channels. The proposed technique enhances the temporal resolution while maintaining quantitative analysis of super-resolution FRET. Experimental validation demonstrates the increased spatial and temporal resolution of dual-channel SISR-FRET and the accuracy of FRET quantification analysis. This advancement contributes to the study of molecular structures and functions in cellular organelles, providing valuable insights into the intricate mechanisms of living cells.
基于结构照明(SI)的超分辨率荧光共振能量转移(SR-FRET)成像技术,被称为SISR-FRET,通过解析活细胞内的亚衍射FRET信号,可以研究细胞器中的分子结构和功能。FRET显微镜为定量检测活细胞内生物分子的动态相互作用和空间分布提供了独特的优势。传统FRET显微镜的空间分辨率受到衍射极限的限制,它只能捕获这些事件的平均行为在传统荧光显微镜的分辨率限制内。SISR-FRET执行三通道SIM图像的顺序线性重建,然后使用基于通用定位掩模的滤波方法进行FRET定量分析。这两步过程确保了重建的SR-FRET信号的保真度,同时有效地去除由SIM伪影引起的假阳性FRET信号。然而,在SISR-FRET成像中,由于激发发射通道的切换导致成像速度较慢,限制了其在快速成像场景中的应用。为了解决这一问题,本研究提出了一种双通道结构照明超分辨率定量FRET成像系统和方法。通过在成像通道中加入FRET双通道成像配准模块,实现了SISR-FRET激发发射通道的空间切换和通道复用。将图像重建算法与通道亚像素配准校正相结合,双通道SISR-FRET技术在保留定量超分辨率FRET分析的同时,将时间分辨率提高了3.5倍。实验结果采用多色SIM系统对表达线粒体外膜FRET标准质粒的活细胞进行超分辨率成像。这些实验验证了双通道SISR-FRET提高的时空分辨率和FRET量化分析的保真度。总之,本研究提出了一种新的双通道结构照明超分辨率FRET成像系统和方法。它通过实现激发发射通道的空间切换和通道复用,克服了SISR-FRET成像速度慢的限制。该技术提高了时间分辨率,同时保持了超分辨率FRET的定量分析。实验验证表明,双通道SISR-FRET提高了空间和时间分辨率,并提高了FRET定量分析的准确性。这一进展有助于细胞器分子结构和功能的研究,为了解活细胞的复杂机制提供有价值的见解。
{"title":"Dual-channel structured illumination super-resolution quantitative FRET imaging","authors":"ZEWEI LUO, GE WU, ZHI CHEN, CHINAN DANG, RONG WAN, Tao Yang, ZHENGFEI ZHUANG, AND TONGSHENG CHEN","doi":"10.7498/aps.72.20230853","DOIUrl":"https://doi.org/10.7498/aps.72.20230853","url":null,"abstract":"The Structured Illumination (SI)-based Super Resolution Fluorescence Resonance Energy Transfer (SR-FRET) imaging technique, known as SISR-FRET, enables the investigation of molecular structures and functions in cellular organelles by resolving sub-diffraction FRET signals within living cells. FRET microscopy offers unique advantages for quantitatively detecting dynamic interactions and spatial distribution of biomolecules within living cells. The spatial resolution of conventional FRET microscopy is limited by the diffraction limit, and it can only capture the average behavior of these events within the resolution limits of conventional fluorescence microscopy. SISR-FRET performs sequential linear reconstruction of the three-channel SIM images followed by FRET quantitative analysis using a common localization mask-based filtering approach. This two-step process ensures the fidelity of the reconstructed SR-FRET signals while effectively removing false-positive FRET signals caused by SIM artifacts. However, the slow imaging speed resulting from the switching of excitation-emission channels in SISR-FRET imaging limits its application in fast imaging scenarios. To address this issue, this study proposes a dual-channel structured illumination super-resolution quantitative FRET imaging system and method. By incorporating a FRET dual-channel imaging and registration module into the imaging pathway, spatial switching and channel multiplexing of the SISR-FRET excitation-emission channels are achieved. Combining the image reconstruction algorithm with channel sub-pixel registration correction, the dual-channel SISR-FRET technique enhances the temporal resolution by 3.5 times while preserving the quantitative super-resolution FRET analysis. Experimental results were obtained using a multi-color SIM system to perform super-resolution imaging of living cells expressing mitochondria outer membrane FRET standard plasmids. These experiments validate the improved spatial and temporal resolution of dual-channel SISR-FRET and the fidelity of FRET quantification analysis. In summary, this research presents a novel dual-channel structured illumination super-resolution FRET imaging system and methodology. It overcomes the limitations of slow imaging speed in SISR-FRET by enabling spatial switching and channel multiplexing of excitation-emission channels. The proposed technique enhances the temporal resolution while maintaining quantitative analysis of super-resolution FRET. Experimental validation demonstrates the increased spatial and temporal resolution of dual-channel SISR-FRET and the accuracy of FRET quantification analysis. This advancement contributes to the study of molecular structures and functions in cellular organelles, providing valuable insights into the intricate mechanisms of living cells.","PeriodicalId":6995,"journal":{"name":"Acta Physica Sinica","volume":null,"pages":null},"PeriodicalIF":1.0,"publicationDate":"2023-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"88924264","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Sharing entanglement of the Werner state by arbitrarily many independent observers 由任意多个独立的观察者共享维尔纳态的纠缠
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20222039
Yu Xin-Miao, Yang Shu-Yuan, He Kan
The problem of sharing quantum correlations is an interesting problem in the study of quantum information theory. Silva et al. proposed the study of sharing quantum nonlocality at first. They studied the fundamental limits on nonlocality, asking whether a single pair of entangled qubits could generate a long sequence of nonlocal correlations. At the same time, the sequential scenario was also introduced first, in which Alice and Bob each have half of a pair of entangled qubit states. The first Bob measures his half and then passes his part to a second Bob who measures again and so on. Obviously, even partial preservation of entanglement in a shared state in spite of a few sequences of local operations performed by the sharing parties can be important for information processing schemes in which entanglement is utilized as a resource. Thus, the problem of sharing quantum entanglement has also been extensively investigated. Recently, C. Srivastava et al. proved that there exist a class of T-states whose entanglement can be shared by arbitrarily many independent observers in[Phys. Rev. A 2022 105 062413]. Here, we want to find whether there are other entangled states that can be shared entanglement arbitrarily many times. In this paper, we consider the problem of sharing quantum entanglement when the initial shared state is a two-qubit entangled Werner state. The goal is to maximize the number of Bobs that can share entanglement with a single Alice. By suitably choosing the entanglement witness operator and the unsharp measurement settings by the Bobs, we prove that there exist two-qubit entangled initial shared Werner states whose entanglement can be detected by arbitrarily many sequential observers Bobs with a single Alice. Then, we also consider the special case of the Werner state, that is, the maximally entangled state as the initial shared state. In this case, its entanglement can also be witnessed arbitrarily many times, and the number of Bobs increases with the decrease of parameter.
共享量子关联问题是量子信息理论研究中的一个有趣问题。Silva等人首先提出了共享量子非定域性的研究。他们研究了非局域性的基本限制,询问一对纠缠量子比特是否可以产生长序列的非局域相关性。同时,还首先引入了顺序场景,其中Alice和Bob各有一对纠缠量子比特状态的一半。第一个鲍勃测量他的那一半,然后把他的那一半交给第二个鲍勃,他再次测量,以此类推。显然,尽管共享方执行了一些局部操作序列,但即使在共享状态下部分保留纠缠,对于将纠缠作为资源利用的信息处理方案也很重要。因此,共享量子纠缠问题也得到了广泛的研究。最近,C. Srivastava等人在物理学中证明了存在一类t态,其纠缠可以被任意多个独立的观察者共享。[j].中国农业大学学报(自然科学版)。在这里,我们想要发现是否存在其他可以任意多次共享纠缠的纠缠态。本文考虑了初始共享态为双量子位纠缠Werner态时的共享量子纠缠问题。我们的目标是最大化可以与同一个Alice共享纠缠的bob的数量。通过适当地选择纠缠见证算子和bob的非尖锐测量设置,我们证明了存在两个量子比特纠缠的初始共享Werner态,其纠缠可以被任意多个具有单个Alice的顺序观察者bob检测到。然后,我们还考虑了Werner状态的特殊情况,即最大纠缠态作为初始共享态。在这种情况下,它的纠缠态也可以被任意多次地观察到,并且随着参数的减小,bob的数量也会增加。
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引用次数: 0
Study on mechanism and characteristics of sound scattering modulation by underwater low frequency oscillating vortex flow field 水下低频振荡涡流场声散射调制机理及特性研究
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20221748
Jing Chen-Xuan, Shi Sheng-Guo, Yang De-Sen, Zhang Jiang-Yi, Li Song
The scattering of sound waves by underwater vortex flow filed is the basic problem of sound waves propagating in complex flow fields, which has important significance in underwater target detection and sound imaging of flow field. The theoretical analysis model and numerical calculation method are established for the problem of sound scattering modulation in underwater low frequency oscillating vortex flow fields, and the generation mechanism and time frequency and space characteristics of the scattering modulation sound field are explored. Firstly, based on the wave equation of the moving medium, under the first-order approximation, the wave equation is decomposed into the flow-sound coupling term and the non flow-sound coupling term by introducing a potential function, and the flow-sound coupling term is analyzed in the frequency domain, revealing the underwater oscillating vortex flow field. Secondly, the discontinuous Galerkin numerical calculation method is used to solve the wave equation of the moving medium, and the sound propagation process in the underwater low frequency oscillating vortex flow field is numerically simulated. Under the condition of low Mach number, the effects of different incident sound frequency, the oscillation frequency of the vortex flow field and the scale of the vortex core on the time-frequency and space characteristics of the scattering modulating sound fields of vortex flow field are analyzed, and theoretical analysis model is used to explain the characteristics.The research results show that: under the condition of low Mach number, the scattering of sound wave by oscillating vortex flow field can produce a scattering modulated sound field containing the harmonic of oscillating frequency side frequency modulation. The amplitude of the scattered sound pressure changes periodically with time, and the forward scattering is much stronger than the backward scattering. The fundamental frequency scattering modulation is much stronger than the frequency doubling scattering modulation. With the increase of the frequency of the incident sound wave and the scale of the vortex core, the intensity of the scattering modulating sound field increases, and the spatial distribution of the total scattering sound field has symmetry and an obvious main lobe, the main lobe is gradually sharpened, the azimuth angle of the main lobe is close to the propagation direction of the incident wave. When the frequency ratio is much greater than 1, the vortex flow field oscillation frequency has little effect on the spatial distribution of the sound field intensity of scattering modulating sound field.
水下涡旋流场对声波的散射是声波在复杂流场中传播的基本问题,在水下目标探测和流场声成像中具有重要意义。建立了水下低频振荡旋涡流场声散射调制问题的理论分析模型和数值计算方法,探讨了声散射调制声场的产生机理和时频空特性。首先,在运动介质波动方程的基础上,在一阶近似下,引入势函数,将波动方程分解为流声耦合项和非流声耦合项,并对流声耦合项进行频域分析,揭示水下振荡涡流场;其次,采用不连续伽辽金数值计算方法求解运动介质的波动方程,数值模拟声音在水下低频振荡涡旋流场中的传播过程。在低马赫数条件下,分析了不同入射声频、旋涡流场振荡频率和旋涡核尺度对旋涡流场散射调制声场时频和空间特性的影响,并采用理论分析模型对这些特性进行了解释。研究结果表明:在低马赫数条件下,振荡涡旋流场对声波的散射可以产生包含振荡频侧调频谐波的散射调制声场。散射声压振幅随时间周期性变化,前向散射比后向散射强得多。基频散射调制比倍频散射调制强得多。随着入射声波频率和涡核尺度的增加,散射调制声场的强度增大,总散射声场的空间分布具有对称性和明显的主瓣,主瓣逐渐锐化,主瓣的方位角接近入射波的传播方向。当频率比远大于1时,旋涡流场振荡频率对散射调制声场声场强度的空间分布影响不大。
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引用次数: 0
Influence of ambient gas to flute instability produced at the interface between laser plasma and external magnetic field 环境气体对激光等离子体与外磁场界面产生的凹槽不稳定性的影响
IF 1 4区 物理与天体物理 Q3 Physics and Astronomy Pub Date : 2023-01-01 DOI: 10.7498/aps.72.20231108
Zhang Zhen-Chi, Tang Hui-Bo, Wang Jin-Chan, Si Hua-Chong, Wang Zhi, Lan Xiang, Hu Guang-Yue
Diamagnetic cavity and flute instability generated by plasma expansion in an external magnetic field are important phenomena in space and fusion physics.We use a nanosecond laser to irradiate a carbon planar target to generate plasma, and at the same time apply a 7T transverse pulsed strong magnetic field to the plasma. The flute instability generated on the surface of the diamagnetic cavity when the plasma expands in an external magnetic field is studied experimentally. Data analysis shows that under our experimental parameters, the radius of gyration of electrons(ρe) is much smaller than the density gradient scale length of the diamagnetic cavity(Ln), while the ion's gyration radius(ρi) is much larger than Ln, indicating that the electrons are magnetized while the ions are non magnetized. The relative drift between electrons and ions provides free energy for the development of instability.The drift velocity is composed of the gravity drift velocity and the diamagnetic gradient drift velocity. The calculation shows that the gravity drift velocity is much larger than the diamagnetic gradient drift velocity in our experiment, so the instability belongs to the Large Larmor Radius Instability. By filling the target chamber with helium, we found that the background gas can significantly inhibit the development of flute instability. When the background gas pressure exceeds 50Pa (about 1% of the interface plasma density), the flute instability is almost is completely suppressed. Kinetic dispersion equations show that ion-ion collisions and electron-ion collision effects are the main factors that inhibit the development of instability. Calculations on the dispersion equation show that ion-ion collisions are the main factor that inhibits the development of instabilities.
等离子体在外磁场中膨胀产生的抗磁腔和抗磁槽不稳定性是空间和核聚变物理中的重要现象。利用纳秒激光照射碳平面靶产生等离子体,同时对等离子体施加7T的横向脉冲强磁场。实验研究了等离子体在外加磁场作用下膨胀时,在抗磁腔表面产生的凹槽不稳定性。数据分析表明,在我们的实验参数下,电子的旋转半径(ρe)远小于反磁腔的密度梯度尺度长度(Ln),而离子的旋转半径(ρi)远大于Ln,说明电子被磁化而离子未被磁化。电子和离子之间的相对漂移为不稳定性的发展提供了自由能。漂移速度由重力漂移速度和反磁梯度漂移速度组成。计算表明,实验中重力漂移速度远大于反磁梯度漂移速度,因此不稳定性属于大拉莫尔半径不稳定性。通过向靶室充入氦气,我们发现背景气体可以显著抑制靶腔不稳定性的发展。当背景气体压力超过50Pa(约为界面等离子体密度的1%)时,凹槽的不稳定性几乎被完全抑制。动力学色散方程表明,离子-离子碰撞和电子-离子碰撞效应是抑制不稳定性发展的主要因素。对色散方程的计算表明,离子-离子碰撞是抑制不稳定性发展的主要因素。
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