2D ferromagnetic (FM) semiconductors/half-metals offer promising prospects for quantum information technologies in miniature devices. However, the low Curie temperature (TC) severely limits their application in spintronic devices. Here, two stable FM transition metal chalcogenides, Ti3S2X2 (X = Se, Te) monolayers, based on first-principles calculations are presented. It is found that the Ti3S2Se2 monolayer is a bipolar magnetic semiconductor with an indirect bandgap of 0.094 eV, while Ti3S2Te2 exhibits be FM half-metallic feature. Notably, the TCs of Ti3S2Se2 monolayer and Ti3S2Te2 monolayer are 641 and 408 K, respectively, much higher than room temperature. Moreover, the TCs and electronic properties of both Ti3S2X2 (X = Se, Te) monolayers can be modulated by applying biaxial strains. These promising properties make Ti3S2X2 (X = Se, Te) monolayers ideal candidates for 2D spintronic devices.
二维铁磁半导体/半金属为量子信息技术在微型器件中的应用提供了广阔的前景。然而,低居里温度严重限制了它们在自旋电子器件中的应用。本文提出了基于第一性原理计算的两种稳定的FM过渡金属硫族化合物Ti3S2X2 (X = Se, Te)单层。结果表明,Ti3S2Se2为双极磁性半导体,间接带隙为0.094 eV, Ti3S2Te2具有FM半金属特征。值得注意的是,Ti3S2Se2单层和Ti3S2Te2单层的TCs分别为641 K和408 K,远高于室温。此外,两种Ti3S2X2 (X = Se, Te)单层的TCs和电子性能都可以通过施加双轴应变来调节。这些有希望的性质使Ti3S2X2 (X = Se, Te)单层膜成为二维自旋电子器件的理想候选者。
{"title":"Robust Ferromagnetism with High Curie Temperature in 2D Tri-Layer Ti3S2X2 (X = Se/Te) Monolayer","authors":"Zijin Wang, Jinlian Lu, Xiaojing Yao, Xiuyun Zhang","doi":"10.1002/qute.202500383","DOIUrl":"https://doi.org/10.1002/qute.202500383","url":null,"abstract":"<p>2D ferromagnetic (FM) semiconductors/half-metals offer promising prospects for quantum information technologies in miniature devices. However, the low Curie temperature (<i>T<sub>C</sub></i>) severely limits their application in spintronic devices. Here, two stable FM transition metal chalcogenides, Ti<sub>3</sub>S<sub>2</sub>X<sub>2</sub> (X = Se, Te) monolayers, based on first-principles calculations are presented. It is found that the Ti<sub>3</sub>S<sub>2</sub>Se<sub>2</sub> monolayer is a bipolar magnetic semiconductor with an indirect bandgap of 0.094 eV, while Ti<sub>3</sub>S<sub>2</sub>Te<sub>2</sub> exhibits be FM half-metallic feature. Notably, the <i>T<sub>C</sub></i>s of Ti<sub>3</sub>S<sub>2</sub>Se<sub>2</sub> monolayer and Ti<sub>3</sub>S<sub>2</sub>Te<sub>2</sub> monolayer are 641 and 408 K, respectively, much higher than room temperature. Moreover, the <i>T<sub>C</sub></i>s and electronic properties of both Ti<sub>3</sub>S<sub>2</sub>X<sub>2</sub> (X = Se, Te) monolayers can be modulated by applying biaxial strains. These promising properties make Ti<sub>3</sub>S<sub>2</sub>X<sub>2</sub> (X = Se, Te) monolayers ideal candidates for 2D spintronic devices.</p>","PeriodicalId":72073,"journal":{"name":"Advanced quantum technologies","volume":"8 11","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-09-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145521498","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Periodically driving a quantum many-body system can drastically change its properties, leading to exotic non-equilibrium states of matter without a static analog. In this scenario, parametric resonances and the complexity of an interacting many-body system are pivotal in establishing non-equilibrium states. A Floquet-engineered transverse field Ising model for the controlled propagation in one dimension of spin waves is reported. The underlying mechanisms behind the proposal rely on high-frequency drivings using characteristic parametric resonances of the spin lattice. Many-body resonances modulating spin-spin exchange or individual spin gaps inhibit interactions between spins thus proving a mechanism for controlling spin-wave propagation and a quantum switch. The schemes may be implemented in circuit QED with direct applications in coupling–decoupling schemes for system-reservoir interaction and routing in quantum networks.
{"title":"Floquet-Engineered System-Reservoir Interaction in the Transverse Field Ising Model","authors":"Maritza Ahumada, Natalia Valderrama-Quinteros, Guillermo Romero","doi":"10.1002/qute.202500031","DOIUrl":"https://doi.org/10.1002/qute.202500031","url":null,"abstract":"<p>Periodically driving a quantum many-body system can drastically change its properties, leading to exotic non-equilibrium states of matter without a static analog. In this scenario, parametric resonances and the complexity of an interacting many-body system are pivotal in establishing non-equilibrium states. A Floquet-engineered transverse field Ising model for the controlled propagation in one dimension of spin waves is reported. The underlying mechanisms behind the proposal rely on high-frequency drivings using characteristic parametric resonances of the spin lattice. Many-body resonances modulating spin-spin exchange or individual spin gaps inhibit interactions between spins thus proving a mechanism for controlling spin-wave propagation and a quantum switch. The schemes may be implemented in circuit QED with direct applications in coupling–decoupling schemes for system-reservoir interaction and routing in quantum networks.</p>","PeriodicalId":72073,"journal":{"name":"Advanced quantum technologies","volume":"8 11","pages":""},"PeriodicalIF":4.3,"publicationDate":"2025-09-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145529887","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Quantum secret sharing (QSS) plays a crucial role in quantum cryptography as a privacy preserving scheme. Designing an efficient QSS protocol requires addressing three key challenges: 1) dynamic agent membership (handling agents joining or leaving during execution), 2) adversarial resilience (ensuring robustness against dishonest agents), and 3) practical optimization (improving computational and communication efficiency while minimizing implementation cost). In this paper, a verifiable dynamic