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Analyzing Surface Plasmon Resonance as a Bio-Sensor through Simulating 表面等离子体共振作为生物传感器的仿真分析
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-07-24 DOI: 10.1007/s11468-025-03181-3
Ali H.Attallah, Saja A. Ibrahim, Farah. J. Kadhum, Ali A. Dawood Al-Zuky

In this study, a theoretical model for a surface plasmon resonance (SPR) sensor was developed using the transfer matrix method (TMM) to simulate and analyze reflectivity as a function of the angle of incidence in a multilayer system. This system consists of a gold layer with a fixed thickness, followed by a layer of SnSe with variable thicknesses within a defined range, and then a thin layer of MoS₂, using water as a biorecognition medium. The study focused on examining the effects of changes in the thickness of the SnSe layer and the wavelength within the range (690 to 1000 nm), as well as the effect of variations in the refractive index of the sensing medium due to contamination. Through numerical simulation, the properties of plasmonic resonance such as the reflection angle, SPR dip width, and SPR dip length were evaluated, along with sensor sensitivity. The sensor response was also analyzed when the refractive index of the sensitive medium changed slightly, reflecting the presence of contaminants, with the aim of studying the sensor’s ability to distinguish between different conditions. The addition of the SnSe layer has proven effective in improving the coupling of the evanescent wave with the sensitive medium, significantly enhancing the sensitivity of the device. A sensitivity of approximately 200°/RIU was achieved at wavelengths of 800 nm and 900 nm with thicknesses of 10 and 60 nm. These results reflect the effectiveness of the proposed design for use in high-precision sensing applications.

本文采用传递矩阵法(TMM)建立了表面等离子体共振(SPR)传感器的理论模型,模拟并分析了反射率随入射角的变化规律。该系统以水为生物识别介质,首先是厚度固定的金层,然后是一定范围内厚度可变的SnSe层,最后是薄薄的MoS 2层。研究重点考察了在690 ~ 1000nm范围内SnSe层厚度和波长变化的影响,以及受污染的传感介质折射率变化的影响。通过数值模拟,评估了等离子体共振的反射角、SPR倾角宽度和SPR倾角长度等特性以及传感器的灵敏度。还分析了当敏感介质的折射率发生轻微变化时,传感器的响应,反映了污染物的存在,目的是研究传感器区分不同条件的能力。事实证明,SnSe层的加入有效地改善了倏逝波与敏感介质的耦合,显著提高了器件的灵敏度。在波长为800 nm和900 nm,厚度为10 nm和60 nm时,灵敏度约为200°/RIU。这些结果反映了所提出的设计在高精度传感应用中的有效性。
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引用次数: 0
A Proposal for Detecting Fuel Adulteration Using Black Phosphorous-Enhanced Tamm Plasmon Polariton Sensor 一种利用黑磷增强Tamm等离子体激元传感器检测燃料掺假的方案
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-07-24 DOI: 10.1007/s11468-025-03184-0
Abinash Panda, Mahmood Basil A. AL-Rawi, Ahmed Zohier Ahmed Elhendi, Mostafa R. Abukhadra, Wail Al Zoubi, Hussein A. Elsayed, Ahmed Mehaney

This works presents a Tamm plasmon polariton (TPP)-based sensor for the identification of the degree of adulteration in petrol. The proposed structure is designed by integrating black phosphorous (BP) with 1D photonic crystal (PhC), where the PhC is realized with an alternate stacking of TiO2 and SiO2. A defect layer is sandwiched between BP and PhC, which is filled with various concentrations of adulterated petrol for sensing purpose. The reflectance spectrum of the sensor is investigated by employing well-known transfer matrix method. The sensing principle is based on the analysis of the shift in the TPP mode wavelength with respect to different percentages of adulteration. The geometrical parameters like thickness of different layers and period of the PhC are suitably optimized to attain maximum performance. The significance of BP is studied and compared with the conventional metal for the generation of TPP mode. Furthermore, the electric field distribution is investigated in the structure. Simulation outcomes show a maximum sensitivity of 4900 nm/RIU, maximum quality factor of 151.42, and minimum detection limit of (1.27times10^{-4}) RIU are achieved with the designed sensor, which proves its potential applications in petrochemical industry.

本文提出了一种基于Tamm等离子体激元(TPP)的传感器,用于识别汽油中的掺假程度。所提出的结构是通过将黑磷(BP)与一维光子晶体(PhC)集成来设计的,其中PhC是通过TiO2和SiO2的交替堆叠来实现的。在BP和PhC之间夹着一层缺陷层,其中填充了不同浓度的掺假汽油,用于检测目的。利用众所周知的传递矩阵法对传感器的反射光谱进行了研究。传感原理是基于对TPP模式波长相对于不同掺假百分比的位移的分析。对不同层的厚度和周期等几何参数进行了适当优化,以获得最佳性能。研究了BP对TPP模式生成的意义,并与常规金属进行了比较。进一步研究了结构中的电场分布。仿真结果表明,该传感器的最大灵敏度为4900 nm/RIU,最大品质因子为151.42,最小检测限为(1.27times10^{-4}) RIU,证明了该传感器在石油化工领域的潜在应用前景。
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引用次数: 0
Optical Bistability in a Nanodimer Made of Two Graphene-Coated Nanoparticles with a Molecule Situated in the Gap Region 由两个石墨烯包覆的纳米二聚体和一个位于间隙区的分子组成的光学双稳定性
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-07-24 DOI: 10.1007/s11468-025-03122-0
Milad Jalilian, Nader Daneshfar, Ali Bahari

In the present work, we theoretically investigate the optical bistability in a dimer consisting of two graphene-coated dielectric nanoparticles with a single molecule placed in the gap region. Assuming this system is exposed to an electromagnetic field, by solving Laplace’s equation in the quasi-static approximation, we obtain the local electric fields in different regions of the proposed system. The results show that the presence of molecule in the gap of dimer significantly affects the bistable behavior and leads to changes in the bistability thresholds and hysteresis loop compared to the dimer without the molecule. Furthermore, we explore the effects of nanoparticle asymmetry and the molecule dipole moment on the bistable response. We found that by increasing the degree of asymmetry, where the two nanoparticles differ in size, the bistability region will be increased and broadened. However, these findings may find practical potential applications in nanophotonic and optoelectronic devices.

在目前的工作中,我们从理论上研究了由两个石墨烯涂层的介电纳米粒子组成的二聚体的光学双稳定性,其中一个分子放置在间隙区域。假设系统暴露在电磁场中,通过求解拟静态近似下的拉普拉斯方程,得到了系统不同区域的局部电场。结果表明,与不含分子的二聚体相比,二聚体间隙中分子的存在显著影响了双稳态行为,导致双稳态阈值和滞回线的变化。此外,我们还探讨了纳米粒子的不对称性和分子偶极矩对双稳态响应的影响。我们发现,通过增加两种纳米颗粒大小不同的不对称程度,双稳区将增加和拓宽。然而,这些发现可能会在纳米光子和光电子器件中找到实际的潜在应用。
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引用次数: 0
Enhanced Surface Plasmon Resonance Detection of Ascorbic Acid Using Carbon Quantum Dots Thin Film 利用碳量子点薄膜增强表面等离子体共振检测抗坏血酸
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-07-23 DOI: 10.1007/s11468-025-03194-y
Wan Mohd Ebtisyam Mustaqim Mohd Daniyal, Yap Wing Fen, Muhamad Zamri Kariming, Nurul Illya Muhamad Fauzi, Hazwani Suhaila Hashim, Muhammad Fahmi Anuar, Ferry Anggoro Ardy Nugroho, Nurul Hidayat, Huda Abdullah, Ahmad Taufiq, Faten Bashar Kamal Eddin

This research investigates the structural and optical properties of carbon quantum dots (CQDs) for the sensitive detection of ascorbic acid (AA), an essential biomolecule used widely in health and industry. Accurate AA detection is critical for pharmaceutical and food safety applications, and this study demonstrates the use of a prism-based surface plasmon resonance (SPR) sensor with a CQD thin film for label-free and real-time monitoring. CQDs were deposited onto a gold (Au) thin film, and their structural properties were characterized through Fourier transform infrared spectroscopy (FTIR) and atomic force microscopy (AFM). FTIR analysis confirmed the presence of C–H, C≡C, C–N, and C–O bonds on the Au/CQDs surface, while AFM characterization revealed that the CQDs formed a uniformly dispersed, spiky surface evenly distributed across the gold layer. The optical properties of the Au/CQDs thin film were studied using ultraviolet–visible (UV–Vis) spectroscopy, showing an absorption peak of approximately 4.44 a.u. in the range of 260–270 nm, with an optical bandgap of 4.072 eV. When integrated into the SPR sensor, the Au/CQDs thin film demonstrated high sensitivity for AA detection, achieving a detection limit as low as 0.001 µM. Further characterization was conducted to explore the interaction between the Au/CQD thin film and AA, highlighting the film’s potential for use in sensitive biochemical sensing applications.

本研究研究了碳量子点(CQDs)的结构和光学性质,用于抗坏血酸(AA)的灵敏检测,AA是一种广泛应用于健康和工业的重要生物分子。准确的AA检测对于制药和食品安全应用至关重要,本研究展示了使用基于棱镜的表面等离子体共振(SPR)传感器与CQD薄膜进行无标签和实时监测。将CQDs沉积在金(Au)薄膜上,通过傅里叶变换红外光谱(FTIR)和原子力显微镜(AFM)对其结构性质进行了表征。FTIR分析证实了Au/CQDs表面存在C - h, C≡C, C - n和C - o键,而AFM表征显示CQDs形成了均匀分散的尖状表面,均匀分布在金层上。利用紫外-可见(UV-Vis)光谱研究了Au/CQDs薄膜的光学性质,在260 ~ 270 nm范围内的吸收峰约为4.44 a.u.,光带隙为4.072 eV。当集成到SPR传感器中时,Au/CQDs薄膜对AA检测具有高灵敏度,检测限低至0.001µM。进一步的表征是为了探索Au/CQD薄膜与AA之间的相互作用,强调了薄膜在敏感生化传感应用中的潜力。
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引用次数: 0
Ionic Plasmon-Polaritons in Neural Signaling II: Control Role of the Myelin over Frequency and Speed of Stimulus in Axons 离子等离子体-极化子在神经信号传导中的作用II:髓磷脂对轴突刺激频率和速度的控制作用
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-07-23 DOI: 10.1007/s11468-025-03212-z
Janusz Jacak, Witold Jacak

This work presents a mechanism for controlling stimulus speed within the plasmon-polariton model of fast stimulus kinetics during saltatory conduction in myelinated axons. Myelin thickness plays a crucial role, but the related mechanism differs from that in the conventional cable model. The thickness of the myelin sheath precisely tunes the plasmon-polariton frequency and the associated signal velocity. This frequency is limited by the timescale of triggering the opening of sodium channels at the nodes of Ranvier, allowing for the initiation of the Huxley-Hodgkin cycles. Synchronization of the plasmon-polariton stimulus frequency with these cycles at consecutive nodes of Ranvier ensures the balance of Ohmic losses and enables arbitrarily long-range axon firing. The myelin layer thickness assessed by the model, considering the molecular structure of sodium channels, is consistent with observations. This model of plasmon-polariton stimulus control in myelinated axons completes the theory of saltatory conduction presented in Ionic Plasmon-Polaritons in Neural Signaling I: Structure and Dynamics of Plasmon-Polaritons in Myelinated Axons, Plasmonics 20, 4195-4220 (2025), https://doi.org/10.1007/s11468-024-02694-7.

本研究提出了一种控制刺激速度的机制,该机制在有髓鞘轴突跃传导过程中的快速刺激动力学的等离子体-极化子模型中。髓鞘厚度起着至关重要的作用,但相关机制与传统的电缆模型不同。髓鞘的厚度精确地调节等离子激子的频率和相关的信号速度。这个频率受到触发朗维耶节点上钠通道打开的时间尺度的限制,从而允许赫胥黎-霍奇金循环的开始。在连续的Ranvier节点上,等离子体-极化激子刺激频率与这些周期的同步确保了欧姆损耗的平衡,并使任意远距离的轴突放电成为可能。考虑到钠通道的分子结构,模型评估的髓磷脂层厚度与观察结果一致。有髓鞘轴突中等离子激元刺激控制模型完善了《神经信号中的离子等离子激元:有髓鞘轴突中等离子激元的结构和动力学》中提出的跃变传导理论,《等离子体动力学》20,4195-4220 (2025),https://doi.org/10.1007/s11468-024-02694-7。
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引用次数: 0
Antibody-Functionalized Gold Nanoparticles for Sensitive Detection of Tetanus Toxoid 抗体功能化金纳米颗粒用于破伤风类毒素的灵敏检测
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-07-23 DOI: 10.1007/s11468-025-02873-0
Pardis Saeedi, Hamideh Rouhani Nejad

Clostridium tetani produce a potent neuro toxoid as tetanus toxoid, which elicits spastic paralysis in humans and warm-blooded animals. Tetanus recognition is crucial; however, existing diagnostic methods have notable limitations. Recently, the localized surface plasmon resonance (LSPR) nano-bio-probe has been established as a promising technique for detecting Clostridium tetani toxoid. The designed nanobioprobe utilizes covalent conjugation between monoclonal anti-tetanus IgG antibodies and gold nanoparticles (GNPs). The dynamic light scattering (DLS) technique was employed to verify successful conjugation. Subsequently, the sensitivity of the LSPR was assessed as a function of tetanus toxoid concentration using a colorimetric assay. The results demonstrated that the LSPR band of functionalized GNPs exhibited a redshift from 530 to 563 nm in the presence of 1 ng of tetanus toxoid, outperforming the ELISA method. This study presents a rapid, sensitive, and selective approach for tetanus toxoid detection in clinical samples.

破伤风梭菌产生一种强效的神经类毒素,如破伤风类毒素,可引起人类和温血动物的痉挛性麻痹。破伤风的识别至关重要;然而,现有的诊断方法有明显的局限性。近年来,局部表面等离子体共振(LSPR)纳米生物探针被认为是一种很有前途的检测破伤风梭菌类毒素的技术。所设计的纳米探针利用单克隆抗破伤风IgG抗体与金纳米颗粒(GNPs)之间的共价偶联。采用动态光散射(DLS)技术验证了共轭的成功。随后,使用比色法评估LSPR的灵敏度作为破伤风类毒素浓度的函数。结果表明,在1 ng破伤风类毒素存在下,功能化GNPs的LSPR波段出现530 ~ 563nm的红移,优于ELISA法。本研究提出了一种快速、灵敏、选择性的破伤风类毒素检测方法。
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引用次数: 0
Machine Learning-Enhanced MXene–Copper–Graphene THz Sensor for Accurate Salinity Sensing in Environmental Applications 机器学习增强的mxene -铜-石墨烯太赫兹传感器用于环境应用中的精确盐度传感
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-07-23 DOI: 10.1007/s11468-025-03222-x
Jagannathan Jayachandran, V. Sivakumar, Vijayalakshmi K, Ngaira Mandela

This study presents a novel terahertz metasurface biosensor incorporating graphene-MXene hybrid materials for enhanced salinity detection across environmental and industrial applications. The sensor features a multilayered architecture with three copper-coated rectangular resonators, concentric MXene-coated circular ring resonators, and a graphene-integrated circular base resonator on a silicon dioxide substrate. Numerical simulations using COMSOL Multiphysics demonstrated tunable electromagnetic response through graphene chemical potential modulation (0.1–0.9 eV) and maintained stable performance across incident angles up to 60°. The optimized sensor achieved a sensitivity of 286 GHz/RIU with a figure of merit of 3.247 RIU⁻1, quality factor of 4.398, and detection limit of 0.022 RIU across a refractive index range of 1.3325–1.3505. Experimental validation showed strong correlation (R2 = 0.80) between theoretical and measured absorption values. The proposed biosensor addresses critical limitations of conventional conductivity-based sensors, offering superior performance in high-salinity and turbid environments while providing real-time monitoring capabilities essential for oceanography, aquaculture, agriculture, and desalination applications.

本研究提出了一种新型的太赫兹超表面生物传感器,结合石墨烯- mxene混合材料,用于增强环境和工业应用中的盐度检测。该传感器具有多层结构,包括三个铜涂层矩形谐振器,同心mxene涂层圆形环形谐振器,以及二氧化硅衬底上的石墨烯集成圆形基谐振器。使用COMSOL Multiphysics进行的数值模拟表明,通过石墨烯化学势调制(0.1-0.9 eV),电磁响应可调谐,并且在60°入射角范围内保持稳定性能。优化后的传感器在1.3325-1.3505折射率范围内的灵敏度为286 GHz/RIU,品质系数为3.247 RIU⁻1,质量因子为4.398,检测限为0.022 RIU。实验验证表明理论吸收值与实测吸收值之间具有很强的相关性(R2 = 0.80)。提出的生物传感器解决了传统电导率传感器的关键局限性,在高盐度和浑浊环境中提供卓越的性能,同时为海洋学、水产养殖、农业和海水淡化应用提供必要的实时监测能力。
{"title":"Machine Learning-Enhanced MXene–Copper–Graphene THz Sensor for Accurate Salinity Sensing in Environmental Applications","authors":"Jagannathan Jayachandran,&nbsp;V. Sivakumar,&nbsp;Vijayalakshmi K,&nbsp;Ngaira Mandela","doi":"10.1007/s11468-025-03222-x","DOIUrl":"10.1007/s11468-025-03222-x","url":null,"abstract":"<div><p>This study presents a novel terahertz metasurface biosensor incorporating graphene-MXene hybrid materials for enhanced salinity detection across environmental and industrial applications. The sensor features a multilayered architecture with three copper-coated rectangular resonators, concentric MXene-coated circular ring resonators, and a graphene-integrated circular base resonator on a silicon dioxide substrate. Numerical simulations using COMSOL Multiphysics demonstrated tunable electromagnetic response through graphene chemical potential modulation (0.1–0.9 eV) and maintained stable performance across incident angles up to 60°. The optimized sensor achieved a sensitivity of 286 GHz/RIU with a figure of merit of 3.247 RIU⁻<sup>1</sup>, quality factor of 4.398, and detection limit of 0.022 RIU across a refractive index range of 1.3325–1.3505. Experimental validation showed strong correlation (R<sup>2</sup> = 0.80) between theoretical and measured absorption values. The proposed biosensor addresses critical limitations of conventional conductivity-based sensors, offering superior performance in high-salinity and turbid environments while providing real-time monitoring capabilities essential for oceanography, aquaculture, agriculture, and desalination applications.</p></div>","PeriodicalId":736,"journal":{"name":"Plasmonics","volume":"20 12","pages":"11349 - 11359"},"PeriodicalIF":4.3,"publicationDate":"2025-07-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145802530","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ultra-sensitive D-Type PCF-SPR Biosensor with Dual-layer Au/TiO₂ Coating for Early Cancer Cell Detection 基于Au/TiO 2双层涂层的超灵敏d型PCF-SPR生物传感器用于早期癌细胞检测
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-07-23 DOI: 10.1007/s11468-025-03185-z
Yuan Sun, Jingwei Lv, Famei Wang, Wei Liu, Jianxin Wang, Zao Yi, Miao Liu, Qiang Liu, Paul K. Chu, Chao Liu

A highly sensitive D-type photonic crystal fiber (PCF) sensor based on surface plasmon resonance (SPR) is proposed for the detection of cancer cells through refractive index (RI) monitoring. The sensor features a semicircular groove on the polished surface, coated with dual layers of gold (Au) and titanium dioxide (TiO₂) to enhance plasmonic coupling. Finite element method (FEM) analysis shows that the sensor has a refractive index range, maximum wavelength sensitivity, and resolution of 1.355–1.395, 54,000 nm/RIU, and 1.85 × 10−6 RIU, respectively, boding well for the early screening of cancer cells with a sensitivity in the range of 2500–24,285 nm/RIU. The compact sensor comprising a standard single-mode fiber with an outer diameter of 125 μm can be produced easily and has large application prospects in fields such as biomedical diagnosis, disease screening, and environmental detection.

提出了一种基于表面等离子体共振(SPR)的高灵敏度d型光子晶体光纤(PCF)传感器,用于通过监测折射率(RI)来检测癌细胞。该传感器在抛光表面上有一个半圆形凹槽,并涂有双层金(Au)和二氧化钛(TiO 2),以增强等离子体耦合。有限元分析表明,该传感器的折射率范围为1.355 ~ 1.395,最大波长灵敏度为54,000 nm/RIU,分辨率为1.85 × 10−6 RIU,灵敏度为2500 ~ 24,285 nm/RIU,有望用于肿瘤细胞的早期筛查。该传感器由外径为125 μm的标准单模光纤组成,制作简单,在生物医学诊断、疾病筛查、环境检测等领域具有广阔的应用前景。
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引用次数: 0
Design of a Silicon and Tantalum Diselenide-Based Multilayer Surface Plasmon Resonance Sensor for Early Detection of Skin Cancer 基于二硒化硅和钽的多层表面等离子体共振传感器用于皮肤癌早期检测的设计
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-07-22 DOI: 10.1007/s11468-025-03182-2
Bhishma Karki, Youssef Trabelsi, Amrindra Pal, Chethan M., Helen Merina Albert, Tapasmini Sahoo, Anita Gehlot

The present study designed a new surface plasmon resonance (SPR) sensor based on a BaF2 prism, silver (Ag), silicon (Si), and tantalum diselenide (TaSe2) 2D material structure for the detection of basal cells. The angular interrogation method allows us to evaluate the performance exponentially at 633 nm. The proposed sensor demonstrates improved sensitivity and accuracy and detects the basal cell uses. The sensor proposed has a maximum sensitivity of 337.47°/RIU, a detection accuracy (DA) of 0.254/°, and a figure of merit (FoM) of 85.87/RIU. The research indicates that the integration of Si and TaSe2 layers with traditional plasmonic metals can enhance sensitivity and provide a platform for further environmental monitoring and medical diagnostics.

本研究设计了一种基于BaF2棱镜、银(Ag)、硅(Si)和二硒化钽(TaSe2)二维材料结构的新型表面等离子体共振(SPR)传感器,用于检测基底细胞。角度询问法允许我们以指数方式评估633 nm的性能。所提出的传感器证明了提高的灵敏度和准确性,并检测基底细胞的用途。该传感器的最大灵敏度为337.47°/RIU,检测精度(DA)为0.254/°,品质因数(FoM)为85.87/RIU。研究表明,硅和TaSe2层与传统等离子体金属的集成可以提高灵敏度,并为进一步的环境监测和医学诊断提供平台。
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引用次数: 0
Graphene Ultraviolet Photoconductive Detector Enhanced by Plasmon Local Field with Sea-Urchin-Like Gold Structure 海胆样金结构等离激元局域场增强石墨烯紫外光导探测器
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-07-22 DOI: 10.1007/s11468-025-03201-2
Guangchen Yin, Kaixi Bi, Miaoli Guo, Cong Li, Donghui Huang, Hao Liu, Longhao Liu, Wenqi Xiong, Jialiang Chen, Huiqi Wang, Linyu Mei

Graphene has attracted much attention in the field of photodetection because of its unique properties such as extremely high carrier mobility and wide-spectrum optical absorption. However, graphene’s poor optical absorption limits its application. In this paper, based on the localized surface plasmon resonance (LSPR) effect of gold nanoparticles (AuNPs) can effectively improve the optical absorption of graphene, we synthesized urchin-like gold nanoparticles with stronger LSPR and prepared gold nanoparticles/graphene (AuNPs/Gr) and graphene (Gr) two kinds of photoelectric detector (PD). AuNPs can produce strong LSPR effect under light to generate hot electrons, which can easily enter into the conduction band of Gr, enhancing the responsivity of graphene. At 365 nm wavelength 5 V bias, the photocurrent of the AuNPs/Gr PD is about 36.91 (mu A), which is 3.5 times higher than the 10.48 (mu A) of the Gr PD. At 365 nm wavelength 1.05 (text{mW}/{text{cm}}^{2}) incident optical power density, with the enhancement of urchin-like AuNPs, the responsivity of AuNPs/Gr PD was increased to 5.02 (text{mA}/text{W}), and the specific detectivity was increased to 1.71 × 108 Jones, which was more than eight times higher than the Gr PD. This work provides a simple method for enhancing PD performances using metal nanoparticles.

石墨烯具有极高的载流子迁移率和广谱光吸收等特性,在光电探测领域受到广泛关注。然而,石墨烯较差的光学吸收限制了它的应用。本文基于金纳米粒子(AuNPs)的局部表面等离子体共振(LSPR)效应能有效提高石墨烯的光学吸收,合成了具有更强LSPR的类海胆金纳米粒子,并制备了金纳米粒子/石墨烯(AuNPs/Gr)和石墨烯(Gr)两种光电探测器(PD)。AuNPs在光照下可以产生很强的LSPR效应,产生热电子,热电子很容易进入Gr的导带,增强了石墨烯的响应性。在365 nm波长5 V偏置下,AuNPs/Gr PD的光电流约为36.91 (mu A),是Gr PD的10.48 (mu A)的3.5倍。在365 nm波长1.05 (text{mW}/{text{cm}}^{2})入射光功率密度下,随着海胆样AuNPs的增强,AuNPs/Gr PD的响应率提高到5.02 (text{mA}/text{W}),比探测率提高到1.71 × 108 Jones,比Gr PD提高了8倍多。这项工作为利用金属纳米颗粒增强PD性能提供了一种简单的方法。
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引用次数: 0
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