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Broadband Terahertz Detection in Dual-Side Gated Graphene 双侧门控石墨烯中的宽带太赫兹探测
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-02 DOI: 10.1007/s11468-025-03067-4
Songbin Meng, Nianjia Zhang, Xiaokai Pan, Huiping Zhang, Anqi Yu, Xin Sun, Yiming Wang, Yichong Zhang, Yinghao Yuan, Yongni Shao, Alexei V. Balakin, Alexander P. Shkurinov, YiMing Zhu

In this work, we fabricated graphene terahertz detectors with dual-side metallic gate. Detectors using only one set of gates showed a monotonic change in responsivity as gate voltage changed, with a peak value of ~ 12 V/W within 0.1 THz, and no distinguishable response above 0.1 THz. The dominating mechanism was found to be the photo-thermoelectric (PTE) effect. Detectors using multiple sets of gates showed monotonic and non-monotonic change in responsivity as gate voltage changed, with peak responsivity of 462 V/W at 0.082 THz and 198 V/W at 2.52 THz. In the frequency ranges where the responsivity changed monotonically, the dominating mechanism was found to be the PTE effect for frequencies. In the frequency ranges where responsivity changed non-monotonically, the dominating mechanism was found to alternate between the plasmon rectification effect and the PTE effect at different gate voltage. The excitation of graphene plasmons promised non-degrading responsivity below 0.105 THz and at 2.52 THz.

在这项工作中,我们制作了双面金属栅极的石墨烯太赫兹探测器。仅使用一组栅极的探测器随着栅极电压的变化响应性呈单调变化,在0.1 THz内峰值为~ 12 V/W,在0.1 THz以上无明显响应。主要机理是光热电(PTE)效应。采用多组栅极的探测器响应率随栅极电压变化呈现单调和非单调变化,在0.082 THz时峰值响应率为462 V/W,在2.52 THz时峰值响应率为198 V/W。在响应度单调变化的频率范围内,发现主导机制是频率的PTE效应。在响应性非单调变化的频率范围内,发现在不同栅极电压下,等离子体整流效应和PTE效应交替起主导作用。在0.105 THz和2.52 THz下,石墨烯等离子激元的激发保证了不退化的响应率。
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引用次数: 0
Innovative Sensor Based on Photonic Crystal Fiber for Efficient Determination of Various Explosives 基于光子晶体光纤的新型爆炸物检测传感器
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-01 DOI: 10.1007/s11468-025-03038-9
Malek G. Daher, Adam R. H. Alhawari, Abdulkarem H. M. Almawgani, Yousif S. Adam, Mahmoud M. M. Abu Hasanein, Hussein S. Gumaih, Shivam Singh, Rajeev Kumar

Today, the advancement of suitable detectors for quick and precise discovery of explosives is a serious necessity for numerous safety and security purposes. Here, a novel trend is presented that employs a photonic crystal fiber device (PCFD) structure for the recognition of various explosives including nitroglycerin explosive (NGE), trinitrotoluene explosive (TTE), and royal demolition explosive (RDE). COMSOL Multiphysics software is employed and the finite element technique is operated to analyze the functioning of the offered PCFD. In the offered PCFD, we struggled to cover the whole fiber zone to exhaust the greatest volume of the incident waves which will boost the performance of the advanced PCFD. With ultra-high relative sensitivity of chosen explosives containing NGE (99.107), TTE (99.556), and RDE (95.940%), the offered PCFD demonstrates its extraordinary aptitudes. Furthermore, the suggested PCFD provides very low confinement loss and effective material loss values, which means tiny loss can happen. These characteristics emphasize its capability to accurately determine even the most slight modifications in the refractive index for the tested samples.

今天,为快速和精确地发现爆炸物而研制合适的探测器是许多安全和安保目的的迫切需要。本文提出了利用光子晶体光纤器件(PCFD)结构对硝酸甘油炸药(NGE)、三硝基甲苯炸药(TTE)、皇室爆破炸药(RDE)等多种炸药进行识别的新趋势。采用COMSOL Multiphysics软件,运用有限元技术对所提供的PCFD进行功能分析。在提供的PCFD中,我们努力覆盖整个光纤区域,以排出最大体积的入射波,这将提高先进PCFD的性能。对于所选的含有NGE(99.107)、TTE(99.556)和RDE(95.940%)的炸药具有超高的相对灵敏度,所提供的PCFD显示了其非凡的能力。此外,所建议的PCFD提供非常低的约束损耗和有效材料损耗值,这意味着可以发生微小的损耗。这些特点强调了它的能力,以准确地确定即使是最轻微的变化,在折射率的测试样品。
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引用次数: 0
Molecular Recognition of Breast Cancer Biomarkers via Localized Surface Plasmon Resonance Method 基于局部表面等离子体共振方法的乳腺癌生物标志物分子识别
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-05-31 DOI: 10.1007/s11468-025-03072-7
Faride Ranjbari, Yasamin Pahlavan, Masoud Khalifezadeh, Mehdi Fathi, Seyed Hossein Khaleghinejad, Hamideh Imanzadeh, Maryam Saberi, Farzaneh Fathi

Breast cancer, a prevalent malignancy worldwide, necessitates the development of highly sensitive and specific diagnostic tools for early detection and personalized treatment. Biomarkers include routine or ordinary, novel, and potential biomolecules consisting of nucleic acids (DNA/RNA), key proteins, genes, and intact cells. Advances in biotechnology and molecular medicine have led to the identification of biomarkers for early diagnosis and therapeutic intervention, particularly through the development of novel biosensors, which hold significant clinical value. In this review article, we first present the main biomarkers involved in breast cancer. Then, the mechanism and different types of SPR techniques including traditional SPR, growth-mediated SPR, etching, and SPR imaging technologies are introduced. Furthermore, we explore various localized SPR (LSPR) biosensor designs, surface functionalization strategies, and signal transduction methods used for breast cancer biomarker detection. This review specifically mentions LSPR sensor designs, surface functionalization strategies, and signal transduction methods, indicating a focus on specific and innovative approaches within the SPR technology. We examine the performance characteristics of these biosensors, including their detection limits and selectivity, and discuss their potential for clinical translation.

Graphical Abstract

乳腺癌是一种世界范围内普遍存在的恶性肿瘤,需要开发高度敏感和特异性的诊断工具,以便早期发现和个性化治疗。生物标志物包括由核酸(DNA/RNA)、关键蛋白、基因和完整细胞组成的常规或普通、新型和潜在的生物分子。生物技术和分子医学的进步导致了早期诊断和治疗干预的生物标志物的识别,特别是通过开发具有重要临床价值的新型生物传感器。在这篇综述文章中,我们首先介绍了与乳腺癌有关的主要生物标志物。然后,介绍了不同类型的SPR技术,包括传统的SPR、生长介导的SPR、蚀刻和SPR成像技术。此外,我们探索了用于乳腺癌生物标志物检测的各种本地化SPR (LSPR)生物传感器设计,表面功能化策略和信号转导方法。这篇综述特别提到了LSPR传感器的设计、表面功能化策略和信号转导方法,表明了SPR技术中具体和创新方法的重点。我们研究了这些生物传感器的性能特征,包括它们的检测限和选择性,并讨论了它们在临床转化方面的潜力。图形抽象
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引用次数: 0
Antimonene, Barium Titanate and Silver Layer–Based Surface Plasmon Resonance Sensor for Dental Application: A Numerical Analysis 锑烯、钛酸钡和银层表面等离子体共振传感器在牙科中的应用:数值分析
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-05-31 DOI: 10.1007/s11468-025-03020-5
Mahmud Uz Zaman, Gufranullah Ansari, Arun Uniyal, Nasser Raqe Alqhtani, Amrindra Pal, Abdullah Saad Alqahtani, Harbinder Singh, Abdullah Bin Nabhan, Khalid Ayidh Alqahtani

One of the most promising techniques for the study of the optical properties of dental materials is the use of surface plasmon resonance (SPR). This optical phenomenon occurs when a monochromatic light beam is incident on a conductive metallic surface. Conventional terms include a prism with a thin film coating of a noble metal, e.g. gold or silver and a 2-dimensional or dielectric material. Interaction of the light metal leads to the oscillation of electrons in the conduction band, thus inducing SPR at the metal–dielectric interface. The phenomenon can be utilized to measure various optical parameters of teeth, e.g. sensitivity and reflectance. A prototype sensor was designed and tested to evaluate the parameters using MATLAB software in combination with the characteristic transfer matrix (CTM). Various performance parameters of interest to the sensor were studied, including a full width at half maximum (FWHM) of 6.266°, a sensitivity of 190.48° per refractive index unit (deg/RIU), a figure of merit of 30.401 RIU1, and detection accuracy of 0.159 degree⁻1. The results show that the proposed sensor is useful for biomedical applications.

表面等离子体共振(SPR)是研究牙科材料光学特性最有前途的技术之一。当单色光束入射到导电金属表面时,就会发生这种光学现象。传统术语包括具有贵金属(例如金或银)薄膜涂层和二维或介电材料的棱镜。轻金属的相互作用导致导电带中电子的振荡,从而在金属-介电界面处诱发SPR。这种现象可以用来测量牙齿的各种光学参数,如灵敏度和反射率。利用MATLAB软件,结合特征传递矩阵(CTM),设计并测试了传感器原型,对传感器参数进行了评估。对该传感器的各种性能参数进行了研究,包括半最大值全宽度(FWHM)为6.266°,每折射率单位(度/RIU)的灵敏度为190.48°,优点值为30.401 RIU - 1,检测精度为0.159度- 1。结果表明,该传感器可用于生物医学领域。
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引用次数: 0
Symmetry Breaking Induced Multiple Fano Resonances for Plasmonic Nanosensing 对称破缺诱导等离子体纳米传感的多范诺共振
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-05-31 DOI: 10.1007/s11468-025-03053-w
Haibo Geng, Zhouping Ni, Xinxin Ma, Tong Li, Yilin Wang, Zhao Chen

High-sensitivity plasmonic refractive index sensors play a crucial role in chemical and biological detection. In this work, we propose a novel and compact sensing structure composed of a MIM waveguide coupled with an asymmetric ellipsoidal resonator. Finite element simulations demonstrate that symmetry breaking in the structure enables the excitation of multiple sharp Fano resonances along with a distinct Lorentzian resonance, significantly enriching the spectral response. Compared with conventional symmetric resonator designs, the proposed structure offers three key advantages: (1) support for multiple narrow Fano modes; (2) independent tunability of both Fano and Lorentz peaks; and (3) directional and selective spatial field distributions of coupled modes, enhancing both sensitivity and resolution. By tuning the geometric parameters, precise control over resonance wavelengths is achieved, showing excellent tunability. The structure reaches a high refractive index sensitivity of ~ 1700 nm/RIU and the FOM up to 2.13 × 104. Furthermore, it exhibits pronounced spectral responses to variations in glucose and plasma concentrations, indicating strong potential for label-free biochemical sensing. This study provides a promising strategy for designing multi-channel, high-resolution plasmonic sensors and integrated photonic devices. 

高灵敏度等离子体折射率传感器在化学和生物检测中起着至关重要的作用。在这项工作中,我们提出了一种由MIM波导耦合非对称椭球腔组成的新颖紧凑的传感结构。有限元模拟表明,结构中的对称性破缺可以激发多个尖锐的法诺共振和一个明显的洛伦兹共振,显著丰富了光谱响应。与传统的对称谐振器设计相比,该结构具有三个主要优点:(1)支持多个窄Fano模式;(2) Fano峰和Lorentz峰的独立可调性;(3)耦合模式的定向和选择性空间场分布,提高了灵敏度和分辨率。通过调整几何参数,实现了对共振波长的精确控制,显示出优异的可调性。该结构具有~ 1700 nm/RIU的高折射率灵敏度,FOM高达2.13 × 104。此外,它对葡萄糖和血浆浓度的变化表现出明显的光谱响应,表明无标记生化传感的强大潜力。该研究为设计多通道、高分辨率等离子体传感器和集成光子器件提供了一种有前途的策略。
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引用次数: 0
Development of a Surface Plasmon Resonance Sensor using 2D Materials, Including Graphene and Black Phosphorus, for Measuring Water Pressure 利用石墨烯和黑磷等二维材料研制表面等离子体共振传感器,用于测量水压
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-05-31 DOI: 10.1007/s11468-025-03066-5
Ali Khodaie, Javad Javidan, Hamid Heidarzadeh

Understanding how the refractive index of water changes with wavelength under different physical and chemical conditions, such as temperature or pressure, is crucial for describing the behavior of light as it travels through, reflects from, and is absorbed by water. The refractive index can act as an in situ indicator of various physical properties of liquids, such as density and pressure. Research has highlighted the influence of pressure on the refractive index at specific visible wavelengths, emphasizing the need for further exploration of these relationships. This research presents a sophisticated surface plasmon resonance (SPR) optical sensor that integrates 2D materials into a Kretschmann setup. The sensor is structured with multiple layers, including a BK7 prism, gold (Au), black phosphorus (BP), and graphene. Its performance was assessed through the finite difference time domain (FDTD) method, allowing for an in-depth analysis of crucial parameters like sensitivity. At a wavelength of 633 nm, the sensor achieved outstanding performance, with a sensitivity of 174.61 deg/RIU and a figure of merit (FOM) of 26.36 RIU−1, surpassing earlier designs. These results demonstrate the sensor’s capability to measure liquid pressure, including that of water, by detecting changes in optical properties associated with varying pressures. The study shows that variations in the refractive index of water can be observed at pressures exceeding 100 or 250 MPa. Operating pressures up to 250 MPa are required for various applications, such as waterjet cutting of thick and hard materials.

了解水的折射率在不同的物理和化学条件下(如温度或压力)是如何随波长变化的,这对于描述光通过水、被水反射和被水吸收的行为至关重要。折射率可以作为液体的各种物理性质的原位指示器,如密度和压力。研究强调了压力对特定可见波长折射率的影响,强调了进一步探索这些关系的必要性。本研究提出了一种复杂的表面等离子体共振(SPR)光学传感器,该传感器将二维材料集成到Kretschmann装置中。该传感器由多层结构组成,包括BK7棱镜、金(Au)、黑磷(BP)和石墨烯。通过时域有限差分(FDTD)方法对其性能进行了评估,允许对灵敏度等关键参数进行深入分析。在633 nm波长处,该传感器的灵敏度为174.61°/RIU,性能值(FOM)为26.36 RIU−1,超过了早期的设计。这些结果证明了传感器通过检测与不同压力相关的光学特性变化来测量液体压力(包括水的压力)的能力。研究表明,在压力超过100或250兆帕时,可以观察到水的折射率变化。各种应用需要高达250mpa的工作压力,例如水射流切割厚而硬的材料。
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引用次数: 0
Terahertz Generation from Anharmonic Nanoparticles under Oblique Laser Excitation 斜激光激发下非谐波纳米粒子产生太赫兹
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-05-31 DOI: 10.1007/s11468-025-03058-5
Anuj Dandain, Shivani Vij, Niti Kant, Oriza Kamboj

This study presents an analytical investigation of terahertz (THz) generation from obliquely incident laser beams interacting with the anharmonic nanoparticles. The model incorporates the effects of nanoparticle density gradients, described by an exponential ramp profile, and the nonlinear response of nanoparticles. Numerical simulations were performed to analyze the influence of incidence angle, density gradient, interparticle spacing, and anharmonicity on THz amplitude. The results demonstrate a strong angular dependence of THz generation, with maximum amplitude at near-normal incidence. The THz amplitude decreases with the increasing slope parameter of the density ramp. The presence of a density ramp enhances THz generation. Smaller interparticle spacings result in higher THz amplitudes, emphasizing the importance of collective effects, while anharmonicity amplifies THz output by increasing the system’s nonlinearity. By exploring the effects of density gradients, inter-particle spacing, and anharmonicity, the model reveals broadband THz emission capabilities. The findings provide insights for optimizing the THz generation from nanoparticles by controlling these parameters and hold significant promise for applications in next-generation wireless communications (5 G/6 G), spectroscopic analysis, and non-invasive medical imaging, where efficient and broadband THz sources are crucial.

本文对斜入射激光束与非谐波纳米粒子相互作用产生的太赫兹(THz)进行了分析研究。该模型结合了纳米粒子密度梯度的影响,由指数斜坡曲线描述,以及纳米粒子的非线性响应。通过数值模拟分析了入射角、密度梯度、粒子间距和非谐性对太赫兹幅值的影响。结果表明太赫兹产生有很强的角依赖性,在接近正入射时振幅最大。太赫兹幅值随密度坡道斜率参数的增大而减小。密度斜坡的存在增强了太赫兹的产生。较小的粒子间距导致较高的太赫兹振幅,强调了集体效应的重要性,而非谐波通过增加系统的非线性来放大太赫兹输出。通过探索密度梯度、粒子间间距和非谐性的影响,该模型揭示了宽带太赫兹发射能力。该研究结果为通过控制这些参数来优化纳米颗粒产生太赫兹提供了见解,并对下一代无线通信(5g / 6g)、光谱分析和非侵入性医学成像的应用具有重要意义,在这些领域,高效和宽带太赫兹源至关重要。
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引用次数: 0
Grey Wolf Optimization Algorithm in Conjunction with the FDTD Method to Analyze the Nanostructure Predicated on a Plasmonic Demultiplexer 灰狼优化算法结合时域有限差分法分析等离子体解复用器的纳米结构
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-05-30 DOI: 10.1007/s11468-025-03016-1
Mohsen Nasrolahi, Ali Farmani, Ashkan Horri, Hossein Hatami

Plasmonics demultiplexers have several potential applications in military contexts, particularly due to their ability to manipulate light at the nanoscale and their advantages in communication and sensing technologies. Plasmonics demultiplexers represent a promising technology for military applications, enhancing communication, sensing, and intelligence capabilities. Their ability to operate at the nanoscale allows for more efficient and compact systems, which is crucial in modern military operations. As research and development in plasmonics continue to advance, their integration into military technologies could lead to significant improvements in operational effectiveness and security. Finite-difference time-domain (FDTD) as a numerical method is used to simulate the proposed plasmonic structure. This allows for the analysis of field distributions, resonance conditions, and coupling efficiencies. The applied Grey Wolf Optimization algorithm here involves updating the positions of wolves iteratively based on a mathematical equation-inspired optimized algorithm for a plasmonics demultiplexer that requires a multifaceted approach, combining simulation and design optimization. By leveraging advanced computational techniques and iterative design processes, it is possible to create highly efficient and effective plasmonic devices for a variety of applications in optical communication and sensing.

等离子体解复用器在军事环境中有几种潜在的应用,特别是由于它们在纳米尺度上操纵光的能力以及它们在通信和传感技术方面的优势。等离子体解复用器代表了一种很有前途的技术,用于军事应用,增强通信,传感和情报能力。它们在纳米尺度上的操作能力允许更高效和紧凑的系统,这在现代军事行动中至关重要。随着等离子体的研究和发展不断推进,它们与军事技术的整合可能会显著提高作战效率和安全性。采用时域有限差分法(FDTD)对所提出的等离子体结构进行了数值模拟。这允许分析场分布、共振条件和耦合效率。本文应用的灰狼优化算法涉及基于数学方程的等离子体解复用器优化算法迭代更新狼的位置,该算法需要多方面的方法,将仿真和设计优化相结合。通过利用先进的计算技术和迭代设计过程,可以为光通信和传感中的各种应用创建高效和有效的等离子体器件。
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引用次数: 0
Highly Sensitive and Self-Calibrating Fiber Optic SPR Methane Sensor Based on Graphene–MoS2 Heterostructure 基于石墨烯- mos2异质结构的高灵敏度自校准光纤SPR甲烷传感器
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-05-29 DOI: 10.1007/s11468-025-03046-9
Pengxiao Xu, Minghui Huo, Xiaokang Wang, Longyu Xu, Jingchao Bao, Aolin Hou, Yundong Liu, Xiaojian Meng, Kun Yu, Yufang Liu

Methane, a highly flammable and explosive gas, poses significant safety risks and challenges for industrial applications. A highly sensitive sensor based on surface plasmon resonance within a photonic crystal fiber is presented and fully analyzed. This sensor measures methane concentration while providing self-calibration. The photonic crystal fiber features a D-type structure with grooves, where composite two-dimensional material film and gold films are deposited. Additionally, a methane-sensitive layer containing cryptophane-A is coated on the surface of the D-type structure. The finite element method is utilized to analyze and compare the coating of different two-dimensional materials (graphene, MoS2, and graphene–MoS2) on the simulation analysis of sensor sensitivity. The use of graphene–MoS2 composite two-dimensional material not only enhances the sensing performance but also excites the double-peak effect. This double-peak effect enables the methane sensor to measure at different wavelengths, with the primary and secondary peaks calibrated against each other to improve the sensor's accuracy. The results show that the surface plasmon resonance based on photonic crystal fiber sensor with graphene–MoS2 composite membrane has better sensing performance. The maximum wavelength sensitivity and average wavelength sensitivity reached 80 and 63.4 nm/%, respectively, over the range of methane concentrations from 0.5 to 3.5%. These properties are significantly better than those of recently reported methane sensors. Therefore, the sensor has excellent application prospects in miniature methane detection field.

甲烷是一种高度易燃易爆的气体,对工业应用构成了重大的安全风险和挑战。提出了一种基于光子晶体光纤表面等离子体共振的高灵敏度传感器,并对其进行了分析。该传感器测量甲烷浓度,同时提供自校准。光子晶体光纤具有带凹槽的d型结构,在凹槽中沉积复合二维材料薄膜和金薄膜。此外,在d型结构的表面涂覆含有隐烷- a的甲烷敏感层。利用有限元方法分析比较了不同二维材料(石墨烯、MoS2和石墨烯- MoS2)涂层对传感器灵敏度的模拟分析。石墨烯-二硫化钼复合二维材料的使用不仅提高了传感性能,而且激发了双峰效应。这种双峰效应使甲烷传感器能够在不同的波长进行测量,主峰和次峰相互校准,以提高传感器的精度。结果表明,基于石墨烯-二硫化钼复合膜的表面等离子体共振光子晶体光纤传感器具有较好的传感性能。在甲烷浓度为0.5 ~ 3.5%范围内,最大波长灵敏度为80 nm/%,平均波长灵敏度为63.4 nm/%。这些性能明显优于最近报道的甲烷传感器。因此,该传感器在微型甲烷检测领域具有良好的应用前景。
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引用次数: 0
Effective Performance of Gold–Zirconia Photodetector Produced via Laser Energy Control Deposited on Porous Silicon 多孔硅上激光能量控制制备金-氧化锆光电探测器的有效性能研究
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-05-29 DOI: 10.1007/s11468-025-03039-8
Ruwaida T. Shbeeb, Falah A.-H. Mutlak

This work reports on the fabrication of gold nanoparticles (Au NPs)/zirconium oxide (ZrO2)/porous silicon photodetector for multi-wavelength detection, particularly for UV detection. This multilayer photodetector is fabricated using more than one method. Au NPs are synthesized by pulsed laser ablation in liquid (PLAL), followed by drop casting on ZrO2 thin films prepared with (600, 800, and 1000 mJ) laser energy through pulsed-laser deposition (PLD) on a porous silicon substrate. For the first time, significant properties of this fabricated photodetector are enhanced, including gain, sensitivity, detectivity, responsivity, and quantum efficiency. X-ray diffraction results revealed that the Au/ZrO2/PSi thin films have a crystalline structure with a face-centered cubic (FCC) phase for Au NPs, while ZrO2 exhibit a dominant monoclinic phase. The uniform particle distribution and nanoscale size range (10–15 nm) for this composite are demonstrated by FE-SEM. High-resolution TEM shows the spherical shape of Au NPs. Furthermore, the J-V characteristic test revealed that photocurrent increased directly with light intensity. The focus here is on UV detection. The photodetector responsivity at an applied bias of 3 V increased from 0.15 to 0.17 A/W at 350 nm with an increase in laser energy from (600 to 1000 mJ), while detectivity reached its highest value of 2.5 × 1011 cm Hz0.5/W for the 600-mJ film. Quantum efficiency demonstrated better results, reaching up to 60.7% for 1000 mJ. The results of the Au/ZrO2 photodiode indicate that the performance of the UV photodiode is enhanced with increased laser pulse energy.

本工作报道了用于多波长探测的金纳米粒子(Au NPs)/氧化锆(ZrO2)/多孔硅光电探测器的制备,特别是用于紫外探测。这种多层光电探测器是用多种方法制成的。采用脉冲激光在液体中烧蚀(PLAL)的方法合成了金纳米粒子,然后在多孔硅衬底上通过脉冲激光沉积(PLD)在(600、800和1000 mJ)激光能量制备的ZrO2薄膜上滴铸。首次提高了光电探测器的增益、灵敏度、探测率、响应率和量子效率。x射线衍射结果表明,Au/ZrO2/PSi薄膜具有面心立方(FCC)相的Au NPs晶体结构,而ZrO2则以单斜相为主。FE-SEM分析表明,该复合材料颗粒分布均匀,粒径范围在10 ~ 15 nm。高分辨率透射电镜显示Au NPs呈球形。J-V特性测试表明,光电流随光强的增加而增加。这里的重点是紫外线检测。当激光能量从(600 ~ 1000 mJ)增加到350 nm时,在施加偏置3 V时,光电探测器的响应率从0.15 A/W增加到0.17 A/W,而在600 mJ的薄膜上,探测率达到了最高的2.5 × 1011 cm Hz0.5/W。量子效率表现出较好的效果,在1000 mJ时达到60.7%。对Au/ZrO2光电二极管的实验结果表明,随着激光脉冲能量的增加,UV光电二极管的性能得到增强。
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引用次数: 0
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Plasmonics
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