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Ultra-High Sensitivity Terahertz Detection Using a 2D-Material-Based Metasurface: Design, Tuning, and Machine Learning Validation 使用基于二维材料的超表面的超高灵敏度太赫兹检测:设计,调谐和机器学习验证
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-25 DOI: 10.1007/s11468-025-03118-w
Vinoth R, Gunasekaran Thangavel, Jacob Wekalao, Amuthakkannan Rajakannu

The quantification of dopamine, a critical catecholamine neurotransmitter, remains a significant challenge in neurological research and clinical diagnostics due to its low physiological concentrations and interference from structurally similar compounds. This study presents a simple metasurface sensor employing graphene-enhanced surface plasmon resonance for ultra-sensitive dopamine detection. Finite element method simulations using COMSOL Multiphysics 6.2 demonstrate exceptional performance with a maximum sensitivity of 500 GHzRIU−1 at 0.805 THz, achieving a figure of merit of 2.110 and quality factor ranging from 3.376 to 3.435. The sensor exhibits tunable response through graphene chemical potential modulation (0.1–0.9 eV), with transmittance varying from 81.6% to 16.4%. Angular stability analysis reveals consistent performance across incidence angles from 0° to 80°. Machine learning integration using XGBoost regression achieves 92–100% prediction accuracy, enabling real-time performance optimization. The proposed sensor surpasses existing designs in sensitivity while maintaining broad refractive index detection range,positioning it as a promising platform for advanced neurochemical sensing applications in Parkinson's disease, schizophrenia, and substance abuse disorder diagnostics.

多巴胺是一种重要的儿茶酚胺神经递质,由于其低生理浓度和结构相似化合物的干扰,多巴胺的定量在神经学研究和临床诊断中仍然是一个重大挑战。本研究提出了一种简单的超表面传感器,采用石墨烯增强表面等离子体共振进行超灵敏多巴胺检测。使用COMSOL Multiphysics 6.2进行有限元模拟,在0.805 THz下的最大灵敏度为500 GHzRIU−1,性能指标为2.110,质量因子范围为3.376至3.435。通过石墨烯化学势调制(0.1 ~ 0.9 eV),传感器具有可调谐的响应,透过率在81.6% ~ 16.4%之间变化。角度稳定性分析显示,从0°到80°的入射角范围内,性能一致。使用XGBoost回归的机器学习集成实现了92-100%的预测精度,实现了实时性能优化。该传感器在灵敏度上超越了现有的设计,同时保持了较宽的折射率检测范围,将其定位为帕金森病、精神分裂症和药物滥用障碍诊断中先进神经化学传感应用的有前途的平台。
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引用次数: 0
Quantum Feedback-Enhanced Discord in V-Shaped Plasmonic Waveguides v形等离子波导中量子反馈增强的不谐
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-24 DOI: 10.1007/s11468-025-03121-1
Hossein Sadeghi, Mehdi Mirzaee

This theoretical and numerical investigation explores the enhancement and preservation of quantum discord in quantum systems coupled through V-shaped plasmonic waveguides (V-PW) using advanced quantum feedback control techniques. We demonstrate that properly engineered quantum feedback can significantly improve quantum discord preservation, particularly in Werner states where we observe enhancements from zero to 0.38 under optimal conditions. The mechanism involves a sophisticated confinement of the quantum state within protected subspaces that are resilient against environmental decoherence. Through detailed theoretical modeling and extensive numerical simulations, we identified the key parameters governing this enhancement process, including waveguide geometry, emitter positioning, and feedback timing. Our results reveal three distinct quantum discord decay temporal regimes and establish optimal operating conditions for maximal quantum correlation preservation. The findings provide fundamental insights into quantum correlation dynamics in nanophotonic systems and practical guidelines for experimental implementations in quantum information processing applications, with particular relevance to room-temperature quantum technologies.

这项理论和数值研究探讨了利用先进的量子反馈控制技术,通过v形等离子体波导(V-PW)耦合的量子系统中量子不和谐的增强和保持。我们证明了适当设计的量子反馈可以显着改善量子不和谐保存,特别是在Werner状态下,我们观察到在最佳条件下从0到0.38的增强。该机制包括在受保护的子空间内对量子态进行复杂的限制,这些子空间对环境退相干具有弹性。通过详细的理论建模和广泛的数值模拟,我们确定了控制这一增强过程的关键参数,包括波导几何形状、发射器定位和反馈定时。我们的研究结果揭示了三种不同的量子不和谐衰变时间机制,并建立了最大量子相关保存的最佳操作条件。这些发现为纳米光子系统中的量子相关动力学提供了基本见解,并为量子信息处理应用的实验实现提供了实用指南,特别是与室温量子技术相关。
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引用次数: 0
Spectral and Modal Tuning of Surface Plasmons in Symmetric Nanocomposite–Metal Configurations 对称纳米复合金属结构中表面等离子体的光谱和模态调谐
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-18 DOI: 10.1007/s11468-025-03054-9
Vivek Saxena

This study presents a detailed investigation into the dispersion and confinement characteristics of surface plasmon polaritons (SPPs) in a symmetric waveguide architecture composed of nanocomposite–metal–nanocomposite (NMC–M–NMC) layers. The nanocomposite claddings incorporate metallic nanoparticles, enabling the simultaneous excitation of propagating surface plasmon modes and localized plasmon resonances. This coupling mechanism leads to superior field confinement and an extended modal wavevector range compared to conventional metal–insulator–metal (MIM) waveguides. The resulting structure supports both long-range SPP (LRSP) and short-range SPP (SRSP) modes, each exhibiting distinct advantages: LRSP modes offer reduced propagation losses and longer transmission distances, while SRSP modes exhibit tight spatial confinement around the metallic core. A key feature of the proposed system is its tunability, achieved by varying the nanoparticle characteristics—such as radius, volume fraction, and interparticle spacing—as well as the thickness of the central metal layer. This flexibility allows dynamic control over the effective wavelength and intensity distribution of the plasmonic modes, making the structure highly adaptable to a wide range of optical design requirements. To further elucidate the material influence on SPP behavior, comparative simulations are performed using two representative nanocomposite systems: silver–silica and gold–alumina. These comparisons reveal material-specific differences in mode dispersion and confinement, thereby providing valuable guidance for material selection in plasmonic device engineering. The demonstrated ability to manipulate SPP propagation and confinement through structural and material parameters underscores the potential of the NMC–M–NMC configuration in advanced photonic applications. In particular, this platform shows strong promise for integration into nanophotonic circuits, plasmonic sensors, optical modulators, and subwavelength light guiding components within next-generation optoelectronic systems.

Graphical Abstract

研究了由纳米复合材料-金属-纳米复合材料(NMC-M-NMC)层构成的对称波导结构中表面等离子激元的色散和约束特性。纳米复合包层包含金属纳米颗粒,能够同时激发传播表面等离子体模式和局部等离子体共振。与传统的金属-绝缘体-金属(MIM)波导相比,这种耦合机制具有优越的场约束和更大的模态波矢量范围。所得到的结构支持远程SPP (LRSP)和短程SPP (SRSP)模式,每种模式都具有明显的优势:LRSP模式提供更小的传播损失和更长的传输距离,而SRSP模式在金属核心周围具有紧密的空间限制。该系统的一个关键特征是其可调性,可通过改变纳米颗粒的特性(如半径、体积分数、颗粒间间距以及中心金属层的厚度)来实现。这种灵活性允许对等离子体模式的有效波长和强度分布进行动态控制,使结构高度适应广泛的光学设计要求。为了进一步阐明材料对SPP行为的影响,使用两种具有代表性的纳米复合体系:银-硅和金-氧化铝进行了比较模拟。这些比较揭示了材料在模色散和约束方面的差异,从而为等离子体器件工程中的材料选择提供了有价值的指导。通过结构和材料参数控制SPP传播和约束的能力强调了NMC-M-NMC结构在先进光子应用中的潜力。特别是,该平台在集成到下一代光电系统中的纳米光子电路、等离子体传感器、光调制器和亚波长光导元件方面显示出强大的前景。图形抽象
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引用次数: 0
Tuning Viscosity and Spin Time to Enhance the Thinnest rGO Film Coating in SPR Sensors 调整粘度和旋转时间以增强SPR传感器中最薄的氧化石墨烯薄膜涂层
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-17 DOI: 10.1007/s11468-025-03110-4
Masruroh, Ghaitza Aqshal Maulana, Imam Mahdi Syarifuddin, Freygieon Ogiek Rizal Sukma, Mahardika Auditia Hanif, Gancang Saroja, Rachmat Triandi Tjahjanto, Dionysius J. D. H. Santjojo

This study examined the optimization of the solution viscosity and spin-coating time to produce thin and uniform rGO layers for surface plasmon resonance (SPR) sensor applications. The viscosity of the rGO solution was controlled by varying the concentration of ascorbic acid as a reducing agent in the rGO synthesis process. Then, characterization was performed using FESEM-EDX, TEM, and thickness and roughness measurements using a topography measurement system (TMS). The characterization results demonstrated that increasing the solution viscosity was directly proportional to the layer thickness, roughness, and the percentage of carbon elements, as determined by EDX mapping. The SEM and TEM analyses revealed a surface morphology that resembled wrinkled paper structures, which overlapped and folded. The SAED pattern indicated the presence of crystallinity relating to the (002), (100), and (110) crystal planes. In addition, as the spin-coating time increased, the thickness and roughness of the layer decreased; however, the thickness-to-roughness ratio increased. SPR sensor testing with the rGO layer was also conducted using ethanol solution analytes with concentrations ranging from 0 to 20%. The results demonstrated that the SPR sensor with the rGO layer exhibited a sensitivity of 2481.42 nm/RIU and a linearity of R2 = 0.96.

本研究考察了溶液粘度和自旋涂膜时间的优化,以制备用于表面等离子体共振(SPR)传感器的薄而均匀的氧化石墨烯层。在还原氧化石墨烯合成过程中,通过改变抗坏血酸作为还原剂的浓度来控制还原氧化石墨烯溶液的粘度。然后,使用FESEM-EDX, TEM进行表征,并使用地形测量系统(TMS)进行厚度和粗糙度测量。表征结果表明,通过EDX作图确定,溶液粘度的增加与层厚度、粗糙度和碳元素百分比成正比。扫描电镜和透射电镜分析显示,表面形貌类似皱褶纸结构,重叠和折叠。SAED模式表明在(002)、(100)和(110)晶面存在结晶度。此外,随着旋涂时间的增加,涂层的厚度和粗糙度减小;然而,厚度-粗糙度比增加。SPR传感器对还原氧化石墨烯层的测试也使用浓度为0 - 20%的乙醇溶液进行。结果表明,含氧化石墨烯层的SPR传感器灵敏度为2481.42 nm/RIU,线性关系R2 = 0.96。
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引用次数: 0
High Sensitivity SPR Refractive Index Sensor Based on D-shaped PCF with Ge-doped SiO2 Core 基于掺锗SiO2 d型PCF的高灵敏度SPR折射率传感器
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-12 DOI: 10.1007/s11468-025-03101-5
Qingcheng You, Yi Zhou, Yukun Zhu, Licui Ji, Yichen Li, Bin Li, Xu Gao, Xing Wang, Honggang Pan

In this study, a D-shaped photonic crystal fiber (PCF) sensor with surface plasmon resonance (SPR) was designed with Ge-doped Si as the fiber core. The surface plasmon wave was excited by gold plating on the D-shaped surface. Numerical simulations by the finite element method (FEM) show that this sensor can realize a wide detection range of refractive index (RI) measurement from 1.330 to 1.445. The maximum wavelength sensitivity (WS) is 45,600 nm/RIU, and the maximum accuracy is 2.19 × 10−6 RIU. Compared with the sensor with a pure SiO2 fiber core, the maximum WS is increased by about 2.87 times, and the average WS is increased by 20.6%. The proposed sensor is characterized by a simple structure, high sensitivity, and a large detection range, which has great potential in cell activity monitoring, food additives, and residue detection.

本文以掺锗硅为光纤芯,设计了一种具有表面等离子体共振(SPR)的d形光子晶体光纤(PCF)传感器。在d形表面镀金激发表面等离子体波。有限元数值模拟结果表明,该传感器可实现1.330 ~ 1.445范围内的折射率测量。最大波长灵敏度(WS)为45600 nm/RIU,最大精度为2.19 × 10−6 RIU。与采用纯SiO2纤芯的传感器相比,最大WS提高约2.87倍,平均WS提高20.6%。该传感器结构简单、灵敏度高、检测范围大,在细胞活性监测、食品添加剂、残留物检测等方面具有很大的应用潜力。
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引用次数: 0
Dual-Plasmonic Coupling in Bidirectional SPR-PCF Biosensors: for Detection of Bacillus cereus via Refractive Index Measurement 双向SPR-PCF生物传感器的双等离子体耦合:折射率测量法检测蜡样芽孢杆菌
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-11 DOI: 10.1007/s11468-025-03108-y
Licui Ji, Honggang Pan, Zihong Zhao, Qingcheng You, Yukun Zhu, Xu Gao, Xing Wang

Employing surface plasmon resonance (SPR) in a specially designed dual-core photonic crystal fiber (PCF) with double-sided polishing, this study demonstrates a biosensor with superior sensitivity for Bacillus cereus identification. The sensor uses silica as a background material, and the structure is optimized by COMSOL Multiphysics software. Under Y-pol, the refractive index (RI) detection ranges were determined as na = 1.31–1.40 for odd mode and na = 1.31–1.39 for even mode. The maximum wavelength sensitivity (WS) reached 30,600 nm/RIU for even mode and 23,800 nm/RIU for odd mode. Within the concentration range of 0.2 × 108–1.4 × 108 CFU/ml, both modes demonstrated concentration-dependent variations in WS and figure of merit (FOM), with the even mode exhibiting superior detection performance. In addition to detecting the Bacillus cereus concentration, it can also detect S. aureus, Salmonella, Shigella, E. coli, Vibrio cholerae, and many other common pathogens that cause food poisoning or serious infections.

利用特殊设计的双核光子晶体光纤(PCF)双面抛光的表面等离子体共振(SPR)技术,研究了一种具有高灵敏度的蜡样芽孢杆菌生物传感器。该传感器以二氧化硅为背景材料,利用COMSOL Multiphysics软件对传感器结构进行优化。在Y-pol下,折射率(RI)检测范围确定为:奇数模式na = 1.31-1.40,偶数模式na = 1.31-1.39。最大波长灵敏度(WS)在偶模下达到30600 nm/RIU,在奇模下达到23800 nm/RIU。在0.2 × 108 ~ 1.4 × 108 CFU/ml的浓度范围内,两种模式的WS和FOM值均表现出浓度依赖性,其中均匀模式的检测性能更好。除了检测蜡样芽孢杆菌浓度外,还可以检测金黄色葡萄球菌、沙门氏菌、志贺氏菌、大肠杆菌、霍乱弧菌等许多引起食物中毒或严重感染的常见病原体。
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引用次数: 0
Plasmon-Enhanced ZnO/Ag Nanoparticles with Synergistic Antibacterial and Anticancer Activities 等离子体增强ZnO/Ag纳米粒子具有协同抗菌和抗癌活性
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-11 DOI: 10.1007/s11468-025-03001-8
Shaymaa Awad Kadhim, Rusul A. Ghazi, Ali Abbasi, Mohammad Waleed M. Sadaka, Forat H. Alsultany, Maryam Hakim Flayih, Ameer F. Shamkhi

Plasmonic nanomaterials have garnered significant attention for their enhanced optical, antibacterial, and anticancer properties, owing to their surface plasmon resonance (SPR) effects. In this study, ZnO and ZnO/Ag nanoparticles were synthesized using green synthesis approach. The structural, morphological, and physicochemical properties of the fabricated nanomaterials were systematically characterized via X-ray diffraction (XRD), Fourier-transform infrared spectroscopy (FT-IR), transmission electron microscopy (TEM), and dynamic light scattering (DLS). XRD analysis confirmed the hexagonal wurtzite structure of ZnO, while additional peaks in ZnO/Ag nanoparticles indicated successful silver incorporation. TEM imaging revealed a spherical morphology with average particle sizes of 35 ± 10 nm for ZnO and 55 ± 10 nm for ZnO/Ag. The antibacterial activity of the nanoparticles was assessed against Klebsiella pneumoniae, Pseudomonas aeruginosa, Escherichia coli, Streptococcus mutans, Staphylococcus aureus, and Enterococcus faecalis using broth microdilution method. ZnO/Ag nanoparticles exhibited superior antibacterial efficacy, particularly against Gram-negative strains, due to the synergistic action of ZnO-mediated oxidative stress and Ag⁺-induced membrane disruption. The plasmonic properties of Ag further contributed to the antibacterial effect by enhancing reactive oxygen species (ROS) generation under light exposure. Moreover, the MTT assay demonstrated a dose-dependent cytotoxic effect on A-549 lung carcinoma cells, with ZnO/Ag nanoparticles displaying a lower IC50 than ZnO. The enhanced anticancer activity was attributed to increased mitochondrial dysfunction, ROS generation, and apoptosis induction, further amplified by plasmonic interactions. These findings highlight the potential of ZnO/Ag nanomaterials as promising candidates for biomedical applications, particularly in antimicrobial and anticancer therapies.

等离子体纳米材料由于其表面等离子体共振(SPR)效应而具有增强的光学、抗菌和抗癌特性,引起了人们的广泛关注。本研究采用绿色合成的方法合成了ZnO和ZnO/Ag纳米颗粒。通过x射线衍射(XRD)、傅里叶变换红外光谱(FT-IR)、透射电子显微镜(TEM)和动态光散射(DLS)对制备的纳米材料的结构、形态和物理化学性质进行了系统表征。XRD分析证实了ZnO的六方纤锌矿结构,而ZnO/Ag纳米颗粒中的附加峰表明银的成功掺入。TEM成像显示ZnO的平均粒径为35±10 nm, ZnO/Ag的平均粒径为55±10 nm。采用微量肉汤稀释法测定纳米颗粒对肺炎克雷伯菌、铜绿假单胞菌、大肠杆菌、变形链球菌、金黄色葡萄球菌和粪肠球菌的抑菌活性。ZnO/Ag纳米颗粒表现出优异的抗菌效果,特别是对革兰氏阴性菌株,这是由于ZnO介导的氧化应激和Ag +诱导的膜破坏的协同作用。Ag的等离子体特性通过增强光照射下活性氧(ROS)的生成进一步促进了抗菌效果。此外,MTT实验显示,ZnO/Ag纳米颗粒对a -549肺癌细胞具有剂量依赖性的细胞毒性作用,其IC50值低于ZnO。增强的抗癌活性归因于线粒体功能障碍,ROS生成和细胞凋亡诱导的增加,并通过等离子体相互作用进一步放大。这些发现突出了ZnO/Ag纳米材料在生物医学应用方面的潜力,特别是在抗菌和抗癌治疗方面。
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引用次数: 0
A Hybrid Plasmonic System Integrating Plasmon-Induced Transparency and Perfect Absorbance 集成等离子体诱导透明和完美吸光度的混合等离子体系统
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-10 DOI: 10.1007/s11468-025-03098-x
Meryem Beyza Avci, Arif E. Cetin

We present a hybrid plasmonic platform that integrates plasmon-induced transparency (PIT) and perfect absorbance (PA) to achieve multi-band, tunable, and highly efficient light–matter interactions in the mid-infrared (mid-IR) spectral region. The system employs a dolmen-shaped nanoantenna configuration engineered to support the hybridization of bright dipole and dark quadrupole resonances. By systematically tuning structural parameters such as antenna separation and dielectric spacer thickness, the platform enables precise control over spectral splitting and absorption strength, giving rise to multiple perfect absorption peaks. To demonstrate the platform’s utility for molecular sensing, we modeled a protein bilayer characterized by vibrational signatures at the Amide I, II and III bands. Our results demonstrate that this PIT–PA integrated platform not only achieves near-unity absorbance across multiple spectral bands but also enables the label-free detection of distinct protein vibrational modes with high sensitivity. The platform holds strong potential for applications in biosensing, photodetection, and infrared energy harvesting, where multi-band operation and spectral precision are critical.

我们提出了一个混合等离子体平台,集成了等离子体诱导的透明度(PIT)和完美的吸光度(PA),以实现中红外光谱区域的多波段、可调谐和高效的光物质相互作用。该系统采用球门形状的纳米天线结构,以支持亮偶极子和暗四极子共振的杂交。通过系统地调整天线间距和介电间隔厚度等结构参数,该平台可以精确控制光谱分裂和吸收强度,从而产生多个完美的吸收峰。为了证明该平台在分子传感方面的实用性,我们模拟了一个蛋白质双分子层,其特征是酰胺I, II和III波段的振动特征。我们的研究结果表明,该PIT-PA集成平台不仅在多个光谱波段实现了接近统一的吸光度,而且能够以高灵敏度实现不同蛋白质振动模式的无标记检测。该平台在多波段操作和光谱精度至关重要的生物传感、光探测和红外能量收集领域具有巨大的应用潜力。
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引用次数: 0
Novel Biosensor Based on Photonic Crystal Fiber with Ultra-High Efficiency 基于超高效光子晶体光纤的新型生物传感器
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-10 DOI: 10.1007/s11468-025-03076-3
Mahmoud M. M. Abu Hasanein, Malek G. Daher, Shivam Singh, Mahmoud M. A. Eid, Yogesh Sharma, Anurag Upadhyay

For females, particularly growing fetuses in the latter stages of pregnancy, progesterone plays a crucial function. However, one female sex hormone that falls within the category of estrogen is estradiol. Egg mellowing and emission are caused by an increase in estradiol degrees during the menstrual cycle. It is responsible for the pollinated eggs imbedding, which causes the uterine coating to solidify. Here, an innovative PCFD is projected to determine progesterone hormone (PH) and estradiol hormone (EH) in blood which involves an easy structure of square hole is treated as a core gap. The suggested PCFD is achieved an ultra-high relative sensitivity (RSE) as 99.92% at 2 THz. Furthermore, the loss in the projected PCFD is very tiny which proves the effectiveness of planned PCFD. Also, this PCFD has tunable design and simple structure; it can be fabricated easily using the prevailing fabrication schemes. As a result, the suggested PCFD will act a key role in chemical and bio-testing in diverse areas swiftly.

对于女性来说,尤其是怀孕后期的胎儿,黄体酮起着至关重要的作用。然而,有一种雌性激素属于雌激素的范畴,那就是雌二醇。卵子软化和排出是由月经周期中雌二醇水平的增加引起的。它负责授粉的卵子嵌入,这导致子宫涂层固化。本文提出了一种新颖的PCFD检测血液中孕酮激素(PH)和雌二醇激素(EH)的方法,该方法采用简单的方孔结构作为核心间隙。建议的PCFD在2太赫兹时达到99.92%的超高相对灵敏度(RSE)。此外,预测的PCFD损耗很小,证明了计划PCFD的有效性。该PCFD设计可调,结构简单;它可以很容易地制造使用现行的制造方案。因此,建议的PCFD将迅速在不同领域的化学和生物测试中发挥关键作用。
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引用次数: 0
Incorporation of Fractional Drude Model to Study the SPP Waves 结合分数阶Drude模型研究SPP波
IF 4.3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2025-06-09 DOI: 10.1007/s11468-025-03059-4
Sher Ali, Qaisar Abbas Naqvi, Aqeel Abbas Syed

Surface plasmon polariton (SPP) waves are electromagnetic (EM) waves that travel over the interface between a metal and a dielectric. Typically, the conventional Drude model (DM), which uses integer order derivatives, has been employed to investigate SPP behavior. Since the classical DM does not exactly match experimental values for metal dielectric constants, it has been modified with the fractional calculus method to improve its modeling capabilities. The fractional method allows us to analyze system behaviors in non-integer domains that classic integer-order models cannot capture. In this paper, we use a fractional Drude model (FDM) with non-integer order derivatives to study SPP wave characteristics. A planar silver-glass interface is unitized to investigate the effect of the fractional-order parameter ( gamma ), which defines the order of the FDM. The impact of small variations of ( gamma ) from unity on dielectric constant and refractive index of metal is explored. Furthermore, important SPP properties such as effective propagation length, dispersion curve, and bandgaps are examined for various values of ( gamma ). Notably, setting ( gamma = 1 ) recovers results in agreement with the standard DM, validating the proposed mechanism. This theoretical study indicates that the optical characteristics are influenced by both the applied electric field frequency ( omega ) and the non-integer order ( gamma ) of FDM. This fractional order of FDM is tuned to ensure a good fit with the experimental data. It is hoped that these findings would be useful to plasmonic researchers.

表面等离子激元(SPP)波是在金属和电介质之间的界面上传播的电磁波(EM)。通常,传统的Drude模型(DM)使用整数阶导数来研究SPP行为。由于经典DM模型与金属介电常数的实验值不完全匹配,本文采用分数阶演算方法对其进行了修正,以提高其建模能力。分数阶方法允许我们分析非整数域的系统行为,这是经典整数阶模型无法捕捉的。本文采用非整数阶导数的分数阶Drude模型(FDM)来研究SPP波的特性。以平面银玻璃界面为单元,研究了分数阶参数( gamma )的影响,该参数定义了FDM的阶数。探讨了( gamma )的微小变化对金属介电常数和折射率的影响。此外,重要的SPP性质,如有效传播长度,色散曲线和带隙被检查的不同值( gamma )。值得注意的是,设置( gamma = 1 )恢复的结果与标准DM一致,验证了提议的机制。理论研究表明,FDM的光学特性受外加电场频率( omega )和FDM的非整数阶( gamma )的双重影响。对FDM的分数阶进行了调整,以确保与实验数据很好地拟合。希望这些发现能对等离子体研究人员有所帮助。
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引用次数: 0
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Plasmonics
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