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Compact Three-Channel Photonic Crystal Fiber Sensor Based on Surface Plasmon Resonance 基于表面等离子体共振的紧凑型三通道光子晶体光纤传感器
IF 3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2024-09-09 DOI: 10.1007/s11468-024-02522-y
Tianli Huo, Xili Jing, Zhiyong Yin, Tianci Gao, Mingshi Song

In order to improve the integration of fiber optic sensors, this paper designs a dual-core three-channel photonic crystal fiber (PCF) optic sensor that can simultaneously measure the refractive index of a liquid, its temperature, and the ambient magnetic field. Based on the PCF as well as SPR principles, the sensor has two D-planes, one coated with PDMS as well as a gold film for detecting temperature and the other coated with a gold film for detecting refractive index and coated with a gold film over the air holes on the side of the core where the refractive index is measured and a magnetic fluid injected into the air holes to detect the magnetic field. The results show a maximum sensitivity of 20,000 nm/RIU for refractive index, a linear sensitivity of 116 pm/Oe for magnetic field, and 5300 pm/°C for temperature when the sample’s refractive index is between 1.36 and 1.42, the temperature is between 0 °C and 50 °C, and the magnetic field is between 20 and 550 Oe. The sensitivity matrix of temperature versus refractive index is also given. The sensor is compact and simple to prepare, providing a new solution for miniaturization and integration of multifunctional photonic devices.

为了提高光纤传感器的集成度,本文设计了一种双核三通道光子晶体光纤(PCF)光学传感器,可同时测量液体的折射率、温度和环境磁场。基于 PCF 和 SPR 原理,该传感器有两个 D 平面,一个涂有 PDMS 和金膜,用于检测温度;另一个涂有金膜,用于检测折射率,并在测量折射率的纤芯一侧气孔上涂有金膜,气孔中注入磁性流体,用于检测磁场。结果显示,当样品的折射率在 1.36 和 1.42 之间,温度在 0 °C 和 50 °C 之间,磁场在 20 和 550 Oe 之间时,折射率的最大灵敏度为 20,000 nm/RIU,磁场的线性灵敏度为 116 pm/Oe,温度的线性灵敏度为 5300 pm/°C。此外,还给出了温度与折射率的灵敏度矩阵。该传感器结构紧凑、制备简单,为多功能光子器件的微型化和集成化提供了一种新的解决方案。
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引用次数: 0
Design of Graphene-Based Core/Shell Nanoparticles to Enhance the Absorption of Thin Film Solar Cells 设计基于石墨烯的核/壳纳米粒子以增强薄膜太阳能电池的吸收能力
IF 3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2024-09-09 DOI: 10.1007/s11468-024-02476-1
Amir Mehrpanah, Hasan Rasooli Saghai, Babak Sakkaki, Ali Daghigh

Plasmonic nanoparticles have had a great impact on the enhancement of the absorption of the thin film solar cell. In this study, we propose two core/shell nanoparticles including graphene/Ag and Ag/graphene nanoparticles. For the design of the graphene/Ag nanoparticle, we utilize a graphene quantum dot (GQD) with a diameter of 66 nm as the core and cover it with Ag with a thickness of 1 nm. We compute the permittivity of the GQD based on the Cole–Cole model. For the design of the Ag/graphene nanoparticle, we cover a spherical Ag nanoparticle with a diameter of 66 nm with a graphene layer with a thickness of 1 nm. We model the surface conductivity of the graphene layer based on the Kubo formula. We consider both nanoparticles as homogeneous nanoparticles and obtain their permittivity based on the equivalent dielectric permittivity model. We incorporate these nanoparticles into an optical simulator and extract their scattering cross sections alongside the Ag nanoparticle. The graphene/Ag nanoparticle shows the best scattering performance; meanwhile, Ag nanoparticle has the weakest scattering performance. Then, we design a Si-based thin film solar cell with Ag nanoparticle and compute its characteristics through the FDTD method. Then, we replace the Ag nanoparticle with our nanoparticles. The short-circuit current density (Jsc) of the Si-based cell improves by 26.3% by embedding of Ag nanoparticle in the absorber layer. This improvement increases by embedding of graphene/Ag and Ag/graphene nanoparticles to 35.3% and 36.8%, respectively.

等离子纳米粒子对提高薄膜太阳能电池的吸收率有很大影响。在本研究中,我们提出了两种核/壳纳米粒子,包括石墨烯/银纳米粒子和银/石墨烯纳米粒子。在设计石墨烯/银纳米粒子时,我们使用了直径为 66 nm 的石墨烯量子点(GQD)作为核心,并在其上覆盖厚度为 1 nm 的银。我们根据科尔-科尔模型计算了 GQD 的介电常数。在设计银/石墨烯纳米粒子时,我们在直径为 66 nm 的球形银纳米粒子上覆盖了厚度为 1 nm 的石墨烯层。我们根据 Kubo 公式建立了石墨烯层的表面电导率模型。我们将这两种纳米粒子视为均质纳米粒子,并根据等效介电常数模型获得它们的介电常数。我们将这些纳米粒子纳入光学模拟器,并提取它们与银纳米粒子的散射截面。石墨烯/银纳米粒子的散射性能最好,而银纳米粒子的散射性能最弱。然后,我们设计了一种含银纳米粒子的硅基薄膜太阳能电池,并通过 FDTD 方法计算了其特性。然后,用我们的纳米粒子替换银纳米粒子。在吸收层中嵌入银纳米粒子后,硅基电池的短路电流密度(Jsc)提高了 26.3%。嵌入石墨烯/银纳米粒子和银/石墨烯纳米粒子后,短路电流密度(Jsc)分别提高了 35.3% 和 36.8%。
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引用次数: 0
A Theoretical Investigation on the Role of Surface Plasmon Excitation in the Cloaking and Protection of Gold Cylindrical Rods Using Metallic Layers of Different Materials 利用不同材料的金属层对表面等离子体激发在金圆柱棒的隐蔽和保护中的作用进行理论研究
IF 3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2024-09-06 DOI: 10.1007/s11468-024-02453-8
Sohila Hajihashemi, Bahram Jazi, Samaneh Najari

This work investigates the excitation of plasmons in the common region between two coaxial cylindrical waveguides nested within each other, utilizing planar electromagnetic waves. The structure under consideration comprises a metallic antenna shielded with another metallic thin layer, both metals assumed to be cylindrical symmetrically without a gap and in a concentric configuration. The conductivity of the metals is evaluated using the Drude theory. An incident electromagnetic wave in B-mode with (B_zne 0) is radiated onto the mentioned antenna. By employing wave scattering theory and solving the field equations in each region, including the vacuum, outer metallic thin layer, and inner metallic core, the surface charge density resulting from the presence of surface plasmons at the interface between the inner metallic core and the outer metallic layer, as well as between the metallic layer and the vacuum region, is calculated and analyzed. The variations in surface plasmon density at the first interface (the common boundary between the two metals) and the interface between the metal and vacuum are investigated concerning changes in the incident wave frequency and the radii of the antenna layers. It is demonstrated that the excitation of plasmons occurs most significantly in the frequency range where the conductivities of the inner metallic core and the metallic layer have opposite signs, leading to synchronization between surface plasmons.

这项研究利用平面电磁波,探讨了在两个相互嵌套的同轴圆柱形波导之间的公共区域激发等离子体的问题。所考虑的结构包括一个用另一个金属薄层屏蔽的金属天线,假定这两种金属都是对称的圆柱形,没有间隙,并呈同心配置。使用德鲁德理论评估了金属的导电性。入射的 B 模式电磁波以 (B_zne 0) 的频率辐射到上述天线上。通过采用波散射理论并求解每个区域(包括真空、外金属薄层和内金属芯)的场方程,计算并分析了内金属芯与外金属层之间以及金属层与真空区域之间界面上存在的表面等离子体所产生的表面电荷密度。根据入射波频率和天线层半径的变化,研究了第一界面(两种金属之间的共同边界)和金属与真空界面上表面等离子体密度的变化。结果表明,在金属内核和金属层的电导率符号相反的频率范围内,等离子体的激发最为显著,从而导致表面等离子体之间的同步。
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引用次数: 0
D-Shaped Photonic Crystal Fiber Plasmonic Sensor Based on Au-Ta2O5 Composite Micro-grating 基于金-Ta2O5 复合微光栅的 D 形光子晶体光纤等离子传感器
IF 3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2024-09-06 DOI: 10.1007/s11468-024-02412-3
Mengqi Li, Hong Gu, Xuan Wu, Xiaotong Li

A novel D-type photonic crystal fiber optical plasma sensor (PCF-SPR) based on a composite micro-grating of Au and tantalum pentoxide (Ta2O5) is proposed. The simulation and corresponding numerical characterization were performed using COMSOL Multiphysic software. In order to obtain a simple and practically feasible structure, the Au plasma material and the sensing medium were placed outside the optical fiber. A thin layer of Ta2O5 is used as a coating to protect the gold layer. This composite micro-grating PCF sensor has a maximum sensitivity of 25,000 nm/RIU and sensor unit with a detection resolution of 4.0 × 10−6/RIU in the near infrared in the refractive index range of 1.34 ~ 1.41. Dependences of loss spectrum on the PCF parameters (air hole diameter and lattice constant) and the grating structure (grating thickness and width) are systematically analyzed. This sensor with grating structure is a more sensitive sensor for broad IR detection, suitable for biosensors, chemical detection, and food safety.

本文提出了一种基于金和五氧化二钽 (Ta2O5) 复合微光栅的新型 D 型光子晶体光纤等离子体传感器 (PCF-SPR)。使用 COMSOL Multiphysic 软件进行了仿真和相应的数值表征。为了获得简单且实际可行的结构,金等离子材料和传感介质被置于光纤外部。一层薄薄的 Ta2O5 被用作保护金层的涂层。这种复合微光栅 PCF 传感器的最大灵敏度为 25,000 nm/RIU,在折射率范围为 1.34 ~ 1.41 的近红外光谱中,传感器单元的检测分辨率为 4.0 × 10-6/RIU。系统分析了损耗谱与 PCF 参数(气孔直径和晶格常数)和光栅结构(光栅厚度和宽度)的关系。这种具有光栅结构的传感器是一种灵敏度更高的宽红外检测传感器,适用于生物传感器、化学检测和食品安全领域。
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引用次数: 0
Enhancing Sensing and Imaging Capabilities Through Surface Plasmon Resonance for Deepfake Image Detection 通过表面等离子体共振增强传感和成像能力,用于深度伪图像检测
IF 3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2024-09-06 DOI: 10.1007/s11468-024-02492-1
R. Uma Maheshwari, B.Paulchamy, Binay Kumar Pandey, Digvijay Pandey

Plasmonic nanomaterials have revolutionized sensing and imaging technologies due to their unique optical properties, particularly surface plasmon resonance (SPR). These materials offer enhanced sensitivity and resolution, making them promising candidates for applications in deepfake image detection, where accurate authentication of digital content is crucial. This work presents the application of plasmonic nanomaterials in enhancing sensing and imaging capabilities for deepfake detection. Gold nanoparticles functionalized with specific ligands are employed to exploit SPR effects, enabling sensitive detection of minute alterations in image content. A spectroscopic setup is utilized to measure the SPR shifts corresponding to changes induced by deepfake manipulations. Experimental results demonstrate that the SPR-based sensing approach achieves a detection accuracy of over 95% in distinguishing deepfake images from authentic ones. The SPR sensor exhibits a high signal-to-noise ratio, providing robust performance even in complex imaging scenarios with varying lighting conditions and image resolutions. Plasmonic nanomaterials, leveraging SPR, offer a reliable method for enhancing deepfake image detection capabilities. The demonstrated high accuracy and sensitivity underscore their potential in combating digital media forgery, contributing to the development of more secure and trustworthy authentication systems for visual content.

由于其独特的光学特性,尤其是表面等离子体共振(SPR),等离子纳米材料为传感和成像技术带来了革命性的变化。这些材料具有更高的灵敏度和分辨率,因此有望应用于对数字内容进行准确验证至关重要的深层伪造图像检测。本研究介绍了等离子纳米材料在增强深度伪造检测的传感和成像能力方面的应用。利用特定配体功能化的金纳米粒子来利用 SPR 效应,从而实现对图像内容微小变化的灵敏检测。利用光谱装置测量与深度伪造操作引起的变化相对应的 SPR 偏移。实验结果表明,基于 SPR 的传感方法在区分深度伪造图像和真实图像方面的检测准确率超过 95%。SPR 传感器具有很高的信噪比,即使在光照条件和图像分辨率各不相同的复杂成像场景中也能提供稳定的性能。利用 SPR 的质子纳米材料为增强深度伪造图像的检测能力提供了一种可靠的方法。所展示的高精确度和灵敏度突显了它们在打击数字媒体伪造方面的潜力,有助于开发更安全、更可信的视觉内容认证系统。
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引用次数: 0
Eccentric Core Optical Fiber SPR Sensor for Refractive Index Sensing Characteristics 偏心芯光纤 SPR 传感器的折射率传感特性
IF 3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2024-09-05 DOI: 10.1007/s11468-024-02508-w
Jianxia Liu, Chang Li, Libo Yuan, Chenghao Li

This study proposes an eccentric core optical fiber biosensor based on the surface plasmon resonance phenomenon, utilizing COMSOL Multiphysics 6.2 finite element method (FEM). An Ag film with a thickness of 30nm is coated on the cladding of the eccentric core optical fiber. The analytical layers employed include air, water, blood plasma, and a self-set refractive index (RI) of 1.373. A 5-nm thick TiO2 layer is coated between the Ag film and the analyte. This TiO2 layer not only prevents the Ag layer from oxidation but also enhances the sensor’s sensitivity. The sensor serves as a theoretical foundation for experimental research. The wavelength sensitivities have been calculated, with the self-set RI of 1.373 exhibiting the maximum sensitivity of 1785.714 nm/RIU and a resolution of 5.60 × 10−5 RIU. The proposed sensor presents itself as a promising candidate for a low-cost, simple-geometry biochemical sensing solution.

本研究利用 COMSOL Multiphysics 6.2 有限元方法(FEM),提出了一种基于表面等离子体共振现象的偏心芯光纤生物传感器。在偏心芯光纤的包层上镀了一层厚度为 30nm 的银膜。采用的分析层包括空气、水、血浆和自定折射率 (RI) 1.373。在银膜和分析物之间涂有 5 纳米厚的二氧化钛层。这层二氧化钛层不仅能防止银层氧化,还能提高传感器的灵敏度。该传感器为实验研究奠定了理论基础。计算得出的波长灵敏度显示,自设 RI 为 1.373 时,最大灵敏度为 1785.714 nm/RIU,分辨率为 5.60 × 10-5 RIU。该传感器有望成为一种低成本、简单几何形状的生化传感解决方案。
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引用次数: 0
Terahertz Plasmonic Biosensor Leveraging Ag-Au-Graphene Heterostructures for Quantitative Hemoglobin Analysis with Machine Learning Algorithms for Performance Optimization 利用银-金-石墨烯异质结构进行血红蛋白定量分析的太赫兹等离子体生物传感器,以及用于性能优化的机器学习算法
IF 3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2024-09-04 DOI: 10.1007/s11468-024-02520-0
Jacob Wekalao, Ngaira Mandela, Costable Lefu, Obed Apochi, Calistus Wamalwa, Wesley Langat

This investigation presents the design, simulation, and performance analysis of a terahertz-based biosensor for hemoglobin detection. The sensor architecture incorporates a synergistic combination of graphene, gold, and silver metasurfaces in a hierarchical resonator structure. Extensive parametric analysis was conducted to optimize the sensor's performance characteristics. The optimized sensor demonstrates high sensitivity, achieving up to 1000 GHzRIU−1, with a figure of merit of 3.289 RIU−1. Experimental results indicate effective detection of hemoglobin concentrations ranging from 10 to 40 g/L, corresponding to refractive indices between 1.34 and 1.43. Electromagnetic field distribution analysis exemplifies peak absorption at 0.65 THz. Furthermore, the sensor’s potential for binary encoding applications was evaluated with remarkable performance. Machine learning optimization, employing a decision tree regressor, demonstrates an optimal R2 score of 100% across various parameter combinations, suggesting potential for the development of accurate sensing systems. The proposed sensor design represents a significant advancement in terahertz biosensing technology, with implications for enhanced medical diagnostics and biomedical research applications.

本研究介绍了一种基于太赫兹的血红蛋白检测生物传感器的设计、模拟和性能分析。传感器结构将石墨烯、金和银元表面协同组合在分层谐振器结构中。为了优化传感器的性能特征,我们进行了广泛的参数分析。优化后的传感器具有很高的灵敏度,可达到 1000 GHzRIU-1,优点系数为 3.289 RIU-1。实验结果表明,可有效检测 10 至 40 g/L 的血红蛋白浓度,折射率介于 1.34 和 1.43 之间。电磁场分布分析表明,吸收峰值为 0.65 太赫兹。此外,还对传感器在二进制编码应用方面的潜力进行了评估,结果表明该传感器性能卓越。利用决策树回归器进行的机器学习优化表明,在各种参数组合中,最佳 R2 得分为 100%,这表明该传感器具有开发精确传感系统的潜力。拟议的传感器设计代表了太赫兹生物传感技术的重大进步,对增强医疗诊断和生物医学研究应用具有重要意义。
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引用次数: 0
Broadband MXene-Based Metasurafce Absorber for Visible Region 用于可见光区域的基于 MXene 的宽带 Metasurafce 吸收器
IF 3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2024-09-04 DOI: 10.1007/s11468-024-02519-7
Neda Daliran, Abdollah Hassanzadeh

Nowadays, controlling the light reflection and transmission by metasurface nanostructures opens pathways for efficient energy harvesting in nanophotonics and optoelectronic devices. This paper demonstrates a metasurface broadband absorber in the visible wavelength region of 400–800 nm using two-dimensional titanium carbide (Ti3C2Tx) MXene. A high average absorption of 97.85% over a wide wavelength region of the incident light (0.4 µm) is achieved. This significant absorption is due to the strong localized surface plasmon caused by the Ti3C2Tx periodic nanoarrays top-mounted on SiO2/Au/glass layers. The proposed MXene-based absorber also shows broadband and high average absorption for both transverse electric (TE) and transverse magnetic (TM) polarizations under a wide range of oblique incidence and azimuthal light angles, especially it reaches over 99% for TM polarization in some ranges. The proposed absorber can be used in photodetectors, sensors, and applications where the incident angle and/or polarization are constantly changing.

如今,通过元表面纳米结构控制光的反射和透射为纳米光子学和光电子器件中的高效能量收集开辟了道路。本文利用二维碳化钛(Ti3C2Tx)MXene 展示了一种在 400-800 纳米可见光波长区域的超表面宽带吸收器。在入射光的较宽波长区域(0.4 µm)内实现了 97.85% 的高平均吸收率。这种显著的吸收率是由于安装在二氧化硅/金/玻璃层上的 Ti3C2Tx 周期性纳米阵列产生了强大的局部表面等离子体。所提出的基于 MXene 的吸收器还能在很宽的斜入射和方位角范围内对横向电(TE)和横向磁(TM)极化显示出宽带和高平均吸收率,特别是在某些范围内对 TM 极化的吸收率达到 99% 以上。所提出的吸收器可用于入射角和/或偏振不断变化的光电探测器、传感器和应用中。
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引用次数: 0
Plasmonic ELISA for Tear Biomarkers: Etching in Plasmonic Paper with Dual-Signal Readout 泪液生物标志物的等离子 ELISA:等离子纸蚀刻与双信号读出
IF 3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2024-08-31 DOI: 10.1007/s11468-024-02512-0
Myeongseong Sim, Hyeokjung Kim, Hyeran Noh

Tear biomarkers have received much attention for non-invasive monitoring of ocular and systemic diseases. Although various approaches have been developed for on-site detection of tear biomarkers, there is still the limited number of simple and reliable sensing platform in the clinical setting. Here, we introduce a plasmonic enzyme-linked immunosorbent assay (ELISA) that utilizes Ag/chitosan plasmonic paper with dual-signal readout to detect immunoglobulin G as a model tear biomarker. The sensing mechanism for a colorimetric and surface-enhanced Raman scattering (SERS) dual-signal readout is attributed to the etching of Ag nanoparticles anchored to the plasmonic paper. This etching induces both a color shift and a reduction in the Raman enhancement of the plasmonic paper. The optimized etching system demonstrates the feasibility of performing simultaneous immunoassay and etching on a plasmonic substrate without requiring an additional etching step. The detection limit was achieved at concentrations approximately 100 times lower than the physiological tear concentration, along with selective detection in simulated tear fluid. Furthermore, the dual-mode detection improves accuracy and efficiency by comparing the results of overlap detection range and enabling pre-screening with colorimetric results prior to SERS analysis. This approach holds promise as a versatile point-of-care sensing platform that can easily and reliably detect tear biomarkers.

泪液生物标志物在无创监测眼部和全身疾病方面受到广泛关注。虽然已经开发出多种现场检测泪液生物标志物的方法,但在临床环境中,简单可靠的传感平台仍然数量有限。在此,我们介绍一种利用 Ag/ 壳聚糖质子纸和双信号读出的质子酶联免疫吸附测定(ELISA)来检测作为泪液生物标记物模型的免疫球蛋白 G。比色和表面增强拉曼散射(SERS)双信号读出的传感机制归因于锚定在电浆纸上的 Ag 纳米粒子的蚀刻。这种蚀刻既导致了质子纸的颜色偏移,也降低了质子纸的拉曼增强效果。优化的蚀刻系统证明了在等离子基底上同时进行免疫测定和蚀刻的可行性,而无需额外的蚀刻步骤。检测浓度比生理泪液浓度低约 100 倍,并能在模拟泪液中进行选择性检测。此外,双模式检测通过比较重叠检测范围的结果提高了准确性和效率,并能在进行 SERS 分析之前用比色法结果进行预筛选。这种方法有望成为一种多功能的护理点传感平台,能够轻松可靠地检测泪液生物标记物。
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引用次数: 0
Synthesis of Copper Oxide Nanoparticles via Laser Ablation in Liquid for Enhancing Spectral Responsivity 在液体中通过激光烧蚀合成纳米氧化铜颗粒以增强光谱响应性
IF 3 4区 物理与天体物理 Q2 CHEMISTRY, PHYSICAL Pub Date : 2024-08-31 DOI: 10.1007/s11468-024-02472-5
Salah M. Abdul Aziz, Uday M. Nayef, Mohammed Rasheed

This research included the production of copper oxide nanoparticles (CuO NPs) using various pulsed laser ablation energy (PLAL) embedded in substrates made of porous silicon (PS). The PS substrates were created using the photoelectrochemical etching (PECE) technique of Si n-type (111). The research examined the impact of pulse laser ablation energy on many attributes of the created samples, involving their structural, electrical, optical, photodetector, and morphological properties. XRD analysis reveals a prominent and broad diffraction peak at an angle of 28.4ο for the porous silicon and other diffraction peaks at different angles, indicating the presence of the CuO NPs phase corresponding to the monoclinic crystal structure. The SEM image demonstrates that PS is sponge-like, while CuO NPs display randomly dispersed spherical grains, and appear to vary in the particle size due to the change in laser pulses energy.

The optical properties of the fabricated specimens were analyzed utilizing photoluminescence and UV–vis absorption spectroscopy. The results suggested that a change in laser pulse energy caused a change in the energy gap that ranges from 2.7 to 3.5 eV. The created samples' current density-voltage (J-V) characteristics were analyzed under two conditions: in dark and light while varying the laser pulse energy. The J-V characteristics curves demonstrate that increasing the pulse energies of laser ablation resulted in higher current density flowing through the samples, particularly when the sample was created at 900 mJ. The photocurrent density exhibited a significant association with the increase in input light intensity, so enabling its utilization as a photodetector device. Nevertheless, altering the laser ablation pulse energy resulted in modifying the photocurrent for all CuO NPs/PS specimens. The inclusion of CuO nanoparticles in the PS samples led to a considerable enhancement in the responsivity (Rλ) when compared to the PS-only sample. The reason for this is that CuO nanoparticles have the ability to absorb light throughout a wide range of wavelengths, from ultraviolet-visible to near-infrared. The highest detectivity (D*) value was recorded when the laser energy was set at 700 mJ. The observed phenomena can be ascribed to fluctuations in the size or morphology of CuO NPs caused by variations in laser ablation pulse energy during its preparation. Furthermore, the constructed photodetector exhibited enhanced external quantum efficiency (Q.E), specifically in the ultraviolet (UV) range. The findings of this research are significant in the progress of optoelectronic and photodetector devices that rely on CuO NPs and PS.

这项研究包括利用嵌入多孔硅(PS)基底的各种脉冲激光烧蚀能量(PLAL)生产氧化铜纳米粒子(CuO NPs)。多孔硅衬底是利用硅 n 型(111)的光电化学蚀刻(PECE)技术制作的。研究考察了脉冲激光烧蚀能量对所制备样品多种属性的影响,包括其结构、电气、光学、光电探测器和形态特性。XRD 分析显示,多孔硅在 28.4ο 角处有一个突出而宽广的衍射峰,在不同角度还有其他衍射峰,表明存在与单斜晶体结构相对应的 CuO NPs 相。扫描电子显微镜图像显示 PS 呈海绵状,而 CuO NPs 则呈随机分散的球形颗粒,并且由于激光脉冲能量的变化而出现粒度变化。利用光致发光和紫外-可见吸收光谱分析了制备试样的光学特性。结果表明,激光脉冲能量的变化会导致能隙的变化,范围在 2.7 至 3.5 eV 之间。在两种条件下分析了所制样品的电流密度-电压(J-V)特性:黑暗和光明,同时改变激光脉冲能量。J-V 特性曲线表明,激光烧蚀脉冲能量的增加导致流过样品的电流密度增大,尤其是当样品的激光能量为 900 mJ 时。光电流密度与输入光强度的增加有明显的关联,因此可以用作光电探测器设备。然而,改变激光烧蚀脉冲能量会改变所有 CuO NPs/PS 样品的光电流。与纯 PS 样品相比,在 PS 样品中加入 CuO 纳米粒子可显著提高响应率(Rλ)。原因在于 CuO 纳米粒子能够吸收从紫外-可见光到近红外等各种波长的光。当激光能量设置为 700 mJ 时,记录到的检测率 (D*) 值最高。观察到的现象可归因于制备过程中激光烧蚀脉冲能量的变化导致的 CuO NPs 尺寸或形态的波动。此外,所构建的光电探测器显示出更高的外部量子效率(Q.E),尤其是在紫外线(UV)范围内。这项研究成果对于依赖 CuO NPs 和 PS 的光电和光电探测器设备的发展具有重要意义。
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引用次数: 0
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Plasmonics
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