首页 > 最新文献

arXiv: Applied Physics最新文献

英文 中文
Surface magnetic structure investigation of a nanolaminated Mn$_2$GaC thin film using a magnetic field microscope based on Nitrogen-Vacancy centers 基于氮空位中心的磁场显微镜研究纳米层状Mn$_2$GaC薄膜的表面磁性结构
Pub Date : 2020-11-11 DOI: 10.1016/J.MATCHEMPHYS.2021.124972
A. Berzins, J. Smits, A. Petruhins, Hugo Grube
{"title":"Surface magnetic structure investigation of a nanolaminated Mn$_2$GaC thin film using a magnetic field microscope based on Nitrogen-Vacancy centers","authors":"A. Berzins, J. Smits, A. Petruhins, Hugo Grube","doi":"10.1016/J.MATCHEMPHYS.2021.124972","DOIUrl":"https://doi.org/10.1016/J.MATCHEMPHYS.2021.124972","url":null,"abstract":"","PeriodicalId":8423,"journal":{"name":"arXiv: Applied Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-11-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"73848577","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Emergent Magnetic Monopole and Dipole Screening by Proximity Effect With Noble Metal 贵金属邻近效应筛选涌现磁单极子和偶极子
Pub Date : 2020-11-10 DOI: 10.21203/rs.3.rs-136395/v1
F. F. Martins, T. S. Paiva, Daniel G. Duarte, J. H. Rodrigues, L. M'ol, Jerome Borme Paulo P. Freitas, C. Araujo
In this work we present emergent screening of magnetic monopole and dipole by the presence of 20nm aluminum cover layer onsquare artificial spin ice (ASI) systems. Our results were obtained in base of magnetic atomic force measurements, performedafter external magnetic field steps application. We show that the evolution of magnetization and monopole population is affectedby the aluminum presence and attribute that phenomena to the proximity effect, which is responsible for the magnetizationvanish of the first atomic layers at the ferromagnetic interface. Using experimental values to estimate the decrease in thenanomagnetic dipole value used in an emergent excitation model and in the switching field distribution heterogeneity usedin simulations, we observe a very good agreement among experimental and simulation results. The presented emergentscreening could be used in new ASI geometries for thermodynamic activation or proposition of devices with selective magneticmonopole mobility.
在这项工作中,我们提出了通过在方形人工自旋冰(ASI)系统上存在20nm铝覆盖层来紧急筛选磁单极子和偶极子。我们的结果是在磁原子力测量的基础上,在外加磁场步骤应用后得到的。我们发现铝的存在影响了磁化和单极子居群的演变,并将这种现象归因于邻近效应,这是导致铁磁界面处第一原子层磁化消失的原因。利用实验值来估计紧急激励模型中使用的异磁偶极子值的减小和模拟中使用的开关场分布不均一性,我们观察到实验结果和模拟结果非常吻合。所提出的紧急筛选可以用于新的ASI几何形状,用于热力学激活或具有选择性磁单极子迁移率的器件的提出。
{"title":"Emergent Magnetic Monopole and Dipole Screening by Proximity Effect With Noble Metal","authors":"F. F. Martins, T. S. Paiva, Daniel G. Duarte, J. H. Rodrigues, L. M'ol, Jerome Borme Paulo P. Freitas, C. Araujo","doi":"10.21203/rs.3.rs-136395/v1","DOIUrl":"https://doi.org/10.21203/rs.3.rs-136395/v1","url":null,"abstract":"\u0000 In this work we present emergent screening of magnetic monopole and dipole by the presence of 20nm aluminum cover layer onsquare artificial spin ice (ASI) systems. Our results were obtained in base of magnetic atomic force measurements, performedafter external magnetic field steps application. We show that the evolution of magnetization and monopole population is affectedby the aluminum presence and attribute that phenomena to the proximity effect, which is responsible for the magnetizationvanish of the first atomic layers at the ferromagnetic interface. Using experimental values to estimate the decrease in thenanomagnetic dipole value used in an emergent excitation model and in the switching field distribution heterogeneity usedin simulations, we observe a very good agreement among experimental and simulation results. The presented emergentscreening could be used in new ASI geometries for thermodynamic activation or proposition of devices with selective magneticmonopole mobility.","PeriodicalId":8423,"journal":{"name":"arXiv: Applied Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-11-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"85643345","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Void engineering in epitaxially regrown GaAs-based photonic crystal surface emitting lasers by grating profile design 基于光栅轮廓设计的外延再生gaas光子晶体表面发射激光器中的空洞工程
Pub Date : 2020-11-09 DOI: 10.1063/5.0035038
A. McKenzie, B. King, K. Rae, S. Thoms, N. Gerrard, J. Orchard, K. Nishi, K. Takemasa, M. Sugawara, R. J. Taylor, D. Childs, D. Maclaren, R. Hogg
We report the engineering of air-voids embedded in GaAs-based photonic crystal surface emitting lasers realised by metalorganic vapour-phase epitaxy regrowth. Two distinct void geometries are obtained by modifying the photonic crystal grating profile within the reactor prior to regrowth. The mechanism of void formation is inferred from scanning transmission electron microscopy analysis, with the evolution of the growth front illustrated though the use of an AlAs/GaAs superlattice structure. Competition between rapid lateral growth of the (100) surface and slow diffusion across higher index planes is exploited in order to increase void volume, leading to an order of magnitude reduction in threshold current and an increase in output power through an increase in the associated grating coupling strength.
本文报道了利用金属有机气相外延再生技术在gaas基光子晶体表面发射激光器中嵌入空腔的工程。在再生之前,通过修改反应器内的光子晶体光栅轮廓,获得了两种不同的空隙几何形状。通过扫描透射电子显微镜分析推断了空洞形成的机制,并通过使用AlAs/GaAs超晶格结构说明了生长锋的演变。(100)表面的快速横向增长和在更高折射率平面上的缓慢扩散之间的竞争被利用,以增加空隙体积,导致阈值电流降低一个数量级,并通过增加相关光栅耦合强度增加输出功率。
{"title":"Void engineering in epitaxially regrown GaAs-based photonic crystal surface emitting lasers by grating profile design","authors":"A. McKenzie, B. King, K. Rae, S. Thoms, N. Gerrard, J. Orchard, K. Nishi, K. Takemasa, M. Sugawara, R. J. Taylor, D. Childs, D. Maclaren, R. Hogg","doi":"10.1063/5.0035038","DOIUrl":"https://doi.org/10.1063/5.0035038","url":null,"abstract":"We report the engineering of air-voids embedded in GaAs-based photonic crystal surface emitting lasers realised by metalorganic vapour-phase epitaxy regrowth. Two distinct void geometries are obtained by modifying the photonic crystal grating profile within the reactor prior to regrowth. The mechanism of void formation is inferred from scanning transmission electron microscopy analysis, with the evolution of the growth front illustrated though the use of an AlAs/GaAs superlattice structure. Competition between rapid lateral growth of the (100) surface and slow diffusion across higher index planes is exploited in order to increase void volume, leading to an order of magnitude reduction in threshold current and an increase in output power through an increase in the associated grating coupling strength.","PeriodicalId":8423,"journal":{"name":"arXiv: Applied Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-11-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"90402720","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 8
Charge coloration dynamics of electrochromic amorphous tungsten oxide studied by simultaneous electrochemical and color impedance measurements 采用电化学和颜色阻抗同步测量方法研究了电致变色非晶氧化钨的电荷着色动力学
Pub Date : 2020-11-08 DOI: 10.1063/5.0038531
Edgar A. Rojas-González, G. Niklasson
The coloration mechanisms in electrochromic (EC) systems can be probed by comparing the dynamics of the electrical and optical responses. In this paper, the linear frequency-dependent electrical and optical responses of an amorphous tungsten oxide thin film were measured simultaneously by a combination of two techniques$text{---}$that is, electrochemical impedance spectroscopy (EIS) and the so-called color impedance spectroscopy (CIS). This was done at different bias potentials, which can be associated with different intercalation levels. Equivalent circuit fitting to the EIS spectra was used to extract the Faradaic components participating in the total impedance response. The latter were assigned to an intermediate adsorption step before the intercalation and to the diffusion of the electron-ion couple in the film. A quantity denoted complex optical capacitance is compared to the complex electrical capacitance$text{---}$in particular, their expressions are related to the Faradaic processes. The coloration at low intercalation levels followed both the adsorption and diffusion phenomena. Conversely, the diffusion contribution was dominant at high intercalation levels and the adsorption one seemed to be negligible in this case. For perfectly synchronized electrical and optical responses, their complex spectra are expected to differ only by a multiplying factor. This was the case at low intercalation levels, apart from small deviations at high frequencies. A clear departure from this behavior was observed as the intercalation level increased. A combination of frequency-dependent techniques, as presented in this work, can help in the understanding of the dynamics of the coloration mechanisms in EC materials at various conditions$text{---}$for example, at different intercalation levels and optical wavelengths.
电致变色(EC)系统的显色机制可以通过比较电响应和光学响应的动力学来探讨。本文采用电化学阻抗谱(EIS)和色阻抗谱(CIS)两种技术的结合,同时测量了非晶氧化钨薄膜的线性频率相关的电学和光学响应。这是在不同的偏置电位下完成的,这可能与不同的插层水平有关。利用等效电路拟合EIS谱,提取参与总阻抗响应的法拉第分量。后者被分配到插入前的中间吸附步骤和薄膜中电子-离子对的扩散。将复光学电容与复电容量$text{—}$进行比较,特别地,它们的表达式与法拉第过程有关。低插层层的着色遵循了吸附和扩散现象。相反,在高插层水平上,扩散作用占主导地位,在这种情况下,吸附作用似乎可以忽略不计。对于完全同步的电学和光学响应,它们的复杂光谱预计只相差一个乘因子。这是在低插入电平的情况,除了在高频率的小偏差。随着嵌入水平的增加,观察到这种行为明显偏离。在这项工作中提出的频率相关技术的组合可以帮助理解EC材料在不同条件下(例如,在不同的插层水平和光学波长下)的着色机制的动力学。
{"title":"Charge coloration dynamics of electrochromic amorphous tungsten oxide studied by simultaneous electrochemical and color impedance measurements","authors":"Edgar A. Rojas-González, G. Niklasson","doi":"10.1063/5.0038531","DOIUrl":"https://doi.org/10.1063/5.0038531","url":null,"abstract":"The coloration mechanisms in electrochromic (EC) systems can be probed by comparing the dynamics of the electrical and optical responses. In this paper, the linear frequency-dependent electrical and optical responses of an amorphous tungsten oxide thin film were measured simultaneously by a combination of two techniques$text{---}$that is, electrochemical impedance spectroscopy (EIS) and the so-called color impedance spectroscopy (CIS). This was done at different bias potentials, which can be associated with different intercalation levels. Equivalent circuit fitting to the EIS spectra was used to extract the Faradaic components participating in the total impedance response. The latter were assigned to an intermediate adsorption step before the intercalation and to the diffusion of the electron-ion couple in the film. A quantity denoted complex optical capacitance is compared to the complex electrical capacitance$text{---}$in particular, their expressions are related to the Faradaic processes. The coloration at low intercalation levels followed both the adsorption and diffusion phenomena. Conversely, the diffusion contribution was dominant at high intercalation levels and the adsorption one seemed to be negligible in this case. For perfectly synchronized electrical and optical responses, their complex spectra are expected to differ only by a multiplying factor. This was the case at low intercalation levels, apart from small deviations at high frequencies. A clear departure from this behavior was observed as the intercalation level increased. A combination of frequency-dependent techniques, as presented in this work, can help in the understanding of the dynamics of the coloration mechanisms in EC materials at various conditions$text{---}$for example, at different intercalation levels and optical wavelengths.","PeriodicalId":8423,"journal":{"name":"arXiv: Applied Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-11-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"82831670","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 5
Designing drones by combining finite element and atomistic simulations: a didactic approach 结合有限元和原子模拟设计无人机:一种教学方法
Pub Date : 2020-11-04 DOI: 10.1478/AAPP.99S1A33
M. Raffaele, M. T. Caccamo, G. Castorina, S. Lanza, S. Magazù, G. Munaò, G. Randazzo
A didactic multiscale approach for drone modeling is proposed. Specifically, we investigate the drone structure at both macroscopic and microscopic scales, by making use of finite element and atomistic simulations, respectively. The structural analysis is performed with the aim to equip the drone with specific sensors and measuring instruments capable to detect the existence of volcanic ash, SO2 , CO2 and other pollutants in the atmosphere after a vulcanic eruption. We show that, by modeling the tubular structure of the drone with a sandwich constituted by a a polystyrene core, carbon fiber skins and epoxy matrix, a weight saving of 7 grams for each drone arm can be obtained, in comparison to the standard commercial drones, although a slight worsening of the mechanical performances is observed. In addition, the molecular structure of the polystyrene chains has been investigated by using atomistic Molecular Dynamics simulations, providing further information on the local structure of the polymer chains. Additional improvements of the weight saving could be obtained by means of the the topological optimization techniques on the body of the drone and on the supports for landing.
提出了一种教学式多尺度无人机建模方法。具体来说,我们研究无人机结构在宏观和微观尺度,分别利用有限元和原子模拟。进行结构分析的目的是为无人机配备特定的传感器和测量仪器,以便在火山爆发后检测大气中是否存在火山灰、二氧化硫、二氧化碳和其他污染物。我们表明,通过对由聚苯乙烯核心、碳纤维皮肤和环氧树脂基体组成的三明治构成的无人机管状结构进行建模,与标准商用无人机相比,每个无人机手臂的重量减轻了7克,尽管观察到机械性能略有恶化。此外,利用原子分子动力学模拟研究了聚苯乙烯链的分子结构,为聚合物链的局部结构提供了进一步的信息。通过对无人机本体和着陆支撑的拓扑优化技术,可以进一步提高无人机的减重效果。
{"title":"Designing drones by combining finite element and atomistic simulations: a didactic approach","authors":"M. Raffaele, M. T. Caccamo, G. Castorina, S. Lanza, S. Magazù, G. Munaò, G. Randazzo","doi":"10.1478/AAPP.99S1A33","DOIUrl":"https://doi.org/10.1478/AAPP.99S1A33","url":null,"abstract":"A didactic multiscale approach for drone modeling is proposed. Specifically, we investigate the drone structure at both macroscopic and microscopic scales, by making use of finite element and atomistic simulations, respectively. The structural analysis is performed with the aim to equip the drone with specific sensors and measuring instruments capable to detect the existence of volcanic ash, SO2 , CO2 and other pollutants in the atmosphere after a vulcanic eruption. We show that, by modeling the tubular structure of the drone with a sandwich constituted by a a polystyrene core, carbon fiber skins and epoxy matrix, a weight saving of 7 grams for each drone arm can be obtained, in comparison to the standard commercial drones, although a slight worsening of the mechanical performances is observed. In addition, the molecular structure of the polystyrene chains has been investigated by using atomistic Molecular Dynamics simulations, providing further information on the local structure of the polymer chains. Additional improvements of the weight saving could be obtained by means of the the topological optimization techniques on the body of the drone and on the supports for landing.","PeriodicalId":8423,"journal":{"name":"arXiv: Applied Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-11-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"79631315","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Cost-Performance Trade-off in thermoelectric air conditioning system with graded and constant material properties 具有分级和恒定材料性能的热电空调系统的成本性能权衡
Pub Date : 2020-11-04 DOI: 10.1016/J.ENBUILD.2021.110931
A. Saini, Sarah J. Watzman, J. Bahk
{"title":"Cost-Performance Trade-off in thermoelectric air conditioning system with graded and constant material properties","authors":"A. Saini, Sarah J. Watzman, J. Bahk","doi":"10.1016/J.ENBUILD.2021.110931","DOIUrl":"https://doi.org/10.1016/J.ENBUILD.2021.110931","url":null,"abstract":"","PeriodicalId":8423,"journal":{"name":"arXiv: Applied Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-11-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"88121837","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 7
Spin wave propagation in corrugated waveguides 自旋波在波纹波导中的传播
Pub Date : 2020-11-02 DOI: 10.1063/5.0041138
Igor Turčan, L. Flajšman, O. Wojewoda, Václav Roučka, O. Man, M. Urbánek
Curvature-induced effects allow us to tailor the static and dynamic response of a magnetic system with a high degree of freedom. We study corrugated magnonic waveguides deposited on a sinusoidally modulated substrate prepared by focused electron beam deposition. The surface curvature in films with thicknesses comparable to the amplitude of modulation locally modifies the contributions of dipolar and exchange energies and results in an effective anisotropy term which can be tuned on-demand based on the exact geometry. We show, by Brillouin light scattering microscopy, that without the presence of an external magnetic field, spin waves propagate over a distance 10$times$larger in the corrugated waveguide than in the planar waveguide. Further, we analyze the influence of the modulation amplitude on spin-wave propagation and conclude that for moderate modulation amplitudes, the spin-wave decay length is not affected. For larger amplitudes, the decay length decreases linearly with increasing modulation.
曲率诱导效应使我们能够高度自由地定制磁系统的静态和动态响应。本文研究了用聚焦电子束沉积法在正弦波调制衬底上沉积的波纹磁波导。厚度与调制幅度相当的薄膜的表面曲率局部改变了偶极和交换能的贡献,并产生了有效的各向异性项,该项可以根据精确的几何形状按需调整。我们通过布里渊光散射显微镜显示,在没有外部磁场存在的情况下,自旋波在波纹波导中的传播距离比在平面波导中的传播距离大10倍。进一步,我们分析了调制幅值对自旋波传播的影响,并得出结论,当调制幅值适中时,自旋波衰减长度不受影响。对于较大的振幅,衰减长度随着调制的增加而线性减小。
{"title":"Spin wave propagation in corrugated waveguides","authors":"Igor Turčan, L. Flajšman, O. Wojewoda, Václav Roučka, O. Man, M. Urbánek","doi":"10.1063/5.0041138","DOIUrl":"https://doi.org/10.1063/5.0041138","url":null,"abstract":"Curvature-induced effects allow us to tailor the static and dynamic response of a magnetic system with a high degree of freedom. We study corrugated magnonic waveguides deposited on a sinusoidally modulated substrate prepared by focused electron beam deposition. The surface curvature in films with thicknesses comparable to the amplitude of modulation locally modifies the contributions of dipolar and exchange energies and results in an effective anisotropy term which can be tuned on-demand based on the exact geometry. We show, by Brillouin light scattering microscopy, that without the presence of an external magnetic field, spin waves propagate over a distance 10$times$larger in the corrugated waveguide than in the planar waveguide. Further, we analyze the influence of the modulation amplitude on spin-wave propagation and conclude that for moderate modulation amplitudes, the spin-wave decay length is not affected. For larger amplitudes, the decay length decreases linearly with increasing modulation.","PeriodicalId":8423,"journal":{"name":"arXiv: Applied Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-11-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"75607928","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 9
Transient grating spectroscopy of photocarrier dynamics in semiconducting polymer thin films 半导体聚合物薄膜中光载流子动力学的瞬态光栅光谱
Pub Date : 2020-10-29 DOI: 10.1063/5.0034773
Wenkai Ouyang, Yu Li, Brett Yurash, N. Schopp, A. Vega-Flick, V. Brus, Thuc‐Quyen Nguyen, Bolin Liao
While charge carrier dynamics and thermal management are both keys to the operational efficiency and stability for energy-related devices, experimental techniques that can simultaneously characterize both properties are still lacking. In this paper, we use laser-induced transient grating (TG) spectroscopy to characterize thin films of the archetypal organic semiconductor regioregular poly(3-hexylthiophene) (P3HT) and its blends with the electron acceptor [6,6]-phenyl-C61-butyric acid methyl ester (PCBM) on glass substrates. While the thermal response is determined to be dominated by the substrates, we show that the recombination dynamics of photocarriers in the organic semiconductor thin films occur on a similar timescale and can be separated from the thermal response. Our measurements indicate that the photocarrier dynamics are determined by multiple recombination processes and our extracted recombination rates are in good agreement with previous reports using other techniques. We further apply TG spectroscopy to characterize another conjugated polymer and a molecular fluorescent material to demonstrate its general applicability. Our study indicates the potential of transient grating spectroscopy to simultaneously characterize thermal transport and photocarrier dynamics in organic optoelectronic devices.
虽然载流子动力学和热管理都是能源相关设备运行效率和稳定性的关键,但能够同时表征这两种特性的实验技术仍然缺乏。在本文中,我们使用激光诱导瞬态光栅(TG)光谱来表征原型有机半导体区域规则聚(3-己基噻吩)(P3HT)及其与电子受体[6,6]-苯基- c61 -丁酸甲酯(PCBM)共混物在玻璃衬底上的薄膜。虽然热响应被确定为由衬底主导,但我们表明有机半导体薄膜中光载流子的重组动力学发生在相似的时间尺度上,并且可以与热响应分离。我们的测量表明,光载流子动力学是由多个重组过程决定的,我们提取的重组率与以前使用其他技术的报道很好地一致。我们进一步应用热重光谱来表征另一种共轭聚合物和一种分子荧光材料,以证明其普遍适用性。我们的研究表明,瞬态光栅光谱可以同时表征有机光电器件中的热输运和光载流子动力学。
{"title":"Transient grating spectroscopy of photocarrier dynamics in semiconducting polymer thin films","authors":"Wenkai Ouyang, Yu Li, Brett Yurash, N. Schopp, A. Vega-Flick, V. Brus, Thuc‐Quyen Nguyen, Bolin Liao","doi":"10.1063/5.0034773","DOIUrl":"https://doi.org/10.1063/5.0034773","url":null,"abstract":"While charge carrier dynamics and thermal management are both keys to the operational efficiency and stability for energy-related devices, experimental techniques that can simultaneously characterize both properties are still lacking. In this paper, we use laser-induced transient grating (TG) spectroscopy to characterize thin films of the archetypal organic semiconductor regioregular poly(3-hexylthiophene) (P3HT) and its blends with the electron acceptor [6,6]-phenyl-C61-butyric acid methyl ester (PCBM) on glass substrates. While the thermal response is determined to be dominated by the substrates, we show that the recombination dynamics of photocarriers in the organic semiconductor thin films occur on a similar timescale and can be separated from the thermal response. Our measurements indicate that the photocarrier dynamics are determined by multiple recombination processes and our extracted recombination rates are in good agreement with previous reports using other techniques. We further apply TG spectroscopy to characterize another conjugated polymer and a molecular fluorescent material to demonstrate its general applicability. Our study indicates the potential of transient grating spectroscopy to simultaneously characterize thermal transport and photocarrier dynamics in organic optoelectronic devices.","PeriodicalId":8423,"journal":{"name":"arXiv: Applied Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-10-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77974503","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 2
Revealing the internal luminescence quantum efficiency of perovskite films via accurate quantification of photon recycling 通过光子回收的精确量化揭示钙钛矿薄膜的内部发光量子效率
Pub Date : 2020-10-24 DOI: 10.1016/J.MATT.2021.01.019
P. Fassl, Vincent Lami, Felix J. Berger, Lukas M. Falk, J. Zaumseil, B. Richards, I. Howard, Y. Vaynzof, U. Paetzold
{"title":"Revealing the internal luminescence quantum efficiency of perovskite films via accurate quantification of photon recycling","authors":"P. Fassl, Vincent Lami, Felix J. Berger, Lukas M. Falk, J. Zaumseil, B. Richards, I. Howard, Y. Vaynzof, U. Paetzold","doi":"10.1016/J.MATT.2021.01.019","DOIUrl":"https://doi.org/10.1016/J.MATT.2021.01.019","url":null,"abstract":"","PeriodicalId":8423,"journal":{"name":"arXiv: Applied Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-10-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"80862163","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 28
Ultrabroadband Acoustic Ventilation Barriers via Hybrid-Functional Metasurfaces 基于混合功能超表面的超宽带声通风屏障
Pub Date : 2020-10-16 DOI: 10.1103/PHYSREVAPPLIED.15.024044
Ruizhi Dong, Dongxing Mao, Xu Wang, Yong Li
Ventilation barriers allowing simultaneous sound blocking and free airflow passage are of great challenge but necessary for particular scenarios calling for sound-proofing ventilation. Previous works based on local resonance or Fano-like interference serve a narrow working range around the resonant or destructive-interference frequency. Efforts made on broadband designs show a limited bandwidth typically smaller than half an octave. Here, we theoretically design an ultra-broadband ventilation barrier via hybridizing dissipation and interference. Confirmed by experiments, the synergistic effect from our hybrid-functional metasurface significantly expand the scope of its working frequencies, leading to an effective blocking of more than 90% of incident energy in the range of 650-2000 Hz, while its structural thickness is only 53 mm $(sim lambda / 10)$. Our design shows great flexibility in customizing the broadband and is capable of handling sound coming from various directions, which has potential in air-permeable yet sound-proofing applications.
能够同时阻挡声音和自由气流通过的通风屏障是一个巨大的挑战,但对于需要隔音通风的特定场景是必要的。以往基于局部共振或类法诺干扰的工作范围在谐振或消毁干扰频率附近很窄。在宽带设计上所做的努力表明,有限的带宽通常小于半个八度。在这里,我们从理论上设计了一种通过杂化耗散和干扰的超宽带通风屏障。实验证实,我们的混合功能超表面的协同效应显着扩大了其工作频率的范围,导致有效阻断超过90% of incident energy in the range of 650-2000 Hz, while its structural thickness is only 53 mm $(sim lambda / 10)$. Our design shows great flexibility in customizing the broadband and is capable of handling sound coming from various directions, which has potential in air-permeable yet sound-proofing applications.
{"title":"Ultrabroadband Acoustic Ventilation Barriers via Hybrid-Functional Metasurfaces","authors":"Ruizhi Dong, Dongxing Mao, Xu Wang, Yong Li","doi":"10.1103/PHYSREVAPPLIED.15.024044","DOIUrl":"https://doi.org/10.1103/PHYSREVAPPLIED.15.024044","url":null,"abstract":"Ventilation barriers allowing simultaneous sound blocking and free airflow passage are of great challenge but necessary for particular scenarios calling for sound-proofing ventilation. Previous works based on local resonance or Fano-like interference serve a narrow working range around the resonant or destructive-interference frequency. Efforts made on broadband designs show a limited bandwidth typically smaller than half an octave. Here, we theoretically design an ultra-broadband ventilation barrier via hybridizing dissipation and interference. Confirmed by experiments, the synergistic effect from our hybrid-functional metasurface significantly expand the scope of its working frequencies, leading to an effective blocking of more than 90% of incident energy in the range of 650-2000 Hz, while its structural thickness is only 53 mm $(sim lambda / 10)$. Our design shows great flexibility in customizing the broadband and is capable of handling sound coming from various directions, which has potential in air-permeable yet sound-proofing applications.","PeriodicalId":8423,"journal":{"name":"arXiv: Applied Physics","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-10-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"75073743","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 18
期刊
arXiv: Applied Physics
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1