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Observation of strong two-electron–one-photon transitions in few-electron ions 少电子离子中强双电子-单光子跃迁的观察
Pub Date : 2020-11-25 DOI: 10.1103/physreva.102.052831
M. Togawa, S. Kühn, C. Shah, P. Amaro, R. Steinbrügge, J. Stierhof, N. Hell, M. Rosner, K. Fujii, M. Bissinger, R. Ballhausen, M. Hoesch, J. Seltmann, Sungnam Park, Filipe Grilo, F. Porter, J. Santos, M. Chung, T. Stöhlker, J. Wilms, T. Pfeifer, G. Brown, M. Leutenegger, S. Bernitt, José R. Crespo López-Urrutia
We resonantly excite the $K$ series of O$^{5+}$ and O$^{6+}$ up to principal quantum number $n=11$ with monochromatic x rays, producing $K$-shell holes, and observe their relaxation by soft-x-ray emission. Some photoabsorption resonances of O$^{5+}$ reveal strong two-electron--one-photon (TEOP) transitions. We find that for the $[(1s,2s)_1,5p_{3/2}]_{3/2;1/2}$ states, TEOP relaxation is by far stronger than the radiative decay and competes with the usually much faster Auger decay path. This enhanced TEOP decay arises from a strong correlation with the near-degenerate upper states $[(1s,2p_{3/2})_1,4s]_{3/2;1/2}$ of a Li-like satellite blend of the He-like $Kalpha$ transition. Even in three-electron systems, TEOP transitions can play a dominant role, and the present results should guide further research on the ubiquitous and abundant many-electron ions where electronic energy degeneracies are far more common and configuration mixing is stronger.
我们用单色x射线共振激发O$^{5+}$和O$^{6+}$到主量子数n=11$的$K$系列,产生$K$壳孔,并通过软x射线发射观察它们的弛豫。O$^{5+}$的一些光吸收共振显示出强的双电子-单光子跃迁。我们发现对于$[(1s,2s)_1,5p_{3/2}]_{3/2;1/2}$态,TEOP弛豫比辐射衰减强得多,并与通常更快的俄歇衰变路径竞争。这种增强的TEOP衰减是由于类锂卫星混合类氦K α跃迁的近简并态$[(1s,2p_{3/2})_1,4s]_{3/2;1/2}$密切相关。即使在三电子体系中,TEOP跃迁也可以发挥主导作用,目前的结果应该指导对普遍存在和丰富的多电子离子的进一步研究,在这些多电子离子中,电子能量简并更为常见,组态混合更强。
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引用次数: 2
Electron-impact ionization and ionic fragmentation of O2 from threshold to 120 eV energy range 从阈值到120ev能量范围O2的电子冲击电离和离子碎裂
Pub Date : 2020-11-24 DOI: 10.1142/S0217979221501046
R. Lomsadze, M. Gochitashvili, R. Kezerashvili, M. Schulz
We study the electron-impact induced ionization of O$_{2}$ from threshold to 120 eV using the electron spectroscopy method. Our approach is simple in concept and embodies the ion source with a collision chamber and a mass spectrometer with a quadruple filter as a selector for the product ions. The combination of these two devices makes it possible to unequivocally collect all energetic fragment ions formed in ionization and dissociative processes and to detect them with known efficiency. The ion source allows to vary and tune the electron-impact ionization energy and the target-gas pressure. We demonstrate that for obtaining reliable results of cross sections for inelastic processes and determining mechanisms for the formation of O$^{+}$($^{4}S,^2{D},^2{P}$) ions, it is crucial to control the electron-impact energy for production of ion and the pressure in the ion source. A comparison of our results with other experimental and theoretical data shows good agreement and proves the validity of our approach.
我们用电子能谱法研究了O$_{2}$从阈值到120 eV的电子碰撞诱导电离。我们的方法在概念上是简单的,包括离子源与碰撞室和质谱仪与四重过滤器作为产物离子的选择器。这两种装置的结合使得明确地收集在电离和解离过程中形成的所有高能碎片离子并以已知的效率检测它们成为可能。离子源允许改变和调整电子冲击电离能和目标气体压力。我们证明了为了获得可靠的非弹性过程截面结果和确定O$^{+}$($^{4}S,^2{D},^2{P}$)离子形成机制,控制离子产生的电子冲击能和离子源压力是至关重要的。将所得结果与其它实验和理论数据进行了比较,结果一致,证明了方法的有效性。
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引用次数: 0
Time- and frequency-domain two-particle correlations of a driven dissipative Bose-Hubbard model 驱动耗散Bose-Hubbard模型的时频域两粒子相关性
Pub Date : 2020-11-23 DOI: 10.1103/PHYSREVA.103.033310
Kingshuk Adhikary, Anushree Dey, Arpita Pal, S. Mal, B. Deb
We theoretically investigate the time- and frequency-domain two-particle correlations of a driven dissipative Bose-Hubbard model (BHM) at and near a dissipative phase transition (DPT). We compute Hanbury Brown-Twiss (HBT) type two-particle temporal correlation function $g^2(tau)$ which, as a function of time delay $tau$, exhibits oscillations with frequencies determined by the imaginary part of Liouvillian gap. As the gap closes near a transition point, the oscillations at that point dies down. For parameters slightly away from the transition point, the HBT correlations show oscillations from super-bunching to anti-bunching regimes. We show that the Fourier transform of HBT correlations into frequency domain provide information about DPT and Liouvillian dynamics. We numerically solve the many-body Lindblad master equation and calculate Wigner distribution of the system in steady state to ascertain DPT. Below certain drive strength, the Fourier transform shows a two-peak structure while above that strength it exhibits either a Lorenzian-like single-peak structure or a structure with two-dips. The width of the single-peak structure is minimum at the phase transition point and the peak of this structure always lies at zero frequency. The positions of the two symmetrical peaks in case of two-peak structure are given by the imaginary parts of the Liouvillian gap while their half width at half maximum (HWHM) is given by the real part of the gap. The positions and the widths of the two dips are also related to low lying eigenvalues of the Liouvillian operator. We discuss quantum statistical properties of the model in terms of the HBT correlation function and its Fourier transform.
我们从理论上研究了驱动耗散玻色-哈伯德模型(BHM)在耗散相变(DPT)及其附近的时域和频域两粒子相关性。我们计算了Hanbury Brown-Twiss (HBT)型两粒子时间相关函数$g^2(tau)$,该函数作为时间延迟$tau$的函数,表现出频率由Liouvillian gap虚部决定的振荡。当间隙在过渡点附近关闭时,该点的振荡就会减弱。对于稍微远离过渡点的参数,HBT相关性显示出从超聚束到反聚束的振荡。我们证明了HBT相关到频域的傅里叶变换提供了DPT和Liouvillian动态的信息。通过数值求解多体Lindblad主方程,计算稳态下系统的Wigner分布来确定DPT。在一定的驱动强度以下,傅里叶变换表现为双峰结构,而在一定的驱动强度以上,傅里叶变换表现为类似洛伦兹的单峰结构或双倾角结构。单峰结构的宽度在相变点处最小,该结构的峰值始终位于零频率处。在双峰结构下,两个对称峰的位置由刘维廉隙的虚部给出,而它们在半最大值时的半宽度(HWHM)由隙的实部给出。两个倾角的位置和宽度也与Liouvillian算子的低特征值有关。我们从HBT相关函数及其傅里叶变换的角度讨论了该模型的量子统计特性。
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引用次数: 0
Enhanced atom-by-atom assembly of arbitrary tweezer arrays 增强任意镊子阵列的原子对原子组装
Pub Date : 2020-11-13 DOI: 10.1103/physreva.102.063107
Kai-Niklas Schymik, Vincent Lienhard, D. Barredo, P. Scholl, H. Williams, A. Browaeys, T. Lahaye
We report on improvements extending the capabilities of the atom-by-atom assembler described in [Barredo et al., Science 354, 1021 (2016)] that we use to create fully-loaded target arrays of more than 100 single atoms in optical tweezers, starting from randomly-loaded, half-filled initial arrays. We describe four variants of the sorting algorithm that (i) allow decrease the number of moves needed for assembly and (ii) enable the assembly of arbitrary, non-regular target arrays. We finally demonstrate experimentally the performance of this enhanced assembler for a variety of target arrays.
我们报告了在[Barredo et al., Science 354,1021(2016)]中描述的扩展原子-原子汇编器功能的改进,我们使用它在光学镊子中创建超过100个单原子的满载目标阵列,从随机加载,半填充的初始阵列开始。我们描述了排序算法的四种变体,它们(i)允许减少组装所需的移动次数,(ii)允许组装任意的、不规则的目标阵列。最后,我们通过实验证明了这种增强的汇编器对各种目标阵列的性能。
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引用次数: 42
Polarization-dependent disappearance of a resonance signal: Indication for optical pumping in a storage ring? 共振信号的偏振相关消失:存储环中光泵浦的指示?
Pub Date : 2020-11-09 DOI: 10.1103/PHYSREVACCELBEAMS.24.024701
W. Nörtershäuser, A. Surzhykov, R. Sánchez, B. Botermann, G. Gwinner, G. Huber, S. Karpuk, T. Kühl, C. Novotny, S. Reinhardt, G. Saathoff, T. Stöhlker, A. Wolf
We report on laser spectroscopic measurements on Li$^+$ ions in the experimental storage ring ESR at the GSI Helmholtz Centre for Heavy Ion Research. Driving the $2s,^3!{S}_1;(F=frac{3}{2}) ,leftrightarrow,2p,^3!P_2;(F=frac{5}{2}) leftrightarrow 2s,^3!{S}_1;(F=frac{5}{2})$ $Lambda$-transition in $^7$Li$^+$ with two superimposed laser beams it was found that the use of circularly polarized light leads to a disappearance of the resonance structure in the fluorescence signal. This can be explained by optical pumping into a dark state of polarized ions. We present a detailed theoretical analysis of this process that supports the interpretation of optical pumping and demonstrates that the polarization induced by the laser light must then be at least partially maintained during the round trip of the ions in the storage ring. Such polarized ion beams in storage rings will provide opportunities for new experiments, especially on parity violation.
我们报道了在GSI亥姆霍兹重离子研究中心的实验存储环ESR中Li $^+$离子的激光光谱测量。用两个叠加的激光束驱动$^7$ Li $^+$中的$2s,^3!{S}_1;(F=frac{3}{2}) ,leftrightarrow,2p,^3!P_2;(F=frac{5}{2}) leftrightarrow 2s,^3!{S}_1;(F=frac{5}{2})$$Lambda$ -跃迁,发现圆偏振光的使用导致荧光信号中的共振结构消失。这可以用光泵入偏振离子的暗态来解释。我们对这一过程进行了详细的理论分析,支持光泵浦的解释,并证明了在存储环中的离子往返期间,激光引起的偏振必须至少部分保持。这种存储环中的极化离子束将为新的实验提供机会,特别是在宇称破坏方面。
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引用次数: 1
Simulation of optical lattice trap loading from a cold atomic ensemble 冷原子系综光学晶格阱加载的模拟
Pub Date : 2020-10-27 DOI: 10.1364/josab.408521
R. S. Watson, J. McFerran
We model the efficiency of loading atoms of various species into a one dimensional optical lattice from a cold ensemble taking into account the initial cloud temperature and size, the lattice laser properties affecting the trapping potential, and atomic parameters. Stochastic sampling and dynamical evolution are used to simulate the transfer, leading to estimates of transfer efficiency for varying trap depth and profile. Tracing the motion of the atoms also enables the evaluation of the equilibrium temperature and site occupancy in the lattice. The simulation compares favourably against a number of experimental results, and is used to compute an optimum lattice-waist to cloud-radius ratio for a given optical power.
我们模拟了将不同种类的原子从冷系综加载到一维光学晶格中的效率,考虑了初始云温和尺寸、影响捕获势的晶格激光特性和原子参数。利用随机抽样和动态演化方法模拟了不同圈闭深度和剖面下的油气传递效率。跟踪原子的运动也可以评估平衡温度和晶格中的位置占用。该模拟与许多实验结果进行了比较,并用于计算给定光功率下的最佳格腰与云半径比。
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引用次数: 0
Fourier transform detection of weak optical transitions in atoms undergoing cyclic routines 循环过程中原子弱光学跃迁的傅里叶变换检测
Pub Date : 2020-10-23 DOI: 10.1063/5.0034217
J. Schelfhout, Lilani D. Toms-Hardman, J. McFerran
We demonstrate a means of detecting weak optical transitions in cold atoms that undergo cyclic routines with high sensitivity. The gain in sensitivity is made by probing atoms on alternate cycles leading to a regular modulation of the ground state atom population when at the resonance frequency. The atomic transition is identified by conducting a fast Fourier transform via algorithm or instrument. We find an enhancement of detection sensitivity compared to more conventional scanning methods of $sim 20$ for the same sampling time, and can detect clock lines with fewer than $10^3$ atoms in a magneto-optical trap. We apply the method to the $(6s^{2})$ $ ^{1}S_{0} - (6s6p)$ $^{3}P_{0}$ clock transition in $^{171}$Yb and $^{173}$Yb. The ac-Stark shift of this line in $^{171}$Yb is measured to be 0.19(3) kHz$cdot$W$^{-1}cdot$m$^2$ at 556 nm.
我们展示了一种检测冷原子中弱光学跃迁的方法,该方法具有高灵敏度。灵敏度的增益是通过在交替周期上探测原子来实现的,当处于共振频率时,导致基态原子居群的规则调制。原子跃迁是通过算法或仪器进行快速傅立叶变换来识别的。我们发现,在相同的采样时间内,与更传统的扫描方法相比,探测灵敏度提高了20美元,并且可以在磁光阱中探测到少于10^3美元原子的时钟线。我们将方法应用于美元(6 s ^ {2}) $ $ ^ {1} S_ {0} - - - - - - (6 s6p) $ $ ^ {3} P_{0}时钟转换美元$ ^ {171}$ Yb和$ ^ {173}Yb美元。这条线在$^{171}$Yb中的ac-Stark位移在556 nm处测量为0.19(3)kHz$cdot$W$^{-1}cdot$m$^2$。
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引用次数: 1
Tune-out wavelengths of the hyperfine components of the ground level of Cs133 atoms 调出Cs133原子底能级超精细成分的波长
Pub Date : 2020-10-21 DOI: 10.1103/physreva.102.042823
Jun Jiang, Xiangyu Li, Xia Wang, C. Dong, Z. Wu
The static and dynamic electric-dipole polarizabilities and tune-out wavelengths for the ground state of Cs atoms are calculated by using a semiempirical relativistic configuration interaction plus core polarization approach. By considering the hyperfine splittings, the static and dynamic polarizabilities, hyperfine Stark shifts, and tune-out wavelengths of the hyperfine components of the ground level of $^{133}$Cs atoms are determined. It is found that the hyperfine shifts of the first primary tune-out wavelengths are about $-$0.0135 nm and 0.0106 nm, which are very close to the hyperfine interaction energies. Additionally, the contribution of the tensor polarizability to the tune-out wavelengths is determined to be about $10^{-5} sim 10^{-6}$ nm.
采用半经验相对论组态相互作用加核心极化方法计算了Cs原子基态的静态和动态电偶极极化率和调谐波长。通过考虑超细分裂,确定了$^{133}$Cs原子地能级超细组分的静态和动态极化率、超细斯塔克位移和调谐波长。发现第一主调谐波长的超精细位移约为$-$0.0135 nm和0.0106 nm,与超精细相互作用能非常接近。此外,张量极化率对调谐波长的贡献约为$10^{-5}sim $10^{-6}$ nm。
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引用次数: 6
Temperature-dependent rotationally inelastic collisions of OH− and He 温度相关的OH -和He的旋转非弹性碰撞
Pub Date : 2020-10-20 DOI: 10.1103/PhysRevA.103.052807
E. Endres, S. Ndengué, O. Lakhmanskaya, Seunghyun Lee, F. Gianturco, R. Dawes, R. Wester
We have studied the fundamental rotational relaxation and excitation collision of OH- J=0 1 with helium at different collision energies. Using state-selected photodetachment in a cryogenic ion trap, the collisional excitation of the first excited rotational state of OH- has been investigated and absolute inelastic collision rate coefficients have been extracted for collision temperatures between 20 and 35 K. The rates are compared with accurate quantum scattering calculations for three different potential energy surfaces. Good agreement is found within the experimental accuracy, but the experimental trend of increasing collision rates with temperature is only in part reflected in the calculations.
我们研究了OH- J=0 1与氦在不同碰撞能量下的基本旋转弛豫和激发碰撞。在低温离子阱中,利用状态选择光剥离,研究了OH-第一激发态的碰撞激发,并提取了碰撞温度在20 ~ 35 K之间的绝对非弹性碰撞率系数。并与三种不同势能面的精确量子散射计算结果进行了比较。在实验精度上得到了很好的一致性,但碰撞率随温度增加的实验趋势在计算中只是部分反映出来。
{"title":"Temperature-dependent rotationally inelastic collisions of \u0000OH−\u0000 and He","authors":"E. Endres, S. Ndengué, O. Lakhmanskaya, Seunghyun Lee, F. Gianturco, R. Dawes, R. Wester","doi":"10.1103/PhysRevA.103.052807","DOIUrl":"https://doi.org/10.1103/PhysRevA.103.052807","url":null,"abstract":"We have studied the fundamental rotational relaxation and excitation collision of OH- J=0 1 with helium at different collision energies. Using state-selected photodetachment in a cryogenic ion trap, the collisional excitation of the first excited rotational state of OH- has been investigated and absolute inelastic collision rate coefficients have been extracted for collision temperatures between 20 and 35 K. The rates are compared with accurate quantum scattering calculations for three different potential energy surfaces. Good agreement is found within the experimental accuracy, but the experimental trend of increasing collision rates with temperature is only in part reflected in the calculations.","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"8 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77781114","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Universal formalism for data sharing and processing in clock comparison networks 时钟比较网络中数据共享和处理的通用形式
Pub Date : 2020-10-20 DOI: 10.1103/physrevresearch.2.043269
J. Lodewyck, R. Le Targat, P. Pottie, E. Benkler, S. Koke, J. Kronjäger
We present a mathematical framework adapted to the comparison of atomic clocks remotely connected by a complex network of optical or microwave links. This framework facilitates the computation of frequency ratios using a generic set of equations that are valid for a wide variety of clock architectures, making the comparison of a large number of clocks practical. This formalism suggests a generic data exchange protocol that can be used in clock comparison collaborations, for which data logging and decision taking are completely local procedures, independently implemented by the participants.
我们提出了一个数学框架,适用于通过光学或微波链路的复杂网络远程连接的原子钟的比较。这个框架便于使用一组通用的方程来计算频率比,这些方程适用于各种时钟架构,使大量时钟的比较变得实用。这种形式提出了一种通用的数据交换协议,可用于时钟比较协作,其中数据记录和决策完全是本地过程,由参与者独立实现。
{"title":"Universal formalism for data sharing and processing in clock comparison networks","authors":"J. Lodewyck, R. Le Targat, P. Pottie, E. Benkler, S. Koke, J. Kronjäger","doi":"10.1103/physrevresearch.2.043269","DOIUrl":"https://doi.org/10.1103/physrevresearch.2.043269","url":null,"abstract":"We present a mathematical framework adapted to the comparison of atomic clocks remotely connected by a complex network of optical or microwave links. This framework facilitates the computation of frequency ratios using a generic set of equations that are valid for a wide variety of clock architectures, making the comparison of a large number of clocks practical. This formalism suggests a generic data exchange protocol that can be used in clock comparison collaborations, for which data logging and decision taking are completely local procedures, independently implemented by the participants.","PeriodicalId":8441,"journal":{"name":"arXiv: Atomic Physics","volume":"36 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"76357970","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 4
期刊
arXiv: Atomic Physics
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