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Direct observation of ion micromotion in a linear Paul trap 线性保罗阱中离子微运动的直接观察
Pub Date : 2020-10-01 DOI: 10.1103/PHYSREVA.103.023105
Liudmila A. Zhukas, Maverick J. Millican, P. Svihra, A. Nomerotski, B. Blinov
In this paper, the first direct observation of micromotion for multiple ions in a laser-cooled trapped ion crystal is discussed along with a novel measurement technique for micromotion amplitude. Micromotion is directly observed using a time-resolving, single-photon sensitive camera that provides both fluorescence and position data for each ion on the nanosecond time scale. Micromotion amplitude and phase for each ion in the crystal is measured which allows this method to be sensitive to tilts and shifts of the ion chain from the null of the radiofrequency quadrupole potential in the linear trap. Spatial resolution makes this micromotion detection technique suitable for complex ion configurations, including two-dimensional geometries. It does not require any additional equipment or laser beams, and the modulation of the cooling lasers or trap voltages is not necessary for detection, as it is in other methods.
本文讨论了激光冷却俘获离子晶体中多个离子微运动的首次直接观测,以及一种新的微运动幅度测量技术。微动是直接观察使用时间分辨,单光子敏感的相机,提供荧光和位置数据,每个离子在纳秒时间尺度。测量了晶体中每个离子的微运动幅度和相位,这使得该方法对线性阱中射频四极电位零点处离子链的倾斜和位移敏感。空间分辨率使得这种微运动检测技术适用于复杂的离子配置,包括二维几何形状。它不需要任何额外的设备或激光束,并且不需要调制冷却激光或陷阱电压,因为它是在其他方法中。
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引用次数: 7
Multiconfiguration Dirac–Hartree–Fock radiative parameters for emission lines in Ce ii–ivions and cerium opacity calculations for kilonovae 铈离子辐射线的多组态Dirac-Hartree-Fock辐射参数和千新星的铈不透明度计算
Pub Date : 2020-09-28 DOI: 10.1093/mnras/staa3729
H. Carvajal Gallego, P. Palmeri, P. Quinet
Large-scale calculations of atomic structures and radiative properties have been carried out for singly, doubly- and trebly ionized cerium. For this purpose, the purely relativistic multiconfiguration Dirac-Hartree-Fock (MCDHF) method was used, taking into account the effects of valence-valence and core-valence electronic correlations in detail. The results obtained were then used to calculate the expansion opacities characterizing the kilonovae observed as a result of neutron star mergers. Comparisons with previously published experimental and theoretical studies have shown that the results presented in this work are the most complete currently available, in terms of quantity and quality, concerning the atomic data and monochromatic opacities for Ce II, Ce III and Ce IV ions.
对单电离、双电离和三电离的铈进行了大规模的原子结构和辐射特性计算。为此,我们采用了纯相对论多组态Dirac-Hartree-Fock (MCDHF)方法,详细考虑了价电子-价电子和核心-价电子相关的影响。得到的结果随后被用来计算中子星合并后观测到的千新星的膨胀不透明度。与先前发表的实验和理论研究的比较表明,在数量和质量方面,本工作中提出的结果是目前可用的最完整的,涉及Ce II, Ce III和Ce IV离子的原子数据和单色不透明度。
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引用次数: 3
Effect of the Stark shift on the low-energy interference structure in strong-field ionization 斯塔克位移对强场电离低能干涉结构的影响
Pub Date : 2020-09-17 DOI: 10.1103/PhysRevA.103.053105
Weifeng Yang, Jie Li, Wen-Wu Jia, Hongdan Zhang, Xiwang Liu, Ming Zhu, Xiaohong Song, Jiale Chen
An improved quantum trajectory Monte Carlo method involving the Stark shift of the initial state, Coulomb potential, and multielectron polarization-induced dipole potential is used to revisit the origin of the low-energy interference structure in the photoelectron momentum distribution of the xenon atom subjected to an intense laser field, and resolve the different contributions of these three effects. In addition to the well-studied radial finger-like interference structure, a ring-like interference structure induced by interference among electron wave packets emitted from multi-cycle time windows of the laser field is found in the low energy part of the photoelectron momentum spectrum. It is attributed to the combined effect of the Coulomb potential and Stark shift. Our finding provides new insight into the imaging of electron dynamics of atoms and molecules with intense laser fields.
采用一种改进的量子轨迹蒙特卡罗方法,利用初始态斯塔克位移、库仑势和多电子极化偶极子势重新考察了氙原子在强激光场作用下光电子动量分布中低能干涉结构的起源,并解析了这三种效应的不同贡献。在光电子动量谱的低能部分,除了已被充分研究的径向指状干涉结构外,还发现了由激光场多周期时间窗发射的电子波包之间的干涉引起的环状干涉结构。这是库仑势和斯塔克位移共同作用的结果。我们的发现为用强激光场成像原子和分子的电子动力学提供了新的见解。
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引用次数: 0
Stern-Gerlach Interferometry with the Atom Chip 施特恩-格拉赫干涉测量与原子芯片
Pub Date : 2020-09-17 DOI: 10.1007/978-3-030-63963-1_14
M. Keil, S. Machluf, Y. Margalit, Zhifan Zhou, Omer Amit, Or Dobkowski, Y. Japha, S. Moukouri, D. Rohrlich, Zina Binstock, Y. Bar-Haim, M. Givon, D. Groswasser, Y. Meir, R. Folman
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引用次数: 7
Cascade superfluorescence in Er:YLF
Pub Date : 2020-09-13 DOI: 10.1103/PHYSREVRESEARCH.3.013138
F. Chiossi, C. Braggio, A. Khanbekyan, G. Carugno, A. Ortolan, G. Ruoso, R. Calabrese, A. Di Lieto, L. Tomassetti, M. Tonelli
We report the analysis of paired photon pulses arising from two cascading transitions in continuously pumped Erbium-doped YLiF$_4$ 1% and 0.01% crystals at 1.6 K. The dependence of the pulse peak intensity on the squared number of involved Erbium ions, between 10$^{11}$ and 10$^{13}$, definitely identifies the cooperative nature of the two pulsed emissions, that are generated by the subsequent, spontaneous formation of coherent states. The observed fluctuations of the time interval between the paired pulses and, most importantly, its correlation with the second pulse duration, demonstrate that the Erbium ions coherence is indeed seeded by vacuum fluctuations.
本文报道了在1.6 K下连续泵浦掺铒YLiF$_4$ 1%和0.01%晶体中由两个级联跃迁产生的成对光子脉冲的分析。脉冲峰值强度对参与的铒离子平方数的依赖,在10$^{11}$和10$^{13}$之间,明确地确定了两个脉冲发射的合作性质,这是由随后自发形成的相干态产生的。观测到的成对脉冲时间间隔的波动,以及最重要的是其与第二个脉冲持续时间的相关性,表明铒离子的相干性确实是由真空波动播下的种子。
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引用次数: 5
Hyperfine-mediated effects in a Lu+ optical clock Lu+光时钟中的超精细介导效应
Pub Date : 2020-09-07 DOI: 10.1103/physreva.102.052834
Zhiqiang Zhang, K. Arnold, R. Kaewuam, Marianna Safronova, M. D. Barrett
We consider hyperfine-mediated effects for clock transitions in $^{176}$Lu$^+$. Mixing of fine structure levels due to the hyperfine interaction bring about modifications to Lande $g$-factors and the quadrupole moment for a given state. Explicit expressions are derived for both $g$-factor and quadrupole corrections, for which leading order terms arise from the nuclear magnetic dipole coupling. High accuracy measurements of the $g$-factors for the $^1S_0$ and $^3D_1$ hyperfine levels are carried out, which provide an experimental determination of the leading order correction terms.
我们考虑了$^{176}$Lu$^+$中时钟跃迁的超精细介导效应。由于超精细的相互作用,精细结构能级的混合导致了给定态的朗德因子和四极矩的改变。导出了$g$因子和四极修正的显式表达式,其中的阶项是由核磁偶极子耦合产生的。对$^1S_0$和$^3D_1$超精细能级的$g$-因子进行了高精度的测量,从而提供了一种测定首阶校正项的实验方法。
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引用次数: 3
High-energy-resolution measurements of an ultracold-atom–ion collisional cross section 超低温原子-离子碰撞截面的高能量分辨率测量
Pub Date : 2020-09-07 DOI: 10.1103/PHYSREVA.103.032805
Ruti Ben-shlomi, Meirav Pinkas, Z. Meir, T. Sikorsky, O. Katz, N. Akerman, R. Ozeri
The cross section of a given process fundamentally quantifies the probability for that given process to occur. In the quantum regime of low energies, the cross section can vary strongly with collision energy due to quantum effects. Here, we report on a method to directly measure the atom-ion collisional cross section in the energy range of 0.2-12 mK$cdot$ k$_B$, by shuttling ultracold atoms trapped in an optical-lattice across a radio-frequency trapped ion. In this method, the average number of atom-ion collisions per experiment is below one such that the energy resolution is not limited by the broad (power-law) steady-state atom-ion energy distribution. Here, we estimate that the energy resolution is below 200 $mu$K$cdot$k$_B$, limited by drifts in the ion's excess micromotion compensation and can be reduced to the 10's $mu$K$cdot$k$_B$ regime. This resolution is one order-of-magnitude better than previous experiments measuring cold atom-ion collisional cross section energy dependence. We used our method to measure the energy dependence of the inelastic collision cross sections of a non-adiabatic Electronic-Excitation-Exchange (EEE) and Spin-Orbit Change (SOC) processes. We found that in the measured energy range, the EEE and SOC cross sections statistically agree with the classical Langevin cross section. This method allows for measuring the cross sections of various inelastic processes and opens up possibilities to search for atom-ion quantum signatures such as shape-resonances.
给定过程的横截面从根本上量化了该给定过程发生的概率。在低能的量子态中,由于量子效应,截面随碰撞能量的变化很大。在这里,我们报告了一种直接测量原子-离子碰撞截面的方法,能量范围为0.2-12 mK$cdot$ k$_B$,通过穿梭在光学晶格中被捕获的超冷原子穿过射频被捕获的离子。在这种方法中,每次实验中原子-离子碰撞的平均次数低于一次,因此能量分辨率不受广义(幂律)稳态原子-离子能量分布的限制。在这里,我们估计能量分辨率低于200 $mu$K$cdot$ K$ _B$,受离子过量微动补偿漂移的限制,可以降低到10的$mu$K$cdot$ K$ _B$机制。这个分辨率比以前测量冷原子-离子碰撞截面能量依赖的实验好一个数量级。我们用我们的方法测量了非绝热电子激发交换(EEE)和自旋轨道变化(SOC)过程的非弹性碰撞截面的能量依赖性。我们发现,在测量的能量范围内,EEE和SOC截面在统计上与经典朗之万截面一致。这种方法允许测量各种非弹性过程的横截面,并开辟了寻找原子-离子量子特征(如形状共振)的可能性。
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引用次数: 6
Direct measurement of the 7s2S1/2→7p2P3/2 transition frequency in Ra+226 Ra+226中7s2S1/2→7p2P3/2跃迁频率的直接测量
Pub Date : 2020-08-30 DOI: 10.1103/PHYSREVA.102.042822
C. A. Holliman, M. Fan, A. Contractor, M. Straus, A. Jayich
We report a direct measurement of the $7s ^2S_{1/2}rightarrow$ $7p ^2P_{3/2}$ electric-dipole transition frequency in $^{226}$Ra$^{+}$. With a single laser-cooled radium ion we determine the transition frequency to be 785722.11(3) GHz by directly driving the transition with frequency doubled light and measuring the frequency of the un-doubled light with an iodine reference. This measurement addresses a discrepancy of five combined standard deviations between previously reported values.
我们报告了直接测量$7s ^2S_{1/2}右划$ $7p ^2P_{3/2}$在$^{226}$Ra$^{+}$中的电偶极子跃迁频率。以激光冷却的镭离子为例,用倍频光直接驱动跃迁,并以碘为参考测量非倍频光的频率,确定跃迁频率为785722.11(3)GHz。该测量解决了先前报告值之间的五个联合标准偏差的差异。
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引用次数: 0
Pulsed Ion Microscope to Probe Quantum Gases 脉冲离子显微镜探测量子气体
Pub Date : 2020-08-19 DOI: 10.1103/PHYSREVX.11.011036
C. Veit, N. Zuber, O. Herrera-Sancho, V. S. Anasuri, T. Schmid, F. Meinert, R. Löw, T. Pfau
The advent of the quantum gas microscope allowed for the in situ probing of ultracold gaseous matter on an unprecedented level of spatial resolution. The study of phenomena on ever smaller length scales as well as the probing of three-dimensional systems is, however, fundamentally limited by the wavelength of the imaging light, for all techniques based on linear optics. Here we report on a high-resolution ion microscope as a versatile and powerful experimental tool to investigate quantum gases. The instrument clearly resolves atoms in an optical lattice with a spacing of $532,text{nm}$ over a field of view of 50 sites and offers an extremely large depth of field on the order of at least $70,mutext{m}$. With a simple model, we extract an upper limit for the achievable resolution of approximately $200,text{nm}$ from our data. We demonstrate a pulsed operation mode which in the future will enable 3D imaging and allow for the study of ionic impurities and Rydberg physics.
量子气体显微镜的出现使得对超冷气体物质的原位探测达到了前所未有的空间分辨率水平。然而,对于所有基于线性光学的技术来说,在更小的长度尺度上对现象的研究以及对三维系统的探测从根本上受到成像光波长的限制。在这里,我们报告了一种高分辨率离子显微镜作为一种多功能和强大的实验工具来研究量子气体。该仪器在50个点的视场范围内清晰地分辨出间距为$532,text{nm}$的光学晶格中的原子,并提供了至少$70,mutext{m}$的极大的视场深度。通过一个简单的模型,我们从我们的数据中提取了大约$200,text{nm}$的可实现分辨率上限。我们演示了一种脉冲操作模式,未来将实现3D成像,并允许离子杂质和里德伯物理的研究。
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引用次数: 19
Trapping, Cooling, and Photodissociation Analysis of State-Selected H2+ Ions Produced by (3+1) Multiphoton Ionization (3+1)多光子电离产生的状态选择H2+离子的俘获、冷却和光解分析
Pub Date : 2020-08-19 DOI: 10.1103/PhysRevApplied.14.024053
Julian Schmidt, T. Louvradoux, J. Heinrich, N. Sillitoe, M. Simpson, J. Karr, L. Hilico
We report on the production of cold, state-selected H$_2^+$ molecular ions in a linear RF trap. The ions are produced by (3+1) resonance-enhanced multi-photon ionisation (REMPI) of H$_2$, and sympathetically cooled by laser-cooled Be$^+$ ions. After demonstrating and characterizing the REMPI process, we use photodissociation by a deep UV laser at 213~nm to verify the high vibrational purity of the produced H$_2^+$ ion samples. Moreover, the large difference between the photodissociation efficiencies of ions created in the $v=0$ and $v=1$ levels provides a way to detect a $v=0 to 1$ transition. These results pave the way towards high-resolution vibrational spectroscopy of H$_2^+$ for fundamental metrology applications.
我们报道了在线性射频阱中产生冷的、状态选择的H$_2^+$分子离子。离子由H$_2$的(3+1)共振增强多光子电离(REMPI)产生,并由激光冷却Be$^+$离子共冷。在演示和表征REMPI过程后,我们利用213~nm深紫外激光光解,验证了所制备的H$_2^+$离子样品的高振动纯度。此外,在$v=0$和$v=1$能级上产生的离子光解效率之间的巨大差异提供了一种检测$v=0 到1$跃迁的方法。这些结果为H$_2^+$的高分辨率振动光谱用于基础计量应用铺平了道路。
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引用次数: 12
期刊
arXiv: Atomic Physics
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