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Resonant propagation of x rays from the linear to the nonlinear regime x射线从线性到非线性的共振传播
Pub Date : 2020-08-16 DOI: 10.1103/physreva.102.053113
Kai Li, M. Labeye, P. Ho, M. Gaarde, L. Young
We present a theoretical study of temporal, spectral, and spatial reshaping of intense, ultrafast x-ray pulses propagating through a resonant medium. Our calculations are based on the solution of a 3D time-dependent Schrodinger-Maxwell equation, with the incident x-ray photon energy on resonance with the core-level 1s-3p transition in neon. We study the evolution of the combined incident and medium-generated field, including the effects of stimulated emission, absorption, ionization and Auger decay, as a function of the input pulse energy and duration. We find that stimulated Raman scattering between core-excited states $1s^{-1}3p$ and $2p^{-1}3p$ occurs at high x-ray intensity, and that the emission around this frequency is strongly enhanced when also including the similar $1s^{-1}-2p^{-1}$ response of the ion. We also explore the dependence of x-ray self-induced transparency (SIT) and self-focusing on the pulse intensity and duration, and we find that the stimulated Raman scattering plays an important role in both effects. Finally, we discuss how these nonlinear effects may potentially be exploited as control parameters for pulse properties of x-ray free-electron laser sources.
我们提出了一个理论研究的时间,光谱和空间重塑的强,超快的x射线脉冲通过共振介质传播。我们的计算是基于三维随时间的薛定谔-麦克斯韦方程的解,入射的x射线光子能量与氖的核心能级1s-3p跃迁共振。我们研究了入射和介质产生的联合场的演化,包括受激发射、吸收、电离和俄歇衰变的影响,作为输入脉冲能量和持续时间的函数。我们发现在高x射线强度下,在核心激发态$1s^{-1}3p$和$2p^{-1}3p$之间的受激拉曼散射发生,并且当离子的类似$1s^{-1}-2p^{-1}$响应时,该频率附近的发射被强烈增强。我们还探讨了x射线自诱导透明(SIT)和自聚焦与脉冲强度和持续时间的关系,发现受激拉曼散射在这两种效应中起着重要作用。最后,我们讨论了如何利用这些非线性效应作为x射线自由电子激光源脉冲特性的控制参数。
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引用次数: 4
Laser cooling of transition-metal atoms 过渡金属原子的激光冷却
Pub Date : 2020-08-14 DOI: 10.1103/physreva.102.053327
Scott Eustice, K. Cassella, D. Stamper-Kurn
We propose the application of laser cooling to a number of transition-metal atoms, allowing numerous bosonic and fermionic atomic gases to be cooled to ultra-low temperatures. The non-zero electron orbital angular momentum of these atoms implies that strongly atom-state-dependent light-atom interactions occur even for light that is far-detuned from atomic transitions. At the same time, many transition-metal atoms have small magnetic dipole moments in their low-energy states, reducing the rate of dipolar-relaxation collisions. Altogether, these features provide compelling opportunities for future ultracold-atom research. Focusing on the case of atomic titanium, we identify the metastable $a ^5F_5$ state as supporting a $J rightarrow J+1$ optical transition with properties similar to the D2 transition of alkali atoms, and suited for laser cooling. The high total angular momentum and electron spin of this state suppresses leakage out of the the nearly closed optical transition to a branching ratio estimated below $sim 10^{-5}$. Following the pattern exemplified by titanium, we identify optical transitions that are suited for laser cooling of elements in the scandium group (Sc, Y, La), the titanium group (Ti, Zr), the vanadium group (V, Nb), the manganese group (Mn, Tc), and the iron group (Fe, Ru).
我们建议将激光冷却应用于一些过渡金属原子,使许多玻色子和费米子原子气体被冷却到超低温。这些原子的非零电子轨道角动量表明,即使对于远离原子跃迁的光,也会发生强烈的原子态依赖的光-原子相互作用。同时,许多过渡金属原子在低能态具有较小的磁偶极矩,从而降低了偶极弛豫碰撞的速率。总之,这些特征为未来的超冷原子研究提供了令人信服的机会。以原子钛为例,我们确定了亚稳$a ^5F_5$态支持$J rightarrow J+1$光学跃迁,其性质与碱原子的D2跃迁相似,适合激光冷却。这种状态的高总角动量和电子自旋抑制了几乎闭合的光学跃迁的泄漏,分支比估计低于$sim 10^{-5}$。按照以钛为例的模式,我们确定了适合于激光冷却钪族(Sc, Y, La),钛族(Ti, Zr),钒族(V, Nb),锰族(Mn, Tc)和铁族(Fe, Ru)元素的光学跃迁。
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引用次数: 5
Numerical time-of-flight analysis of the strong-field photoeffect 强场光效应的飞行时间数值分析
Pub Date : 2020-08-14 DOI: 10.1103/PHYSREVRESEARCH.2.043083
V. Tulsky, D. Bauer
Short-time filtering of the photoionization amplitude extracted straight from the numerical solution of the time-dependent Schr"{o}dinger equation (TDSE) is used to identify dominant pathways that form photoelectron spectra in strong fields. Thereby, the "black-box nature" of TDSE solvers only giving the final spectrum is overcome, and simpler approaches, e.g., semi-classical based on the strong-field approximation, can be tested and improved. The approach also allows to suppress intercycle quantum interference between pathways removing patterns that are usually washed out in experiments.
从时变Schr o}dinger方程(TDSE)的数值解中直接提取的光电离振幅的短时滤波用于识别强场中形成光电子能谱的主要途径。因此,TDSE解算器只给出最终光谱的“黑箱性质”被克服了,更简单的方法,例如基于强场近似的半经典方法,可以被测试和改进。该方法还可以抑制通路之间的周期间量子干涉,从而消除通常在实验中被淘汰的模式。
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引用次数: 2
Inducing Enantiosensitive Permanent Multipoles in Isotropic Samples with Two-Color Fields 双色场诱导各向同性样品的对映敏感永久多极体
Pub Date : 2020-08-14 DOI: 10.1007/978-3-030-63963-1_16
A. Ordonez, O. Smirnova
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引用次数: 0
Single-Photon Stored-Light Interferometry. 单光子存储光干涉法。
Pub Date : 2020-08-11 DOI: 10.15128/r18k71nh124
Y. Jiao, N. L. R. Spong, O. D. Hughes, Chloe So, T. Ilieva, K. Weatherill, C. Adams
We demonstrate a single-photon stored-light interferometer, where a photon is stored in a laser-cooled atomic ensemble in the form of a Rydberg polariton with a spatial extent of $10 times1times1mu m^3$. The photon is subject to a Ramsey sequence, i.e. `split' into a superposition of two paths. After a delay of up to 450 ns, the two paths are recombined to give an output dependent on their relative phase. The superposition time of 450 ns is equivalent to a free-space propagation distance of 135 m. We show that the interferometer fringes are sensitive to external fields, and suggest that stored-light interferometry could be useful for localized sensing applications.
我们演示了一种单光子存储光干涉仪,其中光子以空间范围为$10 times1times1mu m^3$的Rydberg极化子的形式存储在激光冷却的原子系集合中。光子服从拉姆齐序列,即。“分裂”成两条路径的叠加。经过高达450ns的延迟后,两条路径重新组合,以提供依赖于其相对相位的输出。450 ns的叠加时间相当于135 m的自由空间传播距离。我们证明了干涉仪条纹对外部场敏感,并建议存储光干涉法可以用于局部传感应用。
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引用次数: 0
Influence of a quasi-molecular mechanism of recombination on the formation of hydrogen in the early Universe 准分子复合机制对早期宇宙中氢形成的影响
Pub Date : 2020-08-03 DOI: 10.1093/mnras/staa3622
T. Kereselidze, I. Noselidze, J. Ogilvie
In the framework of a quasi-molecular approach, the formation of hydrogen atom in the pre-recombination period of evolution of the universe is analysed quantitatively. Calculations in an adiabatic multi-level representation enable estimates of probabilities of radiative transitions. The quasi-molecular mechanism of recombination allows the formation of hydrogen molecular ion, $H_2^+$, in its ground state. The probability of this process is comparable with the probability of the creation of atomic hydrogen. The participation of a second proton in the recombination increases the binding energy of an electron and decreases the rate of recombination of hydrogen.
在准分子方法的框架下,定量分析了宇宙演化前复合期氢原子的形成。绝热多层表示的计算可以估计辐射跃迁的概率。准分子复合机制允许在基态下形成氢分子离子$H_2^+$。这个过程发生的概率与氢原子产生的概率相当。第二个质子在重组中的参与增加了电子的结合能并降低了氢的重组速率。
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引用次数: 2
Sensitive magnetometry in challenging environments 敏感磁强计在具有挑战性的环境
Pub Date : 2020-07-31 DOI: 10.1116/5.0025186
K. Fu, G. Iwata, A. Wickenbrock, D. Budker
State-of-the-art magnetic field measurements performed in shielded environments with carefully controlled conditions rarely reflect the realities of those applications envisioned in the introductions of peer-reviewed publications. Nevertheless, significant advances in magnetometer sensitivity have been accompanied by serious attempts to bring these magnetometers into the challenging working environments in which they are often required. This review discusses the ways in which various (predominantly optically-pumped) magnetometer technologies have been adapted for use in a wide range of noisy and physically demanding environments.
在精心控制条件的屏蔽环境中进行的最先进的磁场测量很少反映同行评审出版物介绍中设想的应用的现实情况。尽管如此,在磁力计灵敏度方面取得重大进展的同时,也伴随着将这些磁力计带入经常需要它们的具有挑战性的工作环境的认真尝试。这篇综述讨论了各种(主要是光泵浦)磁强计技术已经适应在广泛的噪声和物理要求的环境中使用的方式。
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引用次数: 50
Transition cancellations of 87Rb and 85Rb atoms in a magnetic field 87Rb和85Rb原子在磁场中的跃迁消去
Pub Date : 2020-07-22 DOI: 10.1364/josab.403862
A. Aleksanyan, R. Momier, E. Gazazyan, A. Papoyan, C. Leroy
We have analyzed the magnetic field dependences of intensities of all the optical transitions between magnetic sublevels of hyperfine levels, excited with $sigma^+$, $pi$ and $sigma^-$ polarized light, for the $D_1$ and $D_2$ lines of $^{87}$Rb and $^{85}$Rb atoms. Depending on the type of transition and the quantum numbers of involved levels, the Hamiltonian matrices are of $1times 1$, $2times 2$, $3times 3$ or $4times 4$ dimension. As an example, analytical expressions are presented for the case of $2times 2$ dimension matrices for $D_1$ line of both isotopes. Eigenvalues and eigenkets are given, and the expression for the transition intensity as a function of $B$ has been determined. It is found that some $pi$ transitions of $^{87}$Rb and $^{85}$Rb get completely canceled for certain, extremely precise, values of $B$. No cancellation occurs for $sigma^+$ or $sigma^-$ transitions of $D_1$ line. For matrices with size over $2times 2$, analytical formulas are heavy, and we have performed numerical calculations. All the $B$ values cancelling $sigma^+$, $pi$ and $sigma^-$ transitions of $D_1$ and $D_2$ lines of $^{87}$Rb and $^{85}$Rb are calculated, with an accuracy limited by the precision of the involved physical quantities. We believe our modeling can serve as a tool for determination of standardized values of magnetic field. The experimental implementation feasibility and its possible outcome are addressed. We believe the experimental realization will allow to increase precision of the physical quantities involved, in particular the upper state atomic levels energy.
我们分析了$^{87}$ Rb和$^{85}$ Rb原子的$D_1$和$D_2$线在$sigma^+$、$pi$和$sigma^-$偏振光激发下的超精细能级磁亚能级之间所有光学跃迁强度与磁场的依赖关系。根据跃迁的类型和所涉及能级的量子数,哈密顿矩阵的维度为$1times 1$、$2times 2$、$3times 3$或$4times 4$。作为一个例子,给出了两种同位素$D_1$线的$2times 2$维矩阵的解析表达式。给出了特征值和特征基,并确定了过渡强度作为$B$函数的表达式。我们发现$^{87}$ Rb和$^{85}$ Rb的一些$pi$跃迁对于$B$的某些非常精确的值是完全取消的。$D_1$线的$sigma^+$或$sigma^-$转换不发生取消。对于大小超过$2times 2$的矩阵,解析公式很重,我们进行了数值计算。计算了所有抵消$^{87}$ Rb和$^{85}$ Rb的$D_1$和$D_2$线的$sigma^+$、$pi$和$sigma^-$跃迁的$B$值,其精度受所涉及物理量精度的限制。我们相信我们的模型可以作为确定磁场标准化值的工具。讨论了实验实现的可行性和可能产生的结果。我们相信实验实现将允许提高物理量的精度,特别是高状态原子能级的能量。
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引用次数: 5
Single-Photon-Level Sub-Doppler Pump-Probe Spectroscopy of Rubidium 铷的单光子能级亚多普勒泵浦探测光谱
Pub Date : 2020-07-16 DOI: 10.1103/physrevapplied.14.044046
P. Burdekin, S. Grandi, Rielly Newbold, R. Hoggarth, K. D. Major, A. Clark
We propose and demonstrate pump-probe spectroscopy of rubidium absorption which reveals the sub-Doppler hyperfine structure of the $^{5}$S$_{1/2} leftrightarrow$ $^{5}$P$_{3/2}$ (D2) transitions. The counter propagating pump and probe lasers are independently tunable in frequency, with the probe operating at the single-photon-level. The two-dimensional spectrum measured as the laser frequencies are scanned shows fluorescence, Doppler-broadened absorption dips and sub-Doppler features. The detuning between the pump and probe lasers allows compensation of the Doppler shift for all atomic velocities in the room temperature vapor, meaning we observe sub-Doppler features for all atoms in the beam. We detail a theoretical model of the system which incorporates fluorescence, saturation effects and optical pumping and compare this with the measured spectrum, finding a mean absolute percentage error of 4.17%. In the future this technique could assist in frequency stabilization of lasers, and the single-photon-level probe could be replaced by a single photon source.
我们提出并演示了铷吸收的泵浦探测光谱,揭示了$^{5}$ S $_{1/2} leftrightarrow$$^{5}$ P $_{3/2}$ (D2)跃迁的亚多普勒超精细结构。反向传播泵浦和探针激光器的频率可独立调谐,探针工作在单光子水平。扫描激光频率时测量的二维光谱显示出荧光、多普勒加宽吸收衰减和亚多普勒特征。泵浦激光器和探测激光器之间的失谐可以补偿室温蒸汽中所有原子速度的多普勒频移,这意味着我们可以观察到光束中所有原子的亚多普勒特征。我们详细介绍了该系统的理论模型,其中包括荧光、饱和效应和光泵浦,并将其与实测光谱进行了比较,发现平均绝对百分比误差为4.17%。在未来,该技术可以辅助激光的频率稳定,单光子级探针可以被单光子源取代。
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引用次数: 4
Vacuum characterization of a compact room-temperature trapped ion system 紧凑的室温俘获离子系统的真空特性
Pub Date : 2020-07-15 DOI: 10.1063/5.0029236
Yuhi Aikyo, Geert Vrijsen, T. Noel, A. Kato, M. Ivory, Jungsang Kim
We present the design and vacuum performance of a compact room-temperature trapped ion system for quantum computing, consisting of a ultra-high vacuum (UHV) package, a micro-fabricated surface trap and a small form-factor ion pump. The system is designed to maximize mechanical stability and robustness by minimizing the system size and weight. The internal volume of the UHV package is only 2 cm$^3$, a significant reduction in comparison with conventional vacuum chambers used in trapped ion experiments. We demonstrate trapping of $^{174}$Yb$^+$ ions in this system and characterize the vacuum level in the UHV package by monitoring both the rates of ion hopping in a double-well potential and ion chain reordering events. The calculated pressure in this vacuum package is about 1.5e-11 Torr, which is sufficient for the majority of current trapped ion experiments.
我们提出了一种用于量子计算的紧凑型室温俘获离子系统的设计和真空性能,该系统由超高真空(UHV)封装、微制造表面阱和小尺寸离子泵组成。该系统旨在通过最小化系统尺寸和重量来最大限度地提高机械稳定性和坚固性。UHV封装的内部体积仅为2 cm³,与捕获离子实验中使用的传统真空室相比,这是一个显着的减少。我们证明了该系统中$^{174}$Yb$^+$离子的捕获,并通过监测双阱电位中的离子跳变速率和离子链重排序事件来表征特高压封装中的真空水平。该真空封装的计算压力约为1.5e-11 Torr,足以满足大多数电流捕获离子实验。
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引用次数: 5
期刊
arXiv: Atomic Physics
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