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Light-induced valleytronics in pristine graphene 原始石墨烯中的光致谷电子学
Pub Date : 2020-11-10 DOI: 10.1364/OPTICA.418152
S. MrudulM., 'Alvaro Jim'enez-Gal'an, M. Ivanov, G. Dixit
Electrons in two-dimensional hexagonal materials have valley degree of freedom, which can be used to encode and process quantum information. The valley-selective excitations, governed by the circularly polarised light resonant with the material's band-gap, continues to be the foundation of valleytronics. It is often assumed that achieving valley selective excitation in pristine graphene with all-optical means is not possible due to the inversion symmetry of the system. Here we demonstrate that both valley-selective excitation and valley-selective high-harmonic generation can be achieved in pristine graphene by using the combination of two counter-rotating circularly polarized fields, the fundamental and its second harmonic. Controlling the relative phase between the two colours allows us to select the valleys where the electron-hole pairs and higher-order harmonics are generated. We also describe an all-optical method for measuring valley polarization in graphene with a weak probe pulse. This work offers a robust recipe to write and read valley-selective electron excitations in materials with zero bandgap and zero Berry curvature.
二维六边形材料中的电子具有谷自由度,可用于量子信息的编码和处理。由圆偏振光与材料的带隙共振所控制的谷选择激发,仍然是谷电子学的基础。通常认为,由于系统的反演对称性,在原始石墨烯中用全光手段实现谷选择激发是不可能的。在这里,我们证明了谷选择激发和谷选择高谐波的产生可以通过使用两个反向旋转的圆极化场,基频和二次谐波的组合来实现。控制两种颜色之间的相对相位使我们能够选择产生电子-空穴对和高次谐波的谷。我们还描述了一种用弱探针脉冲测量石墨烯谷偏振的全光方法。这项工作为在零带隙和零贝里曲率的材料中写入和读取谷选择电子激发提供了一个可靠的方法。
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引用次数: 31
Spin waves in the collinear antiferromagnetic phase of Mn5Si3 Mn5Si3共线反铁磁相中的自旋波
Pub Date : 2020-11-10 DOI: 10.1103/PHYSREVB.103.024407
F. J. dos Santos, N. Biniskos, S. Raymond, K. Schmalzl, M. dos Santos Dias, P. Steffens, J. Perßon, S. Blügel, S. Lounis, T. Brückel
By combining two independent approaches, inelastic neutron scattering measurements and density functional theory calculations, we study the spin-waves in the high-temperature collinear antiferromagnetic phase (AFM2) of Mn$_5$Si$_3$. We obtain its magnetic ground-state properties and electronic structure. This study allowed us to determine the dominant magnetic exchange interactions and magnetocrystalline anisotropy in the AFM2 phase of Mn$_5$Si$_3$. Moreover, the evolution of the spin excitation spectrum is investigated under the influence of an external magnetic field perpendicular to the anisotropy easy-axis. The low energy magnon modes show a different magnetic field dependence which is a direct consequence of their different precessional nature. Finally, possible effects related to the Dzyaloshinskii-Moriya interaction are also considered.
结合非弹性中子散射测量和密度泛函理论计算两种独立的方法,研究了Mn$_5$Si$_3$高温共线反铁磁相(AFM2)中的自旋波。我们得到了它的磁性基态性质和电子结构。这项研究使我们能够确定Mn$_5$Si$_3$ AFM2相的主要磁交换相互作用和磁晶各向异性。此外,研究了垂直于各向异性易轴的外磁场作用下自旋激发谱的演化。低能磁振子模式表现出不同的磁场依赖性,这是它们不同岁差性质的直接结果。最后,还考虑了与Dzyaloshinskii-Moriya相互作用有关的可能影响。
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引用次数: 3
Coulomb blockade in field electron emission from carbon nanotubes 碳纳米管场电子发射中的库仑阻滞
Pub Date : 2020-11-10 DOI: 10.1063/5.0039961
V. Kleshch, V. Porshyn, P. Serbun, A. Orekhov, R. Ismagilov, S. Malykhin, V. A. Eremina, P. Obraztsov, E. Obraztsova, D. Lützenkirchen-Hecht
We report the observation of Coulomb blockade in field electron emission (FE) from single-wall carbon nanotubes (SWCNTs), which is manifested as pronounced steps in the FE current-voltage curves and oscillatory variations in the energy distribution of emitted electrons. The appearance of the Coulomb blockade is explained by the formation of nanoscale protrusions at the apexes of SWCNTs due to the electric field-assisted surface diffusion of adsorbates and carbon adatoms. The proposed adsorbate-assisted FE mechanism is substantially different from the well-known resonant tunneling associated with discrete electronic states of adsorbed atoms. The simulations based on the Coulomb blockade theory are in excellent agreement with the experimental results. The SWCNT field emitters controlled by the Coulomb blockade effect are expected to be used to develop on-demand coherent single-electron sources for advanced vacuum nanoelectronic devices.
本文报道了单壁碳纳米管(SWCNTs)在场电子发射(FE)中观察到的库仑阻塞现象,这表现为场电子发射电流-电压曲线的显著阶跃变化和发射电子能量分布的振荡变化。库仑阻滞的出现可以通过电场辅助吸附物和碳原子的表面扩散在SWCNTs的顶端形成纳米级突起来解释。所提出的吸附辅助FE机制与众所周知的与吸附原子的离散电子态相关的共振隧道效应有本质上的不同。基于库仑封锁理论的模拟结果与实验结果非常吻合。利用库仑封锁效应控制的swcnts场发射体有望用于开发先进的真空纳米电子器件的按需相干单电子源。
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引用次数: 3
Heat capacity of nonequilibrium electron-hole plasma in graphene layers and graphene bilayers 石墨烯层和石墨烯双层中非平衡电子空穴等离子体的热容
Pub Date : 2020-11-07 DOI: 10.1103/PhysRevB.103.245414
V. Ryzhii, M. Ryzhii, T. Otsuji, V. Mitin, M. Shur
We analyze the statistical characteristics of the quasi-nonequilibrium two-dimensional electron-hole plasma in graphene layers (GLs) and graphene bilayers (GBLs) and evaluate their heat capacity.The GL heat capacity of the weakly pumped intrinsic or weakly doped GLs normalized by the Boltzmann constant is equal to $c_{GL} simeq 6.58$. With varying carrier temperature the intrinsic GBL carrier heat capacity $c_{GBL}$ changes from $c_{GBL} simeq 2.37$ at $T lesssim 300$~K to $c_{GBL} simeq 6.58$ at elevated temperatures. These values are markedly differentfrom the heat capacity of classical two-dimensional carriers with $c = 1$. The obtained results can be useful for the optimization of different GL- and GBL-based high-speed devices.
本文分析了石墨烯层(GLs)和石墨烯双层(GBLs)中准非平衡二维电子空穴等离子体的统计特性,并评估了它们的热容。经玻尔兹曼常数归一化的弱泵浦本征或弱掺杂GLs的GL热容等于$c_{GL} simeq 6.58$。随着载流子温度的变化,GBL载流子固有热容$c_{GBL}$从$T lesssim 300$ K时的$c_{GBL} simeq 2.37$变为升高温度时的$c_{GBL} simeq 6.58$。这些值与$c = 1$经典二维载流子的热容有明显的不同。所得结果可用于各种基于GL和gbl的高速器件的优化。
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引用次数: 3
Many-body effects in third harmonic generation of graphene 石墨烯三次谐波产生中的多体效应
Pub Date : 2020-11-07 DOI: 10.1103/PHYSREVB.103.125415
H. Rostami, E. Cappelluti
The low-energy (intraband) range of the third harmonic generation of graphene in the terahertz regime is governed by the damping terms induced by the interactions. A controlled many-body description of the scattering processes is thus a compelling and desirable requirement. In this paper, using a Kadanoff-Baym approach, we systematically investigate the impact of many-body interaction on the third-harmonic generation (THG) of graphene, taking elastic impurity scattering as a benchmark example. We predict the onset in the mixed inter-intraband regime of novel incoherent features driven by the interaction at four- and five-photon transition frequencies in the third-harmonic optical conductivity with a spectral weight proportional to the scattering rate.We show also that, in spite of the complex many-body physics, the purely intraband term governing the limit $omega to 0$ resembles the constraints of the phenomenological model. We ascribe this agreement to the fulfilling of the conservation laws enforced by the conserving approach. The overlap with novel incoherent features and the impact of many-body driven multi-photon vertex couplings limit however severely the validity of phenomenological description.
石墨烯在太赫兹波段的三次谐波产生的低能(带内)范围由相互作用引起的阻尼项控制。因此,对散射过程进行受控的多体描述是一个迫切而理想的要求。本文采用Kadanoff-Baym方法,以弹性杂质散射为基准,系统地研究了多体相互作用对石墨烯三次谐波产生(THG)的影响。我们预测了在三次谐波光学电导率中,由四光子和五光子跃迁频率的相互作用驱动的新型非相干特征在混合带内区域的开始,其谱权与散射率成正比。我们还表明,尽管有复杂的多体物理,控制极限的纯带内项类似于现象学模型的约束。我们将这一协议归因于通过保护方法执行的保护法律的履行。然而,新的非相干特征的重叠和多体驱动的多光子顶点耦合的影响严重限制了现象学描述的有效性。
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引用次数: 3
Single- and narrow-line photoluminescence in a boron nitride-supported MoSe 2 /graphene heterostructure 氮化硼负载MoSe 2 /石墨烯异质结构中的单线和窄线光致发光
Pub Date : 2020-11-05 DOI: 10.5802/CRPHYS.58
L. E. P. L'opez, Loic Moczko, J. Wolff, Aditya Singh, Etienne Lorchat, M. Romeo, T. Taniguchi, Kenji Watanabe, S. Berciaud
Heterostructures made from van der Waals materials provide a template to investigate proximity effects at atomically sharp heterointerfaces. In particular, near-field charge and energy transfer in heterostructures made from semiconducting transition metal dichalcogenides (TMD) have attracted interest to design model 2D "donor-acceptor" systems and new optoelectronic components. Here, using of Raman scattering and photoluminescence spectroscopies, we report a comprehensive characterization of a molybedenum diselenide (MoSe$_2$) monolayer deposited onto hexagonal boron nitride (hBN) and capped by mono- and bilayer graphene. Along with the atomically flat hBN susbstrate, a single graphene epilayer is sufficient to passivate the MoSe$_2$ layer and provides a homogenous environment without the need for an extra capping layer. As a result, we do not observe photo-induced doping in our heterostructure and the MoSe$_2$ excitonic linewidth gets as narrow as 1.6~meV, hence approaching the homogeneous limit. The semi-metallic graphene layer neutralizes the 2D semiconductor and enables picosecond non-radiative energy transfer that quenches radiative recombination from long-lived states. Hence, emission from the neutral band edge exciton largely dominates the photoluminescence spectrum of the MoSe$_2$/graphene heterostructure. Since this exciton has a picosecond radiative lifetime at low temperature, comparable with the energy transfer time, its low-temperature photoluminescence is only quenched by a factor of $3.3 pm 1$ and $4.4 pm 1$ in the presence of mono- and bilayer graphene, respectively. Finally, we exploit the valley-contrasting properties of monolayer TMDs and show that our simple stack provides a single-line 2D chiral emitter with degrees of valley polarization and coherence up to $30,%$ and $45,%$ at low temperature under excitation 60 meV above the bright exciton line.
由范德华材料制成的异质结构为研究原子尖锐异质界面的接近效应提供了模板。特别是,由半导体过渡金属二硫族化物(TMD)制成的异质结构中的近场电荷和能量转移引起了人们对设计2D模型“供体-受体”系统和新型光电元件的兴趣。利用拉曼散射和光致发光光谱,我们报道了一种沉积在六方氮化硼(hBN)上并被单层和双层石墨烯覆盖的二硒化钼(MoSe$_2$)单层的全面表征。与原子平面的hBN衬底一起,单个石墨烯涂层足以钝化MoSe$_2$层,并提供均匀的环境,而无需额外的封盖层。结果表明,我们的异质结构中没有光致掺杂现象,并且MoSe$_2$激子线宽窄至1.6~meV,接近均匀极限。半金属石墨烯层中和了2D半导体,并实现了皮秒的非辐射能量传递,从而消除了长寿命态的辐射复合。因此,中性带边缘激子的发射在很大程度上主导了MoSe$_2$/石墨烯异质结构的光致发光光谱。由于该激子在低温下具有皮秒的辐射寿命,与能量传递时间相当,因此在单层和双层石墨烯存在下,其低温光致发光分别仅被淬灭$3.3 pm 1$和$4.4 pm 1$。最后,我们利用单层tmd的谷对比特性,并表明我们的简单堆栈提供了单线二维手性发射器,在低温下,在亮激子线以上60 meV的激励下,谷极化和相干度分别高达$30,%$和$45,%$。
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引用次数: 3
Highly efficient phase-tunable photonic thermal diode 高效相位可调光子热二极管
Pub Date : 2020-11-05 DOI: 10.1063/5.0036485
G. Marchegiani, A. Braggio, F. Giazotto
We investigate the photon-mediated thermal transport between a superconducting electrode and a normal metal. When the quasiparticle contribution can be neglected, the photon-mediated channel becomes an efficient heat transport relaxation process for the superconductor at low temperatures, being larger than the intrinsic contribution due to the electron-phonon interaction. Furthermore, the superconductor-normal metal system acts as a nearly-perfect thermal diode, with a rectification factor up to $10^8$ for a realistic aluminum superconducting island. The rectification factor can be also tuned in a phase-controlled fashion through a non-galvanic coupling, realized by changing the magnetic flux piercing a superconducting quantum interference device (SQUID), which modifies the coupling impedance between the superconductor and the normal metal. The scheme can be exploited for passive cooling in superconducting quantum circuits by transferring heat toward normal metallic pads where it dissipates more efficiently or for more general thermal management purposes.
我们研究了超导电极和普通金属之间的光子介导的热输运。当准粒子的贡献可以忽略不计时,光子介导的通道在低温下成为超导体的有效热输运弛豫过程,大于电子-声子相互作用的本禀贡献。此外,超导体-正常金属系统作为一个近乎完美的热二极管,整流系数高达$10^8$对于一个现实的铝超导岛。通过改变穿透超导量子干涉器件(SQUID)的磁通量,改变超导体与正常金属之间的耦合阻抗,可以通过非电偶耦合以相位控制的方式调节整流因子。该方案可用于超导量子电路的被动冷却,通过将热量传递到更有效地消散的普通金属衬垫或用于更一般的热管理目的。
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引用次数: 8
Level attraction and exceptional points in a resonant spin-orbit torque system 共振自旋轨道转矩系统中的水平吸引和异常点
Pub Date : 2020-11-04 DOI: 10.1103/PhysRevB.103.195409
I. Proskurin, R. Stamps
Level attraction can appear in driven systems where instead of repulsion two modes coalesce in a region separated by two exceptional points. This behavior was proposed for optomechanical and optomagnonic systems, and recently observed for dissipative cavity magnon-polaritons. We demonstrate that such a regime exists in a spin-orbit torque system where a magnetic oscillator is resonantly coupled to an electron reservoir. An instability mechanism necessary for mode attraction can be provided by applying an electric field. The field excites interband transitions between spin-orbit split bands leading to an instability of the magnetic oscillator. Two exceptional points then appear in the oscillator energy spectrum and the region of instability. We discuss conditions under which this can occur and estimate the electric field strength necessary for reaching the attraction region for a spin-orbit torque oscillator with Rashba coupling. A proposal for experimental detection is made using magnetic susceptibility measurements.
水平吸引可以出现在驱动系统中,其中两个模式在由两个例外点分开的区域内合并而不是排斥。这种行为被提出于光力学和光磁系统中,并且最近在耗散腔磁非极化中被观察到。我们证明了在一个磁振子与电子库共振耦合的自旋轨道转矩系统中存在这样的状态。通过施加电场可以提供模吸引所必需的不稳定机制。磁场激发了自旋轨道分裂带间的带间跃迁,导致了磁振子的不稳定性。然后在振子能谱和不稳定区域出现两个异常点。我们讨论了可能发生这种情况的条件,并估计了具有Rashba耦合的自旋-轨道转矩振荡器到达吸引区所需的电场强度。提出了利用磁化率测量进行实验检测的建议。
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引用次数: 2
Effect of retardation on the frequency and linewidth of plasma resonances in a two-dimensional disk of electron gas 延迟对二维电子气盘中等离子体共振频率和线宽的影响
Pub Date : 2020-11-02 DOI: 10.1103/PhysRevB.103.195431
I. V. Zagorodnev, D. A. Rodionov, A. A. Zabolotnykh
We theoretically analyze dominant plasma modes in a two-dimensional disk of electron gas by calculating the absorption of an incident electromagnetic wave. The problem is solved in a self-consistent approximation, taking into account electromagnetic retardation effects. We use the Drude model to describe the conductivity of the system. The absorption spectrum exhibits a series of peaks corresponding to the excitation of plasma waves. The position and linewidth of the peaks designating, respectively, the frequency and damping rate of the plasma modes. We estimate the influence of retardation effects on the frequency and linewidth of the fundamental (dipole) and axisymmetric (quadrupole) plasma modes both numerically and analytically. We find the net damping rate of the modes to be dependent on not only the sum of the radiative and collisional decays but also their intermixture, even for small retardation. We show that the net damping rate can be noticeably less than that determined by collisions alone.
通过计算入射电磁波的吸收,从理论上分析了二维电子气体盘中的主要等离子体模式。该问题在考虑电磁延迟效应的自洽近似下求解。我们用德鲁德模型来描述系统的电导率。吸收光谱显示出一系列与等离子体波激发相对应的峰。峰的位置和线宽分别表示等离子体模式的频率和阻尼率。我们用数值和解析的方法估计了延迟效应对基本(偶极子)和轴对称(四极子)等离子体模式的频率和线宽的影响。我们发现模态的净阻尼率不仅依赖于辐射和碰撞衰减的总和,而且还依赖于它们的混合,即使延迟很小。我们表明,净阻尼率可以明显小于仅由碰撞决定的阻尼率。
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引用次数: 5
Spin-orbital magnetic response of relativistic fermions with band hybridization 带杂化相对论费米子的自旋轨道磁响应
Pub Date : 2020-11-02 DOI: 10.1103/PhysRevResearch.3.023098
Y. Araki, Daiki Suenaga, Kei Suzuki, S. Yasui
Spins of relativistic fermions are related to their orbital degrees of freedom. In order to quantify the relativistic effect in systems composed of both relativistic and nonrelativistic fermions, we focus on the spin-orbital (SO) crossed susceptibility, which becomes finite in the presence of spin-orbit coupling. The SO crossed susceptibility is defined as the response function of their spin polarization to the "orbital" magnetic field, namely the effect of magnetic field on the orbital motion of particles as the vector potential. Once relativistic and nonrelativistic fermions are hybridized, their SO crossed susceptibility gets modified at the Fermi energy around the band hybridization point, leading to spin polarization of nonrelativistic fermions as well. These effects are enhanced under a dynamical magnetic field that violates thermal equilibrium, arising from the interband process permitted by the band hybridization. Its experimental realization is discussed for Dirac electrons in solids with slight breaking of crystalline symmetry or doping, and also for quark matter including dilute heavy quarks strongly hybridized with light quarks, arising in a relativistic heavy-ion collision process.
相对论性费米子的自旋与其轨道自由度有关。为了量化由相对论性和非相对论性费米子组成的系统中的相对论效应,我们关注自旋-轨道交叉磁化率,它在自旋-轨道耦合存在时变得有限。SO交叉磁化率定义为它们的自旋极化对“轨道”磁场的响应函数,即磁场作为矢量势对粒子轨道运动的影响。一旦相对论性费米子和非相对论性费米子杂化,它们的SO交叉磁化率在带杂化点附近的费米能量处被修改,导致非相对论性费米子也出现自旋极化。这些效应在动态磁场下被增强,而动态磁场破坏了热平衡,这是由带间杂化所允许的带间过程引起的。
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引用次数: 6
期刊
arXiv: Mesoscale and Nanoscale Physics
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