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Effect of phase string on single-hole dynamics in the two-leg Hubbard ladder 相柱对两腿Hubbard梯单孔动力学的影响
Pub Date : 2020-11-21 DOI: 10.1103/PHYSREVB.103.035141
K. Shinjo, S. Sota, T. Tohyama
Optical measurements in doped Mott insulators have discovered the emergence of spectral weights at mid-infrared (MIR) upon chemical- and photo-doping. MIR weights may have a relation to string-type excitation of spins, which is induced by a doped hole generating miss-arranged spins with respect to their sublattice. There are two types of string effects: one is $S^z$ string that is repairable by quantum spin flips and the other is phase string irreparable by the spin flips. We investigate the effect of $S^{z}$ and phase strings on MIR weights. Calculating the optical conductivity of single-hole Hubbard and $t$-$J$ models on two-leg ladders by using time-dependent Lanczos and density-matrix renormalization group, we find that phase strings make a crucial effect on the emergence of MIR weights as compared with $S^{z}$ strings. Our findings indicate that a mutual Chern-Simons gauge field acting between spin and charge degrees of freedom, which is the origin of phase strings, is significant for obtaining MIR weights. Conversely, if we remove this gauge field, no phase is picked up by a doped hole. As a result, a spin-polaron accompanied by a local spin distortion emerges and a quasiparticle with a cosine-like energy dispersion is formed in single-particle spectral function. Furthermore, we suggest a Floquet engineering to examine the phase-string effect in cold atoms.
对掺杂的莫特绝缘体进行光学测量,发现化学和光掺杂后中红外(MIR)光谱权重的出现。MIR的权重可能与自旋的弦型激发有关,这是由掺杂空穴产生的自旋相对于它们的亚晶格排列错误引起的。有两种类型的弦效应:一种是可以通过量子自旋翻转修复的S^z弦,另一种是无法通过自旋翻转修复的相弦。我们研究了$S^{z}$和相位串对MIR权值的影响。利用随时间变化的Lanczos和密度矩阵重正化群计算了单孔Hubbard和$t$-$J$模型在两腿梯上的光学电导率,我们发现与$S^{z}$弦相比,相位弦对MIR权值的出现有重要影响。我们的研究结果表明,作用于自旋自由度和电荷自由度之间的相互chen - simons规范场是相位串的起源,对于获得MIR权重是重要的。相反,如果我们去除这个规范场,则没有相位被掺杂孔拾取。结果,在单粒子谱函数中出现了伴随局部自旋畸变的自旋极化子,形成了具有余弦类能量色散的准粒子。此外,我们提出了一种Floquet工程来研究冷原子中的相弦效应。
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引用次数: 4
Predicting impurity spectral functions using machine learning 利用机器学习预测杂质谱函数
Pub Date : 2020-11-21 DOI: 10.1103/PhysRevB.103.245118
Erica J. Sturm, Matthew R. Carbone, D. Lu, A. Weichselbaum, R. Konik
The Anderson Impurity Model (AIM) is a canonical model of quantum many-body physics. Here we investigate whether machine learning models, both neural networks (NN) and kernel ridge regression (KRR), can accurately predict the AIM spectral function in all of its regimes, from empty orbital, to mixed valence, to Kondo. To tackle this question, we construct two large spectral databases containing approximately 410k and 600k spectral functions of the single-channel impurity problem. We show that the NN models can accurately predict the AIM spectral function in all of its regimes, with point-wise mean absolute errors down to 0.003 in normalized units. We find that the trained NN models outperform models based on KRR and enjoy a speedup on the order of $10^5$ over traditional AIM solvers. The required size of the training set of our model can be significantly reduced using furthest point sampling in the AIM parameter space, which is important for generalizing our method to more complicated multi-channel impurity problems of relevance to predicting the properties of real materials.
安德森杂质模型(AIM)是量子多体物理的一个经典模型。在这里,我们研究了机器学习模型,包括神经网络(NN)和核脊回归(KRR),是否可以准确地预测AIM的所有谱函数,从空轨道到混合价态,再到近藤。为了解决这个问题,我们构建了两个大型的光谱数据库,其中包含大约410k和600k的单通道杂质问题的光谱函数。我们表明,神经网络模型可以准确地预测AIM谱函数的所有区域,在归一化单位下,逐点平均绝对误差降至0.003。我们发现训练后的神经网络模型优于基于KRR的模型,并且比传统的AIM求解器加速了10^5美元。使用AIM参数空间中的最远点采样可以显著减少模型所需的训练集大小,这对于将我们的方法推广到与预测实际材料性质相关的更复杂的多通道杂质问题具有重要意义。
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引用次数: 6
Doping the chiral spin liquid: Topological superconductor or chiral metal 掺杂手性自旋液体:拓扑超导体或手性金属
Pub Date : 2020-11-19 DOI: 10.1103/PHYSREVB.103.165138
Xue Song, A. Vishwanath, Ya-Hui Zhang
We point out that there are two different chiral spin liquid states on the triangular lattice and discuss the conducting states that are expected on doping them. These states labeled CS1 and CS2 are associated with two distinct topological orders with different edge states, although they both spontaneously break time reversal symmetry and exhibit the same quantized spin Hall conductance. While CSL1 is related to the Kalmeyer-Laughlin state, CSL2 is the $nu =4$ member of Kitaev's 16 fold way classification. Both states are described within the Abrikosov fermion representation of spins, and the effect of doping can be accessed by introducing charged holons. On doping CSL2, condensation of charged holons leads to a topological d+id superconductor. However on doping CSL1 , in sharp contrast , two different scenarios can arise: first, if holons condense, a chiral metal with doubled unit cell and finite Hall conductivity is obtained. However, in a second novel scenario, the internal magnetic flux adjusts with doping and holons form a bosonic integer quantum Hall (BIQH) state. Remarkably, the latter phase is identical to a $d+id$ superconductor. In this case the Mott insulator to superconductor transition is associated with a bosonic variant of the integer quantum Hall plateau transition for the holon. Finally we connect the above two scenarios to two recent numerical studies of doped chiral spin liquids on triangular lattice. Our work clarifies the complex relation between topological superconductors, chiral spin liquids and quantum criticality .
我们指出三角形晶格上存在两种不同的手性自旋液态,并讨论了掺杂它们所期望的导电态。这些被标记为CS1和CS2的状态与两种具有不同边缘态的不同拓扑序相关,尽管它们都自发地打破时间反转对称并表现出相同的量子化自旋霍尔电导。CSL1与Kalmeyer-Laughlin状态有关,而CSL2是Kitaev 16折道分类中的$nu =4$成员。这两种状态都可以用自旋的Abrikosov费米子表示来描述,并且掺杂效应可以通过引入带电的空子来实现。在掺杂CSL2时,带电空子的缩聚导致了拓扑d+id超导体。然而,在掺杂CSL1时,则会出现两种截然不同的情况:第一,如果粒子凝聚,则会得到具有双晶胞和有限霍尔电导率的手性金属。然而,在第二种新情况下,内部磁通量随掺杂而调整,并且量子形成玻色子整数量子霍尔(BIQH)态。值得注意的是,后一相与$d+id$超导体相同。在这种情况下,莫特绝缘体到超导体的跃迁与整数量子霍尔平台跃迁的玻色子变体有关。最后,我们将上述两种情况与最近两项三角晶格上掺杂手性自旋液体的数值研究联系起来。我们的工作阐明了拓扑超导体、手性自旋液体和量子临界之间的复杂关系。
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引用次数: 20
Electronic multipoles in second harmonic generation and neutron scattering 二次谐波产生中的电子多极子和中子散射
Pub Date : 2020-11-18 DOI: 10.1103/PHYSREVB.103.125124
G. van der Laan, S. Lovesey
Nonlinear optics, and particularly second harmonic generation (SHG), is increasingly used in many modern disciplines from material characterization in physical sciences to bio-imaging in medicine and optical signal processing in information technology. We present a theoretical analysis providing a strong estimate for the energy-integrated SHG response. Requirements of symmetry in time and space are fully respected in the calculation, and estimates of natural and magnetic circular dichroic signals are superior to previous ones. Like symmetry requirements are traced in the amplitude for magnetic neutron scattering, which includes all axial and polar (Dirac) contributions. Our method of working, in terms of spherical multipoles and implementation of symmetry, could be of use in a variety of other probes of electronic properties.
非线性光学,特别是二次谐波产生(SHG),越来越多地应用于许多现代学科,从物理科学中的材料表征到医学中的生物成像和信息技术中的光信号处理。我们提出了一个理论分析,为能量集成的SHG响应提供了一个强有力的估计。在计算中充分考虑了时间和空间对称性的要求,对自然和磁性圆二向色信号的估计优于以往的估计。磁中子散射的振幅也有类似的对称性要求,包括所有轴向和极性(狄拉克)贡献。我们的工作方法,在球形多极和对称的实现方面,可以用于各种其他电子性质的探针。
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引用次数: 1
Bulk-edge correspondence with generalized chiral symmetry 广义手性对称的体边对应
Pub Date : 2020-11-18 DOI: 10.1103/PhysRevB.103.205306
T. Kawarabayashi, Y. Hatsugai
The bulk-edge correspondence in topological phases is extended to systems with the generalized chiral symmetry, where the conventional chiral symmetry is broken. In such systems, we find that the edge state exhibits an unconventional behavior in the presence of the symmetry breaking by the mass, which is explored explicitly in the case of a deformed Su-Schrieffer-Heeger model. The localization length of the edge states diverges at a certain critical mass, where the edge state touches to the bulk band. The edge state is specified by an imaginary wave vector that becomes real at the touching energy.
将拓扑相中的体边对应推广到具有广义手性对称的系统,打破了传统的手性对称。在这样的系统中,我们发现边缘态在质量对称性破缺的情况下表现出一种非常规的行为,这在变形的Su-Schrieffer-Heeger模型中得到了明确的探讨。边缘态的局域化长度在某一临界质量处发散,此时边缘态与体带接触。边缘状态由虚波矢量指定,虚波矢量在接触能量处变为实波矢量。
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引用次数: 3
ABCD of Kondo Effect 近藤效应的ABCD
Pub Date : 2020-11-16 DOI: 10.7566/JPSJ.90.024708
Taro Kimura
We explore the Kondo effect incorporating the localized impurity transforming under generic symmetry group $G$, that we call the $G$-Kondo effect. We derive the one-dimensional effective model coupled with the impurity, and studied the thermodynamic properties based on the boundary conformal field theory approach. We in particular study the impurity entropy at the conformal fixed point, and the low temperature behavior of the specific heat and the susceptibility. We also consider the Wilson ratio based on these results, and mention the case with exceptional group symmetry.
我们探讨了在一般对称群$G$下包含局部杂质变换的近藤效应,我们称之为$G$-近藤效应。导出了与杂质耦合的一维有效模型,并基于边界共形场理论方法研究了其热力学性质。我们特别研究了共形固定点处的杂质熵,以及比热和磁化率的低温行为。我们也在此基础上考虑了威尔森比率,并提到了特殊群对称的情况。
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引用次数: 8
Analytical solution for time integrals in diagrammatic expansions: Application to real-frequency diagrammatic Monte Carlo 图解展开中时间积分的解析解:在实频图解蒙特卡罗中的应用
Pub Date : 2020-11-16 DOI: 10.1103/PHYSREVRESEARCH.3.023082
J. Vučičević, P. Stipsić, M. Ferrero
The past years have seen a revived interest in the diagrammatic Monte Carlo (DiagMC) methods for interacting fermions on a lattice. A promising recent development allows one to now circumvent the analytical continuation of dynamic observables in DiagMC calculations within the Matsubara formalism. This is made possible by symbolic algebra algorithms, which can be used to analytically solve the internal Matsubara frequency summations of Feynman diagrams. In this paper, we take a different approach and show that it yields improved results. We present a closed-form analytical solution of imaginary-time integrals that appear in the time-domain formulation of Feynman diagrams. We implement and test a DiagMC algorithm based on this analytical solution and show that it has numerous significant advantages. Most importantly, the algorithm is general enough for any kind of single-time correlation function series, involving any single-particle vertex insertions. Therefore, it readily allows for the use of action-shifted schemes, aimed at improving the convergence properties of the series. By performing a frequency-resolved action-shift tuning, we are able to further improve the method and converge the self-energy in a non-trivial regime, with only 3-4 perturbation orders. Finally, we identify time integrals of the same general form in many commonly used Monte Carlo algorithms and therefore expect a broader usage of our analytical solution.
在过去的几年里,人们对费米子在晶格上相互作用的图解蒙特卡罗(DiagMC)方法重新产生了兴趣。最近有一个很有希望的发展,允许人们现在绕过在Matsubara形式下的DiagMC计算中动态可观测值的分析延拓。这可以通过符号代数算法实现,该算法可用于解析求解费曼图的内部Matsubara频率求和。在本文中,我们采用了一种不同的方法,并表明它产生了改进的结果。本文给出了费曼图时域公式中虚时间积分的一个封闭解析解。我们实现并测试了基于该解析解的DiagMC算法,并表明它具有许多显着的优点。最重要的是,该算法具有足够的通用性,适用于任何类型的单时间相关函数序列,包括任何单粒子顶点插入。因此,它很容易允许使用动作转换方案,旨在提高级数的收敛性。通过执行频率分辨动作移位调谐,我们能够进一步改进该方法,并在只有3-4个扰动阶的非平凡状态下收敛自能量。最后,我们在许多常用的蒙特卡罗算法中确定了相同一般形式的时间积分,因此期望我们的解析解得到更广泛的应用。
{"title":"Analytical solution for time integrals in diagrammatic expansions: Application to real-frequency diagrammatic Monte Carlo","authors":"J. Vučičević, P. Stipsić, M. Ferrero","doi":"10.1103/PHYSREVRESEARCH.3.023082","DOIUrl":"https://doi.org/10.1103/PHYSREVRESEARCH.3.023082","url":null,"abstract":"The past years have seen a revived interest in the diagrammatic Monte Carlo (DiagMC) methods for interacting fermions on a lattice. A promising recent development allows one to now circumvent the analytical continuation of dynamic observables in DiagMC calculations within the Matsubara formalism. This is made possible by symbolic algebra algorithms, which can be used to analytically solve the internal Matsubara frequency summations of Feynman diagrams. In this paper, we take a different approach and show that it yields improved results. We present a closed-form analytical solution of imaginary-time integrals that appear in the time-domain formulation of Feynman diagrams. We implement and test a DiagMC algorithm based on this analytical solution and show that it has numerous significant advantages. Most importantly, the algorithm is general enough for any kind of single-time correlation function series, involving any single-particle vertex insertions. Therefore, it readily allows for the use of action-shifted schemes, aimed at improving the convergence properties of the series. By performing a frequency-resolved action-shift tuning, we are able to further improve the method and converge the self-energy in a non-trivial regime, with only 3-4 perturbation orders. Finally, we identify time integrals of the same general form in many commonly used Monte Carlo algorithms and therefore expect a broader usage of our analytical solution.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"84 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-11-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"83258895","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 3
Effective magnetic Hamiltonian at finite temperatures for rare-earth chalcogenides 稀土硫族化合物有限温度下的有效磁哈密顿量
Pub Date : 2020-11-12 DOI: 10.1103/PhysRevB.103.184419
Zheng Zhang, Jianshu Li, Weiwei Liu, Zhitao Zhang, J. Ji, F. Jin, Rui Chen, Junfeng Wang, Xiaoqun Wang, Jie Ma, Qing-ming Zhang
Alkali metal rare-earth chalcogenide $ARECh2$ (A=alkali or monovalent metal, RE=rare earth, Ch=O, S, Se, Te), is a large family of quantum spin liquid (QSL) candidates we discovered recently. Unlike $YbMgGaO4$, most members in the family except for the oxide ones, have relatively small crystalline electric-field (CEF) excitation levels, particularly the first ones. This makes the conventional Curie-Weiss analysis at finite temperatures inapplicable and CEF excitations may play an essential role in understanding the low-energy spin physics. Here we considered an effective magnetic Hamiltonian incorporating CEF excitations and spin-spin interactions, to accurately describe thermodynamics in such a system. By taking $NaYbSe2$ as an example, we were able to analyze magnetic susceptibility, magnetization under pulsed high fields and heat capacity in a systematic and comprehensive way. The analysis allows us to produce accurate anisotropic exchange coupling energies and unambiguously determine a crossover temperature ($sim$25 K in the case of $NaYbSe2$), below which CEF effects fade away and pure spin-spin interactions stand out. We further validated the effective picture by successfully explaining the anomalous temperature dependence of electron spin resonance (ESR) spectral width. The effective scenario in principle can be generalized to other rare-earth spin systems with small CEF excitations.
碱金属稀土硫族化合物ARECh2$ (A=碱金属或单价金属,RE=稀土,Ch=O, S, Se, Te)是我们最近发现的一大族量子自旋液体(QSL)候选者。与YbMgGaO4不同,除了氧化物外,家族中的大多数成员具有相对较小的晶体电场(CEF)激发水平,特别是第一个。这使得传统的Curie-Weiss分析在有限温度下不适用,CEF激发可能在理解低能自旋物理中发挥重要作用。在这里,我们考虑了一个有效的磁哈密顿量,包括CEF激励和自旋-自旋相互作用,以准确地描述这种系统中的热力学。以$NaYbSe2$为例,对其磁化率、脉冲强场磁化强度和热容进行了系统全面的分析。分析使我们能够产生准确的各向异性交换耦合能量和明确地确定交叉温度25美元($ sim K在NaYbSe2)美元的情况下,下面的英语影响哪消失和纯自旋自旋相互作用突出。我们成功地解释了电子自旋共振(ESR)谱宽的反常温度依赖性,进一步验证了有效图。原理上的有效情形可以推广到其他具有较小CEF激励的稀土自旋体系。
{"title":"Effective magnetic Hamiltonian at finite temperatures for rare-earth chalcogenides","authors":"Zheng Zhang, Jianshu Li, Weiwei Liu, Zhitao Zhang, J. Ji, F. Jin, Rui Chen, Junfeng Wang, Xiaoqun Wang, Jie Ma, Qing-ming Zhang","doi":"10.1103/PhysRevB.103.184419","DOIUrl":"https://doi.org/10.1103/PhysRevB.103.184419","url":null,"abstract":"Alkali metal rare-earth chalcogenide $ARECh2$ (A=alkali or monovalent metal, RE=rare earth, Ch=O, S, Se, Te), is a large family of quantum spin liquid (QSL) candidates we discovered recently. Unlike $YbMgGaO4$, most members in the family except for the oxide ones, have relatively small crystalline electric-field (CEF) excitation levels, particularly the first ones. This makes the conventional Curie-Weiss analysis at finite temperatures inapplicable and CEF excitations may play an essential role in understanding the low-energy spin physics. Here we considered an effective magnetic Hamiltonian incorporating CEF excitations and spin-spin interactions, to accurately describe thermodynamics in such a system. By taking $NaYbSe2$ as an example, we were able to analyze magnetic susceptibility, magnetization under pulsed high fields and heat capacity in a systematic and comprehensive way. The analysis allows us to produce accurate anisotropic exchange coupling energies and unambiguously determine a crossover temperature ($sim$25 K in the case of $NaYbSe2$), below which CEF effects fade away and pure spin-spin interactions stand out. We further validated the effective picture by successfully explaining the anomalous temperature dependence of electron spin resonance (ESR) spectral width. The effective scenario in principle can be generalized to other rare-earth spin systems with small CEF excitations.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"84 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-11-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"90938625","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 11
Dynamical topological excitations in parafermion chains 对偶子链中的动态拓扑激励
Pub Date : 2020-11-12 DOI: 10.1103/PHYSREVRESEARCH.3.013095
Vilja Kaskela, J. Lado
Topological excitations in many-body systems are one of the paradigmatic cornerstones of modern condensed matter physics. In particular, parafermions are elusive fractional excitations potentially emerging in fractional quantum Hall-superconductor junctions, and represent one of the major milestones in fractional quantum matter. Here, by using a combination of tensor network and kernel polynomial techniques, we demonstrate the emergence of zero modes and finite energy excitations in many-body parafermion chains. We show the appearance of zero energy modes in the many-body spectral function at the edge of a topological parafermion chain, their relation with the topological degeneracy of the system, and we compare their physics with the Majorana bound states of topological superconductors. We demonstrate the robustness of parafermion topological modes with respect to a variety of perturbations, and we show how weakly coupled parafermion chains give rise to in-gap excitations. Our results exemplify the versatility of tensor network methods for studying dynamical excitations of interacting parafermion chains, and highlight the robustness of topological modes in parafermion models.
多体系统中的拓扑激励是现代凝聚态物理的典范基础之一。特别是,对偶粒子是难以捉摸的分数激发,可能出现在分数量子霍尔-超导体结中,代表了分数量子物质的主要里程碑之一。本文通过张量网络和核多项式技术的结合,证明了多体对偶子链中零模和有限能量激发的出现。我们展示了拓扑对偶子链边缘的多体谱函数中零能量模式的出现,它们与系统的拓扑简并的关系,并将它们的物理性质与拓扑超导体的马约拉纳束缚态进行了比较。我们证明了对偶粒子拓扑模式相对于各种扰动的鲁棒性,并且我们展示了弱耦合对偶粒子链如何引起间隙内激发。我们的研究结果证明了张量网络方法在研究相互作用的对偶子链的动力学激励方面的通用性,并突出了对偶子模型中拓扑模式的鲁棒性。
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引用次数: 7
Magnetic order in the chemically substituted frustrated antiferromagnet CsCrF4 化学取代受挫反铁磁体CsCrF4的磁序
Pub Date : 2020-11-12 DOI: 10.1103/PhysRevB.102.174440
S. Hayashida, M. Hagihala, M. Avdeev, Y. Miura, H. Manaka, T. Masuda
The effect of chemical substitution on the ground state of the geometrically frustrated antiferromagnet CsCrF$_4$ has been investigated through a neutron powder diffraction experiment. Magnetic Fe-substituted CsCr$_{0.94}$Fe$_{0.06}$F$_{4}$ and nonmagnetic Al-substituted CsCr$_{0.98}$Al$_{0.02}$F$_{4}$ samples are measured, and magnetic Bragg peaks are clearly observed in both samples. Magnetic structure analysis revealed a 120$^{circ}$ structure having a magnetic propagation vector $mathbf{k}_{rm mag}=(0,0,1/2)$ in CsCr$_{0.94}$Fe$_{0.06}$F$_{4}$. For CsCr$_{0.98}$Al$_{0.02}$F$_{4}$, a quasi-120$^{circ}$ structure having $mathbf{k}_{rm mag}=(1/2,0,1/2)$ is formed. It is notable that the identified magnetic structure in CsCr$_{0.94}$Fe$_{0.06}$F$_{4}$ belongs to a different phase of ground states from those in CsCr$_{0.98}$Al$_{0.02}$F$_{4}$ and the parent CsCrF$_{4}$. These results suggest that the Fe-substitution strongly influences the ground state of CsCrF$_{4}$.
通过中子粉末衍射实验,研究了化学取代对几何受挫反铁磁体CsCrF$_4$基态的影响。测量了磁性Fe-取代CsCr$_{0.94}$Fe$_{0.06}$F$_{4}$和非磁性Al-取代CsCr$_{0.98}$Al$_{0.02}$F$_{4}$样品,在两个样品中都清晰地观察到磁性布拉格峰。磁结构分析表明,在CsCr$_{0.94}$Fe$_{0.06}$F$_{4}$中,120$ $^{circ}$结构具有磁传播向量$mathbf{k}_{rm mag}=(0,0,1/2)$。为CsCr Al美元$ _ {0.98}_ {0.02}$ F $ _{4} $,准- 120 $ ^{保监会}结构拥有美元 mathbf {k} _ { rm杂志}=(1/2,0,1/2)形成美元。值得注意的是,CsCr$_{0.94}$Fe$_{0.06}$F$_{4}$的磁性结构与CsCr$_{0.98}$Al$_{0.02}$F$_{4}$和母体CsCrF$_{4}$的磁性结构属于不同的基态相。这些结果表明,fe取代对CsCrF$_{4}$的基态影响很大。
{"title":"Magnetic order in the chemically substituted frustrated antiferromagnet \u0000CsCrF4","authors":"S. Hayashida, M. Hagihala, M. Avdeev, Y. Miura, H. Manaka, T. Masuda","doi":"10.1103/PhysRevB.102.174440","DOIUrl":"https://doi.org/10.1103/PhysRevB.102.174440","url":null,"abstract":"The effect of chemical substitution on the ground state of the geometrically frustrated antiferromagnet CsCrF$_4$ has been investigated through a neutron powder diffraction experiment. Magnetic Fe-substituted CsCr$_{0.94}$Fe$_{0.06}$F$_{4}$ and nonmagnetic Al-substituted CsCr$_{0.98}$Al$_{0.02}$F$_{4}$ samples are measured, and magnetic Bragg peaks are clearly observed in both samples. Magnetic structure analysis revealed a 120$^{circ}$ structure having a magnetic propagation vector $mathbf{k}_{rm mag}=(0,0,1/2)$ in CsCr$_{0.94}$Fe$_{0.06}$F$_{4}$. For CsCr$_{0.98}$Al$_{0.02}$F$_{4}$, a quasi-120$^{circ}$ structure having $mathbf{k}_{rm mag}=(1/2,0,1/2)$ is formed. It is notable that the identified magnetic structure in CsCr$_{0.94}$Fe$_{0.06}$F$_{4}$ belongs to a different phase of ground states from those in CsCr$_{0.98}$Al$_{0.02}$F$_{4}$ and the parent CsCrF$_{4}$. These results suggest that the Fe-substitution strongly influences the ground state of CsCrF$_{4}$.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"29 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-11-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"86561457","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
arXiv: Strongly Correlated Electrons
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