Pub Date : 2020-10-16DOI: 10.1103/PhysRevB.104.035154
P. Menegasso, J. Souza, I. Vinograd, Z. Wang, S. Edwards, P. Pagliuso, N. Curro, R. Urbano
The transferred hyperfine interaction between nuclear and electron spins in an heavy fermion material depends on the hybridization between the $f$-electron orbitals and those surrounding a distant nucleus. In CeMIn$_5$ (M=Rh, Ir, Co), both the hyperfine coupling to the two indium sites as well as the crystalline electric field at the Ce are strongly dependent on the transition metal. We measure a series of CeRh$_{1-x}$Ir$_x$In$_5$ crystals and find that the hyperfine coupling reflects the orbital anisotropy of the ground state Ce 4$f$ wavefunction. These findings provide direct proof that the localized to itinerant transition is dominated by hybridization out of the Ce-In plane in this system.
在重费米子物质中,原子核和电子自旋之间的超精细相互作用依赖于f电子轨道和远处原子核周围轨道之间的杂化。在CeMIn$_5$ (M=Rh, Ir, Co)中,与两个铟位点的超精细耦合以及Ce处的晶体电场都强烈依赖于过渡金属。我们测量了一系列的CeRh$_{1-x}$Ir$_x$In$_5$晶体,发现超精细耦合反映了基态ce4 $f$波函数的轨道各向异性。这些发现提供了直接的证据,证明在该体系中,定位到流动的转变主要是Ce-In平面外的杂交。
{"title":"Hyperfine couplings as a probe of orbital anisotropy in heavy-fermion materials","authors":"P. Menegasso, J. Souza, I. Vinograd, Z. Wang, S. Edwards, P. Pagliuso, N. Curro, R. Urbano","doi":"10.1103/PhysRevB.104.035154","DOIUrl":"https://doi.org/10.1103/PhysRevB.104.035154","url":null,"abstract":"The transferred hyperfine interaction between nuclear and electron spins in an heavy fermion material depends on the hybridization between the $f$-electron orbitals and those surrounding a distant nucleus. In CeMIn$_5$ (M=Rh, Ir, Co), both the hyperfine coupling to the two indium sites as well as the crystalline electric field at the Ce are strongly dependent on the transition metal. We measure a series of CeRh$_{1-x}$Ir$_x$In$_5$ crystals and find that the hyperfine coupling reflects the orbital anisotropy of the ground state Ce 4$f$ wavefunction. These findings provide direct proof that the localized to itinerant transition is dominated by hybridization out of the Ce-In plane in this system.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"3 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"79840821","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-10-15DOI: 10.21468/SCIPOSTPHYS.10.1.019
D. Poilblanc, M. Mambrini, F. Alet
Within the tensor network framework, the (positive) thermal density operator can be approximated by a double layer of infinite Projected Entangled Pair Operator (iPEPO) coupled via ancilla degrees of freedom. To investigate the thermal properties of the spin-1/2 Heisenberg model on the square lattice, we introduce a family of fully spin-$SU(2)$ and lattice-$C_{4v}$ symmetric on-site tensors (of bond dimensions $D=4$ or $D=7$) and a plaquette-based Trotter-Suzuki decomposition of the imaginary-time evolution operator. A variational optimization is performed on the plaquettes, using a full (for $D=4$) or simple (for $D=7$) environment obtained from the single-site Corner Transfer Matrix Renormalization Group fixed point. The method is benchmarked by a comparison to quantum Monte Carlo in the thermodynamic limit. Although the iPEPO spin correlation length starts to deviate from the exact exponential growth for inverse-temperature $beta gtrsim 2$, the behavior of various observables turns out to be quite accurate once plotted w.r.t the inverse correlation length. We also find that a direct $T=0$ variational energy optimization provides results in full agreement with the $betarightarrowinfty$ limit of finite-temperature data, hence validating the imaginary-time evolution procedure. Extension of the method to frustrated models is described and preliminary results are shown.
{"title":"Finite-temperature symmetric tensor network for spin-1/2 Heisenberg antiferromagnets on the square lattice","authors":"D. Poilblanc, M. Mambrini, F. Alet","doi":"10.21468/SCIPOSTPHYS.10.1.019","DOIUrl":"https://doi.org/10.21468/SCIPOSTPHYS.10.1.019","url":null,"abstract":"Within the tensor network framework, the (positive) thermal density operator can be approximated by a double layer of infinite Projected Entangled Pair Operator (iPEPO) coupled via ancilla degrees of freedom. To investigate the thermal properties of the spin-1/2 Heisenberg model on the square lattice, we introduce a family of fully spin-$SU(2)$ and lattice-$C_{4v}$ symmetric on-site tensors (of bond dimensions $D=4$ or $D=7$) and a plaquette-based Trotter-Suzuki decomposition of the imaginary-time evolution operator. A variational optimization is performed on the plaquettes, using a full (for $D=4$) or simple (for $D=7$) environment obtained from the single-site Corner Transfer Matrix Renormalization Group fixed point. The method is benchmarked by a comparison to quantum Monte Carlo in the thermodynamic limit. Although the iPEPO spin correlation length starts to deviate from the exact exponential growth for inverse-temperature $beta gtrsim 2$, the behavior of various observables turns out to be quite accurate once plotted w.r.t the inverse correlation length. We also find that a direct $T=0$ variational energy optimization provides results in full agreement with the $betarightarrowinfty$ limit of finite-temperature data, hence validating the imaginary-time evolution procedure. Extension of the method to frustrated models is described and preliminary results are shown.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"1 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"72571196","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-10-15DOI: 10.1103/physrevresearch.2.042023
T. Kobayashi, Q. Ding, H. Taniguchi, K. Satoh, A. Kawamoto, Y. Furukawa
The spin-liquid candidate $kappa$-(ET)$_2$Cu$_2$(CN)$_3$ [ET: bis(ethylenedithio)tetrathiafulvalene] does not exhibit magnetic ordering down to a very low temperature, but shows a mysterious anomaly at 6 K. The origin of the so-called 6 K anomaly is still under debate. We carried out nuclear quadrupole resonance (NQR) measurements on the copper sites of the insulating layers, which are sensitive to the charge dynamics unlike the conventional spin-1/2 nuclear magnetic resonance (NMR). The main finding of this study is that the observation of a sharp peak behavior in the nuclear spin-lattice relaxation rate $T_1^{-1}$ of $^{63}$Cu NQR at 6 K while $T_1^{-1}$ of both $^{13}$C and $^{1}$H NMR show no clear anomaly. This behavior can be understood as a second-order phase transition related to charge disproportionation in the ET layers.
{"title":"Charge disproportionation in the spin-liquid candidate \u0000κ−(ET)2Cu2(CN)3\u0000 at 6 K revealed by \u0000Cu63\u0000 NQR measurements","authors":"T. Kobayashi, Q. Ding, H. Taniguchi, K. Satoh, A. Kawamoto, Y. Furukawa","doi":"10.1103/physrevresearch.2.042023","DOIUrl":"https://doi.org/10.1103/physrevresearch.2.042023","url":null,"abstract":"The spin-liquid candidate $kappa$-(ET)$_2$Cu$_2$(CN)$_3$ [ET: bis(ethylenedithio)tetrathiafulvalene] does not exhibit magnetic ordering down to a very low temperature, but shows a mysterious anomaly at 6 K. The origin of the so-called 6 K anomaly is still under debate. We carried out nuclear quadrupole resonance (NQR) measurements on the copper sites of the insulating layers, which are sensitive to the charge dynamics unlike the conventional spin-1/2 nuclear magnetic resonance (NMR). The main finding of this study is that the observation of a sharp peak behavior in the nuclear spin-lattice relaxation rate $T_1^{-1}$ of $^{63}$Cu NQR at 6 K while $T_1^{-1}$ of both $^{13}$C and $^{1}$H NMR show no clear anomaly. This behavior can be understood as a second-order phase transition related to charge disproportionation in the ET layers.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"4 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-10-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"76342167","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}