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Hyperfine couplings as a probe of orbital anisotropy in heavy-fermion materials 超精细耦合作为重费米子材料轨道各向异性的探针
Pub Date : 2020-10-16 DOI: 10.1103/PhysRevB.104.035154
P. Menegasso, J. Souza, I. Vinograd, Z. Wang, S. Edwards, P. Pagliuso, N. Curro, R. Urbano
The transferred hyperfine interaction between nuclear and electron spins in an heavy fermion material depends on the hybridization between the $f$-electron orbitals and those surrounding a distant nucleus. In CeMIn$_5$ (M=Rh, Ir, Co), both the hyperfine coupling to the two indium sites as well as the crystalline electric field at the Ce are strongly dependent on the transition metal. We measure a series of CeRh$_{1-x}$Ir$_x$In$_5$ crystals and find that the hyperfine coupling reflects the orbital anisotropy of the ground state Ce 4$f$ wavefunction. These findings provide direct proof that the localized to itinerant transition is dominated by hybridization out of the Ce-In plane in this system.
在重费米子物质中,原子核和电子自旋之间的超精细相互作用依赖于f电子轨道和远处原子核周围轨道之间的杂化。在CeMIn$_5$ (M=Rh, Ir, Co)中,与两个铟位点的超精细耦合以及Ce处的晶体电场都强烈依赖于过渡金属。我们测量了一系列的CeRh$_{1-x}$Ir$_x$In$_5$晶体,发现超精细耦合反映了基态ce4 $f$波函数的轨道各向异性。这些发现提供了直接的证据,证明在该体系中,定位到流动的转变主要是Ce-In平面外的杂交。
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引用次数: 1
Finite-temperature symmetric tensor network for spin-1/2 Heisenberg antiferromagnets on the square lattice 方形晶格上自旋1/2海森堡反铁磁体的有限温度对称张量网络
Pub Date : 2020-10-15 DOI: 10.21468/SCIPOSTPHYS.10.1.019
D. Poilblanc, M. Mambrini, F. Alet
Within the tensor network framework, the (positive) thermal density operator can be approximated by a double layer of infinite Projected Entangled Pair Operator (iPEPO) coupled via ancilla degrees of freedom. To investigate the thermal properties of the spin-1/2 Heisenberg model on the square lattice, we introduce a family of fully spin-$SU(2)$ and lattice-$C_{4v}$ symmetric on-site tensors (of bond dimensions $D=4$ or $D=7$) and a plaquette-based Trotter-Suzuki decomposition of the imaginary-time evolution operator. A variational optimization is performed on the plaquettes, using a full (for $D=4$) or simple (for $D=7$) environment obtained from the single-site Corner Transfer Matrix Renormalization Group fixed point. The method is benchmarked by a comparison to quantum Monte Carlo in the thermodynamic limit. Although the iPEPO spin correlation length starts to deviate from the exact exponential growth for inverse-temperature $beta gtrsim 2$, the behavior of various observables turns out to be quite accurate once plotted w.r.t the inverse correlation length. We also find that a direct $T=0$ variational energy optimization provides results in full agreement with the $betarightarrowinfty$ limit of finite-temperature data, hence validating the imaginary-time evolution procedure. Extension of the method to frustrated models is described and preliminary results are shown.
在张量网络框架内,(正)热密度算子可以用通过辅助自由度耦合的无限投影纠缠对算子(iPEPO)的双层来近似。为了研究方形晶格上自旋-1/2海森堡模型的热性质,我们引入了一组完全自旋- $SU(2)$和晶格- $C_{4v}$对称的现场张量(键维为$D=4$或$D=7$)和基于空泡的虚时间演化算子的Trotter-Suzuki分解。对斑块进行变分优化,使用从单站点角转移矩阵重整化组固定点获得的完整(对于$D=4$)或简单(对于$D=7$)环境。该方法在热力学极限下与量子蒙特卡罗进行了比较。虽然iPEPO自旋相关长度开始偏离逆温度$beta gtrsim 2$的确切指数增长,但一旦绘制逆相关长度,各种可观测值的行为就变得相当准确。我们还发现,直接$T=0$变分能量优化提供的结果完全符合$betarightarrowinfty$有限温度数据的极限,从而验证了虚时间演化过程。将该方法推广到受挫模型,并给出了初步结果。
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引用次数: 8
Charge disproportionation in the spin-liquid candidate κ−(ET)2Cu2(CN)3 at 6 K revealed by Cu63 NQR measurements Cu63 NQR测量揭示了自旋液体候选物κ−(ET)2Cu2(CN)3在6k时的电荷歧化现象
Pub Date : 2020-10-15 DOI: 10.1103/physrevresearch.2.042023
T. Kobayashi, Q. Ding, H. Taniguchi, K. Satoh, A. Kawamoto, Y. Furukawa
The spin-liquid candidate $kappa$-(ET)$_2$Cu$_2$(CN)$_3$ [ET: bis(ethylenedithio)tetrathiafulvalene] does not exhibit magnetic ordering down to a very low temperature, but shows a mysterious anomaly at 6 K. The origin of the so-called 6 K anomaly is still under debate. We carried out nuclear quadrupole resonance (NQR) measurements on the copper sites of the insulating layers, which are sensitive to the charge dynamics unlike the conventional spin-1/2 nuclear magnetic resonance (NMR). The main finding of this study is that the observation of a sharp peak behavior in the nuclear spin-lattice relaxation rate $T_1^{-1}$ of $^{63}$Cu NQR at 6 K while $T_1^{-1}$ of both $^{13}$C and $^{1}$H NMR show no clear anomaly. This behavior can be understood as a second-order phase transition related to charge disproportionation in the ET layers.
自旋液体候选物$kappa$-(ET)$_2$Cu$_2$(CN)$_3$ [ET: bis(乙二硫代)四硫代烯]在极低温度下不表现出磁有序,但在6 K时表现出神秘的异常。所谓的6k异常的起源仍在争论中。我们对绝缘层铜位进行了核四极共振(NQR)测量,这与传统的自旋1/2核磁共振(NMR)不同,它对电荷动力学敏感。本研究的主要发现是在6 K时,$^{63}$Cu NQR的核自旋-晶格弛豫率$T_1^{-1}$有一个尖峰行为,而$^{13}$C和$^{1}$H的核自旋-晶格弛豫率$T_1^{-1}$没有明显的异常。这种行为可以理解为与ET层中电荷歧化有关的二级相变。
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引用次数: 8
Statistics-tuned entanglement of the boundary modes in coupled Su-Schrieffer-Heeger chains 耦合Su-Schrieffer-Heeger链中边界模的统计调谐纠缠
Pub Date : 2020-10-14 DOI: 10.1103/PhysRevB.103.195134
Saikat Santra, A. Agarwala, S. Bhattacharjee
We show that mutual statistics between quantum particles can be tuned to generate emergent novel few particle quantum mechanics for the boundary modes of symmetry-protected topological phases of matter. As a concrete setting, we study a system of pseudofermions, defined as quantum particles with tunable algebra, which lie on two distinct Su-Schrieffer-Heeger (SSH) chains. We find that as the mutual statistics of the particles are tuned -- the boundary modes present in the two chains gets non-trivially entangled showing a sudden jump in their mutual entanglement entropy. We further show that, such tuning of statistics engenders a first-order transition between two topologically non-trivial phases which differ in the behavior of inter-chain entanglement. Using a combination of analytical and numerical techniques and effective modeling, we uncover the rich physics that this system hosts. The results are of particular relevance in context of the study of the effective low energy quantum mechanics of topological edge modes in one hand and their recent realization in ultracold atoms on the other. This then provides for controlled manipulation of such low energy modes.
我们证明了量子粒子之间的相互统计量可以被调谐,从而为对称保护的物质拓扑相的边界模式产生新兴的少数粒子量子力学。作为一个具体的设置,我们研究了一个假费米子系统,它被定义为具有可调代数的量子粒子,它位于两个不同的Su-Schrieffer-Heeger (SSH)链上。我们发现,当粒子的相互统计量被调整时,两条链中的边界模式变得非平凡地纠缠在一起,显示出它们的相互纠缠熵的突然跳跃。我们进一步表明,这种统计量的调整在两个拓扑上非平凡的相之间产生了一阶跃迁,这两个相在链间纠缠的行为上是不同的。通过结合分析和数值技术以及有效的建模,我们揭示了这个系统所包含的丰富物理特性。这些结果对于拓扑边缘模式的有效低能量子力学的研究以及它们最近在超冷原子中的实现具有特殊的意义。这就提供了这种低能量模式的可控操作。
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引用次数: 2
Formation of spatial patterns by spin-selective excitations of interacting fermions 相互作用费米子的自旋选择性激发形成的空间模式
Pub Date : 2020-10-14 DOI: 10.1103/physrevb.102.235166
T. Köhler, S. Paeckel, C. Meyer, S. Manmana
We describe the formation of charge- and spin-density patterns induced by spin-selective photoexcitations of interacting fermionic systems in the presence of a microstructure. As an example, we consider a one-dimensional Hubbard-like system with a periodic magnetic microstructure, which has a uniform charge distribution in its ground state, and in which a long-lived charge-density pattern is induced by the spin-selective photoexcitation. Using tensor-network methods, we study the full quantum dynamics in the presence of electron-electron interactions and identify doublons as main decay channel for the induced charge pattern. Our setup is compared to the OISTR mechanism, in which ultrafast optically induced spin-transfer in Heusler and magnetic compounds is associated to the difference of the local density of states of the different elements in the alloys. We find that applying a spin-selective excitation there induces spatially periodic patterns in local observables. Implications for pump-probe experiments on correlated materials and experiments with ultracold gases on optical lattices are discussed.
我们描述了在微观结构存在的情况下,由相互作用费米子系统的自旋选择性光激发引起的电荷和自旋密度模式的形成。作为一个例子,我们考虑了一个具有周期性磁微结构的一维类哈伯德系统,该系统在基态具有均匀的电荷分布,并且在自旋选择性光激发下产生了长寿命的电荷密度图。利用张量网络方法,我们研究了电子-电子相互作用下的全量子动力学,并确定了双双子是诱导电荷模式的主要衰变通道。我们的装置与OISTR机制进行了比较,在OISTR机制中,Heusler和磁性化合物中的超快光诱导自旋转移与合金中不同元素的局部态密度的差异有关。我们发现在那里施加自旋选择性激励可以在局部观测中产生空间周期模式。讨论了相关材料的泵探实验和光晶格上的超冷气体实验的意义。
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引用次数: 1
Ab initio construction of the energy density functional for electron systems with the functional-renormalization-group-aided density functional theory 用泛函-重整化-群辅助密度泛函理论从头构造电子系统的能量密度泛函
Pub Date : 2020-10-14 DOI: 10.1103/PhysRevResearch.3.L012015
Takeru Yokota, T. Naito
We show an $textit{ab initio}$ construction of the energy density functional (EDF) for electron systems using the functional renormalization group. The correlation energies of the homogeneous electron gas given in our framework reproduce the exact behavior at high density and agree with the Monte-Carlo data in a wide range of densities. Our analytic technique enables us to get the correlation energies efficiently for various densities, which realizes the determination of EDF in the local density approximation (LDA) without any fitting for physically relevant densities. Applied to the Kohn-Sham calculation for the noble-gas atoms, our EDF shows comparable results to those of other conventional ones in LDA.
我们展示了一个$textit{ab initio}$结构的能量密度泛函(EDF)的电子系统使用功能重整化群。在我们的框架中给出的均相电子气体的相关能再现了高密度下的精确行为,并且在很宽的密度范围内与蒙特卡罗数据一致。我们的分析技术使我们能够有效地获得各种密度的相关能,从而实现了在局部密度近似(LDA)中确定EDF,而无需对物理相关密度进行拟合。应用于稀有气体原子的Kohn-Sham计算,我们的EDF显示出与LDA中其他常规EDF相当的结果。
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引用次数: 3
Generalized diagonalization scheme for many-particle systems 多粒子系统的广义对角化格式
Pub Date : 2020-10-14 DOI: 10.1103/PhysRevB.102.165122
S. Sykora, A. Hubsch, K. Becker
Despite the advances in the development of numerical methods analytical approaches still play the key role on the way towards a deeper understanding of many-particle systems. In this regards, diagonalization schemes for Hamiltonians represent an important direction in the field. Among these techniques the method, presented here, might be that approach with the widest range of possible applications: We demonstrate that both stepwise and continuous unitary transformations to diagonalize the many-particle Hamiltonian as well as perturbation theory and also non-perturbative treatments can be understood within the same theoretical framework. The new method is based on the introduction of generalized projection operators and allows to develop a renormalization scheme which is used to evaluate directly the physical quantities of a many-particle system. The applicability of this approach is shown for two important elementary many-particle problems.
尽管数值方法的发展取得了进步,但分析方法在深入理解多粒子系统的道路上仍然发挥着关键作用。在这方面,哈密顿量的对角化方案代表了该领域的一个重要方向。在这些技术中,这里提出的方法可能是具有最广泛应用范围的方法:我们证明了用于对角化多粒子哈密顿量的逐步和连续幺正变换以及微扰理论和非微扰处理都可以在相同的理论框架内理解。新方法基于广义投影算子的引入,并允许开发一种用于直接评估多粒子系统物理量的重整化方案。对两个重要的初等多粒子问题,证明了这种方法的适用性。
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引用次数: 4
Weakly coupled alternating S=12 chains in the distorted honeycomb lattice compound Na2Cu2TeO6 变形蜂窝晶格化合物Na2Cu2TeO6中弱耦合交替S=12链
Pub Date : 2020-10-14 DOI: 10.1103/physrevb.102.220402
S. Gao, Ling-Fang Lin, A. May, B. Rai, Qiang Zhang, E. Dagotto, A. Christianson, M. Stone
Spin-1/2 chains with alternating antiferromagnetic (AF) and ferromagnetic (FM) couplings exhibit quantum entanglement like the integer-spin Haldane chains and might be similarly utilized for quantum computations. Such alternating AF-FM chains have been proposed to be realized in the distorted honeycomb-lattice compound Na$_2$Cu$_2$TeO$_6$, but to confirm this picture a comprehensive understanding of the exchange interactions including terms outside of the idealized model is required. Here we employ neutron scattering to study the spin dynamics in Na$_2$Cu$_2$TeO$_6$ and accurately determine the coupling strengths through the random phase approximation and density functional theory (DFT) approaches. We find the AF and FM intrachain couplings are the dominant terms in the spin Hamiltonian, while the interchain couplings are AF but perturbative. This hierarchy in the coupling strengths and the alternating signs of the intrachain couplings can be understood through their different exchange paths. Our results establish Na$_2$Cu$_2$TeO$_6$ as a weakly-coupled alternating AF-FM chain compound and reveal the robustness of the gapped ground state in alternating chains under weak interchain couplings.
具有交替反铁磁(AF)和铁磁(FM)耦合的自旋-1/2链表现出像整数自旋霍尔丹链一样的量子纠缠,并且可能类似地用于量子计算。这种交替的AF-FM链已被提出在扭曲的蜂窝状晶格化合物Na$_2$Cu$_2$TeO$_6$中实现,但为了证实这一观点,需要对包括理想模型外的项在内的交换相互作用有全面的了解。本文采用中子散射方法研究了Na$_2$Cu$_2$TeO$_6$中的自旋动力学,并通过随机相位近似和密度泛函理论(DFT)方法精确地确定了耦合强度。我们发现自旋哈密顿量中AF和FM内耦合是主导项,而链间耦合是AF但微扰项。这种耦合强度的层次结构和链内耦合的交替符号可以通过它们不同的交换路径来理解。我们的结果证明Na$_2$Cu$_2$TeO$_6$是一个弱耦合的AF-FM交替链化合物,并揭示了在弱链间耦合下交替链中间隙基态的鲁棒性。
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引用次数: 5
Competing spin modulations in the magnetically frustrated semimetal EuCuSb 磁阻半金属EuCuSb中的竞争自旋调制
Pub Date : 2020-10-14 DOI: 10.1103/physrevb.102.174425
Hidefumi Takahashi, K. Aono, Y. Nambu, R. Kiyanagi, T. Nomoto, M. Sakano, K. Ishizaka, R. Arita, S. Ishiwata
The competing magnetic ground states of the itinerant magnet EuCuSb, which has a hexagonal layered structure, were studied via magnetization, resistivity, and neutron diffraction measurements on single-crystal samples. EuCuSb has a three-dimensional semimetallic band structure as confirmed by band calculation and angle-resolved photoelectron spectroscopy, consistent with the nearly isotropic metallic conductivity in the paramagnetic state. However, below the antiferromagnetic transition temperature of TN1 (8.5 K), the resistivity, especially along the hexagonal axis, increases significantly. This implies the emergence of anisotropic magnetic ordering coupled to the conducting electrons. Neutron diffraction measurements show that the Eu spins, which order ferromagnetically within each layer, are collinearly modulated (up-up-down-down) along the hexagonal axis below TN1, followed by the partial emergence of helical spin modulation below TN2 (6 K). Based on the observation of anomalous magnetoresistance with hysteretic behavior, we discuss the competing nature of the ground state inherent in a frustrated Heisenberg-like spin system with a centrosymmetric structure.
通过对单晶样品的磁化、电阻率和中子衍射测量,研究了具有六边形层状结构的流动磁体EuCuSb的竞争磁基态。通过能带计算和角分辨光电子能谱证实,EuCuSb具有三维半金属能带结构,与顺磁状态下近乎各向同性的金属电导率一致。而在反铁磁转变温度TN1 (8.5 K)以下,电阻率显著升高,特别是沿六方轴的电阻率显著升高。这意味着与导电电子耦合的各向异性磁有序的出现。中子衍射测量表明,Eu自旋在每一层内呈铁磁有序排列,在TN1以下沿六角形轴共线调制(上-上-下-下),随后在TN2 (6 K)以下部分出现螺旋自旋调制。基于对具有滞后行为的异常磁阻的观察,我们讨论了具有中心对称结构的受挫类海森堡自旋系统固有的基态竞争性质。
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引用次数: 5
Quantum operator growth bounds for kicked tops and semiclassical spin chains 踢顶和半经典自旋链的量子算子生长界
Pub Date : 2020-10-13 DOI: 10.1103/PhysRevA.103.042414
Chao Yin, A. Lucas
We present a framework for understanding the dynamics of operator size, and bounding the growth of out-of-time-ordered correlators, in models of large-$S$ spins. Focusing on the dynamics of a single spin, we show the finiteness of the Lyapunov exponent in the large-$S$ limit; our bounds are tighter than the best known Lieb-Robinson-type bounds on these systems. We numerically find our upper bound on Lyapunov exponents is within an order of magnitude of numerically computed values in classical and quantum kicked top models. Generalizing our results to coupled large-$S$ spins on lattices, we show that the butterfly velocity, which characterizes the spatial speed of quantum information scrambling, is finite as $Srightarrowinfty$. We emphasize qualitative differences between operator growth in semiclassical large-spin models, and quantum holographic systems including the Sachdev-Ye-Kitaev model.
我们提出了一个框架来理解算子大小的动力学,并在大- $S$自旋模型中限制非时序相关器的增长。关注于单自旋的动力学,我们证明了Lyapunov指数在大$S$极限下的有限性;我们的界比这些系统上最著名的利布-罗宾逊型界更紧。我们在数值上发现我们的李雅普诺夫指数的上界在经典和量子踢顶模型中数值计算值的一个数量级之内。将我们的结果推广到晶格上耦合的$S$大自旋,我们证明了表征量子信息置乱空间速度的蝴蝶速度是有限的$Srightarrowinfty$。我们强调了半经典大自旋模型和包括Sachdev-Ye-Kitaev模型在内的量子全息系统中算子增长的质的区别。
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引用次数: 17
期刊
arXiv: Strongly Correlated Electrons
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