Pub Date : 2020-09-27DOI: 10.1103/PhysRevB.103.224427
H. Robarts, M. García-Fernández, J. Li, A. Nag, A. Walters, N. E. Headings, S. Hayden, K. Zhou
Resonant inelastic X-ray scattering (RIXS) is a powerful probe of elementary excitations in solids. It is now widely applied to study magnetic excitations. However, its complex cross-section means that RIXS has been more difficult to interpret than inelastic neutron scattering (INS). Here we report high-resolution RIXS measurements of magnetic excitations of La2CuO4, the antiferromagnetic parent of one system of high-temperature superconductors. At high energies (~2 eV), the RIXS spectra show angular-dependent dd orbital excitations which are found to be in good agreement with single-site multiplet calculations. At lower energies (<0.3 eV), we show that the wavevector-dependent RIXS intensities are proportional to the product of the single-ion spin-flip cross section and the dynamical susceptibility of the spin-wave excitations. When the spin-flip crosssection is dividing out, the RIXS magnon intensities show a remarkable resemblance to INS data. Our results show that RIXS is a quantitative probe the dynamical spin susceptibility in cuprate and therefore should be used for quantitative investigation of other correlated electron materials.
{"title":"Dynamical spin susceptibility in \u0000La2CuO4\u0000 studied by resonant inelastic x-ray scattering","authors":"H. Robarts, M. García-Fernández, J. Li, A. Nag, A. Walters, N. E. Headings, S. Hayden, K. Zhou","doi":"10.1103/PhysRevB.103.224427","DOIUrl":"https://doi.org/10.1103/PhysRevB.103.224427","url":null,"abstract":"Resonant inelastic X-ray scattering (RIXS) is a powerful probe of elementary excitations in solids. It is now widely applied to study magnetic excitations. However, its complex cross-section means that RIXS has been more difficult to interpret than inelastic neutron scattering (INS). Here we report high-resolution RIXS measurements of magnetic excitations of La2CuO4, the antiferromagnetic parent of one system of high-temperature superconductors. At high energies (~2 eV), the RIXS spectra show angular-dependent dd orbital excitations which are found to be in good agreement with single-site multiplet calculations. At lower energies (<0.3 eV), we show that the wavevector-dependent RIXS intensities are proportional to the product of the single-ion spin-flip cross section and the dynamical susceptibility of the spin-wave excitations. When the spin-flip crosssection is dividing out, the RIXS magnon intensities show a remarkable resemblance to INS data. Our results show that RIXS is a quantitative probe the dynamical spin susceptibility in cuprate and therefore should be used for quantitative investigation of other correlated electron materials.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"22 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-09-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"87174169","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-24DOI: 10.1103/physrevb.102.235111
M. Kawano, C. Hotta
We examine the performance of the density matrix embedding theory (DMET) recently proposed in [G. Knizia and G. K.-L. Chan, Phys. Rev. Lett. 109, 186404 (2012)]. The core of this method is to find a proper one-body potential that generates a good trial wave function for projecting a large scale original Hamiltonian to a local subsystem with a small number of basis. The resultant ground state of the projected Hamiltonian can locally approximate the true ground state. However, the lack of the variational principle makes it difficult to judge the quality of the choice of the potential. Here we focus on the entanglement spectrum (ES) as a judging criterion; accurate evaluation of the ES guarantees that the corresponding reduced density matrix well reproduces all physical quantities on the local subsystem. We apply the DMET to the Hubbard model on the one-dimensional chain, zigzag chain, and triangular lattice and test several variants of potentials and cost functions. It turns out that a symmetric potential reproduces the ES of the phase that continues from a noninteracting limit. The Mott transition as well as symmetry-breaking transitions can be detected by the singularities in the ES. However, the details of the ES in the strongly interacting parameter region depends much on these choices, meaning that the present algorithm allowing for numerous variants of the DMET is insufficient to fully fix the quantum many-body problem.
{"title":"Comparative study of the density matrix embedding theory for Hubbard models","authors":"M. Kawano, C. Hotta","doi":"10.1103/physrevb.102.235111","DOIUrl":"https://doi.org/10.1103/physrevb.102.235111","url":null,"abstract":"We examine the performance of the density matrix embedding theory (DMET) recently proposed in [G. Knizia and G. K.-L. Chan, Phys. Rev. Lett. 109, 186404 (2012)]. The core of this method is to find a proper one-body potential that generates a good trial wave function for projecting a large scale original Hamiltonian to a local subsystem with a small number of basis. The resultant ground state of the projected Hamiltonian can locally approximate the true ground state. However, the lack of the variational principle makes it difficult to judge the quality of the choice of the potential. Here we focus on the entanglement spectrum (ES) as a judging criterion; accurate evaluation of the ES guarantees that the corresponding reduced density matrix well reproduces all physical quantities on the local subsystem. We apply the DMET to the Hubbard model on the one-dimensional chain, zigzag chain, and triangular lattice and test several variants of potentials and cost functions. It turns out that a symmetric potential reproduces the ES of the phase that continues from a noninteracting limit. The Mott transition as well as symmetry-breaking transitions can be detected by the singularities in the ES. However, the details of the ES in the strongly interacting parameter region depends much on these choices, meaning that the present algorithm allowing for numerous variants of the DMET is insufficient to fully fix the quantum many-body problem.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"32 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-09-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"73859803","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-22DOI: 10.1103/PHYSREVB.103.155107
Minjae Kim, H. Miao, Sang-Jun Choi, M. Zingl, A. Georges, G. Kotliar
We address the question of the degree of spatial non-locality of the self energy in the iron-based superconductors, a subject which is receiving considerable attention. Using LiFeAs as a prototypical example, we extract the self energy from angular-resolved photoemission spectroscopy (ARPES) data. We use two distinct electronic structure references: density functional theory in the local density approximation and linearized quasiparticle self consistent GW (LQSGW). We find that in the LQSGW reference, spatially local dynamical correlations provide a consistent description of the experimental data, and account for some surprising aspects of the data such as the substantial out of plane dispersion of the electron Fermi surface having dominant xz/yz character. Hall effect and resistivity data are shown to be consistent with the proposed description.
{"title":"Spatial locality of electronic correlations in LiFeAs","authors":"Minjae Kim, H. Miao, Sang-Jun Choi, M. Zingl, A. Georges, G. Kotliar","doi":"10.1103/PHYSREVB.103.155107","DOIUrl":"https://doi.org/10.1103/PHYSREVB.103.155107","url":null,"abstract":"We address the question of the degree of spatial non-locality of the self energy in the iron-based superconductors, a subject which is receiving considerable attention. Using LiFeAs as a prototypical example, we extract the self energy from angular-resolved photoemission spectroscopy (ARPES) data. We use two distinct electronic structure references: density functional theory in the local density approximation and linearized quasiparticle self consistent GW (LQSGW). We find that in the LQSGW reference, spatially local dynamical correlations provide a consistent description of the experimental data, and account for some surprising aspects of the data such as the substantial out of plane dispersion of the electron Fermi surface having dominant xz/yz character. Hall effect and resistivity data are shown to be consistent with the proposed description.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"62 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-09-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"90336451","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-22DOI: 10.1103/PhysRevResearch.2.033462
Aifeng Wang, S. Baranets, Yu Liu, X. Tong, E. Stavitski, Jing Zhang, Y. Chai, W. Yin, S. Bobev, C. Petrovic
We report discovery of new antiferromagnetic semimetal EuZnSb$_2$, obtained and studied in the form of single crystals. Electric resistivity, magnetic susceptibility and heat capacity indicate antiferromagnetic order of Eu with $T_N$ = 20 K. The effective moment of Eu$^{2+}$ inferred from the magnetization and specific heat measurement is 3.5 $mu_B$, smaller than the theoretical value of Eu$^{2+}$ due to presence of both Eu$^{3+}$ and Eu$^{2+}$. Magnetic field-dependent resistivity measurements suggest dominant quasi two dimensional Fermi surfaces whereas the first-principle calculations point to the presence of Dirac fermions. Therefore, EuZnSb$_2$ could represent the first platform to study the interplay of dynamical charge fluctuations, localized magnetic 4$f$ moments and Dirac states with Sb orbital character.
{"title":"Magnetic mixed valent semimetal \u0000EuZnSb2\u0000 with Dirac states in the band structure","authors":"Aifeng Wang, S. Baranets, Yu Liu, X. Tong, E. Stavitski, Jing Zhang, Y. Chai, W. Yin, S. Bobev, C. Petrovic","doi":"10.1103/PhysRevResearch.2.033462","DOIUrl":"https://doi.org/10.1103/PhysRevResearch.2.033462","url":null,"abstract":"We report discovery of new antiferromagnetic semimetal EuZnSb$_2$, obtained and studied in the form of single crystals. Electric resistivity, magnetic susceptibility and heat capacity indicate antiferromagnetic order of Eu with $T_N$ = 20 K. The effective moment of Eu$^{2+}$ inferred from the magnetization and specific heat measurement is 3.5 $mu_B$, smaller than the theoretical value of Eu$^{2+}$ due to presence of both Eu$^{3+}$ and Eu$^{2+}$. Magnetic field-dependent resistivity measurements suggest dominant quasi two dimensional Fermi surfaces whereas the first-principle calculations point to the presence of Dirac fermions. Therefore, EuZnSb$_2$ could represent the first platform to study the interplay of dynamical charge fluctuations, localized magnetic 4$f$ moments and Dirac states with Sb orbital character.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"112 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-09-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"87900155","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-21DOI: 10.1103/PhysRevX.11.021040
A. Lerose, M. Sonner, D. Abanin
In this work, we introduce an approach to study quantum many-body dynamics, inspired by the Feynman-Vernon influence functional. Focusing on a family of interacting, Floquet spin chains, we consider a Keldysh path-integral description of the dynamics. The central object in our approach is the influence matrix (IM), which describes the effect of the system on the dynamics of a local subsystem. For translationally invariant models, we formulate a self-consistency equation for the influence matrix. For certain special values of the model parameters, we obtain an exact solution which represents a perfect dephaser (PD). Physically, a PD corresponds to a many-body system that acts as a perfectly Markovian bath on itself: at each period, it measures every spin. For the models considered here, we establish that PD points include dual-unitary circuits investigated in recent works. In the vicinity of PD points, the system is not perfectly Markovian, but rather acts as a bath with a short memory time. In this case, we demonstrate that the self-consistency equation can be solved using matrix-product states (MPS) methods, as the IM temporal entanglement is low. A combination of analytical insights and MPS computations allows us to characterize the structure of the influence matrix in terms of an effective "statistical-mechanics" description. We finally illustrate the predictive power of this description by analytically computing how quickly an embedded impurity spin thermalizes. The influence matrix approach formulated here provides an intuitive view of the quantum many-body dynamics problem, opening a path to constructing models of thermalizing dynamics that are solvable or can be efficiently treated by MPS-based methods, and to further characterizing quantum ergodicity or lack thereof.
{"title":"Influence Matrix Approach to Many-Body Floquet Dynamics","authors":"A. Lerose, M. Sonner, D. Abanin","doi":"10.1103/PhysRevX.11.021040","DOIUrl":"https://doi.org/10.1103/PhysRevX.11.021040","url":null,"abstract":"In this work, we introduce an approach to study quantum many-body dynamics, inspired by the Feynman-Vernon influence functional. Focusing on a family of interacting, Floquet spin chains, we consider a Keldysh path-integral description of the dynamics. The central object in our approach is the influence matrix (IM), which describes the effect of the system on the dynamics of a local subsystem. For translationally invariant models, we formulate a self-consistency equation for the influence matrix. For certain special values of the model parameters, we obtain an exact solution which represents a perfect dephaser (PD). Physically, a PD corresponds to a many-body system that acts as a perfectly Markovian bath on itself: at each period, it measures every spin. For the models considered here, we establish that PD points include dual-unitary circuits investigated in recent works. In the vicinity of PD points, the system is not perfectly Markovian, but rather acts as a bath with a short memory time. In this case, we demonstrate that the self-consistency equation can be solved using matrix-product states (MPS) methods, as the IM temporal entanglement is low. A combination of analytical insights and MPS computations allows us to characterize the structure of the influence matrix in terms of an effective \"statistical-mechanics\" description. We finally illustrate the predictive power of this description by analytically computing how quickly an embedded impurity spin thermalizes. The influence matrix approach formulated here provides an intuitive view of the quantum many-body dynamics problem, opening a path to constructing models of thermalizing dynamics that are solvable or can be efficiently treated by MPS-based methods, and to further characterizing quantum ergodicity or lack thereof.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"27 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-09-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"89895644","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-21DOI: 10.1103/PHYSREVB.102.125135
Monalisa Singh Roy, Manoranjan Kumar, J. Sau, S. Tewari
We examine the properties of a one-dimensional (1D) Fermi gas with attractive intrinsic (Hubbard) interactions in the presence of spin-orbit coupling and Zeeman field by numerically computing the pair binding energy, excitation gap, and susceptibility to local perturbations using the density matrix renormalization group. Such a system can, in principle, be realized in a system of ultracold atoms confined in a 1D optical lattice. We note that, in the presence of spatial interfaces introduced by a smooth parabolic potential, the pair binding and excitation energy of the system decays exponentially with the system size, pointing to the existence of an exponential ground state degeneracy, and is consistent with recent works. However, the susceptibility of the ground state degeneracy of this number-conserving system to local impurities indicates that the energy gap vanishes as a power law with the system size in the presence of local perturbations. We compare this system with the more familiar system of an Ising antiferromagnet in the presence of a transverse field realized with Rydberg atoms and argue that the exponential splitting in the clean number-conserving 1D Fermi system is similar to a phase with only conventional order.
{"title":"Fermion parity gap and exponential ground state degeneracy of the one-dimensional Fermi gas with intrinsic attractive interaction","authors":"Monalisa Singh Roy, Manoranjan Kumar, J. Sau, S. Tewari","doi":"10.1103/PHYSREVB.102.125135","DOIUrl":"https://doi.org/10.1103/PHYSREVB.102.125135","url":null,"abstract":"We examine the properties of a one-dimensional (1D) Fermi gas with attractive intrinsic (Hubbard) interactions in the presence of spin-orbit coupling and Zeeman field by numerically computing the pair binding energy, excitation gap, and susceptibility to local perturbations using the density matrix renormalization group. Such a system can, in principle, be realized in a system of ultracold atoms confined in a 1D optical lattice. We note that, in the presence of spatial interfaces introduced by a smooth parabolic potential, the pair binding and excitation energy of the system decays exponentially with the system size, pointing to the existence of an exponential ground state degeneracy, and is consistent with recent works. However, the susceptibility of the ground state degeneracy of this number-conserving system to local impurities indicates that the energy gap vanishes as a power law with the system size in the presence of local perturbations. We compare this system with the more familiar system of an Ising antiferromagnet in the presence of a transverse field realized with Rydberg atoms and argue that the exponential splitting in the clean number-conserving 1D Fermi system is similar to a phase with only conventional order.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"77 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-09-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"82398980","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-21DOI: 10.1103/PhysRevB.103.155128
Xiao-Li Huang, A. Lucas
We develop the theory of hydrodynamics of an isotropic Fermi liquid of electrons coupled to isotropic acoustic phonons, assuming that umklapp processes may be neglected. At low temperatures, the fluid is approximately Galilean invariant; at high temperatures, the fluid is nearly relativistic; at intermediate temperatures, there are seven additional temperature regimes with unconventional thermodynamic properties and hydrodynamic transport coefficients in a three-dimensional system. We predict qualitative signatures of electron-phonon fluids in incoherent transport coefficients, shear and Hall viscosity, and plasmon dispersion relations. Our theory may be relevant for numerous quantum materials where strong electron-phonon scattering has been proposed to underlie a hydrodynamic regime, including $mathrm{WTe}_2$, $mathrm{WP}_2$, and $mathrm{PtSn}_4$.
{"title":"Electron-phonon hydrodynamics","authors":"Xiao-Li Huang, A. Lucas","doi":"10.1103/PhysRevB.103.155128","DOIUrl":"https://doi.org/10.1103/PhysRevB.103.155128","url":null,"abstract":"We develop the theory of hydrodynamics of an isotropic Fermi liquid of electrons coupled to isotropic acoustic phonons, assuming that umklapp processes may be neglected. At low temperatures, the fluid is approximately Galilean invariant; at high temperatures, the fluid is nearly relativistic; at intermediate temperatures, there are seven additional temperature regimes with unconventional thermodynamic properties and hydrodynamic transport coefficients in a three-dimensional system. We predict qualitative signatures of electron-phonon fluids in incoherent transport coefficients, shear and Hall viscosity, and plasmon dispersion relations. Our theory may be relevant for numerous quantum materials where strong electron-phonon scattering has been proposed to underlie a hydrodynamic regime, including $mathrm{WTe}_2$, $mathrm{WP}_2$, and $mathrm{PtSn}_4$.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"23 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-09-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"87849702","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-20DOI: 10.1103/PhysRevA.103.012204
R. Jafari, A. Akbari
We explore both pure and mixed states Floquet dynamical quantum phase transitions (FDQFTs) in the one-dimensional p-wave superconductor with a time-driven pairing phase. In the Fourier space, the model is recast to the non-interacting quasi-spins subjected to a time-dependent effective magnetic field. We show that FDQFTs occur within a range of driving frequency without resorting to any quenches. Moreover, FDQFTs appear in the region where quasi-spins are in the resonance regime. In the resonance regime, the population completely cycles the population between the spin down and up states. Additionally, we study the conditions for the appearance of FDQFTs using the entanglement spectrum and purity entanglement measure. Our results imply that the entanglement spectrum can truly capture the resonance regime where FDQFTs occur. Particularly, the dynamical topological region results in the degeneracy of the entanglement spectrum. It is shown that the boundary of the driven frequency range, over which the system reveals FDQFTs, signaled by the purity entanglement measure.
{"title":"Floquet dynamical phase transition and entanglement spectrum","authors":"R. Jafari, A. Akbari","doi":"10.1103/PhysRevA.103.012204","DOIUrl":"https://doi.org/10.1103/PhysRevA.103.012204","url":null,"abstract":"We explore both pure and mixed states Floquet dynamical quantum phase transitions (FDQFTs) in the one-dimensional p-wave superconductor with a time-driven pairing phase. In the Fourier space, the model is recast to the non-interacting quasi-spins subjected to a time-dependent effective magnetic field. We show that FDQFTs occur within a range of driving frequency without resorting to any quenches. Moreover, FDQFTs appear in the region where quasi-spins are in the resonance regime. In the resonance regime, the population completely cycles the population between the spin down and up states. Additionally, we study the conditions for the appearance of FDQFTs using the entanglement spectrum and purity entanglement measure. Our results imply that the entanglement spectrum can truly capture the resonance regime where FDQFTs occur. Particularly, the dynamical topological region results in the degeneracy of the entanglement spectrum. It is shown that the boundary of the driven frequency range, over which the system reveals FDQFTs, signaled by the purity entanglement measure.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"39 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-09-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"89172285","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-18DOI: 10.1103/PhysRevB.104.115105
N. Phuc, P. Q. Trung
Interactions between particles in quantum many-body systems play a crucial role in determining the electric, magnetic, optical, and thermal properties of the system. The recent progress in the laser-pulse technique has enabled the manipulations and measurements of physical properties on ultrafast timescales. Here, we propose a method for the direct and ultrafast probing of quantum many-body interaction through coherent two-dimensional (2D) spectroscopy. Up to a moderate interaction strength, the inter-particle interaction manifests itself in the emergence of off-diagonal peaks in the 2D spectrum before all the peaks coalesce into a single diagonal peak as the system approaches the Mott-insulating phase in the strongly interacting regime. The evolution of the 2D spectrum as a function of the time delay between the second and third laser pulses can provide important information on the ultrafast time variation of the interaction.
{"title":"Direct and ultrafast probing of quantum many-body interaction and Mott-insulator transition through coherent two-dimensional spectroscopy","authors":"N. Phuc, P. Q. Trung","doi":"10.1103/PhysRevB.104.115105","DOIUrl":"https://doi.org/10.1103/PhysRevB.104.115105","url":null,"abstract":"Interactions between particles in quantum many-body systems play a crucial role in determining the electric, magnetic, optical, and thermal properties of the system. The recent progress in the laser-pulse technique has enabled the manipulations and measurements of physical properties on ultrafast timescales. Here, we propose a method for the direct and ultrafast probing of quantum many-body interaction through coherent two-dimensional (2D) spectroscopy. Up to a moderate interaction strength, the inter-particle interaction manifests itself in the emergence of off-diagonal peaks in the 2D spectrum before all the peaks coalesce into a single diagonal peak as the system approaches the Mott-insulating phase in the strongly interacting regime. The evolution of the 2D spectrum as a function of the time delay between the second and third laser pulses can provide important information on the ultrafast time variation of the interaction.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"73 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"76844856","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-18DOI: 10.1103/PhysRevB.102.094422
V. Favre, G. Tucker, C. Ritter, R. Sibille, P. Manuel, M. Frontzek, M. Kriener, Lin Yang, H. Berger, A. Magrez, N. Casati, I. Živković, H. Rønnow
We report magnetic properties of a 3d$^9$ (Cu$^{2+}$) magnetic insulator Cu2OSO4 measured on both powder and single crystal. The magnetic atoms of this compound form layers, whose geometry can be described either as a system of chains coupled through dimers or as a Kagom'e lattice where every 3rd spin is replaced by a dimer. Specific heat and DC-susceptibility show a magnetic transition at 20 K, which is also confirmed by neutron scattering. Magnetic entropy extracted from the specific heat data is consistent with a $S=1/2$ degree of freedom per Cu$^{2+}$, and so is the effective moment extracted from DC-susceptibility. The ground state has been identified by means of neutron diffraction on both powder and single crystal and corresponds to a $sim120$ degree spin structure in which ferromagnetic intra-dimer alignment results in a net ferrimagnetic moment. No evidence is found for a change in lattice symmetry down to 2 K. Our results suggest that sample represents a new type of model lattice with frustrated interactions where interplay between magnetic order, thermal and quantum fluctuations can be explored.
{"title":"Ferrimagnetic 120∘magnetic structure inCu2OSO4","authors":"V. Favre, G. Tucker, C. Ritter, R. Sibille, P. Manuel, M. Frontzek, M. Kriener, Lin Yang, H. Berger, A. Magrez, N. Casati, I. Živković, H. Rønnow","doi":"10.1103/PhysRevB.102.094422","DOIUrl":"https://doi.org/10.1103/PhysRevB.102.094422","url":null,"abstract":"We report magnetic properties of a 3d$^9$ (Cu$^{2+}$) magnetic insulator Cu2OSO4 measured on both powder and single crystal. The magnetic atoms of this compound form layers, whose geometry can be described either as a system of chains coupled through dimers or as a Kagom'e lattice where every 3rd spin is replaced by a dimer. Specific heat and DC-susceptibility show a magnetic transition at 20 K, which is also confirmed by neutron scattering. Magnetic entropy extracted from the specific heat data is consistent with a $S=1/2$ degree of freedom per Cu$^{2+}$, and so is the effective moment extracted from DC-susceptibility. The ground state has been identified by means of neutron diffraction on both powder and single crystal and corresponds to a $sim120$ degree spin structure in which ferromagnetic intra-dimer alignment results in a net ferrimagnetic moment. No evidence is found for a change in lattice symmetry down to 2 K. Our results suggest that sample represents a new type of model lattice with frustrated interactions where interplay between magnetic order, thermal and quantum fluctuations can be explored.","PeriodicalId":8511,"journal":{"name":"arXiv: Strongly Correlated Electrons","volume":"37 Suppl 7 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2020-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"78337548","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
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