Pub Date : 2020-09-10DOI: 10.1103/PhysRevB.102.104513
D. Daghero, E. Piatti, Nikolai Zhigadlo, G. Ummarino, N. Barbero, T. Shiroka
Underdoped PrFeAs(O,F), one of the less known members of the 1111 family of iron-based superconductors, was investigated in detail by means of transport, SQUID magnetometry, nuclear magnetic resonance (NMR) measurements and point-contact Andreev-reflection spectroscopy (PCARS). PCARS measurements on single crystals evidence the multigap nature of PrFeAs(O,F) superconductivity, shown to host at least two isotropic gaps, clearly discernible in the spectra, irrespective of the direction of current injection (i.e., along the ab planes or along the c axis). Additional features at higher energy can be interpreted as signatures of a strong electron-boson coupling, as demonstrated by a model which combines Andreev reflection with the Eliashberg theory. Magnetic resonance measurements in the normal phase indicate the lack of a magnetic order in underdoped PrFeAs(O,F), while $^{75}$As NMR spin-lattice relaxation results suggest the presence of significant electronic spin fluctuations, peaking above $T_{c}$ and expected to mediate the superconducting pairing.
{"title":"Superconductivity of underdoped PrFeAs(O,F) investigated via point-contact spectroscopy and nuclear magnetic resonance","authors":"D. Daghero, E. Piatti, Nikolai Zhigadlo, G. Ummarino, N. Barbero, T. Shiroka","doi":"10.1103/PhysRevB.102.104513","DOIUrl":"https://doi.org/10.1103/PhysRevB.102.104513","url":null,"abstract":"Underdoped PrFeAs(O,F), one of the less known members of the 1111 family of iron-based superconductors, was investigated in detail by means of transport, SQUID magnetometry, nuclear magnetic resonance (NMR) measurements and point-contact Andreev-reflection spectroscopy (PCARS). PCARS measurements on single crystals evidence the multigap nature of PrFeAs(O,F) superconductivity, shown to host at least two isotropic gaps, clearly discernible in the spectra, irrespective of the direction of current injection (i.e., along the ab planes or along the c axis). Additional features at higher energy can be interpreted as signatures of a strong electron-boson coupling, as demonstrated by a model which combines Andreev reflection with the Eliashberg theory. Magnetic resonance measurements in the normal phase indicate the lack of a magnetic order in underdoped PrFeAs(O,F), while $^{75}$As NMR spin-lattice relaxation results suggest the presence of significant electronic spin fluctuations, peaking above $T_{c}$ and expected to mediate the superconducting pairing.","PeriodicalId":8514,"journal":{"name":"arXiv: Superconductivity","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-09-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77393401","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-08DOI: 10.1103/physrevb.102.195149
D. Betto, M. Bluschke, D. Putzky, E. Schierle, A. Amorese, K. Fursich, S. Blanco-Canosa, G. Christiani, G. Logvenov, B. Keimer, M. Minola
We used resonant elastic x-ray scattering at the Cu $L_3$ and Dy $M_5$ edges to investigate charge order in thin films of underdoped DyBa$_2$Cu$_3$O$_{6+x}$ (DyBCO) epitaxially grown on NdGaO$_3$ (110) substrates. The films show an orthorhombic crystal structure with short-range ortho-II oxygen order in the charge-reservoir layers. At the Dy $M_5$ edge we observe diffraction peaks with the same planar wavevectors as those of the two-dimensional charge density wave in the CuO$_2$ planes and of the ortho-II oxygen order, indicating the formation of induced ordered states on the rare-earth sublattice. The intensity of the resonant diffraction peaks exhibits a non-monotonic dependence on an external magnetic field. Model calculations on the modulation of the crystalline electric field at the Dy sites by charge and oxygen order capture the salient features of the magnetic field, temperature, and photon energy dependence of the scattering intensity.
{"title":"Imprint of charge and oxygen orders on Dy ions in \u0000DyBa2Cu3O6+x\u0000 thin films probed by resonant x-ray scattering","authors":"D. Betto, M. Bluschke, D. Putzky, E. Schierle, A. Amorese, K. Fursich, S. Blanco-Canosa, G. Christiani, G. Logvenov, B. Keimer, M. Minola","doi":"10.1103/physrevb.102.195149","DOIUrl":"https://doi.org/10.1103/physrevb.102.195149","url":null,"abstract":"We used resonant elastic x-ray scattering at the Cu $L_3$ and Dy $M_5$ edges to investigate charge order in thin films of underdoped DyBa$_2$Cu$_3$O$_{6+x}$ (DyBCO) epitaxially grown on NdGaO$_3$ (110) substrates. The films show an orthorhombic crystal structure with short-range ortho-II oxygen order in the charge-reservoir layers. At the Dy $M_5$ edge we observe diffraction peaks with the same planar wavevectors as those of the two-dimensional charge density wave in the CuO$_2$ planes and of the ortho-II oxygen order, indicating the formation of induced ordered states on the rare-earth sublattice. The intensity of the resonant diffraction peaks exhibits a non-monotonic dependence on an external magnetic field. Model calculations on the modulation of the crystalline electric field at the Dy sites by charge and oxygen order capture the salient features of the magnetic field, temperature, and photon energy dependence of the scattering intensity.","PeriodicalId":8514,"journal":{"name":"arXiv: Superconductivity","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-09-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"74523690","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-07DOI: 10.1103/PHYSREVRESEARCH.3.013162
Saheli Sarkar, M. Grandadam, C. P'epin
A softening of phonon-dispersion has been observed experimentally in under-doped cuprate superconductors at the charge-density wave (CDW) ordering wave vector. Interestingly, the softening occurs below the superconducting (SC) transition temperature T$_{c}$, in contrast to the metallic systems, where the softening occurs usually below the CDW onset temperature T$_{text{CDW}}$. An understanding of the `anomalous' nature of the phonon-softening and its connection to the pseudo-gap phase in under-doped cuprates remain open questions. Within a perturbative approach, we show that a complex interplay among the ubiquitous CDW, SC orders and life-time of quasi-particles associated to thermal fluctuations, can explain the anomalous phonon-softening below T$_{c}$. Furthermore, our formalism captures different characteristics of the low temperature phonon-softening depending on material specificity.
{"title":"Anomalous softening of phonon dispersion in cuprate superconductors","authors":"Saheli Sarkar, M. Grandadam, C. P'epin","doi":"10.1103/PHYSREVRESEARCH.3.013162","DOIUrl":"https://doi.org/10.1103/PHYSREVRESEARCH.3.013162","url":null,"abstract":"A softening of phonon-dispersion has been observed experimentally in under-doped cuprate superconductors at the charge-density wave (CDW) ordering wave vector. Interestingly, the softening occurs below the superconducting (SC) transition temperature T$_{c}$, in contrast to the metallic systems, where the softening occurs usually below the CDW onset temperature T$_{text{CDW}}$. An understanding of the `anomalous' nature of the phonon-softening and its connection to the pseudo-gap phase in under-doped cuprates remain open questions. Within a perturbative approach, we show that a complex interplay among the ubiquitous CDW, SC orders and life-time of quasi-particles associated to thermal fluctuations, can explain the anomalous phonon-softening below T$_{c}$. Furthermore, our formalism captures different characteristics of the low temperature phonon-softening depending on material specificity.","PeriodicalId":8514,"journal":{"name":"arXiv: Superconductivity","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-09-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"76730423","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-04DOI: 10.1103/PhysRevResearch.3.033192
Dorota I. Walicka, Z. Guguchia, J. Lago, O. Blacque, K. Ma, R. Khasanov, F. O. Rohr
It is a well-established fact that the physical properties of compounds follow their crystal symmetries. This has especially pronounced implications on emergent collective quantum states in materials. Specifically, the effect of crystal symmetries on the properties of superconductors is widely appreciated, although the clarification of this relationship is a core effort of on-going research. Emergent phenomena on honeycomb lattices are of special interest, as they can give rise to spectacular phenomenology, as manifested by the recent discovery of correlated states in magic-angle graphene, or by the high-temperature superconductivity in MgB$_2$. Here, we report on the structural and microscopic superconducting properties of a class of ternary superconductors with Al/Si honeycomb layers, i.e. Ca$_{1-x}$Sr$_{x}$AlSi. We show that this solid solution is a remarkable model system with a highly tunable two-gap to single-gap superconducting system on a honeycomb lattice, where the superconductivity is enhanced by a subtle structural instability, i.e. the buckling of the Al/Si layers.
{"title":"Two-gap to Single-gap Superconducting Transition on a Honeycomb Lattice in Ca$_{1-x}$Sr$_{x}$AlSi","authors":"Dorota I. Walicka, Z. Guguchia, J. Lago, O. Blacque, K. Ma, R. Khasanov, F. O. Rohr","doi":"10.1103/PhysRevResearch.3.033192","DOIUrl":"https://doi.org/10.1103/PhysRevResearch.3.033192","url":null,"abstract":"It is a well-established fact that the physical properties of compounds follow their crystal symmetries. This has especially pronounced implications on emergent collective quantum states in materials. Specifically, the effect of crystal symmetries on the properties of superconductors is widely appreciated, although the clarification of this relationship is a core effort of on-going research. Emergent phenomena on honeycomb lattices are of special interest, as they can give rise to spectacular phenomenology, as manifested by the recent discovery of correlated states in magic-angle graphene, or by the high-temperature superconductivity in MgB$_2$. Here, we report on the structural and microscopic superconducting properties of a class of ternary superconductors with Al/Si honeycomb layers, i.e. Ca$_{1-x}$Sr$_{x}$AlSi. We show that this solid solution is a remarkable model system with a highly tunable two-gap to single-gap superconducting system on a honeycomb lattice, where the superconductivity is enhanced by a subtle structural instability, i.e. the buckling of the Al/Si layers.","PeriodicalId":8514,"journal":{"name":"arXiv: Superconductivity","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-09-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"84183736","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-02DOI: 10.1103/PHYSREVB.103.064512
Bo Li, Zhongbo Yan
For strongly anisotropic time-reversal invariant (TRI) insulators in two and three dimensions, the band inversion can occur respectively at all TRI momenta of a high symmetry axis and plane. Although these classes of materials are topologically trivial as the strong and weak $Z_{2}$ indices are all trivial, they can host an even number of unprotected helical gapless edge states or surface Dirac cones on some boundaries. We show in this work that when the gapless boundary states are gapped by $s_{pm}$-wave superconductivity, a boundary time-reversal invariant topological superconductor (BTRITSC) characterized by a $Z_{2}$ invariant can be realized on the corresponding boundary. Since the dimension of the BTRITSC is lower than the bulk by one, the whole system is a second-order TRI topological superconductor. When the boundary of the BTRITSC is further cut open, Majorana Kramers pairs and helical gapless Majorana modes will respectively appear at the corners and hinges of the considered sample in two and three dimensions. Furthermore, a magnetic field can gap the helical Majorana hinge modes of the three-dimensional second-order TRI topological superconductor and lead to the realization of a third-order topological superconductor with Majorana corner modes. Our proposal can potentially be realized in insulator-superconductor heterostructures and iron-based superconductors whose normal states take the desired inverted band structures.
{"title":"Boundary topological superconductors","authors":"Bo Li, Zhongbo Yan","doi":"10.1103/PHYSREVB.103.064512","DOIUrl":"https://doi.org/10.1103/PHYSREVB.103.064512","url":null,"abstract":"For strongly anisotropic time-reversal invariant (TRI) insulators in two and three dimensions, the band inversion can occur respectively at all TRI momenta of a high symmetry axis and plane. Although these classes of materials are topologically trivial as the strong and weak $Z_{2}$ indices are all trivial, they can host an even number of unprotected helical gapless edge states or surface Dirac cones on some boundaries. We show in this work that when the gapless boundary states are gapped by $s_{pm}$-wave superconductivity, a boundary time-reversal invariant topological superconductor (BTRITSC) characterized by a $Z_{2}$ invariant can be realized on the corresponding boundary. Since the dimension of the BTRITSC is lower than the bulk by one, the whole system is a second-order TRI topological superconductor. When the boundary of the BTRITSC is further cut open, Majorana Kramers pairs and helical gapless Majorana modes will respectively appear at the corners and hinges of the considered sample in two and three dimensions. Furthermore, a magnetic field can gap the helical Majorana hinge modes of the three-dimensional second-order TRI topological superconductor and lead to the realization of a third-order topological superconductor with Majorana corner modes. Our proposal can potentially be realized in insulator-superconductor heterostructures and iron-based superconductors whose normal states take the desired inverted band structures.","PeriodicalId":8514,"journal":{"name":"arXiv: Superconductivity","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"89511556","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-09-02DOI: 10.1103/physrevresearch.2.033356
K. Yamazaki, M. Ochi, D. Ogura, K. Kuroki, H. Eisaki, S. Uchida, H. Aoki
The authors introduce a multiorbital model with a Lieb-lattice structure to show that the disrupted CuO network in Ba${}_{2}$CuO${}_{3+ensuremath{delta}}$ can accommodate new pairing mechanisms
{"title":"Superconducting mechanism for the cuprate \u0000Ba2CuO3+δ\u0000 based on a multiorbital Lieb lattice model","authors":"K. Yamazaki, M. Ochi, D. Ogura, K. Kuroki, H. Eisaki, S. Uchida, H. Aoki","doi":"10.1103/physrevresearch.2.033356","DOIUrl":"https://doi.org/10.1103/physrevresearch.2.033356","url":null,"abstract":"The authors introduce a multiorbital model with a Lieb-lattice structure to show that the disrupted CuO network in Ba${}_{2}$CuO${}_{3+ensuremath{delta}}$ can accommodate new pairing mechanisms","PeriodicalId":8514,"journal":{"name":"arXiv: Superconductivity","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-09-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"82678264","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-08-31DOI: 10.1103/physrevb.102.180509
Jia-Long Zhang, Yu Li, Wen Huang, Fu-Chun Zhang
The polar Kerr effect in superconducting Sr$_2$RuO$_4$ implies finite ac anomalous Hall conductivity. Since intrinsic anomalous Hall effect (AHE) is not expected for a chiral superconducting pairing developed on the single Ru $d_{xy}$ orbital, multiorbital chiral pairing actively involving the Ru $d_{xz}$ and $d_{yz}$ orbitals has been proposed as a potential mechanism. Here we propose that AHE could still arise even if the chiral superconductivity is predominantly driven by the $d_{xy}$ orbital. This is demonstrated through two separate models which take into account subdominant orbitals in the Cooper pairing, one involving the oxygen $p_x$ and $p_y$ orbitals in the RuO$_2$ plane, and another the $d_{xz}$ and $d_{yz}$ orbitals. In both models, finite orbital mixing between the dominant $d_{xy}$ and the other orbitals may induce inter-orbital pairing between them, and the resultant states support intrinsic AHE, with Kerr rotation angles that could potentially reconcile with the experimental observation. Our proposal therefore sheds new light on the microscopic pairing in Sr$_2$RuO$_4$. We also show that intrinsic Hall effect is generally absent for non-chiral states such as $mathcal{S}+imathcal{D}$, $mathcal{D}+imathcal{P}$ and $mathcal{D}+imathcal{G}$, which provides a clear constraint on the symmetry of the superconducting order in this material.
{"title":"Hidden anomalous Hall effect in \u0000Sr2RuO4\u0000 with chiral superconductivity dominated by the Ru \u0000dxy\u0000 orbital","authors":"Jia-Long Zhang, Yu Li, Wen Huang, Fu-Chun Zhang","doi":"10.1103/physrevb.102.180509","DOIUrl":"https://doi.org/10.1103/physrevb.102.180509","url":null,"abstract":"The polar Kerr effect in superconducting Sr$_2$RuO$_4$ implies finite ac anomalous Hall conductivity. Since intrinsic anomalous Hall effect (AHE) is not expected for a chiral superconducting pairing developed on the single Ru $d_{xy}$ orbital, multiorbital chiral pairing actively involving the Ru $d_{xz}$ and $d_{yz}$ orbitals has been proposed as a potential mechanism. Here we propose that AHE could still arise even if the chiral superconductivity is predominantly driven by the $d_{xy}$ orbital. This is demonstrated through two separate models which take into account subdominant orbitals in the Cooper pairing, one involving the oxygen $p_x$ and $p_y$ orbitals in the RuO$_2$ plane, and another the $d_{xz}$ and $d_{yz}$ orbitals. In both models, finite orbital mixing between the dominant $d_{xy}$ and the other orbitals may induce inter-orbital pairing between them, and the resultant states support intrinsic AHE, with Kerr rotation angles that could potentially reconcile with the experimental observation. Our proposal therefore sheds new light on the microscopic pairing in Sr$_2$RuO$_4$. We also show that intrinsic Hall effect is generally absent for non-chiral states such as $mathcal{S}+imathcal{D}$, $mathcal{D}+imathcal{P}$ and $mathcal{D}+imathcal{G}$, which provides a clear constraint on the symmetry of the superconducting order in this material.","PeriodicalId":8514,"journal":{"name":"arXiv: Superconductivity","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-08-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"74393717","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Two-dimensional materials are ideal candidates to host Charge density waves (CDWs) that exhibit paramagnetic limiting behavior, similarly to the well known case of superconductors. Here we study how CDWs in two-dimensional systems can survive beyond the Pauli limit when they are subjected to a strong magnetic field by developing a generalized mean-field theory of CDWs under Zeeman fields that includes incommensurability, imperfect nesting and temperature effects and the possibility of a competing or coexisting Spin density wave (SDW) order. Our numerical calculations yield rich phase diagrams with distinct high-field phases above the Pauli limiting field. For perfectly nested commensurate CDWs, a $q$-modulated CDW phase that is completely analogous to the superconducting Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase appears at high-fields. In the more common case of imperfect nesting, the commensurate CDW groundstate undergoes a series of magnetic-field-induced phase transitions first into a phase where commensurate CDW and SDW coexist and subsequently into another phase where CDW and SDW acquire a $q$-modulation that is however distinct from the pure FFLO CDW phase. The commensurate CDW+SDW phase occurs for fields comparable to but less than the Pauli limit and survives above it. Thus this phase provides a plausible mechanism for the CDW to survive at high fields without the need of forming the more fragile FFLO phase. We suggest that the recently discovered 2D materials like the transition metal dichalcogenides offer a promising platform for observing such exotic field induced CDW phenomena.
{"title":"Charge density waves beyond the Pauli paramagnetic limit in 2D systems","authors":"A. Aperis, G. Varelogiannis","doi":"10.1063/5.0015993","DOIUrl":"https://doi.org/10.1063/5.0015993","url":null,"abstract":"Two-dimensional materials are ideal candidates to host Charge density waves (CDWs) that exhibit paramagnetic limiting behavior, similarly to the well known case of superconductors. Here we study how CDWs in two-dimensional systems can survive beyond the Pauli limit when they are subjected to a strong magnetic field by developing a generalized mean-field theory of CDWs under Zeeman fields that includes incommensurability, imperfect nesting and temperature effects and the possibility of a competing or coexisting Spin density wave (SDW) order. Our numerical calculations yield rich phase diagrams with distinct high-field phases above the Pauli limiting field. For perfectly nested commensurate CDWs, a $q$-modulated CDW phase that is completely analogous to the superconducting Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase appears at high-fields. In the more common case of imperfect nesting, the commensurate CDW groundstate undergoes a series of magnetic-field-induced phase transitions first into a phase where commensurate CDW and SDW coexist and subsequently into another phase where CDW and SDW acquire a $q$-modulation that is however distinct from the pure FFLO CDW phase. The commensurate CDW+SDW phase occurs for fields comparable to but less than the Pauli limit and survives above it. Thus this phase provides a plausible mechanism for the CDW to survive at high fields without the need of forming the more fragile FFLO phase. We suggest that the recently discovered 2D materials like the transition metal dichalcogenides offer a promising platform for observing such exotic field induced CDW phenomena.","PeriodicalId":8514,"journal":{"name":"arXiv: Superconductivity","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-08-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"88716024","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-08-27DOI: 10.1103/physrevx.10.041008
Jin Si, Guanyu Chen, Qing Li, Xiyu Zhu, Huan Yang, H. Wen
There are several FeSe based superconductors, including the bulk FeSe, monolayer FeSe thin film, intercalated KxFe2-ySe2 and Li1-xFexOHFeSe, etc. Their normal states all show metallic behavior. The key player here is the FeSe layer which exhibits the highest superconducting transition temperature in the form of monolayer thin film. Recently a new FeSe based compound, CsFe4-xSe4 with the space group of Bmmm was found. Interestingly the system shows a strong insulator-like behavior although it shares the same FeSe planes as other relatives. Density functional theory calculations indicate that it should be a metal, in sharp contrast with the experimental observations. Here we report the emergence of unconventional superconductivity by applying pressure to suppress this insulator-like behavior. At ambient pressure, the insulator-like behavior cannot be modeled as a band insulator, but can be described by the variable-range-hopping model for correlated systems. Furthermore, the specific heat down to 400 mK has been measured and a significant residual coefficient gamma_0=C/T|T->0 is observed, which contrasts the insulator-like state and suggests some quantum freedom of spin dynamics. By applying pressure the insulator-like behavior is gradually suppressed and the system becomes a metal, finally superconductivity is achieved at about 5.1 K. The superconducting transition strongly depends on magnetic field and applied current, indicating a fragile superfluid density. Our results suggest that the superconductivity is established by diluted Cooper pairs on top of a strong correlation background in CsFe4-xSe4.
{"title":"Unconventional Superconductivity Induced by Suppressing an Iron-Selenium-Based Mott Insulator \u0000CsFe4−xSe4","authors":"Jin Si, Guanyu Chen, Qing Li, Xiyu Zhu, Huan Yang, H. Wen","doi":"10.1103/physrevx.10.041008","DOIUrl":"https://doi.org/10.1103/physrevx.10.041008","url":null,"abstract":"There are several FeSe based superconductors, including the bulk FeSe, monolayer FeSe thin film, intercalated KxFe2-ySe2 and Li1-xFexOHFeSe, etc. Their normal states all show metallic behavior. The key player here is the FeSe layer which exhibits the highest superconducting transition temperature in the form of monolayer thin film. Recently a new FeSe based compound, CsFe4-xSe4 with the space group of Bmmm was found. Interestingly the system shows a strong insulator-like behavior although it shares the same FeSe planes as other relatives. Density functional theory calculations indicate that it should be a metal, in sharp contrast with the experimental observations. Here we report the emergence of unconventional superconductivity by applying pressure to suppress this insulator-like behavior. At ambient pressure, the insulator-like behavior cannot be modeled as a band insulator, but can be described by the variable-range-hopping model for correlated systems. Furthermore, the specific heat down to 400 mK has been measured and a significant residual coefficient gamma_0=C/T|T->0 is observed, which contrasts the insulator-like state and suggests some quantum freedom of spin dynamics. By applying pressure the insulator-like behavior is gradually suppressed and the system becomes a metal, finally superconductivity is achieved at about 5.1 K. The superconducting transition strongly depends on magnetic field and applied current, indicating a fragile superfluid density. Our results suggest that the superconductivity is established by diluted Cooper pairs on top of a strong correlation background in CsFe4-xSe4.","PeriodicalId":8514,"journal":{"name":"arXiv: Superconductivity","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-08-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"84996976","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2020-08-25DOI: 10.1103/physrevb.102.180505
S. Kobayashi, A. Furusaki
The interplay of time-reversal and $n$-fold rotation symmetries ($n=2,4,6$) is known to bring a new class of topological crystalline insulators (TCIs) having $n$ surface Dirac cones due to surface rotation anomaly. We show that the proximity-induced $s$-wave superconductivity on the surface of these TCIs yields a topological superconducting phase in which two Majorana zero modes are bound to a vortex, and that $n$-fold rotation symmetry ($n=2,4,6$) enriches the topological classification of a superconducting vortex from $mathbb{Z}_2$ to $mathbb{Z}_2timesmathbb{Z}_2$. Using a model of a three-dimensional high-spin topological insulator with $s$-wave superconductivity and two-fold rotation symmetry, we show that, with increasing chemical potential, the number of Majorana zero modes at one end of a vortex changes as $2to1to0$ through two topological vortex phase transitions. In addition, we show that additional magnetic-mirror symmetry further enhances the topological classification to $mathbb{Z} times mathbb{Z}$
{"title":"Double Majorana vortex zero modes in superconducting topological crystalline insulators with surface rotation anomaly","authors":"S. Kobayashi, A. Furusaki","doi":"10.1103/physrevb.102.180505","DOIUrl":"https://doi.org/10.1103/physrevb.102.180505","url":null,"abstract":"The interplay of time-reversal and $n$-fold rotation symmetries ($n=2,4,6$) is known to bring a new class of topological crystalline insulators (TCIs) having $n$ surface Dirac cones due to surface rotation anomaly. We show that the proximity-induced $s$-wave superconductivity on the surface of these TCIs yields a topological superconducting phase in which two Majorana zero modes are bound to a vortex, and that $n$-fold rotation symmetry ($n=2,4,6$) enriches the topological classification of a superconducting vortex from $mathbb{Z}_2$ to $mathbb{Z}_2timesmathbb{Z}_2$. Using a model of a three-dimensional high-spin topological insulator with $s$-wave superconductivity and two-fold rotation symmetry, we show that, with increasing chemical potential, the number of Majorana zero modes at one end of a vortex changes as $2to1to0$ through two topological vortex phase transitions. In addition, we show that additional magnetic-mirror symmetry further enhances the topological classification to $mathbb{Z} times mathbb{Z}$","PeriodicalId":8514,"journal":{"name":"arXiv: Superconductivity","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2020-08-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"80817861","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
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