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Simplified Josephson-junction fabrication process for reproducibly high-performance superconducting qubits 可重复高性能超导量子比特的简化约瑟夫森结制造工艺
Pub Date : 2020-11-10 DOI: 10.1063/5.0037093
A. Osman, J. Simon, A. Bengtsson, S. Kosen, P. Krantz, D. P. Lozano, M. Scigliuzzo, P. Delsing, J. Bylander, A. Fadavi Roudsari
We introduce a simplified fabrication technique for Josephson junctions and demonstrate superconducting Xmon qubits with $T_1$ relaxation times averaging above 50$~mu$s ($Q>$1.5$times$ 10$^6$). Current shadow-evaporation techniques for aluminum-based Josephson junctions require a separate lithography step to deposit a patch that makes a galvanic, superconducting connection between the junction electrodes and the circuit wiring layer. The patch connection eliminates parasitic junctions, which otherwise contribute significantly to dielectric loss. In our patch-integrated cross-type (PICT) junction technique, we use one lithography step and one vacuum cycle to evaporate both the junction electrodes and the patch. In a study of more than 3600 junctions, we show an average resistance variation of 3.7$%$ on a wafer that contains forty 0.5$times$0.5-cm$^2$ chips, with junction areas ranging between 0.01 and 0.16 $mu$m$^2$. The average on-chip spread in resistance is 2.7$%$, with 20 chips varying between 1.4 and 2$%$. For the junction sizes used for transmon qubits, we deduce a wafer-level transition-frequency variation of 1.7-2.5$%$. We show that 60-70$%$ of this variation is attributed to junction-area fluctuations, while the rest is caused by tunnel-junction inhomogeneity. Such high frequency predictability is a requirement for scaling-up the number of qubits in a quantum computer.
我们介绍了一种简化的约瑟夫森结制造技术,并演示了超导Xmon量子比特的$T_1$弛豫时间平均大于50$~mu$s ($Q>$1.5$乘以$ 10$^6$)。目前用于铝基约瑟夫森结的阴影蒸发技术需要单独的光刻步骤来沉积贴片,从而在结电极和电路布线层之间形成电超导连接。贴片连接消除了寄生结,否则寄生结会显著增加介电损耗。在我们的贴片集成交叉型(PICT)结技术中,我们使用一个光刻步骤和一个真空循环来蒸发结电极和贴片。在对3600多个结的研究中,我们发现在包含40个0.5 × 0.5 cm芯片的晶圆上,平均电阻变化为3.7$ $ %$,结面积在0.01到0.16 $ $ mu$m$ $^2$之间。芯片上电阻的平均价差为2.7美元,其中20个芯片的价差在1.4美元到2美元之间。对于用于transmon量子位的结尺寸,我们推断出晶圆级的过渡频率变化为1.7-2.5美元。我们表明,这种变化的60- 70%归因于结区波动,而其余的是由隧道结的不均匀性引起的。这种高频率的可预测性是扩大量子计算机中量子位数量的必要条件。
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引用次数: 51
Superconductivity beyond Pauli's limit in bulk NbS2: Evidence for the Fulde-Ferrell-Larkin-Ovchinnikov state 体NbS2中超过泡利极限的超导性:Fulde-Ferrell-Larkin-Ovchinnikov态的证据
Pub Date : 2020-11-10 DOI: 10.21203/rs.3.rs-105803/v1
C. Cho, J. Lyu, C. Ng, J. J. He, T. Abdel-Baset, M. Abdel-Hafiez, R. Lortz
We present magnetic torque, specific heat and thermal expansion measurements combined with a piezo rotary positioner of the bulk transition metal dichalcogenide (TMD) superconductor NbS2 in high magnetic fields applied strictly parallel to its layer structure. The upper critical field of superconducting TMDs in the 2D form is known to be dramatically enhanced by a special form of Ising spin orbit coupling. This Ising superconductivity is very robust against the Pauli limit for superconductivity. We find that superconductivity beyond the Pauli limit still exists in bulk single crystals of NbS2. However, the comparison of our upper critical field transition line with numerical simulations rather points to the development of a Fulde-Ferrell-Larkin-Ovchinnikov state above the Pauli limit as a cause. This is also consistent with the observation of a magnetic field driven phase transition in the thermodynamic quantities within the superconducting state near the Pauli limit.
结合压电旋转定位器,研究了大块过渡金属二硫化物超导体NbS2在严格平行于其层状结构的高磁场下的磁转矩、比热和热膨胀。二维超导tmd的上临界场被一种特殊形式的伊辛自旋轨道耦合显著增强。这种伊辛超导性在泡利极限下是非常稳定的。我们发现在NbS2单晶中仍然存在超过泡利极限的超导性。然而,我们的上临界场过渡线与数值模拟的比较更指向了泡利极限以上的富尔德-费雷尔-拉金-奥夫钦尼科夫态的发展。这也与在接近泡利极限的超导态热力学量中磁场驱动相变的观察结果一致。
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引用次数: 1
Zeeman-driven superconductor-insulator transition in strongly disordered MoC films: Scanning tunneling microscopy and transport studies in a transverse magnetic field 强无序MoC薄膜中塞曼驱动的超导体-绝缘体跃迁:扫描隧道显微镜和横向磁场中的输运研究
Pub Date : 2020-11-09 DOI: 10.1103/PhysRevB.102.180508
M. Žemlička, M. Kopčík, P. Szab'o, T. Samuely, J. Kačmarčík, P. Neilinger, M. Grajcar, P. Samuely
Superconductor insulator transition in transverse magnetic field is studied in the highly disordered MoC film with the product of the Fermi momentum and the mean free path $k_F*l$ close to unity. Surprisingly, the Zeeman paramagnetic effects dominate over orbital coupling on both sides of the transition. In superconducting state it is evidenced by a high upper critical magnetic field $B_{c2}$, by its square root dependence on temperature, as well as by the Zeeman splitting of the quasiparticle density of states (DOS) measured by scanning tunneling microscopy. At $B_{c2}$ a logarithmic anomaly in DOS is observed. This anomaly is further enhanced in increasing magnetic field, which is explained by the Zeeman splitting of the Altshuler-Aronov DOS driving the system into a more insulating or resistive state. Spin dependent Altshuler-Aronov correction is also needed to explain the transport behavior above $B_{c2}$.
在高度无序的MoC薄膜中,研究了费米动量与平均自由程$k_F*l$的乘积接近于单位的横向磁场中的超导体绝缘体跃迁。令人惊讶的是,塞曼顺磁效应在跃迁两侧的轨道耦合中占主导地位。在超导状态下,高临界磁场$B_{c2}$,它对温度的平方根依赖,以及用扫描隧道显微镜测量的准粒子态密度(DOS)的塞曼分裂都证明了这一点。在$B_{c2}$处,观察到DOS的对数异常。随着磁场的增加,这种异常进一步增强,这可以解释为Altshuler-Aronov DOS的塞曼分裂使系统进入更加绝缘或电阻的状态。自旋相关的Altshuler-Aronov修正也需要用来解释$B_{c2}$以上的输运行为。
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引用次数: 4
Two-gap time reversal symmetry breaking superconductivity in noncentrosymmetric LaNiC2 非中心对称LaNiC2的双间隙时间反转对称性破缺超导性
Pub Date : 2020-11-04 DOI: 10.1103/PHYSREVB.103.014511
S. Sundar, S. Dunsiger, S. Gheidi, K. Akella, A. M. Cot'e, H. U. Özdemir, N. R. Lee-Hone, D. Broun, E. Mun, F. Honda, Y. Sato, T. Koizumi, R. Settai, Y. Hirose, I. Bonalde, J. Sonier
We report a $mu$SR investigation of a non-centrosymmetric superconductor (LaNiC$_2$) in single crystal form. Compared to previous $mu$SR studies of non-centrosymmetric superconducting polycrystalline and powder samples, the unambiguous orientation of single crystals enables a simultaneous determination of the absolute value of the magnetic penetration depth and the vortex core size from measurements that probe the magnetic field distribution in the vortex state. The magnetic field dependence of these quantities unambiguously demonstrates the presence of two nodeless superconducting energy gaps. In addition, we detect weak internal magnetic fields in the superconducting phase, confirming earlier $mu$SR evidence for a time-reversal symmetry breaking superconducting state. Our results suggest that Cooper pairing in LaNiC$_2$ is characterized by the same interorbital equal-spin pairing model introduced to describe the pairing state in the centrosymmetric superconductor LaNiGa$_2$.
我们报道了单晶形式的非中心对称超导体(LaNiC$_2$)的SR研究。与之前对非中心对称超导多晶和粉末样品的研究相比,单晶的明确取向使得通过测量漩涡状态下的磁场分布可以同时确定磁穿透深度的绝对值和漩涡核的大小。这些量的磁场依赖性明确地证明了两个无节点超导能隙的存在。此外,我们在超导相中检测到微弱的内部磁场,证实了时间反转对称性破缺超导态的早期$mu$SR证据。我们的研究结果表明,LaNiC$_2$中的Cooper配对与描述中心对称超导体LaNiC$_2$中的配对状态的轨道间等自旋配对模型相同。
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引用次数: 4
Superconducting ground state of the topological superconducting candidates Ti3X (X=Ir,Sb) 拓扑超导候选者Ti3X (X=Ir,Sb)的超导基态
Pub Date : 2020-11-04 DOI: 10.1103/PHYSREVB.103.054501
Manasi Mandal, K. P. Sajilesh, R. R. Chowdhury, D. Singh, P. Biswas, A. Hillier, R. P. Singh
The topologically non-trivial band structure of A15 compounds has drawn attention owing to the possible realization of topological superconductivity. Here, we report a microscopic investigation of the superconducting ground state in A15 compound Ti$_{3}$X (X = Ir, Sb) by muon spectroscopy measurements. Zero field muon measurements have shown that time-reversal symmetry is preserved in these materials. Furthermore, specific heat and a transverse field muon spectroscopy measurement rule out any possibility to have a nodal or anisotropic superconducting gap, revealing a conventional s-wave nature in the superconducting ground state. This work classifies A15 compound Ti$_{3}$X (X = Ir, Sb) as a time-reversal preserved topological superconductor.
A15化合物的拓扑非平凡带结构由于可能实现拓扑超导性而引起人们的关注。在这里,我们报告了用μ介子光谱测量对A15化合物Ti$ {3}$X (X = Ir, Sb)超导基态的微观研究。零场μ子测量表明,在这些材料中保持了时间反转对称性。此外,比热和横向场μ子光谱测量排除了存在节点或各向异性超导间隙的任何可能性,揭示了超导基态中的常规s波性质。本工作将A15化合物Ti$ {3}$X (X = Ir, Sb)归类为时间反转保存的拓扑超导体。
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引用次数: 4
Intrinsic mechanism for magnetothermal conductivity oscillations in spin-orbit-coupled nodal superconductors 自旋轨道耦合节点超导体中磁热导率振荡的内在机制
Pub Date : 2020-11-02 DOI: 10.1103/PHYSREVRESEARCH.3.023023
W. Atkinson, A. Kampf
We describe a mechanism by which the longitudinal thermal conductivity $kappa_{xx}$, measured in an in-plane magnetic field, oscillates as a function of field angle in layered nodal superconductors. These oscillations occur when the spin-orbit splitting at the nodes is larger than the nodal scattering rate, and are complementary to vortex-induced oscillations identified previously. In sufficiently anisotropic materials, the spin-orbit mechanism may be dominant. As a particular application, we focus on the cuprate high-temperature superconductor YBa$_2$Cu$_3$O$_{6+x}$. This material belongs to the class of Rashba bilayers, in which individual CuO$_2$ layers lack inversion symmetry although the crystal itself is globally centrosymmetric. We show that spin-orbit coupling endows $kappa_{xx}/T$ with a characteristic dependence on magnetic field angle that should be easily detected experimentally, and argue that for underdoped samples the spin-orbit contribution is larger than the vortex contribution. A key advantage of the magneto-thermal conductivity is that it is a bulk probe of spin-orbit physics, and therefore not sensitive to inversion breaking at surfaces.
我们描述了一种在平面内磁场中测量的纵向导热系数$kappa_{xx}$作为场角函数在层状节点超导体中振荡的机制。当节点上的自旋轨道分裂大于节点散射率时,这些振荡就会发生,并且与之前发现的涡诱导振荡互补。在充分各向异性的材料中,自旋轨道机制可能占主导地位。作为一个特殊的应用,我们重点研究了铜高温超导体YBa$_2$Cu$_3$O$_{6+x}$。该材料属于Rashba双层结构,虽然CuO$_2$晶体本身是全局中心对称的,但个别CuO$_2$层缺乏反演对称性。我们证明了自旋轨道耦合使$kappa_{xx}/T$具有对磁场角的特征依赖,这应该很容易通过实验检测到,并且认为对于欠掺杂样品,自旋轨道的贡献大于涡旋的贡献。磁热导的一个关键优势是它是自旋轨道物理的体探针,因此对表面的反转破裂不敏感。
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引用次数: 0
Chiral Majorana Hinge Modes in Superconducting Dirac Materials 超导狄拉克材料的手性Majorana铰链模式
Pub Date : 2020-10-29 DOI: 10.1103/PhysRevB.103.L180504
Bo Fu, Zi-Ang Hu, Chang-An Li, Jian Li, S. Shen
Chiral Majorana hinge modes are characteristic of a second-order topological superconductor in three dimensions. Here we systematically study pairing symmetry in the point group D_{2h}, and find that the leading pairing channels can be of s-, d-, and s+id-wave pairing in Dirac materials. Except for the odd-parity s-wave pairing superconductivity, the s+id-wave pairing superconductor is topologically nontrivial and possesses Majorana hinge and surface modes. The chiral Majorana hinge modes can be characterized by a winding number of the quadrupole moment, or quantized quadruple moment at the symmetrically invariant point. Our findings suggest the strong spin-orbital coupling, crystalline symmetries and electron-electron interaction in the Dirac materials may provide a microscopic mechanism to realize chiral Majorana hinge modes without utilizing the proximity effect or external fields.
手性马约拉纳铰链模式是三维二阶拓扑超导体的特征。本文系统地研究了点群D_{2h}中的配对对称性,发现了Dirac材料中领先的配对通道可以是s-、d-和s+id波配对。除了奇宇称s波配对超导外,s+id波配对超导在拓扑上是非平凡的,并且具有马约拉纳铰链和表面模式。手性Majorana铰链模式可以用四极矩的圈数或对称不变点的量化四极矩来表征。我们的研究结果表明,Dirac材料中的强自旋-轨道耦合、晶体对称性和电子-电子相互作用可能为不利用邻近效应或外场实现手性Majorana铰链模式提供了微观机制。
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引用次数: 11
Reemergence of superconductivity in pressurized quasi-one-dimensional superconductor K2Mo3As3 加压准一维超导体K2Mo3As3中超导性的再现
Pub Date : 2020-10-28 DOI: 10.1103/PHYSREVMATERIALS.5.L021801
Cheng Huang, Jing Guo, K. Zhao, Fan Cui, Shengshan Qin, Q. Mu, Yazhou Zhou, Shu Cai, Chongli Yang, S. Long, Ke Yang, Aiguo Li, Qi Wu, Z. Ren, Jiangping Hu, Liling Sun
Here we report a pressure-induced reemergence of superconductivity in recently discovered superconductor K2Mo3As3, which is the first experimental case observed in quasi-one-dimensional superconductors. We find that, after full suppression of the ambient-pressure superconducting (SC-I) state at 8.7 GPa, an intermediary non-superconducting state sets in and prevails to the pressure up to 18.2 GPa, however, above this pressure a new superconducting (SC-II) state appears unexpectedly. High pressure x-ray diffraction measurements demonstrate that the pressure-induced dramatic change of the lattice parameter c contributes mainly to the emergence of the SC-II state. Combined with the theioretical calculations on band strcture, our results suggest that the reemergemce of superconductivity is associated with the change of the complicated interplay among different orbital electrons, driven by the pressure-induced unisotropic change of the lattice.
在这里,我们报告了最近发现的超导体K2Mo3As3的压力诱导超导性的重新出现,这是在准一维超导体中观察到的第一个实验案例。我们发现,常压超导态(SC-I)在8.7 GPa完全被抑制后,中间非超导态进入并盛行到18.2 GPa,然而在此压力以上,一个新的超导态(SC-II)意外出现。高压x射线衍射测量表明,压力引起的晶格参数c的剧烈变化是SC-II态出现的主要原因。结合带结构的理论计算,我们的结果表明,超导体的重新出现与不同轨道电子之间复杂的相互作用的变化有关,由压力诱导的晶格的各向同性变化驱动。
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引用次数: 5
Time-reversal-symmetry breaking and unconventional pairing in the noncentrosymmetric superconductor La7Rh3 非中心对称超导体La7Rh3中的时间逆对称破缺和非常规配对
Pub Date : 2020-10-27 DOI: 10.1103/physrevb.102.134511
D. Singh, M. Scheurer, A. Hillier, D. Adroja, R. Singh
Noncentrosymmetric superconductors have sparked significant research interests due to their exciting properties, such as the admixture of spin-singlet and spin-triplet Cooper pairs. Here we report $mu$SR and thermodynamic measurements on the noncentrosymmetric superconductor La7Rh3 which indicate a fully established superconducting gap and spontaneous time-reversal-symmetry breaking at the onset of superconductivity. We show that our results pose severe constraints on any microscopic theory of superconductivity in the system. A symmetry analysis identifies ground states compatible with time-reversal-symmetry breaking and the resulting gap functions are discussed. Furthermore, general energetic considerations indicate the relevance of electron-electron interactions for the pairing mechanism, in accordance with hints of spin-fluctuations revealed in susceptibility measurements.
非中心对称超导体由于其令人兴奋的性质,如自旋单线态和自旋三重态库珀对的混合物,引起了重大的研究兴趣。本文报道了非中心对称超导体La7Rh3的SR和热力学测量结果,表明在超导开始时存在完全建立的超导间隙和自发的时间逆对称性破缺。我们表明,我们的结果对系统中超导的任何微观理论都提出了严格的限制。对称性分析确定了与时间逆对称性破缺相容的基态,并讨论了由此产生的间隙函数。此外,根据磁化率测量显示的自旋波动提示,一般能量考虑表明电子-电子相互作用与配对机制的相关性。
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引用次数: 13
a-axis YBa2Cu3O7−x/PrBa2Cu3O7−x/YBa2Cu3O7−x trilayers with subnanometer rms roughness 具有亚纳米rms粗糙度的a轴YBa2Cu3O7−x/PrBa2Cu3O7−x/YBa2Cu3O7−x三层膜
Pub Date : 2020-10-23 DOI: 10.1063/5.0034648
Y. Suyolcu, Jiaxin Sun, B. Goodge, Jisung Park, J. Schubert, L. Kourkoutis, D. Schlom
We demonstrate a-axis YBa2Cu3O7-x/PrBa2Cu3O7-x/YBa2Cu3O7-x trilayers grown on (100) LaAlO3 substrates with improved interface smoothness. The trilayers are synthesized by ozone-assisted molecular-beam epitaxy. The thickness of the PrBa2Cu3O7-x layer is held constant at 8 nm and the thickness of the YBa2Cu3O7-x layers is varied from 24 nm to 100 nm. X-ray diffraction measurements show all trilayers to have >95% a-axis content. The rms roughness of the thinnest trilayer is < 0.7 nm and this roughness increases with the thickness of the YBa2Cu3O7-x layers. The thickness of the YBa2Cu3O7-x layers also affects the transport properties: while all samples exhibit an onset of the superconducting transition at and above 85 K, the thinner samples show wider transition widths, {Delta}Tc. High-resolution scanning transmission electron microscopy reveals coherent and chemically sharp interfaces, and that growth begins with a cubic (Y,Ba)CuO3-x perovskite phase that transforms into a-axis oriented YBa2Cu3O7-x as the substrate temperature is ramped up.
我们展示了在(100)LaAlO3衬底上生长的a轴YBa2Cu3O7-x/PrBa2Cu3O7-x/YBa2Cu3O7-x三层膜,其界面光滑性得到了改善。采用臭氧辅助分子束外延法制备了三层膜。PrBa2Cu3O7-x层的厚度保持在8 nm, YBa2Cu3O7-x层的厚度在24 ~ 100 nm之间变化。x射线衍射测量表明,所有三层膜的a轴含量为95%。最薄三层的rms粗糙度< 0.7 nm,且粗糙度随YBa2Cu3O7-x层厚度的增加而增大。YBa2Cu3O7-x层的厚度也影响其输运性质:虽然所有样品在85 K及以上都表现出超导转变的开始,但较薄的样品表现出更宽的转变宽度,{Delta}Tc。高分辨率扫描透射电子显微镜显示了相干和化学尖锐的界面,并且随着衬底温度的升高,生长始于立方(Y,Ba)CuO3-x钙钛矿相转变为a轴取向的YBa2Cu3O7-x。
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引用次数: 4
期刊
arXiv: Superconductivity
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