首页 > 最新文献

Current Applied Physics最新文献

英文 中文
Synergistic impact of Al2O3 capping layer and deposition temperature for enhancing the ferroelectricity of undoped-HfO2 thin films
IF 2.4 4区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-28 DOI: 10.1016/j.cap.2024.11.016
Sang Han Ko , Seung-Eon Moon , Sung Min Yoon
Synergistic effects of Al2O3 capping layer and deposition temperature, ranging from 220 to 280 °C, on the ferroelectric properties of undoped HfO2 thin films were investigated. The use of an Al2O3 capping layer during atomic layer deposition (ALD) process was verified to induce a ferroelectric orthorhombic phase in undoped HfO2 thin films, leading to a net remnant polarization (2Pr) of >20 μC/cm2 when deposited <260 °C. The HfO2 thin film deposited at 240 °C showed a low leakage current density of 5.7 × 10−6 A/cm2 at an electric field of 2 MV/cm, accompanied by a high 2Pr and an endurance of >107 cycles. Furthermore, the switching time for ferroelectric polarization reversal was estimated to range from 2.1 to 1.7 μs in the voltage range of 3.5–4.5 V. The results of this work demonstrated the impact of deposition temperature conditions on the ferroelectric properties of the HfO2 thin films by means of the Al2O3 capping process.
{"title":"Synergistic impact of Al2O3 capping layer and deposition temperature for enhancing the ferroelectricity of undoped-HfO2 thin films","authors":"Sang Han Ko ,&nbsp;Seung-Eon Moon ,&nbsp;Sung Min Yoon","doi":"10.1016/j.cap.2024.11.016","DOIUrl":"10.1016/j.cap.2024.11.016","url":null,"abstract":"<div><div>Synergistic effects of Al<sub>2</sub>O<sub>3</sub> capping layer and deposition temperature, ranging from 220 to 280 °C, on the ferroelectric properties of undoped HfO<sub>2</sub> thin films were investigated. The use of an Al<sub>2</sub>O<sub>3</sub> capping layer during atomic layer deposition (ALD) process was verified to induce a ferroelectric orthorhombic phase in undoped HfO<sub>2</sub> thin films, leading to a net remnant polarization (2P<sub>r</sub>) of &gt;20 μC/cm<sup>2</sup> when deposited &lt;260 °C. The HfO<sub>2</sub> thin film deposited at 240 °C showed a low leakage current density of 5.7 × 10<sup>−6</sup> A/cm<sup>2</sup> at an electric field of 2 MV/cm, accompanied by a high 2P<sub>r</sub> and an endurance of &gt;10<sup>7</sup> cycles. Furthermore, the switching time for ferroelectric polarization reversal was estimated to range from 2.1 to 1.7 μs in the voltage range of 3.5–4.5 V. The results of this work demonstrated the impact of deposition temperature conditions on the ferroelectric properties of the HfO<sub>2</sub> thin films by means of the Al<sub>2</sub>O<sub>3</sub> capping process.</div></div>","PeriodicalId":11037,"journal":{"name":"Current Applied Physics","volume":"71 ","pages":"Pages 1-8"},"PeriodicalIF":2.4,"publicationDate":"2024-11-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142747740","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Improved mobility in InAs nanowire FETs with sulfur-based surface treatment
IF 2.4 4区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-26 DOI: 10.1016/j.cap.2024.11.015
Yen Hsueh Wu , Hong Hyuk Kim , Jae Cheol Shin
InAs exhibits high electron mobility, positioning it as a promising candidate for advanced nanoelectronic device materials. Specifically, nanowire structures are particularly advantageous for electronic device applications, offering benefits such as reduced leakage current and minimized short-channel effects due to their distinctive one-dimensional electron transport characteristics. However, the large surface-to-volume ratio of the nanowires not only significantly degrades their electrical properties but also complicates the formation of semiconductor-metal ohmic contacts. In this study, surface treatments involving sulfur and (NH4)2S, along with rapid thermal annealing (RTA) processes, were applied to mitigate these disadvantages, resulting in a marked enhancement of the electrical properties of InAs nanowires. The electron mobility of the InAs nanowires was elevated from 83.06 cm2/V·s to 292.718 cm2/V·s through the application of passivation and RTA processes.
{"title":"Improved mobility in InAs nanowire FETs with sulfur-based surface treatment","authors":"Yen Hsueh Wu ,&nbsp;Hong Hyuk Kim ,&nbsp;Jae Cheol Shin","doi":"10.1016/j.cap.2024.11.015","DOIUrl":"10.1016/j.cap.2024.11.015","url":null,"abstract":"<div><div>InAs exhibits high electron mobility, positioning it as a promising candidate for advanced nanoelectronic device materials. Specifically, nanowire structures are particularly advantageous for electronic device applications, offering benefits such as reduced leakage current and minimized short-channel effects due to their distinctive one-dimensional electron transport characteristics. However, the large surface-to-volume ratio of the nanowires not only significantly degrades their electrical properties but also complicates the formation of semiconductor-metal ohmic contacts. In this study, surface treatments involving sulfur and (NH<sub>4</sub>)<sub>2</sub>S, along with rapid thermal annealing (RTA) processes, were applied to mitigate these disadvantages, resulting in a marked enhancement of the electrical properties of InAs nanowires. The electron mobility of the InAs nanowires was elevated from 83.06 cm<sup>2</sup>/V·s to 292.718 cm<sup>2</sup>/V·s through the application of passivation and RTA processes.</div></div>","PeriodicalId":11037,"journal":{"name":"Current Applied Physics","volume":"70 ","pages":"Pages 81-86"},"PeriodicalIF":2.4,"publicationDate":"2024-11-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142747435","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Graphene/WS2/LaVO3 heterojunction for self-powered, high-speed, and broadband photodetectors 用于自供电、高速和宽带光电探测器的石墨烯/WS2/LaVO3 异质结
IF 2.4 4区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-23 DOI: 10.1016/j.cap.2024.11.014
Dong Hee Shin , Hosun Lee
Recently, there has been interest in developing high-performance self-driven photodetectors (PDs) using 2D-based heterostructures due to their unique optoelectronic properties. Here, we demonstrate that vertical-heterostructures based on graphene (Gr) transparent conductive electrodes, n-type 2D WS2, and p-type LaVO3 realize a broadband-responsive PD covering the wavelength range of 300–850 nm. Due to the formation of an electric field at the WS2/LaVO3 interface and the photovoltaic effect, this structure shows a rectifying operation with a maximum detectivity of 2.1 × 1010 Jones at zero bias. Additionally, it exhibits a fast fall time of 435 μs and a 3 dB bandwidth of 2300 Hz, making it suitable for high-speed self-powered optoelectronic applications. Therefore, the TETA-Gr/WS2/LaVO3 heterojunction is proposed as an excellent candidate for high-performance, self-powered, and broadband PDs.
最近,由于二维异质结构具有独特的光电特性,人们开始关注利用二维异质结构开发高性能自驱动光电探测器(PD)。在这里,我们证明了基于石墨烯(Gr)透明导电电极、n 型二维 WS2 和 p 型 LaVO3 的垂直异质结构可实现波长范围为 300-850 nm 的宽带响应型 PD。由于在 WS2/LaVO3 界面形成的电场和光生伏打效应,这种结构显示出整流操作,在零偏压下的最大检测率为 2.1 × 1010 琼斯。此外,它还具有 435 μs 的快速下降时间和 2300 Hz 的 3 dB 带宽,适合高速自供电光电应用。因此,TETA-Gr/WS2/LaVO3 异质结被认为是高性能、自供电和宽带 PD 的理想候选材料。
{"title":"Graphene/WS2/LaVO3 heterojunction for self-powered, high-speed, and broadband photodetectors","authors":"Dong Hee Shin ,&nbsp;Hosun Lee","doi":"10.1016/j.cap.2024.11.014","DOIUrl":"10.1016/j.cap.2024.11.014","url":null,"abstract":"<div><div>Recently, there has been interest in developing high-performance self-driven photodetectors (PDs) using 2D-based heterostructures due to their unique optoelectronic properties. Here, we demonstrate that vertical-heterostructures based on graphene (Gr) transparent conductive electrodes, n-type 2D WS<sub>2</sub>, and p-type LaVO<sub>3</sub> realize a broadband-responsive PD covering the wavelength range of 300–850 nm. Due to the formation of an electric field at the WS<sub>2</sub>/LaVO<sub>3</sub> interface and the photovoltaic effect, this structure shows a rectifying operation with a maximum detectivity of 2.1 × 10<sup>10</sup> Jones at zero bias. Additionally, it exhibits a fast fall time of 435 μs and a 3 dB bandwidth of 2300 Hz, making it suitable for high-speed self-powered optoelectronic applications. Therefore, the TETA-Gr/WS<sub>2</sub>/LaVO<sub>3</sub> heterojunction is proposed as an excellent candidate for high-performance, self-powered, and broadband PDs.</div></div>","PeriodicalId":11037,"journal":{"name":"Current Applied Physics","volume":"70 ","pages":"Pages 69-75"},"PeriodicalIF":2.4,"publicationDate":"2024-11-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142720527","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Oxidation effects on the optical and electrical properties of MoS2 under controlled baking temperatures 受控烘烤温度下氧化对 MoS2 光学和电学特性的影响
IF 2.4 4区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-22 DOI: 10.1016/j.cap.2024.11.013
Takmo Jeong , Jiyoon Kim , Un Jeong Kim , Hyunjin Ji , Seok Joon Yun
As silicon-based semiconductor technology scales down to the nanoscale, it encounters significant physical limitations, including reduced electron mobility, short-channel effects, and increased heat generation, which hinder device performance and reliability. Two-dimensional (2D) semiconductors, such as molybdenum disulfide (MoS2), offer great potential with superior electrical properties at the nanoscale, but the issue of excessive heat generation in highly integrated circuits persists. Therefore, it is essential to investigate the thermal durability of MoS2 under various heating conditions and its impact on physical properties and device performance. In this study, we systematically investigated the oxidation behavior and related physical property variations of CVD-grown MoS2 monolayers by baking them at different temperatures. It was clearly revealed that high-temperature baking induces p-doping and structural deformation, significantly altering optical and electrical properties. Despite the degradation in device performance, reduced interfacial Coulomb scattering was observed, suggesting potential for improved device stability. This study underscores the importance of understanding thermal stability to accelerate the development of 2D semiconductors for next-generation electronic devices.
当硅基半导体技术缩小到纳米尺度时,它遇到了很大的物理限制,包括电子迁移率降低、短沟道效应和发热量增加,这些都阻碍了器件的性能和可靠性。二维(2D)半导体,如二硫化钼(MoS2),在纳米尺度上具有卓越的电学特性,具有巨大的潜力,但在高度集成电路中产生过多热量的问题依然存在。因此,研究 MoS2 在各种加热条件下的热耐久性及其对物理性质和器件性能的影响至关重要。在本研究中,我们通过在不同温度下烘烤 CVD 生长的 MoS2 单层,系统地研究了它们的氧化行为和相关物理性质变化。研究清楚地表明,高温烘烤会诱导 p 掺杂和结构变形,显著改变光学和电学特性。尽管器件性能下降,但观察到界面库仑散射减少,这表明器件稳定性有可能提高。这项研究强调了了解热稳定性对于加速开发用于下一代电子器件的二维半导体的重要性。
{"title":"Oxidation effects on the optical and electrical properties of MoS2 under controlled baking temperatures","authors":"Takmo Jeong ,&nbsp;Jiyoon Kim ,&nbsp;Un Jeong Kim ,&nbsp;Hyunjin Ji ,&nbsp;Seok Joon Yun","doi":"10.1016/j.cap.2024.11.013","DOIUrl":"10.1016/j.cap.2024.11.013","url":null,"abstract":"<div><div>As silicon-based semiconductor technology scales down to the nanoscale, it encounters significant physical limitations, including reduced electron mobility, short-channel effects, and increased heat generation, which hinder device performance and reliability. Two-dimensional (2D) semiconductors, such as molybdenum disulfide (MoS<sub>2</sub>), offer great potential with superior electrical properties at the nanoscale, but the issue of excessive heat generation in highly integrated circuits persists. Therefore, it is essential to investigate the thermal durability of MoS<sub>2</sub> under various heating conditions and its impact on physical properties and device performance. In this study, we systematically investigated the oxidation behavior and related physical property variations of CVD-grown MoS<sub>2</sub> monolayers by baking them at different temperatures. It was clearly revealed that high-temperature baking induces <em>p</em>-doping and structural deformation, significantly altering optical and electrical properties. Despite the degradation in device performance, reduced interfacial Coulomb scattering was observed, suggesting potential for improved device stability. This study underscores the importance of understanding thermal stability to accelerate the development of 2D semiconductors for next-generation electronic devices.</div></div>","PeriodicalId":11037,"journal":{"name":"Current Applied Physics","volume":"70 ","pages":"Pages 61-68"},"PeriodicalIF":2.4,"publicationDate":"2024-11-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142697807","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Nanosecond electric pulse-induced ultrafast piezoelectric responses in Co3+ substituted BiFeO3 epitaxial thin films Co3+ 取代的 BiFeO3 外延薄膜中的纳秒电脉冲诱导超快压电响应
IF 2.4 4区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-22 DOI: 10.1016/j.cap.2024.11.012
Sanjith Unithrattil , Taewon Min , Gopinathan Anoop , Jun Young Lee , Tae Yeon kim , Shibnath Samanta , Yubo Qi , Jiahao Zhang , Seung Hyun Hwang , Hyeon Jun Lee , Kun Guo , Su Yong Lee , Yasuhiko Imai , Osami Sakata , Keisuke Shimizu , Kei Shigematsu , Hajime Hojo , Kui Yao , Masaki Azuma , Jaekwang Lee , Ji Young Jo
Understanding the ultra-fast dynamics of ferroelectric materials is essential for advancing the development of next-generation high speed electronic and photonic devices. Here, the ultrafast piezoelectric response of cobalt-substituted BiFeO3 (BiFe1-xCoxO3) with x = 0.15, consisting of morphotropic phase boundary of monoclinic MC and MA –type phases is investigated. The real-time piezoelectric response in (001)-oriented BiFe0.85Co0.15O3 (BFCO) epitaxial thin film was monitored using the time-resolved X-ray microdiffraction technique under an applied electric field with pulse widths 70 ns and 100 ns. The BFCO thin film yielded a high piezoelectric strain of approximately 0.53 % along [001] direction, with a giant c/a ratio (∼1.26) at an electric field of 1.3 MV/cm and a pulse width of 100 ns, with a piezoelectric coefficient (d33) of 40 pm/V. This finding is an important step towards the development of a high performance lead-free piezoelectric material for ultrafast operations in advanced technological applications.
了解铁电材料的超快动态对于推动下一代高速电子和光子器件的发展至关重要。本文研究了 x = 0.15 的钴取代 BiFeO3(BiFe1-xCoxO3)的超快压电响应,它由单斜 MC 型相和 MA 型相的各向异性相界组成。在脉冲宽度为 70 ns 和 100 ns 的外加电场下,使用时间分辨 X 射线微衍射技术监测了 (001) 取向 BiFe0.85Co0.15O3 (BFCO) 外延薄膜的实时压电响应。在 1.3 MV/cm 的电场和 100 ns 的脉冲宽度下,BFCO 薄膜沿 [001] 方向产生了约 0.53 % 的高压电应变,具有巨大的 c/a 比 (∼1.26),压电系数 (d33) 为 40 pm/V。这一发现是为先进技术应用中的超快操作开发高性能无铅压电材料迈出的重要一步。
{"title":"Nanosecond electric pulse-induced ultrafast piezoelectric responses in Co3+ substituted BiFeO3 epitaxial thin films","authors":"Sanjith Unithrattil ,&nbsp;Taewon Min ,&nbsp;Gopinathan Anoop ,&nbsp;Jun Young Lee ,&nbsp;Tae Yeon kim ,&nbsp;Shibnath Samanta ,&nbsp;Yubo Qi ,&nbsp;Jiahao Zhang ,&nbsp;Seung Hyun Hwang ,&nbsp;Hyeon Jun Lee ,&nbsp;Kun Guo ,&nbsp;Su Yong Lee ,&nbsp;Yasuhiko Imai ,&nbsp;Osami Sakata ,&nbsp;Keisuke Shimizu ,&nbsp;Kei Shigematsu ,&nbsp;Hajime Hojo ,&nbsp;Kui Yao ,&nbsp;Masaki Azuma ,&nbsp;Jaekwang Lee ,&nbsp;Ji Young Jo","doi":"10.1016/j.cap.2024.11.012","DOIUrl":"10.1016/j.cap.2024.11.012","url":null,"abstract":"<div><div>Understanding the ultra-fast dynamics of ferroelectric materials is essential for advancing the development of next-generation high speed electronic and photonic devices. Here, the ultrafast piezoelectric response of cobalt-substituted BiFeO<sub>3</sub> (BiFe<sub>1-<em>x</em></sub>Co<sub><em>x</em></sub>O<sub>3</sub>) with <em>x</em> = 0.15, consisting of morphotropic phase boundary of monoclinic M<sub>C</sub> and M<sub>A</sub> –type phases is investigated. The real-time piezoelectric response in (001)-oriented BiFe<sub>0.85</sub>Co<sub>0.15</sub>O<sub>3</sub> (BFCO) epitaxial thin film was monitored using the time-resolved X-ray microdiffraction technique under an applied electric field with pulse widths 70 ns and 100 ns. The BFCO thin film yielded a high piezoelectric strain of approximately 0.53 % along [001] direction, with a giant <em>c</em>/<em>a</em> ratio (∼1.26) at an electric field of 1.3 MV/cm and a pulse width of 100 ns, with a piezoelectric coefficient (<span><math><mrow><msub><mi>d</mi><mn>33</mn></msub></mrow></math></span>) of 40 pm/V. This finding is an important step towards the development of a high performance lead-free piezoelectric material for ultrafast operations in advanced technological applications.</div></div>","PeriodicalId":11037,"journal":{"name":"Current Applied Physics","volume":"70 ","pages":"Pages 76-80"},"PeriodicalIF":2.4,"publicationDate":"2024-11-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142720528","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Observation of anomalous Nernst effect in non-collinear antiferromagnets 观测非共线反铁磁体中的反常涅斯特效应
IF 2.4 4区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-20 DOI: 10.1016/j.cap.2024.11.011
Asif Ullah, Thanh-Huong Thi Nguyen, Sanghoon Kim
The field of spin caloritronics, which explores the interplay between spin current and thermal effects, is a promising path for new energy-efficient-electronic devices. However, current thermoelectric technologies are limited by conventional material choices and device designs. Antiferromagnetic materials, with their unique spin structure and magnetic characteristics, provide new opportunities for enhanced thermoelectric performance through spin-dependent effects. This review covers origin and measurement methodologies of anomalous Nernst effect, focusing on non-collinear antiferromagnets. By presenting insights into the relationship between electronic structure and thermoelectric performance as well as their practical measurements, this review aims to pave the way for developing AFM-based thermoelectric devices in advanced energy technologies.
自旋热电领域探索自旋电流与热效应之间的相互作用,是实现新型节能电子器件的一条大有可为的途径。然而,目前的热电技术受到传统材料选择和器件设计的限制。反铁磁材料具有独特的自旋结构和磁性特征,为通过自旋效应提高热电性能提供了新的机遇。这篇综述涵盖了异常奈恩斯特效应的起源和测量方法,重点关注非共轭反铁磁体。通过介绍电子结构与热电性能之间的关系及其实际测量方法,本综述旨在为开发先进能源技术中基于原子力显微镜的热电设备铺平道路。
{"title":"Observation of anomalous Nernst effect in non-collinear antiferromagnets","authors":"Asif Ullah,&nbsp;Thanh-Huong Thi Nguyen,&nbsp;Sanghoon Kim","doi":"10.1016/j.cap.2024.11.011","DOIUrl":"10.1016/j.cap.2024.11.011","url":null,"abstract":"<div><div>The field of spin caloritronics, which explores the interplay between spin current and thermal effects, is a promising path for new energy-efficient-electronic devices. However, current thermoelectric technologies are limited by conventional material choices and device designs. Antiferromagnetic materials, with their unique spin structure and magnetic characteristics, provide new opportunities for enhanced thermoelectric performance through spin-dependent effects. This review covers origin and measurement methodologies of anomalous Nernst effect, focusing on non-collinear antiferromagnets. By presenting insights into the relationship between electronic structure and thermoelectric performance as well as their practical measurements, this review aims to pave the way for developing AFM-based thermoelectric devices in advanced energy technologies.</div></div>","PeriodicalId":11037,"journal":{"name":"Current Applied Physics","volume":"70 ","pages":"Pages 51-60"},"PeriodicalIF":2.4,"publicationDate":"2024-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142698501","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Improved thermoelectric properties of the β-Cu2+xSe/CuInSe2 multilayer films by layer interface scattering 通过层界面散射改善 β-Cu2+xSe/CuInSe2 多层薄膜的热电性能
IF 2.4 4区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-19 DOI: 10.1016/j.cap.2024.11.010
Yu Chen, Guihong Song, Zhihao Ben, Yusheng Wu, Junhua You
The β-Cu2+xSe/CuInSe2 multilayer films with different modulation period were prepared and studied. The results showed that the deposited films possessed obvious layered structure. The room temperature carrier concentration, mobility, electrical conductivity and thermal conductivity decreased, but the Seebeck coefficient and power factor and relative thermoelectric figure of merit increased with reducing modulation period of deposited β-Cu2-xSe/CuInSe2 multilayer films. The linear reduction of carrier concentration and mobility and the decrease in thermal conductivity with modulation period was attributed to the scattering of carriers and phonons by layer interface and grain boundary, respectively. The sample with the smallest modulation period (160 nm) possessed the highest power factor of ∼0.74 at room temperature and ∼1.56 mW m−1 K−2 at 405 °C. The insertion of heterogeneous layer into films is an effective method to increase Seebeck coefficient and decrease thermal conductivity, thus increasing thermoelectric figure of merit of films.
制备并研究了不同调制周期的β-Cu2+xSe/CuInSe2多层薄膜。结果表明,沉积的薄膜具有明显的层状结构。随着调制周期的缩短,β-Cu2+xSe/CuInSe2 多层薄膜的室温载流子浓度、迁移率、电导率和热导率均有所下降,但塞贝克系数、功率因数和相对热电功勋值均有所上升。载流子浓度和迁移率的线性降低以及热导率随调制周期的降低分别归因于层界面和晶界对载流子和声子的散射。调制周期最小(160 nm)的样品在室温下具有最高的功率因数 ∼ 0.74,在 405 °C 时为 ∼ 1.56 mW m-1 K-2。在薄膜中插入异质层是提高塞贝克系数和降低热导率的有效方法,从而提高了薄膜的热电特性。
{"title":"Improved thermoelectric properties of the β-Cu2+xSe/CuInSe2 multilayer films by layer interface scattering","authors":"Yu Chen,&nbsp;Guihong Song,&nbsp;Zhihao Ben,&nbsp;Yusheng Wu,&nbsp;Junhua You","doi":"10.1016/j.cap.2024.11.010","DOIUrl":"10.1016/j.cap.2024.11.010","url":null,"abstract":"<div><div>The β-Cu<sub>2+x</sub>Se/CuInSe<sub>2</sub> multilayer films with different modulation period were prepared and studied. The results showed that the deposited films possessed obvious layered structure. The room temperature carrier concentration, mobility, electrical conductivity and thermal conductivity decreased, but the Seebeck coefficient and power factor and relative thermoelectric figure of merit increased with reducing modulation period of deposited β-Cu<sub>2-x</sub>Se/CuInSe<sub>2</sub> multilayer films. The linear reduction of carrier concentration and mobility and the decrease in thermal conductivity with modulation period was attributed to the scattering of carriers and phonons by layer interface and grain boundary, respectively. The sample with the smallest modulation period (160 nm) possessed the highest power factor of ∼0.74 at room temperature and ∼1.56 mW m<sup>−1</sup> K<sup>−2</sup> at 405 °C. The insertion of heterogeneous layer into films is an effective method to increase Seebeck coefficient and decrease thermal conductivity, thus increasing thermoelectric figure of merit of films.</div></div>","PeriodicalId":11037,"journal":{"name":"Current Applied Physics","volume":"70 ","pages":"Pages 1-10"},"PeriodicalIF":2.4,"publicationDate":"2024-11-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142698494","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Impact analysis of various types of simulated multiple scattering matrices on the numerical simulation of high-resolution imaging in scattering media 各类模拟多重散射矩阵对散射介质中高分辨率成像数值模拟的影响分析
IF 2.4 4区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-19 DOI: 10.1016/j.cap.2024.11.004
Ye-Ryoung Lee
Optical techniques are essential in biomedical research, enabling high-resolution, non-invasive imaging of biological tissues. However, imaging depth in optical microscopy is limited by multiple scattering in scattering media, such as biological tissues. Various methods have been developed to overcome this limitation, and numerical simulations have played an important role in developing new imaging techniques. Traditional simulations often use simple random matrices to represent multiple-scattered waves, which overly simplifies their behavior and may impact the accuracy of image quality assessments. In this study, we introduce various types of simulated multiple scattering matrices to better capture the characteristics of scattered waves. We systematically analyze the correlation properties of these matrices and evaluate their impact on high-resolution imaging quality. This work provides a foundation for selecting appropriate matrix types for simulating multiple scattering effects, aiding in the effective testing and validation of new microscopy techniques in scattering media.
光学技术在生物医学研究中至关重要,它能对生物组织进行高分辨率、非侵入式成像。然而,光学显微镜的成像深度受到生物组织等散射介质中多重散射的限制。为了克服这一限制,人们开发了各种方法,其中数值模拟在开发新的成像技术方面发挥了重要作用。传统的模拟通常使用简单的随机矩阵来表示多重散射波,这过于简化了多重散射波的行为,可能会影响图像质量评估的准确性。在本研究中,我们引入了各种类型的模拟多重散射矩阵,以更好地捕捉散射波的特征。我们系统地分析了这些矩阵的相关特性,并评估了它们对高分辨率成像质量的影响。这项工作为选择合适的矩阵类型来模拟多重散射效应奠定了基础,有助于在散射介质中有效测试和验证新的显微技术。
{"title":"Impact analysis of various types of simulated multiple scattering matrices on the numerical simulation of high-resolution imaging in scattering media","authors":"Ye-Ryoung Lee","doi":"10.1016/j.cap.2024.11.004","DOIUrl":"10.1016/j.cap.2024.11.004","url":null,"abstract":"<div><div>Optical techniques are essential in biomedical research, enabling high-resolution, non-invasive imaging of biological tissues. However, imaging depth in optical microscopy is limited by multiple scattering in scattering media, such as biological tissues. Various methods have been developed to overcome this limitation, and numerical simulations have played an important role in developing new imaging techniques. Traditional simulations often use simple random matrices to represent multiple-scattered waves, which overly simplifies their behavior and may impact the accuracy of image quality assessments. In this study, we introduce various types of simulated multiple scattering matrices to better capture the characteristics of scattered waves. We systematically analyze the correlation properties of these matrices and evaluate their impact on high-resolution imaging quality. This work provides a foundation for selecting appropriate matrix types for simulating multiple scattering effects, aiding in the effective testing and validation of new microscopy techniques in scattering media.</div></div>","PeriodicalId":11037,"journal":{"name":"Current Applied Physics","volume":"70 ","pages":"Pages 21-26"},"PeriodicalIF":2.4,"publicationDate":"2024-11-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142697805","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Near-field infrared spectroscopy: Advanced research method in thin film analysis 近场红外光谱仪:薄膜分析中的先进研究方法
IF 2.4 4区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-16 DOI: 10.1016/j.cap.2024.11.002
Jiho Kim , Boknam Chae , Sangsul Lee
This article introduces several cases of s-SNOM (Scattering-type scanning near-field optical microscopy) based on a SPM (Scanning probe microscopy) for chemical thin film. A highly concentrated near-field infrared performs the chemical analysis of s-SNOM at the sharp apex of the metal-coated atomic microscope tip. This attractive technique, which provides both surface morphology and chemical information of the material simultaneously, various studies have been published, including surface polariton propagation, Moire superlattice, and ballistic valley transport. Further, s-SNOM successfully visualized the formation of lamellar nanostructures of BCP and the latent image of photoresist formed by EUV (extreme ultraviolet). These results were cross-validated through traditional GIWAXS (Grazing-incidence wide-angle X-ray scattering) and FTIR (Fourier transform infrared) analysis. s-SNOM is a useful tool for providing new insights into material analysis by visualizing nanoscale chemical information of local regions that conventional measurements could not confirm.
本文介绍了基于扫描探针显微镜(SPM)的化学薄膜 s-SNOM(散射型扫描近场光学显微镜)的几种情况。高度集中的近场红外线可在金属涂层原子显微镜尖端的尖锐顶点对 s-SNOM 进行化学分析。这项极具吸引力的技术可同时提供材料的表面形态和化学信息,目前已发表了多项研究成果,包括表面极化子传播、莫伊尔超晶格和弹道谷传输。此外,s-SNOM 还成功地观察到了 BCP 的片状纳米结构的形成以及 EUV(极紫外线)形成的光刻胶的潜像。这些结果通过传统的 GIWAXS(Grazing-incidence wide-angle X-ray scattering)和 FTIR(Fourier transform infrared)分析进行了交叉验证。s-SNOM 是一种有用的工具,它通过可视化局部区域的纳米级化学信息,为材料分析提供了新的见解,而传统的测量方法却无法确认这些信息。
{"title":"Near-field infrared spectroscopy: Advanced research method in thin film analysis","authors":"Jiho Kim ,&nbsp;Boknam Chae ,&nbsp;Sangsul Lee","doi":"10.1016/j.cap.2024.11.002","DOIUrl":"10.1016/j.cap.2024.11.002","url":null,"abstract":"<div><div>This article introduces several cases of s-SNOM (Scattering-type scanning near-field optical microscopy) based on a SPM (Scanning probe microscopy) for chemical thin film. A highly concentrated near-field infrared performs the chemical analysis of s-SNOM at the sharp apex of the metal-coated atomic microscope tip. This attractive technique, which provides both surface morphology and chemical information of the material simultaneously, various studies have been published, including surface polariton propagation, Moire superlattice, and ballistic valley transport. Further, s-SNOM successfully visualized the formation of lamellar nanostructures of BCP and the latent image of photoresist formed by EUV (extreme ultraviolet). These results were cross-validated through traditional GIWAXS (Grazing-incidence wide-angle X-ray scattering) and FTIR (Fourier transform infrared) analysis. s-SNOM is a useful tool for providing new insights into material analysis by visualizing nanoscale chemical information of local regions that conventional measurements could not confirm.</div></div>","PeriodicalId":11037,"journal":{"name":"Current Applied Physics","volume":"70 ","pages":"Pages 41-50"},"PeriodicalIF":2.4,"publicationDate":"2024-11-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142698500","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Analysis of electron thermal properties in Ar/O2 inductively coupled plasmas: A global model simulation using Langmuir probe data Ar/O2电感耦合等离子体中的电子热特性分析:利用朗缪尔探针数据进行全局模型模拟
IF 2.4 4区 物理与天体物理 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-11-15 DOI: 10.1016/j.cap.2024.11.003
Hwiwon Seo , Haneul Lee , Ji-Won Kwon , Gwanjoong Kim , Ingyu Lee , Gon-Ho Kim
This study investigates the electron thermal properties in Argon and Ar/O2 inductively coupled plasmas using global model based on Langmuir probe data. The sensor-data driven global model (GM) is improved to simulate the power coupling efficiency and an electron energy distribution simultaneously. It reveals that the heating characteristic changes the thermal state and radical generation with input power, pressure and gas mixture ratio. The analysis results of probe data from the global model provide information on the plasma thermal characteristics under efficient operating conditions of process plasma. It provides the advantage of offering insights into the causes of variations in the plasma thermal equilibrium state with operating conditions in ICP, which are limited to obtain from the sensor or the general GM. This makes it highly promising as a simulation method for developing process recipes.
本研究利用基于朗缪尔探针数据的全局模型,研究了氩气和氩气/氧气电感耦合等离子体中的电子热特性。研究改进了传感器数据驱动的全局模型(GM),以同时模拟功率耦合效率和电子能量分布。它揭示了加热特性会随着输入功率、压力和气体混合比的变化而改变热状态和自由基的生成。全局模型的探测数据分析结果提供了工艺等离子体有效工作条件下的等离子体热特性信息。它的优势在于可以深入了解 ICP 中等离子体热平衡状态随操作条件变化的原因,而这些原因只能从传感器或一般 GM 中获得。因此,作为一种模拟方法,它在开发工艺配方方面大有可为。
{"title":"Analysis of electron thermal properties in Ar/O2 inductively coupled plasmas: A global model simulation using Langmuir probe data","authors":"Hwiwon Seo ,&nbsp;Haneul Lee ,&nbsp;Ji-Won Kwon ,&nbsp;Gwanjoong Kim ,&nbsp;Ingyu Lee ,&nbsp;Gon-Ho Kim","doi":"10.1016/j.cap.2024.11.003","DOIUrl":"10.1016/j.cap.2024.11.003","url":null,"abstract":"<div><div>This study investigates the electron thermal properties in Argon and Ar/O2 inductively coupled plasmas using global model based on Langmuir probe data. The sensor-data driven global model (GM) is improved to simulate the power coupling efficiency and an electron energy distribution simultaneously. It reveals that the heating characteristic changes the thermal state and radical generation with input power, pressure and gas mixture ratio. The analysis results of probe data from the global model provide information on the plasma thermal characteristics under efficient operating conditions of process plasma. It provides the advantage of offering insights into the causes of variations in the plasma thermal equilibrium state with operating conditions in ICP, which are limited to obtain from the sensor or the general GM. This makes it highly promising as a simulation method for developing process recipes.</div></div>","PeriodicalId":11037,"journal":{"name":"Current Applied Physics","volume":"70 ","pages":"Pages 27-40"},"PeriodicalIF":2.4,"publicationDate":"2024-11-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142697806","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Current Applied Physics
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1