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Sulfur-Nickel Foam as Cathode Materials for Lithium-Sulfur Batteries 硫镍泡沫电池正极材料的研究
Pub Date : 2014-12-04 DOI: 10.1149/2.0011502EEL
Juanjuan Cheng, Zhu Jing-tao, Yong Pan, Zengsheng Ma, H. J. Song, Junan Pan, L. Zhenzhen, Chunsheng Lu
Sulfur-nickel foam cathode materials prepared by an in situ solution-based method were served as electrode of lithium-sulfur (Li-S) batteries. At the rate of 0.5 C, the Li-S cells deliver an initial discharge capacity of 1340 mAh g–1 and 493 mAh g–1 after 500 cycles. It is shown that these Li-S cells are of high rate stabilities with a nearly 100% stable coulombic efficiency at various rates from 0.1 C to 5 C. The electrochemical stability of Li-S batteries is mainly due to the strong binding between the highly dispersed sulphur and nickel foam skeletons.
采用原位溶液法制备了硫镍泡沫正极材料作为锂硫电池的电极。在0.5 C的速率下,锂电池在500次循环后的初始放电容量为1340 mAh g-1和493 mAh g-1。结果表明,在0.1℃~ 5℃范围内,这些锂硫电池具有很高的速率稳定性,库仑效率接近100%。锂硫电池的电化学稳定性主要是由于高度分散的硫和泡沫镍骨架之间的强结合。
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引用次数: 27
Effects of Self-Catalyzed Polyaniline Coating on the Electrochemical Performance of 0.4Li2MnO3·0.6LiMn0.33Ni0.33Co0.33O2 Electrodes 自催化聚苯胺涂层对0.4Li2MnO3·0.6LiMn0.33Ni0.33Co0.33O2电极电化学性能的影响
Pub Date : 2014-11-21 DOI: 10.1149/2.0141501EEL
Kug‐Seung Lee, J. Gim, P. Chirawatkul, Jaekook Kim, T. Shin, Docheon Ahn
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引用次数: 3
Temperature-Dependent Impedance Spectroscopy of Molten Alkali-Halide Salt Binary Mixtures 熔融碱-卤化物二元混合物的温度相关阻抗谱
Pub Date : 2014-11-21 DOI: 10.1149/2.0131501EEL
Y. Cohen, Yitzhak Gabay, Y. Cohen
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引用次数: 6
Corrosion Resistance of Current Collector Materials in Bisamide Based Electrolyte for Magnesium Batteries 镁电池用双酰胺基电解液集流材料的耐腐蚀性能
Pub Date : 2014-11-18 DOI: 10.1149/2.0111501EEL
Clemens Wall, Z. Zhao‐Karger, M. Fichtner
The compatibility of Ti, Cr, Ni, Fe, Al, steel type 304, Inconel 625, Hastelloy B and carbon coated current collectors with bisamide based electrolyte for Mg-batteries was investigated. Pitting corrosion of current collectors made from 3d-transition metals and steel type 304 was observed at potentials between 2.2–3.1 V vs. Mg/Mg2+. Anodic stability up to 3.8 V and resistance against corrosion for 48 h at a potential of 2.5 V vs. Mg/Mg2+ and above was found for Inconel 625, Hastelloy B, graphite and carbon coated Al foil. © The Author(s) 2014. Published by ECS. This is an open access article distributed under the terms of the Creative Commons Attribution Non-Commercial No Derivatives 4.0 License (CC BY-NC-ND, http://creativecommons.org/licenses/by-nc-nd/4.0/), which permits non-commercial reuse, distribution, and reproduction in any medium, provided the original work is not changed in any way and is properly cited. For permission for commercial reuse, please email: oa@electrochem.org. [DOI: 10.1149/2.0111501eel] All rights reserved.
研究了Ti、Cr、Ni、Fe、Al、304钢、Inconel 625、哈氏合金B和碳包覆集流器与铋酰胺基电解质的相容性。由3d过渡金属和304钢制成的集流器在2.2 ~ 3.1 V vs. Mg/Mg2+电位范围内观察到点蚀现象。Inconel 625、Hastelloy B、石墨和碳涂层Al箔的阳极稳定性高达3.8 V,在2.5 V vs. Mg/Mg2+及以上电位下耐腐蚀48 h。©作者2014。由ECS出版。这是一篇在知识共享署名非商业禁止衍生品4.0许可(CC BY-NC-ND, http://creativecommons.org/licenses/by-nc-nd/4.0/)条款下发布的开放获取文章,该许可允许在任何媒介上进行非商业重用、分发和复制,前提是原始作品不以任何方式改变并适当引用。如需商业使用许可,请发邮件至oa@electrochem.org。[DOI: 10.1149/2.0111501]版权所有。
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引用次数: 55
Erratum: A Manganese Porphyrin Intercalated Lanthanum Niobic Acid Nanocomposite Utilized for Electrocatalytic Oxidation of Nitrite [ECS Electrochem. Lett., 3, H17 (2014)] 一种用于亚硝酸盐电催化氧化的卟啉锰插层铌酸镧纳米复合材料[ECS]。列托人。, 3, h17 (2014)]
Pub Date : 2014-11-15 DOI: 10.1149/2.0121501EEL
Xiaobo Zhang, Jiasheng Xu, Mingyan Wang, Gaowa Siqin, Ruibo Xu, Juanjuan Ma, Lin Liu, Dongen Zhang, Zhiwei Tong
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引用次数: 1
Determining the Exchange Current Density and Tafel Constant for Uranium in LiCl/KCl Eutectic LiCl/KCl共晶中铀的交换电流密度和塔菲尔常数的测定
Pub Date : 2014-11-13 DOI: 10.1149/2.0101501EEL
M. Rose, M. Williamson, J. Willit
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引用次数: 28
An Electrochemical Method for Measuring Localized Corrosion under Cathodic Protection 阴极保护下局部腐蚀的电化学测量方法
Pub Date : 2014-11-12 DOI: 10.1149/2.0091501EEL
F. Varela, M. Tan, M. Forsyth
A new method has been developed to measure metal corrosion rates and their distribution under cathodic protection (CP). This method uses an electrochemically integrated multi-electrode array to take local measurements of cathodic current density while simulating a continuous metallic surface. The distribution of cathodic current densities obtained under CP was analyzed to estimate the anodic current component at each electrode of the array. Corrosion patterns determined by this new method have shown good correlation with visual inspection and surface profilometry of the multi-electrode array surface.
提出了一种在阴极保护下测量金属腐蚀速率及其分布的新方法。该方法采用电化学集成多电极阵列,在模拟连续金属表面的同时,对阴极电流密度进行局部测量。分析了阴极电流密度分布,估算了阵列各电极处的阳极电流分量。该方法测定的腐蚀模式与多电极阵列表面的目视检测和表面轮廓测量具有良好的相关性。
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引用次数: 18
Composite Anodes for Secondary Magnesium Ion Batteries Prepared via Electrodeposition of Nanostructured Bismuth on Carbon Nanotube Substrates 碳纳米管衬底电沉积纳米结构铋制备二次镁离子电池复合阳极
Pub Date : 2014-11-12 DOI: 10.1149/2.0081501EEL
R. DiLeo, Qing Zhang, A. Marschilok, K. Takeuchi, E. Takeuchi
Magnesium-ion batteries are attractive in part due to the high environmental abundance and low cost of magnesium metal. Anode materialsotherthanMgmetalcanprovideaccesstonewelectrochemistriesinnon-corrosiveMg2+ electrolytes.Acyclicvoltammetric method for the preparation of bismuth (Bi) based anodes was developed by systematically exploring electrodeposition using a quartz crystal microbalance. Controlled deposition of Bi on carbon nanotubes substrates could be achieved, enabling the first electrochemical investigation of bismuth-carbon nanotube (Bi-CNT) composite electrodes. Quasi-reversible Mg electrochemistry of Bi-CNT composite electrodes in non-corrosive magnesium-based electrolyte was demonstrated, with an initial delivered capacity exceeding 180 mAh/g. While the initial capacities were high, significant capacity decreases were observed with repeated cycling,
镁离子电池具有很高的环境丰度和较低的成本。阳极材料,而不是金属镁,可以提供无障碍的电化学无腐蚀性的emg2 +电解质。利用石英晶体微天平对电沉积进行了系统的探索,提出了一种制备铋基阳极的非环伏安法。可以实现铋在碳纳米管衬底上的可控沉积,使铋-碳纳米管(Bi- cnt)复合电极的首次电化学研究成为可能。证实了Bi-CNT复合电极在无腐蚀性镁基电解质中的准可逆Mg电化学,其初始输送容量超过180 mAh/g。虽然初始容量很高,但随着反复循环,容量明显下降。
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引用次数: 39
Field-Limited Migration of Li-Ions in Li-Ion Battery 锂离子电池中锂离子的场限制迁移
Pub Date : 2014-11-10 DOI: 10.1149/2.0071501EEL
Fuqian Yang
The migration of Li-ions in lithium-ion battery cannot be simply described by Fick’s second law; the interactions among ionic migration, field, and stress need to be taken into account when analyzing the migration of Li-ions. Using the theory of thermal activation process, the flux for ionic migration under concurrent action of electric field and mechanical stress is found to be a nonlinear function of the gradient of electric potential and the gradient of stress. Electric field can either accelerate or retard the growth of the lithiation layer, depending on polarity of the field.
锂离子电池中锂离子的迁移不能简单地用菲克第二定律来描述;在分析锂离子迁移时,需要考虑离子迁移、电场和应力之间的相互作用。利用热活化过程理论,发现电场和机械应力共同作用下离子迁移通量是电势梯度和应力梯度的非线性函数。电场可以加速或阻碍锂化层的生长,这取决于电场的极性。
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引用次数: 12
Accurate Determination of Battery Electrode Loading (Mass) from Electrochemical Impedance Spectroscopy 电化学阻抗谱法精确测定电池电极负载(质量)
Pub Date : 2014-11-10 DOI: 10.1149/2.0061501EEL
Jože Moškon, Maja Pivko, R. Dominko, M. Gaberšček
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引用次数: 5
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