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Ionizing terahertz waves with 260 MV/cm from scalable optical rectification 通过可扩展的光学整流技术实现 260 MV/cm 的太赫兹电离波
Pub Date : 2024-05-27 DOI: 10.1038/s41377-024-01462-w
Hyeongmun Kim, Chul Kang, Dogeun Jang, Yulan Roh, Sang Hwa Lee, Joong Wook Lee, Jae Hee Sung, Seong Ku Lee, Ki-Yong Kim

Terahertz (THz) waves, known as non-ionizing radiation owing to their low photon energies, can actually ionize atoms and molecules when a sufficiently large number of THz photons are concentrated in time and space. Here, we demonstrate the generation of ionizing, multicycle, 15-THz waves emitted from large-area lithium niobate crystals via phase-matched optical rectification of 150-terawatt laser pulses. A complete characterization of the generated THz waves in energy, pulse duration, and focal spot size shows that the field strength can reach up to 260 megavolts per centimeter. In particular, a single-shot THz interferometer is employed to measure the THz pulse duration and spectrum with complementary numerical simulations. Such intense THz pulses are irradiated onto various solid targets to demonstrate THz-induced tunneling ionization and plasma formation. This study also discusses the potential of nonperturbative THz-driven ionization in gases, which will open up new opportunities, including nonlinear and relativistic THz physics in plasma.

太赫兹(THz)波因光子能量低而被称为非电离辐射,但当足够多的太赫兹光子在时间和空间上集中时,实际上可以电离原子和分子。在这里,我们展示了通过对 150 太瓦激光脉冲进行相位匹配光学整流,从大面积铌酸锂晶体中产生电离、多周期、15 太赫兹波。对所产生的太赫兹波的能量、脉冲持续时间和焦斑大小进行的完整表征表明,场强可达每厘米 260 兆伏特。特别是采用了单发太赫兹干涉仪来测量太赫兹脉冲持续时间和频谱,并辅以数值模拟。这种强烈的太赫兹脉冲被照射到各种固体目标上,以演示太赫兹诱导的隧道电离和等离子体的形成。本研究还讨论了气体中非微扰太赫兹驱动电离的潜力,这将带来新的机遇,包括等离子体中的非线性和相对论太赫兹物理学。
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引用次数: 0
Light People: Professor Fanglin Bao and his cover story 光明人物包芳林教授和他的封面故事
Pub Date : 2024-05-22 DOI: 10.1038/s41377-024-01434-0
Ji Wang

Qu Yuan, a renowned ancient Chinese poet, once pondered in his work Heavenly Inquiry: “If the sun’s light is absent, from where does the radiance of the Hero Flower emanate?” The ability to see clearly in the darkest of nights has long been a sought-after magical power by humans. It holds not only immense technological significance for computer vision and remote sensing but also profound implications for transcending the dichotomy between day and night in our daily lives. Professor Fanglin Bao from Westlake University has made significant breakthroughs in this field, bringing us closer to a world where we can transform night into day. His groundbreaking research on Heat-Assisted Detection and Ranging (HADAR) and night vision was featured as the cover story in Nature on July 26, 2023.

For this issue of “Light People”, Professor Fanglin Bao will share his research journey and the captivating story behind HADAR.

中国古代著名诗人屈原曾在他的作品《天问》中思考:"如果没有太阳的光辉,英雄花的光芒又从何而来?"能在漆黑的夜晚看清东西,一直以来都是人类追求的神奇力量。它不仅对计算机视觉和遥感技术有着巨大的技术意义,而且对我们日常生活中超越白天和黑夜的对立有着深远的影响。西湖大学的包方林教授在这一领域取得了重大突破,使我们离黑夜变白昼的世界更近了一步。他在热辅助探测与测距(HADAR)和夜视方面的开创性研究于 2023 年 7 月 26 日成为《自然》杂志的封面故事。本期 "光影人物",鲍方林教授将分享他的研究历程和 HADAR 背后的动人故事。
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引用次数: 0
Enhancing crystal integrity and structural rigidity of CsPbBr3 nanoplatelets to achieve a narrow color-saturated blue emission 增强 CsPbBr3 纳米片的晶体完整性和结构刚度,实现窄色饱和蓝光发射
Pub Date : 2024-05-11 DOI: 10.1038/s41377-024-01441-1
Qianqian Huang, Wenxu Yin, Bo Gao, Qingsen Zeng, Dong Yao, Hao Zhang, Yinghe Zhao, Weijia Zheng, Jiaqi Zhang, Xuyong Yang, Xiaoyu Zhang, Andrey L. Rogach

Quantum-confined CsPbBr3 perovskites are promising blue emitters for ultra-high-definition displays, but their soft lattice caused by highly ionic nature has a limited stability. Here, we endow CsPbBr3 nanoplatelets (NPLs) with atomic crystal-like structural rigidity through proper surface engineering, by using strongly bound N-dodecylbenzene sulfonic acid (DBSA). A stable, rigid crystal structure, as well as uniform, orderly-arranged surface of these NPLs is achieved by optimizing intermediate reaction stage, by switching from molecular clusters to mono-octahedra, while interaction with DBSA resulted in formation of a CsxO monolayer shell capping the NPL surface. As a result, both structural and optical stability of the CsPbBr3 NPLs is enhanced by strong covalent bonding of DBSA, which inhibits undesired phase transitions and decomposition of the perovskite phase potentially caused by ligand desorption. Moreover, rather small amount of DBSA ligands at the NPL surface results in a short inter-NPL spacing in their closely-packed films, which facilitates efficient charge injection and transport. Blue photoluminescence of the produced CsPbBr3 NPLs is bright (nearly unity emission quantum yield) and peaks at 457 nm with an extremely narrow bandwidth of 3.7 nm at 80 K, while the bandwidth of the electroluminescence (peaked at 460 nm) also reaches a record-narrow value of 15 nm at room temperature. This value corresponds to the CIE coordinates of (0.141, 0.062), which meets Rec. 2020 standards for ultra-high-definition displays.

量子约束 CsPbBr3 包晶石是很有希望用于超高清显示器的蓝色发光体,但其高离子性导致的软晶格稳定性有限。在这里,我们利用强结合的 N-十二烷基苯磺酸(DBSA),通过适当的表面工程赋予 CsPbBr3 纳米片(NPLs)原子晶体般的结构刚性。通过优化中间反应阶段,将分子簇转换成单八面体,从而实现了这些 NPL 稳定、坚硬的晶体结构以及均匀、有序排列的表面,而与 DBSA 的相互作用则形成了覆盖 NPL 表面的 CsxO 单层壳。因此,DBSA 的强共价键增强了 CsPbBr3 NPL 的结构和光学稳定性,抑制了配体解吸可能导致的不希望的相变和包晶相分解。此外,NPL 表面的 DBSA 配体数量相当少,导致其紧密堆积的薄膜中 NPL 间距较短,有利于电荷的有效注入和传输。所制备的 CsPbBr3 NPL 具有明亮的蓝色光致发光(发射量子产率几乎为零),在 80 K 时的峰值为 457 nm,带宽极窄,仅为 3.7 nm,而电致发光的带宽(峰值为 460 nm)在室温下也达到了创纪录的 15 nm 窄值。该值与 CIE 坐标(0.141, 0.062)相对应,符合 Rec.2020 超高清显示标准。
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引用次数: 0
Entangled photon pair generation in an integrated SiC platform 在集成式碳化硅平台中产生纠缠光子对
Pub Date : 2024-05-09 DOI: 10.1038/s41377-024-01443-z
Anouar Rahmouni, Ruixuan Wang, Jingwei Li, Xiao Tang, Thomas Gerrits, Oliver Slattery, Qing Li, Lijun Ma

Entanglement plays a vital role in quantum information processing. Owing to its unique material properties, silicon carbide recently emerged as a promising candidate for the scalable implementation of advanced quantum information processing capabilities. To date, however, only entanglement of nuclear spins has been reported in silicon carbide, while an entangled photon source, whether it is based on bulk or chip-scale technologies, has remained elusive. Here, we report the demonstration of an entangled photon source in an integrated silicon carbide platform for the first time. Specifically, strongly correlated photon pairs are efficiently generated at the telecom C-band wavelength through implementing spontaneous four-wave mixing in a compact microring resonator in the 4H-silicon-carbide-on-insulator platform. The maximum coincidence-to-accidental ratio exceeds 600 at a pump power of 0.17 mW, corresponding to a pair generation rate of (9 ± 1) × 103 pairs/s. Energy-time entanglement is created and verified for such signal-idler photon pairs, with the two-photon interference fringes exhibiting a visibility larger than 99%. The heralded single-photon properties are also measured, with the heralded g(2)(0) on the order of 10−3, demonstrating the SiC platform as a prospective fully integrated, complementary metal-oxide-semiconductor compatible single-photon source for quantum applications.

纠缠在量子信息处理中起着至关重要的作用。由于其独特的材料特性,碳化硅最近成为了可扩展地实现先进量子信息处理能力的理想候选材料。然而,迄今为止,在碳化硅中只报道了核自旋的纠缠,而纠缠光子源,无论是基于块体还是芯片级技术,都仍然遥不可及。在这里,我们首次报告了在集成碳化硅平台中展示纠缠光子源的情况。具体来说,通过在 4H 碳化硅-绝缘体平台的紧凑型微波谐振器中实施自发四波混合,在电信 C 波段有效地产生了强相关光子对。在泵浦功率为 0.17 mW 时,最大巧合-偶然比超过 600,对应的光对生成率为 (9 ± 1) × 103 对/秒。能量-时间纠缠的产生并验证了这种信号-闲置光子对,双光子干涉条纹的可见度大于 99%。此外,还测量了预示单光子特性,预示 g(2)(0) 为 10-3 量级,这表明 SiC 平台有望成为用于量子应用的全集成互补金属氧化物半导体兼容单光子源。
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引用次数: 0
Optical probing of ultrafast laser-induced solid-to-overdense-plasma transitions 超快激光诱导的固体到过密等离子体转变的光学探测
Pub Date : 2024-05-08 DOI: 10.1038/s41377-024-01444-y
Yasmina Azamoum, Georg Alexander Becker, Sebastian Keppler, Guillaume Duchateau, Stefan Skupin, Mickael Grech, Fabrice Catoire, Sebastian Hell, Issa Tamer, Marco Hornung, Marco Hellwing, Alexander Kessler, Franck Schorcht, Malte Christoph Kaluza

Understanding the solid target dynamics resulting from the interaction with an ultrashort laser pulse is a challenging fundamental multi-physics problem involving atomic and solid-state physics, plasma physics, and laser physics. Knowledge of the initial interplay of the underlying processes is essential to many applications ranging from low-power laser regimes like laser-induced ablation to high-power laser regimes like laser-driven ion acceleration. Accessing the properties of the so-called pre-plasma formed as the laser pulse’s rising edge ionizes the target is complicated from the theoretical and experimental point of view, and many aspects of this laser-induced transition from solid to overdense plasma over picosecond timescales are still open questions. On the one hand, laser-driven ion acceleration requires precise control of the pre-plasma because the efficiency of the acceleration process crucially depends on the target properties at the arrival of the relativistic intensity peak of the pulse. On the other hand, efficient laser ablation requires, for example, preventing the so-called “plasma shielding”. By capturing the dynamics of the initial stage of the interaction, we report on a detailed visualization of the pre-plasma formation and evolution. Nanometer-thin diamond-like carbon foils are shown to transition from solid to plasma during the laser rising edge with intensities < 1016 W/cm². Single-shot near-infrared probe transmission measurements evidence sub-picosecond dynamics of an expanding plasma with densities above 1023 cm−3 (about 100 times the critical plasma density). The complementarity of a solid-state interaction model and kinetic plasma description provides deep insight into the interplay of initial ionization, collisions, and expansion.

理解固体目标与超短激光脉冲相互作用产生的动力学是一个具有挑战性的基本多物理问题,涉及原子和固体物理、等离子体物理和激光物理。从激光诱导烧蚀等低功率激光状态到激光驱动离子加速等高功率激光状态,了解基本过程的初始相互作用对于许多应用都至关重要。从理论和实验的角度来看,获取激光脉冲上升沿电离目标时形成的所谓前等离子体的特性是非常复杂的,而且这种激光诱导的从固态到皮秒时间尺度的过密等离子体转变的许多方面仍然是未决问题。一方面,激光驱动离子加速需要对预等离子体进行精确控制,因为加速过程的效率在很大程度上取决于脉冲相对论强度峰到达时的目标特性。另一方面,高效的激光烧蚀需要防止所谓的 "等离子体屏蔽"。通过捕捉相互作用初始阶段的动态,我们报告了前等离子体形成和演变的详细可视化过程。在强度为 1016 W/cm² 的激光上升沿期间,纳米级薄的类金刚石碳箔从固体转变为等离子体。单次近红外探针透射测量证明了密度超过 1023 cm-3(约为临界等离子体密度的 100 倍)的膨胀等离子体的亚皮秒动态。固态相互作用模型和动力学等离子体描述的互补性使我们能够深入了解初始电离、碰撞和膨胀的相互作用。
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引用次数: 0
Small and simple: next-generation miniaturized diffraction-based spectrometer with computational reconstruction algorithms 小而简:采用计算重建算法的下一代微型衍射光谱仪
Pub Date : 2024-05-07 DOI: 10.1038/s41377-024-01449-7
Markus Suta

An ultra-simple and miniaturized spectrometer using an arbitrarily shaped pinhole as diffraction element reconstructs a broadband spectrum from the information of diffraction of monochromatic radiation by clever computational reconstruction algorithms. This circumvents complex calibration procedures and paves the way to cost-effective on-chip spectrometers combining fast acquisition without significant loss in spectral resolution.

一种超简单微型光谱仪使用任意形状的针孔作为衍射元件,通过巧妙的计算重建算法,从单色辐射的衍射信息中重建宽带光谱。这就避免了复杂的校准程序,并为具有成本效益的片上光谱仪铺平了道路,使其能够在不明显降低光谱分辨率的情况下实现快速采集。
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引用次数: 0
A head-mounted photoacoustic fiberscope for hemodynamic imaging in mobile mice 用于移动小鼠血液动力学成像的头戴式光声纤维镜
Pub Date : 2024-05-07 DOI: 10.1038/s41377-024-01454-w
Xiaoyan Zheng, Shuai Na

A miniaturized photoacoustic fiberscope has been developed, featuring a lateral resolution of 9 microns and a lightweight design at 4.5 grams. Engineered to capture hemodynamic processes at single-blood-vessel resolution at a rate of 0.2 Hz, this device represents an advancement in head-mounted tools for exploring intricate brain activities in mobile animals.

我们开发出了一种微型光声纤维镜,其横向分辨率为 9 微米,设计轻巧,仅重 4.5 克。该设备能以 0.2 Hz 的速率捕捉单血管分辨率的血液动力学过程,是探索移动动物复杂脑部活动的头戴式工具的一大进步。
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引用次数: 0
Deep learning sheds new light on non-orthogonal optical multiplexing 深度学习为非正交光学复用带来新启示
Pub Date : 2024-05-06 DOI: 10.1038/s41377-024-01460-y
Zhengzhong Huang, Liangcai Cao

A deep neural network for non-orthogonal input channel encoding is proposed to recover speckle images through a multimode fiber. This novel approach could shed new light on the non-orthogonal optical multiplexing over a scattering medium.

本文提出了一种用于非正交输入信道编码的深度神经网络,以恢复通过多模光纤的斑点图像。这种新方法可为散射介质上的非正交光复用带来新的启示。
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引用次数: 0
Beyond the lab: a nanoimprint metalens array-based augmented reality 实验室之外:基于纳米压印金属阵列的增强现实技术
Pub Date : 2024-05-06 DOI: 10.1038/s41377-024-01429-x
Chi Li, Haoran Ren

A see-through augmented reality prototype has been developed based on an ultrathin nanoimprint metalens array, opening up a full-colour, video-rate, and low-cost 3D near-eye display.

基于超薄纳米压印金属膜阵列开发出了一种透视增强现实原型,开辟了一种全彩、视频速率高、成本低的三维近眼显示屏。
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引用次数: 0
Pure-high-even-order dispersion bound solitons complexes in ultra-fast fiber lasers 超高速光纤激光器中的纯高均阶色散约束孤子复合物
Pub Date : 2024-05-06 DOI: 10.1038/s41377-024-01451-z
Ying Han, Bo Gao, Honglin Wen, Chunyang Ma, Jiayu Huo, Yingying Li, Luyao Zhou, Qi Li, Ge Wu, Lie Liu

Temporal solitons have been the focus of much research due to their fascinating physical properties. These solitons can form bound states, which are fundamentally crucial modes in fiber laser and present striking analogies with their matter molecules counterparts, which means they have potential applications in large-capacity transmission and all-optical information storage. Although traditionally, second-order dispersion has been the dominant dispersion for conventional solitons, recent experimental and theoretical research has shown that pure-high-even-order dispersion (PHEOD) solitons with energy-width scaling can arise from the interaction of arbitrary negative-even-order dispersion and Kerr nonlinearity. Despite these advancements, research on the bound states of PHEOD solitons is currently non-existent. In this study, we obtained PHEOD bound solitons in a fiber laser using an intra-cavity spectral pulse shaper for high-order dispersion management. Specifically, we experimentally demonstrate the existence of PHEOD solitons and PHEOD bound solitons with pure-quartic, -sextic, -octic, and -decic dispersion. Numerical simulations corroborate these experimental observations. Furthermore, vibrating phase PHEOD bound soliton pairs, sliding phase PHEOD bound soliton pairs, and hybrid phase PHEOD bound tri-soliton are discovered and characterized. These results broaden the fundamental understanding of solitons and show the universality of multi-soliton patterns.

由于其迷人的物理特性,时域孤子一直是研究的焦点。这些孤子可以形成束缚态,而束缚态是光纤激光器的基本关键模式,与物质分子的对应模式有着惊人的相似之处,这意味着它们在大容量传输和全光信息存储方面有着潜在的应用前景。虽然传统上二阶色散一直是传统孤子的主要色散,但最近的实验和理论研究表明,具有能宽缩放的纯高均阶色散(PHEOD)孤子可以在任意负均阶色散和克尔非线性的相互作用下产生。尽管取得了这些进展,但目前还没有关于 PHEOD 孤子束缚态的研究。在这项研究中,我们利用腔内光谱脉冲整形器进行高阶色散管理,在光纤激光器中获得了 PHEOD 约束孤子。具体来说,我们通过实验证明了 PHEOD 孤子和 PHEOD 约束孤子在纯四方、六方、北极和十方色散情况下的存在。数值模拟证实了这些实验观察结果。此外,还发现并描述了振动相 PHEOD 结合孤子对、滑动相 PHEOD 结合孤子对和混合相 PHEOD 结合三孤子。这些结果拓宽了对孤子的基本认识,并显示了多孤子模式的普遍性。
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引用次数: 0
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Light-Science & Applications
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