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A monolithic microcavity laser with simultaneous upconversion and frequency-doubled lasing via crystal-in-glass engineering. 利用玻璃晶体技术实现上变频和倍频激光同步的单片微腔激光器。
Q1 OPTICS Pub Date : 2026-01-26 DOI: 10.1038/s41377-025-02162-9
Shengda Ye,Jianhao Chen,Jiayue He,Weiwei Chen,Xiongjian Huang,Xiaofeng Liu,Jianrong Qiu,Zhongmin Yang,Guoping Dong
This work demonstrates a novel crystal-in-glass composite structure for multifunctional micro-nano light sources in integrated photonics. Based on a Er3+/Yb3+-codoped glass-ceramic (GC) whispering gallery mode (WGM) microcavity incorporating Ba2TiGe2O8 (BTG) crystals, this microcavity enables dual-mode responses combining upconversion (UC) and frequency-doubled lasing. Made from a low-phonon-energy germanate glass matrix codoped with Er3+/Yb3+ for UC gain, the microcavity is crystallized to form BTG microcrystals for second harmonic generation (SHG). By leveraging the high-quality factor (Q ≈ 5.7 × 104) and small mode volume, we achieve green (550 nm) and red (660 nm) UC lasing in a 30-μm-diameter microcavity with low thresholds of 13.31 μW and 12.97 μW, respectively. Benefitted from the random quasi-phase-matching (RQPM) mechanism in BTG GC, the microcavity also demonstrates an ultrabroadband frequency-doubling response from 900 to 1200 nm. By combining tapered fiber near-field coupling and femtosecond free-space pumping, we achieve simultaneous output of green/red UC lasing and frequency-doubled lasing within a single microcavity. We believe this work offers insights into hybrid material design and cooperative optical field manipulation for tunable lasers and on-chip nonlinear photonic systems.
本研究展示了一种用于集成光子学中多功能微纳光源的新型玻璃晶体复合结构。该微腔基于含Ba2TiGe2O8 (BTG)晶体的Er3+/Yb3+共掺玻璃陶瓷(GC)窃窃廊模式(WGM)微腔,实现了结合上转换(UC)和倍频激光的双模响应。该微腔由低声子能量锗酸盐玻璃基体与Er3+/Yb3+共掺杂以获得UC增益,形成二次谐波产生(SHG)的BTG微晶。利用高质量因子(Q≈5.7 × 104)和小模体积,我们在直径为30 μm的微腔中实现了绿色(550 nm)和红色(660 nm)的UC激光,阈值分别为13.31 μW和12.97 μW。得益于BTG GC中的随机准相位匹配(RQPM)机制,该微腔在900 ~ 1200nm范围内表现出超宽带倍频响应。通过结合锥形光纤近场耦合和飞秒自由空间泵浦,我们实现了在单个微腔内同时输出绿/红UC激光和倍频激光。我们相信这项工作为可调谐激光器和片上非线性光子系统的混合材料设计和协同光场操纵提供了见解。
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引用次数: 0
Highly luminescent organic-inorganic hybrid antimony halide scintillators for real-time dynamic and 3D X-ray imaging 用于实时动态和三维x射线成像的高发光有机-无机杂化卤化锑闪烁体
Q1 OPTICS Pub Date : 2026-01-26 DOI: 10.1038/s41377-025-02152-x
Haixia Cui, Wanjiao Li, Qianxi Li, Shaolong Wang, Mingye Zhu, Yongjing Deng, Shujuan Liu, Qiang Zhao
Real-time dynamic and three-dimensional (3D) X-ray imaging are the most challenging types of X-ray imaging technology, placing more rigorous standards on scintillators. Lead-based (Pb 2+ ) organic-inorganic hybrid halide (OIHH) scintillators with high X-ray absorption coefficients have been demonstrated to exhibit excellent scintillation performance. However, their toxicity and instability hindered further development, and it is necessary to explore novel low-toxic metal-based OIHHs possessing excellent scintillation performance. Antimony-based (Sb 3+ ) OIHHs are not only environmentally friendly, but also show good stability compared to Pb 2+ -based OIHHs, which make them promising candidates as excellent scintillators. Currently, the understanding of Sb 3+ -based OIHH scintillators for X-ray detection and imaging is still in infancy and requires further exploration. Herein, we designed two Sb 3+ -based OIHH crystals of (BPP) 2 SbCl 5 (CP1) and (BPP) 2 SbCl 5 0.5 H 2 O (CP2), which have very similar crystal structures except the introduction of water molecules in CP2. Experimental and theoretical results reveal that CP2 has larger lattice distortion and smaller freedom of motion, which can promote the self-trapped excitons emissions. A flexible scintillator screen based on CP2 crystals was prepared and applied for real-time dynamic and 3D X-ray imaging, which is the first time for Sb 3+ -based OIHH scintillators and significantly broadens the potential of Sb 3+ -based OIHH scintillators.
实时动态和三维(3D) x射线成像是最具挑战性的x射线成像技术,对闪烁体提出了更严格的标准。铅基(pb2 +)有机-无机杂化卤化物(OIHH)闪烁体具有很高的x射线吸收系数,具有优异的闪烁性能。然而,它们的毒性和不稳定性阻碍了它们的进一步发展,因此有必要探索具有良好闪烁性能的新型低毒金属基oihs。与pb2 +基OIHHs相比,锑基(sb3 +) OIHHs不仅对环境友好,而且具有良好的稳定性,这使其成为极好的闪烁体。目前,对基于sb3 +的OIHH闪烁体用于x射线探测和成像的了解仍处于起步阶段,需要进一步探索。本文设计了(BPP) 2 SbCl 5 (CP1)和(BPP) 2 SbCl 5 0.5 h2o (CP2)两种基于sb3 +的OIHH晶体,除了CP2中引入了水分子外,它们的晶体结构非常相似。实验和理论结果表明,CP2具有较大的晶格畸变和较小的运动自由度,可以促进自俘获激子的发射。制备了一种基于CP2晶体的柔性闪烁体屏,并将其应用于实时动态和三维x射线成像,这是基于sb3 +的OIHH闪烁体的首次应用,大大拓宽了基于sb3 +的OIHH闪烁体的潜力。
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引用次数: 0
Sensitizing effect of lanthanide luminescence by Mo4+/Ag+ in double perovskites: great enhancement of near-infrared emission via wide range of excitation (250–850 nm) 双钙钛矿中Mo4+/Ag+对镧系发光的增敏效应:宽激发范围(250 ~ 850 nm)对近红外发射的显著增强
Q1 OPTICS Pub Date : 2026-01-26 DOI: 10.1038/s41377-025-02159-4
Yingsheng Wang, Peipei Dang, Zixun Zeng, Dongjie Liu, Guodong Zhang, Long Tian, Kai Li, Ping’an Ma, Yi Wei, Hongzhou Lian, Zhiyao Hou, Guogang Li, Jun Lin
Lead-free halide double perovskites (LFHDPs) have gained prominence as eco-friendly optoelectronic materials due to their structural stability and flexible tunability. Lanthanide (Ln 3+ ) ions have rich energy levels, which can endow LFHDP materials with emissions ranging from visible to near-infrared (NIR) region through the ion doping strategy. However, their NIR applications remain limited by narrowband emission and low photoluminescence quantum yield (PLQY) due to weak absorption cross-section. Herein, Cs 2 NaInCl 6 :Ln 3+ were successfully synthesized, and the problem of low absorption of Ln 3+ ions is effectively solved. Incorporating Mo 4+ /Ag + ions achieves a near-unity PLQY and expands the excitation spectrum across the full visible range and a small part of NIR region (250–850 nm). Mechanism analysis revealed synergistic energy transfer pathways involving self-trapping excitons and intermediate energy states of Mo 4+ ion, enhancing both photon absorption and PLQY. The universal applicability of this approach has been validated across Bi-based and multiple lanthanide ions (Ln: Ho, Er, Tm, Yb). These optimized materials demonstrate exceptional broadband emission characteristics suitable for multi-scenario NIR applications, including light-emitting-diodes (LEDs), night vision, imaging, anti-counterfeiting technologies. This co-doping methodology establishes a versatile framework for overcoming inherent limitations in Ln 3+ -activated materials, offering new possibilities for efficient NIR optoelectronic devices.
无铅卤化物双钙钛矿(lfhdp)由于其结构稳定性和柔性可调性而成为生态友好型光电材料。镧系(ln3 +)离子具有丰富的能级,可以通过离子掺杂策略赋予LFHDP材料从可见光到近红外(NIR)区域的发射。然而,它们的近红外应用仍然受到窄带发射和弱吸收截面导致的低光致发光量子产率(PLQY)的限制。本文成功地合成了c2naincl6: ln3 +,有效地解决了ln3 +离子的低吸收问题。加入mo4 + /Ag +离子实现了接近统一的PLQY,并扩展了整个可见光范围和一小部分近红外区域(250-850 nm)的激发光谱。机理分析揭示了mo4 +离子自俘获激子和中间能态的协同能量传递途径,增强了光子吸收和PLQY。这种方法的普遍适用性已经在铋基和多种镧系离子(Ln: Ho, Er, Tm, Yb)中得到验证。这些优化的材料具有卓越的宽带发射特性,适用于多场景近红外应用,包括发光二极管(led),夜视,成像,防伪技术。这种共掺杂方法为克服Ln 3+活化材料的固有局限性建立了一个通用的框架,为高效的近红外光电器件提供了新的可能性。
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引用次数: 0
Deterministic entanglement-assisted quantum communication over 20 km fiber channel 20公里光纤信道上的确定性纠缠辅助量子通信
Q1 OPTICS Pub Date : 2026-01-23 DOI: 10.1038/s41377-025-02173-6
Siyu Ren, Yanru Yan, Yalin Li, Chao Li, Dongmei Han, Xuezhi Zhu, Meihong Wang, Xiaolong Su
Entanglement-assisted quantum communication has substantial advantages in surpassing the power of classical communication by utilizing the entangled state. Up to now, most of entanglement-assisted quantum communications with dense coding are limited to the proof-of-principle experiments. Here, we experimentally demonstrate the deterministic entanglement-assisted quantum communication based on the continuous-variable (CV) entangled state over 20 km commercial fiber channels. We propose a new CV dense coding scheme with improved classical signals and show that the transmission distance of CV entanglement-assisted quantum communication can be extended compared with that using fixed classical signals. By applying the frequency division multiplexing technique, we simultaneously decode 10 classical signals submerged in the shot noise of coherent state with the help of CV entangled state after the transmission through a 20.121 km fiber channel. The results show that around 3 times of channel capacity in classical communication with coherent state are achieved in the CV entanglement-assisted communication with the frequency division multiplexing technique. Our result takes a crucial step towards realizing the deterministic metropolitan entanglement-assisted quantum communication in practical quantum channels.
纠缠辅助量子通信在利用纠缠态超越经典通信的能力方面具有实质性的优势。目前,密集编码的纠缠辅助量子通信大多局限于原理验证实验。在此,我们通过实验证明了基于连续变量(CV)纠缠态的确定性纠缠辅助量子通信在20公里商用光纤信道上的实现。我们提出了一种改进经典信号的CV密集编码方案,并证明了与使用固定经典信号相比,CV纠缠辅助量子通信的传输距离可以得到延长。采用频分复用技术,利用CV纠缠态对淹没在相干态散粒噪声中的10个经典信号进行了同步解码,传输距离为20.121 km。结果表明,利用频分复用技术实现的CV纠缠辅助通信的信道容量是相干态经典通信的3倍左右。我们的研究结果为在实际量子信道中实现确定性大都市纠缠辅助量子通信迈出了关键的一步。
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引用次数: 0
III-Nitrides empower miniaturized spectral imager in ultraviolet. 氮化物增强了小型化紫外光谱成像仪的功能。
Q1 OPTICS Pub Date : 2026-01-23 DOI: 10.1038/s41377-025-02132-1
Yuji Zhao,Tao Li,Boon Ooi
A high-performance miniaturized on-chip spectral imager operating in the ultraviolet region is demonstrated based on an AlGaN/GaN cascaded photodiode array. This work extends spectral imaging into the ultraviolet regimes by leveraging the mature III-nitride technologies and establishes a scalable pathway toward massive production of compact, high-resolution spectral imagers.
介绍了一种基于AlGaN/GaN级联光电二极管阵列的高性能小型化紫外光谱成像仪。这项工作通过利用成熟的iii -氮化物技术将光谱成像扩展到紫外线区域,并为大规模生产紧凑、高分辨率的光谱成像仪建立了可扩展的途径。
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引用次数: 0
Spectral-acoustic-coordinated astigmatic metalens for wide field-of-view and high spatiotemporal resolution 3D imaging 用于宽视场和高时空分辨率三维成像的光谱-声学协调像散超透镜
Q1 OPTICS Pub Date : 2026-01-23 DOI: 10.1038/s41377-025-02180-7
Shujian Gong, Yinghui Guo, Xiaoyin Li, Mingbo Pu, Peng Tian, Qi Zhang, Lianwei Chen, Wenyi Ye, Heping Liu, Fei Zhang, Mingfeng Xu, Xiangang Luo
Metasurface-based light detection and ranging (LiDAR) is essential for high spatiotemporal resolution three-dimensional (3D) imaging in robotic and autonomous systems. Recent advances in inertia-free scanning techniques—such as acousto-optic and spectral scanning—have propelled the field forward. Nevertheless, key spatiotemporal metrics, including point acquisition rate (PAR), field-of-view (FOV), and imaging resolution, remain fundamentally constrained. These challenges are particularly acute in dual-axis LiDARs, where inter-axis rate mismatch and beam astigmatism degrade temporal and spatial resolution, respectively. Here, we present a wide-FOV, high spatiotemporal resolution LiDAR architecture with astigmatic metalens (AML) coordinated spectral-acousto-optic scanning. Consequently, a frame-wise point acquisition rate (FPAR) of 36.6 MHz (∼5-fold improvement over existing reports) and a wide FOV of 102° are simultaneously achieved. This breakthrough redefines LiDAR’s potential for ultra-high-speed, high-precision perception, enhancing applications such as autonomous driving with improved obstacle detection and safety at high speeds.
基于超表面的光探测和测距(LiDAR)对于机器人和自主系统中的高时空分辨率三维(3D)成像至关重要。无惯性扫描技术的最新进展,如声光扫描和光谱扫描,推动了该领域的发展。然而,关键的时空指标,包括点采集率(PAR)、视场(FOV)和成像分辨率仍然受到基本限制。这些挑战在双轴激光雷达中尤其严重,轴间速率不匹配和光束散光分别降低了时间和空间分辨率。在这里,我们提出了一种宽视场、高时空分辨率的激光雷达架构,具有像散超透镜(AML)协调的光谱-声光扫描。因此,同时实现了36.6 MHz的逐帧点采集率(FPAR)(比现有报告提高约5倍)和102°的宽视场。这一突破重新定义了激光雷达在超高速、高精度感知方面的潜力,增强了自动驾驶等应用,提高了高速障碍物检测和安全性。
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引用次数: 0
Robust ultrahigh-Q resonances in tetramer metasurfaces through centroid symmetry protection and area conservation 通过质心对称保护和面积守恒实现四聚体超表面的鲁棒超高q共振
Q1 OPTICS Pub Date : 2026-01-23 DOI: 10.1038/s41377-025-02164-7
Chaobiao Zhou, Rong Jin, Haoxuan He, Jing Huang, Guanhai Li, Lujun Huang
Ultrahigh-Q optical resonances are the cornerstone of next-generation nanophotonic technologies, but their simultaneous realization of robustness and on-chip practicality remains a significant challenge. In this work, we present tetramer composite metasurfaces capable of supporting two distinct classes of ultrahigh-Q resonances: centroid symmetry-protected bound states in the continuum (SP-BICs) and area-conserved guided-mode resonances (GMRs). By employing a four-hole supercell design, we demonstrate that centering each hole within its subcell preserves C 4v symmetry, thereby enabling SP-BICs. Controlled lateral displacement transforms them into quasi-BICs with Q > 10⁶. Independently, enforcing diagonal-hole area conservation within the super unit cell generates degenerate GMRs with Q > 10⁸, which exhibit remarkable stability across a broad wave vector range. Breaking this area conservation splits the GMRs into paired ultrahigh-Q resonances, while adjusting the center-to-center distance of air holes lifts their degeneracy. Experimentally, we validate both resonance types using silicon photonic crystal slabs, achieving measured Q-factors exceeding 10,000, with a maximum value of 43,700. Such ultrahigh-Q composite-metasurfaces provide a versatile platform of enhancing light-matter interactions.
超高q光共振是下一代纳米光子技术的基石,但同时实现鲁棒性和片上实用性仍然是一个重大挑战。在这项工作中,我们提出了能够支持两种不同类型的超高q共振的四聚体复合超表面:连续介质中质心对称保护的束缚态(sp - bic)和面积守恒的导模共振(GMRs)。通过采用四孔超级单体设计,我们证明每个孔在其子胞内居中保持c4v对称性,从而实现sp - bic。控制侧向位移将其转化为具有Q >; 10 26的准bic。独立地,在超单元胞内强制对角孔面积守恒产生Q >; 10⁸的简并gmr,在宽波矢量范围内表现出显著的稳定性。打破这一区域守恒将gmr分裂成成对的超高q共振,而调整气孔中心到中心的距离可以提高它们的简并度。实验上,我们使用硅光子晶体板验证了这两种共振类型,实现了超过10,000的测量q因子,最大值为43,700。这种超高q复合超表面提供了一个增强光-物质相互作用的通用平台。
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引用次数: 0
Experimental demonstration of spatiotemporal analog computation in ultrafast optics. 超快光学中时空模拟计算的实验论证。
Q1 OPTICS Pub Date : 2026-01-22 DOI: 10.1038/s41377-025-02109-0
Junyi Huang,Dong Zhao,Jixuan Shi,Hongliang Zhang,Hengyi Wang,Fang-Wen Sun,Qiwen Zhan,Shiyao Zhu,Kun Huang,Zhichao Ruan
It is intractable to perform information processing and computation on single ultrafast optical pulses, within picoseconds or even femtoseconds. Here, we experimentally demonstrate an optical spatiotemporal differentiator, a mirror-symmetry-breaking dielectric metagrating, which performs analog computations of both spatial and temporal differentiations on single ultrafast optical wavepackets. The spatiotemporal differentiator is designed with a transfer function with linear dependence on spatial wavevector and temporal frequency and fabricated by using a double-exposure E-beam lithography process. We achieve the first-order spatiotemporal differentiation with experimental resolutions of approximately 14 μm (in space) and 260 fs (in time). Furthermore, we report a parabolic relationship between the transverse velocity of a front-tilted photonic wavepacket and the normalized intensity of its first-order spatiotemporal-differentiation wavepacket. This relationship allows direct measurement of the transverse velocity using only the normalized intensity, fundamentally simplifying velocity detection. These capabilities of optical spatiotemporal computation endow emerging space-time optics with fundamental computation blocks.
单超快光脉冲在皮秒甚至飞秒内进行信息处理和计算是非常困难的。在这里,我们通过实验展示了一种光学时空微分器,一种镜像对称破缺的介电介介,它可以对单个超快光波包进行空间和时间微分器的模拟计算。采用双曝光电子束光刻工艺制作时空微分器,并设计了与空间波矢量和时间频率线性相关的传递函数。我们以大约14 μm(空间)和260 fs(时间)的实验分辨率实现了一阶时空分异。此外,我们报道了前倾斜光子波包的横向速度与其一阶时空分异波包的归一化强度之间的抛物线关系。这种关系允许仅使用归一化强度直接测量横向速度,从根本上简化了速度检测。这些光学时空计算能力为新兴的空时光学提供了基本的计算模块。
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引用次数: 0
Generation of vectorial generalized vortex array with metasurfaces. 具有超表面的矢量广义涡阵的生成。
Q1 OPTICS Pub Date : 2026-01-22 DOI: 10.1038/s41377-025-02102-7
Qingsong Yao,Zile Li,Guoxing Zheng
The ability to create complex three-dimensional structures of light is extremely challenging. Now, a technique combining Dammann optimization with metasurfaces has been developed, enabling control over all parameters, including polarization, phase, angular momentum, and spatial modes. The generation of three-dimensional generalized vortex beams can open new horizons for their applications in photonics.
创造复杂的三维光结构的能力是极具挑战性的。现在,一种将Dammann优化与超表面相结合的技术已经开发出来,可以控制所有参数,包括偏振、相位、角动量和空间模式。三维广义涡旋光束的产生为其在光子学中的应用开辟了新的领域。
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引用次数: 0
Dispersion engineering by rotational symmetry breaking in an optical microcavity. 光学微腔中旋转对称破缺的色散工程。
Q1 OPTICS Pub Date : 2026-01-22 DOI: 10.1038/s41377-025-02169-2
Jian-Zheng Ren,Li-Jie Li,Rui-Qi Zhang,Zhi-Yan Wang,Qi-Tao Cao,Yun-Feng Xiao
Dispersion engineering is pivotal for nonlinear optics, yet it often faces challenges posed by material and structural limitations. Here, we establish rotational symmetry breaking as the guiding principle for dispersion engineering in optical microcavities. Through boundary deformation, multi-branch global dispersion emerges in island modes, and local dispersion is controlled via resonance-assisted tunneling between quasi-whispering gallery modes. Enabled by the global dispersion, the optical parametric oscillation is predicted in blue-violet light spectrum with high efficiency (>55%) and large frequency separation (>180 THz). Using the local dispersion engineering, the doubly-resonant enhancement of second-harmonic generation is regulated by the resonance-assisted tunneling.
色散工程是非线性光学研究的关键,但由于材料和结构的限制,色散工程经常面临挑战。在此,我们建立了旋转对称破缺作为光学微腔色散工程的指导原则。通过边界变形,在孤岛模式中产生多分支的全局色散,在准耳语通道模式之间通过共振辅助隧道控制局部色散。在全局色散的作用下,在蓝紫光光谱中预测了高效率(>55%)和大频率分离(>180 THz)的光学参量振荡。利用局域色散工程,利用共振辅助隧穿调节二次谐波产生的双共振增强。
{"title":"Dispersion engineering by rotational symmetry breaking in an optical microcavity.","authors":"Jian-Zheng Ren,Li-Jie Li,Rui-Qi Zhang,Zhi-Yan Wang,Qi-Tao Cao,Yun-Feng Xiao","doi":"10.1038/s41377-025-02169-2","DOIUrl":"https://doi.org/10.1038/s41377-025-02169-2","url":null,"abstract":"Dispersion engineering is pivotal for nonlinear optics, yet it often faces challenges posed by material and structural limitations. Here, we establish rotational symmetry breaking as the guiding principle for dispersion engineering in optical microcavities. Through boundary deformation, multi-branch global dispersion emerges in island modes, and local dispersion is controlled via resonance-assisted tunneling between quasi-whispering gallery modes. Enabled by the global dispersion, the optical parametric oscillation is predicted in blue-violet light spectrum with high efficiency (>55%) and large frequency separation (>180 THz). Using the local dispersion engineering, the doubly-resonant enhancement of second-harmonic generation is regulated by the resonance-assisted tunneling.","PeriodicalId":18069,"journal":{"name":"Light-Science & Applications","volume":"5 1","pages":"81"},"PeriodicalIF":0.0,"publicationDate":"2026-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146015312","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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Light-Science & Applications
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