Light-Science & Applications最新文献

Hanbury-Brown and Twiss (HBT) effect is the foundation for stellar intensity interferometry. However, it is a phase insensitive two-photon interference effect. Here we extend the HBT interferometer by mixing intensity-matched reference fields with the input fields before intensity correlation measurement. With the freely available coherent state serving as the reference field, we experimentally demonstrate the phase sensitive two-photon interference effect when the input fields are thermal fields in either continuous wave or non-stationary pulsed wave and measure the complete complex second-order coherence function of the input fields without bringing them together from separate locations. Moreover, we discuss how to improve the signal level by using the more realistic continuous wave broadband anti-bunched light fields as the reference field. Our investigations pave the way for developing new technology of remote sensing and interferometric imaging with applications in long baseline high-resolution astronomy.

Coherent broadband light generation has attracted massive attention due to its numerous applications ranging from metrology, sensing, and imaging to communication. In general, spectral broadening is realized via third-order and higher-order nonlinear optical processes (e.g., self-phase modulation, Raman transition, four-wave mixing, multiwave mixing), which are typically weak and thus require a long interaction length and the phase matching condition to enhance the efficient nonlinear light-matter interaction for broad-spectrum generation. Here, for the first time, we report octave-spanning coherent light generation at the nanometer scale enabled by a phase-matching-free frequency down-conversion process. Up to octave-spanning coherent light generation with a −40dB spectral width covering from ~565 to 1906 nm is demonstrated in discreate manner via difference-frequency generation, a second-order nonlinear process in gallium selenide and niobium oxide diiodide crystals at the 100-nanometer scale. Compared with conventional coherent broadband light sources based on bulk materials, our demonstration is ~5 orders of magnitude thinner and requires ~3 orders of magnitude lower excitation power. Our results open a new way to possibly create compact, versatile and integrated ultra-broadband light sources.

We propose and demonstrate a data-driven plasmonic metascreen that efficiently absorbs incident light over a wide spectral range in an ultra-thin silicon film. By embedding a double-nanoring silver array within a 20 nm ultrathin amorphous silicon (a-Si) layer, we achieve a significant enhancement of light absorption. This enhancement arises from the interaction between the resonant cavity modes and localized plasmonic modes, requiring precise tuning of plasmon resonances to match the absorption region of the silicon active layer. To facilitate the device design and improve light absorption without increasing the thickness of the active layer, we develop a deep learning framework, which learns to map from the absorption spectra to the design space. This inverse design strategy helps to tune the absorption for selective spectral functionalities. Our optimized design surpasses the bare silicon planar device, exhibiting a remarkable enhancement of over 100%. Experimental validation confirms the broadband enhancement of light absorption in the proposed configuration. The proposed metascreen absorber holds great potential for light harvesting applications and may be leveraged to improve the light conversion efficiency of ultra-thin silicon solar cells, photodetectors, and optical filters.

Graphene has unique properties paving the way for groundbreaking future applications. Its large optical nonlinearity and ease of integration in devices notably makes it an ideal candidate to become a key component for all-optical switching and frequency conversion applications. In the terahertz (THz) region, various approaches have been independently demonstrated to optimize the nonlinear effects in graphene, addressing a critical limitation arising from the atomically thin interaction length. Here, we demonstrate sample architectures that combine strategies to enhance THz nonlinearities in graphene-based structures. We achieve this by increasing the interaction length through a multilayered design, controlling carrier density with an electrical gate, and modulating the THz field spatial distribution with a metallic metasurface substrate. Our study specifically investigates third harmonic generation (THG) using a table-top high-field THz source. We measure THG enhancement factors exceeding thirty and propose architectures capable of achieving a two-order-of-magnitude increase. These findings underscore the potential of engineered graphene-based structures in advancing THz frequency conversion technologies for signal processing and wireless communication applications.

Exceptional points (EPs) have been extensively explored in mechanical, acoustic, plasmonic, and photonic systems. However, little is known about the role of EPs in tailoring the dynamic tunability of optical devices. A specific type of EPs known as chiral EPs has recently attracted much attention for controlling the flow of light and for building sensors with better responsivity. A recently demonstrated route to chiral EPs via lithographically defined symmetric Mie scatterers on the rim of resonators has not only provided the much-needed mechanical stability for studying chiral EPs, but also helped reduce losses originating from nanofabrication imperfections, facilitating the in-situ study of chiral EPs and their contribution to the dynamics and tunability of resonators. Here, we use asymmetric Mie scatterers to break the rotational symmetry of a microresonator, to demonstrate deterministic thermal tuning across a chiral EP, and to demonstrate EP-mediated chiral optical nonlinear response and efficient electro-optic tuning. Our results indicate asymmetric electro-optic modulation with up to 17 dB contrast at GHz and CMOS-compatible voltage levels. Such wafer-scale nano-manufacturing of chiral electro-optic modulators and the chiral EP-tailored tunning may facilitate new micro-resonator functionalities in quantum information processing, electromagnetic wave control, and optical interconnects.

A unique optoelectronic synaptic device has been developed, leveraging the negative photoconductance property of a single-crystal material system called Cs₂CoCl₄. This device exhibits a simultaneous volatile resistive switching response and sensitivity to optical stimuli, positioning Cs₂CoCl₄ as a promising candidate for optically enhanced neuromorphic applications.

Nanostructured dielectric metasurfaces offer unprecedented opportunities to control light-matter momentum exchange, and thereby the forces and torques that light can exert on matter. Here we introduce optical metasurfaces as components of ultracompact untethered microscopic metaspinners capable of efficient light-induced rotation in a liquid environment. Illuminated by weakly focused light, a metaspinner generates torque via photon recoil through the metasurfaces’ ability to bend light towards high angles despite their sub-wavelength thickness, thereby creating orbital angular momentum. We find that a metaspinner is subject to an anomalous transverse lateral optical gradient force that acts in concert with the classical gradient force. Consequently, when two or more metaspinners are trapped together in a laser beam, they collectively orbit the optical axis in the opposite direction to their spinning motion, in stark contrast to rotors coupled through hydrodynamic or mechanical interactions. The metaspinners delineated herein not only serve to illustrate the vast possibilities of utilizing optical metasurfaces for fundamental exploration of optical torques, but they also represent potential building-blocks of artificial active matter systems, light-driven micromachinery, and general-purpose optomechanical devices.

Non-Hermitian topological photonics plays a key role in bridging topological matter with gain and loss engineering in optics. Here we report the experimental observation of the break of chiral currents in a Hall ladder from the non-Hermiticity by constructing synthetic frequency dimension in two rings, where currents on both legs of the ladder co-propagate in the same direction. The origin of such phenomena is resulted from the interplay between the effective magnetic flux and the on-site gain and loss. Such non-Hermitian co-propagating currents exhibit characteristics of unidirectional frequency conversion in both rings, and moreover, different from the counterpart in Hermitian systems, can provide a method to probe the signatures of the non-Hermitian skin effect from steady-state bulk dynamics. Our model is further extended to models including next-nearest-neighbor couplings, pointing to a way for observing the non-Hermitian signature with higher winding number, and provides a new control knob for light manipulation with the topological dissipation engineering.

Common-signal-induced synchronization of semiconductor lasers have promising applications in physical-layer secure transmission with high speed and compatibility with the current fiber communication. Here, we propose an ultra-long-distance laser synchronization scheme by utilizing random digital optical communication signal as the common drive signal. By utilizing the long-haul optical coherent communication techniques, high-fidelity fiber transmission of the digital drive can be achieved and thus ultra-long-distance synchronization is expected. Experiments were implemented with distributed feedback lasers injected by a random-digital phase-modulated drive light. Results show that high-quality synchronization can be achieved as the drive signal rate is larger than the laser relaxation frequency and the transmission bit error ratio is below a critical value. Chaos synchronization over 8191-km fiber transmission was experimentally achieved. Compared to traditional common-signal-induced synchronization using analog drive signal such as chaos, the distance is increased by 8 times, and complicated hardware devices for channel impairment compensation are no longer required. In addition, the proposed method does not sacrifice communication capacity like traditional methods which need a channel to transmit analog drive signal. It is therefore believed that this common-digital-signal induced laser synchronization paves a way for secure backbone and submarine transmission.

Perovskite quantum dots (PQDs) show promise in light-emitting diodes (LEDs). However, near-infrared (NIR) LEDs employing PQDs exhibit inferior external quantum efficiency related to the PQD emitting in the visible range. One fundamental issue arises from the PQDs dynamic surface: the ligand loss and ions migration to the interfacial sites serve as quenching centers, resulting in trap-assisted recombination and carrier loss. In this work, we developed a chemical treatment strategy to eliminate the interface quenching sites and achieve high carrier utilization. We employ a bidentate and liquid agent (Formamidine thiocyanate, FASCN) with tight binding to suppress the ligand loss and the formation of interfacial quenching sites: the FASCN-treated films exhibit fourfold higher binding energy than the original oleate ligands. Furthermore, the short ligands (carbon chain <3) enable the treated films to show eightfold higher conductivity; and the liquid characteristics of FASCN avoid the use of high polar solvents and guarantee better passivation. The high conductivity ensures efficient charge transportation, enabling PQD-based NIR-LEDs to have a record-low voltage of 1.6 V at 776 nm. Furthermore, the champion EQE of the treated LEDs is ~23%: this is twofold higher than the control, and represents the highest among reported PQD-based NIR-LEDs.