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New insights into plasmonic hot-electron dynamics 对等离子体热电子动力学的新认识
Q1 OPTICS Pub Date : 2024-09-10 DOI: 10.1038/s41377-024-01594-z
Dangyuan Lei, Dong Su, Stefan A. Maier
Recent advances in understanding the intricate hot-electron dynamics in plasmonic nanostructures enable efficient hot-carrier generation, transport, and manipulation, driving technological innovations in photodetection, solar cells, photocatalysis, and ultrafast nanophotonics.
近来,人们对等离子纳米结构中错综复杂的热电子动力学的理解取得了进展,从而能够高效地生成、传输和操纵热载流子,推动了光探测、太阳能电池、光催化和超快纳米光子学领域的技术创新。
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引用次数: 0
Broadband infrared imaging governed by guided-mode resonance in dielectric metasurfaces 介电元表面导模共振控制的宽带红外成像
Q1 OPTICS Pub Date : 2024-09-10 DOI: 10.1038/s41377-024-01535-w
Ze Zheng, Daria Smirnova, Gabriel Sanderson, Ying Cuifeng, Demosthenes C. Koutsogeorgis, Lujun Huang, Zixi Liu, Rupert Oulton, Arman Yousefi, Andrey E. Miroshnichenko, Dragomir N. Neshev, Mary O’Neill, Mohsen Rahmani, Lei Xu

Nonlinear metasurfaces have experienced rapid growth recently due to their potential in various applications, including infrared imaging and spectroscopy. However, due to the low conversion efficiencies of metasurfaces, several strategies have been adopted to enhance their performances, including employing resonances at signal or nonlinear emission wavelengths. This strategy results in a narrow operational band of the nonlinear metasurfaces, which has bottlenecked many applications, including nonlinear holography, image encoding, and nonlinear metalenses. Here, we overcome this issue by introducing a new nonlinear imaging platform utilizing a pump beam to enhance signal conversion through four-wave mixing (FWM), whereby the metasurface is resonant at the pump wavelength rather than the signal or nonlinear emissions. As a result, we demonstrate broadband nonlinear imaging for arbitrary objects using metasurfaces. A silicon disk-on-slab metasurface is introduced with an excitable guided-mode resonance at the pump wavelength. This enabled direct conversion of a broad IR image ranging from >1000 to 4000 nm into visible. Importantly, adopting FWM substantially reduces the dependence on high-power signal inputs or resonant features at the signal beam of nonlinear imaging by utilizing the quadratic relationship between the pump beam intensity and the signal conversion efficiency. Our results, therefore, unlock the potential for broadband infrared imaging capabilities with metasurfaces, making a promising advancement for next-generation all-optical infrared imaging techniques with chip-scale photonic devices.

非线性元表面因其在红外成像和光谱学等各种应用中的潜力,最近经历了快速发展。然而,由于元表面的转换效率较低,人们采用了多种策略来提高其性能,包括在信号波长或非线性发射波长上采用共振。这种策略导致非线性超表面的工作频带较窄,从而制约了许多应用,包括非线性全息、图像编码和非线性金属透镜。在这里,我们引入了一种新的非线性成像平台,利用泵浦光束通过四波混合(FWM)增强信号转换,从而使元表面在泵浦波长而非信号或非线性发射处产生共振,从而克服了这一问题。因此,我们利用元表面演示了任意物体的宽带非线性成像。我们在泵浦波长处引入了可激发导模共振的硅片盘元表面。这样就能将范围从 1000 纳米到 4000 纳米的宽红外图像直接转换为可见光图像。重要的是,通过利用泵浦光束强度与信号转换效率之间的二次关系,采用 FWM 技术大大降低了非线性成像对高功率信号输入或信号光束共振特征的依赖。因此,我们的研究结果释放了利用超表面实现宽带红外成像功能的潜力,为利用芯片级光子器件实现下一代全光红外成像技术带来了希望。
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引用次数: 0
Visualizing mitochondrial dynamics at the nanoscale 纳米级线粒体动态可视化
Q1 OPTICS Pub Date : 2024-09-09 DOI: 10.1038/s41377-024-01582-3
Till Stephan, Peter Ilgen, Stefan Jakobs

The study of mitochondria is a formidable challenge for super-resolution microscopy due to their dynamic nature and complex membrane architecture. In this issue, Ren et al. introduce HBmito Crimson, a fluorogenic and photostable mitochondrial probe for STED microscopy and investigate how mitochondrial dynamics influence the spatial organization of mitochondrial DNA.

由于线粒体的动态性质和复杂的膜结构,对其进行研究是超分辨率显微镜的一项艰巨挑战。在本期中,Ren 等人介绍了用于 STED 显微镜的线粒体探针 HBmito Crimson,它是一种荧光性和光稳性线粒体探针,研究了线粒体动力学如何影响线粒体 DNA 的空间组织。
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引用次数: 0
Quasicrystal metasurface for optical holography and diffraction 用于光学全息和衍射的准晶体元表面
Q1 OPTICS Pub Date : 2024-09-09 DOI: 10.1038/s41377-024-01578-z
Xin Wen, Zixian Hu, Heng Wang, Yu Chen, Qichang Ma, Guixin Li

Quasicrystal metasurfaces, a kind of two-dimensional artificial optical materials with subwavelength meta-atoms arranged in quasi-periodic tiling schemes, have attracted extensive attentions due to their novel optical properties. In a recent work, a dual-functional quasicrystal metasurface, which can be used to simultaneously generate the diffraction pattern and holographic image, is experimentally demonstrated. The proposed method expands the manipulation dimensions for multi-functional quasicrystal metasurfaces and may have important applications in microscopy, optical information processing, optical encryption, etc.

准晶元表面是一种具有亚波长元原子的二维人工光学材料,以准周期平铺方式排列,因其新颖的光学特性而受到广泛关注。在最近的一项研究中,实验证明了一种可同时生成衍射图样和全息图像的双功能准晶元表面。所提出的方法拓展了多功能准晶元表面的操作维度,可能在显微镜、光学信息处理、光学加密等领域有重要应用。
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引用次数: 0
Photon shifting and trapping in perovskite solar cells for improved efficiency and stability 在过氧化物太阳能电池中进行光子转移和捕获以提高效率和稳定性
Q1 OPTICS Pub Date : 2024-09-05 DOI: 10.1038/s41377-024-01559-2
Sirazul Haque, Miguel Alexandre, António T. Vicente, Kezheng Li, Christian S. Schuster, Sui Yang, Hugo Águas, Rodrigo Martins, Rute A. S. Ferreira, Manuel J. Mendes

Advanced light management techniques can enhance the sunlight absorption of perovskite solar cells (PSCs). When located at the front, they may act as a UV barrier, which is paramount for protecting the perovskite layer against UV-enabled degradation. Although it was recently shown that photonic structures such as Escher-like patterns could approach the theoretical Lambertian-limit of light trapping, it remains challenging to also implement UV protection properties for these diffractive structures while maintaining broadband absorption gains. Here, we propose a checkerboard (CB) tile pattern with designated UV photon conversion capability. Through a combined optical and electrical modeling approach, this photonic structure can increase photocurrent and power conversion efficiency in ultrathin PSCs by 25.9% and 28.2%, respectively. We further introduce a luminescent down-shifting encapsulant that converts the UV irradiation into Visible photons matching the solar cell absorption spectrum. To this end, experimentally obtained absorption and emission profiles of state-of-the-art down-shifting materials (i.e., lanthanide-based organic-inorganic hybrids) are used to predict potential gains from harnessing the UV energy. We demonstrate that at least 94% of the impinging UV radiation can be effectively converted into the Visible spectral range. Photonic protection from high-energy photons contributes to the market deployment of perovskite solar cell technology, and may become crucial for Space applications under AM0 illumination. By combining light trapping with luminescent downshifting layers, this work unravels a potential photonic solution to overcome UV degradation in PSCs while circumventing optical losses in ultrathin cells, thus improving both performance and stability.

先进的光管理技术可以提高过氧化物太阳能电池(PSC)对阳光的吸收能力。当位于前部时,它们可以起到紫外线屏障的作用,这对于保护包晶石层防止紫外线导致的降解至关重要。虽然最近有研究表明,类似埃舍尔图案的光子结构可以接近理论上的朗伯极限光捕获,但要在保持宽带吸收增益的同时为这些衍射结构实现紫外线防护特性,仍然具有挑战性。在此,我们提出了一种具有指定紫外线光子转换能力的棋盘格(CB)瓦片图案。通过结合光学和电学建模方法,这种光子结构可将超薄 PSC 的光电流和功率转换效率分别提高 25.9% 和 28.2%。我们进一步引入了一种发光下移封装剂,它能将紫外线辐照转化为与太阳能电池吸收光谱相匹配的可见光光子。为此,我们利用从实验中获得的最先进下变换材料(即镧系有机-无机混合材料)的吸收和发射曲线来预测利用紫外线能量的潜在收益。我们证明,至少 94% 的紫外线辐射可以有效地转换到可见光谱范围。对高能光子的光子保护有助于包晶体太阳能电池技术的市场部署,并可能成为 AM0 照明下太空应用的关键。通过将光捕获与发光下移层相结合,这项研究揭示了一种潜在的光子解决方案,可克服聚光晶体太阳能电池中的紫外线衰减,同时规避超薄电池中的光学损耗,从而提高性能和稳定性。
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引用次数: 0
Lens-free on-chip 3D microscopy based on wavelength-scanning Fourier ptychographic diffraction tomography 基于波长扫描傅立叶平片衍射层析成像技术的无透镜片上三维显微技术
Q1 OPTICS Pub Date : 2024-09-05 DOI: 10.1038/s41377-024-01568-1
Xuejuan Wu, Ning Zhou, Yang Chen, Jiasong Sun, Linpeng Lu, Qian Chen, Chao Zuo

Lens-free on-chip microscopy is a powerful and promising high-throughput computational microscopy technique due to its unique advantage of creating high-resolution images across the full field-of-view (FOV) of the imaging sensor. Nevertheless, most current lens-free microscopy methods have been designed for imaging only two-dimensional thin samples. Lens-free on-chip tomography (LFOCT) with a uniform resolution across the entire FOV and at a subpixel level remains a critical challenge. In this paper, we demonstrated a new LFOCT technique and associated imaging platform based on wavelength scanning Fourier ptychographic diffraction tomography (wsFPDT). Instead of using angularly-variable illuminations, in wsFPDT, the sample is illuminated by on-axis wavelength-variable illuminations, ranging from 430 to 1200 nm. The corresponding under-sampled diffraction patterns are recorded, and then an iterative ptychographic reconstruction procedure is applied to fill the spectrum of the three-dimensional (3D) scattering potential to recover the sample’s 3D refractive index (RI) distribution. The wavelength-scanning scheme not only eliminates the need for mechanical motion during image acquisition and precise registration of the raw images but secures a quasi-uniform, pixel-super-resolved imaging resolution across the entire imaging FOV. With wsFPDT, we demonstrate the high-throughput, billion-voxel 3D tomographic imaging results with a half-pitch lateral resolution of 775 nm and an axial resolution of 5.43 μm across a large FOV of 29.85 mm2 and an imaging depth of >200 μm. The effectiveness of the proposed method was demonstrated by imaging various types of samples, including micro-polystyrene beads, diatoms, and mouse mononuclear macrophage cells. The unique capability to reveal quantitative morphological properties, such as area, volume, and sphericity index of single cell over large cell populations makes wsFPDT a powerful quantitative and label-free tool for high-throughput biological applications.

无透镜芯片显微镜是一种功能强大、前景广阔的高通量计算显微镜技术,因为它具有在成像传感器的全视场(FOV)范围内创建高分辨率图像的独特优势。然而,目前大多数无透镜显微镜方法都是为二维薄样品成像而设计的。无透镜片上断层成像(LFOCT)在整个视场(FOV)和亚像素水平上具有均匀的分辨率,这仍然是一个严峻的挑战。在本文中,我们展示了一种基于波长扫描傅立叶平片衍射断层扫描(wsFPDT)的新型 LFOCT 技术和相关成像平台。wsFPDT 不使用角度可变的光源,而是使用轴向波长可变的光源(波长范围从 430 纳米到 1200 纳米)照射样品。记录相应的欠采样衍射图样,然后采用迭代式分色重建程序来填充三维(3D)散射势的光谱,从而恢复样品的三维折射率(RI)分布。波长扫描方案不仅消除了图像采集和原始图像精确配准过程中的机械运动需求,还确保了整个成像 FOV 范围内的准均匀、像素超分辨成像分辨率。利用 wsFPDT,我们展示了高通量、十亿体素三维断层成像结果,在 29.85 平方毫米的大视野和 200 微米的成像深度内,半间距横向分辨率为 775 纳米,轴向分辨率为 5.43 微米。通过对各种类型的样品(包括微聚苯乙烯珠、硅藻和小鼠单核巨噬细胞)进行成像,证明了该方法的有效性。wsFPDT 能够揭示单细胞在大量细胞群中的定量形态特性,如面积、体积和球形度指数,这种独特的能力使其成为高通量生物应用中一种强大的定量和无标记工具。
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引用次数: 0
Aberration-robust monocular passive depth sensing using a meta-imaging camera 使用元成像相机进行抗像差单目被动深度传感
Q1 OPTICS Pub Date : 2024-09-05 DOI: 10.1038/s41377-024-01609-9
Zhexuan Cao, Ning Li, Laiyu Zhu, Jiamin Wu, Qionghai Dai, Hui Qiao

Depth sensing plays a crucial role in various applications, including robotics, augmented reality, and autonomous driving. Monocular passive depth sensing techniques have come into their own for the cost-effectiveness and compact design, offering an alternative to the expensive and bulky active depth sensors and stereo vision systems. While the light-field camera can address the defocus ambiguity inherent in 2D cameras and achieve unambiguous depth perception, it compromises the spatial resolution and usually struggles with the effect of optical aberration. In contrast, our previously proposed meta-imaging sensor1 has overcome such hurdles by reconciling the spatial-angular resolution trade-off and achieving the multi-site aberration correction for high-resolution imaging. Here, we present a compact meta-imaging camera and an analytical framework for the quantification of monocular depth sensing precision by calculating the Cramér–Rao lower bound of depth estimation. Quantitative evaluations reveal that the meta-imaging camera exhibits not only higher precision over a broader depth range than the light-field camera but also superior robustness against changes in signal-background ratio. Moreover, both the simulation and experimental results demonstrate that the meta-imaging camera maintains the capability of providing precise depth information even in the presence of aberrations. Showing the promising compatibility with other point-spread-function engineering methods, we anticipate that the meta-imaging camera may facilitate the advancement of monocular passive depth sensing in various applications.

深度感应在机器人、增强现实和自动驾驶等各种应用中发挥着至关重要的作用。单目被动深度传感技术因其成本效益高、设计紧凑而大放异彩,成为昂贵而笨重的主动深度传感器和立体视觉系统的替代品。虽然光场照相机可以解决二维照相机固有的离焦模糊性问题,并实现清晰的深度感知,但它会影响空间分辨率,而且通常会受到光学像差的影响。与此相反,我们之前提出的元成像传感器1 克服了这些障碍,在空间分辨率和角分辨率之间进行了权衡,并实现了多点像差校正,从而获得了高分辨率成像。在此,我们介绍了一种紧凑型元成像相机,以及通过计算深度估计的克拉梅尔-拉奥下界来量化单眼深度感应精度的分析框架。定量评估结果表明,元成像相机不仅在更广的深度范围内表现出比光场相机更高的精度,而且在信号-背景比变化时也表现出卓越的鲁棒性。此外,模拟和实验结果都表明,即使存在像差,元成像相机也能保持提供精确深度信息的能力。元成像照相机与其他点扩散函数工程方法具有良好的兼容性,我们预计元成像照相机将促进单眼被动深度传感技术在各种应用中的发展。
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引用次数: 0
Thresholdless coherence in a superradiant laser 超辐射激光器中的无阈相干性
Q1 OPTICS Pub Date : 2024-09-05 DOI: 10.1038/s41377-024-01591-2
Seung-Hoon Oh, Jinuk Kim, Junseo Ha, Gibeom Son, Kyungwon An

Lasing threshold in the conventional lasers is the minimum input power required to initiate laser oscillation. It has been widely accepted that the conventional laser threshold occurring around a unity intracavity photon number can be eliminated in the input-output curve by making the so-called β parameter approach unity. The recent experiments, however, have revealed that even in this case the photon statistics still undergo a transition from coherent to thermal statistics when the intracavity mean photon number is decreased below unity. Since the coherent output is only available above the diminished threshold, the long-sought promise of thresholdless lasers to produce always coherent light has become questionable. Here, we present an always-coherent thresholdless laser based on superradiance by two-level atoms in a quantum superposition state with the same phase traversing a high-Q cavity. Superradiant lasing was observed without the conventional lasing threshold around the unity photon number and the photon statistics remained near coherent even below it. The coherence was improved by reducing the coupling constant as well as the excited-state amplitude in the superposition state. Our results pave a way toward always-coherent thresholdless lasers with more practical media such as quantum dots, nitrogen-vacancy centers and doped ions in crystals.

传统激光器中的激光阈值是启动激光振荡所需的最小输入功率。人们普遍认为,通过使所谓的 β 参数接近于 1,就可以在输入-输出曲线中消除在腔内光子数达到 1 时出现的传统激光阈值。然而,最近的实验表明,即使在这种情况下,当腔内平均光子数降至一以下时,光子统计仍会从相干统计过渡到热统计。由于相干输出只在阈值降低时才会出现,因此人们长期追求的无阈值激光器产生始终相干光的承诺就变得值得怀疑了。在这里,我们提出了一种基于量子叠加态中的两级原子以相同相位穿越高 Q 腔的超辐射的始终相干无阈值激光器。超辐射激光在光子数统一附近没有传统的激光阈值,即使低于该阈值,光子统计也保持近乎相干。通过降低耦合常数以及叠加态中的激发态振幅,相干性得到了改善。我们的研究结果为利用量子点、氮空位中心和晶体中的掺杂离子等更实用的介质实现始终相干的无阈值激光器铺平了道路。
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引用次数: 0
Neural network-based processing and reconstruction of compromised biophotonic image data 基于神经网络处理和重建受损生物光子图像数据
Q1 OPTICS Pub Date : 2024-09-04 DOI: 10.1038/s41377-024-01544-9
Michael John Fanous, Paloma Casteleiro Costa, Çağatay Işıl, Luzhe Huang, Aydogan Ozcan

In recent years, the integration of deep learning techniques with biophotonic setups has opened new horizons in bioimaging. A compelling trend in this field involves deliberately compromising certain measurement metrics to engineer better bioimaging tools in terms of e.g., cost, speed, and form-factor, followed by compensating for the resulting defects through the utilization of deep learning models trained on a large amount of ideal, superior or alternative data. This strategic approach has found increasing popularity due to its potential to enhance various aspects of biophotonic imaging. One of the primary motivations for employing this strategy is the pursuit of higher temporal resolution or increased imaging speed, critical for capturing fine dynamic biological processes. Additionally, this approach offers the prospect of simplifying hardware requirements and complexities, thereby making advanced imaging standards more accessible in terms of cost and/or size. This article provides an in-depth review of the diverse measurement aspects that researchers intentionally impair in their biophotonic setups, including the point spread function (PSF), signal-to-noise ratio (SNR), sampling density, and pixel resolution. By deliberately compromising these metrics, researchers aim to not only recuperate them through the application of deep learning networks, but also bolster in return other crucial parameters, such as the field of view (FOV), depth of field (DOF), and space-bandwidth product (SBP). Throughout this article, we discuss various biophotonic methods that have successfully employed this strategic approach. These techniques span a wide range of applications and showcase the versatility and effectiveness of deep learning in the context of compromised biophotonic data. Finally, by offering our perspectives on the exciting future possibilities of this rapidly evolving concept, we hope to motivate our readers from various disciplines to explore novel ways of balancing hardware compromises with compensation via artificial intelligence (AI).

近年来,深度学习技术与生物光子装置的整合为生物成像开辟了新天地。该领域的一个引人注目的趋势是,为了在成本、速度和外形等方面设计出更好的生物成像工具,故意牺牲某些测量指标,然后通过利用在大量理想、卓越或替代数据上训练的深度学习模型来弥补由此产生的缺陷。由于这种战略方法具有增强生物光子成像各个方面的潜力,因此越来越受欢迎。采用这种策略的主要动机之一是追求更高的时间分辨率或更快的成像速度,这对捕捉精细的动态生物过程至关重要。此外,这种方法还有望简化硬件要求和复杂性,从而使先进的成像标准在成本和/或尺寸方面更容易获得。本文深入评述了研究人员在其生物光子装置中有意损害的各种测量方面,包括点扩散函数(PSF)、信噪比(SNR)、采样密度和像素分辨率。通过故意损害这些指标,研究人员不仅希望通过应用深度学习网络恢复这些指标,还希望反过来增强其他关键参数,如视场(FOV)、景深(DOF)和空间-带宽乘积(SBP)。在本文中,我们将讨论成功采用这种战略方法的各种生物光子方法。这些技术的应用范围广泛,展示了深度学习在生物光子数据妥协背景下的多功能性和有效性。最后,我们希望通过对这一快速发展的概念令人兴奋的未来可能性的展望,激励不同学科的读者探索通过人工智能(AI)来平衡硬件妥协与补偿的新方法。
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引用次数: 0
Harnessing the capabilities of VCSELs: unlocking the potential for advanced integrated photonic devices and systems 利用 VCSEL 的功能:释放先进集成光子设备和系统的潜力
Q1 OPTICS Pub Date : 2024-09-03 DOI: 10.1038/s41377-024-01561-8
Guanzhong Pan, Meng Xun, Xiaoli Zhou, Yun Sun, Yibo Dong, Dexin Wu

Vertical cavity surface emitting lasers (VCSELs) have emerged as a versatile and promising platform for developing advanced integrated photonic devices and systems due to their low power consumption, high modulation bandwidth, small footprint, excellent scalability, and compatibility with monolithic integration. By combining these unique capabilities of VCSELs with the functionalities offered by micro/nano optical structures (e.g. metasurfaces), it enables various versatile energy-efficient integrated photonic devices and systems with compact size, enhanced performance, and improved reliability and functionality. This review provides a comprehensive overview of the state-of-the-art versatile integrated photonic devices/systems based on VCSELs, including photonic neural networks, vortex beam emitters, holographic devices, beam deflectors, atomic sensors, and biosensors. By leveraging the capabilities of VCSELs, these integrated photonic devices/systems open up new opportunities in various fields, including artificial intelligence, large-capacity optical communication, imaging, biosensing, and so on. Through this comprehensive review, we aim to provide a detailed understanding of the pivotal role played by VCSELs in integrated photonics and highlight their significance in advancing the field towards efficient, compact, and versatile photonic solutions.

垂直腔面发射激光器(VCSEL)具有功耗低、调制带宽高、占地面积小、可扩展性好以及与单片集成兼容等优点,因此已成为开发先进集成光子器件和系统的多功能且前景广阔的平台。通过将 VCSEL 的这些独特性能与微/纳米光学结构(如元表面)提供的功能相结合,可实现各种多功能的高能效集成光子器件和系统,这些器件和系统具有体积小、性能高、可靠性和功能性更好的特点。本综述全面概述了基于 VCSEL 的最先进的多功能集成光子器件/系统,包括光子神经网络、涡旋光束发射器、全息器件、光束偏转器、原子传感器和生物传感器。通过利用 VCSEL 的功能,这些集成光子器件/系统为人工智能、大容量光通信、成像、生物传感等各个领域带来了新的机遇。通过本综述,我们旨在详细介绍 VCSEL 在集成光子学中发挥的关键作用,并强调其在推动该领域实现高效、紧凑和多功能光子解决方案方面的重要意义。
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引用次数: 0
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