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Experimental demonstration of spatiotemporal analog computation in ultrafast optics. 超快光学中时空模拟计算的实验论证。
Q1 OPTICS Pub Date : 2026-01-22 DOI: 10.1038/s41377-025-02109-0
Junyi Huang,Dong Zhao,Jixuan Shi,Hongliang Zhang,Hengyi Wang,Fang-Wen Sun,Qiwen Zhan,Shiyao Zhu,Kun Huang,Zhichao Ruan
It is intractable to perform information processing and computation on single ultrafast optical pulses, within picoseconds or even femtoseconds. Here, we experimentally demonstrate an optical spatiotemporal differentiator, a mirror-symmetry-breaking dielectric metagrating, which performs analog computations of both spatial and temporal differentiations on single ultrafast optical wavepackets. The spatiotemporal differentiator is designed with a transfer function with linear dependence on spatial wavevector and temporal frequency and fabricated by using a double-exposure E-beam lithography process. We achieve the first-order spatiotemporal differentiation with experimental resolutions of approximately 14 μm (in space) and 260 fs (in time). Furthermore, we report a parabolic relationship between the transverse velocity of a front-tilted photonic wavepacket and the normalized intensity of its first-order spatiotemporal-differentiation wavepacket. This relationship allows direct measurement of the transverse velocity using only the normalized intensity, fundamentally simplifying velocity detection. These capabilities of optical spatiotemporal computation endow emerging space-time optics with fundamental computation blocks.
单超快光脉冲在皮秒甚至飞秒内进行信息处理和计算是非常困难的。在这里,我们通过实验展示了一种光学时空微分器,一种镜像对称破缺的介电介介,它可以对单个超快光波包进行空间和时间微分器的模拟计算。采用双曝光电子束光刻工艺制作时空微分器,并设计了与空间波矢量和时间频率线性相关的传递函数。我们以大约14 μm(空间)和260 fs(时间)的实验分辨率实现了一阶时空分异。此外,我们报道了前倾斜光子波包的横向速度与其一阶时空分异波包的归一化强度之间的抛物线关系。这种关系允许仅使用归一化强度直接测量横向速度,从根本上简化了速度检测。这些光学时空计算能力为新兴的空时光学提供了基本的计算模块。
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引用次数: 0
Generation of vectorial generalized vortex array with metasurfaces. 具有超表面的矢量广义涡阵的生成。
Q1 OPTICS Pub Date : 2026-01-22 DOI: 10.1038/s41377-025-02102-7
Qingsong Yao,Zile Li,Guoxing Zheng
The ability to create complex three-dimensional structures of light is extremely challenging. Now, a technique combining Dammann optimization with metasurfaces has been developed, enabling control over all parameters, including polarization, phase, angular momentum, and spatial modes. The generation of three-dimensional generalized vortex beams can open new horizons for their applications in photonics.
创造复杂的三维光结构的能力是极具挑战性的。现在,一种将Dammann优化与超表面相结合的技术已经开发出来,可以控制所有参数,包括偏振、相位、角动量和空间模式。三维广义涡旋光束的产生为其在光子学中的应用开辟了新的领域。
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引用次数: 0
Dispersion engineering by rotational symmetry breaking in an optical microcavity. 光学微腔中旋转对称破缺的色散工程。
Q1 OPTICS Pub Date : 2026-01-22 DOI: 10.1038/s41377-025-02169-2
Jian-Zheng Ren,Li-Jie Li,Rui-Qi Zhang,Zhi-Yan Wang,Qi-Tao Cao,Yun-Feng Xiao
Dispersion engineering is pivotal for nonlinear optics, yet it often faces challenges posed by material and structural limitations. Here, we establish rotational symmetry breaking as the guiding principle for dispersion engineering in optical microcavities. Through boundary deformation, multi-branch global dispersion emerges in island modes, and local dispersion is controlled via resonance-assisted tunneling between quasi-whispering gallery modes. Enabled by the global dispersion, the optical parametric oscillation is predicted in blue-violet light spectrum with high efficiency (>55%) and large frequency separation (>180 THz). Using the local dispersion engineering, the doubly-resonant enhancement of second-harmonic generation is regulated by the resonance-assisted tunneling.
色散工程是非线性光学研究的关键,但由于材料和结构的限制,色散工程经常面临挑战。在此,我们建立了旋转对称破缺作为光学微腔色散工程的指导原则。通过边界变形,在孤岛模式中产生多分支的全局色散,在准耳语通道模式之间通过共振辅助隧道控制局部色散。在全局色散的作用下,在蓝紫光光谱中预测了高效率(>55%)和大频率分离(>180 THz)的光学参量振荡。利用局域色散工程,利用共振辅助隧穿调节二次谐波产生的双共振增强。
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引用次数: 0
TRIXS: a multilayer grating solution towards highly efficient resonant inelastic tender X-ray scattering. TRIXS:一种多层光栅解决方案,用于高效共振非弹性弱x射线散射。
Q1 OPTICS Pub Date : 2026-01-21 DOI: 10.1038/s41377-025-02172-7
Ke-Jin Zhou,Qiushi Huang,Mirian Garcia-Fernandez,Yeqi Zhuang,Stefano Agrestini,Shengyou Wen,Thomas Rice,Sahil Tippireddy,Jaewon Choi,Andrew Walters,Igor V Kozhevnikov,Zhe Zhang,Runze Qi,Zhong Zhang,Hongchang Wang,Zhanshan Wang
Resonant inelastic X-ray scattering (RIXS) is a photon-in/photon-out spectroscopic technique which has become increasingly important for the condensed matter physics community. The development of the RIXS instrumentation in soft X-ray and hard X-ray range facilitated the research in 3d and 5d transition metal (TM)-based materials, respectively. However, the tender X-ray (2000-3000 eV) RIXS covering most of 4d TM-based materials severely falls behind due to the lack of high-performance energy dispersive optics. Here, we demonstrate the design and fabrication of a laterally graded multilayer grating (MLG) optics for the establishment of the tender RIXS at the I21 RIXS beamline in Diamond Light Source. The successful implementation of the MLG boosts the photon flux by more than an order of magnitude at the Sulfur K-edge (2475 eV) and the Ru L3-edge (2838 eV) in comparison to the solution of a single-layer coated grating (SLG). More importantly, MLG retains the high energy resolution of the SLG design (~10,000) and works continuously across the full range of 2000-3000 eV. It renders the I21 beamline as the very first RIXS facility in the world that covers both soft and tender X-rays (280-3000 eV) using a grating-based spectrometer for a wide range of science applications.
共振非弹性x射线散射(RIXS)是一种光子进/光子出光谱技术,在凝聚态物理界已变得越来越重要。RIXS仪器在软x射线和硬x射线范围内的发展分别促进了3d和5d过渡金属(TM)基材料的研究。然而,由于缺乏高性能的能量色散光学器件,覆盖大多数4d tm基材料的柔嫩x射线(2000-3000 eV) RIXS严重落后。在这里,我们展示了一个横向渐变多层光栅(MLG)光学器件的设计和制造,用于在钻石光源的I21 RIXS光束线上建立tender RIXS。与单层涂层光栅(SLG)相比,MLG的成功实现使硫k边(2475 eV)和钌l3边(2838 eV)的光子通量提高了一个数量级以上。更重要的是,MLG保留了SLG设计的高能量分辨率(~10,000),并在2000-3000 eV的全范围内连续工作。它使I21光束线成为世界上第一个覆盖软x射线和软x射线(280-3000 eV)的RIXS设施,使用基于光栅的光谱仪用于广泛的科学应用。
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引用次数: 0
High-efficiency femtosecond laser fabrication of graphene-hybrid planar micro-supercapacitors with micro/nanostructured electrodes. 带微/纳米结构电极的石墨烯-杂化平面微型超级电容器的高效飞秒激光制备。
Q1 OPTICS Pub Date : 2026-01-21 DOI: 10.1038/s41377-025-02182-5
Yuyuan Zhang,Tingting Zou,Haobo Jiang,Xiuyan Fu,Wei Xin,Yiyang Meng,Xilin Li,Jun-Ming Cao,Lin Yang,Yuanzheng Li,Weizhen Liu,Dongdong Han,Xing-Long Wu,Jianjun Yang,Haiyang Xu,Yichun Liu
The integration of surface-regular micro/nanostructured electrodes within a limited footprint area is promising to enhance the electrochemical performance of planar micro-supercapacitors (P-MSCs), while developing simple yet efficient manufacturing methods for such electrodes remains a challenge. Here, we propose a universal strategy combining femtosecond laser plasma lithography with spatial light modulation (SLM-FPL), fabricating well-ordered sub-wavelength micro/nanostructured electrodes of interdigital P-MSCs (SEP-MSCs) on graphene oxide (GO) films. Achieving 500/50 µm finger widths/spacings and 680 nm internal grating periods, this method enables device densities >25 units inch-2 with processing efficiency orders of magnitude higher than conventional laser direct writing. Further performance optimizations via wettability modification, electric field engineering, and hybrid composites (GO-MXene/COF) yield outstanding specific capacitance (~41.4 F cm-3) and cycling stability (93% retention over 5000 cycles), supporting applications in flexible sensors and compact power supplies. This SLM-FPL technology shows strong potential for high-performance, spatially efficient SEP-MSCs in next-generation integrated systems.
在有限的占地面积内集成表面规则的微/纳米结构电极有望提高平面微超级电容器(P-MSCs)的电化学性能,但开发简单而高效的制造方法仍然是一个挑战。在这里,我们提出了一种将飞秒激光等离子体光刻与空间光调制(SLM-FPL)相结合的通用策略,在氧化石墨烯(GO)薄膜上制备有序的亚波长间P-MSCs (SEP-MSCs)微/纳米结构电极。该方法实现了500/50 μ m的指宽/间距和680 nm的内部光栅周期,使器件密度达到25单位英寸-2,处理效率比传统的激光直接写入高几个数量级。通过润湿性改性、电场工程和混合复合材料(GO-MXene/COF)进一步优化性能,可获得出色的比电容(~41.4 F cm-3)和循环稳定性(超过5000次循环保持93%),支持柔性传感器和紧凑型电源的应用。这种SLM-FPL技术显示了下一代集成系统中高性能、空间高效SEP-MSCs的强大潜力。
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引用次数: 0
Integrated-photonics-based systems for polarization-gradient cooling of trapped ions 捕获离子偏振梯度冷却的集成光子学系统
Q1 OPTICS Pub Date : 2026-01-15 DOI: 10.1038/s41377-025-02094-4
Sabrina M. Corsetti, Ashton Hattori, Ethan R. Clements, Felix W. Knollmann, Milica Notaros, Reuel Swint, Tal Sneh, Patrick T. Callahan, Gavin N. West, Dave Kharas, Thomas Mahony, Colin D. Bruzewicz, Cheryl Sorace-Agaskar, Robert McConnell, Isaac L. Chuang, John Chiaverini, Jelena Notaros
Trapped ions are a promising modality for quantum systems, with demonstrated utility as the basis for quantum processors and optical clocks. However, traditional trapped-ion systems are implemented using complex free-space optical configurations, whose large size and susceptibility to vibrations and drift inhibit scaling to large numbers of qubits. In recent years, integrated-photonics-based systems have been demonstrated as an avenue to address the challenge of scaling trapped-ion systems while maintaining high fidelities. While these previous demonstrations have implemented both Doppler and resolved-sideband cooling of trapped ions, these cooling techniques are fundamentally limited in efficiency. In contrast, polarization-gradient cooling can enable faster and more power-efficient cooling and, therefore, improved computational efficiencies in trapped-ion systems. While free-space implementations of polarization-gradient cooling have demonstrated advantages over other cooling mechanisms, polarization-gradient cooling has never previously been implemented using integrated photonics. In this paper, we design and experimentally demonstrate key polarization-diverse integrated-photonics devices and utilize them to implement a variety of integrated-photonics-based polarization-gradient-cooling systems, culminating in the first experimental demonstration of polarization-gradient cooling of a trapped ion by an integrated-photonics-based system. By demonstrating polarization-gradient cooling using an integrated-photonics-based system and, in general, opening up the field of polarization-diverse integrated-photonics-based devices and systems for trapped ions, this work facilitates new capabilities for integrated-photonics-based trapped-ion platforms.
捕获离子是量子系统的一种有前途的模式,作为量子处理器和光学时钟的基础已被证明具有实用价值。然而,传统的捕获离子系统是使用复杂的自由空间光学结构实现的,其大尺寸和对振动和漂移的敏感性阻碍了对大量量子比特的缩放。近年来,基于集成光子学的系统已被证明是解决在保持高保真度的同时缩放捕获离子系统的挑战的一种途径。虽然这些先前的演示已经实现了捕获离子的多普勒和解决边带冷却,但这些冷却技术在效率上基本上是有限的。相比之下,极化梯度冷却可以实现更快、更节能的冷却,因此可以提高捕获离子系统的计算效率。虽然自由空间实现的偏振梯度冷却已经证明了比其他冷却机制的优势,但偏振梯度冷却以前从未使用集成光子学实现过。在本文中,我们设计并实验演示了关键的偏振多样化集成光子器件,并利用它们实现了各种基于集成光子的偏振梯度冷却系统,最终在基于集成光子系统的捕获离子的偏振梯度冷却的第一个实验演示中达到了高潮。通过展示使用集成光子学系统的偏振梯度冷却,总的来说,开辟了偏振多样的集成光子学捕获离子的设备和系统领域,这项工作促进了基于集成光子学的捕获离子平台的新功能。
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引用次数: 0
Deciphering light transformation in chiral metasurface in real space and time by ultrafast electron microscopy. 用超快电子显微镜解译实时空手性超表面的光变换。
Q1 OPTICS Pub Date : 2026-01-14 DOI: 10.1038/s41377-025-02163-8
Ling Tong,Fei Xie,Xiaochen Gao,Yuxuan Chen,Shaozheng Ji,Bin Zhang,Jing Li,Jiangteng Guo,Fang Liu,Cuntao Gao,Min Feng,Wei Wu,Shibin Deng,Yiming Pan,Yunquan Liu,Jingjun Xu,Mengxin Ren,Xuewen Fu
Optical activity in chiral structures, i.e., circular dichroism (CD), has led to significant advances in nanoscale optical manipulation, including chiral metasurfaces, helicoid crystals, and chiral macromolecules. Although the local geometric design of chiral structures fundamentally governs their optical responses, the microscopic origin of CD remains unresolved due to the inability to probe optical chirality generation and local geometry effects with sufficient spatiotemporal resolution. Here, we unveil the light transformation process in a Γ-shaped chiral metasurface by combining far-field ellipticity measurements with direct near-field imaging at nanometer-femtosecond scale using photon-induced near-field electron microscopy (PINEM). By decomposing the near-field distributions into local symmetric and asymmetric components, we define a near-field ellipticity that quantitatively follows the wavelength-dependent far-field ellipticity. Finite-element simulations reveal that an electric dipole at the top-right corner of the Γ-shaped meta-atom dominates the ellipticity, which increases as the dipole contribution grows with wavelength. Crucially, time-resolved PINEM reveals that asymmetric near-fields dissipate faster than the symmetric counterparts by tens to hundreds of femtoseconds, indicating chiral-geometry-dependent energy dissipation pathways. This work provides microscopic insight into light transformation in chiral structures and lays the foundation for advanced chiral photonic device design.
手性结构的光学活性,即圆二色性(CD),导致了纳米级光学操作的重大进展,包括手性超表面、螺旋晶体和手性大分子。虽然手性结构的局部几何设计从根本上控制了它们的光学响应,但由于无法以足够的时空分辨率探测光学手性的产生和局部几何效应,CD的微观起源仍然没有解决。在这里,我们利用光子诱导近场电子显微镜(PINEM),结合远场椭圆度测量和直接近场成像,揭示了Γ-shaped手性超表面的光转换过程。通过将近场分布分解为局部对称和非对称分量,我们定义了一个定量地遵循波长相关远场椭圆度的近场椭圆度。有限元模拟表明,在Γ-shaped元原子右上角的电偶极子主导着椭圆度,随着波长的增加,偶极子的贡献增加。至关重要的是,时间分辨的PINEM显示,不对称的近场耗散速度比对称的快几十到几百飞秒,这表明了手性几何相关的能量耗散途径。本研究为手性结构中的光转换提供了微观视角,为先进的手性光子器件设计奠定了基础。
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引用次数: 0
Multi-dimensional camouflage against VIS-NIR hyperspectral, MIR intensity, and MIR polarization imaging. 针对VIS-NIR高光谱、MIR强度和MIR偏振成像的多维伪装。
Q1 OPTICS Pub Date : 2026-01-12 DOI: 10.1038/s41377-025-02145-w
Rui Qin,Huanzheng Zhu,Rongxuan Zhu,Pintu Ghosh,Min Qiu,Qiang Li
Camouflage is essential in modern security and military operations, playing a critical role in evading detection and enhancing the survivability of equipment. However, most existing camouflage devices operate in a single dimension, rendering them inadequate against emerging multi-dimensional detection techniques, including visible to near-infrared (VIS-NIR) hyperspectral imaging and mid-infrared (MIR) polarization imaging. In this work, we propose a multi-dimensional camouflage strategy that realizes simultaneous VIS-NIR spectrum camouflage, MIR intensity, and polarization camouflage by a hierarchical structure. The multi-dimensional camouflage device exhibits an emissivity of 0.7, a low degree of linear polarization (< 1.5%) at large observation angles in MIR range, and high spectral similarity (>96.9%) in the VIS-NIR range. Moreover, it deceives hyperspectral classification in vegetative background and blends into its environment under MIR intensity and polarization imaging. This work introduces a novel paradigm for multi-dimensional camouflage techniques and opens up new avenues for electromagnetic waves manipulation.
在现代安全和军事行动中,伪装是必不可少的,在逃避侦查和提高装备的生存能力方面发挥着关键作用。然而,大多数现有的伪装装置在单一维度上工作,使得它们不足以应对新兴的多维探测技术,包括可见到近红外(VIS-NIR)高光谱成像和中红外(MIR)偏振成像。在这项工作中,我们提出了一种多维伪装策略,通过分层结构实现同时进行VIS-NIR光谱伪装、MIR强度伪装和极化伪装。该多维伪装装置的发射率为0.7,在MIR范围内大观测角度线偏振度低(< 1.5%),在VIS-NIR范围内光谱相似度高(>96.9%)。此外,在植物背景下,它可以欺骗高光谱分类,并在MIR强度和偏振成像下融入其环境。这项工作为多维伪装技术引入了一种新的范式,为电磁波操纵开辟了新的途径。
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引用次数: 0
Meta-device for sensing subwavelength lateral displacement. 传感亚波长横向位移的元装置。
Q1 OPTICS Pub Date : 2026-01-12 DOI: 10.1038/s41377-025-02067-7
Shufan Chen,Yubin Fan,Hao Li,Xiaodong Qiu,Ben Wang,Lijian Zhang,Shumin Xiao,Din Ping Tsai
Accurate transverse displacement measurement is essential for precise mask-to-wafer positioning in lithography. While lateral displacement metrology has achieved nanometer-level precision, the limitations imposed by coherent state and grating challenge in-situ measurement speed and precision. Here, we introduce a two-photon state transverse displacement measurement method utilizing a polarization gradient metasurface by employing two-photon state interference. Compared with the classical method, our new method can experimentally reduce the number of detected photons to around 3% with equivalent precision. These attributes make the two-photon state polarization gradient metasurface approach highly suitable for integration with semiconductor lithography processes and show its promise in realizing equivalent measurement precision within notably shorter acquisition durations, providing a robust solution for next-generation transverse displacement measurement requirements.
精确的横向位移测量对于光刻中掩模到晶圆的精确定位至关重要。虽然横向位移测量已经达到纳米级精度,但由于相干态和光栅的限制,原位测量的速度和精度受到了挑战。本文介绍了一种利用双光子态干涉的偏振梯度超表面测量双光子态横向位移的方法。与传统的方法相比,我们的新方法在实验中可以将检测到的光子数量减少到3%左右,并且具有等效的精度。这些特性使得双光子态偏振梯度超表面方法非常适合与半导体光刻工艺集成,并显示出其在显着较短的采集时间内实现等效测量精度的承诺,为下一代横向位移测量需求提供了强大的解决方案。
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引用次数: 0
Integrated, ultrafast all-optical polariton transistors with sub-wavelength grating microcavities. 具有亚波长光栅微腔的集成超快全光极化子晶体管。
Q1 OPTICS Pub Date : 2026-01-12 DOI: 10.1038/s41377-025-02050-2
Pietro Tassan,Darius Urbonas,Bartos Chmielak,Jens Bolten,Thorsten Wahlbrink,Max C Lemme,Michael Forster,Ullrich Scherf,Rainer F Mahrt,Thilo Stöferle
All-optical logic has the potential to overcome the operation speed barrier that has persisted in electronic circuits for two decades. However, the development of scalable architectures has been prevented so far by the lack of materials with sufficiently strong nonlinear interactions needed to realize compact and efficient ultrafast all-optical switches with optical gain. Microcavities with embedded organic material in the strong light-matter interaction regime have recently enabled all-optical transistors operating at room temperature with picosecond switching times. However, the vertical cavity geometry, which is predominantly used in polaritonics, is not suitable for complex circuits with on-chip coupled transistors. Here, by leveraging state-of-the-art silicon photonics technology, we have achieved exciton-polariton condensation at ambient conditions in fully integrated high-index contrast sub-wavelength grating microcavities filled with a π-conjugated polymer as optically active material. We demonstrate ultrafast all-optical transistor action by coupling two resonators and utilizing seeded polariton condensation. With a device area as small as 2 × 2 µm2, we realize picosecond switching and amplification up to 60x, with extinction ratio up to 8:1. This compact ultrafast transistor device with in-plane integration is a key component for a scalable platform for all-optical logic circuits that could operate two orders of magnitude faster than electronic counterparts.
全光逻辑有潜力克服在电子电路中存在了20年的运算速度障碍。然而,到目前为止,由于缺乏具有足够强的非线性相互作用的材料来实现具有光增益的紧凑和高效的超快全光开关,因此阻碍了可扩展架构的发展。在强光-物质相互作用下嵌入有机材料的微腔最近使全光晶体管能够在室温下以皮秒的开关时间工作。然而,垂直腔的几何结构,主要用于极化电子学,是不适合复杂的电路与片上耦合晶体管。在这里,我们利用最先进的硅光子学技术,在完全集成的高折射率对比亚波长光栅微腔中实现了激子-极化子凝聚,微腔中填充了π共轭聚合物作为光学活性材料。我们通过耦合两个谐振腔和利用种子极化子凝聚来演示超快全光晶体管的作用。器件面积仅为2 × 2µm2,可实现皮秒开关和放大60倍,消光比高达8:1。这种具有平面内集成的紧凑超快晶体管器件是可扩展的全光逻辑电路平台的关键组件,其运行速度比电子器件快两个数量级。
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引用次数: 0
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Light-Science & Applications
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