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Source term estimation for the MARIA research reactor and model of atmospheric dispersion of radionuclides with dry deposition MARIA研究反应堆的源项估计和干沉降放射性核素大气扩散模型
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-07-06 DOI: 10.2478/nuka-2020-0028
M. Lipka
Abstract Source term is the amount of radionuclide activity, measured in becquerels, released to the atmosphere from a nuclear reactor, together with the plume composition, over a specific period. It is the basis of radioprotection-related calculation. Usually, such computations are done using commercial codes; however, they are challenging to be used in the case of the MARIA reactor due to its unique construction. Consequently, there is a need to develop a method that will be able to deliver useful results despite the complicated geometry of the reactor site. Such an approach, based upon the Bateman balance equation, is presented in the article, together with the results of source term calculation for the MARIA reactor. Additionally, atmospheric dispersion of the radionuclides, analysed with the Gauss plume model with dry deposition, is presented.
摘要源项是指在特定时期内,从核反应堆释放到大气中的放射性核素活度(以贝克勒尔为单位)以及羽流成分。它是辐射防护相关计算的基础。通常,此类计算是使用商业代码进行的;然而,由于其独特的结构,它们在MARIA反应堆的情况下使用具有挑战性。因此,需要开发一种方法,尽管反应堆场地的几何形状复杂,但仍能提供有用的结果。本文提出了一种基于贝特曼平衡方程的方法,并给出了MARIA反应堆源项的计算结果。此外,还用干沉降高斯羽流模型分析了放射性核素在大气中的扩散。
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引用次数: 1
Fission chambers for space effect reduction in the application of the area method: A new approach 裂变室在空间效应减小中的应用:面积法的新途径
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-07-06 DOI: 10.2478/nuka-2020-0026
J. Janczyszyn, G. Domańska, P. Stanisz
Abstract The possibility of preparing fission chambers for the experimental determination of subcriticality without time-consuming corrections has been presented. The reactor detectors set consists of monoisotopic chambers. Each chamber is intended for a specific position in the system. Individual weights, rated a priori for all detectors in their positions, allow for quick calculation of whole system subcriticality. The inconveniences related to the spatial effect are minimized. This is achieved by computational simulation of the area method results, for each detector position and all possible fissionable and fissile nuclides. Next, one nuclide is selected, specific for the given position, presenting the smallest difference from the MCNP KCODE precisely estimated kkcode. The case study is made using the model of VENUS-F core.
摘要提出了在不进行耗时校正的情况下,为亚临界实验测定准备裂变室的可能性。反应堆探测器组由单同位素室组成。每个腔室用于系统中的特定位置。所有探测器在其位置上的单独权重都是先验的,可以快速计算整个系统的亚临界度。与空间效果相关的不便被最小化。这是通过对每个探测器位置和所有可能的可裂变和可裂变核素的面积法结果进行计算模拟来实现的。接下来,选择一个特定于给定位置的核素,与MCNP-KCODE精确估计的kkcode的差异最小。利用VENUS-F堆芯模型进行了实例研究。
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引用次数: 2
Summer–winter contrast in carbon isotope and elemental composition of total suspended particulate matter in the urban atmosphere of Krakow, Southern Poland 波兰南部克拉科夫城市大气中总悬浮颗粒物的碳同位素和元素组成的夏冬季对比
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-07-06 DOI: 10.2478/nuka-2020-0029
M. Zimnoch, F. Morawski, T. Kuc, L. Samek, J. Bartyzel, Z. Gorczyca, A. Skiba, K. Różański
Abstract The city of Krakow located in southern Poland ranks among the most polluted urban agglomerations in Europe. There are persisting controversies with respect to impact of different pollution sources operating in Krakow agglomeration on air quality within the city. The presented pilot study was aimed at exploring the possibilities offered by elemental and carbon isotope composition of total suspended particulate matter (TSPM) for better characterization of its sources in Krakow atmosphere. The analyses of carbon isotope composition of total carbon in the investigated TSPM samples were supplemented by parallel analyses of radiocarbon content in atmospheric carbon dioxide (CO2). This study revealed large seasonal variability of carbon isotope composition in the analysed TSPM samples. This large variability reflects seasonally varying contribution of different sources of fossil and modern carbon to the TSPM pool. The elemental composition of TSPM also reveals distinct seasonal variability of the analysed elements, reflecting varying mixture of natural and anthropogenic sources of those elements. A linear relationship between the fossil carbon load in the TSPM samples and the fossil carbon load in the atmospheric CO2 was found, pointing to the presence of additional source of anthropogenic carbonaceous particles not associated with burning of fossil fuels. Wearing of tyres and asphalt pavement is most probably the main source of such particles.
摘要位于波兰南部的克拉科夫市是欧洲污染最严重的城市群之一。关于克拉科夫聚集区不同污染源对城市空气质量的影响,一直存在争议。所提出的试点研究旨在探索总悬浮颗粒物(TSPM)的元素和碳同位素组成为更好地表征其在克拉科夫大气中的来源提供的可能性。通过对大气二氧化碳(CO2)中放射性碳含量的平行分析,补充了对所研究的TSPM样品中总碳的碳同位素组成的分析。这项研究揭示了所分析的TSPM样品中碳同位素组成的巨大季节变化。这种巨大的可变性反映了化石和现代碳的不同来源对TSPM库的季节性变化贡献。TSPM的元素组成也揭示了所分析元素的明显季节变化,反映了这些元素的自然和人为来源的不同混合。TSPM样品中的化石碳负荷和大气CO2中的化石炭负荷之间存在线性关系,表明存在与化石燃料燃烧无关的人为碳质颗粒的额外来源。轮胎和沥青路面的磨损很可能是这些颗粒的主要来源。
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引用次数: 7
Indoor and outdoor 222Rn and 220Rn and their progeny levels surrounding Bayan Obo mine, China 白云鄂博矿区室内外222Rn、220Rn及其子代水平
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0023
Nanping Wang, Miao Hu, Weihua Zeng, Cong Yu, Binlin Jia, Zhijie Yang
Abstract More than half of the total natural ionizing radiation dose received by the human population is caused by radon and thoron (Rn and Tn) and their progeny. To estimate the level of radiation due to radon and thoron and their progeny, an investigation was conducted in a residential area near the world’s largest open-pit mine of Bayan Obo in Inner Mongolia, China. The concentration of Rn, Tn, and their decay products in air and soil were studied by using AlphaGUARD, RAD7, and ERS-RDM-2S for a discrete period of time in three different locations. The average indoor concentration of radon and thoron was 62.6 ± 44.6 Bq/m3 and 108.3 ± 94.5 Bq/m3 respectively, and the outdoor concentration was 12.9 ± 6.3 Bq/m3 and 55.8 ± 18.5 Bq/m3, respectively. Relatively high concentrations were recorded in the area near to the mine, with a significant increasing trend observed in indoor thoron concentration. A prominent hotspot in thoron concentration was found in a single-story house with values 747 ± 150 Bq/m3. The equilibrium equivalent thoron concentration (EECTn) varies from 0.48 Bq/m3 to 2.36 Bq/m3 with an arithmetic mean of 1.37 ± 0.64 Bq/m3, and comparatively higher than EECRn. Concluding that the mining activity at Bayan Obo mine is significantly increasing the level of indoor thoron and its progeny in surroundings. It is suggested to further systematically investigate the indoor Rn and Tn progeny concentrations in the residential dwellings of the Bayan Obo mining area, and 232Th content of the building materials, to provide a basis for calculating the radiation dose.
摘要人类接受的总自然电离辐射剂量的一半以上是由氡和钍(Rn和Tn)及其后代引起的。为了估计氡和钍及其后代的辐射水平,在中国内蒙古白云鄂博世界最大露天矿附近的一个居民区进行了一项调查。使用AlphaGUARD、RAD7和ERS-RDM-2S在三个不同的位置研究了空气和土壤中Rn、Tn及其衰变产物的离散时间。室内氡和钍的平均浓度分别为62.6±44.6 Bq/m3和108.3±94.5 Bq/m3,室外浓度分别为12.9±6.3 Bq/m3、55.8±18.5 Bq/m3。矿井附近区域的浓度相对较高,室内钍浓度呈显著上升趋势。在一栋单层房屋中发现了一个显著的钍浓度热点,其值为747±150 Bq/m3。平衡当量钍浓度(EECTn)在0.48 Bq/m3至2.36 Bq/m3之间变化,算术平均值为1.37±0.64 Bq/m3,相对高于EECRn。结论:白云鄂博矿的采矿活动显著提高了室内钍及其后代在周围环境中的水平。建议进一步系统地调查巴彦奥博矿区居民住宅的室内Rn和Tn子代浓度以及建筑材料中232Th的含量,为计算辐射剂量提供依据。
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引用次数: 1
Using a scale model room to assess the contribution of building material of volcanic origin to indoor radon 使用比例模型室评估火山成因建筑材料对室内氡的贡献
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0010
C. Lucchetti, M. Castelluccio, M. Altamore, A. Briganti, G. Galli, M. Soligo, P. Tuccimei, M. Voltaggio
Abstract In the frame of Radon rEal time monitoring System and Proactive Indoor Remediation (RESPIRE), a LIFE 2016 project funded by the European Commission, the contribution of building materials of volcanic origin to indoor radon concentration was investigated. First, total gamma radiation and related outdoor dose rates of geological materials in the Caprarola area (Central Italy) were measured to define main sources of radiation. Second, 222Rn and 220Rn exhalation rates of these rocks used as building materials were measured using an accumulation chamber connected in a closed loop with a RAD7 radon monitor. Among others, the very porous “Tufo di Gallese” ignimbrite provided the highest values. This material was then used to construct a scale model room of 62 cm × 50 cm × 35 cm (inner length × width × height, respectively) to assess experimental radon and thoron activity concentration at equilibrium and study the effects of climatic conditions and different coatings on radon levels. A first test was carried out at ambient temperature to determine experimental 222Rn and 220Rn equilibrium activities in the model room, not covered with plaster or other coating materials. Experimental 222Rn equilibrium was recorded in just two days demonstrating that the room “breaths”, exchanging air with the outdoor environment. This determines a dilution of indoor radon concentration. Other experiments showed that inner covers (such as plasterboard and different kinds of paints) partially influence 222Rn but entirely cut the short-lived 220Rn. Finally, decreases in ambient temperature reduce radon exhalation from building material and, in turn, indoor activity concentration.
摘要在欧盟委员会资助的LIFE 2016项目氡实时监测系统和室内主动补救(RESPIRE)的框架内,研究了火山成因建筑材料对室内氡浓度的贡献。首先,测量了Caprarola地区(意大利中部)地质材料的总伽马辐射和相关室外剂量率,以确定主要辐射源。其次,这些用作建筑材料的岩石的222Rn和220Rn呼气率是使用与RAD7氡监测仪闭环连接的积聚室测量的。其中,多孔的“Tufo di Gallese”熔结凝灰岩提供了最高的价值。然后用这种材料建造了一个62cm×50cm×35cm(内部长度×宽度×高度分别为)的比例模型室,以评估平衡状态下的实验氡和钍活性浓度,并研究气候条件和不同涂层对氡水平的影响。第一次测试是在环境温度下进行的,以确定模型室中的实验222Rn和220Rn平衡活性,该模型室没有覆盖石膏或其他涂层材料。在短短两天内记录了222Rn的实验平衡,证明房间“呼吸”,与室外环境交换空气。这决定了室内氡浓度的稀释度。其他实验表明,内覆盖物(如石膏板和不同种类的油漆)部分影响222Rn,但完全切断了寿命短的220Rn。最后,环境温度的降低降低了建筑材料中氡的析出,进而降低了室内活动的浓度。
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引用次数: 6
214Bi/214Pb radioactivity ratio three-year monitoring in rainwater in Prague 布拉格雨水的214Bi/214Pb放射性比三年监测
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0018
F. Ambrosino, L. Thinová, M. Hýža, C. Sabbarese
Abstract Continuous monitoring of natural gamma radiation in air has been carried out, during December 2014 – January 2018, with 1-min cyclic measurement in Prague, Czech Republic using a NaI(Tl) probe. The 214Bi/214Pb ratio as a tracer in rainwater has been investigated to study its variations related to both the ambient dose equivalent rate per hour and the amount of rainfall. A hybrid methodology for time series analysis, composed of the aggregation of two signal decomposition methods (multiple linear regression and empirical mode decomposition) and one forecasting method (support vector regression), has been applied to identify the anomalies in the studied signals in order to better find correlations among them. The results show a strong correlation between the ambient dose equivalent rate and the 214Bi/214Pb ratio values and between both these signals and rainfall amount ≥5 mm/h. Furthermore, the considered descendants of radon are mainly responsible for the overall ambient dose equivalent rate.
2014年12月至2018年1月,在捷克共和国布拉格使用NaI(Tl)探针进行了空气中天然伽马辐射的连续监测,周期测量为1分钟。以214Bi/214Pb为示踪剂,研究了其随环境剂量当量每小时率和降雨量的变化规律。采用混合时间序列分析方法,将两种信号分解方法(多元线性回归和经验模态分解)和一种预测方法(支持向量回归)组合在一起,识别研究信号中的异常,以便更好地发现它们之间的相关性。结果表明,环境剂量当量率与214Bi/214Pb比值值之间、与降雨量≥5 mm/h之间存在较强的相关性。此外,氡的后代被认为是造成总环境剂量当量率的主要原因。
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引用次数: 19
A new geostatistical tool for the analysis of the geographical variability of the indoor radon activity 一种新的用于分析室内氡活动的地理变异的地质统计学工具
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0015
F. Loffredo, A. Scala, G. M. Adinolfi, F. Savino, M. Quarto
Abstract The population is continuously exposed to a background level of ionizing radiation due to the natural radioactivity and, in particular, with radon (222Rn). Radon gas has been classified as the second leading cause of lung cancer after tobacco smoke [1]. In the confined environment, radon concentration can reach harmful level and vary accordingly to many factors. Since the primary source of radon in dwellings is the subsurface, the risk assessment and reduction cannot disregard the identification of the local geology and the environmental predisposing factors. In this article, we propose a new methodology, based on the computation of the Gini coefficients at different spatial scales, to estimate the spatial correlation and the geographical variability of radon concentrations. This variability can be interpreted as a signature of the different subsurface geological conditions. The Gini coefficient computation is a statistical tool widely used to determine the degree of inhomogeneity of different kinds of distributions. We generated several simulated radon distributions, and the proposed tool has been validated by comparing the variograms based on the semi-variance computation with those ones based on the Gini coefficient. The Gini coefficient variogram is shown to be a good estimator of the inhomogeneity degree of radon concentration. Indeed, it allows to better constrain the critical distance below which the radon geological source can be considered as uniform at least for the investigated length scales of variability; it also better discriminates the fluctuations due to the environmental predisposing factors from those ones due to the random spatially uncorrelated noise.
由于天然放射性,特别是氡(222Rn),人口持续暴露于电离辐射的本底水平。氡气已被列为肺癌的第二大原因,仅次于烟草烟雾。在密闭环境中,氡的浓度会达到有害水平,并受多种因素的影响而发生相应的变化。由于住宅氡的主要来源是地下,因此风险评估和降低不能忽视对当地地质和环境诱发因素的识别。本文提出了一种基于不同空间尺度上的基尼系数计算方法来估算氡浓度的空间相关性和地理变异性。这种变化可以解释为不同地下地质条件的标志。基尼系数计算是一种广泛用于确定不同分布的不均匀程度的统计工具。我们生成了几个模拟的氡分布,并通过比较基于半方差计算的变异函数和基于基尼系数的变异函数来验证所提出的工具。基尼系数变异图可以很好地估计氡浓度的不均匀程度。事实上,它可以更好地限制至少在所研究的变率长度尺度内氡地质源可被视为均匀的临界距离;它还能更好地区分环境因素引起的波动和随机空间不相关噪声引起的波动。
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引用次数: 12
Exposures from radon, thoron, and thoron progeny in high background radiation area in Takandeang, Mamuju, Indonesia 印度尼西亚马木朱省Takandeang高本底辐射区氡、氡和氡子代的暴露
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0013
Miki Arian Saputra, Eka Djatnika Nugraha, Tri Purwanti, Rokhmat Arifianto, Roza Indra Laksmana, R. P. Hutabarat, M. Hosoda, S. Tokonami
Abstract The exposure from radon, thoron, and thoron progeny was measured for 45 dwellings in high background radiation area in Takandeang, Indonesia with ambient dose equivalent rate ranging from 0.34 μSv h−1 to 1.90 μSv h−1. The measurement was taken using passive radon and thoron discriminative detector and thoron progeny detector. This measurement was taken from November 2018 to October 2019, and within one month the detector would be replaced with a new detector. The concentrations of radon, thoron, and thoron progeny were calculated as 42–490 Bq m−3, 20–618 Bq m−3, and 4–40 Bq m−3, respectively. The concentrations for outdoor were 49–435 Bq m−3, 23–457 Bq m−3, and 4–37 Bq m−3, respectively, and the annual effective dose was 9.8–28.6 mSv y−1. Based on the result of Spearman’s correlations analysis between the indoor radon and thoron concentrations and between the indoor thoron progeny and thoron concentrations, we suggest that exposure to thoron cannot be predicted from exposure to radon, and the equilibrium equivalent thoron concentration has a large uncertainty when it is estimated from thoron concentration assuming a single thoron equilibrium factor.
摘要以0.34 ~ 1.90 μSv h - 1的环境剂量当量率,对印度尼西亚Takandeang高本底辐射区45户居民的氡、钍和钍子代暴露进行了测量。采用被动氡钍鉴别检测器和钍子代检测器进行测量。该测量于2018年11月至2019年10月进行,并在一个月内将探测器更换为新探测器。氡、钍和钍子体浓度分别为42 ~ 490 Bq m−3、20 ~ 618 Bq m−3和4 ~ 40 Bq m−3。室外浓度分别为49 ~ 435 Bq m−3、23 ~ 457 Bq m−3和4 ~ 37 Bq m−3,年有效剂量为9.8 ~ 28.6 mSv y−1。基于Spearman对室内氡与氡浓度、室内氡子代与氡浓度的相关性分析结果,认为氡暴露不能预测室内氡暴露,且假设单一氡平衡因子,由氡浓度估算出的平衡当量氡浓度存在较大不确定性。
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引用次数: 15
Seasonal variation of radon and CO2 in the Važecká Cave, Slovakia 斯洛伐克Važecká洞穴中氡和CO2的季节变化
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0025
I. Smetanová, K. Holý, Ľubica Luhová, K. Csicsay, Dagmar Haviarová, L. Kunáková
Abstract The continuous monitoring of 222Rn activity concentration, CO2 concentration, and microclimatologic parameters (internal air temperature and relative humidity) in the Važecká Cave (Northern Slovakia) is being carried out at three monitoring stations, namely, Gallery, Lake Hall, and Entrance Hall. Radon activity concentration and CO2 concentration exhibited a clear annual variation. The daily average of radon concentration ranged 1300–27 700 Bq/m3 at the Lake Hall station and 3600–42 200 Bq/m3 at the Gallery station. Radon reached its maximum in the summer months, from June to September. The annual maximum of CO2 concentration is registered approximately one month later than radon maximum. The annual variation of radon and CO2 is controlled by the seasonal change of ventilation regime associated with the seasonal variation of the difference between the temperature measured inside the cave and the atmospheric temperature.
摘要对北斯洛伐克Važecká洞穴内的222Rn活性浓度、CO2浓度和小气候参数(室内温度和相对湿度)进行了连续监测,监测站分别为画廊、湖厅和入口厅。氡活度浓度和CO2浓度具有明显的年际变化。湖霍尔站氡日平均值为1300 ~ 27700 Bq/m3,画廊站氡日平均值为3600 ~ 42200 Bq/m3。氡在夏季的6 - 9月达到最大值。二氧化碳的年最高浓度比氡的年最高浓度大约晚一个月。氡和CO2的年变化受通风制度的季节变化和洞内测温与大气温度之差的季节变化的控制。
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引用次数: 9
Radon intercomparison tests – Katowice, 2016 氡相互比较试验——卡托维兹,2016年
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0020
S. Chałupnik, K. Skubacz, M. Wysocka, J. Mazur, M. Bonczyk, K. Kozak, D. Grządziel, P. Urban, D. Tchorz-Trzeciakiewicz, B. Kozłowska, A. Walencik-Łata, A. Podstawczyńska, J. Olszewski, J. Bartak, M. Karpińska, K. Wołoszczuk, M. Dohojda, J. Nowak, M. Długosz-Lisiecka, E. Foerster, T. Przylibski
Abstract At the beginning of the year 2016, the representatives of the Polish Radon Centre decided to organize proficiency tests (PTs) for measurements of radon gas and radon decay products in the air, involving radon monitors and laboratory passive techniques. The Silesian Centre for Environmental Radioactivity of the Central Mining Institute (GIG), Katowice, became responsible for the organization of the PT exercises. The main reason to choose that location was the radon chamber in GIG with a volume of 17 m3, the biggest one in Poland. Accordingly, 13 participants from Poland plus one participant from Germany expressed their interest. The participants were invited to inform the organizers about what types of monitors and methods they would like to check during the tests. On this basis, the GIG team prepared the proposal for the schedule of exercises, such as the required level(s) of radon concentrations, the number and periods of tests, proposed potential alpha energy concentration (PAEC) levels and also the overall period of PT. The PT activity was performed between 6th and 17th June 2016. After assessment of the results, the agreement between radon monitors and other measurement methods was confirmed. In the case of PAEC monitors and methods of measurements, the results of PT exercises were consistent and confirmed the accuracy of the calibration procedures used by the participants. The results of the PAEC PTs will be published elsewhere; in this paper, only the results of radon intercomparison are described.
摘要2016年初,波兰氡中心的代表决定组织能力测试,以测量空气中的氡气和氡衰变产物,包括氡监测器和实验室被动技术。卡托维兹中央矿业研究所西里西亚环境放射性中心负责PT演习的组织工作。选择该位置的主要原因是GIG中体积为17 m3的氡室,是波兰最大的氡室。因此,来自波兰的13名与会者加上来自德国的一名与会者表达了他们的兴趣。参与者被邀请告知组织者他们希望在测试期间检查哪些类型的监视器和方法。在此基础上,GIG团队编制了演习时间表的提案,如所需的氡浓度水平、测试次数和周期、拟议的潜在α能量浓度(PAEC)水平以及PT的整个周期。PT活动于2016年6月6日至17日进行。在对结果进行评估后,确认了氡监测仪与其他测量方法之间的一致性。在PAEC监测器和测量方法的情况下,PT练习的结果是一致的,并证实了参与者使用的校准程序的准确性。PAEC PT的结果将在其他地方公布;本文仅介绍氡相互比较的结果。
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引用次数: 3
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