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Combined analysis of onco-epidemiological studies of the relationship between lung cancer and indoor radon exposure 癌症与室内氡暴露关系的肿瘤流行病学联合分析
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0012
I. Yarmoshenko, G. Malinovsky
Abstract Objectives: Recent results of epidemiological and medical statistics studies of lung cancer and indoor radon in different regions of the world make a relevant new combined analysis of residential exposure health effects. In particular, new data were obtained by means of a meta-analysis of case-control studies as well as taking into account a confounding effect of human papillomavirus infection in studies of geographically aggregated data. Materials and methods: Two sources of epidemiological data are considered: (1) studies of ecological design and (2) case-control studies. Ecological studies included the analysis performed for the USA counties and Russian oblasts with adjusting for the main confounders. Data on the case-control studies were gained from the meta-analysis of 31 individual studies with a weighting of obtained odds ratios according to the quality of radon exposure reconstruction and size of the reference group. Estimations of lung cancer excess relative risk (ERR) associated with indoor radon exposure are combined. Results: Two types of epidemiological study design provided generally consistent EER estimations. The combined value of ERR due to radon exposure is 0.14 (90% CI: 0.10–0.18) per 100 Bq/m3. Conclusion: Available geographically aggregated data in regions of Russia and the United States and the meta-analysis of case-control studies conducted in a large number of countries confirm the association of lung cancer with indoor radon exposure.
摘要目的:根据近年来世界不同地区肺癌和室内氡流行病学及医学统计研究结果,对居住暴露对健康的影响进行了新的综合分析。特别是,新数据是通过病例对照研究的荟萃分析获得的,并在地理汇总数据的研究中考虑了人乳头瘤病毒感染的混淆效应。材料和方法:考虑了两种流行病学数据来源:(1)生态设计研究和(2)病例对照研究。生态学研究包括对美国各县和俄罗斯各州进行的分析,并对主要混杂因素进行了调整。病例对照研究的数据来自对31项单独研究的荟萃分析,并根据氡暴露重建的质量和参照组的规模对获得的优势比进行加权。合并了与室内氡暴露有关的肺癌过度相对危险度(ERR)的估计。结果:两种类型的流行病学研究设计提供了大致一致的EER估计。氡暴露ERR的综合值为每100 Bq/m3 0.14 (90% CI: 0.10-0.18)。结论:俄罗斯和美国地区现有的地理汇总数据以及在许多国家进行的病例对照研究的荟萃分析证实,肺癌与室内氡暴露有关。
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引用次数: 5
Characterizing urban pollution variability in Central Poland using radon-222 用氡-222表征波兰中部城市污染变异性
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0008
S. Chambers, A. Podstawczyńska
Abstract Four years of observations of radon, meteorology and atmospheric pollution was used to demonstrate the efficacy of combined diurnal and synoptic timescale radon-based stability classification schemes in relating atmospheric mixing state to urban air quality in Zgierz, Central Poland. Nocturnal radon measurements were used to identify and remove periods of non-stationary synoptic behaviour (13–18% of each season) and classify the remaining data into five mixing states, including persistent temperature inversion (PTI) conditions, and non-PTI conditions with nocturnal conditions ranging from well mixed to stable. Mixing state classifications were performed completely independently of site meteorological measurements. World Health Organization guideline values for daily PM2.5/PM10 were exceeded only under strong PTI conditions (3–15% of non-summer months) or often under non-PTI stable nocturnal conditions (14–20% of all months), when minimum nocturnal mean wind speeds were also recorded. In non-summer months, diurnal amplitudes of NO (CO) increased by the factors of 2–12 (3–7) from well-mixed nocturnal conditions to PTI conditions, with peak concentrations occurring in the morning/evening commuting periods. Analysis of observations within radon-derived atmospheric mixing ‘class types’ was carried out to substantially clarify relationships between meteorological and air quality parameters (e.g. wind speed vs. PM2.5 concentration, and atmospheric mixing depth vs. PM10 concentration).
摘要利用四年来对氡、气象和大气污染的观测,证明了基于氡的日尺度和天气时间尺度组合稳定性分类方案在将波兰中部兹捷尔茨的大气混合状态与城市空气质量联系起来方面的有效性。夜间氡测量用于识别和消除非平稳天气行为的周期(每个季节的13-18%),并将剩余数据分为五种混合状态,包括持续逆温(PTI)条件和夜间条件从良好混合到稳定的非PTI条件。混合状态分类完全独立于现场气象测量进行。世界卫生组织每日PM2.5/PM10的指导值仅在强烈的PTI条件下(非夏季月份的3-15%)或通常在非PTI稳定的夜间条件下(所有月份的14-20%)超过,同时还记录了最低夜间平均风速。在非夏季月份,从混合良好的夜间条件到PTI条件,NO(CO)的日振幅增加了2–12(3–7)倍,峰值浓度出现在早晚通勤时段。对氡衍生的大气混合“类别”内的观测结果进行了分析,以充分阐明气象和空气质量参数之间的关系(例如风速与PM2.5浓度的关系,以及大气混合深度与PM10浓度的关系)。
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引用次数: 1
Radon in houses of Kowary – Sudety Mountains, Poland 波兰苏德代山脉科瓦里房屋中的氡
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0024
J. Olszewski, K. Walczak
Abstract The presence of uranium makes the Kowary area characterized by an increased concentration of radon in the air and the living houses. Measurements of periodic radon concentrations in dwellings of Kowary were carried out three times in the last 20 years. It can be observed that 20 years ago level of radon concentrations in houses of Kowary were lower than today. Measurements carried out in Kowary over 20 years have shown that residents are exposed to radon concentrations, which often exceed 300 Bq m−3 – a reference level recommended by the European Union. The present geometric mean of radon concentration in houses of Kowary (260 Bq m−3) exceeds the geometric mean of radon concentration of buildings in the rest of Poland (142 Bq m−3).
铀的存在使科瓦里地区的空气和居住房屋中的氡浓度增加。在过去20年中,我们三次测量了科瓦里民居的周期性氡浓度。可以观察到,20年前的房屋氡浓度水平比今天要低。20多年来在科瓦利进行的测量表明,居民接触的氡浓度经常超过300 Bq m - 3,这是欧盟建议的参考水平。目前科瓦里房屋氡浓度的几何平均值(260 Bq m−3)超过波兰其他地区建筑物氡浓度的几何平均值(142 Bq m−3)。
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引用次数: 0
Radon and thoron exhalation rate measurements from building materials used in Serbia 塞尔维亚使用的建筑材料的氡和钍排放率测量
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0017
I. Čeliković, G. Pantelić, M. Živanović, I. Vukanac, J. K. Krneta Nikolić, A. Kandić, B. Lončar
Abstract The second most important source of indoor radon, after soil beneath dwelling, is building material. With the increase in environmental awareness and new energy-saving policies, residents tend to replace the existing windows with tighter windows, which leads to a decrease in air exchange rate and consequently an increase in indoor radon concentration. In case of low exchange rates, dose caused by inhalation of radon and its progeny can exceed external dose originating from the radium content in the surrounding building material. In this paper, surface exhalation rates of radon (222Rn) and thoron (220Rn) from typical building materials used for construction and interior decoration of houses in Serbia were investigated. Surface exhalation rate measurements were performed using the closed-chamber method, while concentrations of radon and thoron in the chamber were continuously measured using an active device, RTM1688-2, produced by SARAD® GmbH. Finally, the impact of the replacement of windows on the indoor radon concentration was estimated.
室内氡的第二大来源是建筑材料,仅次于住宅下面的土壤。随着环保意识的增强和新的节能政策,居民倾向于用更紧的窗户取代现有的窗户,这导致空气交换率降低,从而导致室内氡浓度增加。在低交换率的情况下,吸入氡及其子体所引起的剂量可能超过由周围建筑材料中镭含量引起的外部剂量。本文调查了塞尔维亚用于建筑和室内装饰的典型建筑材料中氡(222Rn)和钍(220Rn)的表面呼出率。表面呼出率测量采用封闭室法进行,而氡和钍的浓度连续测量使用有源装置,RTM1688-2,由SARAD®GmbH生产。最后,估计了更换窗户对室内氡浓度的影响。
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引用次数: 3
Parameter sensitivity analysis of the theoretical model of a CR-39-based direct 222Rn/220Rn progeny monitor 基于CR-39的222Rn/220Rn子代监测仪理论模型的参数敏感性分析
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0014
Jun Hu, M. Hosoda, S. Tokonami
Abstract The deposition-based direct indoor 222Rn and 220Rn progeny measurement techniques are mostly affected by the indoor environmental conditions, such as the ventilation, concentration of condensation nuclei, and reactions with the structure and its furnishings. In this study, a theoretical model of a direct 222Rn and 220Rn progeny monitor based on allyl diglycol carbonate (ADC or CR-39) was established to analyse the factors that influence the detection process by using the parameter sensitivity analysis. The aerosol parameters contributed the highest to the variance, followed by the aerodynamic parameters. With respect to the result of the Spearman’s correlation analysis, the aerosol-related and the room-related parameters are positive, whereas the aerodynamic parameters – which affect the turbulence of indoor deposition – are negative. It means that both the attachment process and the deposition process of 222Rn and 220Rn progenies are important to the performance of the progeny monitor.
摘要基于沉积的室内222Rn和220Rn子代直接测量技术主要受室内环境条件的影响,如通风、冷凝核浓度以及与结构及其家具的反应。在本研究中,建立了基于碳酸烯丙基二甘醇(ADC或CR-39)的222Rn和220Rn子代直接监测仪的理论模型,通过参数灵敏度分析来分析影响检测过程的因素。气溶胶参数对方差的贡献最大,其次是空气动力学参数。关于Spearman相关性分析的结果,气溶胶相关参数和房间相关参数为正,而影响室内沉积湍流的空气动力学参数为负。这意味着222Rn和220Rn后代的附着过程和沉积过程对后代监测器的性能都很重要。
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引用次数: 2
Radon on the ground floor in the buildings of pre-university education in Montenegro 黑山大学预科教育大楼一楼的氡
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0007
P. Vukotic, R. Zekić, Tomislav Andjelić, N. Svrkota, A. Djurovic, A. Dlabac
Abstract A national radon survey was performed recently in all buildings of pre-university education in Montenegro. During the school year 2016/2017, radon (222Rn) was measured with passive detectors (Radosys, RSFV type) in 2855 ground-floor rooms of 468 buildings. The average 9-month radon activity concentrations above the level of 300 Bq/m3 were found in 728 rooms, which belong to 213 buildings, while in 111 rooms, belonging to 47 buildings, they were above 1000 Bq/m3. Radon concentrations in the educational buildings, averaged over all sampled ground-floor rooms in a building, range from 16 Bq/m3 to 2810 Bq/m3, with arithmetic mean (AM) = 275 Bq/m3. They follow a log-normal distribution with geometric mean (GM) = 174 Bq/m3 and geometric standard deviation (GSD) = 2.58. There are 135 buildings with average indoor radon concentrations on the ground floor above 300 Bq/m3 and 18 buildings where they are above 1000 Bq/m3. The influence of the nine factors (climate, urban/rural area, age of building, number of stories, building materials, basement, foundation slab, window frames, and heating) on radon concentrations in the buildings was analysed by univariate (UVA) and multivariate (MVA) methods. The univariate analysis revealed the significant relationship of the four factors: age of buildings, basement, building materials, and window frames with radon concentrations on the ground floor in the buildings, while multivariate analysis added to those factors urban/rural area and number of stories, but excluded building materials as a factor influencing significantly radon concentrations.
摘要最近在黑山所有大学前教育的建筑中进行了一次全国氡调查。2016/2017学年,在468栋建筑的2855个底层房间中,使用无源探测器(Radosys,RSFV型)测量了氡(222Rn)。在213栋建筑的728个房间中发现了超过300 Bq/m3水平的9个月平均氡活动浓度,而在47栋建筑的111个房间中,氡活动浓度超过1000 Bq/m3。教育建筑中的氡浓度,在一栋建筑的所有底层房间取样的平均值范围为16 Bq/m3至2810 Bq/m3,算术平均值(AM)=275 Bq/m3。它们遵循对数正态分布,几何平均值(GM)=174Bq/m3,几何标准差(GSD)=2.58。一楼有135栋建筑的室内氡平均浓度超过300 Bq/m3,18栋建筑的氡平均浓度高于1000 Bq/m3。采用单变量(UVA)和多变量(MVA)方法分析了九个因素(气候、城市/农村地区、建筑年代、层数、建筑材料、地下室、地基板、窗框和供暖)对建筑物中氡浓度的影响。单变量分析揭示了四个因素:建筑物的年龄、地下室、建筑材料和窗框与建筑物底层氡浓度的显著关系,而多变量分析增加了城市/农村地区和层数的因素,但排除了建筑材料作为显著影响氡浓度的因素。
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引用次数: 2
National comparison of methods for determination of radon in water 水中氡测定方法的全国比较
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0011
J. Mazur, K. Kozak, D. Grządziel, Szymon Guguła, M. Mroczek, B. Kozłowska, A. Walencik-Łata, Zuzanna Podgórska, K. Wołoszczuk, T. Przylibski, A. Kowalska, Elżbieta Domin, M. Wysocka, S. Chałupnik, I. Chmielewska, M. Długosz-Lisiecka, P. Szajerski, N. D. Chau, P. Krakowska, T. Pliszczyński, J. Ośko, Małgorzata Dymecka, D. Mazurek
Abstract The article describes three interlaboratory experiments concerning 222Rn determination in water samples. The first two experiments were carried out with the use of artificial radon waters prepared by the Laboratory of Radiometric Expertise (LER), Institute of Nuclear Physics, Polish Academy of Sciences in Kraków in 2014 and 2018. The third experiment was performed using natural environment waters collected in the vicinity of the former uranium mine in Kowary in 2016. Most of the institutions performing radon in water measurements in Poland were gathered in the Polish Radon Centre Network, and they participated in the experiments. The goal of these exercises was to evaluate different measurement techniques used routinely in Polish laboratories and the laboratories’ proficiency of radon in water measurements. In the experiment performed in 2018, the reference values of 222Rn concentration in water were calculated based on the method developed at LER. The participants’ results appeared to be worse for low radon concentration than for high radon concentrations. The conclusions drawn on that base indicated the weaknesses of the used methods and probably the sampling. The interlaboratory experiments, in term, can help to improve the participants’ skills and reliability of their results.
摘要本文介绍了水样中222Rn测定的三个实验室间实验。前两次实验分别于2014年和2018年在Kraków使用波兰科学院核物理研究所辐射专业实验室(LER)制备的人工氡水进行。第三个实验是2016年在科瓦里前铀矿附近收集的自然环境水。在波兰进行水中氡测量的大多数机构都聚集在波兰氡中心网络,它们参加了实验。这些活动的目的是评价波兰实验室常规使用的不同测量技术以及实验室在水测量中对氡的熟练程度。在2018年进行的实验中,基于LER开发的方法计算了水中222Rn浓度参考值。参与者的结果似乎在低氡浓度下比在高氡浓度下更差。在此基础上得出的结论表明所使用方法的弱点,可能也包括抽样的弱点。从术语上讲,实验室间实验可以帮助提高参与者的技能和结果的可靠性。
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引用次数: 0
Configuration of the parameters for scanner-based track detector evaluation system 基于扫描仪的轨道探测器评估系统的参数配置
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0021
A. Csordás, E. Tóth-Bodrogi, T. Kovács
Abstract According to the new European Union Basic Safety Standards (EU-BSS), preparation of the National Radon Action Plan is obligatory for the Member States. One of the plan’s aims is to carry out an indoor radon survey to identify radon-prone areas. In the radon surveys, track detector methods are used. At the University of Pannonia (Veszprém, Hungary), a new scanner-based detector evaluation system has been developed. For the application of the new system, the selection of appropriate parameters is necessary. In this study, selection of the applied track detectors and setting of the etching conditions have been carried out. Two different types of allyl diglycol carbonate (ADC or CR-39) track detectors were investigated, taking into account the detector’s background and response during the exposure (determination of calibration factor). The Baryotrak’s background track density (0–1.5 tracks mm−2) was lower than that of the 0.8–4 tracks mm−2. The response of the Tastrak was higher, but the deviation of the calibration factor was much higher (1.2–5.3 × 10−3 tracks mm−2/(Bq day m−3)) than in the case of the Baryotrak (1.4–2.8 × 10−3 tracks mm−2/(Bq day m−3)). After the systematic review of the etching system, a new method was developed. For the determination of the optimal track diameter, the argon fluoride (ArF) laser was applied to create tracks with diameters in the range of 10–100 μm. The optimum track size was in the range of 40–60 μm. On this basis, new etching conditions were determined: 6.25 M NaOH solution, a temperature of 90°C, and time period of 8 hours.
摘要根据新的欧洲联盟基本安全标准(EU-BSS),制定国家氡行动计划是成员国的义务。该计划的目标之一是进行室内氡调查,以确定氡易发地区。在氡调查中,使用了轨道探测器方法。在潘诺尼亚大学(匈牙利Veszprém),开发了一种新的基于扫描仪的探测器评估系统。为了应用新系统,有必要选择适当的参数。在本研究中,选择了应用的轨道探测器和设置了蚀刻条件。研究了两种不同类型的碳酸二甘醇烯丙酯(ADC或CR-39)轨道探测器,考虑了探测器的背景和暴露过程中的响应(校准因子的确定)。Baryotrak的背景轨道密度(0–1.5轨道毫米-2)低于0.8–4轨道毫米-2。Tastrak的响应更高,但校准因子的偏差(1.2–5.3×10−3轨道mm−2/(Bq day m−3))远高于Baryotrak的情况(1.4–2.8×10−3-轨道mm−3/(Bq daym−3。在对蚀刻系统进行系统回顾后,开发了一种新的方法。为了确定最佳轨道直径,应用氟化氩(ArF)激光创建直径在10–100μm范围内的轨道。最佳轨道尺寸在40–60μm范围内。在此基础上,确定了新的蚀刻条件:6.25M NaOH溶液,温度为90°C,时间为8小时。
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引用次数: 1
Radon soil-gas measurement campaign in Hessen: an approach to identifying areas with enhanced geogenic radon 黑森州氡土气测量活动:确定地源性氡增强地区的方法
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0022
T. Kuske, Steffen Kerker, J. Breckow, R. Lehné, Tatjana Laupenmühlen, Lena Jedmowski
Abstract The new radiation protection law in Germany, which came into effect 2018, puts greater emphasis on the protection against naturally occurring radiation, especially radon as a known health hazard. The law requires the delineation of radon priority areas, where prevention and remediation of high indoor radon concentrations should be taken with priority. In Germany, radiation protection is the administrative responsibility of the federal states. The state of Hesse has early on decided to fully survey the state for radon priority areas. To identify radon priority areas, the geogenic radon potential has to be determined. To achieve that radon, soil-gas measurements combined with soil permeability are a necessity. The University of Applied Sciences (THM) in Giessen is responsible for the radon soil-gas measurement campaign in Hessen. To achieve a statistically sound survey of the state of Hessen with an achievable amount of different measurement locations, and in the given time-frame, a geology-based concept has been designed. Taking into account the known geological information about geological structures in combination with the administrative counties, a survey strategy has been established. Prior known information regarding soil thickness, moisture, digability, and other technical limitations are used to determine the exact measuring locations. At every location, the radon activity in soil gas is measured. The soil permeability is determined for every measurement as well. Three measurements are performed at each location. Having completed the first set of measurements, the design criteria of the campaign and the practical experiences will be presented.
德国新的辐射保护法于2018年生效,更加强调对自然产生的辐射的保护,特别是氡作为已知的健康危害。法律要求划定氡优先区域,在这些区域应优先采取预防和补救室内高浓度氡的措施。在德国,辐射防护是联邦各州的行政责任。黑森州很早就决定全面调查该州的氡优先区域。为了确定氡优先区,必须确定地质氡势。为了获得氡,土壤气体测量与土壤渗透性相结合是必要的。位于吉森的应用科学大学(THM)负责黑森州的氡土壤气体测量活动。为了在给定的时间框架内实现对黑森州进行统计上合理的调查,并实现不同测量地点的可实现数量,设计了基于地质的概念。考虑到已知的地质构造地质信息,结合行政县,制定了调查策略。先前已知的有关土壤厚度、湿度、易碎性和其他技术限制的信息被用来确定精确的测量位置。在每个地点,测量土壤气体中的氡活度。每一次测量都要确定土壤渗透性。在每个位置进行三次测量。在完成第一组测量后,将介绍活动的设计标准和实践经验。
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引用次数: 0
A technology of drinking water decontamination from radon and its decay products 饮用水氡及其衰变产物的净化技术
IF 0.7 4区 物理与天体物理 Q4 CHEMISTRY, INORGANIC & NUCLEAR Pub Date : 2020-05-29 DOI: 10.2478/nuka-2020-0009
I. Voinov, V. P. Remez, A. A. Ioshin, V. Semenishchev, Dmitry A. Gorchakov
Abstract Underground water is one of the main sources of radon for households. This article focuses on the estimation and removal of radon from underground water using the technology and inorganic sorbents developed by EKSORB Ltd., Russia for liquid radioactive waste treatment in the nuclear power industry. The article presents the results of tests of a system for the removal of radon and radon daughters from water patented by EKSORB. This is achieved by filtering water through RATZIR sorbent, followed by periodic load regeneration. Over a period of three years, the plant is successful in removing radon from the water that had an initial radon content of approximately 1500 Bq/L to less than 60 Bq/L, without releasing radon to indoor/outdoor air.
摘要地下水是家庭氡的主要来源之一。本文主要介绍了利用俄罗斯EKSORB有限公司开发的用于核电工业放射性液体废物处理的技术和无机吸附剂对地下水中氡的估计和去除。本文介绍了一种由EKSORB专利的用于去除水中氡和氡子体的系统的测试结果。这是通过RATZIR吸附剂过滤水,然后定期负荷再生来实现的。在三年的时间里,该工厂成功地从最初氡含量约为1500 Bq/L至低于60 Bq/L的水中去除氡,而没有将氡释放到室内/室外空气中。
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引用次数: 1
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