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Electric‐field‐tunable bipolar linear magnetoelectric effect in zigzag graphene nanoribbon‐based antiferromagnet 基于之字形石墨烯纳米带的反铁磁体中电场可调双极线性磁电效应
Pub Date : 2023-08-30 DOI: 10.1002/pssr.202300228
W. Xie, Zhenzhen Qin, Yu Song, Bin Shao, Xu Zuo
Modern electronic devices are moving toward miniaturization and integration. Therefore, achieving electrical control of magnetization effectively in one‐dimensional materials represents a promising field for the practical applications in memory elements. In this study, it is discovered, from first‐principles calculations, that an electric‐field‐tunable bipolar linear magnetoelectric effect can be realized in one‐dimensional antiferromagnet based on double‐Gd‐adsorbed graphene nanoribbon with four zigzag carbon chains (2Gd‐4ZGNR). We find that, compared with the bare 4ZGNR, the adsorption of two Gd atoms on the 4ZGNR reduces the bandgap. As a result, 2Gd‐4ZGNR transits from antiferromagnetic semiconductor to ferrimagnetic metal at a relatively low critical external transverse (perpendicular) electric field, where the net magnetic moment can be induced. The antiferromagnetism and inversion‐symmetrical crystal structure further allow to realize a bipolar linear magnetoelectric effect, where the 2Gd‐4ZGNR form two groups of independent linear magnetic response states, acting as a magnetoelectric memory element.This article is protected by copyright. All rights reserved.
现代电子设备正朝着小型化和集成化的方向发展。因此,在一维材料中实现有效的磁化电控制是存储元件实际应用的一个有前景的领域。在这项研究中,从第一性原理计算中发现,电场可调的双极线性磁电效应可以在一维反铁磁体中实现,该反铁磁体基于双Gd吸附的具有四条之字形碳链的石墨烯纳米带(2Gd‐4ZGNR)。我们发现,与裸4ZGNR相比,两个Gd原子在4ZGNR上的吸附减小了带隙。结果,2Gd‐4ZGNR在相对较低的临界外部横向(垂直)电场下从反铁磁半导体过渡到铁磁金属,在那里可以诱导净磁矩。反铁磁性和反对称晶体结构进一步实现了双极线性磁电效应,其中2Gd‐4ZGNR形成两组独立的线性磁响应状态,充当磁电存储元件。这篇文章受版权保护。版权所有。
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引用次数: 0
Iridium/Silicon Ultrathin Film for Ultraviolet Photodetection: Harnessing Hot Plasmonic Effects 用于紫外光探测的铱/硅超薄膜:利用热等离子体效应
Pub Date : 2023-08-29 DOI: 10.1002/pssr.202300257
Mohamed A. Basyooni, M. Tihtih, I. Boukhoubza, J. F. Ibrahim, R. En-nadir, Ahmed M. Abdelbar, Khalid Rahmani, Shrouk E. Zaki, Ş. Ateş, Yasin Ramazan Eker
The phenomenon of hot carriers, which are generated through the nonradiative decay of surface plasmons in ultrathin metallic films, offers an intriguing opportunity for sub‐bandgap photodetection even at room temperature. These hot carriers possess sufficient energy to inject into the conduction band of a semiconductor material. The groundbreaking use of Iridium (Ir) ultrathin film as an ultraviolet (UV) plasmonic material on silicon (Si) for high‐performance photodetectors (PHDs) has been successfully demonstrated. Elevating the thickness of the sputtered Ir film to 4 nm yielded a notable surge in photocurrent, registering an impressive 600 µA under 365 nm UV illumination with electron mobility of 1.37E3 cm²/V·s. This PHD exhibited excellent OFF‐ON Photoresponses at various applied voltages ranging from 0 V to 5 V, maintaining a stable photocurrent. Under UV illumination, it displayed exceptional performance, achieving a high detectivity of 1.25E14 Jones and a responsivity of 1.28 A/W. These outstanding results underscore the significant advantages of increasing the thickness of the Ir film in PHDs, leading to improvements in conductivity, detectivity, external quantum efficiency, responsivity, as well as superior sensitivity for light detection.This article is protected by copyright. All rights reserved.
热载流子现象是由超薄金属薄膜中表面等离子体的非辐射衰变产生的,即使在室温下也为亚带隙光探测提供了一个有趣的机会。这些热载流子具有足够的能量注入半导体材料的导带。突破性地使用铱(Ir)超薄膜作为硅(Si)上的紫外(UV)等离子体材料,用于高性能光电探测器(博士)已经成功证明。将溅射Ir薄膜的厚度增加到4nm,光电流显著增加,在365nm紫外光照射下达到600µa,电子迁移率为1.37E3 cm²/V·s。该PHD在0 V至5 V的不同施加电压下表现出优异的OFF - ON光响应,保持稳定的光电流。在紫外线照射下,它表现出优异的性能,具有1.25E14 Jones的高探测率和1.28 a /W的响应率。这些突出的结果强调了增加Ir薄膜厚度的显着优势,从而提高了电导率,探测性,外量子效率,响应性以及光探测的优越灵敏度。这篇文章受版权保护。版权所有。
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引用次数: 1
Locally reconfigurable exchange bias for tunable spintronics by pulsed current injection 脉冲电流注入可调谐自旋电子学的局部可重构交换偏置
Pub Date : 2023-08-29 DOI: 10.1002/pssr.202300303
Wenli Wang, Yicheng Chen, Bo Wang, Lisong Wang, Yongliang Han, W. Su, Zhongqiang Hu, Zhiguang Wang, Meilin Liu
Unidirectional magnetic anisotropy induced by exchange bias (EB) between ferromagnetic and antiferromagnetic layers is of paramount importance in various spintronic devices. Traditional setting and optimization of EB involves cooling through the Néel temperature of the antiferromagnets under biasing field in vacuum furnace which takes hours of time and could not realize localized control of EB. Here, we report an alternative process to configure EB by injection of microsecond current impulse for locally heating of the heterostructure. 180‐degree exchange bias switching has been realized in both anisotropic magnetoresistance and giant magnetoresistance units, resulting in tunable magnetic field sensing functionalities. This mechanism for pinpoint control of EB provides more freedom for design and optimization of various sensing and logic spintronics.This article is protected by copyright. All rights reserved.
由铁磁层和反铁磁层之间的交换偏置(EB)引起的单向磁各向异性在各种自旋电子器件中至关重要。传统的EB设定和优化是在真空炉中对偏置场下的反铁磁体进行n温度冷却,耗时数小时,无法实现EB的局部控制。在这里,我们报告了一种通过注入微秒电流脉冲来局部加热异质结构来配置EB的替代工艺。在各向异性磁阻和巨磁阻单元中都实现了180度交换偏置开关,从而实现了可调谐的磁场传感功能。这种精确控制机制为各种传感和逻辑自旋电子学的设计和优化提供了更大的自由度。这篇文章受版权保护。版权所有。
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引用次数: 0
Nickel‐related centers in HPHT microdiamonds for near‐infrared luminescent thermometry 用于近红外发光测温的HPHT微金刚石中的镍相关中心
Pub Date : 2023-08-29 DOI: 10.1002/pssr.202300277
N. S. Kurochkin, V. Sychev, A. V. Gritsienko, D. Bi
Nano‐ and microcrystals of diamond are attractive for optical thermometry applications and possess unique optical properties as well as high chemical stability and biocompatibility. For biological application there are interest of diamonds with color centers that emit in the biological transparency window. One such defect is nickel‐related color centers that radiate in the near‐infrared range (1.4‐eV Ni centers), but have not yet been sufficiently investigated. This study reports the optical characteristics of HPHT diamond microcrystals with average sizes of 4 μm and 30 μm containing 1.4‐eV Ni centers. The temperature dependence of the spectral and temporal properties of Ni center emissions in the range from room temperature to 85 °C was demonstrated and thereby the possibility of appliance these centers as temperature sensors. The relative temperature sensitivities of luminescence peak intensity and lifetime for Ni centers were found to be 1.3% K−1 and 0.42% K−1, respectively. Moreover, the temperature determination accuracy reached better than 1 K.This article is protected by copyright. All rights reserved.
金刚石的纳米晶体和微晶体在光学测温应用中具有吸引力,具有独特的光学特性以及高化学稳定性和生物相容性。对于生物应用,人们对具有在生物透明窗口中发光的色心的金刚石感兴趣。其中一个缺陷是镍相关的色心,它在近红外范围内辐射(1.4 eV镍中心),但尚未得到充分的研究。本研究报道了平均尺寸为4 μm和30 μm的含1.4 eV Ni中心的HPHT金刚石微晶的光学特性。在室温至85°C范围内,Ni中心发射光谱和时间特性的温度依赖性得到了证明,从而证明了应用这些中心作为温度传感器的可能性。Ni中心发光峰强度和寿命的相对温度敏感度分别为1.3% K−1和0.42% K−1。测温精度达到1 K以上。这篇文章受版权保护。版权所有。
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引用次数: 0
Doping modification of Cs3Bi2I9 single crystals for high performance X‐ray detectors 用于高性能X射线探测器的Cs3Bi2I9单晶掺杂改性
Pub Date : 2023-08-25 DOI: 10.1002/pssr.202300306
Anfeng Li, Manman Yang, Aoxi He, Peng Tang, X. Hao, Lili Wu, Wenbo Tian, Dingyu Yang, Jingquan Zhang
Cs3Bi2I9 (CBI) is a promising material for direct X‐ray detectors. However, for the solution method, due to the difference in the chemical potential of Cs+, Bi3+, ​​I‐ ions in the solvent, the composition of Cs3Bi2I9 single crystals (SC) prepared by the solution method often deviates from the stoichiometric ratio, resulting in the formation of many defects in the material, which degrades the quality of the SC. In this work, Br‐ and Cl‐ were used as dopants to produce CBI SCs by the top seed solution method. It can be speculated that the dopant ions could reduce the VI defects in the CBI by means of density functional theory (DFT) calculations. The carrier lifetimes of CBI SCs doped with Br‐ and Cl‐ have been increased to 41.7 ns and 13.0 ns, respectively. Meanwhile, the defect densities of the SCs were reduced to 1.02×109 cm‐3 and 1.85×109 cm‐3, respectively. X‐ray detectors based on Br‐doped CBI and Cl‐doped CBI SCs exhibited high X‐ray sensitivity of 23071.3 μC Gyair‐1cm‐2 and 18525.3 μC Gyair‐1cm‐2 at an electric field of 40 V mm‐1, respectively. In addition, the X‐ray detection limit reaches 1.07 nGyairs‐1 and 1.35 nGyairs‐1 at an electric field of 2.5 V mm‐1, respectively.This article is protected by copyright. All rights reserved.
Cs3Bi2I9 (CBI)是一种很有前途的X射线直接探测器材料。然而,溶液法制备的Cs3Bi2I9单晶(SC)由于溶剂中Cs+、Bi3+、I‐离子的化学势不同,其组成往往偏离化学计量比,导致材料中形成许多缺陷,从而降低了SC的质量。本研究以Br‐和Cl‐为掺杂剂,采用top seed溶液法制备了CBI SC。通过密度泛函理论(DFT)计算可以推测,掺杂离子可以减少CBI中的VI缺陷。掺入Br‐和Cl‐的CBI SCs的载流子寿命分别提高到41.7 ns和13.0 ns。同时,sc的缺陷密度分别降至1.02×109 cm‐3和1.85×109 cm‐3。基于Br掺杂CBI和Cl掺杂CBI sc的X射线探测器在40 V mm‐1电场下分别表现出23071.3 μC Gyair‐1cm‐2和18525.3 μC Gyair‐1cm‐2的高X射线灵敏度。此外,在2.5 V mm‐1电场下,X射线检测极限分别达到1.07和1.35 nGyairs‐1。这篇文章受版权保护。版权所有。
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引用次数: 0
Visible to Short Wave Infrared Broadband p‐WSe2/n‐Ge Heterojunction Phototransistor with an Annular Shallow‐Trench Schottky Barrier Collector 短波红外可见宽带p - WSe2/n - Ge异质结光电晶体管与环形浅沟肖特基势垒集电极
Pub Date : 2023-08-25 DOI: 10.1002/pssr.202300276
Shuo Li, Xinwei Cai, Haokun Ding, Qiang Wu, Songsong Wu, Guangyang Lin, Wei Huang, Songyan Chen, Cheng Li
Van der Waals (vdW) heterostructures based on two‐dimensional materials and conventional group IV semiconductors have shown great potential for wide spectrum, highly sensitive photodetectors owing to their broadband absorption, high‐quality interface, and compatibility with complementary metal‐oxide‐semiconductor (CMOS) technology. Here, we propose a unique heterojunction phototransistor composed of an indium tin oxide (ITO) capped p‐WSe2/n‐Ge vdW heterojunction serving as the emitter and an annular shallow‐trench Al/Ge Schottky junction acting as the collector. The mixed‐dimensional phototransistor exhibiting high responsivities up to 66 A W‐1 at 405 nm and 124 A W‐1 at 1550 nm demonstrates a brilliant wide spectrum response performance. The high photocurrent gain can be attributed to the extra‐large carrier injection ratio of the heterojunction. The short transient response time in the order of 100 µs is achieved with the modified lateral electrical field by the annular shallow‐trench Schottky barrier collector. The combination of p‐WSe2/n‐Ge vdW heterojunction and the annular shallow‐trench Al/n‐Ge Schottky junction renders a low‐cost, high‐performance photodetector fabricated in a simple and CMOS compatible way for visible to short wave infrared (SWIR) broadband detection.This article is protected by copyright. All rights reserved.
基于二维材料和传统IV族半导体的范德华(vdW)异质结构由于其宽带吸收、高质量界面和与互补金属氧化物半导体(CMOS)技术的兼容性,在宽光谱、高灵敏度光电探测器方面显示出巨大的潜力。在这里,我们提出了一种独特的异质结光电晶体管,由氧化铟锡(ITO)覆盖的p‐WSe2/n‐Ge vdW异质结作为发射极和环形浅沟Al/Ge肖特基结作为集电极组成。该混合维光电晶体管在405 nm处和1550 nm处分别表现出高达66 A和124 A的高响应度,具有出色的宽光谱响应性能。高光电流增益可归因于异质结的超大载流子注入比。环形浅沟肖特基势垒集电极在改变侧向电场的情况下,实现了100µs左右的瞬态响应时间。p - WSe2/n - Ge vdW异质结和环形浅沟槽Al/n - Ge肖特基结的结合,以简单和CMOS兼容的方式制造了一种低成本,高性能的光电探测器,用于可见光到短波红外(SWIR)宽带检测。这篇文章受版权保护。版权所有。
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引用次数: 1
In‐Plane Anisotropic Phonon‐Polaritonic Resonances with α‐MoO3 microdisks α - MoO3微盘的平面内各向异性声子极化共振
Pub Date : 2023-08-21 DOI: 10.1002/pssr.202300302
Hongjie Zhang, Xiang Li, Tong Qin, Lan Zhang, Wei Du, Peining Li, Tao Wang
Phonon polaritons (PhPs) in two‐dimensional van der Waals (vdW) crystals exhibit strong spatial confinement and long polariton lifetimes, making them promising for developing novel nanophotonic devices at mid‐infrared frequencies. Here, using α‐phase molybdenum trioxide (α‐MoO3) microdisks, we have demonstrated in‐plane anisotropic PhP resonances with degree of polarization (DoP) of almost 100% from far field observation. Such in‐plane polarization‐dependent PhP resonances, originating from the anisotropic crystal structure of α‐MoO3, are readily tuned by the disk length and fits well to numerical simulations. Our findings show new possibility for engineering in‐plane polarizers based on vdW crystals and may promote the development of functional polarization‐sensitive optoelectronic devices at mid‐infrared frequencies.This article is protected by copyright. All rights reserved.
二维范德华(vdW)晶体中的声子极化子(PhPs)具有很强的空间约束和较长的极化子寿命,这使得它们在开发中红外频率的新型纳米光子器件方面具有很大的前景。在这里,我们利用α相三氧化钼(α‐MoO3)微盘,在远场观测中证明了平面内各向异性的PhP共振,极化度(DoP)几乎为100%。这种源自α‐MoO3各向异性晶体结构的面内极化相关的PhP共振很容易受到圆盘长度的调节,并且很好地符合数值模拟。我们的发现显示了基于vdW晶体的工程平面偏振器的新可能性,并可能促进中红外频率功能偏振敏感光电子器件的发展。这篇文章受版权保护。版权所有。
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引用次数: 0
Multi‐subband Polar Optical Phonon Scattering in InAlN/AlN/GaN Heterostructures InAlN/AlN/GaN异质结构中的多子带极性光学声子散射
Pub Date : 2023-08-13 DOI: 10.1002/pssr.202300238
Qun Li, Yao Li, Yachao Zhang, Jincheng Zhang
The high density of two‐dimensional electron gas (2DEG) in InAlN/AlN/GaN heterostructures results in significant occupation of higher subbands, it is thus imperative to consider multi‐subband occupation and inter‐subband scattering in the calculations of polar optical phonon (POP) scattering. The physical parameters, such as subband energies, wave functions of the four lowest subbands, and Fermi level of InAlN/AlN/GaN heterostructures, are calculated by solving the Schrödinger‐Poisson equations and applied to the multi‐subband POP scattering model. The dependence of mobility, which is limited by multi‐subband POP scattering, on temperature and 2DEG density is studied. The results show that multi‐subband occupation and inter‐subband scattering play important roles in electron transport. The higher subbands contribute 26% to room‐temperature electron mobility. Two simplified POP scattering models, which either ignore multi‐subband occupation or simplify the in‐scattering processes are evaluated. The results show that both simplified models introduce significant deviations in the mobilities that are limited by POP scattering. The relative magnitudes of mobility in each subband depend on the energy dependence of momentum relaxation time and the energy distribution of each subband.This article is protected by copyright. All rights reserved.
在InAlN/AlN/GaN异质结构中,二维电子气体(2DEG)的高密度导致了较高子带的占据,因此在计算极性光学声子(POP)散射时必须考虑多子带占据和子带间散射。通过求解Schrödinger‐Poisson方程,计算了InAlN/AlN/GaN异质结构的子带能量、四个最低子带的波函数和费米能级等物理参数,并将其应用于多子带POP散射模型。研究了受多子带POP散射限制的迁移率与温度和2℃密度的关系。结果表明,多子带占据和子带间散射在电子输运中起重要作用。较高的子带对室温电子迁移率贡献了26%。对两种忽略多子带占用和简化内散射过程的简化POP散射模型进行了评价。结果表明,两种简化模型在受POP散射限制的移动量上都引入了明显的偏差。各子带中迁移率的相对大小取决于动量弛豫时间的能量依赖性和各子带的能量分布。这篇文章受版权保护。版权所有。
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引用次数: 0
A Tunable Fano Resonator with High Sensitivity Based on Black Phosphorus in the Terahertz Band 一种基于太赫兹黑磷的高灵敏度可调谐法诺谐振器
Pub Date : 2023-08-08 DOI: 10.1002/pssr.202300207
Hao Zhang, Xue-shi Li, Weijun Sun, Yonghui Huang, Yuanmei Xu, K. Wen, Naixing Feng
A Fano resonator using black phosphorus, capable of tuning the operating band while possessing high sensitivity, is proposed. A ring and a groove are respectively etched above and below the main channel to produce the Fano resonance, resulting in a highly sensitive Fano resonator. Such a sensor can capture slight changes in the surrounding environment. Moreover, adding black phosphorus into the ring above the channel and into the groove below the channel, the electron doping of black phosphorus can be altered to adjust the resonant frequency of the Fano resonator. The shiftable frequency of the Fano resonator designed herein can reach 57 GHz at the second‐order resonance around 1.895 THz, an ability highly attractive in fields that require high sensitivity and adjustability. It is essential in the area of integrated electronics, offers fresh perspectives for innovations in integrated electronic gadgets, and paves the way for flexible terahertz systems.
提出了一种使用黑磷的法诺谐振器,该谐振器在具有高灵敏度的同时能够调节工作频带。在主通道的上方和下方分别蚀刻环形和凹槽以产生法诺谐振,从而产生高灵敏度的法诺谐振器。这种传感器可以捕捉到周围环境的细微变化。此外,在通道上方的环形和通道下方的凹槽中加入黑磷,可以改变黑磷的电子掺杂,从而调节Fano谐振器的谐振频率。本文设计的法诺谐振器在1.895太赫兹左右二阶谐振时可调频率可达57 GHz,在需要高灵敏度和可调性的领域具有很强的吸引力。它在集成电子领域是必不可少的,为集成电子产品的创新提供了新的视角,并为灵活的太赫兹系统铺平了道路。
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引用次数: 0
Ge2Sb2Te5 thin film as a promising heat‐mode resist for high‐resolution direct laser writing lithography Ge2Sb2Te5薄膜作为一种有前途的热模抗蚀剂用于高分辨率直接激光书写光刻
Pub Date : 2023-08-05 DOI: 10.1002/pssr.202300262
Xingwang Chen, Lei Chen, Lihao Sun, Tao Wei, Yun Ling, Jing Hu, Miao Cheng, Qianqian Liu, Ruirui Wang, Wanfei Li, Bo Liu
Ge2Sb2Te5 thin film is investigated as a positive heat‐mode resist and environmentally‐friendlily FeCl3 solution is as means an efficient developer. The corrosion selectivity of exposed to as‐deposited thin film reaches 2.3 and the etching selectivity of Si to Ge2Sb2Te5 thin film is as high as 15.75. Moreover, high‐resolution nanostructures with minimum linewidth of 180 nm and period of 400 nm are obtained along with high resolution of 130 nm. In addition, the mechanism of corrosion selectivity between as‐deposited and exposed thin film is further elucidated based on microstructural analysis. Hence, Ge2Sb2Te5 thin film is a promising positive resist for high‐resolution direct laser writing lithography.This article is protected by copyright. All rights reserved.
研究了Ge2Sb2Te5薄膜作为一种正热模抗蚀剂和环境友好的FeCl3溶液作为一种高效的显影剂。暴露于沉积薄膜的腐蚀选择性达到2.3,Si对Ge2Sb2Te5薄膜的腐蚀选择性高达15.75。此外,还获得了最小线宽为180 nm,周期为400 nm的高分辨率纳米结构,并获得了130 nm的高分辨率。此外,基于微观结构分析,进一步阐明了沉积薄膜和暴露薄膜之间的腐蚀选择性机理。因此,Ge2Sb2Te5薄膜是一种很有前途的高分辨率直接激光书写光刻正极抗蚀剂。这篇文章受版权保护。版权所有。
{"title":"Ge2Sb2Te5 thin film as a promising heat‐mode resist for high‐resolution direct laser writing lithography","authors":"Xingwang Chen, Lei Chen, Lihao Sun, Tao Wei, Yun Ling, Jing Hu, Miao Cheng, Qianqian Liu, Ruirui Wang, Wanfei Li, Bo Liu","doi":"10.1002/pssr.202300262","DOIUrl":"https://doi.org/10.1002/pssr.202300262","url":null,"abstract":"Ge2Sb2Te5 thin film is investigated as a positive heat‐mode resist and environmentally‐friendlily FeCl3 solution is as means an efficient developer. The corrosion selectivity of exposed to as‐deposited thin film reaches 2.3 and the etching selectivity of Si to Ge2Sb2Te5 thin film is as high as 15.75. Moreover, high‐resolution nanostructures with minimum linewidth of 180 nm and period of 400 nm are obtained along with high resolution of 130 nm. In addition, the mechanism of corrosion selectivity between as‐deposited and exposed thin film is further elucidated based on microstructural analysis. Hence, Ge2Sb2Te5 thin film is a promising positive resist for high‐resolution direct laser writing lithography.This article is protected by copyright. All rights reserved.","PeriodicalId":20059,"journal":{"name":"physica status solidi (RRL) – Rapid Research Letters","volume":"28 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2023-08-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"88591643","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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physica status solidi (RRL) – Rapid Research Letters
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