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Entropically driven phase separation and effective multibody interactions in block copolymers. 嵌段共聚物中熵驱动相分离和有效多体相互作用。
IF 2.4 3区 物理与天体物理 Q1 Mathematics Pub Date : 2024-11-01 DOI: 10.1103/PhysRevE.110.054502
Xinyue Zhang, Mingge Zhao, Junhan Cho

The need for effective multibody interactions is asserted in understanding the entropically driven phase separation of diblock copolymers, arising from disparity in self cohesion and association between dissimilar components. Through Landau analysis combined with a molecular equation of state to describe associability, it is demonstrated that diblock copolymers can exhibit dual critical points. We highlight the significance of multibody effects in correctly locating these critical points. Additionally, a region of first-order transition beyond the ϕ^{4} Landau framework is identified, which is further examined using a companion self-consistent field theory.

在理解二嵌段共聚物的熵驱动相分离时,需要有效的多体相互作用,这是由不同组分之间的自内聚力和关联的差异引起的。通过朗道分析结合分子状态方程来描述结合性,证明了二嵌段共聚物具有双临界点。我们强调了多体效应在正确定位这些临界点方面的重要性。此外,一阶跃迁的区域超越了φ ^{4}朗道框架被确定,这是进一步检查使用一个伴随自洽场理论。
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引用次数: 0
Current fluctuations in the symmetric zero-range process below and at critical density. 在对称零范围过程中的电流波动低于临界密度。
IF 2.4 3区 物理与天体物理 Q1 Mathematics Pub Date : 2024-11-01 DOI: 10.1103/PhysRevE.110.L052103
Tanmoy Chakraborty, Punyabrata Pradhan, Kavita Jain

Characterizing current fluctuations in a steady state is of fundamental interest and has attracted considerable attention in the recent past. However, the bulk of the studies are limited to systems that either do not exhibit a phase transition or are far from criticality. Here we consider a symmetric zero-range process on a ring that is known to show a phase transition in the steady state. We analytically calculate two density-dependent transport coefficients, namely, the bulk-diffusion coefficient and the particle mobility, that characterize the first two cumulants of the time-integrated current. We show that on the hydrodynamic scale, away from the critical point, the variance of the time-integrated current in the steady state grows with time t as sqrt[t] and t at short and long times, respectively. Moreover, we find an expression of the full scaling function for the variance of the time-integrated current and thereby the amplitude of the temporal growth of the current fluctuations. At the critical point, using a scaling theory, we find that, while the above-mentioned long-time scaling of the variance of the cumulative current continues to hold, the short-time behavior is anomalous in that the growth exponent is larger than one-half and varies continuously with the model parameters.

表征稳定状态下的电流波动具有重要意义,近年来已引起了广泛关注。然而,大部分研究都局限于不显示相变或远离临界的系统。在这里,我们考虑了一个已知在稳态下会出现相变的环上对称零程过程。我们分析计算了两个与密度相关的传输系数,即体扩散系数和粒子迁移率,它们是时间积分电流前两个累积量的特征。我们的研究表明,在流体力学尺度上,远离临界点时,稳态下时间积分电流的方差随时间 t 的增长分别为 sqrt[t] 和 t(短时间和长时间)。此外,我们还找到了时间积分电流方差的全比例函数表达式,从而找到了电流波动的时间增长幅度。在临界点,利用缩放理论,我们发现虽然上述累积电流方差的长时缩放继续成立,但短时行为却异常,即增长指数大于二分之一,并随模型参数连续变化。
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引用次数: 0
Intermediate scattering function of a gravitactic circle swimmer. 重力圆游泳者的中间散射函数。
IF 2.4 3区 物理与天体物理 Q1 Mathematics Pub Date : 2024-11-01 DOI: 10.1103/PhysRevE.110.054606
Regina Rusch, Oleksandr Chepizhko, Thomas Franosch

We analyze gravitaxis of a Brownian circle swimmer by deriving and analytically characterizing the experimentally measurable intermediate scattering function (ISF). To solve the associated Fokker-Planck equation, we use a spectral-theory approach, finding formal expressions in terms of eigenfunctions and eigenvalues of the overdamped-noisy-driven pendulum problem. We further perform a Taylor series of the ISF in the wavevector to extract the cumulants up to the fourth order. We focus on the skewness and kurtosis analyzed for four observation directions in the 2D plane. Validating our findings involves conducting Langevin-dynamics simulations and interpreting the results using a harmonic approximation. The skewness and kurtosis are amplified as the orienting torque approaches the intrinsic angular drift of the circle swimmer from above, highlighting deviations from Gaussian behavior. Transforming the ISF to the comoving frame, a measurable quantity, reveals gravitactic effects and diverse behaviors spanning from diffusive motion at low wavenumbers to circular motion at intermediate wavenumbers and directed motion at higher wavenumbers.

通过推导并解析表征实验可测量的中间散射函数(ISF),分析了布朗环游泳者的引力轴。为了求解相关的Fokker-Planck方程,我们使用谱理论方法,找到了过阻尼噪声驱动摆问题的特征函数和特征值的形式表达式。我们进一步在波矢量中对ISF进行泰勒级数,以提取高达四阶的累积量。重点分析了二维平面上四个观测方向的偏度和峰度。验证我们的发现包括进行朗格万动力学模拟和使用谐波近似解释结果。偏度和峰度被放大,当定向扭矩接近从上面的圆游泳者的固有角漂移,突出偏离高斯行为。将ISF转换为一个可测量的量,揭示了引力效应和各种行为,从低波数的扩散运动到中间波数的圆周运动和高波数的定向运动。
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引用次数: 0
Cell theories for the chiral crystal phase of hard equilateral triangles. 硬等边三角形手性晶体相的细胞理论。
IF 2.4 3区 物理与天体物理 Q1 Mathematics Pub Date : 2024-11-01 DOI: 10.1103/PhysRevE.110.054701
Yuri Martínez-Ratón, Enrique Velasco

We derive several versions of the cell theory for a crystal phase of hard equilateral triangles. To that purpose we analytically calculated the free area of a frozen oriented or freely rotating particle inside the cavity formed by its neighbors in a chiral configuration of their orientations. From the most successful versions of the theory we predict an equation of state which, despite being derived from a crystal configuration of particles, describes very reasonably the equation of state of the 6-atic liquid-crystal phase at packing fractions not very close from the isotropic-6-atic bifurcation. Also, the same equation of state performs well when compared to that from MC simulations for the stable crystal phase. The agreement can even be improved by selecting adequate values for the angle of chirality. Despite the success of two versions of the theory, we show that the free energy is an increasing function of the angle of chirality, implying that the most stable phase is the achiral phase. Furthermore, we show that possible clustering effects, such as the formation of perfect chiral hexagonal clusters, which in turn crystallize into an hexagonal lattice, cannot explain the presence of the chirality observed in simulations.

我们推导了硬等边三角形晶体相的几个版本的细胞理论。为此,我们分析计算了由其相邻粒子在其取向的手性构型中形成的空腔内冻结取向或自由旋转粒子的自由面积。从该理论最成功的版本中,我们预测了一个状态方程,尽管它是从粒子的晶体构型推导出来的,但它非常合理地描述了与各向同性6-atic分岔不太接近的堆积分数处的6-atic液晶相的状态方程。同样的状态方程,与MC模拟的稳定晶体相的状态方程相比,也表现得很好。甚至可以通过选择合适的手性角值来改善这种一致性。尽管两个版本的理论都取得了成功,但我们证明了自由能是手性角的递增函数,这意味着最稳定的相是非手性相。此外,我们表明可能的聚类效应,如形成完美的手性六边形团簇,进而结晶成六边形晶格,不能解释在模拟中观察到的手性的存在。
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引用次数: 0
Chimera states in pulse-coupled oscillator systems. 脉冲耦合振荡器系统中的奇美拉态。
IF 2.4 3区 物理与天体物理 Q1 Mathematics Pub Date : 2024-11-01 DOI: 10.1103/PhysRevE.110.054214
Arke Vogell, Udo Schilcher, Jorge F Schmidt, Christian Bettstetter

Coupled oscillator systems can lead to states in which synchrony and chaos coexist. These states are called "chimera states." The mechanism that explains the occurrence of chimera states is not well understood, especially in pulse-coupled oscillators. We study a variation of a pulse-coupled oscillator model that has been shown to produce chimera states, demonstrate that it reproduces several of the expected chimera properties, like the formation of multiple heads and the ability to control the natural drift that Kuramoto's chimera states experience in a ring, and explain how chimera states emerge. Our contribution is defining the model, analyzing the mechanism leading to chimera states, and comparing it with examples from the field of Kuramoto oscillators.

耦合振荡系统可以导致同步和混沌共存的状态。这些状态被称为“嵌合体状态”。解释嵌合体状态发生的机制尚不清楚,特别是在脉冲耦合振荡器中。我们研究了一种脉冲耦合振荡器模型的变体,该模型已被证明可以产生嵌合体状态,证明它再现了几种预期的嵌合体特性,如形成多个头部和控制Kuramoto嵌合体状态在环中经历的自然漂移的能力,并解释了嵌合体状态是如何出现的。我们的贡献是定义模型,分析导致嵌合体状态的机制,并将其与Kuramoto振子领域的例子进行比较。
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引用次数: 0
Rigorous hydrodynamics from linear Boltzmann equations and viscosity-capillarity balance. 从线性玻尔兹曼方程和粘度-气相平衡出发的严格流体力学。
IF 2.4 3区 物理与天体物理 Q1 Mathematics Pub Date : 2024-11-01 DOI: 10.1103/PhysRevE.110.055105
Florian Kogelbauer, Ilya Karlin

Exact closure for hydrodynamic variables is rigorously derived from the linear Boltzmann kinetic equation. Our approach, based on spectral theory, structural properties of eigenvectors, and the theory of slow manifolds, allows us to define a unique, optimal reduction in phase space close to equilibrium. The hydrodynamically constrained system induces a modification of entropy that ensures pure dissipation on the hydrodynamic manifold, which is interpreted as a nonlocal variant of Korteweg's theory of viscosity-capillarity balance. The rigorous hydrodynamic equations are exemplified on the Knudsen minimum paradox in a channel flow.

从线性玻尔兹曼动力学方程严格推导出流体动力变量的精确闭包。我们的方法,基于谱理论,特征向量的结构性质,以及慢流形理论,允许我们在接近平衡的相空间中定义一个独特的,最优的减少。水动力约束系统诱导熵的修正,以确保在水动力流形上的纯粹耗散,这被解释为Korteweg的黏性-毛细平衡理论的非局部变体。用Knudsen最小悖论举例说明了通道流的严格水动力方程。
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引用次数: 0
Noise-induced peak intensity fluctuations in class B laser systems. B类激光系统中噪声引起的峰值强度波动。
IF 2.4 3区 物理与天体物理 Q1 Mathematics Pub Date : 2024-11-01 DOI: 10.1103/PhysRevE.110.054120
Jason Hindes, Ira B Schwartz

Random perturbations and noise can excite instabilities in population systems that result in large fluctuations. Important examples involve class B lasers, where the dynamics are determined by the number of carriers and photons in a cavity with noise appearing in the electric-field dynamics. When such lasers are brought above threshold, the field intensity grows away from an unstable equilibrium, exhibiting transient relaxation oscillations with fluctuations due to noise. In this work, we focus on the first peak in the intensity during this transient phase in the presence of noise, and calculate its probability distribution using a Wentzel-Kramers-Brillouin approximation. In particular, we show how each value of the first peak is determined by a unique fluctuational momentum, calculate the peak intensity distribution in the limit where the ratio of photon-to-carrier lifetimes is small, and analyze the behavior of small fluctuations with respect to deterministic theory. Our approach is easily extended to the analysis of transient, noise-induced large fluctuations in general population systems exhibiting relaxation dynamics.

随机扰动和噪声可以激发种群系统的不稳定性,从而导致大的波动。重要的例子包括B类激光器,其动力学是由在电场动力学中出现噪声的腔中载流子和光子的数量决定的。当这样的激光器超过阈值时,场强度从不稳定的平衡状态增长,表现出由于噪声而产生的瞬态弛豫振荡。在这项工作中,我们专注于在存在噪声的瞬态阶段中强度的第一个峰值,并使用Wentzel-Kramers-Brillouin近似计算其概率分布。特别是,我们展示了第一个峰值的每个值是如何由一个独特的波动动量决定的,计算了在光子与载流子寿命之比很小的极限下的峰值强度分布,并分析了相对于确定性理论的小波动的行为。我们的方法很容易扩展到分析具有松弛动力学的一般种群系统中的瞬态、噪声引起的大波动。
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引用次数: 0
Signatures of self-organized dynamics in rapidly driven critical sandpiles. 快速驱动临界砂堆自组织动力学特征。
IF 2.4 3区 物理与天体物理 Q1 Mathematics Pub Date : 2024-11-01 DOI: 10.1103/PhysRevE.110.054203
Bosiljka Tadić, Alexander Shapoval, Mikhail Shnirman

We study two prototypical models of self-organized criticality, namely sandpile automata with deterministic (Bak-Tang-Wiesenfeld) and probabilistic (Manna model) dynamical rules, focusing on the nature of stress fluctuations induced by driving-adding grains during avalanche propagation, and dissipation through avalanches that hit the system boundary. Our analysis of stress evolution time series reveals robust cyclical trends modulated by collective fluctuations with dissipative avalanches. These modulated cycles attain higher harmonics, characterized by multifractal measures within a broad range of timescales. The features of the associated singularity spectra capture the differences in the dynamic rules behind the self-organized critical states at adiabatic driving and their pertinent response to the increased driving rate, which alters the process of stochasticity and causes a loss of avalanche scaling. In sequences of outflow current carried by dissipative avalanches, the first return distributions follow the q-Gaussian law in the adiabatic limit. They appear to follow different laws at an intermediate scale with an increased driving rate, describing different pathways to the gradual loss of cooperative behavior in these two models. The robust appearance of cyclical trends and their multifractal modulation thus represents another remarkable feature of self-organized dynamics beyond the scaling of avalanches. It can also help identify the prominence of self-organizational phenomenology in an empirical time series when underlying interactions and driving modes remain hidden.

我们研究了自组织临界性的两个原型模型,即具有确定性(Bak-Tang-Wiesenfeld)和概率性(Manna 模型)动力学规则的砂堆自动机,重点是雪崩传播过程中由驱动添加晶粒引起的应力波动的性质,以及通过撞击系统边界的雪崩进行的耗散。我们对应力演变时间序列的分析揭示了由集体波动与耗散雪崩调制的强周期趋势。这些被调制的周期达到了高次谐波,在广泛的时间尺度范围内具有多分形测量的特征。相关奇异谱的特征捕捉到了绝热驱动下自组织临界状态背后的动态规则差异,以及它们对驱动速率增加的相关响应,驱动速率的增加改变了随机性过程并导致雪崩缩放的损失。在耗散雪崩所携带的外流电流序列中,首次回流分布在绝热极限下遵循 q-Gaussian 规律。在驱动速率增加的中间尺度,它们似乎遵循不同的规律,描述了这两种模型中逐渐丧失合作行为的不同途径。因此,周期趋势的强劲出现及其多分形调制代表了自组织动力学在雪崩规模之外的另一个显著特点。当潜在的相互作用和驱动模式仍被隐藏时,它还有助于识别经验时间序列中突出的自组织现象。
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引用次数: 0
Computational microscopy beyond perfect lenses. 超越完美透镜的计算显微镜。
IF 2.4 3区 物理与天体物理 Q1 Mathematics Pub Date : 2024-11-01 DOI: 10.1103/PhysRevE.110.054407
Xingyuan Lu, Minh Pham, Elisa Negrini, Damek Davis, Stanley J Osher, Jianwei Miao

We demonstrate that in situ coherent diffractive imaging (CDI), which leverages the coherent interference between strong and weak beams to illuminate static and dynamic structures, can serve as a highly dose-efficient imaging method. At low doses, in situ CDI can achieve higher resolution than perfect lenses with the point spread function as a delta function. Both our numerical simulations and experimental results demonstrate that combining in situ CDI with ptychography can reduce the required dose by up to two orders of magnitude compared with ptychography alone. We anticipate that computational microscopy based on in situ CDI can be applied across various imaging modalities using photons and electrons for low-dose imaging of radiation-sensitive materials and biological samples.

我们证明,利用强光束和弱光束之间的相干干涉来照亮静态和动态结构的原位相干衍射成像(CDI)可作为一种高剂量效率的成像方法。在低剂量情况下,原位 CDI 可以达到比点扩散函数为三角函数的完美透镜更高的分辨率。我们的数值模拟和实验结果表明,与单独的点阵图相比,将原位 CDI 与点阵图相结合可将所需剂量降低两个数量级。我们预计,基于原位 CDI 的计算显微技术可应用于各种成像模式,使用光子和电子对辐射敏感材料和生物样本进行低剂量成像。
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引用次数: 0
Heat production in a stochastic system with nonlinear time-delayed feedback. 具有非线性延时反馈的随机系统中的热量产生。
IF 2.4 3区 物理与天体物理 Q1 Mathematics Pub Date : 2024-11-01 DOI: 10.1103/PhysRevE.110.054126
Robin A Kopp, Sabine H L Klapp

Using the framework of stochastic thermodynamics we study heat production related to the stochastic motion of a particle driven by repulsive, nonlinear, time-delayed feedback. Recently it has been shown that this type of feedback can lead to persistent motion above a threshold in parameter space [R. A. Kopp et al., Phys. Rev. E 107, 024611 (2023)2470-004510.1103/PhysRevE.107.024611]. Here we investigate, numerically and by analytical methods, the rate of heat production in the different regimes around the threshold to persistent motion. We find a nonzero average heat production rate, 〈q[over ̇]〉, already below the threshold, indicating the nonequilibrium character of the system even at small feedback. In this regime, we compare to analytical results for a corresponding linearized delayed system and a small-delay approximation which provides a reasonable description of 〈q[over ̇]〉 at small repulsion (or delay time). Beyond the threshold, the rate of heat production is much larger and shows a maximum as a function of the delay time. In this regime, 〈q[over ̇]〉 can be approximated by that of a system subject to a constant force stemming from the long-time velocity in the deterministic limit. The distribution of dissipated heat, however, is non-Gaussian, contrary to the constant-force case.

利用随机热力学框架,我们研究了与受排斥性、非线性、延时反馈驱动的粒子随机运动有关的热量产生。最近的研究表明,这种类型的反馈可以导致超过参数空间阈值的持续运动 [R. A. Kopp et al.A. Kopp 等人,Phys. Rev. E 107, 024611 (2023)2470-004510.1103/PhysRevE.107.024611]。在这里,我们通过数值和分析方法研究了持续运动阈值附近不同状态下的产热率。我们发现平均产热率〈q[over 〉〉在阈值以下就已经不为零了,这表明即使在小反馈时系统也是非平衡的。在这一系统中,我们比较了相应线性化延迟系统的分析结果和小延迟近似值,后者合理地描述了小排斥力(或延迟时间)下的〈q[over ■ng]〉。超过阈值后,产热速率会更大,并显示出延迟时间函数的最大值。在这种情况下,〈q[over ■ng]〉可以近似为一个系统在确定性极限中受到源于长时速度的恒定力的作用。然而,与恒力情况相反,散热分布是非高斯分布。
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引用次数: 0
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Physical review. E
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