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Deformation of drops at low Reynolds number impact 低雷诺数冲击下的液滴变形
IF 2.7 3区 物理与天体物理 Q2 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-08-01 DOI: 10.1103/physrevfluids.9.083601
L. Jørgensen
Drop impact experiments are performed with very viscous fluids to propose a description of the drop deformation at low Reynolds number. We focus on a specific case where dimensionless parameters other than the Reynolds number play no role, which means that only kinetic energy and viscous dissipation determine the final deformation. The same situation in the case of a Reynolds number larger than ten has been clarified years ago. The maximum diameter of the spread drop is well described by a 1/5 power law of the Reynolds number only. Here the deformation of the drop, defined as the contact diameter rescaled by the drop size, is also a power law of the Reynolds number. From experimental data and scaling arguments, the exponent of the power law is shown to be 1/3.
通过对粘性很强的流体进行液滴冲击实验,提出了低雷诺数时液滴变形的描述方法。我们关注的是一种特殊情况,即除雷诺数外的无量纲参数不起作用,这意味着只有动能和粘性耗散决定最终变形。雷诺数大于 10 时的相同情况早在几年前就已阐明。扩散液滴的最大直径可以很好地用雷诺数的 1/5 幂定律来描述。在这里,液滴的变形(定义为接触直径乘以液滴大小)也是雷诺数的幂律。根据实验数据和比例论证,幂律的指数为 1/3。
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引用次数: 0
Equatorial blowup and polar caps in drop electrohydrodynamics 水滴电动流体力学中的赤道吹胀和极冠
IF 2.7 3区 物理与天体物理 Q2 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-08-01 DOI: 10.1103/physrevfluids.9.083701
Gunnar G. Peng, Rodolfo Brandão, Ehud Yariv, Ory Schnitzer
We illuminate effects of surface-charge convection intrinsic to leaky-dielectric electrohydrodynamics by analyzing the symmetric steady state of a circular drop in an external field at arbitrary electric Reynolds number <math xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>Re</mi><mi>E</mi></msub></math>. In formulating the problem, we identify an exact factorization that reduces the number of dimensionless parameters from four—<math xmlns="http://www.w3.org/1998/Math/MathML"><msub><mi>Re</mi><mi>E</mi></msub></math> and the conductivity, permittivity and viscosity ratios—to two: a modified electric Reynolds number <math xmlns="http://www.w3.org/1998/Math/MathML"><mover accent="true"><mi>Re</mi><mo>̃</mo></mover></math> and a charging parameter <math xmlns="http://www.w3.org/1998/Math/MathML"><mi>ϖ</mi></math>. In the case <math xmlns="http://www.w3.org/1998/Math/MathML"><mrow><mi>ϖ</mi><mo><</mo><mn>0</mn></mrow></math>, where charge relaxation in the drop phase is slower than in the suspending phase, and, as a consequence, the interface polarizes antiparallel to the external field, we find that above a critical <math xmlns="http://www.w3.org/1998/Math/MathML"><mover accent="true"><mi>Re</mi><mo>̃</mo></mover></math> value the solution exhibits a blowup singularity such that the surface-charge density diverges antisymmetrically with the <math xmlns="http://www.w3.org/1998/Math/MathML"><mrow><mo>−</mo><mn>1</mn><mo>/</mo><mn>3</mn></mrow></math> power of distance from the equator. We use local analysis to uncover the structure of that blowup singularity, wherein surface charges are convected by a locally induced flow towards the equator where they annihilate. To study the blowup regime, we devise a numerical scheme encoding that local structure where the blowup prefactor is determined by a global charging-annihilation balance. We also employ asymptotic analysis to construct a universal problem governing the blowup solutions in the regime <math xmlns="http://www.w3.org/1998/Math/MathML"><mrow><mover accent="true"><mi>Re</mi><mo>̃</mo></mover><mo>≫</mo><mn>1</mn></mrow></math>, far beyond the blowup threshold. In the case <math xmlns="http://www.w3.org/1998/Math/MathML"><mrow><mi>ϖ</mi><mo>></mo><mn>0</mn></mrow></math>, where charge relaxation is faster in the drop phase and the interface polarizes parallel to the external field, we numerically observe and asymptotically characterize the formation at large <math xmlns="http://www.w3.org/1998/Math/MathML"><mover accent="true"><mi>Re</mi><mo>̃</mo></mover></math> of stagnant, perfectly conducting surface-charge caps about the drop poles. The cap size grows and the cap voltage decreases monotonically with increasing conductivity or decreasing permittivity of the drop phase relative to the suspending phase. The flow in this scenario is nonlinearly driven by electrical shear stresses at the complement of the caps. In both polarization scenarios, the flow at large <math xmlns="http://www.w3.o
我们通过分析任意电雷诺数 ReE 条件下圆形液滴在外场中的对称稳态,阐明了漏介质电动流体力学固有的表面电荷对流效应。在ϖ<0的情况下,液滴相中的电荷弛豫比悬浮相中的慢,因此界面极化与外场反平行,我们发现在临界 Rẽ值以上,溶液表现出炸裂奇异性,表面电荷密度随距赤道距离的-1/3次方反对称发散。我们利用局部分析揭示了炸裂奇点的结构,即表面电荷被局部诱导流对流向赤道,并在那里湮灭。为了研究炸毁机制,我们设计了一种数值方案,对局部结构进行编码,其中炸毁前因子由全局电荷-湮灭平衡决定。我们还采用渐近分析法,构建了一个普遍问题,用以控制远超过炸毁阈值的 Rẽ≫1 制度中的炸毁解。在ϖ>0的情况下,电荷弛豫在液滴阶段更快,界面极化平行于外部磁场,我们数值观察到在大Rẽ时,液滴两极周围会形成停滞的、完全导电的表面电荷帽,并对其进行了渐近表征。随着液滴相相对于悬浮相的电导率增大或介电常数减小,电帽尺寸增大,电帽电压单调降低。这种情况下的流动是由电帽互补处的电剪应力非线性驱动的。在这两种极化情况下,大 Rẽ 时的流动与外部磁场的大小成线性比例,这与我们熟悉的弱磁场下的二次方比例形成鲜明对比。
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引用次数: 0
Static Bell test in pilot-wave hydrodynamics 先导波流体力学静态贝尔试验
IF 2.7 3区 物理与天体物理 Q2 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-08-01 DOI: 10.1103/physrevfluids.9.084001
Konstantinos Papatryfonos, Louis Vervoort, André Nachbin, Matthieu Labousse, John W. M. Bush
Since its discovery in 2005, the hydrodynamic pilot-wave system has provided a concrete macroscopic realization of wave-particle duality and concomitant classical analogs of a growing number of quantum effects. The question naturally arises as to how closely particle-particle correlations achieved with this classical system can mimic those arising on the quantum scale. We here introduce a new platform for addressing this question, a numerical model of cooperative tunneling in a bipartite pilot-wave hydrodynamic system. We execute a static Bell test, in which the system geometry is fixed and the two subsystems are coupled through the intervening wave field. This wave-mediated coupling is not congruent with the assumptions made in deriving Bell's inequality, and so allows one to rationalize the reported violations. Nevertheless, these violations are elusive, and arise only in a limited corner of parameter space.
自 2005 年发现以来,流体动力先导波系统为波粒二象性提供了一个具体的宏观实现方式,同时也为越来越多的量子效应提供了经典模拟。自然而然就会产生这样一个问题:在这一经典系统中实现的粒子-粒子相关性能在多大程度上模拟量子尺度上产生的相关性。我们在此引入了一个解决这一问题的新平台,即一个双方先导波流体动力系统中的合作隧道数值模型。我们进行了静态贝尔测试,其中系统的几何形状是固定的,两个子系统通过中间的波场耦合。这种以波为媒介的耦合与推导贝尔不等式时所作的假设并不一致,因此可以合理解释所报告的违规现象。然而,这些违规现象难以捉摸,而且只出现在参数空间的有限角落。
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引用次数: 0
Thermocapillary instability of a surfactant-laden shear-imposed film flow 含有表面活性剂的剪切膜流的热毛细管不稳定性
IF 2.7 3区 物理与天体物理 Q2 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-08-01 DOI: 10.1103/physrevfluids.9.084002
Arnab Choudhury, Arghya Samanta
We examine the linear thermocapillary instability of a two-dimensional gravity-driven shear-imposed incompressible viscous film flowing over a uniformly heated inclined wall when the film surface is covered by an insoluble surfactant. The aim is to expand the prior research [Wei, Phys. Fluids 17, 012103 (2005)] to the case of a nonisothermal viscous film. As a result, the energy equation is incorporated into the governing equations along with the mass conservation and momentum equations. In the present study, we have found two additional thermocapillary S- and P-modes in the low to moderate Reynolds number regime, along with the known H-mode (surface mode) and surfactant mode. The long-wave analysis predicts that the surfactant Marangoni number, which measures the surface tension gradient due to a change in insoluble surfactant concentration, has a stabilizing impact on the H-mode, but the thermal Marangoni number, which measures the surface tension gradient due to a change in temperature, has a destabilizing impact. These opposing effects produce an analytical relationship between them for which the critical Reynolds number for the H-mode instability of the nonisothermal film flow coincides with that of the isothermal film flow. On the other hand, the numerical result exhibits that the surfactant Marangoni number has a stabilizing influence on the thermocapillary S-mode and P-mode. More specifically, these thermocapillary instabilities diminish with an increase in the value of the surfactant Marangoni number. However, these thermocapillary instabilities can be made stronger by increasing the value of the thermal Marangoni number. Furthermore, the thermal Marangoni number destabilizes the surfactant mode instability, but the onset of instability is not affected in the presence of the thermal Marangoni number, which is in contrast to the influence of the surfactant Marangoni number on the onset of surfactant mode instability. Interestingly, the Biot number, which measures the ratio of heat convection and heat conduction, shows a dual role in the surfactant mode instability, even though the threshold of instability remains the same. In the high Reynolds number regime, the shear mode appears and is stabilized by the surfactant Marangoni number but destabilized by the thermal Marangoni number. Moreover, the comparison of results with inertia and without inertia exhibits a stabilizing role of inertia in the surfactant mode.
我们研究了当薄膜表面被不溶表面活性剂覆盖时,二维重力驱动剪切不可压缩粘性薄膜流过均匀加热斜壁时的线性热毛细管不稳定性。目的是将先前的研究[Wei,Phys. Fluids 17, 012103 (2005)]扩展到非等温粘性薄膜的情况。因此,能量方程与质量守恒和动量方程一起被纳入了控制方程。在本研究中,除了已知的 H 模式(表面模式)和表面活性剂模式之外,我们还发现了在低到中等雷诺数条件下的两种额外的热毛细管 S 模式和 P 模式。长波分析预测,表面活性剂马兰戈尼数(用于测量因不溶性表面活性剂浓度变化而产生的表面张力梯度)对 H 模式有稳定作用,而热马兰戈尼数(用于测量因温度变化而产生的表面张力梯度)则有破坏作用。这些相反的影响在它们之间产生了一种分析关系,即非等温膜流 H 模式不稳定的临界雷诺数与等温膜流的临界雷诺数相吻合。另一方面,数值结果表明,表面活性剂马兰戈尼数对热毛细管 S 模式和 P 模式具有稳定影响。更具体地说,这些热毛细管不稳定性随着表面活性剂马兰戈尼数的增加而减弱。然而,这些热毛细管不稳定性会随着热马兰戈尼数的增加而增强。此外,热马兰戈尼数会破坏表面活性剂模式不稳定性,但在存在热马兰戈尼数的情况下,不稳定性的发生并不受影响,这与表面活性剂马兰戈尼数对表面活性剂模式不稳定性发生的影响形成了鲜明对比。有趣的是,衡量热对流和热传导比率的比奥特数在表面活化剂模式不稳定性中显示出双重作用,尽管不稳定性阈值保持不变。在高雷诺数条件下,剪切模式出现,并通过表面活性剂马兰戈尼数而稳定,但通过热马兰戈尼数而失稳。此外,有惯性和无惯性结果的比较表明,惯性对表面活性剂模式起稳定作用。
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引用次数: 0
Correlations between thermodynamic fluctuations in shock wave/turbulent boundary layer interaction 冲击波/湍流边界层相互作用中热力学波动之间的相关性
IF 2.7 3区 物理与天体物理 Q2 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-07-31 DOI: 10.1103/physrevfluids.9.073401
Ximeng Hou, Dehao Xu, Jianchun Wang, Shiyi Chen
The second moment correlations between thermodynamic fluctuations in incident shock wave/turbulent boundary layer interaction flows at Mach 2.25 are systematically investigated by direct numerical simulation. The concerned fluctuations are those of pressure, entropy, temperature, and density {p,s,T,ρ}. Effects of wall temperature and Reynolds number are studied. Kovásznay decomposition is introduced to decompose the fluctuations into acoustic and entropic modes. It is shown that all the six concerned correlations are determined by merely two parameters, which are interpreted as intermodal competition and intermodal correlation, respectively. Accordingly, the flow field is divided into several zones, each with distinct physical properties, to analyze the contributing factors to the correlations. In addition, a model is proposed where the correlations are deemed as functions of the root-mean-square values of thermodynamic fluctuations, as in Gerolymos and Vallet [J. Fluid Mech. 851, 447 (2018)] but simpler. The formula for each correlation has the same form. The accuracy of the model is validated in boundary layers where the intermodal correlation is weak.
通过直接数值模拟,系统地研究了马赫数为 2.25 的入射冲击波/湍流边界层相互作用流中热力学波动的第二矩相关性。相关波动包括压力、熵、温度和密度 {p′,s′,T′,ρ′}。研究了壁温和雷诺数的影响。引入 Kovásznay 分解法将波动分解为声学模式和熵模式。结果表明,所有相关的六种相关性仅由两个参数决定,这两个参数分别被解释为模式间竞争和模式间相关性。因此,将流场划分为几个区域,每个区域都具有不同的物理特性,以分析相关性的促成因素。此外,还提出了一个模型,将相关性视为热力学波动均方根值的函数,如 Gerolymos 和 Vallet [J. Fluid Mech. 851, 447 (2018)],但更为简单。每种相关性的公式形式相同。模型的准确性在模式间相关性较弱的边界层中得到了验证。
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引用次数: 0
Newtonian fluid dynamics in a misaligned parallel-plate rheometer 错位平行板流变仪中的牛顿流体动力学
IF 2.7 3区 物理与天体物理 Q2 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-07-31 DOI: 10.1103/physrevfluids.9.074103
Jian Teng, Sungwon La, Jesse T. Ault
A parallel-plate rotational rheometer measures the viscosity of a fluid by rotating the top plate relative to the bottom plate in order to induce a shear on the fluid and measuring the torques and forces that result as a function of the induced rotation rate. Manufacturing imperfections can often lead to unintentional misalignment of the plates of the rheometer, where the top and bottom plates are not perfectly parallel, and this misalignment can affect the fluid dynamics inside the rheometer. This study examines the effect that misalignment has on the viscosity measurements of Newtonian fluids in the limit of small rheometer gap heights. A theoretical model for the behavior of a general Newtonian fluid in a misaligned rheometer with a small gap height is derived using perturbation expansions. The theoretical results show that at small gap heights, misalignment can produce additional secondary velocity components and pressures in the fluid, which affect the forces and moments in the rheometer. In such cases at small Reynolds numbers, the dominant forces and moments acting on the top plate of the rheometer are the viscous force in the direction parallel to the tilt axis, the pressure moment in the direction perpendicular to the tilt axis and in the cross-sectional plane, and the viscous moment in the direction along the height of the rheometer. These forces and moments on the top plate were found to increase as the misalignment tilt angle increased, leading to an increase in the error of viscosity measurement by the rheometer. Three-dimensional numerical simulations validate the theoretical predictions.
平行板旋转流变仪通过旋转顶板和底板来测量流体的粘度,从而对流体产生剪切力,并测量作为诱导旋转速率函数的扭矩和力。制造缺陷往往会导致流变仪的顶板和底板无意中错位,即顶板和底板并非完全平行,这种错位会影响流变仪内部的流体动力学。本研究探讨了在流变仪间隙高度较小的情况下,错位对牛顿流体粘度测量的影响。利用扰动展开法推导出了一般牛顿流体在间隙高度较小的错位流变仪中的行为理论模型。理论结果表明,在间隙高度较小时,错位会在流体中产生额外的次级速度分量和压力,从而影响流变仪中的力和力矩。在这种情况下,当雷诺数较小时,作用在流变仪顶板上的主要力和力矩是平行于倾斜轴方向的粘性力、垂直于倾斜轴方向和横截面上的压力力矩以及沿流变仪高度方向的粘性力矩。这些作用在顶板上的力和力矩会随着错位倾斜角的增大而增大,从而导致流变仪测量粘度的误差增大。三维数值模拟验证了理论预测。
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引用次数: 0
How small droplets form in turbulent multiphase flows 小液滴如何在湍流多相流中形成
IF 2.7 3区 物理与天体物理 Q2 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-07-29 DOI: 10.1103/physrevfluids.9.l072301
M. Crialesi-Esposito, G. Boffetta, L. Brandt, S. Chibbaro, S. Musacchio
The formation of small droplets and bubbles in turbulent flows is a crucial process in geophysics and engineering, whose underlying physical mechanism remains a puzzle. In this Letter, we address this problem by means of high-resolution numerical simulations, comparing a realistic multiphase configuration with a numerical experiment in which we attenuate the presence of strong velocity gradients either across the whole mixture or in the disperse phase only. Our results show unambiguously that the formation of small droplets is governed by the internal dynamics which occurs during the breakup of large drops and that the high vorticity and the extreme dissipation associated to these events are the consequence and not the cause of the breakup.
在湍流中形成小液滴和气泡是地球物理学和工程学中的一个关键过程,其基本物理机制仍然是一个谜。在这封信中,我们通过高分辨率数值模拟解决了这一问题,将现实的多相配置与数值实验进行了比较,在实验中,我们削弱了整个混合物或仅在分散相中存在的强速度梯度。我们的结果明确显示,小液滴的形成受大液滴破裂时发生的内部动力学的支配,与这些事件相关的高涡度和极度耗散是破裂的结果而不是原因。
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引用次数: 0
Modal and nonmodal stability of the laminar flow in a channel with longitudinal riblets 带有纵向波纹的水道中层流的模态和非模态稳定性
IF 2.7 3区 物理与天体物理 Q2 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-07-29 DOI: 10.1103/physrevfluids.9.073903
Antoine Jouin, Jean-Christophe Robinet, Stefania Cherubini
Modal and nonmodal stability analysis of a channel flow with longitudinal riblets are investigated. To this extent, a method based on the coupling between a two-dimensional stability problem and a computational framework for n-periodic systems based on Bloch waves is proposed. Unstable modes from linear stability can be retrieved. The influence of the riblets on the most amplified flow structures is investigated through a transient growth analysis: a resonance is found when the riblet wavenumber is equal to the wavenumber of the optimal streaks in a smooth channel flow. For large riblet spacing, a wavenumber lock-in regime, in which the streaks dynamics and wavelength are totally controlled by the riblet spacing, is observed. Physically, a modulation of the streaks amplitude in the spanwise direction via a beating mechanism is seen. These phenomena are characteristic of dynamic systems spatially forced and may exhibit geometric frustration. Similar results were found in the study of secondary flows in Rayleigh-Bénard convection with wavy walls. A resolvent analysis is also performed: it is found that riblets lead to the development of oblique waves that may trigger an early transition.
研究了具有纵向波纹的渠道流的模态和非模态稳定性分析。为此,提出了一种基于二维稳定性问题与基于布洛赫波的 n 周期系统计算框架之间耦合的方法。可以从线性稳定性中检索出不稳定模式。通过瞬态增长分析研究了波纹对最放大流动结构的影响:当波纹的波数等于平滑通道流中最佳条纹的波数时,就会产生共振。在波纹间距较大的情况下,会观察到一个波长锁定机制,其中条纹的动态和波长完全由波纹间距控制。从物理角度看,条纹振幅在跨度方向上通过跳动机制进行调制。这些现象是空间受迫动态系统的特征,可能表现出几何挫折。在研究具有波浪壁的雷利-贝纳德对流中的二次流时也发现了类似的结果。还进行了解析分析:发现波纹导致斜波的发展,可能引发早期过渡。
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引用次数: 0
Dissociation of red blood cell aggregates in extensional flow 延伸流中红细胞聚集体的解离
IF 2.7 3区 物理与天体物理 Q2 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-07-29 DOI: 10.1103/physrevfluids.9.l071101
Midhun Puthumana Melepattu, Guillaume Maîtrejean, Thomas Podgorski
Blood rheology and microcirculation are strongly influenced by red blood cell aggregation. We investigate the dissociation rates of red cell aggregates in extensional flow using hyperbolic microfluidic constrictions and image analysis by a convolutional neural network (CNN). Our findings reveal that aggregate dissociation increases sharply when a critical extension rate is reached which falls within the range of microcirculatory conditions, suggesting that large variations of aggregate sizes should be expected in vivo. This work contributes to a deeper understanding of the behavior of red blood cell aggregates in response to extensional stress in microcirculatory networks, provides crucial experimental data to validate theoretical and numerical models, and constitutes the basis for improved evaluation of blood aggregability in clinical contexts.
血液流变学和微循环受红细胞聚集的影响很大。我们利用双曲微流体收缩和卷积神经网络(CNN)的图像分析,研究了红细胞聚集体在伸展流中的解离率。我们的研究结果表明,当达到微循环条件范围内的临界延伸率时,聚集体解离率会急剧增加,这表明聚集体大小在体内会有很大的变化。这项研究有助于深入了解红细胞聚集体在微循环网络中响应延伸压力的行为,为验证理论和数值模型提供了重要的实验数据,并为改进临床血液聚集性评估奠定了基础。
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引用次数: 0
Ion steric interactions and electrostatic correlations on electro-osmotic flow in charged nanopores with multivalent electrolytes 离子立体相互作用和静电相关性对多价电解质带电纳米孔内电渗流的影响
IF 2.7 3区 物理与天体物理 Q2 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-07-26 DOI: 10.1103/physrevfluids.9.074201
Shubhra Sahu, Bapan Mondal, Somnath Bhattacharyya
Atomistic and coarse-grained simulations show the formation of a condensed layer of counterions near a charged surface in contact with multivalent or monovalent electrolytes of high concentration. This condensed layer may overscreen the surface charge, and eventually a coion-dominated region may arise within the electric double layer, which again draws a layer of counterions and so on till the charge density approaches zero. Such a type of overscreening and charge density oscillation cannot be predicted through the mean-field based models as it does not account for the correlations between discrete charges. In the present study the mean-field-based model has been extended to consider the many-body interactions to analyze the electro-osmosis and ion transport of multivalent electrolytes in a highly charged nanopore. The ions are considered to be finite-sized, which is accounted for by considering the hydrodynamic steric interactions and modification of the suspension medium viscosity. Consideration of the electrostatic correlation leads to a fourth-order Poisson-Fermi equation for an electric field. Such a type of continuum model is easy to handle and to use to predict the layered structure of the EDL. Our model captures the existing experimental and molecular dynamics simulation correctly. Based on the modified model, we have analyzed the volume flow rate, current density, and ion selectivity of the pore in multivalent electrolytes for different electrostatic conditions. The present model shows that the counterion size has an impact on the condensed layer and hence overscreening. We demonstrate that the EOF reversal of multivalent electrolytes can be suppressed by mixing with monovalent slats.
原子模拟和粗粒模拟显示,在与高浓度多价或单价电解质接触的带电表面附近,会形成一层凝聚的反离子层。这种凝聚层可能会遮蔽表面电荷,最终在电双层内形成一个以共价离子为主的区域,该区域又会吸引一层反离子,如此反复,直到电荷密度趋近于零。这种过屏蔽和电荷密度振荡无法通过基于平均场的模型来预测,因为它没有考虑离散电荷之间的相关性。在本研究中,基于均方场的模型被扩展到考虑多体相互作用,以分析多价电解质在高电荷纳米孔中的电渗和离子传输。考虑到流体力学立体相互作用和悬浮介质粘度的改变,离子被认为是有限大小的。考虑到静电相关性,可得出电场的四阶泊松-费米方程。这种连续模型易于处理,可用于预测 EDL 的分层结构。我们的模型正确捕捉了现有的实验和分子动力学模拟结果。根据修改后的模型,我们分析了多价电解质中不同静电条件下孔隙的体积流量、电流密度和离子选择性。本模型表明,反离子的大小对凝聚层有影响,因此会产生过屏蔽。我们证明,多价电解质的 EOF 反转可以通过与单价板条混合来抑制。
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引用次数: 0
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Physical Review Fluids
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