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Thermal hysteresis in wettability and the Leidenfrost phenomenon 润湿性的热滞后和莱顿弗罗斯特现象
Pub Date : 2024-09-12 DOI: 10.1103/physrevresearch.6.033287
Yutaku Kita, Kensuke Kida, Takaaki Ariyoshi, Sumitomo Hidaka, Masamichi Kohno, Yasuyuki Takata
The Leidenfrost temperature (TL), at which the liquid drop lifetime peaks on a superheated surface, is believed to be wettability dependent. Here, we show that the wettability effect on TL is subject to the history of the surface temperature. Observing a water drop evaporating on a polished stainless-steel surface heated from 100 to 400C in argon gas, we find TL265C. We then repeat the experiment along decreasing temperature and find a TL increase by 10 K, i.e., TL275C. This thermal hysteresis is due to a reduced contact angle during heating. Once hydrophilized, the hysteresis disappears until the contact angle recovers. Similar observations are made in the air where oxidation is possible.
莱顿弗罗斯特温度(TL)是过热表面上液滴寿命达到峰值的温度,它被认为与润湿性有关。在这里,我们证明了润湿性对 TL 的影响受表面温度历史的影响。通过观察在氩气中加热 100 至 400∘C 的抛光不锈钢表面上蒸发的水滴,我们发现 TL≈265∘C 。然后,我们沿温度递减方向重复实验,发现 TL 增加了 10 K,即 TL≈275∘C 。这种热滞后现象是由于加热过程中接触角减小所致。一旦亲水,滞后现象就会消失,直到接触角恢复。在可能发生氧化的空气中也能观察到类似现象。
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引用次数: 0
Universality classes in out-of-equilibrium systems: An encompassing theorem for a one-dimensional fusing particles model 非平衡系统中的普遍性类别:一维融合粒子模型的包含定理
Pub Date : 2024-09-12 DOI: 10.1103/physrevresearch.6.033288
Daniel Fraiman
This paper supports the idea that some out-of-equilibrium systems can be described by universality classes. A specific out-of-equilibrium fusing particles model is studied in detail, resulting in a method for determining the number and mass of the final particles based solely on the initial conditions, eliminating the need to evolve the particle system. This method reveals the basis for a universality class encompassing theorem, which is developed to define other models within the same universality class. This result establishes an infinite number of models with the same behavior and scaling, two of which are described in detail.
本文支持这样一种观点,即某些失衡系统可以用普遍性类别来描述。本文详细研究了一个特定的失衡融合粒子模型,并由此提出了一种方法,可完全根据初始条件确定最终粒子的数量和质量,而无需演化粒子系统。这种方法揭示了一个普遍性类别包含定理的基础,该定理可用于定义同一普遍性类别中的其他模型。这一结果确定了具有相同行为和缩放的无数模型,本文将详细介绍其中的两个模型。
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引用次数: 0
Protocols for trainable and differentiable quantum generative modeling 可训练和可微分量子生成建模协议
Pub Date : 2024-09-12 DOI: 10.1103/physrevresearch.6.033291
Oleksandr Kyriienko, Annie E. Paine, Vincent E. Elfving
We propose an approach for learning probability distributions as differentiable quantum circuits (DQC) that enable efficient quantum generative modeling (QGM) and synthetic data generation. Contrary to existing QGM approaches, we perform training of a DQC-based model, where data is encoded in a latent space with the proposed phase feature map of exponential capacity. This is followed by a trainable quantum circuit, forming the model. We then map the trained model to the bit basis using a fixed unitary transformation, in this case corresponding to a quantum Fourier transform circuit. It allows fast sampling from parametrized distributions using a single-shot readout. Importantly, latent space training provides models that are automatically differentiable, and we show how samples from solutions of stochastic differential equations (SDEs) can be accessed by solving stationary and time-dependent Fokker-Planck equations with a quantum protocol. Our approach opens a route to multidimensional generative modeling with qubit registers explicitly correlated via a (fixed) entangling layer. In this case quantum computers can offer advantage as efficient samplers, which perform complex inverse transform sampling enabled by the fundamental laws of quantum mechanics. On a technical side the advances are multiple, as we introduce the phase feature map, analyze its properties, and develop frequency-taming techniques that include qubitwise training and feature map sparsification.
我们提出了一种将概率分布作为可微分量子电路(DQC)来学习的方法,从而实现高效的量子生成模型(QGM)和合成数据生成。与现有的 QGM 方法不同,我们对基于 DQC 的模型进行了训练,在训练过程中,数据被编码到具有指数容量的相位特征图的潜在空间中。随后,可训练量子电路形成模型。然后,我们使用固定的单元变换将训练好的模型映射到比特基础上,在这种情况下,单元变换与量子傅里叶变换电路相对应。它允许使用单次读出从参数化分布中快速采样。重要的是,潜空间训练提供了可自动微分的模型,我们展示了如何通过量子协议求解静态和时变福克-普朗克方程,从随机微分方程(SDE)的解中获取样本。我们的方法为多维生成建模开辟了一条途径,其量子位寄存器通过(固定的)纠缠层明确相关。在这种情况下,量子计算机可以提供高效采样器的优势,在量子力学基本定律的支持下执行复杂的反变换采样。技术方面的进步是多方面的,我们引入了相位特征图,分析了它的特性,并开发了包括量子比特训练和特征图稀疏化在内的频率驯服技术。
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引用次数: 0
In-depth analysis of music structure as a text network 深入分析作为文本网络的音乐结构
Pub Date : 2024-09-11 DOI: 10.1103/physrevresearch.6.033279
Ping-Rui Tsai, Yen-Ting Chou, Nathan-Christopher Wang, Hui-Ling Chen, Hong-Yue Huang, Zih-Jia Luo, Tzay-Ming Hong
Music, enchanting and poetic, permeates every corner of human civilization. Although music is not unfamiliar to people, our understanding of its essence remains limited, and there is still no universally accepted scientific description. This is primarily due to music being regarded as a product of reason and emotion, making it difficult to define. This article treats musical texts as a complex system. This view echoes linguist John Rupert Firth's insight that understanding a word involves defining it through its surrounding relationships. To construct the network we first build a linear regression model with threshold values to assign conditions to the links among note, time, and volume. Then a clustering coefficient representing regional characteristics is utilized to define the word. Finally, the statistical distribution of the text is strictly required to adhere to the grammatical properties of statistical linguistics, such as Zipf's law, to adjust the weights of the linear regression model and achieve optimal results. These processes enable us to comprehend the structural differences in music across different periods with scientific rigor. Relying on the advantages of structuralism, we concentrate on the relationships and order between the physical elements of music, rather than getting entangled in the blurred boundaries of science and philosophy. Aside from serving as a bridge connecting music to natural language processing and knowledge graphs, the technical methods developed in this work offer a more intuitive approach to elucidate the relationships among elements of a complex network.
音乐,充满魅力和诗意,渗透到人类文明的每一个角落。尽管人们对音乐并不陌生,但对其本质的理解却依然有限,至今仍没有一个公认的科学描述。这主要是由于音乐被认为是理性和情感的产物,因而难以定义。本文将音乐文本视为一个复杂的系统。这一观点与语言学家约翰-鲁珀特-费斯(John Rupert Firth)的见解不谋而合,即理解一个词需要通过其周围的关系对其进行定义。为了构建网络,我们首先建立了一个线性回归模型,用阈值为音符、时间和音量之间的联系分配条件。然后,利用代表区域特征的聚类系数来定义单词。最后,严格要求文本的统计分布符合统计语言学的语法特性,如齐普夫定律,以调整线性回归模型的权重,达到最佳效果。这些过程使我们能够以科学严谨的态度理解不同时期音乐的结构差异。依托结构主义的优势,我们专注于音乐物理元素之间的关系和秩序,而不是纠缠于科学和哲学的模糊界限。除了作为连接音乐与自然语言处理和知识图谱的桥梁外,这项工作中开发的技术方法还为阐明复杂网络元素之间的关系提供了一种更直观的方法。
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引用次数: 0
Optimal control transport of neutral atoms in optical tweezers at finite temperature 有限温度下光学镊子中中性原子的优化控制传输
Pub Date : 2024-09-11 DOI: 10.1103/physrevresearch.6.033282
Alice Pagano, Daniel Jaschke, Werner Weiss, Simone Montangero
The transport of neutral atoms in Rydberg quantum computers is a crucial step for the initial arrangement of the grid as well as the dynamic connectivity, recently successfully demonstrated. We study the application of optimal control and the quantum speed limit for the transport of neutral atoms in optical tweezers at finite temperatures and analyze how laser noise affects transport fidelity. Open-loop optimal control significantly enhances transport fidelity, achieving an improvement up to 89% for the lowest analyzed temperature of 1µK for a distance of 3µm. Furthermore, we simulate how the transport fidelity behaves in release-and-capture measurements, which are realizable in the experiment to estimate transport efficiency and implement closed-loop optimal control.
中性原子在雷德堡量子计算机中的传输是网格初始排列和动态连接的关键步骤,这一点最近已被成功证明。我们研究了最优控制和量子速度极限在有限温度下光电镊子中中性原子传输中的应用,并分析了激光噪声如何影响传输保真度。开环优化控制显著提高了传输保真度,在 3µm 距离内,最低分析温度为 1µK,传输保真度提高了 89%。此外,我们还模拟了传输保真度在释放和捕获测量中的表现,这些测量可在实验中实现,以估算传输效率并实施闭环优化控制。
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引用次数: 0
Efficient learning of continuous-variable quantum states 连续可变量子态的高效学习
Pub Date : 2024-09-11 DOI: 10.1103/physrevresearch.6.033280
Ya-Dong Wu, Yan Zhu, Giulio Chiribella, Nana Liu
The characterization of continuous-variable quantum states is crucial for applications in quantum communication, sensing, simulation, and computing. However, a full characterization of multimode quantum states requires a number of experiments that grows exponentially with the number of modes. Here we propose an alternative approach where the goal is not to reconstruct the full quantum state, but rather to estimate its characteristic function at a given set of points. For multimode states with reflection symmetry, we show that the characteristic function at M points can be estimated using only O(logM) copies of the state, independently of the number of modes. When the characteristic function is known to be positive, as in the case of squeezed vacuum states, the estimation is achieved by an experimentally friendly setup using only beamsplitters and homodyne measurements.
连续可变量子态的表征对于量子通信、传感、模拟和计算领域的应用至关重要。然而,要对多模量子态进行全面表征,需要进行大量实验,而实验数量会随着模数的增加呈指数增长。在这里,我们提出了一种替代方法,其目标不是重建完整的量子态,而是估算其在给定点上的特征函数。对于具有反射对称性的多模态,我们证明只需使用 O(logM) 份状态副本就能估算出 M 个点上的特征函数,而与模数无关。当已知特征函数为正时,如在挤压真空态的情况下,只需使用分光镜和同调测量,就能通过实验友好型装置实现估算。
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引用次数: 0
Deterministic and multiuser quantum teleportation network of continuous-variable polarization states 确定性和多用户连续可变偏振态量子远距传输网络
Pub Date : 2024-09-11 DOI: 10.1103/physrevresearch.6.l032062
Jieli Yan, Xiaoyu Zhou, Yue Qin, Zhihui Yan, Xiaojun Jia, Changde Xie, Kunchi Peng
Quantum teleportation is widely applied as a key ingredient in quantum information science, and quantum network provides unique abilities for upscaling its applications. Polarization state of light is a vital degree of freedom with the advantages of remote transfer and direct light-atom interaction. To construct a multiuser quantum network, deterministic quantum teleportation of polarization state in more users' network remains challenging. Compared with photonic quantum state, the deterministic quantum teleportation network of polarization state is realized with a single set of continuous-variable entangled states. The key techniques include only one set of quadrature entangled network, single quadrature controller, and active polarization controller. Arbitrary polarization state is deterministically and controllably teleported in such a system involving four or three users. This system is deterministic and scalable with user number, which enables the potential application in deterministic metropolitan quantum network.
量子远距传输作为量子信息科学的关键要素被广泛应用,而量子网络则为扩大其应用提供了独特的能力。光的偏振态是一个重要的自由度,具有远程传输和光原子直接相互作用的优势。要构建多用户量子网络,在更多用户网络中实现偏振态的确定性量子远传仍是一项挑战。与光子量子态相比,偏振态的确定性量子远传网络是通过单组连续可变的纠缠态实现的。其关键技术包括只有一组正交纠缠网络、单一正交控制器和主动偏振控制器。在这样一个涉及四个或三个用户的系统中,可以确定并可控地传送任意偏振态。该系统具有确定性,并可随用户数量的增加而扩展,因此有可能应用于确定性城域量子网络。
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引用次数: 0
Strong coupling electron-photon dynamics: A real-time investigation of energy redistribution in molecular polaritons 强耦合电子光子动力学:分子极化子能量再分配的实时研究
Pub Date : 2024-09-11 DOI: 10.1103/physrevresearch.6.033283
Matteo Castagnola, Marcus T. Lexander, Enrico Ronca, Henrik Koch
We analyze the real-time electron-photon dynamics in long- and short-range energy transfer using a real-time quantum electrodynamics coupled cluster model, which allows for spatial and temporal visualization of transport processes. We compute the time evolution of photonic and molecular observables, such as the dipole moment and the photon coordinate, following the excitation of the system induced by short laser pulses. Our simulations show that intermolecular interactions and light-matter strong coupling lead to modified electronic polarization compared to the undressed molecules. The developed method can simulate multiple high-intensity laser pulses while explicitly retaining electronic and electron-photon correlation and is thus suited for nonlinear optics and transient absorption spectroscopies of molecular polaritons.
我们利用实时量子电动力学耦合簇模型分析了长程和短程能量传递中的实时电子-光子动力学,该模型可实现传输过程的空间和时间可视化。我们计算了短激光脉冲激发系统后光子和分子观测值(如偶极矩和光子坐标)的时间演化。模拟结果表明,与未穿衣服的分子相比,分子间相互作用和光-物质强耦合会导致电子极化的改变。所开发的方法可以模拟多个高强度激光脉冲,同时明确保留电子和电子光子相关性,因此适用于分子极化子的非线性光学和瞬态吸收光谱。
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引用次数: 0
From nonreciprocal to charge-4e supercurrent in Ge-based Josephson devices with tunable harmonic content 具有可调谐波含量的 Ge 基约瑟夫森器件中的非互惠到电荷-4e 超电流
Pub Date : 2024-09-11 DOI: 10.1103/physrevresearch.6.033281
Axel Leblanc, Chotivut Tangchingchai, Zahra Sadre Momtaz, Elyjah Kiyooka, Jean-Michel Hartmann, Gonzalo Troncoso Fernandez-Bada, Zoltán Scherübl, Boris Brun, Vivien Schmitt, Simon Zihlmann, Romain Maurand, Étienne Dumur, Silvano De Franceschi, François Lefloch
Hybrid superconductor(S)-semiconductor(Sm) devices bring a range of functionalities into superconducting circuits. In particular, hybrid parity-protected qubits and Josephson diodes were recently proposed and experimentally demonstrated. Such devices leverage the nonsinusoidal character of the Josephson current-phase relation (CPR) in highly transparent S-Sm-S junctions. Here, we report an experimental study of superconducting quantum-interference devices (SQUIDs) embedding Josephson field-effect transistors fabricated from a SiGe/Ge/SiGe heterostructure grown on a 200-mm silicon wafer. The single-junction CPR shows up to three harmonics with gate-tunable amplitude. In the presence of microwave irradiation, the ratio of the first two dominant harmonics, corresponding to single and double Cooper-pair transport processes, is consistently reflected in relative weight of integer and half-integer Shapiro steps. A combination of magnetic-flux and gate-voltage control enables tuning the SQUID functionality from a nonreciprocal Josephson-diode regime with 27% asymmetry to a π-periodic Josephson regime suitable for the implementation of parity-protected superconducting qubits. These results illustrate the potential of Ge-based hybrid devices as versatile and scalable building blocks of superconducting quantum circuits.
混合超导体(S)-半导体(Sm)器件为超导电路带来了一系列功能。特别是,混合奇偶校验保护量子比特和约瑟夫森二极管最近被提出并得到实验验证。这类器件利用了高透明 S-Sm-S 结中约瑟夫森电流相位关系(CPR)的非正弦特性。在此,我们报告了对嵌入约瑟夫森场效应晶体管的超导量子干涉器件(SQUID)的实验研究,该器件由生长在 200 毫米硅晶片上的 SiGe/Ge/SiGe 异质结构制成。单结 CPR 最多可显示三次谐波,其振幅可通过栅极调节。在微波辐照下,前两次主要谐波(对应于单库珀对传输过程和双库珀对传输过程)的比率始终反映在整数和半整数夏皮罗阶跃的相对权重上。结合磁通量和栅极电压控制,可以将 SQUID 的功能从具有 27% 不对称的非对等约瑟夫森二极管机制调整到适合实现奇偶保护超导量子位的π周期约瑟夫森机制。这些结果说明了基于 Ge 的混合器件作为超导量子电路的多功能和可扩展构件的潜力。
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引用次数: 0
Role of electrostatic doping on the resistance of metal and two-dimensional materials edge contacts 静电掺杂对金属和二维材料边缘接触电阻的影响
Pub Date : 2024-09-10 DOI: 10.1103/physrevresearch.6.033278
Madhuchhanda Brahma, Maarten L. Van de Put, Edward Chen, Massimo V. Fischetti, William G. Vandenberghe
In this theoretical study, we compare electrostatically doped metal-transition metal dichalcogenide (TMD) edge-contacts versus substitutionally doped edge-contacts in terms of their contact resistance. Our approach involves the utilization of electrostatic doping achieved by applying back-gate bias to the metal-TMD edge contacts, where carrier injection is primarily governed by the Schottky barrier at the interface. To analyze these contacts, we employ the Wentzel-Kramers-Brillouin (WKB) approximation to calculate the transmission coefficient and use density functional theory (DFT)-derived band structures. We numerically solve the Poisson equation to capture the electrostatic potential. We also account for the impact of the image force using Green's function for the Poisson equation with boundary conditions appropriate to our specific geometry. Our findings reveal that electrostatically doped TMD edge contacts exhibit higher contact resistance compared to impurity-doped edge contacts at equivalent carrier concentrations. At the same time, we find that, among the electrostatically doped edge contacts, a low-κ back-gate oxide in conjunction with low-κ top oxide is preferable in terms of improvement in contact resistance. For instance, in a metal-TMD edge contact scenario involving a monolayer MoS2 as the channel, SiO2 as the infinitely thick top oxide, and a SiO2 back-gate oxide with an equivalent oxide thickness (EOT) of 1nm, we demonstrate that it is possible to achieve an impressively low contact resistance of 50Ωµm when the back-gate bias exceeds or equals 2 V.
在这项理论研究中,我们比较了静电掺杂金属-过渡金属二卤化物(TMD)边缘接触与替代掺杂边缘接触的接触电阻。我们的方法是利用静电掺杂,通过向金属-TMD 边缘接触施加后栅偏压来实现,载流子注入主要受界面上肖特基势垒的控制。为了分析这些接触,我们采用 Wentzel-Kramers-Brillouin (WKB) 近似计算传输系数,并使用密度泛函理论 (DFT) 导出的带结构。我们通过数值求解泊松方程来捕捉静电势。我们还使用格林函数来计算图像力的影响,该函数用于泊松方程,边界条件适合我们特定的几何形状。我们的研究结果表明,在载流子浓度相当的情况下,静电掺杂的 TMD 边缘触点比杂质掺杂的边缘触点表现出更高的接触电阻。同时,我们还发现,在静电掺杂的边缘触点中,低κ后栅氧化物与低κ顶氧化物的结合更有利于改善接触电阻。例如,在以单层 MoS2 作为沟道、SiO2 作为无限厚的顶层氧化物、SiO2 作为等效氧化物厚度 (EOT) 为 1nm 的后栅氧化物的金属-TMD 边缘接触方案中,我们证明了当后栅偏压超过或等于 2 V 时,可以实现 50Ωµm 的超低接触电阻。
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引用次数: 0
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Physical Review Research
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