首页 > 最新文献

Journal of Magnetism and Magnetic Materials最新文献

英文 中文
Engineering skyrmion and helical states in FeGe nanocylinders through angular field control 通过角场控制控制FeGe纳米圆柱体的旋转和螺旋状态
IF 3 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-03-15 Epub Date: 2026-02-09 DOI: 10.1016/j.jmmm.2026.173916
Eduardo Saavedra , Lucy A. Valdez , Pablo Díaz , Noelia Bajales , Juan Escrig
We investigate how the orientation of an external magnetic field influences magnetization reversal and spin textures in FeGe nanocylinders using micromagnetic simulations based on the Landau–Lifshitz–Gilbert equation in MuMax3. FeGe, a prototypical chiral magnet with Dzyaloshinskii–Moriya interaction (DMI), stabilizes nontrivial spin textures such as skyrmions. We analyze nanocylinders of fixed length (50 nm) and diameters of 50–100 nm, subjected to fields applied at angles from 1° to 91° relative to the cylinder axis. Results show a pronounced angular dependence of coercivity and remanence, with sharp drops at diameter-dependent critical angles marking transitions from skyrmion-mediated reversal to trivial helical modes. Topological charge analysis confirms that below the critical angle, slices exhibit values near unity, while above it, the topological character vanishes. For larger diameters (90–100 nm), S-shaped helices linked to remanence minima emerge. These findings highlight angular control as a design parameter in spintronic devices exploiting topological textures.
我们利用基于Landau-Lifshitz-Gilbert方程的MuMax3微磁模拟研究了外磁场方向如何影响FeGe纳米柱的磁化反转和自旋结构。FeGe是一种典型的手性磁体,具有Dzyaloshinskii-Moriya相互作用(DMI),可以稳定非平凡自旋织构(如skyrmions)。我们分析了固定长度(50 nm)、直径为50 - 100 nm的纳米圆柱体,这些圆柱体受到相对于圆柱体轴线角度为1°至91°的电场作用。结果表明,矫顽力和剩余力具有明显的角依赖性,在与直径相关的临界角处急剧下降,标志着从天旋子介导的反转到微不足道的螺旋模式的转变。拓扑电荷分析证实,在临界角以下,薄片表现出接近统一的值,而在临界角以上,拓扑特征消失。对于更大的直径(90-100纳米),出现了与剩余物最小值相关的s形螺旋。这些发现突出了角控制作为利用拓扑结构的自旋电子器件的设计参数。
{"title":"Engineering skyrmion and helical states in FeGe nanocylinders through angular field control","authors":"Eduardo Saavedra ,&nbsp;Lucy A. Valdez ,&nbsp;Pablo Díaz ,&nbsp;Noelia Bajales ,&nbsp;Juan Escrig","doi":"10.1016/j.jmmm.2026.173916","DOIUrl":"10.1016/j.jmmm.2026.173916","url":null,"abstract":"<div><div>We investigate how the orientation of an external magnetic field influences magnetization reversal and spin textures in FeGe nanocylinders using micromagnetic simulations based on the Landau–Lifshitz–Gilbert equation in MuMax3. FeGe, a prototypical chiral magnet with Dzyaloshinskii–Moriya interaction (DMI), stabilizes nontrivial spin textures such as skyrmions. We analyze nanocylinders of fixed length (50 nm) and diameters of 50–100 nm, subjected to fields applied at angles from 1° to 91° relative to the cylinder axis. Results show a pronounced angular dependence of coercivity and remanence, with sharp drops at diameter-dependent critical angles marking transitions from skyrmion-mediated reversal to trivial helical modes. Topological charge analysis confirms that below the critical angle, slices exhibit values near unity, while above it, the topological character vanishes. For larger diameters (90–100 nm), S-shaped helices linked to remanence minima emerge. These findings highlight angular control as a design parameter in spintronic devices exploiting topological textures.</div></div>","PeriodicalId":366,"journal":{"name":"Journal of Magnetism and Magnetic Materials","volume":"642 ","pages":"Article 173916"},"PeriodicalIF":3.0,"publicationDate":"2026-03-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146185905","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Modulation of the magnetic soliton lattice by Fe doping in Cr1/3NbS2 铁掺杂Cr1/3NbS2对磁孤子晶格的调制
IF 3 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-03-15 Epub Date: 2026-02-07 DOI: 10.1016/j.jmmm.2026.173917
Shichao Zhang , Shuang Pan , Kaixin Zhu , Yuqing Bai , Chengcheng Xu , Xinji Xiang , Jun Liu , Feng Xu , Guizhou Xu
The magnetic chiral soliton lattice (CSL) is a topological spin texture with remarkable stability, arising from the competition between monoaxial Dzyaloshinskii–Moriya (DM) interaction and Heisenberg exchange interaction. In this study, we introduce Fe substitution into the prototypical CSL system Cr1/3NbS2, which effectively reduces its in-plane magnetic anisotropy. Notably, both the chiral helical order and the CSL state persist in the (Cr1-xFex)1/3NbS2 compound at x = 0.13, exhibiting a stripe period of approximately 72 nm at zero magnetic field. Combined with atomistic spin model simulations, we suggest that the enlarged period of magnetic stripes, compared to pristine Cr1/3NbS2, can originate from the DM change or reduced magnetic anisotropy. This work elucidates the important role of magnetic anisotropy in determining the CSL state.
磁手性孤子晶格(CSL)是由单轴Dzyaloshinskii-Moriya (DM)相互作用和海森堡交换相互作用竞争产生的具有显著稳定性的拓扑自旋织构。在本研究中,我们在原型CSL体系Cr1/3NbS2中引入Fe取代,有效地降低了其面内磁各向异性。值得注意的是,在x = 0.13时,(Cr1-xFex)1/3NbS2化合物的手性螺旋有序态和CSL态仍然存在,在零磁场下呈现出约72 nm的条纹周期。结合原子自旋模型的模拟,我们认为与原始Cr1/3NbS2相比,磁条周期的增大可能是由于DM的变化或磁各向异性的降低。这项工作阐明了磁各向异性在确定CSL状态中的重要作用。
{"title":"Modulation of the magnetic soliton lattice by Fe doping in Cr1/3NbS2","authors":"Shichao Zhang ,&nbsp;Shuang Pan ,&nbsp;Kaixin Zhu ,&nbsp;Yuqing Bai ,&nbsp;Chengcheng Xu ,&nbsp;Xinji Xiang ,&nbsp;Jun Liu ,&nbsp;Feng Xu ,&nbsp;Guizhou Xu","doi":"10.1016/j.jmmm.2026.173917","DOIUrl":"10.1016/j.jmmm.2026.173917","url":null,"abstract":"<div><div>The magnetic chiral soliton lattice (CSL) is a topological spin texture with remarkable stability, arising from the competition between monoaxial Dzyaloshinskii–Moriya (DM) interaction and Heisenberg exchange interaction. In this study, we introduce Fe substitution into the prototypical CSL system Cr<sub>1/3</sub>NbS<sub>2</sub>, which effectively reduces its in-plane magnetic anisotropy. Notably, both the chiral helical order and the CSL state persist in the (Cr<sub>1-x</sub>Fe<sub>x</sub>)<sub>1/3</sub>NbS<sub>2</sub> compound at <em>x</em> = 0.13, exhibiting a stripe period of approximately 72 nm at zero magnetic field. Combined with atomistic spin model simulations, we suggest that the enlarged period of magnetic stripes, compared to pristine Cr<sub>1/3</sub>NbS<sub>2</sub>, can originate from the DM change or reduced magnetic anisotropy. This work elucidates the important role of magnetic anisotropy in determining the CSL state.</div></div>","PeriodicalId":366,"journal":{"name":"Journal of Magnetism and Magnetic Materials","volume":"642 ","pages":"Article 173917"},"PeriodicalIF":3.0,"publicationDate":"2026-03-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146185936","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Ferromagnetic ordering and magnetodielectric coupling in paraelectric Dy2CoMnO6 perovskite 准电Dy2CoMnO6钙钛矿的铁磁有序和磁介电耦合
IF 3 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-03-15 Epub Date: 2026-02-07 DOI: 10.1016/j.jmmm.2026.173908
Gaoshang Gong , Xiaoying Chen , Yanxin Gao , Mengmeng Lun , Maocai Wei , Yongqiang Wang , Yuling Su
The double perovskite Dy2CoMnO6 polycrystalline was synthesized successfully. Its structure, magnetization and dielectric properties were studied. Refinement of the XRD diffraction data reveals a monoclinic structure for Dy2CoMnO6 compound. Unlike multiferroic Lu2CoMnO6, no spontaneous ferroelectric polarization is detected in Dy2CoMnO6. This difference can be attributed to that the different ionic radii of rare earth affect the sign and strength of the super-exchange interaction of Co2+-O-Mn4+. It causes the Dy2CoMnO6 to have a ferromagnetic ground state. Therefore, the spatial inversion symmetry in Dy2CoMnO6 can't be broken and spontaneous ferroelectricity is absent. But the Dy2CoMnO6 still present obvious magnetodielectric coupling. By investing the magnetic field dependent dielectric permittivity and dielectric loss, we demonstrate that the intrinsic coupling effect such as the reorientation of Co2+-Mn4+ dipole and the magnetostriction play the dominant role at low temperature. At high temperature the magnetoelectric coupling of Dy2CoMnO6 mainly comes from the magnetoresistance and Maxwell-Wagner effect.
成功合成了双钙钛矿型Dy2CoMnO6多晶。研究了其结构、磁化性能和介电性能。细化XRD衍射数据,发现Dy2CoMnO6化合物具有单斜晶型结构。与多铁性的Lu2CoMnO6不同,Dy2CoMnO6没有自发铁电极化。这种差异可归因于稀土离子半径的不同影响了Co2+-O-Mn4+超交换作用的符号和强度。它使Dy2CoMnO6具有铁磁基态。因此,Dy2CoMnO6的空间反演对称性不会被打破,不存在自发铁电性。但Dy2CoMnO6仍存在明显的磁介电耦合。通过研究与磁场相关的介电常数和介电损耗,我们证明了在低温下,Co2+-Mn4+偶极子的重定向和磁致伸缩等本征耦合效应起主导作用。在高温下,Dy2CoMnO6的磁电耦合主要来自磁电阻和麦克斯韦-瓦格纳效应。
{"title":"Ferromagnetic ordering and magnetodielectric coupling in paraelectric Dy2CoMnO6 perovskite","authors":"Gaoshang Gong ,&nbsp;Xiaoying Chen ,&nbsp;Yanxin Gao ,&nbsp;Mengmeng Lun ,&nbsp;Maocai Wei ,&nbsp;Yongqiang Wang ,&nbsp;Yuling Su","doi":"10.1016/j.jmmm.2026.173908","DOIUrl":"10.1016/j.jmmm.2026.173908","url":null,"abstract":"<div><div>The double perovskite Dy<sub>2</sub>CoMnO<sub>6</sub> polycrystalline was synthesized successfully. Its structure, magnetization and dielectric properties were studied. Refinement of the XRD diffraction data reveals a monoclinic structure for Dy<sub>2</sub>CoMnO<sub>6</sub> compound. Unlike multiferroic Lu<sub>2</sub>CoMnO<sub>6</sub>, no spontaneous ferroelectric polarization is detected in Dy<sub>2</sub>CoMnO<sub>6</sub>. This difference can be attributed to that the different ionic radii of rare earth affect the sign and strength of the super-exchange interaction of Co<sup>2+</sup>-O-Mn<sup>4+</sup>. It causes the Dy<sub>2</sub>CoMnO<sub>6</sub> to have a ferromagnetic ground state. Therefore, the spatial inversion symmetry in Dy<sub>2</sub>CoMnO<sub>6</sub> can't be broken and spontaneous ferroelectricity is absent<sub>.</sub> But the Dy<sub>2</sub>CoMnO<sub>6</sub> still present obvious magnetodielectric coupling. By investing the magnetic field dependent dielectric permittivity and dielectric loss, we demonstrate that the intrinsic coupling effect such as the reorientation of Co<sup>2+</sup>-Mn<sup>4+</sup> dipole and the magnetostriction play the dominant role at low temperature. At high temperature the magnetoelectric coupling of Dy<sub>2</sub>CoMnO<sub>6</sub> mainly comes from the magnetoresistance and Maxwell-Wagner effect.</div></div>","PeriodicalId":366,"journal":{"name":"Journal of Magnetism and Magnetic Materials","volume":"642 ","pages":"Article 173908"},"PeriodicalIF":3.0,"publicationDate":"2026-03-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146185938","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Correlated structural, magnetic and colossal magnetoresistance properties of La1-xSrxMnO3: Insights from XPS and 55Mn IFNMR La1-xSrxMnO3的相关结构、磁性和巨磁阻性质:来自XPS和55Mn IFNMR的见解
IF 3 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-03-15 Epub Date: 2026-01-31 DOI: 10.1016/j.jmmm.2026.173899
Arun Kumar S M , M Manjunatha , G Srinivasa Reddy , S Anandh Jesuraj , Basavaraj Angadi , David Laroze , Thipperudrappa J
We report the structural, magnetic, and colossal magnetoresistance (CMR) properties of Sr2+ − doped lanthanum manganites La1-xSrxMnO3 (x = 0.3, 0.4, 0.5) (LSMO) synthesized via the gel combustion method. X – ray diffraction (XRD) confirmed the formation of a single – phase rhombohedral perovskite structure (space group Rc), with refined lattice parameters showing a systematic decrease in the c-axis and crystallite sizes increasing from 20.85 to 23.02 nm as Sr2+ content increased. Fourier-transform infrared (FTIR) spectra exhibited Mn – O bending (∼ 500 cm−1) and stretching (∼ 640 cm−1) modes, with peak shifts and intensity changes confirming lattice strain and successful Sr2+ substitution. Raman spectroscopy revealed eight phonon modes (199–727 cm−1), including A1g and Eg symmetries, indicating local lattice distortions and Jahn – Teller effects due to Sr2+ doping. Magnetic properties were studied using vibrating sample magnetometry (VSM) and ferromagnetic resonance (FMR). VSM results showed decreasing saturation magnetization (MS) (57.10–34.69 emu/g) and increasing coercivity with Sr2+ doping, attributed to reduced double exchange interactions and increased Mn4+ content. FMR analysis showed enhanced g-factors (>2.00), with low – temperature data (77 K) indicating increased ferromagnetic ordering and static Jahn – Teller distortion. X – ray photoelectron spectroscopy (XPS) and 55Mn internal field nuclear magnetic resonance (IFNMR) were employed to analyze oxidation states and local magnetic environments, quantifying Mn3+/Mn4+ ratios and their role in magnetic behavior. CMR properties measured at 77 K revealed significant magnetoresistance, affirming the potential of these materials for applications in magnetic sensing, data storage, and spintronic devices.
本文报道了用凝胶燃烧法合成的Sr2+−掺杂镧锰酸盐La1-xSrxMnO3 (x = 0.3, 0.4, 0.5) (LSMO)的结构、磁性和巨大磁阻(CMR)性能。X射线衍射(XRD)证实形成了一种单相菱面体钙钛矿结构(空间群R3′c),随着Sr2+含量的增加,细化后的晶格参数c轴逐渐减小,晶粒尺寸从20.85 nm增大到23.02 nm。傅里叶变换红外(FTIR)光谱显示Mn - O弯曲(~ 500 cm−1)和拉伸(~ 640 cm−1)模式,峰移和强度变化证实了晶格应变和Sr2+成功取代。拉曼光谱显示了8种声子模式(199-727 cm−1),包括A1g和Eg对称性,表明Sr2+掺杂导致了局部晶格畸变和Jahn - Teller效应。利用振动样品磁强计(VSM)和铁磁共振(FMR)研究了其磁性能。VSM结果表明,Sr2+的掺杂降低了饱和磁化强度(MS) (57.10 ~ 34.69 emu/g),提高了矫顽力,这主要是由于双重交换作用的减少和Mn4+含量的增加。FMR分析显示g因子增强(>2.00),低温数据(77 K)表明铁磁有序和静态Jahn - Teller畸变增加。利用X射线光电子能谱(XPS)和55Mn内场核磁共振(IFNMR)分析氧化态和局部磁环境,量化Mn3+/Mn4+比值及其对磁行为的影响。在77 K下测量的CMR特性显示出显著的磁电阻,证实了这些材料在磁传感、数据存储和自旋电子器件中的应用潜力。
{"title":"Correlated structural, magnetic and colossal magnetoresistance properties of La1-xSrxMnO3: Insights from XPS and 55Mn IFNMR","authors":"Arun Kumar S M ,&nbsp;M Manjunatha ,&nbsp;G Srinivasa Reddy ,&nbsp;S Anandh Jesuraj ,&nbsp;Basavaraj Angadi ,&nbsp;David Laroze ,&nbsp;Thipperudrappa J","doi":"10.1016/j.jmmm.2026.173899","DOIUrl":"10.1016/j.jmmm.2026.173899","url":null,"abstract":"<div><div>We report the structural, magnetic, and colossal magnetoresistance (CMR) properties of Sr<sup>2+</sup> − doped lanthanum manganites La<sub>1-<em>x</em></sub>Sr<sub><em>x</em></sub>MnO<sub>3</sub> (<em>x</em> = 0.3, 0.4, 0.5) (LSMO) synthesized via the gel combustion method. X – ray diffraction (XRD) confirmed the formation of a single – phase rhombohedral perovskite structure (space group <em>R</em>3̅<em>c</em>), with refined lattice parameters showing a systematic decrease in the <em>c</em>-axis and crystallite sizes increasing from 20.85 to 23.02 nm as Sr<sup>2+</sup> content increased. Fourier-transform infrared (FTIR) spectra exhibited Mn – O bending (∼ 500 cm<sup>−1</sup>) and stretching (∼ 640 cm<sup>−1</sup>) modes, with peak shifts and intensity changes confirming lattice strain and successful Sr<sup>2+</sup> substitution. Raman spectroscopy revealed eight phonon modes (199–727 cm<sup>−1</sup>), including A<sub>1g</sub> and E<sub>g</sub> symmetries, indicating local lattice distortions and Jahn – Teller effects due to Sr<sup>2+</sup> doping. Magnetic properties were studied using vibrating sample magnetometry (VSM) and ferromagnetic resonance (FMR). VSM results showed decreasing saturation magnetization (<em>M</em><sub><em>S</em></sub>) (57.10–34.69 emu/g) and increasing coercivity with Sr<sup>2+</sup> doping, attributed to reduced double exchange interactions and increased Mn<sup>4+</sup> content. FMR analysis showed enhanced <em>g</em>-factors (&gt;2.00), with low – temperature data (77 K) indicating increased ferromagnetic ordering and static Jahn – Teller distortion. X – ray photoelectron spectroscopy (XPS) and <sup>55</sup>Mn internal field nuclear magnetic resonance (IFNMR) were employed to analyze oxidation states and local magnetic environments, quantifying Mn<sup>3+</sup>/Mn<sup>4+</sup> ratios and their role in magnetic behavior. CMR properties measured at 77 K revealed significant magnetoresistance, affirming the potential of these materials for applications in magnetic sensing, data storage, and spintronic devices.</div></div>","PeriodicalId":366,"journal":{"name":"Journal of Magnetism and Magnetic Materials","volume":"642 ","pages":"Article 173899"},"PeriodicalIF":3.0,"publicationDate":"2026-03-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146185799","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Magnetic properties of a three-dimensional system of ordered nanoparticles with cubic anisotropy: A Monte Carlo study 具有立方各向异性的有序纳米粒子三维体系的磁性:蒙特卡罗研究
IF 3 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-03-15 Epub Date: 2026-02-04 DOI: 10.1016/j.jmmm.2026.173903
M. Marchwiany , A. Majhofer , J. Szczytko , A. Twardowski
We investigate magnetic properties of a three-dimensional (3D) system of identical, spherical, single-domain, ferromagnetic nanoparticles with cubic magnetocrystalline anisotropy. Particles are immobilised in a nonmagnetic medium. Using the Monte Carlo techniques we simulate zero field cooled (ZFC) and field cooled (FC) experiments and calculate hysteresis curves for systems with different inter-particle distances. We compare results obtained when particles occupy sites of a simple cubic lattice with their anisotropy axes oriented randomly (Case A) and when particles are distributed randomly in space but with exactly parallel anisotropy axes of all nanoparticles (Case B). Values of the physical parameters used in our simulations correspond to the particles built of fcc-Co.
我们研究了具有立方磁晶各向异性的相同球形单畴铁磁纳米颗粒的三维(3D)系统的磁性。粒子固定在非磁性介质中。利用蒙特卡罗技术模拟了零场冷却(ZFC)和场冷却(FC)实验,并计算了不同粒子间距离系统的滞后曲线。我们比较了两种情况下得到的结果,一种是粒子占据简单立方晶格的位置,它们的各向异性轴随机取向(案例a),另一种是粒子在空间中随机分布,但所有纳米粒子的各向异性轴完全平行(案例B)。在我们的模拟中使用的物理参数值对应于由fcc-Co构成的粒子。
{"title":"Magnetic properties of a three-dimensional system of ordered nanoparticles with cubic anisotropy: A Monte Carlo study","authors":"M. Marchwiany ,&nbsp;A. Majhofer ,&nbsp;J. Szczytko ,&nbsp;A. Twardowski","doi":"10.1016/j.jmmm.2026.173903","DOIUrl":"10.1016/j.jmmm.2026.173903","url":null,"abstract":"<div><div>We investigate magnetic properties of a three-dimensional (3D) system of identical, spherical, single-domain, ferromagnetic nanoparticles with cubic magnetocrystalline anisotropy. Particles are immobilised in a nonmagnetic medium. Using the Monte Carlo techniques we simulate zero field cooled (ZFC) and field cooled (FC) experiments and calculate hysteresis curves for systems with different inter-particle distances. We compare results obtained when particles occupy sites of a simple cubic lattice with their anisotropy axes oriented randomly (Case A) and when particles are distributed randomly in space but with exactly parallel anisotropy axes of all nanoparticles (Case B). Values of the physical parameters used in our simulations correspond to the particles built of fcc-Co.</div></div>","PeriodicalId":366,"journal":{"name":"Journal of Magnetism and Magnetic Materials","volume":"642 ","pages":"Article 173903"},"PeriodicalIF":3.0,"publicationDate":"2026-03-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146185803","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Alleviating the peritectic phase formation of Mn–Bi hard magnets: Effect of isovalent Sb-doping and prospective short-time thermal-assisted annealing 减轻Mn-Bi硬磁体的包晶相形成:等价sb掺杂的影响和预期的短时间热辅助退火
IF 3 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-03-15 Epub Date: 2026-02-09 DOI: 10.1016/j.jmmm.2026.173918
Pham Thi Thanh , Nguyen Mau Lam , Nguyen Huy Ngoc , Kieu Xuan Hau , Nguyen Hai Yen , Do Khanh Tung , Huu T. Do , Jung-Goo Lee , Nguyen Huy Dan
Binary manganese-bismuthide-based (MnBi) alloys emerge as an exceptional archetype for a promising transition-metal-bearing hard magnet, but the high-quality alloying formation of the ferromagnetic phases is predominantly hindered by the peritectic reaction of transition metal Mn and semimetal Bi during the solidification procedure, as well as usually containing non-magnetic impurities. To alleviate these issues, we employed the well-established bottom-up procedure, including rapid melt-spinning, followed by a thermal crystalline-growth-assisted annealing process, to fabricate high-performance stoichiometric Mn54Bi46 alloying ribbon and its Sb-doped samples. Substituting a small amount (up to 4 at. %) of isovalent configuration (s2p3) Sb for Bi in the samples pronounces the particle-size reduction, resulting in a typically positive effect of coercivity force in phase formation as well as fractional enhancement of the ferromagnetic MnBi phases. In particular, the underlying permanent magnetic features, such as coercivity (Hc) and saturation magnetization (Ms), reach corresponding values of 14 kOe with 20 emu/g and 10.5 kOe with 52.5 emu/g, with a typical (BH)max = 3.9 MGOe for 2 at. % Sb-doping concentration before and after the annealing conditions of 200 °C for 2 h. While magnetocrystalline anisotropy K1 is a missing piece in previous studies of Sb-doped MnBi materials, by applying the law of approach to saturation magnetization to high-field magnetic data, we obtain K1 = 0.92–1.1 MJ/m3 for the 0–3 at. % Sb-doping annealed samples, which overlap with the known value of pristine MnBi alloys.
二元锰铋基(MnBi)合金是一种非常有前途的含过渡金属的硬磁体,但铁磁相的高质量合金形成主要受到凝固过程中过渡金属Mn和半金属Bi的包晶反应的阻碍,并且通常含有非磁性杂质。为了解决这些问题,我们采用了自底向上的方法,包括快速熔融纺丝,然后是热晶体生长辅助退火工艺,来制造高性能的化学计量Mn54Bi46合金带及其sb掺杂样品。代入少量(直到4 at)。%)的等价构型(s2p3) Sb对样品中的Bi表示颗粒尺寸减小,导致相形成中矫顽力的典型积极影响以及铁磁性MnBi相的分数增强。其中,20emu /g时矫顽力(Hc)和饱和磁化强度(Ms)分别达到14koe和10.5 kOe (52.5 emu/g), 2 at时典型的(BH)max = 3.9 MGOe。在200°C退火2 h的条件下,磁晶各向异性K1是以往sb掺杂MnBi材料研究中缺失的一块,通过将饱和磁化趋近定律应用于高磁场数据,我们得到0-3 at的K1 = 0.92-1.1 MJ/m3。% sb掺杂退火样品,与原始MnBi合金的已知值重叠。
{"title":"Alleviating the peritectic phase formation of Mn–Bi hard magnets: Effect of isovalent Sb-doping and prospective short-time thermal-assisted annealing","authors":"Pham Thi Thanh ,&nbsp;Nguyen Mau Lam ,&nbsp;Nguyen Huy Ngoc ,&nbsp;Kieu Xuan Hau ,&nbsp;Nguyen Hai Yen ,&nbsp;Do Khanh Tung ,&nbsp;Huu T. Do ,&nbsp;Jung-Goo Lee ,&nbsp;Nguyen Huy Dan","doi":"10.1016/j.jmmm.2026.173918","DOIUrl":"10.1016/j.jmmm.2026.173918","url":null,"abstract":"<div><div>Binary manganese-bismuthide-based (MnBi) alloys emerge as an exceptional archetype for a promising transition-metal-bearing hard magnet, but the high-quality alloying formation of the ferromagnetic phases is predominantly hindered by the peritectic reaction of transition metal Mn and semimetal Bi during the solidification procedure, as well as usually containing non-magnetic impurities. To alleviate these issues, we employed the well-established bottom-up procedure, including rapid melt-spinning, followed by a thermal crystalline-growth-assisted annealing process, to fabricate high-performance stoichiometric Mn<sub>54</sub>Bi<sub>46</sub> alloying ribbon and its Sb-doped samples. Substituting a small amount (up to 4 at. %) of isovalent configuration (s<span><math><msup><mrow></mrow><mrow><mn>2</mn></mrow></msup></math></span>p<span><math><msup><mrow></mrow><mrow><mn>3</mn></mrow></msup></math></span>) Sb for Bi in the samples pronounces the particle-size reduction, resulting in a typically positive effect of coercivity force in phase formation as well as fractional enhancement of the ferromagnetic MnBi phases. In particular, the underlying permanent magnetic features, such as coercivity (<span><math><msub><mrow><mi>H</mi></mrow><mrow><mi>c</mi></mrow></msub></math></span>) and saturation magnetization (<span><math><msub><mrow><mi>M</mi></mrow><mrow><mi>s</mi></mrow></msub></math></span>), reach corresponding values of 14 kOe with 20 emu/g and 10.5 kOe with 52.5 emu/g, with a typical <span><math><msub><mrow><mrow><mo>(</mo><mi>B</mi><mi>H</mi><mo>)</mo></mrow></mrow><mrow><mtext>max</mtext></mrow></msub></math></span> = 3.9 MGOe for 2 at. % Sb-doping concentration before and after the annealing conditions of 200 °C for 2 h. While magnetocrystalline anisotropy <span><math><msub><mrow><mi>K</mi></mrow><mrow><mn>1</mn></mrow></msub></math></span> is a missing piece in previous studies of Sb-doped MnBi materials, by applying the law of approach to saturation magnetization to high-field magnetic data, we obtain <span><math><msub><mrow><mi>K</mi></mrow><mrow><mn>1</mn></mrow></msub></math></span> = 0.92–1.1 MJ/m<span><math><msup><mrow></mrow><mrow><mn>3</mn></mrow></msup></math></span> for the 0–3 at. % Sb-doping annealed samples, which overlap with the known value of pristine MnBi alloys.</div></div>","PeriodicalId":366,"journal":{"name":"Journal of Magnetism and Magnetic Materials","volume":"642 ","pages":"Article 173918"},"PeriodicalIF":3.0,"publicationDate":"2026-03-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146185902","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Planar microresonator-assisted nonlinear magnetization dynamics based on strong magnon-photon coupling 基于强磁子-光子耦合的平面微谐振辅助非线性磁化动力学
IF 3 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-03-15 Epub Date: 2026-02-07 DOI: 10.1016/j.jmmm.2026.173877
Xinhui Ma, Guanqi Ye, Fusheng Ma
With the development of quantum information technologies, the nonlinear effects of coupled magnon-photon systems have drawn great attention. In this work, we design and fabricate an R-shaped planar microresonator (PMR) with high quality factor and high microwave conversion efficiency. The strong coupling between microwave photons in PMR and magnons in YIG is achieved under different configurations of bias magnetic field. Interestingly, under out-of-plane bias field and high microwave power, the spectrum displays two characteristics: the blue shift of magnon mode and the comb-like feature. The blue shift of magnon mode originates from the intrinsic magnon nonlinearity, and the comb-like spectrum originates from the hybridization of magnon mode with microwave photon mode and phonon modes. Our findings indicate the potential of PMR for exploring nonlinear cavity magnonics and on-chip integrated quantum information technologies.
随着量子信息技术的发展,耦合磁-光子系统的非线性效应引起了人们的广泛关注。在本工作中,我们设计并制造了一个具有高品质因数和高微波转换效率的r型平面微谐振器(PMR)。在不同的偏置磁场配置下,实现了PMR中的微波光子与YIG中的磁振子之间的强耦合。有趣的是,在面外偏置场和高微波功率下,光谱呈现出磁振子模式蓝移和梳状特征。磁振子模式的蓝移源于磁振子的本征非线性,梳状光谱源于磁振子模式与微波光子模式和声子模式的杂化。我们的发现表明了PMR在探索非线性腔磁学和片上集成量子信息技术方面的潜力。
{"title":"Planar microresonator-assisted nonlinear magnetization dynamics based on strong magnon-photon coupling","authors":"Xinhui Ma,&nbsp;Guanqi Ye,&nbsp;Fusheng Ma","doi":"10.1016/j.jmmm.2026.173877","DOIUrl":"10.1016/j.jmmm.2026.173877","url":null,"abstract":"<div><div>With the development of quantum information technologies, the nonlinear effects of coupled magnon-photon systems have drawn great attention. In this work, we design and fabricate an R-shaped planar microresonator (PMR) with high quality factor and high microwave conversion efficiency. The strong coupling between microwave photons in PMR and magnons in YIG is achieved under different configurations of bias magnetic field. Interestingly, under out-of-plane bias field and high microwave power, the spectrum displays two characteristics: the blue shift of magnon mode and the comb-like feature. The blue shift of magnon mode originates from the intrinsic magnon nonlinearity, and the comb-like spectrum originates from the hybridization of magnon mode with microwave photon mode and phonon modes. Our findings indicate the potential of PMR for exploring nonlinear cavity magnonics and on-chip integrated quantum information technologies.</div></div>","PeriodicalId":366,"journal":{"name":"Journal of Magnetism and Magnetic Materials","volume":"642 ","pages":"Article 173877"},"PeriodicalIF":3.0,"publicationDate":"2026-03-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146185935","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Unveiling magnetic transition in Fe2SiO4 fayalites via magnetocaloric effect 利用磁热效应揭示Fe2SiO4合金中的磁跃迁
IF 3 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-03-15 Epub Date: 2026-02-09 DOI: 10.1016/j.jmmm.2026.173920
Y. Errouyessi , M. Lassri , S. El Ouahbi , L. Bessais , B. Manoun , H. Lassri , R. Moubah
This study explores the magnetic and magnetocaloric properties of Fe2SiO4 fayalite. While classical magnetization measurements at a magnetic field of 0.01 T reveal the existence of only one transition from an inclined antiferromagnetic state to a collinear antiferromagnetic state at 30 K. Magnetic entropy (-ΔSm) across different temperatures and magnetic fields, reveals the existence of two well defined peaks corresponding to two magnetic transitions. One transition located at the Critical Temperature (TCr) around 30 K, and a second transition located at Néel temperature (TN) around 70 K marks the change from a collinear antiferromagnetic state to a paramagnetic state. This latter transition is not visible in the conventional magnetization at low fields versus temperature measurements. The phase transition induced by magnetic fields is identified as second order based on Arrott plots. The relative cooling power (RCP) was found to depend on the magnetic field according to a power law. These results demonstrate that the magnetocaloric effect is a particularly effective probe for detecting and studying complex magnetic transitions.
本研究探讨了Fe2SiO4铁矾的磁性和磁热学性质。而在0.01 T磁场下的经典磁化测量表明,在30k时,从倾斜反铁磁态到共线反铁磁态只存在一次跃迁。磁熵(-ΔSm)跨越不同的温度和磁场,揭示了两个明确的峰对应于两个磁跃迁的存在。在30 K左右的临界温度(TCr)和70 K左右的nsamel温度(TN)发生的第二次转变标志着共线反铁磁态向顺磁态的转变。后一种转变是不可见的,在传统的磁化在低场与温度测量。根据Arrott图,确定了磁场诱导的相变为二阶相变。相对冷却功率(RCP)根据幂律与磁场有关。这些结果表明,磁热效应是一种特别有效的探测和研究复杂磁跃迁的探针。
{"title":"Unveiling magnetic transition in Fe2SiO4 fayalites via magnetocaloric effect","authors":"Y. Errouyessi ,&nbsp;M. Lassri ,&nbsp;S. El Ouahbi ,&nbsp;L. Bessais ,&nbsp;B. Manoun ,&nbsp;H. Lassri ,&nbsp;R. Moubah","doi":"10.1016/j.jmmm.2026.173920","DOIUrl":"10.1016/j.jmmm.2026.173920","url":null,"abstract":"<div><div>This study explores the magnetic and magnetocaloric properties of <span><math><msub><mi>Fe</mi><mn>2</mn></msub><msub><mi>SiO</mi><mn>4</mn></msub></math></span> fayalite. While classical magnetization measurements at a magnetic field of 0.01 T reveal the existence of only one transition from an inclined antiferromagnetic state to a collinear antiferromagnetic state at 30 K. Magnetic entropy (<em>-ΔS</em><sub><em>m</em></sub>) across different temperatures and magnetic fields, reveals the existence of two well defined peaks corresponding to two magnetic transitions. One transition located at the Critical Temperature (<em>T</em><sub><em>Cr</em></sub>) around 30 K, and a second transition located at Néel temperature (<em>T</em><sub><em>N</em></sub>) around 70 K marks the change from a collinear antiferromagnetic state to a paramagnetic state. This latter transition is not visible in the conventional magnetization at low fields versus temperature measurements. The phase transition induced by magnetic fields is identified as second order based on Arrott plots. The relative cooling power (<em>RCP</em>) was found to depend on the magnetic field according to a power law. These results demonstrate that the magnetocaloric effect is a particularly effective probe for detecting and studying complex magnetic transitions.</div></div>","PeriodicalId":366,"journal":{"name":"Journal of Magnetism and Magnetic Materials","volume":"642 ","pages":"Article 173920"},"PeriodicalIF":3.0,"publicationDate":"2026-03-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146185904","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Perpendicularly magnetized Tb/Co multilayers featuring tilted uniaxial anisotropy: Experiments and modeling 具有倾斜单轴各向异性的垂直磁化Tb/Co多层层:实验与建模
IF 3 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-03-15 Epub Date: 2026-01-22 DOI: 10.1016/j.jmmm.2026.173830
J.C. Rodriguez E. , L. Avilés-Félix , M.H. Aguirre , L.M. Rodríguez , D. Salomoni , S. Auffret , R.C. Sousa , I.L. Prejbeanu , A.E. Bruchhausen , E. De Biasi , J. Curiale
Rare earth/transition metal (RE/TM) multilayers with perpendicular magnetic anisotropy are key ingredients for the development of spintronic applications. Their compensation temperature depends on the ratio of the thicknesses of rare earth and transition metal, allowing their magnetic properties to be tuned with temperature while maintaining their anisotropy even in nanometer-scale devices. In this work, we performed a thorough structural characterization and systematically investigate the magnetic properties of a whole family of ferrimagnetic [Tb/Co]×5 multilayers varying the Tb thickness in the range of 0.4nm - 1.25nm. A linear dependence of the compensation temperature on the Tb layer thickness was observed. Moreover, a uniaxial anisotropy constant of (330±30)kJ/m3, which is close to the values reported by other authors, was estimated. Additionally, we proposed a model to gain a better understanding of the angular dependence of the magnetization loops and the linear dependence of the compensation temperature. We present strong evidence demonstrating that the perpendicular anisotropy must be tilted away from the perpendicular axis in order to explain the observed features, particularly the hysteresis in the in-plane loops. Our work advances the understanding of DC magnetic properties in thin RE/TM ferrimagnetic films, which has the potential to impact different fields where these materials are involved.
具有垂直磁各向异性的稀土/过渡金属(RE/TM)多层材料是发展自旋电子应用的关键因素。它们的补偿温度取决于稀土和过渡金属厚度的比例,这使得它们的磁性能随温度调整,同时即使在纳米级器件中也能保持它们的各向异性。在这项工作中,我们进行了彻底的结构表征,并系统地研究了整个家族的铁磁[Tb/Co]×5多层膜的磁性能,其Tb厚度在0.4nm - 1.25nm范围内变化。补偿温度与Tb层厚度呈线性关系。此外,估计的单轴各向异性常数为(330±30)kJ/m3,与其他作者报道的值接近。此外,我们提出了一个模型来更好地理解磁化回路的角依赖性和补偿温度的线性依赖性。我们提出了强有力的证据,证明垂直各向异性必须倾斜远离垂直轴,以解释观察到的特征,特别是面内环的滞后。我们的工作促进了对薄RE/TM铁磁薄膜直流磁性的理解,这有可能影响这些材料所涉及的不同领域。
{"title":"Perpendicularly magnetized Tb/Co multilayers featuring tilted uniaxial anisotropy: Experiments and modeling","authors":"J.C. Rodriguez E. ,&nbsp;L. Avilés-Félix ,&nbsp;M.H. Aguirre ,&nbsp;L.M. Rodríguez ,&nbsp;D. Salomoni ,&nbsp;S. Auffret ,&nbsp;R.C. Sousa ,&nbsp;I.L. Prejbeanu ,&nbsp;A.E. Bruchhausen ,&nbsp;E. De Biasi ,&nbsp;J. Curiale","doi":"10.1016/j.jmmm.2026.173830","DOIUrl":"10.1016/j.jmmm.2026.173830","url":null,"abstract":"<div><div>Rare earth/transition metal (RE/TM) multilayers with perpendicular magnetic anisotropy are key ingredients for the development of spintronic applications. Their compensation temperature depends on the ratio of the thicknesses of rare earth and transition metal, allowing their magnetic properties to be tuned with temperature while maintaining their anisotropy even in nanometer-scale devices. In this work, we performed a thorough structural characterization and systematically investigate the magnetic properties of a whole family of ferrimagnetic [Tb/Co]<span><math><msub><mrow></mrow><mrow><mo>×</mo><mn>5</mn></mrow></msub></math></span> multilayers varying the Tb thickness in the range of 0.4nm - 1.25nm. A linear dependence of the compensation temperature on the Tb layer thickness was observed. Moreover, a uniaxial anisotropy constant of <span><math><mrow><mrow><mo>(</mo><mn>330</mn><mo>±</mo><mn>30</mn><mo>)</mo></mrow><mspace></mspace><mstyle><mstyle><mi>k</mi><mi>J</mi></mstyle></mstyle><mo>/</mo><msup><mrow><mstyle><mstyle><mi>m</mi></mstyle></mstyle></mrow><mrow><mn>3</mn></mrow></msup></mrow></math></span>, which is close to the values reported by other authors, was estimated. Additionally, we proposed a model to gain a better understanding of the angular dependence of the magnetization loops and the linear dependence of the compensation temperature. We present strong evidence demonstrating that the perpendicular anisotropy must be tilted away from the perpendicular axis in order to explain the observed features, particularly the hysteresis in the in-plane loops. Our work advances the understanding of DC magnetic properties in thin RE/TM ferrimagnetic films, which has the potential to impact different fields where these materials are involved.</div></div>","PeriodicalId":366,"journal":{"name":"Journal of Magnetism and Magnetic Materials","volume":"642 ","pages":"Article 173830"},"PeriodicalIF":3.0,"publicationDate":"2026-03-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146057463","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Perpendicular magnetized flexible CoFeB/pt multilayers with pt thickness dependent interfacial magnetic anisotropy 具有pt厚度相关界面磁各向异性的垂直磁化柔性CoFeB/pt多层膜
IF 3 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-03-15 Epub Date: 2026-01-27 DOI: 10.1016/j.jmmm.2026.173878
Yan Liu , Bin Lao , Yali Xie , Huali Yang , Xilai Bao , Huatao Jiang , Ruoan Zou , Pengfei Xin , Yao Ying , Run-Wei Li
Earlier demonstration of magnetic film-based functionalities on flexible substrates have highlighted the importance of perpendicular magnetic anisotropy (PMA) in flexible electronics. Here we studied magnetic anisotropic properties of flexible CoFeB/Pt multilayers with various structural parameters including substrate roughness, layer thickness, and stacking period, to anatomy the involved variables on PMA magnitude. A robust PMA is achieved in flexible CoFeB/Pt multilayers after improving surface roughness of flexible substrate, which is identical to that grown on rigid substrate. CoFeB and Pt thickness dependent magnetic anisotropy analysis confirms that the PMA is originated from CoFeB/Pt interface with a constant magnitude of 0.39 erg/cm2 regardless of the stack period. However, for Pt thickness below 1.5 nm, the interfacial PMA is gradually decrease, resulting in the magnetic easy axis shifts from perpendicular to planar orientation as the stacking period increases. After excluding possible influences from interfacial roughness and magnetic interlayer interactions, the reduction in PMA is attributed to limited orbital hybridization at the interface caused by the insufficient thickness of the Pt layer.
早期在柔性衬底上的基于磁膜的功能演示突出了垂直磁各向异性(PMA)在柔性电子中的重要性。本文研究了不同结构参数(衬底粗糙度、层厚和堆叠周期)下柔性CoFeB/Pt多层膜的磁各向异性,分析了PMA量级的相关变量。通过改善柔性基板的表面粗糙度,在柔性CoFeB/Pt多层材料中获得了与刚性基板相同的坚固PMA。与CoFeB和Pt厚度相关的磁各向异性分析证实,PMA来源于CoFeB/Pt界面,无论堆叠周期如何,PMA的恒定量级为0.39 erg/cm2。而Pt厚度在1.5 nm以下时,界面PMA逐渐减小,导致磁易轴由垂直方向向平面方向偏移。在排除了界面粗糙度和磁层间相互作用的可能影响后,PMA的减少归因于Pt层厚度不足导致的界面上轨道杂化有限。
{"title":"Perpendicular magnetized flexible CoFeB/pt multilayers with pt thickness dependent interfacial magnetic anisotropy","authors":"Yan Liu ,&nbsp;Bin Lao ,&nbsp;Yali Xie ,&nbsp;Huali Yang ,&nbsp;Xilai Bao ,&nbsp;Huatao Jiang ,&nbsp;Ruoan Zou ,&nbsp;Pengfei Xin ,&nbsp;Yao Ying ,&nbsp;Run-Wei Li","doi":"10.1016/j.jmmm.2026.173878","DOIUrl":"10.1016/j.jmmm.2026.173878","url":null,"abstract":"<div><div>Earlier demonstration of magnetic film-based functionalities on flexible substrates have highlighted the importance of perpendicular magnetic anisotropy (PMA) in flexible electronics. Here we studied magnetic anisotropic properties of flexible CoFeB/Pt multilayers with various structural parameters including substrate roughness, layer thickness, and stacking period, to anatomy the involved variables on PMA magnitude. A robust PMA is achieved in flexible CoFeB/Pt multilayers after improving surface roughness of flexible substrate, which is identical to that grown on rigid substrate. CoFeB and Pt thickness dependent magnetic anisotropy analysis confirms that the PMA is originated from CoFeB/Pt interface with a constant magnitude of 0.39 erg/cm<sup>2</sup> regardless of the stack period. However, for Pt thickness below 1.5 nm, the interfacial PMA is gradually decrease, resulting in the magnetic easy axis shifts from perpendicular to planar orientation as the stacking period increases. After excluding possible influences from interfacial roughness and magnetic interlayer interactions, the reduction in PMA is attributed to limited orbital hybridization at the interface caused by the insufficient thickness of the Pt layer.</div></div>","PeriodicalId":366,"journal":{"name":"Journal of Magnetism and Magnetic Materials","volume":"642 ","pages":"Article 173878"},"PeriodicalIF":3.0,"publicationDate":"2026-03-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"146076817","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Journal of Magnetism and Magnetic Materials
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1