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Absolute timing of laser-driven radiation sources interacting in matter 激光驱动辐射源在物质中相互作用的绝对定时
Pub Date : 2023-06-08 DOI: 10.1117/12.2665624
J. P. Kennedy, Colm Fitzpatrick, M. Coughlan, M. Yeung, B. Dromey
A major challenge facing the study of radiation in matter on ultrafast time scales is the need for an absolute timing reference. Typically, these type of experiments are performed using pulses of ions from radio frequency accelerators which have nanosecond scale pulse durations and timing jitter making high temporal resolution measurements difficult to achieve. Here, we show that a combination of a highly synchronised probe pulse with a muti-species laser-driven radiation source can allow for the absolute timing of radiation in matter. This is primarily due to the generation of a X-ray calibration fiducial enabling the study of ion-induced dynamics in matter on ultrafast timescales.
在超快时间尺度上研究物质辐射面临的一个主要挑战是需要一个绝对的时间参考。通常,这些类型的实验是使用来自射频加速器的离子脉冲进行的,这些脉冲具有纳秒级的脉冲持续时间和定时抖动,使得高时间分辨率的测量难以实现。在这里,我们展示了高度同步的探针脉冲与多物种激光驱动辐射源的组合可以允许物质中辐射的绝对定时。这主要是由于x射线校准基准的产生,使得离子诱导的物质动力学研究在超快时间尺度上。
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引用次数: 0
Photomobile films based on liquid crystal polymer-carbon black composites 基于液晶聚合物-炭黑复合材料的光电薄膜
Pub Date : 2023-06-08 DOI: 10.1117/12.2673120
F. Loffredo, Anna De Girolamo Del Mauro, F. Villani, M. F. Caso, T. Fasolino, R. Miscioscia, A. Vestri, D. Sagnelli, Amalia D'Avino, L. Petti, G. Nenna
Films based on a composite of a liquid crystal polymer (LC-POL) with acrylic backbone and carbon black (CB) were manufactured and characterized to develop a new smart material able to move under light. In detail, the effect of 0.1wt% of CB, a high absorption and thermal conductive filler, on morphological, optical and photomobile properties was investigated and compared with pristine LC-POL films. To study photomobile behaviuor the films were irradiated with 457nm-laser at different powers and the responses to these stimuli were compared in terms of bending angle and response time. The work shows that the presence of CB induces photomobile properties in an inactive LC polymer matrix and the mechanical response under light is fast and reversible.
制备了一种基于丙烯酸骨架和炭黑(CB)的液晶聚合物(LC-POL)复合材料的薄膜,并对其进行了表征,以开发一种能够在光下移动的新型智能材料。详细地研究了0.1wt%的高吸收率和导热填料CB对LC-POL薄膜形貌、光学和光电迁移性能的影响,并与原始LC-POL薄膜进行了比较。为了研究薄膜的光电移动行为,我们用不同功率的457nm激光照射薄膜,并比较了薄膜在这些刺激下的弯曲角度和响应时间。研究表明,CB的存在诱导了非活性LC聚合物基质的光电迁移特性,并且在光下的机械响应是快速和可逆的。
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引用次数: 0
Picosecond ramp of ultrashort laser pulse: its effect on laser-driven ion acceleration or plasma shutter 超短激光脉冲皮秒斜坡:对激光驱动离子加速或等离子体快门的影响
Pub Date : 2023-06-08 DOI: 10.1117/12.2665514
J. Psikal
The effect of picosecond ramp of ultrashort laser pulse is investigated with the help of particle-in-cell simulations. It is shown that the ramp changes cutoff energies and numbers of ions accelerated from laser-irradiated target depending on laser pulse intensity. It can also substantially change the interaction of the main high-intensity part of the pulse with thin membrane used as a plasma shutter to shape laser pulse temporal profile.
利用粒子池模拟研究了超短激光脉冲皮秒斜坡的影响。结果表明,随着激光脉冲强度的变化,激光辐照靶加速的截止能量和离子数发生了变化。它还可以从本质上改变脉冲的主要高强度部分与薄膜的相互作用,薄膜用作等离子体快门来塑造激光脉冲的时间轮廓。
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引用次数: 0
Structural and luminescent properties of dysprosium ions-doped tungstate phosphor for w-LEDs w- led用镝离子掺杂钨酸盐荧光粉的结构和发光性能
Pub Date : 2023-06-08 DOI: 10.1117/12.2669275
Anu ., Nisha Deopa, A. Rao
In the present research work, a Dy3+ doped Tungstate phosphor that emits light in white region has been synthesized using conventional solid-state reaction. An X-ray diffraction (XRD) pattern for the as-synthesized phosphor material was recorded for structural analysis and phase identification. The diffraction peaks of the tungstate phosphor match very well with the standard JCPDS pattern. The optical band gap value of the as-synthesized phosphor has been measured using diffuse reflectance spectra (DRS). The photoluminescence (PL) spectral features recorded for the Dy3+ ions activated tungstate phosphor under 360 nm excitation reveal strong emission peaks in blue (490 nm), a relatively less intense peak in the yellow region (580 nm) and a significantly less intense red peak (683 nm). From the recorded PL spectra, the CIE chromaticity coordinates (0.33046, 0.37422) estimated for 1.0 mol% doping concentration of Dy3+ ions in the as-prepared phosphor material are falling in the white region. CCT value (5580K) signifies its application for cool white light-emitting diode (w-LEDs). The PL decay spectral profile recorded at 480 nm emission under 360 nm excitation shows double exponential behaviour. The temperature-dependent PL (TDPL) measurements demonstrate relatively better thermal stability for the as-synthesized phosphor. All the investigations carried out finally allow us to contemplate the suitability of Dy3+ ions doped tungstate phosphor for w-LED.
在本研究中,采用常规固相反应合成了一种在白色区域发光的掺杂Dy3+的钨酸盐荧光粉。合成的荧光粉材料的x射线衍射(XRD)图被记录下来用于结构分析和物相鉴定。钨酸盐荧光粉的衍射峰与标准的JCPDS模式匹配良好。利用漫反射光谱(DRS)测量了合成荧光粉的光学带隙值。在360 nm激发下,Dy3+离子激活的钨酸盐荧光粉的光致发光(PL)光谱特征显示,蓝色区域(490 nm)有较强的发光峰,黄色区域(580 nm)有较弱的发光峰,红色区域(683nm)有较弱的发光峰。从记录的PL光谱来看,在制备的荧光粉材料中掺杂浓度为1.0 mol%的Dy3+离子时,CIE色度坐标(0.33046,0.37422)落在白色区域。CCT值(5580K)表示其应用于冷白光发光二极管(w- led)。在360nm激发下,在480nm处记录的PL衰减光谱曲线表现出双指数行为。温度相关的PL (TDPL)测量表明,合成的荧光粉具有相对较好的热稳定性。所有的研究最终使我们能够考虑Dy3+离子掺杂钨酸盐荧光粉用于w-LED的适用性。
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引用次数: 1
Recent experiments and advances at the high-repetition-rate attosecond beamlines of ELI ALPS ELI ALPS高重复率阿秒光束的实验与进展
Pub Date : 2023-06-08 DOI: 10.1117/12.2664845
L. Gulyás Oldal, T. Csizmadia, Z. Filus, T. Grósz, M. De Marco, P. Jójárt, I. Seres, Z. Bengery, B. Gilicze, K. Varjú, S. Kahaly, B. Major
The High-Repetition-rate laser-driven Gas-based High-order Harmonic Generation (HR GHHG) beamlines of the Extreme Light Infrastructure Attosecond Light Pulse Source (ELI ALPS) have started their operation in the recent years. Both beamlines, one designed for gas-phase targets – the HR GHHG Gas beamline –, and one for condensed-phase samples – the HR GHHG Condensed beamline –, now provide high-flux, extreme ultraviolet (XUV) radiation with pump-probe capabilities at 100 kHz repetition rate. The HR GHHG Cond beamline is equipped with a time-compensated XUV monochromator, allowing for tuning the spectral properties while maintaining short, close to Fourier-limited pulse duration in the femtosecond regime. Cutting-edge experimental end stations are also available, for example a Reaction Microscope and a NanoESCA device. Both beamlines are past their first commissioning user experiments. In this presentation the capabilities along with some recent developments and latest experiments will be presented for these two unique attosecond sources.
近年来,极光基础设施阿秒脉冲光源(ELI ALPS)的高重复率激光驱动气体基高次谐波产生(HR GHHG)光束线已经开始运行。这两条波束线,一条是为气相目标设计的——HR GHHG气体波束线,另一条是为冷凝相样品设计的——HR GHHG冷凝波束线,现在可以提供高通量的极紫外线(XUV)辐射,具有100 kHz重复率的泵探测能力。HR GHHG Cond光束线配备了一个时间补偿的XUV单色器,允许调整光谱特性,同时在飞秒状态下保持短,接近傅立叶限制的脉冲持续时间。尖端的实验终端站也可用,例如反应显微镜和纳米esca设备。两条光束线都已经过了首次用户试验。在本报告中,将介绍这两种独特的阿秒源的性能以及一些最新的发展和最新的实验。
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引用次数: 0
Instruments for best target position determination in the high-intensity laser-solid interaction experiment 高强度激光-固体相互作用实验中最佳目标位置确定仪器
Pub Date : 2023-06-08 DOI: 10.1117/12.2665527
E. Vishnyakov, A. Sagisaka, K. Ogura, T. Pikuz, C. Armstrong, S. Pikuz, B. González-Izquierdo, T. Esirkepov, Wenchao Yan, T. Jeong, Sushil Singh, P. Hadjisolomou, O. Finke, G. Grittani, M. Nevrkla, C. Lazzarini, A. Velyhan, T. Hayakawa, Y. Fukuda, J. Koga, M. Ishino, Kotaro Kondo, Y. Miyasaka, A. Kon, M. Nishikino, E. V. Nosach, D. Khikhlukha, I. Tsygvintsev, D. Kumar, J. Nejdl, D. Margarone, P. Sasorov, M. Kando, H. Kiriyama, G. Korn, K. Kondo, S. V. Bulanov, T. Kawachi, A. Pirozhkov
We review a number of instruments employed in a high-intensity J-KAREN-P laser-solid interaction experiment and discuss the applicability of the diagnostics to the best target position determination with a ~10 μm accuracy, while the focal spot size was ~1 μm and peak intensity was up to 7×1021 W/cm2. We discuss both front- and back-side diagnostics, some of them operated in the infrared, visible and ultraviolet ranges, while others in the extreme ultraviolet, soft X-ray and gamma-ray ranges. We found that the applicability of some of the instruments to the best at-focus target position determination depends on the thickness of the target.
对高强度J-KAREN-P激光-固体相互作用实验中使用的几种仪器进行了综述,讨论了该诊断方法在焦斑尺寸为~1 μm、峰强度可达7×1021 W/cm2时,最佳目标位置确定精度为~10 μm的适用性。我们讨论了前部和后部的诊断,其中一些在红外、可见光和紫外线范围内操作,而另一些在极紫外线、软x射线和伽马射线范围内操作。我们发现,一些仪器对最佳聚焦目标位置确定的适用性取决于目标的厚度。
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引用次数: 0
Towards high-sensitivity and low-dose medical imaging with laser x-ray sources 利用激光x射线源实现高灵敏度、低剂量医学成像
Pub Date : 2023-06-08 DOI: 10.1117/12.2664833
D. Stutman, N. Safca, P. Tomassini, E. Anghel, C. A. Ur
Phase contrast X-ray imaging can be much more sensitive to soft tissue lesions than conventional absorption contrast X-ray imaging, being a potential game changer for medical imaging. A phase contrast method well suited for clinical implementation is the grating interferometry. We show that by using μm period multi-meter long interferometers one can strongly increase the phase sensitivity and lower the dose towards soft tissue imaging applications such mammography. Conventional X-ray tubes do not provide, however, sufficient X-ray flux for clinical imaging with such long interferometers. Instead, 100-TW class lasers could produce highly directional and intense X-ray sources ideal for high sensitivity medical interferometry. We present the X-ray source characteristics required for clinical interferometry, advantages and disadvantages of betatron versus inverse Compton scattering sources for clinical application, and some practical considerations towards laser based interferometric medical imaging.
相衬x射线成像可以比传统的吸收对比x射线成像对软组织病变更敏感,是医学成像的潜在改变者。一种非常适合临床实施的相衬法是光栅干涉法。我们表明,通过使用μm周期的多米长干涉仪,可以大大提高相灵敏度,降低剂量,用于软组织成像应用,如乳房x光检查。然而,传统的x射线管不能提供足够的x射线通量,用于使用如此长的干涉仪进行临床成像。相反,100-TW级激光器可以产生高度定向和强烈的x射线源,非常适合高灵敏度医疗干涉测量。我们介绍了临床干涉测量所需的x射线源特性,betatron与逆康普顿散射源在临床应用中的优缺点,以及激光干涉医学成像的一些实际考虑。
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引用次数: 0
Five years operation experience with the AGIPD detectors at the European XFEL 在欧洲XFEL有5年AGIPD探测器的操作经验
Pub Date : 2023-06-08 DOI: 10.1117/12.2666402
I. Klačková, J. Sztuk-Dambietz, H. Graafsma, S. M. Hosseini-Saber, A. Klyuev, T. Laurus, O. Meyer, T. Preston, N. Raab, R. Shayduk, M. Sikorski, S. Stern, C. Strohm, U. Trunk, M. Turcato
The European X-ray Free Electron Laser (EuXFEL) began its user operation five years ago, opening and offering new research possibilities. The facility delivers high brilliance, ultra-short, spatially coherent x-ray pulses with a high repetition rate to six instruments (FXE, SPB/SFX, MID, HED, SCS and SQS) by means of three different beamlines (SASE 1, SASE 2 and SASE 3). One of the first detectors used for early-stage experiments was the Adaptive Gain Integrating Pixel Detector (AGIPD), custom designed to meet the challenging needs of scientific instruments. The AGIPD is a megahertz-rate integrating hybrid megapixel camera with a per-pixel adaptive gain amplification, allowing the integration of up to 104 of 12 keV photons per pixel in its low gain stage. Currently, three scientific instruments, namely SPB/SFX, MID and HED employ the AGIPD systems, the latter mentioned using a prototype, half-megapixel camera with an upgraded version of readout ASICs. The AGIPDs at EuXFEL are successfully used for experimental techniques like serial femtosecond crystallography, MHz single particle imaging, MHz x-ray photon correlation spectroscopy or MHz diffraction of materials under high pressures in a diamond anvil cell. Since September 2017, the AGIPD is continuously used and has become an established detector technology, with further advancements and developments planned. Delivering quality experimental data requires reliable and reproducible detector characterisation and calibration that have to be performed regularly with a continuous improvement of correction methods in close collaboration with scientific instruments. This work summarises five years of experience operating the AGIPD detectors at the EuXFEL scientific instruments. It gives an overview of scientific capabilities and examples of successful studies performed with AGIPD detectors. Moreover, challenges concerning detector calibration and characterisation are presented.
欧洲x射线自由电子激光器(EuXFEL)于五年前开始其用户操作,打开并提供了新的研究可能性。该设备通过三种不同的光束线(SASE 1、SASE 2和SASE 3)向六台仪器(FXE、SPB/SFX、MID、HED、SCS和SQS)提供高重复率的高亮度、超短、空间相干x射线脉冲。用于早期实验的首批探测器之一是自适应增益集成像素探测器(AGIPD),该探测器是为满足科学仪器的挑战性需求而定制的。AGIPD是一种兆赫速率集成混合百万像素相机,具有逐像素自适应增益放大功能,允许在其低增益阶段每像素集成多达104个12 keV光子。目前,三种科学仪器,即SPB/SFX, MID和HED采用AGIPD系统,后者使用原型,50万像素相机和升级版读出asic。EuXFEL的agipd已成功用于连续飞秒晶体学、MHz单粒子成像、MHz x射线光子相关光谱或钻石砧细胞高压下材料的MHz衍射等实验技术。自2017年9月以来,AGIPD一直在使用,并已成为一项既定的探测器技术,并计划进一步推进和发展。提供高质量的实验数据需要可靠和可重复的探测器特性和校准,必须定期执行,并与科学仪器密切合作,不断改进校正方法。这项工作总结了五年来在EuXFEL科学仪器上操作AGIPD探测器的经验。它给出了科学能力的概述和成功的研究与AGIPD探测器执行的例子。此外,还提出了探测器校准和表征方面的挑战。
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引用次数: 1
Bendable grating for monochromatization in the extreme-ultraviolet 可弯曲的极紫外单色光栅
Pub Date : 2023-06-08 DOI: 10.1117/12.2665625
Gabriele Zeni, F. Frassetto, A. Vanzo, S. Bonora, L. Poletto
Broadband light monochromatization in the extreme ultraviolet requires typically the use of diffraction gratings at grazing incidence, where the grating is rotated and eventually translated to perform the wavelength scanning. Several configurations have been proposed, using plane or concave gratings with uniform or variable line spacing. We propose here a low-cost experimental setup in which a thin plane diffraction grating is bended to an almost cylindrical shape to perform at the same time the spectral selection and the focalization of the selected spectral component. In such a way, the number of optical elements needed to realize the monochromator is reduced to two: the grating and the focusing mirror. A bendable grating has been tested in the 13-50 eV region, very good focal properties have been measured with very low residual aberrations. Furthermore, the shape of the bended surface has been measured using a wavefront sensor in order to confirm the effectiveness of the bending technique. The proposed solution can be used to achieve monochromatization both in large-scale facilities such as FELs or synchrotrons, but also in table-top setups, such as those exploiting high-order harmonic generation, that are often used for the preparatory phase of experiments to be later performed at FEL facilities.
在极紫外光下,宽带光单色化通常需要在掠入射处使用衍射光栅,其中光栅旋转并最终平移以执行波长扫描。提出了几种配置,使用均匀或可变线距的平面或凹光栅。本文提出了一种低成本的实验装置,该装置将薄平面衍射光栅弯曲成近乎圆柱形,同时进行光谱选择和所选光谱分量的聚焦。这样,实现单色器所需的光学元件的数量减少到两个:光栅和聚焦镜。在13-50 eV范围内对可弯曲光栅进行了测试,测量出了良好的焦性和极低的残余像差。此外,利用波前传感器测量了弯曲表面的形状,以证实弯曲技术的有效性。所提出的解决方案可用于在大型设施中实现单色化,例如在FEL或同步加速器中,也可用于桌面设置,例如那些利用高次谐波产生的设备,这些设备通常用于稍后在FEL设施中进行的实验的准备阶段。
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引用次数: 0
Spectroscopic real-time temperature diagnostic for laser-heated thin gold foils 激光加热薄金箔的光谱实时温度诊断
Pub Date : 2023-06-08 DOI: 10.1117/12.2665472
Veronika Kratzer, L. Geulig, Erin Grace Fitzpatrick, F. Lindner, Vitus Magin, Maximilian Julius Weiser, P. Thirolf
Target pre-heating has proven to be beneficial for laser-driven heavy-ion acceleration. As it allows to remove omnipresent carbohydrate surface contaminants, heating can affect the cutoff energy and increase the efficient acceleration of heavy ions as, e.g., required for the novel fission-fusion nuclear reaction scheme where kinetic energies of fissile species around 7 MeV/u are targeted. At the Centre for Advanced Laser Applications in Garching we use a 3W Nd:YAG cw laser to heat the (in our case gold) target foil in order to investigate the dependency of efficient gold ion acceleration on heating parameters. For real-time assessment of the surface temperature the thermal spectrum is measured with a NIR spectrometer to which Planck’s law is fitted.
目标预热已被证明是有利于激光驱动的重离子加速。由于加热可以去除无所不在的碳水化合物表面污染物,因此加热可以影响截止能量并增加重离子的有效加速,例如,在新的裂变-聚变核反应方案中,可裂变物质的动能在7 MeV/u左右。在Garching的先进激光应用中心,我们使用3W Nd:YAG连续激光器加热(在我们的案例中是金)目标箔,以研究有效金离子加速对加热参数的依赖性。为了实时评估表面温度,热谱是用一个贴合普朗克定律的近红外光谱仪测量的。
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引用次数: 0
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