To investigate the associations between particulate matter (PM) and hospital admissions for stroke and its subtypes among hypertension patients. We proposed a new modifier named high-concentration duration (HCD). Data on daily hospital admissions, air pollution, and meteorological factors were collected from 2014 to 2018 in Beijing, China. We included all patients with hypertension who were admitted to hospitals of secondary-level and above for stroke. Time-series analysis was conducted by fitting a generalized additive model. An interaction term of daily concentration and an HCD stratum indicator were included in the model. Sex subgroup analysis was performed in four age groups to detect vulnerable populations. A total of 358,577 admissions were identified. The PM was significantly associated with stroke admissions in patients with hypertension. The maximum excess risk (ER) (%) per 10 μg/m3 increase in fine particulate matter (PM2.5) was 0.23% (95% confidence interval (CI): 0.15%, 0.31%) for overall stroke, 0.25% (95% CI: 0.16%, 0.33%) for ischemic stroke (IS). The maximum ER (%) per 10 μg/m3 increase in inhalable particle (PM10) was 0.14% (95% CI: 0.06%, 0.23%) for overall stroke, 0.15% (95% CI: 0.06%, 0.23%) for IS. For hemorrhagic stroke, significant associations were also observed among males and patients < 55 years. ER (%) in long-HCD strata was significantly larger than that in short-HCD strata. The effects of PM2.5 were significant in long-HCD strata, but insignificant in short-HCD strata. HCD might be a modifier in the association between air pollution and health effects. While controlling the daily average concentration, it is also important to reduce HCD on a given day.
{"title":"Effect modification by high-concentration duration in the association between particulate matters and stroke hospital admissions among hypertension patients in Beijing, China","authors":"Zemeng Zhao, Moning Guo, Peng Tan, Xue Tian, Yuhan Zhao, Lulu Liu, Lili Luo, Hui Luo, Xiaonan Wang, Xiangtong Liu, Xiuhua Guo, Yanxia Luo","doi":"10.1007/s11869-023-01412-2","DOIUrl":"10.1007/s11869-023-01412-2","url":null,"abstract":"<div><p>To investigate the associations between particulate matter (PM) and hospital admissions for stroke and its subtypes among hypertension patients. We proposed a new modifier named high-concentration duration (HCD). Data on daily hospital admissions, air pollution, and meteorological factors were collected from 2014 to 2018 in Beijing, China. We included all patients with hypertension who were admitted to hospitals of secondary-level and above for stroke. Time-series analysis was conducted by fitting a generalized additive model. An interaction term of daily concentration and an HCD stratum indicator were included in the model. Sex subgroup analysis was performed in four age groups to detect vulnerable populations. A total of 358,577 admissions were identified. The PM was significantly associated with stroke admissions in patients with hypertension. The maximum excess risk (ER) (%) per 10 μg/m<sup>3</sup> increase in fine particulate matter (PM<sub>2.5</sub>) was 0.23% (95% confidence interval (CI): 0.15%, 0.31%) for overall stroke, 0.25% (95% CI: 0.16%, 0.33%) for ischemic stroke (IS). The maximum ER (%) per 10 μg/m<sup>3</sup> increase in inhalable particle (PM<sub>10</sub>) was 0.14% (95% CI: 0.06%, 0.23%) for overall stroke, 0.15% (95% CI: 0.06%, 0.23%) for IS. For hemorrhagic stroke, significant associations were also observed among males and patients < 55 years. ER (%) in long-HCD strata was significantly larger than that in short-HCD strata. The effects of PM<sub>2.5</sub> were significant in long-HCD strata, but insignificant in short-HCD strata. HCD might be a modifier in the association between air pollution and health effects. While controlling the daily average concentration, it is also important to reduce HCD on a given day.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-08-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"71909608","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-08-14DOI: 10.1007/s11869-023-01406-0
Peizhi Deng, Yan Li, Shenxin Li, Yuxin Feng, Donghui Jin, Yiping Yang, Yang Xie, Yao Lu, Qiuping Zhao, Hong Yuan
The evidence of non-optimum ambient temperature and humidity-related mortality is widely reported. However, the joint effects of high humidity and extreme temperatures on mortality remain to understand. We collected mortality data and meteorological variables for 91 counties in central China, from 2017 to 2020. A traditional time-series model with a distributed lag non-linear model was first employed to estimate the location-specific associations between extreme temperatures or high humidity and extreme temperatures and mortality. Then, we conducted a meta-analysis to pool the county-specific estimated effect values. A total of 1,196,916 non-accidental deaths occurred during the study period. Extreme heat increased non-accidental mortality with a relative risk (RR) of 1.071 ((95% confidence interval (CI):1.022, 1.121), while extreme cold worsened the risk of stroke mortality by 2.817 (95 CI%: 1.084, 7.321). For the effect of extreme cold, high humidity increased the RR of 3.908 (95 CI%: 2.721, 5.612) in non-accidental mortality and the effect was strongest in stroke with 5.320 (95 CI%: 3.395 vs 8.338). Under the joint effect of extreme cold and high humidity, there is a lagged association with the mortality risks peaked at 12d for non-accidental mortality. High humidity significantly enhances the risk of extreme cold-related non-accidental mortality, especially regarding stroke. Our findings will assist in the development of preparedness and prevention strategies in Hunan Province and even throughout China to reduce the immediate weather-related impacts.
{"title":"The role of high humidity on extreme-temperature-related mortality in central China","authors":"Peizhi Deng, Yan Li, Shenxin Li, Yuxin Feng, Donghui Jin, Yiping Yang, Yang Xie, Yao Lu, Qiuping Zhao, Hong Yuan","doi":"10.1007/s11869-023-01406-0","DOIUrl":"10.1007/s11869-023-01406-0","url":null,"abstract":"<div><p>The evidence of non-optimum ambient temperature and humidity-related mortality is widely reported. However, the joint effects of high humidity and extreme temperatures on mortality remain to understand. We collected mortality data and meteorological variables for 91 counties in central China, from 2017 to 2020. A traditional time-series model with a distributed lag non-linear model was first employed to estimate the location-specific associations between extreme temperatures or high humidity and extreme temperatures and mortality. Then, we conducted a meta-analysis to pool the county-specific estimated effect values. A total of 1,196,916 non-accidental deaths occurred during the study period. Extreme heat increased non-accidental mortality with a relative risk (RR) of 1.071 ((95% confidence interval (CI):1.022, 1.121), while extreme cold worsened the risk of stroke mortality by 2.817 (95 CI%: 1.084, 7.321). For the effect of extreme cold, high humidity increased the RR of 3.908 (95 CI%: 2.721, 5.612) in non-accidental mortality and the effect was strongest in stroke with 5.320 (95 CI%: 3.395 vs 8.338). Under the joint effect of extreme cold and high humidity, there is a lagged association with the mortality risks peaked at 12d for non-accidental mortality. High humidity significantly enhances the risk of extreme cold-related non-accidental mortality, especially regarding stroke. Our findings will assist in the development of preparedness and prevention strategies in Hunan Province and even throughout China to reduce the immediate weather-related impacts.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-08-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"71909443","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Extremely low frequency oscillating magnetic field (OMF-ELF) can stimulate the growth of pathogenic fungi. This work aims to assess the tropic response of a dimorphic pathogenic strain Candida guilliermondii by the effect of OMF-ELF. The pathogenic strain C. guilliermondii was isolated from an indoor environment and a brewing strain Saccharomyces cerevisiae was used as a positive control. OMF-ELF of 3 mT of 60 Hz for 2 h was applied to the cultures of both strains. After treatment, images were taken every 30 min for 24 h using Digital Image Processing (DIP) to determine the superficial growth rate of both strains and the length of the pseudohyphae, and the tropic response of C. guilliermondii. However, C. guilliermondii showed a tropic response depending on the OMF-ELF applied growing 3 to 60 times faster than the control strain, with a maximum value of 1.27 μm2/min between 1.5 and 2.5 h. C. guillermondii is resistant to OMF-ELF, a factor that stimulated its superficial growth rate and the elongation of its pseudohyphae, facilitated its cellular dimorphism, and oriented its ramifications to increase reproduction. This increase constitutes a risk to human health indoor environments where there is microbiological and electromagnetic contamination. Due to the use of DIP in real time with an adapted microculture technique, this is the first study to analyze “in vivo” magnetotropism of C. guilliermondii, as indicative of its invasive behavior for a possible infestation to humans exposed to this type of non-ionizing radiation in an indoor environment.
{"title":"Magnetotropism: a tropic response of Candida guillemondii by the effect of the oscillating magnetic field of extremely low frequency","authors":"Matilde Anaya, Erasmo Gámez-Espinosa, Sofía Borrego, Eduardo Barbará","doi":"10.1007/s11869-023-01408-y","DOIUrl":"10.1007/s11869-023-01408-y","url":null,"abstract":"<div><p>Extremely low frequency oscillating magnetic field (OMF-ELF) can stimulate the growth of pathogenic fungi. This work aims to assess the tropic response of a dimorphic pathogenic strain <i>Candida guilliermondii</i> by the effect of OMF-ELF. The pathogenic strain <i>C. guilliermondii</i> was isolated from an indoor environment and a brewing strain <i>Saccharomyces cerevisiae</i> was used as a positive control. OMF-ELF of 3 mT of 60 Hz for 2 h was applied to the cultures of both strains. After treatment, images were taken every 30 min for 24 h using Digital Image Processing (DIP) to determine the superficial growth rate of both strains and the length of the pseudohyphae, and the tropic response of <i>C. guilliermondii</i>. However, <i>C. guilliermondii</i> showed a tropic response depending on the OMF-ELF applied growing 3 to 60 times faster than the control strain, with a maximum value of 1.27 μm<sup>2</sup>/min between 1.5 and 2.5 h. <i>C. guillermondii</i> is resistant to OMF-ELF, a factor that stimulated its superficial growth rate and the elongation of its pseudohyphae, facilitated its cellular dimorphism, and oriented its ramifications to increase reproduction. This increase constitutes a risk to human health indoor environments where there is microbiological and electromagnetic contamination. Due to the use of DIP in real time with an adapted microculture technique, this is the first study to analyze “in vivo” magnetotropism of <i>C. guilliermondii</i>, as indicative of its invasive behavior for a possible infestation to humans exposed to this type of non-ionizing radiation in an indoor environment.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-08-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"79437852","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
The dithiothreitol (DTT) assay was used to investigate the oxidative potential (OP) of atmospheric fine particles (PM2.5) during fireworks (Diwali) at Agra, India. The 12-h mean PM2.5 was reported to be 263 ±151 μg m−3 during the study period. Increased levels of gaseous pollutants (NOx, SO2, CO, and O3) and metals Ba, Pb, Cu, Fe, Mg, K, Al, and Mn were also observed during fireworks. The results showed that the typical diurnal pattern of trace gases was observed, except their overall concentrations remained elevated during peak hours of the fireworks activity. The highest value of OP of PM was detected on the next morning of Diwali, with a volume-based DTT value (OPv) of 1.4 nmol min−1 m−3 and a mass-based DTT value (OPm) of 11.8 pmol min−1 μg−1, implying higher PM-related DTT activity due to fireworks. A positive association was found between redox-active metals like Cr, Cu, Ni, and V and DTT activity which could be due to the ability of these metals to catalyze reactive oxygen species (ROS) generation in ambient air. Ba and Se concentrations in the particulate matter, which are key components of firecrackers, were likewise highly linked to DTT activity. During the daytime, ozone levels were strongly correlated (r2 = 0.9) with OPv activity; this may be due to photochemical processes which may lead to the formation of tropospheric O3. Elements C, O, Al, Si, S, K, and Ba were found to be the most prevalent in elemental mappings, which suggests that fireworks may have contributed to their abundance. A comparison of the daily OPv activity and hazard index (HI) suggests that the HI may be a poor metric for measuring the health impacts of PM exposure on human health.
{"title":"Dynamic changes in the characteristics of fine particles and their oxidative potential in the city of Taj (Agra, India): the untold story of fireworks display","authors":"Isha Goyal, Puneet Kumar Verma, Kandikonda Maharaj Kumari, Anita Lakhani","doi":"10.1007/s11869-023-01402-4","DOIUrl":"10.1007/s11869-023-01402-4","url":null,"abstract":"<p>The dithiothreitol (DTT) assay was used to investigate the oxidative potential (OP) of atmospheric fine particles (PM<sub>2.5</sub>) during fireworks (Diwali) at Agra, India. The 12-h mean PM<sub>2.5</sub> was reported to be 263 ±151 μg m<sup>−3</sup> during the study period. Increased levels of gaseous pollutants (NOx, SO<sub>2</sub>, CO, and O<sub>3</sub>) and metals Ba, Pb, Cu, Fe, Mg, K, Al, and Mn were also observed during fireworks. The results showed that the typical diurnal pattern of trace gases was observed, except their overall concentrations remained elevated during peak hours of the fireworks activity. The highest value of OP of PM was detected on the next morning of Diwali, with a volume-based DTT value (OPv) of 1.4 nmol min<sup>−1</sup> m<sup>−3</sup> and a mass-based DTT value (OPm) of 11.8 pmol min<sup>−1</sup> μg<sup>−1</sup>, implying higher PM-related DTT activity due to fireworks. A positive association was found between redox-active metals like Cr, Cu, Ni, and V and DTT activity which could be due to the ability of these metals to catalyze reactive oxygen species (ROS) generation in ambient air. Ba and Se concentrations in the particulate matter, which are key components of firecrackers, were likewise highly linked to DTT activity. During the daytime, ozone levels were strongly correlated (<i>r</i><sup>2</sup> = 0.9) with OPv activity; this may be due to photochemical processes which may lead to the formation of tropospheric O<sub>3</sub>. Elements C, O, Al, Si, S, K, and Ba were found to be the most prevalent in elemental mappings, which suggests that fireworks may have contributed to their abundance. A comparison of the daily OPv activity and hazard index (HI) suggests that the HI may be a poor metric for measuring the health impacts of PM exposure on human health.</p>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-08-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"71909623","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-08-10DOI: 10.1007/s11869-023-01401-5
Selin Yıldırım, Ebru Koçak
Polycyclic aromatic hydrocarbons (PAHs) were measured in size-segregated particulate matters (PMs) in a range of 0.43 to 10.0 μm, categorized into two as fine particles (0.43 μm < d < 2.1 μm) and coarse particles (2.1 μm < d < 10.0 μm), during summer and winter seasons in an urban atmosphere of Aksaray, Turkey. The primary purpose of this study was to investigate size distribution, temporal variation, and related health risks of PAHs. During the winter season, concentrations of PAHs in the sampling site were almost ten times higher than in summer, and approximately 85% of the PAHs belonged to the fine PM fraction. On the other hand, it was determined that the emission sources of the detected PAHs in the summer season were traffic-related emissions. The smallest particle size range (0.45–0.63 μm) consisted of the maximum PAH concentration (1.22±0.05 ng m−3) about other particle sizes during the summer season. Fluoranthene (Flt) was the main PAH species determined during winter, indicating that coal combustion is a dominant pollution source. The size distribution properties of PAHs showed similar characteristics for coarse particles, which was also the case for fine particles. In addition, as the ring number of PAHs increases, the height of the peaks decreases in the size distribution plots of coarse particles. Higher molecular weight (HMW) PAHs show higher carcinogenicity potential, mainly found in the fine PM fraction. A health risk assessment was estimated by toxicity equivalent quantity (TEQ) and inhalation cancer risk (ICR), indicating medium risk for the fine PMs and low risk for the coarse PMs.
在土耳其阿克萨雷的夏季和冬季,在城市大气中测量了尺寸分离的颗粒物(PM)中的多环芳烃(PAHs),颗粒物范围为0.43至10.0μm,分为细颗粒物(0.43μm<;d<;2.1μm)和粗颗粒物(2.1μm<;d<;10.0μm)。本研究的主要目的是调查多环芳烃的大小分布、时间变化和相关的健康风险。在冬季,采样点的多环芳烃浓度几乎是夏季的十倍,大约85%的多环芳烃属于细颗粒物。另一方面,确定夏季检测到的多环芳烃的排放源是与交通有关的排放。最小粒径范围(0.45–0.63μm)由夏季其他粒径的最大PAH浓度(1.22±0.05 ng m−3)组成。荧蒽(Flt)是冬季测定的主要PAH物种,表明燃煤是主要污染源。PAHs的尺寸分布特性在粗颗粒中表现出类似的特征,细颗粒也是如此。此外,随着多环芳烃环数的增加,粗颗粒尺寸分布图中峰的高度减小。高分子量PAHs表现出更高的致癌性潜力,主要存在于细颗粒物中。健康风险评估通过毒性当量(TEQ)和吸入癌症风险(ICR)进行估计,表明细PM的中等风险和粗PM的低风险。
{"title":"Measurement of size-segregated airborne particulate bound polycyclic aromatic hydrocarbons and health risk assessment: a case study in Aksaray atmosphere, Turkey","authors":"Selin Yıldırım, Ebru Koçak","doi":"10.1007/s11869-023-01401-5","DOIUrl":"10.1007/s11869-023-01401-5","url":null,"abstract":"<div><p>Polycyclic aromatic hydrocarbons (PAHs) were measured in size-segregated particulate matters (PMs) in a range of 0.43 to 10.0 μm, categorized into two as fine particles (0.43 μm < <i>d</i> < 2.1 μm) and coarse particles (2.1 μm < <i>d</i> < 10.0 μm), during summer and winter seasons in an urban atmosphere of Aksaray, Turkey. The primary purpose of this study was to investigate size distribution, temporal variation, and related health risks of PAHs. During the winter season, concentrations of PAHs in the sampling site were almost ten times higher than in summer, and approximately 85% of the PAHs belonged to the fine PM fraction. On the other hand, it was determined that the emission sources of the detected PAHs in the summer season were traffic-related emissions. The smallest particle size range (0.45–0.63 μm) consisted of the maximum PAH concentration (1.22±0.05 ng m<sup>−3</sup>) about other particle sizes during the summer season. Fluoranthene (Flt) was the main PAH species determined during winter, indicating that coal combustion is a dominant pollution source. The size distribution properties of PAHs showed similar characteristics for coarse particles, which was also the case for fine particles. In addition, as the ring number of PAHs increases, the height of the peaks decreases in the size distribution plots of coarse particles. Higher molecular weight (HMW) PAHs show higher carcinogenicity potential, mainly found in the fine PM fraction. A health risk assessment was estimated by toxicity equivalent quantity (TEQ) and inhalation cancer risk (ICR), indicating medium risk for the fine PMs and low risk for the coarse PMs.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-08-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"71909488","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-08-08DOI: 10.1007/s11869-023-01404-2
Yougeng Lu
Due to a paucity of human movement data, the traditional method for estimating pollution exposure is static: Exposure is based on place of residence. However, local air quality varies over both time and space. This study explores exposure measurement errors associated with ignoring human mobility and its impact on exposure-health effect estimates. Using a random forest classification model, this study examines the impact of a variety of factors on potential measurement errors in personal exposure to outdoor PM2.5. Mobility data at the individual level was combined with hourly PM2.5 surfaces at the neighborhood level to estimate and compare residence-based and mobility-based exposures for 100,784 Los Angeles County residents. The results show that exposure measurement errors increase for individuals with high mobility levels. Significant sociodemographic disparities are observed across different exposure classification groups. Exposures of low-income people who have high mobility and reside in polluted neighborhoods tend to be overestimated. In contrast, exposures of high-income people living in neighborhoods with cleaner air are likely to be underestimated. The result on the exposure-health effect suggests that health risks of the socially disadvantaged after exposure to PM2.5 is likely to be underestimated due to the exposure measurement error introduced by ignoring human mobility.
{"title":"Assessing air pollution exposure misclassification using high-resolution PM2.5 concentration model and human mobility data","authors":"Yougeng Lu","doi":"10.1007/s11869-023-01404-2","DOIUrl":"10.1007/s11869-023-01404-2","url":null,"abstract":"<div><p>Due to a paucity of human movement data, the traditional method for estimating pollution exposure is static: Exposure is based on place of residence. However, local air quality varies over both time and space. This study explores exposure measurement errors associated with ignoring human mobility and its impact on exposure-health effect estimates. Using a random forest classification model, this study examines the impact of a variety of factors on potential measurement errors in personal exposure to outdoor PM<sub>2.5</sub>. Mobility data at the individual level was combined with hourly PM<sub>2.5</sub> surfaces at the neighborhood level to estimate and compare residence-based and mobility-based exposures for 100,784 Los Angeles County residents. The results show that exposure measurement errors increase for individuals with high mobility levels. Significant sociodemographic disparities are observed across different exposure classification groups. Exposures of low-income people who have high mobility and reside in polluted neighborhoods tend to be overestimated. In contrast, exposures of high-income people living in neighborhoods with cleaner air are likely to be underestimated. The result on the exposure-health effect suggests that health risks of the socially disadvantaged after exposure to PM<sub>2.5</sub> is likely to be underestimated due to the exposure measurement error introduced by ignoring human mobility.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-08-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"71909567","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-08-08DOI: 10.1007/s11869-023-01403-3
Dietmar Oettl, Raphael Reifeltshammer
The rather complex terrain in Austria requires that wind fields with sub-kilometer resolutions have to be generated prior to any kind of dispersion modeling due to the large demand on computation times required by non-hydrostatic prognostic mesoscale models. Proper modeling of highly resolved flows in Alpine regions is still a matter of research, and no harmonized methodology is available at the moment. In order to harmonize the meteorological input for dispersion modeling at the regional level, authorities in Austria aim at providing so-called wind-field libraries for a certain reference year for all stakeholders involved in air quality assessments for regulatory purposes. The region of Styria was the first to establish such a library using the prognostic, non-hydrostatic mesoscale model GRAMM with a horizontal resolution of 300 m in 2015. Over the years, attempts have been made for improving the quality of the wind fields. One of the most challenging issues is the interaction between synoptic-scale flows and local thermally driven winds. In this work, the newly developed mesoscale model GRAMM-SCI is presented, which is driven by ERA5 reanalysis data. Especially, novel nudging techniques allow for nesting and dynamic downscaling wind fields with a horizontal resolution of 100–200 m. Moreover, a methodology called “match-to-observation” (MTO) is presented, which greatly improves the final quality of wind fields. For the first time, a wind-field library for the reference year 2017 has been generated for Styria with this new approach.
{"title":"Recent developments in high-resolution wind field modeling in complex terrain for dispersion simulations using GRAMM-SCI","authors":"Dietmar Oettl, Raphael Reifeltshammer","doi":"10.1007/s11869-023-01403-3","DOIUrl":"10.1007/s11869-023-01403-3","url":null,"abstract":"<div><p>The rather complex terrain in Austria requires that wind fields with sub-kilometer resolutions have to be generated prior to any kind of dispersion modeling due to the large demand on computation times required by non-hydrostatic prognostic mesoscale models. Proper modeling of highly resolved flows in Alpine regions is still a matter of research, and no harmonized methodology is available at the moment. In order to harmonize the meteorological input for dispersion modeling at the regional level, authorities in Austria aim at providing so-called wind-field libraries for a certain reference year for all stakeholders involved in air quality assessments for regulatory purposes. The region of Styria was the first to establish such a library using the prognostic, non-hydrostatic mesoscale model GRAMM with a horizontal resolution of 300 m in 2015. Over the years, attempts have been made for improving the quality of the wind fields. One of the most challenging issues is the interaction between synoptic-scale flows and local thermally driven winds. In this work, the newly developed mesoscale model GRAMM-SCI is presented, which is driven by ERA5 reanalysis data. Especially, novel nudging techniques allow for nesting and dynamic downscaling wind fields with a horizontal resolution of 100–200 m. Moreover, a methodology called “match-to-observation” (MTO) is presented, which greatly improves the final quality of wind fields. For the first time, a wind-field library for the reference year 2017 has been generated for Styria with this new approach.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-08-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"71909513","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-08-08DOI: 10.1007/s11869-023-01405-1
Yago Alonso Cipoli, Leonardo Furst, Manuel Feliciano, Célia Alves
Inhalation of particulate matter (PM) has been extensively associated with the worsening and onset of cardiorespiratory diseases, being responsible for millions of deaths annually. Assessment of PM deposition in the human respiratory tract is critical to better understand the health risks from environmental exposure of vulnerable age groups. In this study, PM2.5 and PM10 day-night monitoring campaigns during the cold season were carried out in Bragança, Portugal. The multiple-path particle dosimetry (MPPD) model was used to quantify total and regional depositions in the human respiratory tract for four different age groups: infant (3 months), child (9 years), adult (21 years) and elderly (65 years). The results showed that concentrations for both PM fractions were higher during the night, a period marked by the burning of biomass for residential heating. Regional deposition fractions (DF) for PM2.5 were in the ranges 17–38% (head), 4–14% (tracheobronchial) and 20–28% (pulmonary), while for PM10 were 24–67% (head), 4–27% (tracheobronchial) and 12–22% (pulmonary). Children and the elderly were found to be the most vulnerable groups to PM deposition, especially for the TB and H regions, respectively. The lifetime cancer and non-cancer risks associated with exposure to PM2.5 exceeded the recommended limits, especially for children <10 years old. These findings provide useful information to alert authorities to the need to take action to reduce the pollution burden and protect the health, in particular of those most susceptible.
{"title":"Respiratory deposition dose of PM2.5 and PM10 during night and day periods at an urban environment","authors":"Yago Alonso Cipoli, Leonardo Furst, Manuel Feliciano, Célia Alves","doi":"10.1007/s11869-023-01405-1","DOIUrl":"10.1007/s11869-023-01405-1","url":null,"abstract":"<p>Inhalation of particulate matter (PM) has been extensively associated with the worsening and onset of cardiorespiratory diseases, being responsible for millions of deaths annually. Assessment of PM deposition in the human respiratory tract is critical to better understand the health risks from environmental exposure of vulnerable age groups. In this study, PM<sub>2.5</sub> and PM<sub>10</sub> day-night monitoring campaigns during the cold season were carried out in Bragança, Portugal. The multiple-path particle dosimetry (MPPD) model was used to quantify total and regional depositions in the human respiratory tract for four different age groups: infant (3 months), child (9 years), adult (21 years) and elderly (65 years). The results showed that concentrations for both PM fractions were higher during the night, a period marked by the burning of biomass for residential heating. Regional deposition fractions (DF) for PM<sub>2.5</sub> were in the ranges 17–38% (head), 4–14% (tracheobronchial) and 20–28% (pulmonary), while for PM<sub>10</sub> were 24–67% (head), 4–27% (tracheobronchial) and 12–22% (pulmonary). Children and the elderly were found to be the most vulnerable groups to PM deposition, especially for the TB and H regions, respectively. The lifetime cancer and non-cancer risks associated with exposure to PM<sub>2.5</sub> exceeded the recommended limits, especially for children <10 years old. These findings provide useful information to alert authorities to the need to take action to reduce the pollution burden and protect the health, in particular of those most susceptible.</p>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-08-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"71909566","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-08-07DOI: 10.1007/s11869-023-01394-1
Nomathemba Themba, Linda L. Sibali, Tlou B. Chokwe
Polychlorinated dibenzo-p-dioxins and dibenzo-furans (PCDD/Fs) are notorious pollutants classified as persistent organic pollutants (POPs), which even at trace levels can bio-accumulate in the environment and have negative effects on organisms. Due to their adverse health effects, countries around the globe have introduced stringent emission standards to reduce the formation of PCDD/Fs. Using data in the literature over the past two decades (2001 to 2023), this review discussed the PCDD/F emissions from incineration facilities, E-waste recycling, iron sintering, secondary metal smelting plants, and crematories. But the review only focused on pollutants and remediation strategies from the incineration processes. There are two heterogeneous mechanism pathways that lead to the formation of PCDD/Fs, firstly, the De novo phase, using macromolecules of carbon or polycyclic aromatic hydrocarbons to begin the synthesis, and secondly, the condensation reaction beginning with the rearrangement of the molecular structure of the precursor compound. On the remediation strategies, adsorption injections were the most preferred method; however, recent studies reported other strategies such as catalytic filtration systems, an electron beam system, and good combustion practices. This review concluded that a lot has been done to manage and prevent PCDD/F formation efficiently to the level which no longer poses a hazard to human health and the environment.
{"title":"A review on the formation and remediations of polychlorinated dibenzo p-dioxins and dibenzo-furans (PCDD/Fs) during thermal processes with a focus on MSW process","authors":"Nomathemba Themba, Linda L. Sibali, Tlou B. Chokwe","doi":"10.1007/s11869-023-01394-1","DOIUrl":"10.1007/s11869-023-01394-1","url":null,"abstract":"<p>Polychlorinated dibenzo-<i>p</i>-dioxins and dibenzo-furans (PCDD/Fs) are notorious pollutants classified as persistent organic pollutants (POPs), which even at trace levels can bio-accumulate in the environment and have negative effects on organisms. Due to their adverse health effects, countries around the globe have introduced stringent emission standards to reduce the formation of PCDD/Fs. Using data in the literature over the past two decades (2001 to 2023), this review discussed the PCDD/F emissions from incineration facilities, E-waste recycling, iron sintering, secondary metal smelting plants, and crematories. But the review only focused on pollutants and remediation strategies from the incineration processes. There are two heterogeneous mechanism pathways that lead to the formation of PCDD/Fs, firstly, the De novo phase, using macromolecules of carbon or polycyclic aromatic hydrocarbons to begin the synthesis, and secondly, the condensation reaction beginning with the rearrangement of the molecular structure of the precursor compound. On the remediation strategies, adsorption injections were the most preferred method; however, recent studies reported other strategies such as catalytic filtration systems, an electron beam system, and good combustion practices. This review concluded that a lot has been done to manage and prevent PCDD/F formation efficiently to the level which no longer poses a hazard to human health and the environment.</p>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-08-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s11869-023-01394-1.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50458048","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-08-07DOI: 10.1007/s11869-023-01400-6
Fatma Esen, Daniel Alejandro Cordova Del Aguila, Mehmet Ferhat Sari
The study of persistent organic pollutants (POPs) in different environments has helped to understand the behavior and distribution of these pollutants worldwide. Many developed and developing countries have extensive data on the presence of these pollutants, especially in ambient air and soil. However, the simultaneous measurement of air and soil is less frequent, despite offering the opportunity to characterize air-soil exchange. Moreover, such measurements in upper-middle-income countries such as Turkey are very limited and null in Peru. Both countries also offer unique opportunities to characterize the air-soil exchange since Peru has a semi-arid subtropical desert climate and Turkey has a Mediterranean climate. Therefore, the aim of this study is to determine the simultaneous POP concentrations (polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), and organochlorine pesticides (OCPs)) in ambient air and soil in Turkey and Peru and to reveal the POP exchange between air and soil and flux amounts in the gas phase. POP concentrations in ambient air were measured higher at sampling points in Turkey, while POPs in soil were measured similarly in both countries. Also, the air-soil fugacity fractions indicated net volatilization for low molecular weight PAH and PCB congeners, but net deposition for high molecular weight congeners; equilibrium states were found for medium molecular weight congeners. Fugacity fractions did not change with their molecular weights for OCPs. It has been determined that soil acts as a “secondary source” for low molecular weight PAH and PBC congeners in the atmosphere, while the atmosphere acts as a “sink” for high molecular weight PAH and PCB congeners in the soil. Finally, cancer risk calculations for adults and children have been made, both via inhalation of atmospheric POPs and uptake of POPs from the soil. According to the calculations, no health risks were found for both air and soil for adults and children.
{"title":"Air and soil concentrations of persistent organic pollutants in Bursa (Türkiye) and Yurimaguas (Peru): air-soil exchange and gas-phase flux","authors":"Fatma Esen, Daniel Alejandro Cordova Del Aguila, Mehmet Ferhat Sari","doi":"10.1007/s11869-023-01400-6","DOIUrl":"10.1007/s11869-023-01400-6","url":null,"abstract":"<div><p>The study of persistent organic pollutants (POPs) in different environments has helped to understand the behavior and distribution of these pollutants worldwide. Many developed and developing countries have extensive data on the presence of these pollutants, especially in ambient air and soil. However, the simultaneous measurement of air and soil is less frequent, despite offering the opportunity to characterize air-soil exchange. Moreover, such measurements in upper-middle-income countries such as Turkey are very limited and null in Peru. Both countries also offer unique opportunities to characterize the air-soil exchange since Peru has a semi-arid subtropical desert climate and Turkey has a Mediterranean climate. Therefore, the aim of this study is to determine the simultaneous POP concentrations (polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), and organochlorine pesticides (OCPs)) in ambient air and soil in Turkey and Peru and to reveal the POP exchange between air and soil and flux amounts in the gas phase. POP concentrations in ambient air were measured higher at sampling points in Turkey, while POPs in soil were measured similarly in both countries. Also, the air-soil fugacity fractions indicated net volatilization for low molecular weight PAH and PCB congeners, but net deposition for high molecular weight congeners; equilibrium states were found for medium molecular weight congeners. Fugacity fractions did not change with their molecular weights for OCPs. It has been determined that soil acts as a “secondary source” for low molecular weight PAH and PBC congeners in the atmosphere, while the atmosphere acts as a “sink” for high molecular weight PAH and PCB congeners in the soil. Finally, cancer risk calculations for adults and children have been made, both via inhalation of atmospheric POPs and uptake of POPs from the soil. According to the calculations, no health risks were found for both air and soil for adults and children.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-08-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"71909007","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}