Pub Date : 2023-07-08DOI: 10.1007/s11869-023-01390-5
Ashfaq Ahmad, Muhammad Mobeen Shafqat, Muhammad Ilyas, Muhammad Umair Ashraf, Afshan Urooj, Zhao Yu huan
This research investigates the validation of the environment Kuznets curve (EKC) at aggregate and sectoral levels for the Indian economy both. The study covers the period 1970–2020. The stationarity of the variables was also confirmed by some traditional unit root tests, and structural breaks were also determined by the Zivot-Andrews test. The autoregression distributive lag model (ARDL) bound test is deployed to observe the cointegration between variables with different structural breaks. Additionally, we investigate short-run, long-run, and combined causal relations among the variables by employing the vector error correction model (VECM) test. The results validate the presence of EKC not only at the aggregate level but also at the sectoral level. Moreover, energy consumption increases CO2 emissions, while economic globalization reduces CO2 emissions. The findings reveal that economic globalization is beneficial to environmental quality, while energy consumption hampers it in India. As a result of these findings, policymakers in India should include economic globalization as an essential element in the carbon emissions function while designing an enhanced economic policy framework that leads to low carbon-driven, sustainable, and inclusive economic growth at the aggregate and disaggregated levels.
{"title":"Validation of the environmental Kuznets curve and role of economic globalization: an aggregate and sectoral analysis of an Indian economy","authors":"Ashfaq Ahmad, Muhammad Mobeen Shafqat, Muhammad Ilyas, Muhammad Umair Ashraf, Afshan Urooj, Zhao Yu huan","doi":"10.1007/s11869-023-01390-5","DOIUrl":"10.1007/s11869-023-01390-5","url":null,"abstract":"<div><p>This research investigates the validation of the environment Kuznets curve (EKC) at aggregate and sectoral levels for the Indian economy both. The study covers the period 1970–2020. The stationarity of the variables was also confirmed by some traditional unit root tests, and structural breaks were also determined by the Zivot-Andrews test. The autoregression distributive lag model (ARDL) bound test is deployed to observe the cointegration between variables with different structural breaks. Additionally, we investigate short-run, long-run, and combined causal relations among the variables by employing the vector error correction model (VECM) test. The results validate the presence of EKC not only at the aggregate level but also at the sectoral level. Moreover, energy consumption increases CO<sub>2</sub> emissions, while economic globalization reduces CO<sub>2</sub> emissions. The findings reveal that economic globalization is beneficial to environmental quality, while energy consumption hampers it in India. As a result of these findings, policymakers in India should include economic globalization as an essential element in the carbon emissions function while designing an enhanced economic policy framework that leads to low carbon-driven, sustainable, and inclusive economic growth at the aggregate and disaggregated levels.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-07-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s11869-023-01390-5.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50463201","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-07-07DOI: 10.1007/s11869-023-01354-9
Loghman Fathollahi, Falin Wu, Reza Maleki, Barbara Pongracic
The harmful effects of ambient air pollution on human health have been consistently documented by many epidemiological studies around the world, and it is estimated that at least seven million deaths worldwide each year are caused by the effects of air pollution. Harmful airborne particles are identified by the Particulate Matter (PM) parameter, which is a term that used for solid and liquid particles in varying size, shape, composition and with different sources, suspended in the air. The aim of this study is to build (PM_{2.5}) concentrations estimation model with meteorological data such as PBLH, and a combination of two AOD’s data retrieved from MODIS satellite (MAIAC - MODIS AOD product) using machine learning methods. The study area is in the Western part of Iran, where dust storms as one of the most important sources of air pollutants increasing sharply in recent decades, and this increase has caused numerous health and environmental problems. The data period is four years from 1 January 2018 to 31 December 2021, and three machine learning methods, LightGBM, MLP, and Random Forest algorithms were used. For the three typical machine learning methods, the RF model presents the best result by obtaining the lowest RMSE (30.1 (mu g/m^{3})) and MAE (25.0 (mu g/m^{3})) values in combination with the highest (R^{2}) (0.64) value for daily predictions.
{"title":"(PM_{2.5}) concentrations estimation using machine learning methods with combination of MAIAC - MODIS AOD product - a case study in western Iran","authors":"Loghman Fathollahi, Falin Wu, Reza Maleki, Barbara Pongracic","doi":"10.1007/s11869-023-01354-9","DOIUrl":"10.1007/s11869-023-01354-9","url":null,"abstract":"<div><p>The harmful effects of ambient air pollution on human health have been consistently documented by many epidemiological studies around the world, and it is estimated that at least seven million deaths worldwide each year are caused by the effects of air pollution. Harmful airborne particles are identified by the Particulate Matter (PM) parameter, which is a term that used for solid and liquid particles in varying size, shape, composition and with different sources, suspended in the air. The aim of this study is to build <span>(PM_{2.5})</span> concentrations estimation model with meteorological data such as PBLH, and a combination of two AOD’s data retrieved from MODIS satellite (MAIAC - MODIS AOD product) using machine learning methods. The study area is in the Western part of Iran, where dust storms as one of the most important sources of air pollutants increasing sharply in recent decades, and this increase has caused numerous health and environmental problems. The data period is four years from 1 January 2018 to 31 December 2021, and three machine learning methods, LightGBM, MLP, and Random Forest algorithms were used. For the three typical machine learning methods, the RF model presents the best result by obtaining the lowest RMSE (30.1 <span>(mu g/m^{3})</span>) and MAE (25.0 <span>(mu g/m^{3})</span>) values in combination with the highest <span>(R^{2})</span> (0.64) value for daily predictions.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-07-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50459536","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
To investigate the atmospheric pollutant emission from residential coal combustion (RCC) in BTH region in 2020, based on the bottom-up methodology, a high spatial and temporal resolution air pollutant emission inventory was established. The results showed that the emissions of PM10, PM2.5, BC, OC, CO, NOx, SO2, and VOCs in BTH region in 2020 were 19.58, 15.67, 2.98, 8.33, 296.96, 3.51, 36.67, and 5.87 million tons, respectively. Chengde contributed the most PM2.5, BC, OC, and VOCs in BTH region, accounted for 11.48%, 13.71%, 11.52%, and 12.72%, respectively. While Shijiazhuang contributed the most PM10, CO, NOx, and SO2 in BTH region, accounted for 11.55%, 11.60%, 11.55%, and 12.10%, respectively. The spatial distribution characteristics of pollutants showed that high emissions concentrated in northern, eastern, and southern areas of BTH region. Based on the time distribution factor obtained from the long-term follow-up survey data of RCC of households in BTH region, the annual emissions of different cities were allocated according to the temporal resolution of monthly, daily, and hourly. It was found that for each pollutant, the highest emissions appeared in January; the higher emissions occurred in mid-December, early January, and mid-February; and the peak emission appeared at 8:00, 11:00, 18:00, and 21:00. Furthermore, the uncertainty analysis of the emission inventory was carried out by using the Monte Carlo method. This study provides a more high temporal and spatial resolution emission inventory of RCC for air quality model, which can accurately simulate regional pollutant emission scenarios.
{"title":"Emission inventory of air pollutants from residential coal combustion over the Beijing-Tianjin-Hebei Region in 2020","authors":"Ruting Zhang, Chuanmin Chen, Songtao Liu, Huacheng Wu, Weiqing Zhou, Peng Li","doi":"10.1007/s11869-023-01375-4","DOIUrl":"10.1007/s11869-023-01375-4","url":null,"abstract":"<div><p>To investigate the atmospheric pollutant emission from residential coal combustion (RCC) in BTH region in 2020, based on the bottom-up methodology, a high spatial and temporal resolution air pollutant emission inventory was established. The results showed that the emissions of PM<sub>10</sub>, PM<sub>2.5</sub>, BC, OC, CO, NO<sub><i>x</i></sub>, SO<sub>2</sub>, and VOCs in BTH region in 2020 were 19.58, 15.67, 2.98, 8.33, 296.96, 3.51, 36.67, and 5.87 million tons, respectively. Chengde contributed the most PM<sub>2.5</sub>, BC, OC, and VOCs in BTH region, accounted for 11.48%, 13.71%, 11.52%, and 12.72%, respectively. While Shijiazhuang contributed the most PM<sub>10</sub>, CO, NO<sub><i>x</i></sub>, and SO<sub>2</sub> in BTH region, accounted for 11.55%, 11.60%, 11.55%, and 12.10%, respectively. The spatial distribution characteristics of pollutants showed that high emissions concentrated in northern, eastern, and southern areas of BTH region. Based on the time distribution factor obtained from the long-term follow-up survey data of RCC of households in BTH region, the annual emissions of different cities were allocated according to the temporal resolution of monthly, daily, and hourly. It was found that for each pollutant, the highest emissions appeared in January; the higher emissions occurred in mid-December, early January, and mid-February; and the peak emission appeared at 8:00, 11:00, 18:00, and 21:00. Furthermore, the uncertainty analysis of the emission inventory was carried out by using the Monte Carlo method. This study provides a more high temporal and spatial resolution emission inventory of RCC for air quality model, which can accurately simulate regional pollutant emission scenarios.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-07-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s11869-023-01375-4.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50451903","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-06-26DOI: 10.1007/s11869-023-01384-3
Prashant Patel, Shankar G. Aggarwal, Thi-Cuc Le, Khem Singh, Daya Soni, Chuen-Jinn Tsai
Size-segregated sampling of particulate matter (PM) using impactor suffers from D50 cutoff shift due to particle loading and re-entrainment problems. Cyclonic separation is a viable option to overcome the above problem. However, conventional reverse flow cyclone design having a single inlet and upward-facing outlet also presents a common issue of sample (particle) loss during sampling and requires several arrangements to convert it into an efficient PM sampler. Therefore, here we present a high-volume (HV) PM10 multi-inlet cyclone (MIC) design with a downward-facing outlet, which overcomes existing problems and has additional advantages, such as omnidirectional sampling where a filter collector is placed in a straight line below the cyclone outlet to minimize sample loss. Moreover, like the existing USEPA reference low-volume PM2.5 sampler inlet design, which consists of 2-impactor stages (PM10 followed by PM2.5) in a straight path, this developed HV PM10 MIC sampler can accommodate a second size fractionator (e.g., PM2.5 impactor) to sample finer-size PM on a filter. D50 cutoff of developed PM10 MIC is numerically and experimentally investigated. Since the study regarding cutoff size of another type PM10 cyclone, called respirable dust sampler (RDS) is not available in the public domain and is widely used for PM10 monitoring in India, we investigated its cutoff size empirically and experimentally, and also performed field comparisons. Collocating field evaluation of PM10 MIC and PM10 RDS cyclone was done under a wide range of particle mass loading, and results were compared with USEPA-approved high-volume PM10 impactor sampler and with a real-time particle sizer. The D50 cutoff of PM10 MIC is experimentally achieved to be 9.89 ± 0.3 µm, which is close to 9.94 µm predicted numerically and lies in the range of 9.5–10.5 µm size measured by others for PM10 impactor sampler (USEPA). The D50 cutoff of the PM10 RDS cyclone is experimentally determined to be 3.56 ± 0.1 µm, which is surprisingly lower than its claimed cutoff of 10 µm mentioned in numerous articles, where it has been used for air quality reporting and studies related to aerosol science. The field comparison correlation of PM10 MIC for PM10-2.5 levels with PM10 sampler (USEPA) (R = 0.99) and particle sizer (R = 0.94) correlated well, and the mean deviations are found to be 6.2% and 3%, respectively. While PM10 (RDS) cyclone poorly correlates (R = 0.67), and the mean deviation is 68%. Overall, the developed PM10 MIC overcomes issues associated with existing impactor and conventional cyclone sampler, and can be a better option for high-volume PM10 sampling, especially under a wide range of amb
{"title":"Design and development of a PM10 multi-inlet cyclone and comparison with reference cyclones","authors":"Prashant Patel, Shankar G. Aggarwal, Thi-Cuc Le, Khem Singh, Daya Soni, Chuen-Jinn Tsai","doi":"10.1007/s11869-023-01384-3","DOIUrl":"10.1007/s11869-023-01384-3","url":null,"abstract":"<div><p>Size-segregated sampling of particulate matter (PM) using impactor suffers from D<sub>50</sub> cutoff shift due to particle loading and re-entrainment problems. Cyclonic separation is a viable option to overcome the above problem. However, conventional reverse flow cyclone design having a single inlet and upward-facing outlet also presents a common issue of sample (particle) loss during sampling and requires several arrangements to convert it into an efficient PM sampler. Therefore, here we present a high-volume (HV) PM<sub>10</sub> multi-inlet cyclone (MIC) design with a downward-facing outlet, which overcomes existing problems and has additional advantages, such as omnidirectional sampling where a filter collector is placed in a straight line below the cyclone outlet to minimize sample loss. Moreover, like the existing USEPA reference low-volume PM<sub>2.5</sub> sampler inlet design, which consists of 2-impactor stages (PM<sub>10</sub> followed by PM<sub>2.5</sub>) in a straight path, this developed HV PM<sub>10</sub> MIC sampler can accommodate a second size fractionator (e.g., PM<sub>2.5</sub> impactor) to sample finer-size PM on a filter. D<sub>50</sub> cutoff of developed PM<sub>10</sub> MIC is numerically and experimentally investigated. Since the study regarding cutoff size of another type PM<sub>10</sub> cyclone, called respirable dust sampler (RDS) is not available in the public domain and is widely used for PM<sub>10</sub> monitoring in India, we investigated its cutoff size empirically and experimentally, and also performed field comparisons. Collocating field evaluation of PM<sub>10</sub> MIC and PM<sub>10</sub> RDS cyclone was done under a wide range of particle mass loading, and results were compared with USEPA-approved high-volume PM<sub>10</sub> impactor sampler and with a real-time particle sizer. The D<sub>50</sub> cutoff of PM<sub>10</sub> MIC is experimentally achieved to be 9.89 ± 0.3 µm, which is close to 9.94 µm predicted numerically and lies in the range of 9.5–10.5 µm size measured by others for PM<sub>10</sub> impactor sampler (USEPA). The D<sub>50</sub> cutoff of the PM<sub>10</sub> RDS cyclone is experimentally determined to be 3.56 ± 0.1 µm, which is surprisingly lower than its claimed cutoff of 10 µm mentioned in numerous articles, where it has been used for air quality reporting and studies related to aerosol science. The field comparison correlation of PM<sub>10</sub> MIC for PM<sub>10-2.5</sub> levels with PM<sub>10</sub> sampler (USEPA) (<i>R</i> = 0.99) and particle sizer (<i>R</i> = 0.94) correlated well, and the mean deviations are found to be 6.2% and 3%, respectively. While PM<sub>10</sub> (RDS) cyclone poorly correlates (<i>R</i> = 0.67), and the mean deviation is 68%. Overall, the developed PM<sub>10</sub> MIC overcomes issues associated with existing impactor and conventional cyclone sampler, and can be a better option for high-volume PM<sub>10</sub> sampling, especially under a wide range of amb","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-06-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50515714","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Operation room personnel are exposed to high concentrations of surgical smoke during electrosurgery and laser treatment. Surgical smoke contains viral aerosol, particulate matter, volatile organic compounds, and microorganisms. Current local exhaust ventilation control methods can be noisy, bulky, and expensive. In this study, we are the first to build a cost-effective air curtain device to remove surgical smoke. Experiments were conducted in an operating room by cutting porcine samples with electrosurgical units. An air curtain system was installed below the surgical light. We measured the particle number and mass concentrations in the breathing zone. The concentrations were recorded under four scenarios: no control, commercial smoke evacuation pencil, low-velocity air curtain, and high-velocity air curtain. Results indicate that the air curtain reduces the concentration of particulate matter and produces less noise than commercial smoke evacuation pencils. The particle number removal efficiencies for the smoke evacuation pencil, low-velocity air curtain, and high-velocity air curtain were 88.52%, 70.79%, and 91.29%, respectively. The respective PM2.5 removal efficiencies were 90.92%, 85.38%, and 97.99%. Thus, installing an air curtains under surgical lights is a promising method for reducing surgical smoke and protecting medical personnel.
{"title":"Applying an air curtain to reduce surgical smoke concentration","authors":"Xuan-Huy Ninh, Hung-Yu Tzeng, Tak-Wah Wong, Yu-Ting Wu, Yao-Lung Kuo, Ming-Yeng Lin","doi":"10.1007/s11869-023-01383-4","DOIUrl":"10.1007/s11869-023-01383-4","url":null,"abstract":"<div><p>Operation room personnel are exposed to high concentrations of surgical smoke during electrosurgery and laser treatment. Surgical smoke contains viral aerosol, particulate matter, volatile organic compounds, and microorganisms. Current local exhaust ventilation control methods can be noisy, bulky, and expensive. In this study, we are the first to build a cost-effective air curtain device to remove surgical smoke. Experiments were conducted in an operating room by cutting porcine samples with electrosurgical units. An air curtain system was installed below the surgical light. We measured the particle number and mass concentrations in the breathing zone. The concentrations were recorded under four scenarios: no control, commercial smoke evacuation pencil, low-velocity air curtain, and high-velocity air curtain. Results indicate that the air curtain reduces the concentration of particulate matter and produces less noise than commercial smoke evacuation pencils. The particle number removal efficiencies for the smoke evacuation pencil, low-velocity air curtain, and high-velocity air curtain were 88.52%, 70.79%, and 91.29%, respectively. The respective PM<sub>2.5</sub> removal efficiencies were 90.92%, 85.38%, and 97.99%. Thus, installing an air curtains under surgical lights is a promising method for reducing surgical smoke and protecting medical personnel.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-06-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50515713","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-06-24DOI: 10.1007/s11869-023-01386-1
Mihalis Lazaridis
Dosimetry models for the estimation of particle deposition in the human respiratory tract (RT) in conjunction with clearance transport models are vital components to relate human exposure with internal dose in a quantitative manner. The current work highlights knowledge and modelling approaches on particle deposition and translocation in the human body in an effort to determine health risks in respect to different particle physicochemical properties and human physiology parameters. These include breathing conditions, variability of the geometry of the RT, chemical composition and size of deposits. Different dosimetry modelling approaches have been studied including empirical formulations, one-dimensional flow modelling and computational fluid dynamic methods (CFD). The importance of a realistic modelling of hygroscopicity has been also investigated. A better understanding of the relationship between health effects and inhaled particle dose may be elaborated using dosimetry and clearance modelling tools. A future required approach is to combine dosimetry models with physiologically based pharmacokinetic models (PBPK) to simulate the transport and cumulative dose of particle-bound chemical species in different organs and tissues of the human body.
{"title":"Modelling approaches to particle deposition and clearance in the human respiratory tract","authors":"Mihalis Lazaridis","doi":"10.1007/s11869-023-01386-1","DOIUrl":"10.1007/s11869-023-01386-1","url":null,"abstract":"<div><p>Dosimetry models for the estimation of particle deposition in the human respiratory tract (RT) in conjunction with clearance transport models are vital components to relate human exposure with internal dose in a quantitative manner. The current work highlights knowledge and modelling approaches on particle deposition and translocation in the human body in an effort to determine health risks in respect to different particle physicochemical properties and human physiology parameters. These include breathing conditions, variability of the geometry of the RT, chemical composition and size of deposits. Different dosimetry modelling approaches have been studied including empirical formulations, one-dimensional flow modelling and computational fluid dynamic methods (CFD). The importance of a realistic modelling of hygroscopicity has been also investigated. A better understanding of the relationship between health effects and inhaled particle dose may be elaborated using dosimetry and clearance modelling tools. A future required approach is to combine dosimetry models with physiologically based pharmacokinetic models (PBPK) to simulate the transport and cumulative dose of particle-bound chemical species in different organs and tissues of the human body.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-06-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s11869-023-01386-1.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50510588","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-06-24DOI: 10.1007/s11869-023-01387-0
Sung-Chul Seo, Woo-Je Lee, Doo-Young Kim, Ki-Youn Kim
Currently odor problems caused by animal feeding operation play a role in provoking environmental civil petition. The objectives of this study were to investigate the monthly distribution characteristics of 22 offensive odor compounds in swine houses, which are under regulation in Korea, and to compare their levels according to ventilation type and manure treatment mode. During the 1 year survey between July 2021 and June 2022, air samples were collected. In this study, ammonia was observed at the highest levels (the annual mean, 13.9 × 103 ppb) among other offensive odorous compound regardless of the types of swine house and seasons, followed by fatty acids (139.9 ppb), sulfuric odorous compounds (52.3 ppb), volatile organic compounds (27.5 ppb), and trimethyl amine (24.5 ppb). Furthermore, hydrogen sulfide among sulfur compounds, methyl ethyl ketone among volatile organic compounds, and propionic acid and n-butylic acid among fatty acids were observed to the highest level of several hundreds of ppb. In particular, five aldehydes (acetaldehyde, propionaldehyde, butyraldehyde, n-valeraldehyde, and i-valeraldehyde) among the 22 offensive odor-generating compounds were not detected in any season. The levels of odorous compounds were the highest in winter (Dec.–Feb.) and lowest in summer (June–Aug.). For comparison of overall distribution regarding concentrations of odorous compounds by ventilation type and manure removal mode, relatively lower concentrations were observed in swine houses with forced ventilation or with scrapper type. Our findings indicate that annual monitoring for these odorous compounds would be necessary for establishment of control strategy. Also, installation of active ventilation, as well as the increase of removal frequency of pig manure could contribute to lower concentrations of odorous compounds in swine buildings.
{"title":"Temporal distribution characteristics of odorous compounds in swine houses of South Korea","authors":"Sung-Chul Seo, Woo-Je Lee, Doo-Young Kim, Ki-Youn Kim","doi":"10.1007/s11869-023-01387-0","DOIUrl":"10.1007/s11869-023-01387-0","url":null,"abstract":"<div><p>Currently odor problems caused by animal feeding operation play a role in provoking environmental civil petition. The objectives of this study were to investigate the monthly distribution characteristics of 22 offensive odor compounds in swine houses, which are under regulation in Korea, and to compare their levels according to ventilation type and manure treatment mode. During the 1 year survey between July 2021 and June 2022, air samples were collected. In this study, ammonia was observed at the highest levels (the annual mean, 13.9 × 10<sup>3</sup> ppb) among other offensive odorous compound regardless of the types of swine house and seasons, followed by fatty acids (139.9 ppb), sulfuric odorous compounds (52.3 ppb), volatile organic compounds (27.5 ppb), and trimethyl amine (24.5 ppb). Furthermore, hydrogen sulfide among sulfur compounds, methyl ethyl ketone among volatile organic compounds, and propionic acid and n-butylic acid among fatty acids were observed to the highest level of several hundreds of ppb. In particular, five aldehydes (acetaldehyde, propionaldehyde, butyraldehyde, n-valeraldehyde, and i-valeraldehyde) among the 22 offensive odor-generating compounds were not detected in any season. The levels of odorous compounds were the highest in winter (Dec.–Feb.) and lowest in summer (June–Aug.). For comparison of overall distribution regarding concentrations of odorous compounds by ventilation type and manure removal mode, relatively lower concentrations were observed in swine houses with forced ventilation or with scrapper type. Our findings indicate that annual monitoring for these odorous compounds would be necessary for establishment of control strategy. Also, installation of active ventilation, as well as the increase of removal frequency of pig manure could contribute to lower concentrations of odorous compounds in swine buildings.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-06-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s11869-023-01387-0.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50510730","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-06-23DOI: 10.1007/s11869-023-01382-5
Ruhui Cao, Binru Luo, Kaixuan Liu, Zhanyong Wang, Ming Cai, Xisheng Hu, Jinqiang Xu, Zhongmou Fan
The ongoing improvement of urban air quality urgently needs refined understanding of air pollution variation. For urban roads, due to the changeable traffic flow and complex road environments, commuters usually confront with a direct but uncertain exposure to traffic-induced air pollutants. However, the current lack of fine-grained measurements and reliable analytical methods restricts our knowledge of road air pollution risk. Therefore, we designed a bicycling experiment to collect fine-scale concentration samples of PM2.5, PM10, and black carbon (BC) in non-motorized lanes beside an expressway. Mobile measurements revealed high particle pollution at the building-intensive roadside, and the background pollution concentration removal clarified high-polluted sections. Generalized additive models demonstrated that the background pollution concentrations dominated the overall pattern of particles, and meteorological factors had significant but varied impacts on local variations of particles. Riverside winds lowered PM2.5 and PM10 levels most time, while BC was more affected by roadside greenery, distance from roadway and diesel vehicles. At the hotspots, an increase of 100 diesel vehicles per hour could increase roadside BC by about 2% per kilometer but brought no obvious increase in PM2.5 and PM10. These results confirm the availability of mobile measurements and generalized additive models in high-resolution pollution analysis, and are beneficial to countermeasures of reducing personal exposure risk of slow-moving traffic.
{"title":"Characterizing and interpreting the spatial variation of traffic pollution in urban non-motorized lanes using mobile measurements","authors":"Ruhui Cao, Binru Luo, Kaixuan Liu, Zhanyong Wang, Ming Cai, Xisheng Hu, Jinqiang Xu, Zhongmou Fan","doi":"10.1007/s11869-023-01382-5","DOIUrl":"10.1007/s11869-023-01382-5","url":null,"abstract":"<div><p>The ongoing improvement of urban air quality urgently needs refined understanding of air pollution variation. For urban roads, due to the changeable traffic flow and complex road environments, commuters usually confront with a direct but uncertain exposure to traffic-induced air pollutants. However, the current lack of fine-grained measurements and reliable analytical methods restricts our knowledge of road air pollution risk. Therefore, we designed a bicycling experiment to collect fine-scale concentration samples of PM<sub>2.5</sub>, PM<sub>10</sub>, and black carbon (BC) in non-motorized lanes beside an expressway. Mobile measurements revealed high particle pollution at the building-intensive roadside, and the background pollution concentration removal clarified high-polluted sections. Generalized additive models demonstrated that the background pollution concentrations dominated the overall pattern of particles, and meteorological factors had significant but varied impacts on local variations of particles. Riverside winds lowered PM<sub>2.5</sub> and PM<sub>10</sub> levels most time, while BC was more affected by roadside greenery, distance from roadway and diesel vehicles. At the hotspots, an increase of 100 diesel vehicles per hour could increase roadside BC by about 2% per kilometer but brought no obvious increase in PM<sub>2.5</sub> and PM<sub>10</sub>. These results confirm the availability of mobile measurements and generalized additive models in high-resolution pollution analysis, and are beneficial to countermeasures of reducing personal exposure risk of slow-moving traffic.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-06-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50507440","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Mounting studies explored associations between fine particulate matter (PM2.5) and preterm birth (PTB); however, individual and combined impacts of PM2.5 constituents on PTB were less known. PM2.5 and its seven constituents were assessed by V4.CH.02 product of the Dalhousie University Atmospheric Composition Analysis Group, a dataset containing combined geophysical-statistical estimates of PM2.5 across China. Effects of PM2.5 and its constituents on PTB and gestational age were firstly explored. Furthermore, weighted quantile sum (WQS) regression was conducted to reveal the impacts of total PM2.5 mass and identify contributing constituents. An interquartile range (IQR) increase in PM2.5 was associated with increased odds ratio (OR) of PTB. PM2.5 constituents were widely associated with PTB and reduced gestational age, with different time window. The total mass of PM2.5 (per IQR increment) in the first and the second trimester was positively associated with PTB by WQS regression (Trimester 1: OR = 1.38, 95%CI: 1.15, 1.65; Trimester 2: OR = 1.47, 95%CI: 1.21, 1.79). The most contributing factors were black carbon in the first trimester and sulphate ion in the second trimester, respectively. Especially, sea salt was identified as contributing constituent during the first trimester. The study indicated that prenatal exposure to PM2.5 and its constituents was individually and jointly associated with PTB and reduced gestational age. Sea salt was firstly identified as a risk factor of PTB in the seaside city, which needs further exploration.
{"title":"Independent and combined effects of PM2.5 and its constituents on preterm birth: a retrospective study in a seaside city","authors":"Chao Dong, Mingzhi Zhang, Yuhong Zhang, Xiaochen Zhang, Yin Zhuang, Yifen Wang, Qian Qian, Wei Li, Yanyan Yu, Yankai Xia","doi":"10.1007/s11869-023-01363-8","DOIUrl":"10.1007/s11869-023-01363-8","url":null,"abstract":"<div><p>Mounting studies explored associations between fine particulate matter (PM<sub>2.5</sub>) and preterm birth (PTB); however, individual and combined impacts of PM<sub>2.5</sub> constituents on PTB were less known. PM<sub>2.5</sub> and its seven constituents were assessed by V4.CH.02 product of the Dalhousie University Atmospheric Composition Analysis Group, a dataset containing combined geophysical-statistical estimates of PM<sub>2.5</sub> across China. Effects of PM<sub>2.5</sub> and its constituents on PTB and gestational age were firstly explored. Furthermore, weighted quantile sum (WQS) regression was conducted to reveal the impacts of total PM<sub>2.5</sub> mass and identify contributing constituents. An interquartile range (IQR) increase in PM<sub>2.5</sub> was associated with increased odds ratio (OR) of PTB. PM<sub>2.5</sub> constituents were widely associated with PTB and reduced gestational age, with different time window. The total mass of PM<sub>2.5</sub> (per IQR increment) in the first and the second trimester was positively associated with PTB by WQS regression (Trimester 1: OR = 1.38, 95%CI: 1.15, 1.65; Trimester 2: OR = 1.47, 95%CI: 1.21, 1.79). The most contributing factors were black carbon in the first trimester and sulphate ion in the second trimester, respectively. Especially, sea salt was identified as contributing constituent during the first trimester. The study indicated that prenatal exposure to PM<sub>2.5</sub> and its constituents was individually and jointly associated with PTB and reduced gestational age. Sea salt was firstly identified as a risk factor of PTB in the seaside city, which needs further exploration.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-06-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50505628","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2023-06-21DOI: 10.1007/s11869-023-01385-2
Rui Zhang, Norhashidah Awang
Fine particulate matter (PM2.5) is a hazardous air pollutant with an aerodynamic diameter of 2.5 μm or less, which can lead to severe health impacts such as cardiovascular disease, respiratory illnesses, and various types of cancer. Therefore, accurate forecasting of PM2.5 concentrations is crucial for public health and policy-making. However, due to the stochastic nature of PM2.5, achieving high prediction accuracy and efficiency remains a challenge. To address this challenge, this study proposes a hybrid deep learning model consisting of principal component analysis (PCA), discrete stationary wavelet transform (DSWT), and Nested LSTM (NLSTM) neural network to predict PM2.5 concentrations. The proposed model aims to leverage the strengths of each technique to achieve better accuracy and efficiency in PM2.5 forecasting. Specifically, PCA is employed as the feature extraction method to reduce the dimensionality of the data and improve computing efficiency. Additionally, DSWT is utilized to decompose the reduced-dimensional data into several sub-signals that are more regular and stable, enabling the NLSTM network to learn each sub-signal separately. Finally, the predicted values of each sub-signal are reconstructed to obtain the final PM2.5 forecast. The proposed model is validated using daily air pollutants and meteorological variables collected in Taiyuan, China, from January 1, 2016, to December 31, 2020. The long-term, medium-term, and short-term forecast results demonstrate that the proposed model achieves better accuracy and efficiency compared to existing models. Overall, the proposed hybrid deep learning model provides a promising solution for accurate and efficient forecasting of PM2.5 concentrations, and the findings of this study have important implications for public health and environmental policy.
{"title":"An ensemble NLSTM-based model for PM2.5 concentrations prediction considering feature extraction and data decomposition","authors":"Rui Zhang, Norhashidah Awang","doi":"10.1007/s11869-023-01385-2","DOIUrl":"10.1007/s11869-023-01385-2","url":null,"abstract":"<div><p>Fine particulate matter (PM2.5) is a hazardous air pollutant with an aerodynamic diameter of 2.5 μm or less, which can lead to severe health impacts such as cardiovascular disease, respiratory illnesses, and various types of cancer. Therefore, accurate forecasting of PM2.5 concentrations is crucial for public health and policy-making. However, due to the stochastic nature of PM2.5, achieving high prediction accuracy and efficiency remains a challenge. To address this challenge, this study proposes a hybrid deep learning model consisting of principal component analysis (PCA), discrete stationary wavelet transform (DSWT), and Nested LSTM (NLSTM) neural network to predict PM2.5 concentrations. The proposed model aims to leverage the strengths of each technique to achieve better accuracy and efficiency in PM2.5 forecasting. Specifically, PCA is employed as the feature extraction method to reduce the dimensionality of the data and improve computing efficiency. Additionally, DSWT is utilized to decompose the reduced-dimensional data into several sub-signals that are more regular and stable, enabling the NLSTM network to learn each sub-signal separately. Finally, the predicted values of each sub-signal are reconstructed to obtain the final PM2.5 forecast. The proposed model is validated using daily air pollutants and meteorological variables collected in Taiyuan, China, from January 1, 2016, to December 31, 2020. The long-term, medium-term, and short-term forecast results demonstrate that the proposed model achieves better accuracy and efficiency compared to existing models. Overall, the proposed hybrid deep learning model provides a promising solution for accurate and efficient forecasting of PM2.5 concentrations, and the findings of this study have important implications for public health and environmental policy.</p></div>","PeriodicalId":49109,"journal":{"name":"Air Quality Atmosphere and Health","volume":null,"pages":null},"PeriodicalIF":5.1,"publicationDate":"2023-06-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"50502843","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}