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Gaseous pollutants linked to pulmonary diseases: East meets West 气体污染物与肺部疾病有关:东西方文化的碰撞
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2024-07-12 DOI: 10.1007/s11869-024-01608-0
Fatim Sannoh, Haider A. Khwaja, Zafar Fatmi, Nadeem A. Rizvi, Aftab Turabi, Mirza M. Hussain, Azhar Siddique, David O. Carpenter

Air pollution represents a critical global health challenge, especially in densely populated urban areas of developing countries such as Pakistan, where it ranks among the top five most affected Asian nations. Despite its significance, data on the health impacts of gaseous pollutants (O₃, NO, NO₂, HNO₃, and SO₂) are scant due to economic constraints and inadequate measurement infrastructure. This pioneering study is the first to quantitatively assess the morbidity risks associated with exposure to these pollutants in Karachi, a megacity in Pakistan, utilizing a robust cross-sectional design. We collected 400 air quality samples over four distinct seasons, correlating these with health data from over 12,000 hospital admissions for respiratory issues. Our results reveal significant associations between ozone exposure and a range of pulmonary diseases—including asthma, tuberculosis, and shortness of breath—across both genders. Specifically, sulfur dioxide (SO2) exposure was linked to increased shortness of breath in males, while exposure to nitric acid was more likely to cause COPD in males than in females. Additionally, nitrogen oxides (HNO3) were primarily associated with asthma in males. These associations were particularly pronounced in the 0–50 age group, suggesting a demographic at greater risk. These findings not only corroborate the global body of research on the health implications of urban air pollution but also provide critical new insights into the severe impacts within Karachi. The evidence presented underscores the urgent need for enhanced air pollution control policies and public health strategies tailored to the needs of rapidly urbanizing areas in Pakistan.

空气污染是一项严峻的全球健康挑战,尤其是在巴基斯坦等发展中国家人口稠密的城市地区,那里是亚洲受影响最严重的五个国家之一。尽管意义重大,但由于经济限制和测量基础设施不足,有关气态污染物(O₃、NO、NO₂、HNO₃ 和 SO₂)对健康影响的数据却很少。这项开创性的研究首次采用稳健的横断面设计,对巴基斯坦大城市卡拉奇与接触这些污染物相关的发病风险进行了定量评估。我们在四个不同的季节收集了 400 份空气质量样本,并将这些样本与 12,000 多名因呼吸系统问题入院的患者的健康数据进行了关联。我们的研究结果表明,臭氧暴露与一系列肺部疾病--包括哮喘、肺结核和呼吸急促--之间存在明显的相关性。具体来说,男性接触二氧化硫(SO2)会导致呼吸急促,而男性接触硝酸比女性更容易导致慢性阻塞性肺病。此外,氮氧化物(HNO3)主要与男性哮喘有关。这些关联在 0-50 岁年龄组中尤为明显,表明该年龄组的人群面临更大的风险。这些研究结果不仅证实了全球范围内关于城市空气污染对健康影响的研究,而且为了解卡拉奇的严重影响提供了重要的新见解。所提供的证据突出表明,迫切需要针对巴基斯坦快速城市化地区的需求,加强空气污染控制政策和公共卫生战略。
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引用次数: 0
Higher temperatures are associated with increased asthma-related emergency department visits among children: a time series analysis of environmental exposures in Montreal, Canada 气温升高与儿童哮喘急诊就诊人数增加有关:对加拿大蒙特利尔环境暴露的时间序列分析
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2024-07-11 DOI: 10.1007/s11869-024-01610-6
Sze Man Tse, Sadio Sambahke, Masoumeh Sajedi, Jocelyn Gravel, Esli Osmanlliu

Asthma exacerbations are a leading cause of emergency department (ED) visits in children. Outdoor exposures such as air pollutants and meteorological factors have been associated with risk of asthma exacerbations. We evaluated the association between ambient temperature, relative humidity, and air quality on pediatric asthma-related ED visits in Montréal, Canada. In this retrospective study, we included children ≤ 17 years presenting with asthma to two pediatric EDs between January 1, 2017 and December 31st, 2020. Temperature and relative humidity data were obtained daily for Montréal through Weather Source™ and the Air Quality Health Index (AQHI) through Environment Canada. We evaluated the association between environmental exposures and the incidence of asthma-related ED visits using a quasi-Poisson regression analysis, adjusting for seasonality. We examined 21 201 asthma-related ED visits. Increased temperature was associated with an increased number of asthma-related ED visits. Compared to the reference decile (2.8 to 7.5⁰C), the strongest association with incident ED visits was for a temperature of 15.8 to 19.3⁰C, associated with a 37% increase in the number of asthma-related ED visits (IRR = 1.37, 95% CI 1.22, 1.54). Current day relative humidity, AQHI, and changes of the exposure levels over the previous 1 to 7 days did not have an effect on asthma-related ED visits. Adjusting for seasonality, higher temperatures were associated with an increased number of asthma-related ED visits among children while humidity and air quality were not. At a population level, this can inform hospitals of upcoming trends in ED visits.

哮喘加重是儿童看急诊(ED)的主要原因。空气污染物和气象因素等室外暴露与哮喘加重的风险有关。我们评估了环境温度、相对湿度和空气质量与加拿大蒙特利尔市儿童哮喘相关急诊就诊率之间的关系。在这项回顾性研究中,我们纳入了 2017 年 1 月 1 日至 2020 年 12 月 31 日期间在两家儿科急诊室就诊的≤17 岁的哮喘儿童。我们通过 Weather Source™ 获得了蒙特利尔市每天的温度和相对湿度数据,并通过加拿大环境部获得了空气质量健康指数 (AQHI)。我们采用准泊松回归分析法评估了环境暴露与哮喘相关急诊就诊率之间的关系,并对季节性因素进行了调整。我们研究了 21 201 例哮喘相关的急诊就诊。温度升高与哮喘相关的急诊就诊人数增加有关。与参考十分位数(2.8 至 7.5⁰C)相比,气温在 15.8 至 19.3 ⁰C 之间与急诊室就诊人数的关联性最强,与哮喘相关的急诊室就诊人数增加了 37%(IRR = 1.37,95% CI 1.22,1.54)。当日相对湿度、空气质量健康指数以及过去 1 到 7 天的暴露水平变化对哮喘相关急诊就诊人数没有影响。在对季节性因素进行调整后,气温升高与儿童哮喘相关的急诊就诊人数增加有关,而湿度和空气质量则没有影响。在人口层面,这可以让医院了解急诊室就诊人数的未来趋势。
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引用次数: 0
An orthogonal experiment study of NH3 concentration and its influencing factors in non-newly constructed university dormitories 非新建大学宿舍 NH3 浓度及其影响因素的正交实验研究
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2024-07-10 DOI: 10.1007/s11869-024-01605-3
Chanjuan Sun, Jianjie Ma, Jingyu Chen, Chen Huang, Jingguang Li

The Air quality in university dormitories influences the learning efficiency and health of students. This study aims to evaluate the degree of influencing factors on NH3 concentration in non-newly constructed university dormitories. On-site monitoring was conducted in 136 dormitories between winter in 2021 and summer in 2022 in Shanghai. Five factors, including indoor temperature, indoor humidity, room ventilation, dormitory toilet, and cooking conditions, were identified as objects of the study. A typical student dormitory, consisting of a toilet, a storage room and a main room, was chosen to conduct orthogonal experiments. Results are as follows: The average NH3 concentration in dormitories was 0.59 mg/m3. 48% of the concentration levels exceeded the limits (0.20 mg/m3) specified in the Standards for indoor air quality (GB/T18883-2022). The range sizes of indoor temperature, indoor humidity, room ventilation, toilet, and cooking conditions were 0.01, 0.74, 1.01, 0.05, and 0.52 respectively, and the respective square sum of deviations were 0.000, 0.274, 0.510, 0.001, and 0.135. Consequently, the order of impact on NH3 concentration ranks as follows: room ventilation > indoor humidity > cooking conditions > toilet > indoor temperature. The optimal environmental conditions for achieving the lowest NH3 concentration in dormitory are found to be: ventilation (with fully open windows), low temperature (18 °C), low humidity (50%), absent cooking, and no usage of the toilet. These findings can trigger attention to NH3 pollution in dormitories, leading to more effective advice for controlling NH3 concentration in dormitories of non-newly constructed university and reducing its effects on students’ health.

大学宿舍的空气质量影响着学生的学习效率和身体健康。本研究旨在评估非新建高校宿舍中 NH3 浓度的影响因素程度。在 2021 年冬季至 2022 年夏季期间,对上海 136 间宿舍进行了现场监测。室内温度、室内湿度、室内通风、宿舍厕所和烹饪条件等五个因素被确定为研究对象。选取一个由厕所、储藏室和主卧室组成的典型学生宿舍进行正交实验。实验结果如下宿舍内的 NH3 平均浓度为 0.59 mg/m3。48%的浓度水平超过了《室内空气质量标准》(GB/T18883-2022)中规定的限值(0.20 mg/m3)。室内温度、室内湿度、室内通风、卫生间和烹饪条件的范围大小分别为 0.01、0.74、1.01、0.05 和 0.52,偏差平方和分别为 0.000、0.274、0.510、0.001 和 0.135。因此,对 NH3 浓度影响的排序依次为:房间通风;室内湿度;烹饪条件;厕所;室内温度。要使宿舍内的 NH3 浓度最低,最佳的环境条件是:通风(窗户全开)、低温(18 °C)、低湿度(50%)、不做饭和不使用厕所。这些发现可引起人们对宿舍内 NH3 污染的关注,从而为控制非新建大学宿舍内的 NH3 浓度和减少其对学生健康的影响提供更有效的建议。
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引用次数: 0
An empirical analysis of agricultural and rural carbon emissions under the background of rural revitalization strategy–based on machine learning algorithm 基于机器学习算法的乡村振兴战略背景下农业与农村碳排放实证分析
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2024-07-08 DOI: 10.1007/s11869-024-01606-2
XiaoYu Niu, YuZhu Tian, ManLai Tang, ZhiBao Mian

Agricultural and rural carbon (ARC) emissions are a major source of greenhouse gas emissions in China and have profound implications for implementing the rural revitalization strategy. This study takes Shandong Province, a leading agricultural province in China, as a case study to explore the relationship between ARC emissions and their influencing factors. It employs the Logarithmic Mean Divisia Index (LMDI) model to decompose changes in ARC emissions from 2000 to 2021, analyzing the contributions of factors such as agricultural production efficiency and agricultural industrial structure. The study then expands the indicator system and applies feature selection methods to identify the main influencing factors. It establishes Bayes model averaging (BMA), STIRPAT-Ridge regression and Long Short-Term Memory (LSTM) models to evaluate their performance in modeling historical ARC emissions. Finally, the study makes prospective forecasts of ARC emissions in Shandong Province from 2022 to 2050 under low, medium and high speed development scenarios. The findings show that from 2000 to 2021, ARC emission intensity decreased by 71.86% in Shandong. Key factors like agricultural production efficiency and agricultural industrial structure exhibited emission reduction effects. Agricultural production efficiency, electricity consumption, agricultural economic level, and transportation travel positively impact ARC emissions, with agricultural production efficiency and electricity consumption as the dominant factors. Under the development high-speed scenario, ARC emissions are projected to peak around 2030. Reducing carbon emissions intensity, improving resource use efficiency and maintaining steady economic growth are crucial for controlling future ARC emissions and achieving sustainable development in Shandong Province.

农业和农村碳排放(ARC)是中国温室气体排放的主要来源,对实施乡村振兴战略具有深远影响。本研究以中国农业大省山东省为例,探讨农业农村碳排放与其影响因素之间的关系。研究采用对数均值指数(LMDI)模型对 2000 年至 2021 年 ARC 排放量的变化进行分解,分析了农业生产效率、农业产业结构等因素的贡献。然后,研究扩展了指标体系,并应用特征选择方法确定了主要影响因素。研究建立了贝叶斯模型平均法(BMA)、STIRPAT-岭回归法和长短期记忆法(LSTM)模型,以评估它们在建立 ARC 历史排放量模型方面的性能。最后,研究对山东省 2022 年至 2050 年在低、中、高速发展情景下的 ARC 排放量进行了前瞻性预测。研究结果表明,从 2000 年到 2021 年,山东省 ARC 排放强度下降了 71.86%。农业生产效率、农业产业结构等关键因素表现出减排效果。农业生产效率、用电量、农业经济水平和交通出行对 ARC 排放有正向影响,其中农业生产效率和用电量是主导因素。在高速发展情景下,预计 ARC 排放量将在 2030 年左右达到峰值。降低碳排放强度、提高资源利用效率、保持经济稳定增长是控制未来 ARC 排放、实现山东省可持续发展的关键。
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引用次数: 0
The impact of respirable dust exposure on lung function parameters of motorcycle taxi drivers in Bangkok and adjacent provinces, Thailand 可吸入粉尘暴露对泰国曼谷及邻近省份摩的司机肺功能参数的影响
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2024-06-29 DOI: 10.1007/s11869-024-01599-y
Kamonwan Samana, Kimihito Ito, Orasa Suthienkul, Arroon Ketsakorn

The motorcycle taxi drivers of Bangkok and adjacent provinces in Thailand may have been heavily exposed to ambient air pollution and the impact of this on their lungs has been neither documented nor studied. In this study, we recruited a total of 343 motorcycle taxi drivers in Bangkok and adjacent provinces in Thailand and their lung function parameters were analyzed using spirometry in May and June 2022. Of these, 153 participants were selected and their exposure to respirable dust during working was measured by personal air sampling. Respirable dust concentrations collected with personal air sampling suggested that motorcycle taxi drivers working at workstations where they were exposed to respirable dust at high concentrations tended to have a low percent predicted FEV1. Twelve% and 7.3% of motorcycle taxi drivers recruited in this study had the symptoms of chronic bronchitis and acute bronchitis, respectively. These results suggested that some motorcycle taxi drivers around Bangkok and adjacent provinces had a high risk of occupational exposure to ambient air pollution. The government needs to establish a medical check-up system for motorcycle taxi drivers to monitor their health status.

泰国曼谷及邻近省份的摩托车出租车司机可能大量暴露于环境空气污染中,而这种污染对他们肺部的影响尚未被记录或研究。在这项研究中,我们在泰国曼谷和邻近省份共招募了 343 名摩托车出租车司机,并于 2022 年 5 月和 6 月使用肺活量测定法对他们的肺功能参数进行了分析。其中,我们选取了 153 名参与者,通过个人空气采样测量了他们在工作期间暴露于可吸入粉尘的情况。通过个人空气采样收集的可吸入粉尘浓度表明,在暴露于高浓度可吸入粉尘的工作场所工作的摩托车出租车司机的预测 FEV1 百分比往往较低。在这项研究中,分别有 12% 和 7.3% 的摩的司机有慢性支气管炎和急性支气管炎的症状。这些结果表明,曼谷及邻近省份的一些摩托车出租车司机职业暴露于环境空气污染的风险很高。政府需要为摩托车出租车司机建立体检制度,以监测他们的健康状况。
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引用次数: 0
Developing a novel hybrid model based on deep neural networks and discrete wavelet transform algorithm for prediction of daily air temperature 开发基于深度神经网络和离散小波变换算法的新型混合模型,用于预测日气温
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2024-06-29 DOI: 10.1007/s11869-024-01595-2
Redvan Ghasemlounia, Amin Gharehbaghi, Farshad Ahmadi, Mohammad Albaji

The precise predicting of air temperature has a significant influence in many sectors such as agriculture, industry, modeling environmental processes. In this work, to predict the mean daily time series air temperature in Muğla city (ATm), Turkey, initially, five different layer structures of Long Short-Term Memory (LSTM) and Gated Recurrent Unit (GRU) deep learning-based neural network models through the seq2seq regression forecast module are developed. Then, based on performance evaluation metrics, an optimal DL-based layer network structure designed is chosen to hybridize with the wavelet transform (WT) algorithm (i.e., WT-DNN model) to enhance the estimation capability. In this direction, among potential meteorological variables considered, the average daily sunshine duration (SSD) (hours), total global solar radiation (TGSR) (kw. hour/m2), and total global insolation intensity (TGSI) (watt/m2) from Jan 2014 to Dec 2019 are picked as the most effective input variables through correlation analysis to predict ATm. To thwart overfitting and underfitting problems, different algorithm tuning along with trial-and-error procedures through diverse types of hyper-parameters are performed. Consistent with the performance evaluation standards, comparison plots, and Total Learnable Parameters (TLP) value, the state-of-the-art and unique proposed hybrid WT-(LSTM × GRU) model (i.e., hybrid WT with the coupled version of LSTM and GRU models via Multiplication layer ((times))) is confirmed as the best model developed. This hybrid model under the ideal hyper-parameters resulted in an R2 = 0.94, an RMSE = 0.56 (°C), an MBE = -0.5 (°C), AICc = -382.01, and a running time of 376 (s) in 2000 iterations. Nonetheless, the standard single LSTM layer network model as benchmark model resulted in an R2 = 0.63, an RMSE = 4.69 (°C), an MBE = -0.89 (°C), AICc = 1021.8, and a running time of 186 (s) in 2000 iterations.

气温的精确预测对农业、工业、环境过程建模等许多领域都有重要影响。在这项工作中,为了预测土耳其穆拉市(ATm)的日平均时间序列气温,首先通过 seq2seq 回归预测模块,开发了五种不同层结构的基于长短期记忆(LSTM)和门控递归单元(GRU)的深度学习神经网络模型。然后,根据性能评估指标,设计出基于 DL 层的最佳网络结构,并与小波变换(WT)算法(即 WT-DNN 模型)进行混合,以增强估计能力。为此,通过相关性分析,在考虑的潜在气象变量中,选取了2014年1月至2019年12月的日平均日照时数(SSD)(小时)、全球太阳辐射总量(TGSR)(千瓦时/平方米)和全球总日照强度(TGSI)(瓦特/平方米)作为预测ATm的最有效输入变量。为了避免过拟合和欠拟合问题,通过不同类型的超参数进行了不同的算法调整和试错程序。根据性能评估标准、对比图和总可学习参数(TLP)值,最新且独特的混合 WT-(LSTM × GRU)模型(即通过乘法层((times))耦合 LSTM 和 GRU 模型的混合 WT)被确认为最佳模型。在理想超参数下,该混合模型的 R2 = 0.94,RMSE = 0.56(℃),MBE = -0.5(℃),AICc = -382.01,在 2000 次迭代中的运行时间为 376(s)。然而,作为基准模型的标准单 LSTM 层网络模型的 R2 = 0.63,RMSE = 4.69 (°C),MBE = -0.89 (°C),AICc = 1021.8,在 2000 次迭代中的运行时间为 186 (s)。
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引用次数: 0
Long-term changes of surface ozone and ozone sensitivity over the North China Plain based on 2015–2021 satellite retrievals 基于 2015-2021 年卫星检索的华北平原地表臭氧和臭氧敏感性的长期变化
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2024-06-29 DOI: 10.1007/s11869-024-01598-z
Chuanyong Zhu, Yichao Gai, Zhenguo Liu, Lei Sun, Siyuan Fu, Kun Liu, Leifeng Yang, Guang Pan, Baolin Wang, Chen Wang, Na Yang, Zhisheng Li, Chongqing Xu, Guihuan Yan

Despite the implementation of stringent pollution control measures, surface ozone (O3) pollution remains a significant issue in the North China Plain (NCP) in recent years. Here we examined long-term changes in surface O3 concentrations during 2015–2021 in the NCP. The mean summer maximum daily 8-hour average ozone concentration exhibited an annual increase of 12.77 µg m− 3 (p < 0.01) from 2015 to 2019, followed by a decline from 174 µg m− 3 in 2019 to 157 µg m− 3 in 2021. Subsequently, satellite-based formaldehyde (HCHO) and nitrogen dioxide (NO2) columns were used to track volatile organic compounds (VOCs) and nitrogen oxides (NOx) emissions to evaluate the causes of O3 changes. Results showed that the increase of HCHO column and the sharp decline of NO2 column have indeed led to no decrease in O3 concentration and even contributed to O3 enhancement in most areas in 2015–2019. However, the sharp decline of HCHO and NO2 columns contributed to the decline of O3 concentration since 2020. The HCHO/NO2 values showed a transitional regime ranging from 4.23 to 5.05 and the O3 sensitivities were predominantly VOC-limited and transitional regimes in 2019–2021, varying among different mega-city clusters. The HCHO/NO2 increased from 2.62 ± 2.41 in 2015 to 2.99 ± 3.49 in 2019 but decreased since then, facilitating O3 formation regime transition from NOx-limited to transitional (or from transitional to VOC-limited) regimes, which contributed to the decline in O3 levels. The study determined that the optimal ratio of HCHO to NO2 for reducing O3 concentration is 4.66 for the NCP.

尽管实施了严格的污染控制措施,但近年来华北平原(NCP)的地表臭氧(O3)污染仍然是一个重要问题。在此,我们研究了华北平原 2015-2021 年间地表臭氧浓度的长期变化。从2015年到2019年,夏季最大日均8小时臭氧浓度年均上升12.77微克/立方米(p < 0.01),随后从2019年的174微克/立方米下降到2021年的157微克/立方米。随后,利用基于卫星的甲醛(HCHO)和二氧化氮(NO2)柱跟踪挥发性有机化合物(VOCs)和氮氧化物(NOx)的排放,以评估臭氧变化的原因。结果表明,2015-2019年,HCHO柱的增加和NO2柱的急剧下降确实没有导致O3浓度的下降,甚至在大部分地区导致了O3浓度的升高。然而,自 2020 年以来,HCHO 和 NO2 柱的急剧下降导致了 O3 浓度的下降。2019-2021年,HCHO/NO2值呈现出4.23-5.05的过渡机制,O3敏感性主要为VOC限制和过渡机制,不同特大城市群之间存在差异。HCHO/NO2从2015年的2.62±2.41上升到2019年的2.99±3.49,但此后有所下降,促进了O3形成机制从氮氧化物限制型向过渡型(或从过渡型向挥发性有机物限制型)过渡,这也是O3水平下降的原因之一。研究确定,在国家清洁计划中,降低 O3 浓度的最佳 HCHO 与 NO2 比率为 4.66。
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引用次数: 0
Ozone production sensitivity in the highland city of Lhasa: a comparative analysis with Beijing 高原城市拉萨的臭氧生成敏感性:与北京的比较分析
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2024-06-27 DOI: 10.1007/s11869-024-01604-4
Yi Chen, Suzhen Chi, Yaru Wang, Shuzheng Guo, Chong Zhang, Chunxiang Ye, Weili Lin

As Lhasa experiences accelerated urbanization and increased pollutant emission intensity, controlling ozone pollution becomes more challenging due to increased photochemical reactions—a problem exacerbated by the city’s already high solar UV radiation and background ozone levels. In order to reveals the intricacies of ozone formation, this study conducted direct ozone production rate (OPR) measurements in Lhasa in June 2021, comparing them to findings in Beijing in similar climatic conditions. Despite lower NOx levels, Lhasa exhibited a higher OPR with reduced variations (12.8 ± 6.0 ppbv h-1) due to stronger UVR and OH reactivity (VOC-kOH) influenced by oxidized volatile organic compounds when compared to Beijing (9.4 ± 11.0 ppbv h-1). When adjusting for comparable UVR conditions, Lhasa demonstrated a less pronounced NO turning point in OPR compared to Beijing. Lhasa’s unique bridge-shaped VOC-kOH diel variation favored daytime peroxy radical production, pushing the NO turning point higher from morning to noon, resulting in a NOx-limited regime except in the early morning. Furthermore, the accumulation of OVOCs in the Lhasa River valley, coupled with rapid photochemical production despite relatively low VOCs emissions, explained the elevated VOC-kOH levels. This suggests that OVOCs and, consequently, O3 pollution could worsen with future VOCs emission increases, possibly triggered by factors like rapid warming and local afforestation initiatives. Our findings highlight the complex and sensitive nature of O3 pollution in Lhasa and other Tibetan Plateau cities, emphasizing the need for continued monitoring and in-depth research to develop effective control strategies.

随着拉萨城市化进程的加快和污染物排放强度的增加,由于光化学反应的加剧,控制臭氧污染变得更具挑战性。为了揭示臭氧形成的复杂性,本研究于 2021 年 6 月在拉萨进行了臭氧生成率(OPR)的直接测量,并将其与气候条件相似的北京的测量结果进行了比较。与北京(9.4 ± 11.0 ppbv h-1)相比,尽管拉萨的氮氧化物水平较低,但由于受氧化挥发性有机化合物的影响,紫外线辐射和羟基反应(VOC-kOH)较强,拉萨的臭氧生成率较高,且变化较小(12.8 ± 6.0 ppbv h-1)。在调整可比紫外线辐射条件后,与北京相比,拉萨在 OPR 方面的 NO 转折点并不明显。拉萨独特的桥形 VOC-kOH 日间变化有利于白天过氧自由基的产生,从而将 NO 拐点从早晨推高到中午,导致除清晨外的 NOx 限制机制。此外,拉萨河流域 OVOCs 的积累,加上尽管 VOCs 排放量相对较低但光化学生成迅速,也解释了 VOC-kOH 水平升高的原因。这表明,随着未来 VOCs 排放量的增加,OVOCs 以及随之而来的 O3 污染可能会恶化,而这可能是由快速变暖和当地植树造林活动等因素引发的。我们的研究结果凸显了拉萨和其他青藏高原城市臭氧污染的复杂性和敏感性,强调了持续监测和深入研究以制定有效控制策略的必要性。
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引用次数: 0
Evaluation of size–segregated bioaerosols concentration, deposition fraction and inhalation dose in individuals of an educational institute: a case study for health risk assessment 评估一所教育机构中生物气溶胶的大小分隔浓度、沉积分数和个人吸入剂量:健康风险评估案例研究
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2024-06-26 DOI: 10.1007/s11869-024-01601-7
Chirashree Ghosh, Kritika Bisht, Ankita Shelly, Rekha Kumari

Bioaerosols, airborne biological particles, are present ubiquitously in nature. When inhaled, ingested, or exposed to the skin, can pose various health risks. Bioaerosols sampling is crucial for educational institutes in view of high occupancy, long exposure duration and proximity between occupants. A comprehensive study was designed to determine size-segregated bioaerosols concentration, size-wise deposition fraction, and the dose inhaled by the exposed population. The bacterial and fungal bioaerosols concentrations were measured at 4 locations viz. undergraduate laboratory (IN 1), Molecular Biotechnology and Bioinformatics Laboratory (IN 2), college nursery (OUT 1) and open cafeteria (OUT 2). Sampling was conducted using a 6-stage viable Andersen cascade impactor and culturable bioaerosols were counted by colony counting method. The highest average concentrations of bacterial and fungal bioaerosols were found in IN 1 and OUT 1. The bioaerosols concentration was influenced by a complex interplay of factors, majorly including ventilation, footfall, occupancy, and surrounding vegetation. The size distribution analysis showed that a significant portion was in the respirable size range (< 4.5 μm), capable of reaching the lower respiratory tract and causing potential health issues. The dosimetry modelling further assisted in predicting the bioaerosols dose deposition in different regions of the human respiratory tract. Subsequently, to discern the connection between bioaerosols exposure and respiratory ailments, bioaerosols exposure awareness and health survey was conducted for individuals in the vicinity of sampling locations. The knowledge garnered from the study can make the basis for the health risk assessment due to bioaerosols exposure in educational environments to appraise potential health hazards.

Graphical Abstract

生物气溶胶,即空气中的生物微粒,在自然界中无处不在。一旦吸入、摄入或接触到皮肤,就会对健康造成各种危害。生物气溶胶采样对教育机构来说至关重要,因为教育机构的入住率高,接触时间长,而且入住者之间距离很近。我们设计了一项综合研究,以确定生物气溶胶的大小分隔浓度、大小沉积分数以及暴露人群的吸入剂量。细菌和真菌生物气溶胶浓度是在 4 个地点测量的,即本科生实验室(IN 1)、分子生物技术和生物信息学实验室(IN 2)、学院苗圃(OUT 1)和开放式食堂(OUT 2)。使用 6 级安徒生级联冲击器进行采样,并采用菌落计数法对可培养的生物气溶胶进行计数。细菌和真菌生物气溶胶的平均浓度在 IN 1 和 OUT 1 中最高。生物气溶胶浓度受多种复杂因素的影响,主要包括通风、人流量、占用率和周围植被。粒径分布分析表明,相当大一部分属于可吸入粒径范围(< 4.5 μm),能够进入下呼吸道,造成潜在的健康问题。剂量测定模型进一步帮助预测了生物气溶胶在人体呼吸道不同区域的剂量沉积。随后,为了确定生物气溶胶暴露与呼吸系统疾病之间的联系,对采样地点附近的个人进行了生物气溶胶暴露意识和健康调查。从这项研究中获得的知识可作为评估教育环境中生物气溶胶暴露造成的健康风险的基础,以评估潜在的健康危害。
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引用次数: 0
Evaluation of air pollution tolerance index of urban roadside young leaf and the correlation with its capturing capacity for water-insoluble fine particulate matters 城市路边嫩叶的空气污染耐受指数及其与水不溶性细颗粒物捕获能力的相关性评价
IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Pub Date : 2024-06-25 DOI: 10.1007/s11869-024-01603-5
Chen He, Zhuofan Zhang, Qi Wang, Yupeng Zhang, Chenhui Wei, Lin Zhang, Zhuo Li, Hongqian Yu, Chunyan Chang, Yilong Zhang

The selection of plant species has been accepted as a crucial factor when developing roadside greenbelts which act as a cost-effective and eco-friendly passive method for the reduction of traffic related particle pollution. Plants growing alongside roads are mostly affected because they are primary recipients to different pollutants and show varied sensitivity and tolerance. Taking this into account, young leaves of eight kinds of common roadside plants (Ligustrum lucidum, Prunus cerasifera, Photinia fraseri, Photinia serratifolia, Nandina domestica, Paeonia suffruticosa Andr., Nerium oleander, and Eriobotrya japonica) in central China were collected and their air pollution tolerance index (APTI) was calculated by assessing four biochemical parameters i.e., relative water content, total chlorophyll content, ascorbic acid, leaf extract pH. The results demonstrated that young leaves of N. oleander and L. lucidum showed higher APTI value (8.90–9.45 and 8.73 to 9.17 respectively) in the three tested springtime month and were the most tolerant species, while young leaves of E. japonica kept to be sensitive (with the APTI value around 5.72 to 8.29) during the whole spring. In addition, inconsistent with previous studies, relative water content other than ascorbic acid was found to be more crucial for young leaves of test plants to be more tolerant to particle pollution in relatively dry condition in spring (r = 0.996 at p < 0.01 level). At last, except significant impact on the capture of PM2.5, the tolerance of young leaves has limited impacts on their ability to reduce other size fine particle such as TSP and PM10. In summary, N. oleander and L. lucidum are recommended to be used as particle sink when developing urban green belt, and E. japonica is more suitable as a bio-monitor of air quality.

在开发路边绿化带时,植物物种的选择被认为是一个至关重要的因素,因为路边绿化带是减少与交通有关的颗粒污染的一种具有成本效益和生态友好型的被动方法。生长在路边的植物大多会受到影响,因为它们是不同污染物的主要接受者,并表现出不同的敏感性和耐受性。有鉴于此,我们对八种常见的路边植物(女贞、苹果树、蕨类光照植物、绢叶光照植物、南丹、芍药和夹竹桃)的嫩叶进行了研究、通过评估相对含水量、总叶绿素含量、抗坏血酸和叶提取物 pH 值这四个生化参数,计算了它们的空气污染耐受指数(APTI)。结果表明,夹竹桃和露珠草的嫩叶在测试的三个春季月份中都显示出较高的 APTI 值(分别为 8.90-9.45 和 8.73-9.17),是耐受性最强的物种,而荏苒粳稻的嫩叶在整个春季都保持敏感(APTI 值约为 5.72-8.29 )。此外,与之前的研究不一致的是,在春季相对干燥的条件下,相对含水量(抗坏血酸除外)对试验植物幼叶对颗粒物污染的耐受性更为关键(r = 0.996,p < 0.01水平)。最后,除了对捕获 PM2.5 有显著影响外,幼叶的耐受性对其减少其他粒径的细颗粒物(如 TSP 和 PM10)的能力影响有限。总之,在发展城市绿化带时,建议将夹竹桃和露珠草用作颗粒物汇,而荏苒更适合用作空气质量的生物监测器。
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Air Quality Atmosphere and Health
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