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Hyperspectral dark-field optical microscopy correlated to atomic force microscopy for the analysis of single plasmonic nanoparticles: tutorial 与原子力显微镜相关的高光谱暗场光学显微镜用于分析单个等离子纳米粒子:教程
Pub Date : 2024-06-17 DOI: 10.1364/josab.523547
Claire Abadie, Mingyang Liu, Yoann Prado, Olivier Pluchery
Plasmonic nanostructures are actively investigated for their optical properties and for a wide range of applications in nanophotonics, biosensing, photocatalysis, hot carrier physics, and advanced cancer therapies. The localized surface plasmon resonance (LSPR) can be excited in gold or silver nanoparticles or in more complex nanostructures and gives rise to a wide range of unique optical properties. It is often critical to be able to localize individual plasmonic nanoparticles and simultaneously measure their spectrum. This is known as hyperspectral microscopy. In this tutorial, we describe and carefully explain how to achieve this goal with an optical microscope equipped with a dark-field objective and an optical spectrometer. The images and the scattering spectra of spherical gold nanoparticles with diameters of 90, 70, 50, and 25 nm are recorded. We compare them with the scattering spectra predicted with the Mie formula (LSPR peaks measured at 553, 541, 535, and 534 nm, respectively). The optical images are limited by the diffraction, and this is discussed in the framework of the Abbe equation. We also describe a strategy to easily correlate the optical images with atomic force microscope images of the samples. This allows us to precisely relate the morphology of the nanoparticles with their optical images, their color, and their optical spectrum. The case of non-spherical nanostructures, namely, dimers of nanoparticles, is also discussed. This approach allows a relatively low-cost setup and efficient characterization method that will be helpful for teachers who want to introduce their students to the wide topics of plasmonics. This will also be useful for labs seeking an affordable method to investigate the plasmonic properties of single nanostructures.
人们正在积极研究等离子纳米结构的光学特性,并将其广泛应用于纳米光子学、生物传感、光催化、热载流子物理学和先进的癌症疗法。局部表面等离子体共振(LSPR)可在金或银纳米粒子或更复杂的纳米结构中激发,并产生各种独特的光学特性。能够定位单个等离子纳米粒子并同时测量其光谱往往至关重要。这就是所谓的高光谱显微技术。在本教程中,我们将描述并仔细讲解如何使用配备暗视野物镜和光学光谱仪的光学显微镜来实现这一目标。我们记录了直径分别为 90、70、50 和 25 纳米的球形金纳米粒子的图像和散射光谱。我们将它们与用米氏公式预测的散射光谱(分别在 553、541、535 和 534 纳米处测得 LSPR 峰值)进行了比较。光学图像受到衍射的限制,我们将在阿贝方程的框架内对此进行讨论。我们还介绍了一种将光学图像与样品的原子力显微镜图像轻松关联起来的策略。这样,我们就能将纳米粒子的形态与它们的光学图像、颜色和光谱精确地联系起来。我们还讨论了非球形纳米结构(即纳米粒子的二聚体)的情况。这种方法可以实现相对低成本的设置和高效的表征方法,对希望向学生介绍等离子体学广泛主题的教师很有帮助。这也将有助于实验室寻找一种经济实惠的方法来研究单个纳米结构的等离子特性。
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引用次数: 0
Multi-hop fault-tolerant teleportation of arbitrary two-qubit states with cluster channel 利用集群信道实现任意双量子比特态的多跳容错远程传输
Pub Date : 2024-06-17 DOI: 10.1364/josab.523965
TianTian Meng, YuZhen Wei, Hong Chen, Xu Huang, Min Jiang
In this paper, we propose one multi-hop fault-tolerant teleportation scheme leveraging non-maximally entangled cluster states as the quantum channel, which is crucial for efficient transmission over extended distances. During quantum communication, environmental noise may introduce operational errors between adjacent nodes. In order to uphold the maximum transmission efficiency, error correction operations are exclusively conducted by the ultimate receiver rather than intermediate nodes. Error outcomes from each node can be synchronously relayed to the receiver via the classical channel, effectively diminishing the delays and operational intricacies, thereby significantly bolstering the transmission efficiency. Moreover, we utilize the Quirk simulation software to simulate the teleportation process.
本文提出了一种多跳容错远程传输方案,利用非最大纠缠簇态作为量子信道,这对于远距离高效传输至关重要。在量子通信过程中,环境噪声可能会在相邻节点之间引入操作错误。为了保持最大的传输效率,纠错操作完全由最终接收器而非中间节点进行。各节点的纠错结果可通过经典信道同步传递给接收器,从而有效地减少了延迟和操作的复杂性,大大提高了传输效率。此外,我们还利用 Quirk 仿真软件来模拟远距离传输过程。
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引用次数: 0
First-principles simulations of high-order harmonics generation in thin films of wide bandgap materials [Invited] 宽带隙材料薄膜中高阶谐波产生的第一原理模拟 [特邀]
Pub Date : 2024-06-13 DOI: 10.1364/josab.512444
Albert Mathew, Sergey Kruk, Shunsuke Yamada, Kazuhiro Yabana, Anatoli Kheifets
High-order harmonics generation (HHG) is the only process that enables tabletop-sized sources of extreme ultraviolet (XUV) light. The HHG process typically involves light interactions with gases or plasma––material phases that hinder wider adoption of such sources. This motivates the research in HHG from nanostructured solids. Here, we employ the time-dependent density function theory (TDDFT) to investigate material platforms for HHG at the nanoscale using first-principles supercomputer simulations. We reveal that wide bandgap semiconductors, aluminum nitride (AlN) and silicon nitride (Si3N4), are highly promising for XUV light generation when compared to silicon, one of the most common nonlinear nanophotonic materials. In our calculations, we assume excitation with a 100 fs pulse duration, 1×1013W/cm2 peak power, and 800 nm central wavelength. We demonstrate that in AlN material the interplay between the crystal symmetry and the incident light direction and polarization can enable the generation of both even and odd harmonics. Our results should advance the development of high-harmonics generation of XUV light from nanostructured solids.
高阶谐波发生(HHG)是实现桌面大小的极紫外(XUV)光源的唯一工艺。高阶谐波发生(HHG)过程通常涉及光与气体或等离子体的相互作用--这些物质相阻碍了此类光源的广泛应用。这激发了对来自纳米结构固体的 HHG 的研究。在此,我们采用时间相关密度函数理论(TDDFT),利用第一原理超级计算机模拟研究纳米级 HHG 的材料平台。我们发现,与硅这种最常见的非线性纳米光子材料相比,氮化铝(AlN)和氮化硅(Si3N4)这两种宽带隙半导体在 XUV 光生成方面具有很高的前景。在计算中,我们假定激励脉冲持续时间为 100 fs,峰值功率为 1×1013W/cm2 ,中心波长为 800 nm。我们证明,在氮化铝材料中,晶体对称性与入射光方向和偏振之间的相互作用能够产生偶次谐波和奇次谐波。我们的研究成果将推动从纳米结构固体中产生高谐波 XUV 光的发展。
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引用次数: 0
Optical solitons in multimode fibers: recent advances 多模光纤中的光孤子:最新进展
Pub Date : 2024-06-10 DOI: 10.1364/josab.528242
Mario Zitelli
Optical solitons in multimode fibers were predicted 40 years ago and extensively investigated theoretically. Transmission experiments in nonlinear multimode fibers have gained renewed interest, motivated by their potential to extend the capacity of long-distance transmission systems; only in the last few years, new experiments have revealed unexpected properties of optical solitons propagating in graded-index and step-index multimode fibers, partially re-writing the existing theory. Here we provide an overview of the recent experimental, numerical, and theoretical studies that revealed those new properties. It will be shown that multimode fiber solitons form with specific pulse width and energy dependent on the wavelength, and that they naturally evolve toward fundamental-mode Raman solitons. New soliton fission mechanisms, governed by the modal dispersion, will be explained. Possible applications in space-division multiplexed systems will be discussed. A recent thermodynamic approach to soliton condensation will be described.
多模光纤中的光孤子早在 40 年前就已被预测,并得到了广泛的理论研究。在非线性多模光纤中进行的传输实验再次引起了人们的兴趣,因为它们具有扩展长距离传输系统容量的潜力;直到最近几年,新的实验才揭示了光孤子在梯度指数和阶梯指数多模光纤中传播时所具有的意想不到的特性,从而部分改写了现有理论。在此,我们将概述揭示这些新特性的最新实验、数值和理论研究。研究表明,多模光纤孤子的形成具有特定的脉冲宽度和能量,与波长有关,并自然地向基模拉曼孤子演化。还将解释由模态色散控制的新孤子裂变机制。还将讨论在空间分复用系统中的可能应用。此外,还将介绍孤子凝聚的最新热力学方法。
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引用次数: 0
Tutorial on nonperturbative cavity quantum electrodynamics: is the Jaynes–Cummings model still relevant? 非微扰空穴量子电动力学教程:杰恩斯-康明斯模型是否仍然适用?
Pub Date : 2024-06-05 DOI: 10.1364/josab.522786
Daniele De Bernardis, Alberto Mercurio, Simone De Liberato
In this tutorial review, we briefly discuss the role that the Jaynes–Cummings model occupies in present-day research in cavity quantum electrodynamics with a particular focus on the so-called ultrastrong-coupling regime. We start by critically analyzing the various approximations required to distill such a simple model from standard quantum electrodynamics. We then discuss how many of those approximations can be, and often have been, broken in recent experiments. The consequence of these failures has been the need to abandon the Jaynes–Cummings model for more complex models. In this, the quantum Rabi model has the most prominent role, and we will rapidly survey its rich and peculiar phenomenology. We conclude the paper by showing how the Jaynes–Cummings model still plays a crucial role even in nonperturbative light–matter coupling regimes.
在这篇教程综述中,我们将简要讨论杰恩斯-康明斯模型在当今空穴量子电动力学研究中所扮演的角色,并特别关注所谓的超强耦合机制。我们首先批判性地分析了从标准量子电动力学中提炼出这样一个简单模型所需的各种近似值。然后,我们讨论在最近的实验中,这些近似如何被打破,而且经常被打破。这些失败的后果就是需要放弃杰恩斯-康明斯模型,转而采用更复杂的模型。其中,量子拉比模型的作用最为突出,我们将迅速考察其丰富而奇特的现象学。在本文的最后,我们将展示杰恩斯-康明斯模型是如何在非微扰光-物质耦合机制中发挥关键作用的。
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引用次数: 0
Spectral and dynamical validity of the rotating-wave approximation in the quantum and semiclassical Rabi models [Invited] 量子和半经典拉比模型中旋转波近似的光谱和动力学有效性 [特邀]
Pub Date : 2024-06-04 DOI: 10.1364/josab.524837
H. F. A. Coleman, E. K. Twyeffort
Ultrastrong coupling (USC) in the quantum Rabi model, characterized by the breakdown of the rotating-wave approximation (RWA), has emerged as a topic of considerable interest and study. This critical reevaluation of the validity of the RWA concludes that the accepted definition of USC in terms of a fixed ratio of coupling to field frequency is inadequate. Connecting an improved spectral validity criterion with the derivation of the semiclassical limit suggests that the dynamical validity of the quantum RWA should be linked to that of the corresponding semiclassical model. This, however, is not supported by numerical calculations of coherent-state dynamics, which unambiguously demonstrate that spectral validity does not imply dynamical validity and reveal surprisingly complicated dependence on coupling and field amplitude.
量子拉比(Rabi)模型中的超强耦合(USC)以旋转波近似(RWA)的崩溃为特征,已成为一个颇受关注和研究的课题。这篇对旋转波近似有效性的批判性重新评估得出的结论是,以耦合与场频的固定比率来定义超强耦合是不充分的。将改进的频谱有效性标准与半经典极限的推导联系起来,表明量子 RWA 的动态有效性应与相应的半经典模型的动态有效性联系起来。然而,相干态动力学的数值计算并不支持这一点,它明确地证明了频谱有效性并不意味着动力学有效性,而且揭示了与耦合和场振幅之间令人惊讶的复杂依赖关系。
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引用次数: 0
Radial quadrature method for evaluating the beam shape coefficients of the Laguerre–Gaussian beam 评估拉盖尔-高斯光束形状系数的径向正交法
Pub Date : 2024-05-30 DOI: 10.1364/josab.525649
Mengyang Wang, Siqi Tang, Jianqi Shen
Calculation of the beam shape coefficients (BSCs) is crucial in analyzing the interaction between the shaped beam and spherical particle. In this paper, the radial quadrature method is used to formulate the BSCs of the Laguerre–Gaussian beam. The expressions of the BSCs for the Laguerre–Gaussian beam are obtained in terms of integrals, infinite series, and FS. It is proved that the FS expressions of the BSCs are the same as those achieved in the FS technique. The validity of the BSCs is numerically checked in the BSC calculation and the beam’s reconstruction. It is concluded that the infinite series expressions of the radial quadrature BSCs are efficient and reliable.
光束形状系数(BSCs)的计算对于分析异形光束与球形粒子之间的相互作用至关重要。本文采用径向正交法来计算 Laguerre-Gaussian 光束的 BSCs。通过积分、无穷级数和 FS 得到了拉盖尔-高斯光束的 BSCs 表达式。实验证明,BSCs 的 FS 表达式与 FS 技术中的表达式相同。在 BSC 计算和光束重建中对 BSC 的有效性进行了数值检验。结论是径向正交 BSC 的无穷序列表达式是高效可靠的。
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引用次数: 0
Experimental neodymium-doped microlaser with theoretical analysis of the thermo-optic effect 掺钕微激光实验及热光效应理论分析
Pub Date : 2024-05-30 DOI: 10.1364/josab.524249
Huibo Fan, Xinrui Chen, Huili Fan, Arui Wang, Ruijuan Chang
Ultralow-threshold laser emission from a neodymium-doped silica toroidal microcavity is theoretically analyzed and experimentally demonstrated, along with the detailed analysis and compensation of the thermo-optic effect in this microlaser system. The threshold power and slope efficiency of microlaser emission are derived based on coupled-mode theory and analytic formulas, associated with the demonstration of their dependence on neodymium ion concentration and the quality factor of the microtoroid. In the experiment, a single-mode laser and multi-mode laser with threshold power as low as 1.6 µW at the wavelength of 1064 nm band are obtained via changing the coupling condition of the cavity-tapered fiber system, resonant pump wavelength, and pump power, respectively. The single-mode laser emission at the 910 nm band is also realized with the threshold power of about 108.5 µW. Furthermore, considering the potential application, non-resonant pumping for the laser emission at the 1064 nm band is characterized with threshold power of 137 µW due to the influence of the thermo-optic effect and low slope efficiency of non-resonant pumping. By coating UV-glue with a negative thermo-optic coefficient on the microtoroid surface, the compensation of the thermo-optic effect of the microtoroid is analyzed theoretically, which on the other hand can also be used for the potential application of high-sensitivity temperature sensing with sensitivity of −0.138nm/C.
对掺钕二氧化硅环形微腔的超低阈值激光发射进行了理论分析和实验演示,并对该微激光系统中的热光学效应进行了详细分析和补偿。根据耦合模式理论和解析公式推导出了微激光发射的阈值功率和斜率效率,并证明了它们与钕离子浓度和微空腔品质因数的关系。实验中,通过改变腔锥形光纤系统的耦合条件、谐振泵浦波长和泵浦功率,分别获得了波长为 1064 nm 波段、阈值功率低至 1.6 µW 的单模激光器和多模激光器。此外,还实现了 910 nm 波段的单模激光发射,阈值功率约为 108.5 µW。此外,考虑到潜在的应用,由于热光学效应的影响和非谐振泵浦的低斜率效率,用于 1064 nm 波段激光发射的非谐振泵浦的阈值功率为 137 µW。通过在微晶体表面涂覆具有负热光系数的紫外线胶水,从理论上分析了补偿微晶体热光效应的方法,另一方面,这种方法也可用于灵敏度为 -0.138nm/∘C 的高灵敏度温度传感的潜在应用。
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引用次数: 0
Double-excitation transfer in dimer and trimer three-level systems using laser pulses and single photons 利用激光脉冲和单光子在二聚体和三聚体三电平系统中进行双激发转移
Pub Date : 2024-05-30 DOI: 10.1364/josab.523990
Abuenameh Aiyejina, Ethan Wyke, Roger Andrews, Andrew D. Greentree
We derive and simulate the wavefunctions and double-excitation probabilities for dimer and trimer three-level systems. Perfect state transfer occurs for pulse strengths that are odd multiples of π/2 when the parameter Jt equals odd multiples of π/2 and π/2 for the dimer and trimer, respectively. Near-perfect state transfer with a single photon occurred for photon coupling strength g=2J when Jt=1.99,19.87 in the dimer and Jt=2.62,25.51 in the trimer. The nature of perfect state transfer is due to localization and transfer of double excitations for given pulse strengths and times.
我们推导并模拟了二聚体和三聚体三电平系统的波函数和双激发概率。当参数 Jt 分别等于二聚体和三聚体的 π/2 和 π/2 的奇数倍时,当脉冲强度为 π/2 的奇数倍时,会发生完美的状态转移。当二聚体中的 Jt=1.99,19.87 和三聚体中的 Jt=2.62,25.51 时,光子耦合强度 g=2J 的单光子发生了近乎完美的状态转移。在给定的脉冲强度和时间下,完美状态转移的本质是双激发的定位和转移。
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引用次数: 0
Non-classical correlations of light in the Jaynes-Cummings model 杰尼斯-康明斯模型中的非经典光相关性
Pub Date : 2024-05-29 DOI: 10.1364/josab.523919
D. V. Maslennikov, V. Yu. Shishkov, E. S. Andrianov
The problems concerning the influence of spectral filters on the quantum properties of light have recently attracted great attention in connection with quantum cryptography and quantum data transmission. In this paper, we consider the influence of a spectral filter on the second-order coherence function of a field of a resonator mode and a two-level atom in the framework of the Jaynes-Cummings model. Since the Heisenberg equations for the operators of the field of the resonator mode and the atom can be solved exactly, it is possible to obtain exact analytical Fourier transformation of the dynamics of operators of the resonator mode and two-level atom. We demonstrate that the second-order coherence function of the resonator mode and the two-level atom is equal to zero for all possible frequencies in the spectrum of operator oscillations. We find the interbeam second-order coherence function between different frequencies of the Fourier spectrum and show that in the limit of a large number of quanta, it can take the values in the range from zero to two. Thus, non-classical correlations are formed between certain frequencies in the Fourier spectrum of emitted light. We demonstrate that in the limit of a large number of quanta in the resonator mode, when the filter sums up the frequencies near the resonator eigenfrequency, the second-order coherence function of the field of the resonator mode is not affected by the interaction with the two-level atom.
光谱滤波器对光的量子特性的影响问题最近在量子密码学和量子数据传输方面引起了极大关注。在本文中,我们在杰恩斯-康明斯模型的框架内考虑了光谱滤波器对共振模式场和两级原子的二阶相干函数的影响。由于共振模式场和原子算子的海森堡方程可以精确求解,因此可以得到共振模式和两级原子算子动态的精确分析傅里叶变换。我们证明了共振模和两级原子的二阶相干函数在算子振荡频谱的所有可能频率上都等于零。我们找到了傅立叶频谱不同频率之间的束间二阶相干函数,并证明在大量量子的情况下,它的取值范围从零到二。因此,发射光的傅立叶光谱中的某些频率之间形成了非经典的相关性。我们证明,在谐振器模式中存在大量量子的情况下,当滤波器将谐振器特征频率附近的频率相加时,谐振器模式场的二阶相干函数不会受到与两级原子相互作用的影响。
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引用次数: 0
期刊
Journal of the Optical Society of America B
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