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Role of Organic and Biochar Amendments on Enhanced Bioremediation of Soils Contaminated with Persistent Organic Pollutants (POPs) 有机和生物炭改良剂对持久性有机污染物污染土壤的生物修复作用
IF 8.1 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-06-04 DOI: 10.1007/s40726-025-00361-x
Shailja Sharma, Shiv Bolan, Santanu Mukherjee, Gianniantonio Petruzzelli, Francesca Pedron, Elisabetta Franchi, Wasana Fonseka, Hasintha Wijesekara, Liuwei Wang, Deyi Hou, Kadambot H. M. Siddique, Nanthi Bolan

Purpose of Review

This review provides a comprehensive understanding about the mechanisms and technologies for the enhanced remediation of persistent organic pollutants (POPs)-contaminated soils by organic and biochar amendments. This article discusses the practical implications in relation to degradation, mobility, and bioavailability of POPs in soils.

Recent Findings

The application of organic (and carbonaceous) amendment lead to changes in soil’s pH, OM, and soluble organic carbon levels which might shift POPs from solid to aqueous phases, increasing their availability for microbial breakdown. Biochar can be useful as an electron donor, acceptor, or shuttle for microorganisms that degrade POPs (via different biological or chemical reactions) apart from its high surface area and excellent sorption properties (π–π interactions).

Summary

Large amounts of organic such as composted manure, biosolids, municipal solid waste, and biochar amendments are utilized as a soil conditioner to enhance soil health and crop productivity as well as a source of carbon and nutrients, which can also impact the interactions of POPs in soil.

综述了有机和生物炭对持久性有机污染物(POPs)污染土壤的修复机制和技术的研究进展。本文讨论了持久性有机污染物在土壤中的降解、迁移和生物利用度的实际意义。最近的发现有机(和碳)改剂的应用导致土壤pH值、有机质和可溶性有机碳水平的变化,这可能使持久性有机污染物从固体相转变为水相,增加了它们对微生物分解的有效性。生物炭除了具有高表面积和优异的吸附特性(π -π相互作用)外,还可作为降解持久性有机污染物的微生物的电子供体、受体或穿梭体(通过不同的生物或化学反应)。大量有机肥料,如堆肥、生物固体、城市固体废物和生物炭改良剂被用作土壤调理剂,以增强土壤健康和作物生产力,同时也是碳和营养物质的来源,这也会影响土壤中持久性有机污染物的相互作用。
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引用次数: 0
The Paradox of Microplastic Removal in WWTP: Redistribution of Micropollutants in the Environment 污水处理厂微塑料去除的悖论:微污染物在环境中的再分配
IF 8.1 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-06-03 DOI: 10.1007/s40726-025-00370-w
Agata Zdarta, Guoqiang Li

Purpose of the Review

High amounts of microplastics (MPs) are collected and then disposed of in sewage treatment plants. This review aims to identify the effects of wastewater treatment processes on the physical and chemical properties of MPs as well as their fragmentation and ageing, which are rarely reported and have not yet been revised.

Recent Findings

The amount of microplastic particles introduced into the WWTP depends on many factors, such as the area and population, treatment processes, migration of people, and weather conditions. As a result, WWTP effluents were identified as the source of MP pollution. Selected treatment methods and chemicals used in wastewater treatment may contribute to the deterioration of MP.

Summary

The impact of individual physical, mechanical, and chemical factors on the fate of microplastics in the WWTP was analysed. In the case of preliminary and primary treatment processes, the fragmentation of MP particles is mainly affected by mechanical interactions such as physical abrasion and water shearing force. However, during tertiary treatment processes, chemical factors such as advanced oxidation processes, chlorination, and ozonation play a leading role in MP deterioration. The paradox of so-called microplastic removal in WWTPs has been highlighted, and the concept of defining wastewater treatment plants as sources of tertiary microplastic pollution has been proposed.

Graphical Abstract

研究目的大量的微塑料被收集并在污水处理厂处理。这篇综述旨在确定废水处理过程对MPs物理和化学性质的影响,以及它们的破碎和老化,这些很少被报道,也尚未被修订。最近的发现进入污水处理厂的微塑料颗粒的数量取决于许多因素,如地区和人口、处理过程、人口迁移和天气条件。结果表明,污水处理厂废水是MP污染的主要来源。废水处理中使用的特定处理方法和化学品可能会导致MP的恶化。摘要分析了各个物理、机械和化学因素对污水处理厂微塑料命运的影响。在初级和初级处理过程中,MP颗粒的破碎主要受物理磨损和水剪切力等力学相互作用的影响。然而,在三级处理过程中,化学因素如高级氧化过程、氯化和臭氧化在MP恶化中起主导作用。在污水处理厂中所谓的微塑料去除的悖论已经被强调,并且已经提出了将废水处理厂定义为三级微塑料污染源的概念。图形抽象
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引用次数: 0
Atmospheric Amines: Advances in Analytical Techniques, Emission Inventories, Regional Pollution, and Roles in New Particle Formation 大气胺:分析技术进展,排放清单,区域污染,以及在新粒子形成中的作用
IF 8.1 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-06-03 DOI: 10.1007/s40726-025-00364-8
Qi Yu, Nan Fu, Jiajia Lu, Yukai Zhang, Wei Du, Junfeng Wang

Purpose of Review

Amines, as atmospheric pollutants, significantly impact air quality, climate change, and human health because they readily react with acidic gases in the atmosphere to form secondary organic aerosols (SOA) and participate in the formation of fine particulate matter (PM2.5). This review summarizes the research progress on atmospheric amine, including analytical methods, emission inventory, and regional pollution, as well as their significance in the course of new particle formation (NPF).

Recent Findings

At present, the detection methods for amines mainly include chromatography and mass spectrometry, among which the development of online measurement technology helps to improve time resolution and research depth. The severe lack of field-measured emission factors has hindered the model’s simulation of amine effects. The concentration and main components of particulate amines show significant differences in different regions and seasons. The sulfuric acid (H2SO4)-H2O-amine ternary nucleation theory is widely recognized, but field measurements have also revealed the influence of other organic compounds. In general, amines have a critical impact on atmospheric chemical reactions, particularly their support in the generation of new particles and SOA, which makes them a vital factor in climate transform research.

Summary

This review not only provides the latest research findings on amines but also points out the deficiencies in current studies. It emphasizes the need for systematic research on the emissions, the mechanisms of NPF. The ultimate goal is to contribute to mitigating atmospheric pollution and protecting public health.

胺作为大气污染物,极易与大气中的酸性气体反应形成二次有机气溶胶(SOA)并参与细颗粒物(PM2.5)的形成,对空气质量、气候变化和人类健康产生重大影响。本文综述了大气中胺的研究进展,包括分析方法、排放清单和区域污染,以及它们在新颗粒形成过程中的意义。目前,胺类化合物的检测方法主要有色谱法和质谱法,其中在线测量技术的发展有助于提高时间分辨率和研究深度。严重缺乏现场测量的排放因子阻碍了模型对胺效应的模拟。颗粒物胺的浓度和主要成分在不同地区和季节存在显著差异。硫酸(H2SO4)-水胺三元成核理论得到广泛认可,但现场测量也揭示了其他有机化合物的影响。总的来说,胺类物质对大气化学反应有重要影响,特别是它们对新粒子和SOA生成的支持作用,这使它们成为气候变化研究中的重要因素。本文综述了胺类化合物的最新研究成果,并指出了目前研究的不足。强调有必要对NPF的排放、机制进行系统研究。最终目标是为减轻大气污染和保护公众健康作出贡献。
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引用次数: 0
The Impact of Dissolved Organic Matter in Natural Receiving Systems on the Formation Potential and Toxicity of Disinfection By-products: Insights from Origins, Chemical Properties, and Transformations 天然接收系统中溶解有机物对消毒副产物形成潜力和毒性的影响:从起源、化学性质和转化的见解
IF 8.1 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-06-02 DOI: 10.1007/s40726-025-00350-0
Wei-Yu Li, Yun Chen, Wen-Long Wang, Yan-Lin Chen, Qian-Yuan Wu

Purpose of Review

This study aims to examine the role of dissolved organic matter (DOM) as a key precursor to disinfection by-products (DBPs) in aquatic environments. Key objectives include elucidating how DOM sources, chemical properties, and environmental transformations influence DBP speciation and toxicity. The study also evaluates strategies for mitigating DBP risks in drinking water treatment and identifies critical knowledge gaps in linking DOM dynamics to DBP toxicity profiles.

Recent Findings

Recent studies highlight that the sources of DOM and its chemical characteristics, including SUVA254 and humification index (HIX), strongly influence disinfection by-product formation potential (DBPFP). Photochemical and microbial transformations significantly alter the reactivity of DOM, with photodegradation typically reducing DBPFP while biodegradation increasing it. Despite these findings, the relationship between DOM transformations and DBP toxicity remains underexplored. Advanced mass spectrometry and fluorescence-based techniques have improved the ability to characterize DOM, offering new insights into the molecular-level dynamics of DBP formation. While traditional water treatment methods remain essential, enhanced coagulation, adsorption, and advanced oxidation processes are increasingly necessary to efficiently remove DOM and mitigate DBP formation.

Summary

This review provides a comprehensive examination of the DOM-DBP relationship, offering insights into the speciation and toxicity of DBP. It is highlighted that the sources, chemical properties, and natural transformations of DOM complicate the DBP precursor pool, affecting DOM reactivity and DBP production during disinfection. Advances in analytical techniques could improve our understanding of molecular-level interactions between DOM and DBP. Future research should prioritize comprehensive DOM characterization and predictive models to link DOM subfractions with toxicity explicitly. Furthermore, enhanced removal strategies must be developed to balance disinfection efficacy with minimized health and ecological risks, thereby ensuring water quality safety.

摘要本研究旨在探讨水生环境中溶解性有机物(DOM)作为消毒副产物(DBPs)的关键前体的作用。主要目标包括阐明DOM来源、化学性质和环境转化如何影响DBP的形态和毒性。该研究还评估了减轻饮用水处理中DBP风险的策略,并确定了将DOM动力学与DBP毒性概况联系起来的关键知识空白。最近的研究表明,DOM的来源及其化学特性,包括SUVA254和腐殖化指数(HIX),对消毒副产物形成电位(DBPFP)有很大的影响。光化学和微生物转化显著改变DOM的反应性,光降解通常会降低DBPFP,而生物降解则会增加DBPFP。尽管有这些发现,DOM转化和DBP毒性之间的关系仍未得到充分探讨。先进的质谱技术和基于荧光的技术提高了表征DOM的能力,为DBP形成的分子水平动力学提供了新的见解。虽然传统的水处理方法仍然必不可少,但为了有效去除DOM和减缓DBP的形成,强化混凝、吸附和高级氧化工艺越来越必要。本文综述了DOM-DBP关系的全面研究,为DBP的形成和毒性提供了见解。强调DOM的来源、化学性质和自然转化使DBP前体池复杂化,影响了消毒过程中DOM的反应性和DBP的产生。分析技术的进步可以提高我们对DOM和DBP分子水平相互作用的理解。未来的研究应优先考虑全面的DOM表征和预测模型,以明确地将DOM亚组分与毒性联系起来。此外,必须制定强化的去除策略,以平衡消毒效果与最小化健康和生态风险,从而确保水质安全。
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引用次数: 0
Enhancing the Pollutant Removal Performance of Bacteria and Microalgae Through Random Mutagenesis Technology: A Comprehensive Review of Effect and Mechanism 通过随机诱变技术提高细菌和微藻的污染物去除性能:效果和机制综述
IF 8.1 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-05-31 DOI: 10.1007/s40726-025-00366-6
Zeyuan Wang, Yu Hong

Purpose of Review

This review intends to comprehensively introduce random mutagenesis technology and summarize the up-to-date advances for utilizing it to enhance the pollutant removal abilities of bacteria, microalgae, and microalgae-bacteria consortia. In addition, this review also proposes future improvement strategies to further enhance the strengthening effect of random mutagenesis technology.

Recent Findings

Environmental pollution caused by wastewater, residual antibiotics, and other pollutants has caused severe disservice to the ecosystem and the development of human society. Pure bacterial systems, pure microalgal systems, and microalgae-bacteria consortia have been extensively applied to treat pollutants because of their excellent treatment effects, low cost, and other preponderances. Nevertheless, the pollutant removal abilities of bacteria and microalgae are limited by the individual species characteristics and adverse environmental factors. Fortunately, random mutagenesis technology can effectively solve the above problems. At present, random mutagenesis technology has been proven to significantly improve the removal efficiency of bacteria and microalgae for pollutants such as nutrients, petroleum hydrocarbons, and CO2.

Summary

This review first systematically describes the overall research situation of random mutagenesis technology through the bibliometric tools and related literature. Then, the applications of random mutagenesis technology in enhancing the pollutant removal capacity of bacteria, microalgae, and microalgae-bacteria consortia are introduced, respectively. This review also innovatively summarizes the principles of enhancing the pollutant removal performance of microalgae and bacteria through random mutagenesis technology. The challenges this technology faces in the current research are analyzed in depth, and corresponding improvement methods are given.

Graphical Abstract

综述目的综述了随机诱变技术在提高细菌、微藻和微藻-菌群对污染物去除能力方面的最新研究进展。此外,本文还提出了未来的改进策略,以进一步提高随机诱变技术的强化效果。废水、抗生素残留等污染物造成的环境污染对生态系统和人类社会的发展造成了严重的危害。纯细菌系统、纯微藻系统和微藻-细菌联合体因其处理效果好、成本低等优势,在污染物处理中得到了广泛的应用。然而,细菌和微藻的污染物去除能力受到物种个体特征和不利环境因素的限制。幸运的是,随机诱变技术可以有效地解决上述问题。目前,随机诱变技术已被证明可以显著提高细菌和微藻对营养物、石油烃、CO2等污染物的去除效率。本文首先通过文献计量学工具和相关文献系统地介绍了随机诱变技术的总体研究现状。然后分别介绍了随机诱变技术在提高细菌、微藻和微藻-菌群对污染物去除能力方面的应用。本文还创新性地总结了利用随机诱变技术提高微藻和细菌对污染物去除性能的原理。深入分析了该技术在当前研究中面临的挑战,并给出了相应的改进方法。图形抽象
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引用次数: 0
A Comprehensive Review on the Impact of Black-Odorous Water Bodies on the Physiological Ecology of Vallisneria natans and Its Associated Microbial Community 黑臭水体对水蛭生理生态及相关微生物群落影响的综述
IF 6.4 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-05-16 DOI: 10.1007/s40726-025-00359-5
Fares Hamoud, Yazid Bedouh, Linda Saili, Fatma Zohra Mellouk, Sofiane Ali Rachedi, Ines Bekhouche

Purpose of Review

Black-odorous water bodies (BOWBs) pose significant environmental challenges, characterized by excessive nutrients, heavy metals, and organic pollutants that degrade aquatic ecosystems. This review examines the impact of BOWBs on the physiological ecology of Vallisneria natans, a submersed macrophyte known for its phytoremediation potential, and its associated biofilm microbial community.

Recent Findings

Vallisneria natans interacts symbiotically with biofilm communities, which facilitate nutrient cycling, pollutant degradation, and enhance overall plant health. However, pollutants like heavy metals, microplastics, pharmaceuticals, and pesticides disrupt this symbiotic relationship, leading to oxidative stress, impaired nutrient uptake, and reduced growth. These effects limit the effectiveness of V. natans in natural restoration processes, highlighting the need for targeted remediation strategies.

Summary

Understanding the complex interactions between V. natans and its biofilm community under the stress of BOWBs is essential for developing effective, eco-friendly restoration strategies. This review identifies key knowledge gaps and proposes future research directions to optimize restoration efforts in degraded aquatic systems.

黑臭水体(bowb)的特征是营养物质、重金属和有机污染物超标,对水生生态系统造成了严重的环境挑战。本文综述了bowb对水蛭藻生理生态的影响及其相关生物膜微生物群落。水蛭藻是一种以植物修复潜力而闻名的水下大型植物。研究结果表明,南芥与生物膜群落共生,促进养分循环、污染物降解和植物整体健康。然而,重金属、微塑料、药物和农药等污染物破坏了这种共生关系,导致氧化应激、营养吸收受损和生长减缓。这些影响限制了水草在自然恢复过程中的有效性,强调了有针对性的修复策略的必要性。了解bowb胁迫下紫菀与其生物膜群落之间复杂的相互作用,对于制定有效的生态修复策略至关重要。本文总结了退化水生系统修复的关键知识缺口,并提出了未来的研究方向。
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引用次数: 0
A Data-Driven Analysis to Identify Research Hotspots and Trends in the Treatment of Algal Toxins in Water Environment
IF 6.4 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-05-13 DOI: 10.1007/s40726-025-00356-8
Zhao Xue, Lili Jin, Longhao Zhang, Junjie Lu, Naiyuan Zuo, Xiangzhou Sun, Hui Huang, Hongqiang Ren

Purpose of Review

Over the past 2 decades, due to eutrophication and other factors, algal toxins in water bodies have become increasingly prevalent, posing a significant threat to aquatic ecosystems and human health. The complex properties of algal toxins and the potential environmental risks they pose urgently demand comprehensive research and effective solutions. 

Recent Findings

Currently, the methods to address this issue mainly cover physical, chemical, and biological means. Oxidation, photocatalysis, and adsorption have emerged as the primary techniques. However, each has its own advantages and disadvantages in terms of removal efficiency, cost, and environmental impact. Previous studies were mostly small-scale laboratory explorations and failed to analyze the overall research trends of algal toxins from a macroscopic perspective. This study, by employing bibliometrics and patent analysis methods, comprehensively examines the research status and development trends of treating algal toxins in water. 

Summary

This study carried out a data-driven analysis of 3354 papers and 380 patents from the Web of Science Core Collection and Derwent Innovation Index databases up until 2023. The keyword co-occurrence network analysis and technology classification jointly revealed the main knowledge structure of algal toxin research, which is formed and interconnected by contaminants, treatment processes, toxicity, and degradation characteristics. Moreover, current research indicates that oxidation, photocatalysis, and adsorption are the main removal methods. Further exploration found that hot areas include the low-carbon degradation of algal toxins in eutrophic waters. In recent years, cylindrospermopsin and nodularin have become hot pollutants in algal toxin treatment. Currently, the research focuses more on the removal mechanism of algal toxins and the risk assessment under the exposure to cylindrospermopsin and nodularin. This study also summarizes the removal efficiencies and principles of physical, chemical, and biological methods in the algal toxin removal process, providing key information and guidance for researchers to have a deeper understanding of the field of treating algal toxins in water. 

近20年来,由于水体富营养化等因素的影响,水体中藻类毒素日益普遍,对水生生态系统和人类健康构成了重大威胁。藻类毒素的复杂特性及其潜在的环境风险迫切需要全面的研究和有效的解决方案。目前,解决这一问题的方法主要包括物理、化学和生物手段。氧化、光催化和吸附已成为主要的技术。然而,在去除效率、成本和环境影响方面,每种方法都有自己的优缺点。以往的研究多为小规模的实验室探索,未能从宏观角度分析藻类毒素的整体研究趋势。本研究采用文献计量学和专利分析法,全面考察了水体藻类毒素处理的研究现状和发展趋势。本研究对Web of Science核心馆藏和Derwent创新指数数据库中截至2023年的3354篇论文和380项专利进行了数据驱动分析。关键词共现网络分析和技术分类共同揭示了藻毒素研究的主要知识结构,该知识结构是由污染物、处理工艺、毒性和降解特性形成并相互关联的。此外,目前的研究表明,氧化、光催化和吸附是主要的去除方法。进一步探索发现热点领域包括富营养化水体中藻类毒素的低碳降解。近年来,藻毒素处理的热点污染物是柱精子素和结节素。目前的研究主要集中在藻毒素的去除机制以及暴露于柱精子素和结节素下的风险评估。本研究还总结了藻毒素去除过程中物理、化学和生物方法的去除效率和原理,为研究人员深入了解水中藻毒素处理领域提供了关键信息和指导。
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引用次数: 0
Bioaerosols in Various Working and Living Environments and Their Control Measure: A Review 各种工作和生活环境中的生物气溶胶及其控制措施综述
IF 6.4 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-04-26 DOI: 10.1007/s40726-025-00354-w
Ke Lu, Jiali Zhang, Zhe Li, Yanpeng Li

Purpose of Review

This review aims to reveal the pollution characteristics of bioaerosols across various working and living environments and evaluate existing control technologies. This will help enhance public awareness of bioaerosol pollution and the available control methods, and promote the diversity, efficiency, and operability of these technologies.

Recent Findings

Bioaerosols exhibit varying concentrations and community distributions across different environments due to diverse emission sources and environmental factors. Exposure to airborne pathogens poses health hazards, highlighting necessity for efficient antimicrobial techniques. While various technologies exhibit effective bactericidal capabilities, they also encounter numerous limitations in practical applications.

Summary

It is crucial to establish microbial risk assessment methods and develop efficient and low-cost control measures across various fields to create safe and healthy environments. This work lays the foundation for future research on bioaerosol pollution and control technologies, offering valuable insights for bioaerosol management and the protection of public health.

本文旨在揭示生物气溶胶在各种工作和生活环境中的污染特征,并对现有的控制技术进行评价。这将有助于提高公众对生物气溶胶污染和现有控制方法的认识,并促进这些技术的多样性、效率和可操作性。由于不同的排放源和环境因素,生物气溶胶在不同的环境中表现出不同的浓度和群落分布。暴露于空气传播的病原体会对健康造成危害,这突出了高效抗菌技术的必要性。虽然各种技术表现出有效的杀菌能力,但在实际应用中也遇到了许多限制。建立微生物风险评估方法,制定跨领域高效、低成本的控制措施,创造安全、健康的环境至关重要。本研究为今后生物气溶胶污染与控制技术的研究奠定了基础,为生物气溶胶管理和公众健康保护提供了有价值的见解。
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引用次数: 0
Next Generation Air Quality Models: Dynamical Mesh, New Insights into Mechanism, Datasets and Applications 下一代空气质量模型:动态网格,机制,数据集和应用的新见解
IF 6.4 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-04-26 DOI: 10.1007/s40726-025-00355-9
Jinxi Li, Yijie Li, Zifa Wang, Jiang Zhu, Lei Kong, Jie Li, Huangjian Wu, Leisheng Li, Xiao Tang, Zhen Cheng, Lanyi Zhang, Pu Gan, Xiaole Pan, Wenyi Yang, Kai Cao, Jie Zheng

Purpose of Review

Air quality modelling and forecasting have been well recognised to play important roles in environmental research as well as government policy assessments and management strategies. To address the recent progresses in air quality modelling, we conduct a literature review focusing on air quality forecasting models and reanalysis datasets.

Recent Findings

First of all, the implementation of three-dimensional adaptive meshes/horizontal resolution-variable grids in air quality models offers a crucial insight on multi-scale simulations down to the hectometre level. These models balance high accuracy with computational efficiency. Secondly, current reanalysis still has limitations in its horizontal resolution (dozens of kilometres) that are insufficient to support the analysis and management of air pollution at factory levels or neighbourhood scales. The development of adaptive mesh resolution method provides a promising way to deal with this issue and allows the construction of the chemistry reanalysis at ultra-high resolutions (< 1 km). However, the use of adaptive mesh method in data assimilation is currently still restricted to the column-based one-dimensional models. Thirdly, the application of graphics processing units to air quality predictions enables more optimised resource usage and enhances model performance through hardware acceleration effects, while machine learning methods can both maintain the consistency with numerical solutions and increase the accuracy of air quality predictions for specific chemical species. Furthermore, parameters that describe more complicated processes and mechanisms have been added into pre-existing physical and chemical parameterisations to enable more accurate representation of various small-scale features, such as the parameterisation of inorganic chemistry on the surface of aerosols, as well as various photolysis schemes.

Summary

The increase of resolution brings computational burdens and shifts the boundary of resolved and sub-grid phenomena in air quality prediction, which in turn stimulates the development and usage of new technologies (e.g. adaptive mesh techniques, graphics processing unit acceleration, machine learning methods). They are conducive to the improvement of prediction accuracies and the acquisition of new insights on atmospheric physical and chemical mechanisms. However, new challenges also ensued, including the selection criteria for mesh refinement, the acquisition of high-resolution observational data and the integration of artificial intelligence-hybrid air quality models. More efforts are required to develop the adaptive irregular mesh grid data assimilation method to overcome the resolution problems of current chemical reanalysis.

研究目的空气质素模拟及预测在环境研究、政府政策评估及管理策略中扮演重要角色。为了解决空气质量模型的最新进展,我们对空气质量预测模型和再分析数据集进行了文献综述。首先,在空气质量模型中实施三维自适应网格/水平分辨率可变网格为低至百米水平的多尺度模拟提供了至关重要的见解。这些模型平衡了高精度和计算效率。其次,目前的再分析在水平分辨率(几十公里)上仍然有局限性,不足以支持工厂水平或社区尺度上的空气污染分析和管理。自适应网格分辨率方法的发展为解决这一问题提供了一种有希望的方法,并允许在超高分辨率(< 1 km)下构建化学再分析。然而,自适应网格法在数据同化中的应用目前仍局限于基于列的一维模型。第三,将图形处理单元应用于空气质量预测,可以更优化资源使用,并通过硬件加速效应增强模型性能,而机器学习方法既可以保持与数值解的一致性,又可以提高特定化学物质空气质量预测的准确性。此外,描述更复杂过程和机制的参数已被添加到先前存在的物理和化学参数化中,以便更准确地表示各种小尺度特征,例如气溶胶表面无机化学的参数化,以及各种光解方案。在空气质量预测中,分辨率的提高带来了计算负担,并改变了已分辨和亚网格现象的边界,这反过来又刺激了新技术的发展和使用(如自适应网格技术、图形处理单元加速、机器学习方法)。它们有利于提高预报精度和获得关于大气物理和化学机制的新见解。然而,新的挑战也随之而来,包括网格细化的选择标准,高分辨率观测数据的获取以及人工智能混合空气质量模型的集成。为了克服目前化学再分析的分辨率问题,需要进一步发展自适应不规则网格数据同化方法。
{"title":"Next Generation Air Quality Models: Dynamical Mesh, New Insights into Mechanism, Datasets and Applications","authors":"Jinxi Li,&nbsp;Yijie Li,&nbsp;Zifa Wang,&nbsp;Jiang Zhu,&nbsp;Lei Kong,&nbsp;Jie Li,&nbsp;Huangjian Wu,&nbsp;Leisheng Li,&nbsp;Xiao Tang,&nbsp;Zhen Cheng,&nbsp;Lanyi Zhang,&nbsp;Pu Gan,&nbsp;Xiaole Pan,&nbsp;Wenyi Yang,&nbsp;Kai Cao,&nbsp;Jie Zheng","doi":"10.1007/s40726-025-00355-9","DOIUrl":"10.1007/s40726-025-00355-9","url":null,"abstract":"<div><h3>Purpose of Review</h3><p>Air quality modelling and forecasting have been well recognised to play important roles in environmental research as well as government policy assessments and management strategies. To address the recent progresses in air quality modelling, we conduct a literature review focusing on air quality forecasting models and reanalysis datasets.</p><h3>Recent Findings</h3><p>First of all, the implementation of three-dimensional adaptive meshes/horizontal resolution-variable grids in air quality models offers a crucial insight on multi-scale simulations down to the hectometre level. These models balance high accuracy with computational efficiency. Secondly, current reanalysis still has limitations in its horizontal resolution (dozens of kilometres) that are insufficient to support the analysis and management of air pollution at factory levels or neighbourhood scales. The development of adaptive mesh resolution method provides a promising way to deal with this issue and allows the construction of the chemistry reanalysis at ultra-high resolutions (&lt; 1 km). However, the use of adaptive mesh method in data assimilation is currently still restricted to the column-based one-dimensional models. Thirdly, the application of graphics processing units to air quality predictions enables more optimised resource usage and enhances model performance through hardware acceleration effects, while machine learning methods can both maintain the consistency with numerical solutions and increase the accuracy of air quality predictions for specific chemical species. Furthermore, parameters that describe more complicated processes and mechanisms have been added into pre-existing physical and chemical parameterisations to enable more accurate representation of various small-scale features, such as the parameterisation of inorganic chemistry on the surface of aerosols, as well as various photolysis schemes.</p><h3>Summary</h3><p>The increase of resolution brings computational burdens and shifts the boundary of resolved and sub-grid phenomena in air quality prediction, which in turn stimulates the development and usage of new technologies (e.g. adaptive mesh techniques, graphics processing unit acceleration, machine learning methods). They are conducive to the improvement of prediction accuracies and the acquisition of new insights on atmospheric physical and chemical mechanisms. However, new challenges also ensued, including the selection criteria for mesh refinement, the acquisition of high-resolution observational data and the integration of artificial intelligence-hybrid air quality models. More efforts are required to develop the adaptive irregular mesh grid data assimilation method to overcome the resolution problems of current chemical reanalysis.</p></div>","PeriodicalId":528,"journal":{"name":"Current Pollution Reports","volume":"11 1","pages":""},"PeriodicalIF":6.4,"publicationDate":"2025-04-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s40726-025-00355-9.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"143877685","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Scenario Setting in Life Cycle Assessments for Wastewater Treatment: A Comprehensive Review 污水处理生命周期评估中的情景设置:综合综述
IF 6.4 2区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-04-25 DOI: 10.1007/s40726-025-00353-x
Changkun Lin, Fengbin Sun, Jingsi Gao, Jian Wu, Fei Guo

Purpose of Review

This review aims to explore the application of scenario setting in life cycle assessment (LCA) studies related to wastewater treatment. Given the variability in LCA results based on different scenario settings, this paper seeks to categorize these settings, assess their impact, and provide a reference for future research in optimizing wastewater treatment industry.

Recent Findings

To achieve a more comprehensive understanding of the wastewater treatment field, recent studies have incorporated a more diverse range of scenarios for comparative analysis. These scenarios can generally be categorized into small-scale and large-scale scenarios, including those set up to compare different wastewater treatment technologies, demonstrate the potential of new versus traditional processes, predict future developments, and analyze regional impacts spanning entire countries, among others. Scenario setting plays a critical role throughout the LCA process, influencing model construction, data analysis, and result interpretation.

Summary

The motivation behind scenario setting lies in comparison, and it can be integrated throughout LCA research, serving distinct roles at various stages. This review categorizes scenario setting into three steps: baseline scenario setting, main scenario setting, and supplementary scenario setting. Proper scenario setting is crucial for enhancing the accuracy and depth of wastewater treatment life cycle assessments, enabling researchers to provide valuable insights into the environmental, economic, and social impacts of wastewater treatment technologies. This structured approach supports decision-makers in optimizing treatment processes and developing more sustainable wastewater management policies.

本文旨在探讨情景设置在污水处理相关生命周期评估(LCA)研究中的应用。考虑到不同情景设置下LCA结果的差异,本文试图对这些情景进行分类,评估其影响,为未来污水处理行业优化研究提供参考。为了更全面地了解废水处理领域,最近的研究纳入了更多样化的情景进行比较分析。这些情景通常可分为小规模和大规模情景,包括为比较不同的废水处理技术、展示新工艺与传统工艺的潜力、预测未来发展以及分析跨越整个国家的区域影响等而设置的情景。场景设置在整个LCA过程中起着关键作用,影响模型构建、数据分析和结果解释。情景设置的动机在于比较,它可以贯穿于整个LCA研究中,在不同的阶段起着不同的作用。本综述将场景设置分为三个步骤:基线场景设置、主场景设置和补充场景设置。适当的情景设置对于提高废水处理生命周期评估的准确性和深度至关重要,使研究人员能够对废水处理技术的环境、经济和社会影响提供有价值的见解。这种结构化方法支持决策者优化处理过程和制定更可持续的废水管理政策。
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引用次数: 0
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Current Pollution Reports
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