Improving the fracture toughness of concrete is key to improving the resilience and longevity of structures throughout our built environment. Microstructural heterogeneity and resulting crack propagation and arrest mechanisms are central to concrete’s fracture toughness. While nanoindentation has shed light on the heterogeneity of moduli and hardness in concrete, more research is needed to understand how individual microstructural phases contribute independently and collectively to macroscopic fracture properties. Here, we combine three-point bend experiments on microbeams of concrete with pre- and post-test X-ray imaging and finite element modeling to investigate the influence of individual phases of concrete on crack propagation mechanisms. We pay careful attention to incorporating realistic fracture properties of the individual phases in modeling based on recent experiments using nanoindentation, microscratch testing, and acoustic emission. Our combined experimental and modeling study reveals that the contrast in the elastic and fracture properties of phases, and microstructural features such as the size and shape of inclusion phases, largely influence the crack propagation mechanisms and effective toughness of the concrete composite. The results provide useful insights into engineering the next generation of tough cementitious materials.
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