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Ultrafast Terahertz Superconductor Van der Waals Metamaterial Photonic Switch 超快太赫兹超导体范德华超材料光子开关
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-10-07 DOI: 10.1002/adpr.202470029
Kaveh Delfanazari

2D Layered Superconductors

In article number 2400045, Kaveh Delfanazari showcases methods for the realization of ultrafast terahertz (THz) metamaterial photonic switches on a few nanometer-thick layered high-temperature superconductor van der Waals (vdWs). The metamaterial array offers active modulation of THz amplitude and phase with an ultrafast-picosecond-switching timescale. The device holds promise for the development of future THz communication circuits and systems operating at cryogenic temperatures.

二维层状超导体 在编号为 2400045 的文章中,Kaveh Delfanazari 展示了在几纳米厚的层状高温超导体范德华(vdWs)上实现超快太赫兹(THz)超材料光子开关的方法。该超材料阵列可主动调制太赫兹振幅和相位,开关时间超快,可达皮秒级。该装置有望用于开发未来在低温条件下运行的太赫兹通信电路和系统。
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引用次数: 0
Structural Colors Derived from the Combination of Core–Shell Particles with Cellulose 核壳粒子与纤维素结合产生的结构色彩
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-10-07 DOI: 10.1002/adpr.202470027
Regina Leiner, Lukas Siegwardt, Catarina Ribeiro, Jonas Dörr, Christian Dietz, Robert W. Stark, Markus Gallei

Core–Shell Particles

Essential features of functional optical materials are their interaction with light and underlying structures. In article number 2400091, Markus Gallei and co-workers report the combination of structural colors with cellulose, a renewable and biodegradable biopolymer. The latter acts as reinforcement agents, maintaining the polymer opal film’s structural color and mechanochromic material behavior.

核壳粒子 功能性光学材料的基本特征是与光和底层结构的相互作用。在文章编号 2400091 中,Markus Gallei 及其合作者报告了结构色与纤维素(一种可再生和生物降解的生物聚合物)的结合。纤维素是一种可再生、可生物降解的生物聚合物,可作为增强剂,保持聚合物蛋白石薄膜的结构颜色和机械变色材料特性。
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引用次数: 0
A Two-Stage Polymerization Strategy for Preparing Polymer-Network Liquid Crystals with Oxygen-Sensing Property 制备具有氧传感特性的聚合物网络液晶的两阶段聚合策略
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-09 DOI: 10.1002/adpr.202470026
Zongdai Liu, Zhibo Zhang, Yi Zhang, Dan Luo, Kun-Lin Yang

Polymer-Network Liquid Crystals

In article number 2300340, Dan Luo, Kun-Lin Yang, and co-workers show that after partially completed photopolymerization, the polymer network liquid crystal undergoes a secondary polymerization to form an isotropic polymer network when it is heated beyond its clearing point, resulting in an irreversible optical appearance change from transparent to cloudy. It enables applications such as a heating stopwatch and oxygen sensing.

聚合物网络液晶 在编号为 2300340 的文章中,Dan Luo、Kun-Lin Yang 及合作者展示了聚合物网络液晶在部分完成光聚合后,当加热超过其清澈点时,会发生二次聚合,形成各向同性的聚合物网络,从而导致从透明到浑浊的不可逆光学外观变化。它可用于加热秒表和氧气传感等应用。
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引用次数: 0
Progress on Coherent Perovskites Emitters: From Light-Emitting Diodes under High Current Density Operation to Laser Diodes 相干 Perovskites 发射器的研究进展:从高电流密度下的发光二极管到激光二极管
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-09 DOI: 10.1002/adpr.202470024
Gayoung Lee, Yejin Jun, Hyeonji Lee, Kwangdong Roh

Coherent Perovskites Emitters

In article number 2400033, Kwangdong Roh and co-workers provide a comprehensive overview of the historical progress in perovskite lasers and light-emitting didoes, along with important design considerations essential for their development.

相干过氧化物发光器 在编号为 2400033 的文章中,Kwangdong Roh 及其合作者全面概述了过氧化物激光器和发光二级管的历史进展,以及对其发展至关重要的重要设计考虑因素。
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引用次数: 0
Formation Mechanisms and Fluorescence Properties of Carbon Dots in Coal Burning Dust from Coal-Fired Power Plants 燃煤电厂燃煤粉尘中碳点的形成机理和荧光特性
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-09-02 DOI: 10.1002/adpr.202400010
Zhexian Zhao, Weizuo Zhang, Jin Zhang, Yuzhao Li, Han Bai, Fangming Zhao, Zhongcai Jin, Ju Tang, Yiming Xiao, Wen Xu, Yanfei Lü

Carbon dots (CDs) show great application potential with their unique and excellent performances. Coal and its derivatives are rich in aromatic ring structure, which is suitable for preparing CDs in microstructure. Coal-burning dust from coal-fired power plants can be utilized as a rich resource to separate and extract CDs. It is shown in the results that there are two main possible mechanisms for the formation of CDs in coal-burning dust. One is the self-assembly of polycyclic aromatic hydrocarbons contained in coal or produced by incomplete combustion of coal. The other mechanism is that the bridge bonds linking different aromatic structures in coal break, which will form CDs with different functional groups when the coals burn at high temperature. Under violet light excitation at 310–340 nm or red light at 610–640 nm, CDs extracted from coal-burning dust can emit purple fluorescence around 410 nm. The mechanism of up-conversion fluorescence emission of CDs is due to a two-photon absorption process. The recycling of CDs from coal-burning dust from coal-fired power plants are not only good to protect environment but will also be helpful for mass production of CDs.

碳点(CD)以其独特而优异的性能显示出巨大的应用潜力。煤及其衍生物富含芳香环结构,适合制备微结构的碳点。燃煤电厂的燃煤粉尘是分离和提取 CD 的丰富资源。研究结果表明,燃煤粉尘中 CD 的形成可能有两种主要机制。一种是煤中含有的或煤不完全燃烧产生的多环芳烃的自组装。另一种机制是煤炭中连接不同芳香结构的桥键断裂,在高温燃烧时会形成具有不同官能团的 CD。在波长为 310-340 纳米的紫光或波长为 610-640 纳米的红光激发下,从燃煤粉尘中提取的 CD 可在波长为 410 纳米左右发出紫色荧光。CD 上转换荧光发射的机理是双光子吸收过程。从燃煤电厂的燃煤粉尘中回收 CD 不仅有利于保护环境,还有助于大规模生产 CD。
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引用次数: 0
All-Bands-Flat Floquet Topological Photonic Insulators with Microring Lattices 具有微oring 晶格的全带平面浮凸拓扑光子绝缘体
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-04 DOI: 10.1002/adpr.202470021
Hanfa Song, Vien Van

Topological Photonic Insulators

In article number 2400023, Vien Van and Hanfa Song present the design and realization of (2 + 1)D topological photonic insulators hosting all flat bands, which exhibit novel properties such as anomalous Floquet insulator phase, ultra-wide edge mode continuum, super robustness to disorder, and photon caging in compact localized bulk states. These lattices have broadband applications in topologically-protected quantum photonics and programmable photonic circuits.

拓扑光子绝缘体 在编号为 2400023 的文章中,Vien Van 和 Hanfa Song 介绍了 (2 + 1)D 拓扑光子绝缘体的设计与实现,这种绝缘体承载所有平带,具有新颖的特性,如反常的 Floquet 绝缘体相位、超宽边缘模式连续体、对无序的超强鲁棒性,以及在紧凑局部体态中的光子笼。这些晶格可广泛应用于拓扑保护量子光子学和可编程光子电路。
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引用次数: 0
Upconversion of Infrared Light by Graphitic Microparticles Due to Photoinduced Structural Modification 光诱导结构改性导致石墨微粒对红外光的上转换
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-04 DOI: 10.1002/adpr.202470023
Rohin Sharma, Nishma Bhattarai, Rijan Maharjan, Lilia M. Woods, Nirajan Ojha, Ashim Dhakal

Photoinduced Structural Modification

In article number 2300326, Ashim Dhakal and co-workers show that photo-induced metastable modification of electronic structure in graphite allows for multiphoton processes that can up-convert an O-band infrared excitation to visible-NIR band in graphite powder. Theoretically, this process can upconvert an infrared light near the wavelength of 3 μm to VIS-NIR wavelengths. It opens exciting new avenues for applications in visible light generation and low-noise imaging using infrared light excitation.

光诱导结构修饰 在编号为 2300326 的文章中,Ashim Dhakal 及其合作者展示了光诱导石墨中电子结构的陨变修饰,从而实现了多光子过程,可将石墨粉中的 O 波段红外激发上转换为可见光-近红外波段。从理论上讲,这一过程可将波长为 3 μm 附近的红外线上转换为可见光-近红外波段。它为利用红外光激发可见光生成和低噪声成像的应用开辟了令人兴奋的新途径。
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引用次数: 0
Improvement of the Internal Quantum Efficiency of III-Nitride Blue Micro-Light-Emitting Diodes by the Hole Accelerator at the Low Current Density 低电流密度下利用空穴加速器提高 III 氮化物蓝色微型发光二极管的内部量子效率
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-04 DOI: 10.1002/adpr.202300262
An-Chi Wei, Sheng-Hsiang Wang, Jyh-Rou Sze, Quoc-Hung Pham

The hole accelerator is proven to benefit the hole injection for traditional light-emitting diodes (LEDs) because the induced electric field provides the holes with more kinetic energy to pass through the electron-blocking layer, enhancing the hole injection efficiency. Herein, the effect of the hole accelerator (HA) layer on the micro-LEDs by modeling the characteristics of the devices with a current density of lower than 10 A cm−2 is investigated. The simulation results show that the appended HA layer brings a knot of the electric field in the HA layer, leading to higher internal quantum efficiency (IQE) than the device without HA under the low current density. The thickness and composition of HA, the quantum number, and the material of quantum barrier are also simulated and analyzed. The simulated radiative, Shockley–Read–Hall, and Auger recombination rates show that the IQE of the micro-LED with the HA layer is higher than that without the HA layer under the current density of lower than 10 A cm−2.

事实证明,空穴加速器有利于传统发光二极管(LED)的空穴注入,因为诱导电场为空穴提供了更多的动能,使其能够穿过电子阻挡层,从而提高了空穴注入效率。本文通过模拟电流密度低于 10 A cm-2 的器件特性,研究了空穴加速器(HA)层对微型发光二极管的影响。模拟结果表明,在低电流密度下,附着的 HA 层会带来 HA 层中的电场结,从而使器件的内部量子效率(IQE)高于不附着 HA 层的器件。此外,还对 HA 的厚度和成分、量子数以及量子势垒的材料进行了模拟和分析。模拟的辐射、肖克利-雷德-霍尔和奥格重组率表明,在低于 10 A cm-2 的电流密度下,有 HA 层的微型 LED 的 IQE 比没有 HA 层的要高。
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引用次数: 0
Design and Fabrication of 3D-Printed Lab-On-A-Chip Devices for Fiber-Based Optical Chromatography and Sorting 设计和制造用于光纤色谱和分拣的三维打印片上实验室设备
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-08-01 DOI: 10.1002/adpr.202400011
Ole Milark, Marc Buttkewitz, Emil Agócs, Beate Legutko, Benjamin Bergmann, Janina Bahnemann, Alexander Heisterkamp, Maria Leilani Torres-Mapa

Microfluidic lab-on-a-chip (LOC) devices have become essential tools for multitudes of applications in various research fields. 3D printing of microfluidic LOC devices offers many advantages over more traditional manufacturing processes, including rapid prototyping and single-step fabrication of complex 3D structures. In this work, 3D-printed microfluidic devices are designed and fabricated for optical chromatography and sorting. Optical chromatography is performed by inserting a single-mode optical fiber into the device creating a counter-propagating laser beam to the fluid flow. Particles are separated depending on refractive index and size. To demonstrate optical sorting, a cross-type sorter 3D-printed microfluidic device is fabricated that directs the laser beam perpendicular to the flow direction. Design features such as a sloping channel and a channel configuration for 3D hydrodynamic focusing (to aid in controlled sample flow and particle position) help to optimize sorting performance. Stable optofluidic trapping and sorting are successfully achieved using the fabricated microfluidic devices. These results highlight the tremendous potential of 3D printing of microfluidic LOC devices for applications aimed at the optofluidic manipulation of micron-sized particles.

微流控芯片实验室(LOC)设备已成为各研究领域众多应用的重要工具。与传统制造工艺相比,三维打印微流控芯片设备具有许多优势,包括快速原型设计和复杂三维结构的单步制造。在这项工作中,我们设计并制造了用于光学色谱和分拣的三维打印微流控设备。光学色谱法是通过将单模光纤插入设备,在流体流动中产生一束反向传播的激光束来实现的。颗粒根据折射率和大小进行分离。为了演示光学分拣,我们制作了一个交叉型分拣机 3D 打印微流控装置,该装置可将激光束垂直于流动方向。倾斜通道和三维流体动力聚焦通道配置(有助于控制样品流和颗粒位置)等设计特点有助于优化分拣性能。利用制造的微流体设备成功实现了稳定的光流体捕获和分拣。这些结果凸显了三维打印微流体 LOC 设备在微米级颗粒光流体操纵应用中的巨大潜力。
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引用次数: 0
Chiral Emission from Optical Metasurfaces and Metacavities 光学元表面和元腔的手性发射
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-07-22 DOI: 10.1002/adpr.202400060
Jungho Han, Heejoo Jang, Yeonsoo Lim, Seong S. Kim, Jeheon Lee, Young Chul Jun
Chiral emission exhibiting a large degree of circular polarization (DCP) is important in diverse applications ranging from displays and optical storage to optical communication, bioimaging, and medical diagnostics. Although chiral luminescent materials can generate chiral emissions directly, they frequently suffer from either low DCP or low quantum efficiencies. Achieving high DCP and quantum efficiencies simultaneously remains extremely challenging. This review introduces an alternative approach to chiral emission. Chiral emission with large DCP can be readily achieved by combining conventional achiral emitters with chiral metasurfaces. Particularly, this article focuses on recent experimental and theoretical studies on perovskite metasurfaces and metacavities that employ achiral perovskite materials. First, chiral photoluminescence from extrinsic and intrinsic perovskite metasurfaces is explained together with theoretical discussions on metasurface design based on reciprocity and critical coupling. Chiral photoluminescence from other achiral materials is also explained. Subsequently, chiral electroluminescence from perovskite metacavities and other achiral materials is discussed. Finally, it is concluded with future perspectives. This review provides physical insights into how ideal chiral emission can be realized by optimizing the design of metasurfaces and metacavities. Compact chiral light sources with both near‐unity DCP and strong emission intensities can have far‐reaching consequences in a wide range of future applications.
在从显示器和光存储到光通信、生物成像和医疗诊断等各种应用中,表现出高度圆偏振(DCP)的手性发射非常重要。虽然手性发光材料可以直接产生手性发射,但它们经常受到低 DCP 或低量子效率的困扰。同时实现高 DCP 和量子效率仍然极具挑战性。本综述介绍了手性发射的另一种方法。通过将传统的非手性发射器与手性元表面相结合,可以轻松实现大 DCP 的手性发射。本文特别关注了最近关于采用非手性包晶材料的包晶元表面和元腔的实验和理论研究。首先,解释了来自外在性和内在性包晶元表面的手性光致发光,并对基于互易性和临界耦合的元表面设计进行了理论探讨。还解释了其他非手性材料的手性光致发光。随后,讨论了来自包晶体元腔和其他非手性材料的手性电致发光。最后,以未来展望作结。这篇综述从物理角度阐述了如何通过优化元表面和元腔的设计来实现理想的手性发射。同时具有近乎统一 DCP 和强发射强度的紧凑型手性光源将在未来的广泛应用中产生深远影响。
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引用次数: 0
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Advanced Photonics Research
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