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Time-Domain Near-Field Scanning Microscopy of Terahertz Metasurfaces 太赫兹超表面的时域近场扫描显微镜
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-01-19 DOI: 10.1002/adpr.202500268
Ruxue Wei, Soren Petersen, Weili Zhang

Metasurfaces have emerged as an ultrathin, versatile method for manipulating terahertz surface plasma waves that are critical for subwavelength optical control but are very challenging to be excited and characterized. This review presents recent advances in terahertz surface plasmon waves, focusing on three functional areas: excitation through resonant coupling, beam shaping through phase gradient design, and complex field encoding using metaholography. To validate and analyze these phenomena, near-field scanning terahertz microscopy (NSTM) is recently developed as a powerful tool for mapping the field distribution of surface plasmon waves, spin- and polarization-sensitive responses, and vector wavefront structures with subwavelength resolution. Representative metasurfaces architectures are highlighted, including periodic and nonperiodic resonators, dynamic phase modulators, and multiplexed holographic encoders, and summarize how their performance can be directly observed through the NSTM platform. Together, these studies demonstrate the synergy between metasurfaces design and near-field characterization. The integration of reconfigurable metasurfaces with an advanced near-field scanning platform will be key to realizing high-capacity, tunable terahertz photonic devices.

超表面已经成为一种超薄、通用的方法来操纵太赫兹表面等离子体波,这对于亚波长光学控制至关重要,但很难激发和表征。本文综述了太赫兹表面等离子体波的最新进展,重点介绍了三个功能领域:通过共振耦合激发,通过相位梯度设计的波束整形,以及使用金相术的复杂场编码。为了验证和分析这些现象,近场扫描太赫兹显微镜(NSTM)最近发展成为一种强大的工具,用于绘制表面等离子体波的场分布,自旋和极化敏感响应,以及具有亚波长分辨率的矢量波前结构。重点介绍了具有代表性的元表面结构,包括周期和非周期谐振器、动态相位调制器和多路全息编码器,并总结了如何通过NSTM平台直接观察它们的性能。总之,这些研究证明了超表面设计和近场表征之间的协同作用。可重构元表面与先进的近场扫描平台的集成将是实现高容量、可调谐太赫兹光子器件的关键。
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引用次数: 0
Dynamically Tunable Coherent Perfect Absorption Based on Bound States in the Continuum in Borophene Metamaterials 基于硼罗芬超材料连续体束缚态的动态可调谐相干完美吸收
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-01-16 Epub Date: 2025-10-17 DOI: 10.1002/adpr.202500174
Xue-Yan Wu, Yan-Xi Zhang, Qi Lin, Xiang Zhai, Ling-Ling Wang, Gui-Dong Liu

A symmetry-protected bound states in the continuum (BIC) mechanism based on borophene metamaterials, achieving broadband coherent perfect absorption (CPA) with dual-band absorption peaks in the near-infrared waveband, is proposed. Through coupled mode theory analysis incorporating near-field and far-field coupling effects, structural parameter optimization enables synchronized strong critical coupling states for both absorption bands. Benefiting from weak angular dispersion induced by the flat-band characteristics of deep subwavelength periodic structures, the system demonstrates high stability in absorption efficiency and resonant wavelengths under wide-angle incidence (within 60°). Under coherent beam excitation, the system not only achieves CPA states but also realizes absorption switching functionality via precise control of the inter-beam phase difference. Notably, dynamic carrier density modulation significantly broadens the CPA operational bandwidth, effectively overcoming the narrowband limitations inherent to conventional CPA systems. This study establishes a novel theoretical framework and implementation strategy for advancing multifunctional tunable absorbers and all-optically controlled devices.

提出了一种基于硼罗芬超材料的对称保护的连续介质束缚态机制,实现了近红外波段双频吸收峰的宽带相干完美吸收。通过结合近场和远场耦合效应的耦合模式理论分析,优化结构参数,使两个吸收波段的强临界耦合状态同步。得益于深亚波长周期结构的平带特性引起的弱角色散,该系统在广角入射(60°以内)下具有较高的吸收效率和共振波长稳定性。在相干光束激励下,系统不仅实现了CPA状态,而且通过精确控制光束间的相位差实现了吸收开关功能。值得注意的是,动态载波密度调制显着拓宽了CPA操作带宽,有效地克服了传统CPA系统固有的窄带限制。本研究为推进多功能可调吸收器和全光控器件建立了新的理论框架和实现策略。
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引用次数: 0
Metasurface-Encoded Single-Pixel Hyperspectral Imaging 超表面编码的单像素高光谱成像
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-01-16 Epub Date: 2025-11-06 DOI: 10.1002/adpr.202500181
Haitao Nie, Yaping Zhao, Yifei Zhang, Yanmin Zhu, Jingyan Chen, Yunfei Tian, Edmund Y. Lam

Hyperspectral imaging in the visible spectrum offers significant potential for diverse applications, but is often constrained by bulky hardware and limited robustness in low-light conditions. To overcome these challenges, a simulation-based proof-of-concept for a metasurface-encoded single-pixel hyperspectral imaging system (MESH) is presented, in which structured spatial modulation is combined with a compact set of 50 broadband metasurface filters designed using a binary pattern generation strategy to ensure low interfilter correlation. Hyperspectral datacubes comprising 301 channels from 400 to 700 nm are reconstructed via a sparsity-constrained optimization algorithm, while a physics-enhanced deep learning model is further introduced to enable fast and accurate recovery. Simulation results demonstrate that MESH achieves a spectral resolution of 1.17 nm. Even at a total compression ratio of 2.1%, the deep learning model maintains high reconstruction quality, with a peak signal-to-noise ratio of 30.96 dB, structural similarity of 0.8526, and spectral angle mapping of 0.0742 rad, indicating accurate intensity recovery, structural preservation, and spectral integrity. The present study provides a simulation-based verification of feasibility and design guidelines, laying the groundwork for future experimental validation of the MESH system, which is expected to further demonstrate its practical applicability and performance for deployment in low-light and resource-constrained environments.

可见光谱中的高光谱成像为各种应用提供了巨大的潜力,但通常受到笨重的硬件和弱光条件下有限的鲁棒性的限制。为了克服这些挑战,本文提出了一种基于仿真的超表面编码单像素高光谱成像系统(MESH)的概念验证,其中结构化空间调制与一组紧凑的50个宽带超表面滤波器相结合,这些滤波器使用二进制模式生成策略设计,以确保低滤波器间相关性。通过稀疏约束优化算法重建包含400至700 nm范围内301个通道的高光谱数据集,同时进一步引入物理增强深度学习模型,以实现快速准确的恢复。仿真结果表明,MESH的光谱分辨率为1.17 nm。即使在总压缩比为2.1%的情况下,深度学习模型仍保持了较高的重建质量,峰值信噪比为30.96 dB,结构相似度为0.8526,光谱角映射为0.0742 rad,表明了准确的强度恢复、结构保存和光谱完整性。本研究提供了基于仿真的可行性验证和设计指南,为未来MESH系统的实验验证奠定了基础,有望进一步证明其在低光照和资源受限环境下部署的实际适用性和性能。
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引用次数: 0
VO2 Nanocomposite Thin Films Integrated on Glass Substrates for Tunable Properties 集成在玻璃基板上的VO2纳米复合薄膜具有可调性能
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-01-16 Epub Date: 2025-10-05 DOI: 10.1002/adpr.202500124
Claire A. Mihalko, Juanjuan Lu, Yizhi Zhang, Zihao He, Nirali A. Bhatt, Lizabeth Quigley, Hongyi Dou, James P. Barnard, Aleem M. Siddiqui, Raktim Sarma, Haiyan Wang

Successful tuning of the metal-to-insulator transition (MIT) near room temperature for VO2 thin films has been previously reported via a variety of methods, from strain and defect engineering to energy band restructuring. In this study, a nanocomposite VO2 design is integrated on glass substrates resulting in tuning the transition, morphology, and optical and electrical properties. Specifically, VO2-Au nanocomposite and VO2 thin films are grown using pulsed laser deposition on glass with a ZnO buffer layer. The variations in film composition and buffer layer result in unique morphology, phase change properties, and optical properties. Notably, the introduction of the ZnO buffer layer results in a redshift of the surface plasmon resonance wavelength and unique epsilon-near-zero characteristic for the buffered films. Overall, this work discusses the effect on the tuning of the MIT and optical properties through a novel multifaceted approach using both defect engineering and energy band restructuring. These VO2 and VO2 nanocomposite films integrated on amorphous glass substrates show promise for future applications in sensing, thermochromics, and optical switching.

从应变和缺陷工程到能带重组等多种方法,已经报道了VO2薄膜在室温附近金属到绝缘体转变(MIT)的成功调谐。在这项研究中,将纳米复合VO2设计集成在玻璃基板上,从而调整转变,形态以及光学和电学性质。具体来说,利用脉冲激光沉积技术在带有ZnO缓冲层的玻璃上生长了VO2- au纳米复合材料和VO2薄膜。薄膜组成和缓冲层的变化导致了独特的形貌、相变特性和光学特性。值得注意的是,ZnO缓冲层的引入导致了表面等离子体共振波长的红移和缓冲膜独特的epsilon近零特性。总的来说,这项工作通过使用缺陷工程和能带重构的新颖多方面方法讨论了对MIT和光学性质调谐的影响。这些VO2和VO2纳米复合薄膜集成在非晶玻璃衬底上,在传感、热致变色和光开关等领域具有广阔的应用前景。
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引用次数: 0
Toward Rapid Low-Cost Fabrication of Single-Nanowire Photodetectors via the Utilization of Dielectrophoresis 利用介质电泳技术快速低成本制造单纳米线光电探测器
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-01-16 Epub Date: 2025-10-05 DOI: 10.1002/adpr.202500213
Siriny Laumier, Matteo Bosi, Luca Seravalli, Ian Sandall

The scalable fabrication of high-performance nanowire (NW) photodetectors remains a critical challenge for the integration of nanoscale optoelectronics into practical technologies. This work presents a simple, rapid, and cost-effective method for the deterministic assembly of single germanium (Ge) NWs between electrode pairs using a modified dielectrophoresis (DEP) setup. By introducing a voltage-divider configuration with a series resistor, the method enables self-limiting NW alignment, eliminating the need for nanoscale electrodes or extensive pre-optimization. Devices fabricated via this approach exhibit high responsivity—exceeding 6 × 105 A W−1 at both 700 and 1550 nm—among the highest reported for single Ge NW photodetectors. This enhanced performance is attributed to asymmetric Schottky junctions and possible optical resonances within the NWs. The method enables the rapid production of single-NW photodetectors with tunable properties, offering a versatile platform for low-cost optoelectronic device manufacturing and advancing the feasibility of NW-based sensing, imaging, and communication technologies.

高性能纳米线(NW)光电探测器的可扩展制造仍然是将纳米光电子技术集成到实际技术中的关键挑战。这项工作提出了一种简单、快速、经济有效的方法,用于在电极对之间使用改进的介电电泳(DEP)装置进行单锗(Ge) NWs的确定性组装。通过引入带有串联电阻的分压器配置,该方法可以实现自限制NW对齐,从而消除了对纳米级电极或大量预优化的需要。通过这种方法制造的器件在700和1550 nm处的响应度都超过了6 × 105 A W−1,是单Ge NW光电探测器中最高的。这种增强的性能归因于非对称肖特基结和NWs内可能的光学共振。该方法能够快速生产具有可调谐特性的单nw光电探测器,为低成本光电器件制造提供了一个通用平台,并推进了基于nw的传感、成像和通信技术的可行性。
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引用次数: 0
Boosting the Magnetic Response of a Composite Nanostructure in the Near-Visible Region with a Fano Resonance 范诺共振增强复合纳米结构近可见光区的磁响应
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-01-16 Epub Date: 2025-10-26 DOI: 10.1002/adpr.202500191
Maximilian Grimmer, Monika Fleischer

Plasmonic nanostructures can show a magnetic response in addition to an electrical one by guiding the plasmonic displacement current along a circular loop, inducing a magnetic dipole. Achieving a magnetic response at optical frequencies requires composite nanostructures with multiple elements to prevent saturation effects. A composite nanostructure consisting of three nanorods is presented that form a split-ring resonator with two additional gaps. The optical behavior of this nanostructure is investigated with both numerical simulation and experimental fabrication and measurement. Moreover, it is demonstrated that adding a nanorod below the central element facilitates an additional dark magnetic mode that causes a Fano resonance in the structure, increasing the magnetic near-field enhancement and the overall magnetic response of the nanostructure.

等离子体纳米结构可以通过引导等离子体位移电流沿圆形环路,产生磁偶极子,从而显示出磁响应和电响应。在光学频率下实现磁响应需要具有多个元素的复合纳米结构来防止饱和效应。提出了一种由三个纳米棒组成的复合纳米结构,形成了一个带有两个附加间隙的劈裂环谐振器。通过数值模拟和实验制作与测量研究了该纳米结构的光学特性。此外,研究表明,在中心元件下方添加纳米棒有助于增加暗磁模式,从而在结构中引起法诺共振,从而提高磁性近场增强和纳米结构的整体磁响应。
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引用次数: 0
Multiclass Identification of Van der Waals Semiconductors via Attention Neural Networks 基于注意神经网络的范德华半导体多类识别
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-01-14 Epub Date: 2025-10-26 DOI: 10.1002/adpr.202500197
Xingchen Dong, Jiayi Ma, Kun Wang, Martin Jakobi, Ali K. Yetisen, Alexander W. Koch

Intelligent characterization of van der Waals semiconductors is an essential process for industrial manufacturing and laboratory fabrication. A combination of microscopic images and artificial intelligence models is an efficient way for wafer-scale layer number identification of van der Waals semiconductors. This methodology overcomes the bottleneck of the conventional manual layer number counting approach, which requires a long period of manual inspection and induces high error rates when distinguishing layers with similar appearance. Here, a convolutional architecture that involves a fused network of ResNet-Inception with Attention Layer (RIAL) is developed for accurate multiclass classification of randomly distributed layers of chemical vapor deposition (CVD)-grown van der Waals semiconductors. RIAL model is first validated on the single-label datasets CIFAR-10/100, and subsequently fine-tuned on the custom-built microscopic image datasets of CVD-grown MoS2. To compare with semantic segmentation, U-Net with Attention Layer (UNAL) is further implemented for pixel-wise classification of multiclass semiconductors. The quantitative analysis of RIAL and UNAL illustrates the versatility of attention convolutional network models in the wafer-scale identification of van der Waals semiconductors.

范德华半导体的智能表征是工业制造和实验室制造的重要过程。显微图像与人工智能模型相结合是范德华半导体晶圆尺度层数识别的有效方法。该方法克服了传统人工层数计数方法的瓶颈,该方法需要长时间的人工检查,并且在区分外观相似的层时错误率高。本文开发了一种包含ResNet-Inception与注意层(RIAL)融合网络的卷积架构,用于对随机分布的化学气相沉积(CVD)生长的范德华半导体层进行精确的多类分类。RIAL模型首先在单标签数据集CIFAR-10/100上进行验证,随后在定制的cvd生长MoS2显微图像数据集上进行微调。为了与语义分割相比较,进一步实现了带注意层的U-Net (UNAL)多类半导体的逐像素分类。RIAL和UNAL的定量分析说明了注意卷积网络模型在范德华半导体晶圆尺度识别中的多功能性。
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引用次数: 0
Monolithically Integrated Fourier Injected REsonator (FIRE) for Passive Coherent Laser Combination 用于被动相干激光组合的单片集成傅里叶注入腔(FIRE)
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-01-14 Epub Date: 2025-10-30 DOI: 10.1002/adpr.202500211
Lance Sweatt, Xiaolei Zhao, Taylor LeVaur, Mohamed Baghdady, Mohan Ghimire, Md. Arefin Islam, Shafia Sultana, Kexin Li, Christopher J. Corcoran, Lin Zhu

Passively phased coherent laser systems have been extensively studied for their potential to reduce design complexity in applications requiring high radiance. In this letter, the experimental demonstration of a five-element angled laser diode array coupled to a slab waveguide cavity integrated onto a single chip in a monolithic FIRE configuration is presented. Using this configuration, the common FIRE cavity performs coherent combination of the individual lasers in the array, providing high inter-element coupling and reduced edge losses to allow single supermode operation. Quasi-continuous-wave operation and high-visibility fringes in the far field (V = 98%) that demonstrate excellent coherence of the laser array are experimentally demonstrated.

被动相控相干激光系统因其在高辐射应用中降低设计复杂性的潜力而受到广泛研究。在这封信中,实验演示了一个五元角度激光二极管阵列耦合到平板波导腔集成到单片单片FIRE结构。使用这种配置,常见的FIRE腔执行阵列中单个激光器的相干组合,提供高元件间耦合并减少边缘损耗,从而允许单模超模操作。实验证明了准连续波操作和远场高可见度条纹(V = 98%)显示了激光阵列的良好相干性。
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引用次数: 0
Synthesis of Self-Healing Microbeam by Superposition of Self-Decelerating Corner-Diffraction Beams 自减速角衍射光束叠加合成自愈微光束
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-01-13 Epub Date: 2025-10-17 DOI: 10.1002/adpr.202500205
Jinsu Yoon, Jaeyoun Kim, Yongtaek Hong

Quasi-nondiffracting (QND) optical beams are well known for their long-range propagation and self-healing capabilities. Shrinking their beam width down to the mesoscale regime can open up many new applications in microtechnology, but the complexity of the beam-forming platform remains the major hindrance to its realization. In contrast, the photonic nanojets (PNJs) boast simple platforms for their generation and inherently small beam size, but their utilization has been limited mainly to near-field applications. This work aims to hybridize the QND and PNJ beam concepts, eventually realizing microscale, self-healing QND beams using a simple, PNJ-style platform. To that end, the microscale cuboids made of low-index dielectric materials are dually utilized, first to generate two self-decelerating corner-diffraction beams and then to superpose them into a long-range (10λ–100λ) microbeam. The QND–PNJ hybridization concept and model will contribute synergistically to the study and application of the microscale optical beams.

准无衍射(QND)光束以其远距离传播和自愈能力而闻名。将它们的波束宽度缩小到中尺度范围可以在微技术中开辟许多新的应用,但波束形成平台的复杂性仍然是其实现的主要障碍。相比之下,光子纳米射流(PNJs)具有简单的生成平台和固有的小光束尺寸,但它们的应用主要局限于近场应用。这项工作旨在混合QND和PNJ光束的概念,最终使用一个简单的PNJ风格的平台实现微尺度、自修复的QND光束。为此,利用低折射率介质材料制成的微尺度长方体,首先产生两个自减速角衍射光束,然后将它们叠加成一个远程(10λ-100λ)微光束。QND-PNJ杂化概念和模型将为微尺度光束的研究和应用提供协同作用。
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引用次数: 0
Impact of A-Site Cation Substitution on Electronic and Optical Properties of 0D Perovskite Derivatives A4PbCl6 (A = Li, Na, K, Rb, Cs) A位阳离子取代对0D钙钛矿衍生物A4PbCl6 (A = Li, Na, K, Rb, Cs)电子和光学性质的影响
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2026-01-13 Epub Date: 2025-11-03 DOI: 10.1002/adpr.202500117
Aiqiang Hou, Zao Yi, Xifang Chen, Zigang Zhou, Hua Yang, Chaojun Tang, Fan Gao, Junqiao Wang, Boxun Li

Zero-dimensional (0D) perovskite derivatives A4PbCl6 (A = Li, Na, K, Rb, Cs) are promising for optoelectronic applications due to their unique properties. However, synthesizing pure-phase samples is challenging, and the impact of A-site cation substitution remains less explored. Addressing these challenges, first-principles calculations based on density functional theory (DFT) are employed to investigate the electronic and optical properties of A4PbCl6 perovskite derivatives. The calculations reveal that the substitution of A-site cations not only modifies the lattice parameters but also alters the distribution of the local electrostatic field within the crystal. These changes lead to variations in the electron density around the Cl and A atoms, thereby tuning the electronic structure and optical properties of the system. Specifically, Cs4PbCl6 exhibits the highest extinction coefficient in the ultraviolet (UV) region, indicating enhanced optical activity, while K4PbCl6 shows greater transparency due to its lower extinction coefficient. The results not only elucidate the impact of A-site cation substitution on the properties of 0D perovskite derivatives but also provide essential theoretical insights for the rational design of new optoelectronic materials, particularly for UV detection and transparent applications.

零维(0D)钙钛矿衍生物A4PbCl6 (A = Li, Na, K, Rb, Cs)由于其独特的性质,在光电应用中具有广阔的前景。然而,合成纯相样品是具有挑战性的,并且a位阳离子取代的影响仍然很少被探索。为了解决这些问题,采用基于密度泛函理论(DFT)的第一性原理计算来研究A4PbCl6钙钛矿衍生物的电子和光学性质。计算结果表明,a位阳离子的取代不仅改变了晶格参数,而且改变了晶体内部局部静电场的分布。这些变化导致Cl和A原子周围电子密度的变化,从而调整系统的电子结构和光学性质。其中,Cs4PbCl6在紫外区的消光系数最高,表明其光学活性增强,而K4PbCl6的消光系数较低,显示出更高的透明度。研究结果不仅阐明了a位阳离子取代对0D钙钛矿衍生物性能的影响,而且为合理设计新型光电材料,特别是紫外检测和透明应用提供了重要的理论见解。
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引用次数: 0
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Advanced Photonics Research
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