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Resonance Energy Transfer and Purcell Effect in a Cu2O/Au Hybrid Optical Antenna Cu2O/Au混合光学天线中的共振能量传递和Purcell效应
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-10-07 DOI: 10.1002/adpr.70084
Nishan Khatri, Ravi Teja Addanki Tirumala, Susheng Tan, Marimuthu Andiappan, Ali Kaan Kalkan

Optical Antennas

A nanosphere(Cu2O)-film(Au) hybrid resonator traps a visible photon and funnels the energy to creation of an electron-hole pair in gold. The resonant enhancements enable monitoring of interband transitions in Au for single Cu2O particles. The reverse process, fluorescence from gold, is also observed for single particles with giant Purcell factors. More information can be found in the Research Article by Ali Kaan Kalkan and co-workers (10.1002/adpr.202400126).

nasa纳米球(Cu2O)-薄膜(Au)混合谐振器捕获一个可见光子,并将能量输送到金中,形成电子-空穴对。共振增强可以监测单个Cu2O粒子在Au中的带间跃迁。相反的过程,来自金的荧光,也被观察到具有巨大珀塞尔因子的单粒子。更多信息可以在Ali Kaan Kalkan及其同事的研究文章(10.1002/adpr.202400126)中找到。
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引用次数: 0
Impact of System-Model Mismatch in Fourier Ptychographic Microscopy 系统模型失配对傅里叶显微成像的影响
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-10-05 DOI: 10.1002/adpr.202500180
Tuo Yin, Gookho Song, Doeon Lee, Jaeyeon Oh, Mooseok Jang

Fourier ptychography microscope (FPM) is a computational imaging technique that can achieve a large field-of-view and high-resolution retrieval of complex-amplitude object function from a set of low-resolution intensity images. This study investigates the effects of system-model discrepancies in FP reconstruction under diverse scenarios characterized by experimental errors, including axial mispositioning of specimens, sample thickness, and factors affecting k-vector sampling positions—magnification, light-emitting diode (LED) height, and positional errors of LED elements. With the systematic investigation using experimental data and Gauss-Newton algorithm, we provided the level of tolerance for different types of experimental errors and its general relation to configurational parameters for FPM, such as the numerical aperture of objective lens, synthetic numerical aperture, and the spectrum overlapping ratio of low-resolution images. Also, we found that different types of errors can generate characteristic effects on the appearance of the reconstructed images, and therefore, reconstruction results could be highly inconsistent under various conditions of system-model mismatch, even if the reconstructed images are seemingly plausible. The investigation highlights the need for an improved algorithmic approach to physically accurate retrieval of complex-amplitude maps using a FPM.

傅里叶平面摄影显微镜(FPM)是一种计算成像技术,可以从一组低分辨率强度图像中实现大视场和高分辨率的复杂振幅目标函数检索。本研究探讨了不同实验误差情况下系统模型差异对FP重建的影响,实验误差包括样品轴向定位错误、样品厚度、k矢量采样位置影响因素——放大倍率、发光二极管(LED)高度和LED元件位置误差。通过对实验数据和高斯牛顿算法的系统研究,给出了FPM不同类型实验误差的容差水平及其与物镜数值孔径、合成数值孔径和低分辨率图像光谱重叠比等配置参数的一般关系。此外,我们发现不同类型的误差会对重建图像的外观产生特征影响,因此,即使重建图像看似可信,在各种系统模型不匹配的条件下,重建结果也可能高度不一致。该研究强调需要一种改进的算法方法来使用FPM精确地检索复杂振幅图。
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引用次数: 0
Record Negative Photoconductivity in N-Polar AlGaN/GaN Quantum-Well Heterostructures n极性AlGaN/GaN量子阱异质结构中记录的负光电性
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-10-01 DOI: 10.1002/adpr.202500130
Maciej Matys, Atsushi Yamada, Toshihiro Ohki, Kouji Tsunoda

The AlGaN/GaN quantum-well heterostructures typically exhibit a positive photoconductivity (PPC) during the light illumination. Surprisingly, the introducing the GaN/AlN superlattice (SL) back barrier into N-polar AlGaN/GaN quantum-well heterostructures induces a transition in these heterostructures from PPC to negative photoconductivity (NPC) as the SL period number increases at room temperature. This transition occurs under an infrared light illumination and can be well explained in terms of the excitation of hot electrons from the 2D electron gas and subsequent trapping them in a SL structure. The NPC effect observed in N-polar AlGaN/GaN heterostructures with SL back barrier exhibits photoconductivity yield exceeding 85%$%$ and thus is the largest ones reported so far for semiconductors. In addition, the NPC signal remains relatively stable at high temperatures up to 400 K. The obtained results can be interesting for the development of NPC related devices such as photoelectric logic gates, photoelectronic memory, and infrared photodetectors.

在光照射下,AlGaN/GaN量子阱异质结构通常表现出正的光电导率(PPC)。令人惊讶的是,在室温下,将GaN/AlN超晶格(SL)背势垒引入n极性AlGaN/GaN量子阱异质结构中,随着SL周期数的增加,这些异质结构从PPC转变为负光电性(NPC)。这种转变发生在红外光照射下,可以很好地解释为来自二维电子气体的热电子的激发和随后在SL结构中捕获它们。在具有SL背势垒的n极性AlGaN/GaN异质结构中观察到的NPC效应显示出超过85%的光导率,因此是迄今为止报道的半导体中最大的光导率。此外,NPC信号在高达400k的高温下保持相对稳定。所得结果对NPC相关器件如光电逻辑门、光电存储器和红外光电探测器的开发具有重要意义。
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引用次数: 0
Simple and Environmentally Friendly Solution Synthesis of CsPbI3 Nanoribbons: Investigating the Reversible δ- to γ-Phase Transition 简单和环保的溶液合成CsPbI3纳米带:研究可逆δ-到γ-相变
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-09-27 DOI: 10.1002/adpr.202500059
Lorenzo Sirna, Anna Lucia Pellegrino, Luca Pulvirenti, Maria Miritello, Vanna Torrisi, Giuseppe Bengasi, Marina Foti, Graziella Malandrino

The all-inorganic lead halide perovskites, including cesium lead iodide (CsPbI3), have attracted significant attention due to their possible applications in photovoltaics, light-emitting devices, and other optoelectronic technologies, driven by their intrinsic optoelectronic properties. This study introduces a simple, green, and scalable solution synthesis method for the CsPbI3 perovskite fabrication, utilizing β-diketonate [Cs(hfa)]n and [Pb(hfa)2diglyme]2 precursors and ethanol as solvent. The as-synthesized nanoribbons are initially fabricated in the pure yellow δ-phase, as confirmed by X-ray diffraction and energy-dispersive X-ray analysis. Thermal analysis through differential scanning calorimetry highlights the reversible phase transition from δ-CsPbI3 to the black cubic α-phase. The photoactive and metastable black γ-CsPbI3 is obtained via high-temperature annealing and rapid cooling under inert conditions. Optical characterizations have been performed in order to extrapolate a bandgap of 2.89 eV for the δ-phase and 1.62 eV for the γ-phase, while the photoluminescence analysis displays intense emissions at 530 and 700 nm for the δ- and γ-phase, respectively. Ambient photoemission spectroscopy further elucidates the energy levels of the γ-phase, determining a highest occupied molecular orbital energy of 5.68 eV and a work function of 4.32 eV. These findings demonstrate the possibility to synthesize pure CsPbI3 and obtain the γ-CsPbI3 phase with promising applications.

全无机卤化铅钙钛矿,包括碘化铯铅(CsPbI3),由于其固有的光电特性,在光伏、发光器件和其他光电技术中具有潜在的应用前景,引起了人们的广泛关注。本研究介绍了一种简单、绿色、可扩展的制备CsPbI3钙钛矿的溶液合成方法,利用β-二酮酸[Cs(hfa)]n和[Pb(hfa)2二莱肟]2前驱体和乙醇为溶剂。经x射线衍射和能量色散x射线分析证实,合成的纳米带最初以纯黄色δ相制备。差示扫描量热分析表明,δ-CsPbI3向黑色立方α-相转变为可逆相。在惰性条件下,通过高温退火和快速冷却制备了具有光活性和亚稳态的黑色γ-CsPbI3。光学表征表明,δ相和γ相的带隙分别为2.89 eV和1.62 eV,而光致发光分析显示,δ相和γ相分别在530 nm和700 nm处有强发射。环境光发射光谱进一步阐明了γ相的能级,确定了最高已占分子轨道能量为5.68 eV,功函数为4.32 eV。这些发现证明了合成纯CsPbI3和获得具有应用前景的γ-CsPbI3相的可能性。
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引用次数: 0
Implantable Nongenetic Optoelectronic Biointerfaces for Neuromodulation 用于神经调节的可植入非遗传光电生物接口
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-09-27 DOI: 10.1002/adpr.202500176
Jinglin Ye, Jinwei Huang, Wenyu Nie, Jianming Xu, Xing Sheng, Huachun Wang

Electroceuticals are a novel type of therapeutics that employ electrical stimulation to modulate neural circuits and recover impaired physiological functions. Traditional systems using implanted leads as electrode and/or connecting wires pose several clinical challenges, including infection risk, anatomical incompatibilities, and leads dislodgement. Recent progress in optoelectronic biointerfaces is establishing new paradigms for electroceutical intervention by enabling precise, minimally invasive, and nongenetic neuromodulation through light-driven wireless technologies. In this review, first, the modulation mechanism of representative organic and inorganic semiconductor-based optoelectronic biointerfaces is demonstrated, which can be designed into flexible and tissue-conforming architectures. Then, further their capabilities to modulate structures at various levels, including neurons, nerve tissues, and the cerebral cortex are emphasized. Beyond neuromodulation, their promising therapeutic value and translational potential are highlighted, encompassing vision restoration, nerve regeneration, and treatment of Parkinson's disease. Together, these advancements mark a transformative shift toward next-generation bioelectronic medicine.

电疗法是一种利用电刺激来调节神经回路和恢复受损生理功能的新型治疗方法。使用植入导线作为电极和/或连接导线的传统系统存在一些临床挑战,包括感染风险、解剖不兼容和导线脱位。光电生物接口的最新进展是通过光驱动无线技术实现精确、微创和非遗传性神经调节,为电干预建立新的范例。本文首先阐述了具有代表性的有机和无机半导体光电生物接口的调制机制,并将其设计成柔性和符合组织结构的结构。然后,进一步强调了它们在不同水平上调节结构的能力,包括神经元、神经组织和大脑皮层。除了神经调节外,它们的治疗价值和转化潜力也得到了强调,包括视力恢复、神经再生和帕金森病的治疗。总之,这些进步标志着下一代生物电子医学的转型转变。
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引用次数: 0
Modal Theory of Phase-Modulated and Frequency-Shifting Ring Cavities 调相移频环腔的模态理论
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-09-25 DOI: 10.1002/adpr.202500098
Miguel Cuenca, Haroldo Maestre, Carlos R. Fernández-Pousa

A theoretical and experimental characterization of the optical modes of dispersionless ring cavities incorporating phase modulators (PM) and/or frequency shifters (FS) is presented. Using linear operator theory, the exact response of these cavities to arbitrary modulating waveforms and optical inputs is computed and shown to be a filtering process that selects a certain class of fields, invariant under multiple roundtrips, which are identified with the cavity's optical modes. The different types of PM/FS cavity modes are analyzed. This approach also leads to a representation of these cavities as unmodulated resonators preceded and followed by complementary phase modulations, which are linearly related to the imparted intracavity phase modulation or frequency shift. The theory is experimentally validated by the external injection of engineered phase and frequency modulated cavity modes in an Er:fiber PM fiber loop, and also compared with the emission modes of frequency modulated lasers and continuous wave (CW) frequency shifted feedback lasers. These results provide a unified view for the linear analysis of systems employing PM/FS active cavities or resonators, of interest in the field of photonic signal generation and processing.

本文从理论和实验两方面对含相位调制器和/或移频器的无色散环形腔的光学模式进行了研究。利用线性算符理论,计算了这些腔对任意调制波形和光输入的精确响应,并证明了这是一个滤波过程,该过程选择了某类场,在多次往返下不变,这些场与腔的光学模式相识别。分析了不同类型的PM/FS型腔模态。这种方法还导致将这些腔表示为未调制谐振器,其前后是互补相位调制,这与所赋予的腔内相位调制或频移线性相关。通过在Er:光纤PM光纤环路中注入工程相位和调频腔模式,对该理论进行了实验验证,并与调频激光器和连续波(CW)移频反馈激光器的发射模式进行了比较。这些结果为采用PM/FS有源腔或谐振器的系统的线性分析提供了统一的观点,对光子信号的产生和处理领域感兴趣。
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引用次数: 0
Techniques and Advances in Ultrafast Photography 超快摄影技术与进展
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-09-24 DOI: 10.1002/adpr.202500184
Chen Huang, Xin Zhang, Renjie Han, Jiaoyu Fan, Hui Jiang, Yiwen Zhang, Jinghua Yu, Jiamin Wang, Yi Chen, Junjie Sun, Fei Chen

Ultrafast events, from the rapid propagation of shock waves to molecular vibrations and electron dynamics, can unfold on timescales as short as femtoseconds. Limited by the imaging speed of charge-coupled device and complementary metal-oxide-semiconductor sensors, conventional imaging systems cannot capture such high-speed phenomena. Researchers have developed various ultrafast photography techniques to address this challenge, incorporating electronic, mechanical, and optical methods to achieve imaging speed in the trillion frames per second. This review categorizes ultrafast photography into four types: multishot passive technique, multishot active technique, single-shot passive technique, and single-shot active technique. It examines the evolution from early mechanical and electronic high-speed cameras to modern optical and computational imaging. These innovations have broad applications in physics, chemistry, biology, and engineering, providing new insights into ultrafast dynamics. This review discusses the latest developments, compares key techniques, and explores future directions in ultrafast photography research.

超快事件,从冲击波的快速传播到分子振动和电子动力学,可以在短至飞秒的时间尺度上展开。受限于电荷耦合器件和互补金属氧化物半导体传感器的成像速度,传统的成像系统无法捕捉到这种高速现象。研究人员已经开发出各种超快摄影技术来应对这一挑战,结合电子、机械和光学方法来实现每秒万亿帧的成像速度。本文将超快摄影分为四种类型:多镜头被动技术、多镜头主动技术、单镜头被动技术和单镜头主动技术。它考察了从早期的机械和电子高速相机到现代光学和计算成像的演变。这些创新在物理、化学、生物和工程领域有着广泛的应用,为超快动力学提供了新的见解。本文综述了超快摄影的最新进展,比较了关键技术,并对未来的研究方向进行了展望。
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引用次数: 0
Topological Valley Photonic Waveguides: Scattering Matrix Evaluation for Linear Computing 拓扑谷光子波导:线性计算的散射矩阵评估
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-09-22 DOI: 10.1002/adpr.202500006
Christian Johnson-Richards, Alex Yakovlev, Victor Pacheco-Peña

Topological boundary modes utilizing valley mode waveguides have opened opportunities in, for instance, the design of high transmission waveguides with tolerance to geometrical defects and sharp bends. Applications of these waveguides include linear computational processes and the emulation of logic gates using linear structures, among other scenarios. Herein, the design of a 6-port junction that exhibits equal power splitting to three other ports when excited at single port with no reflections is presented. In studying this structure, a scattering matrix is extracted at telecom wavelengths (around 1550 nm). The linearity of the system along with the scattering matrix is exploited to produce linear operations such as routing of information considering two incident signals or multiple signals applied from different ports. These results may be exploited to analytically design larger networks without the need of computationally expensive trial and error methods.

利用谷模式波导的拓扑边界模式开辟了机会,例如,高透射波导的设计具有几何缺陷和尖锐弯曲的容错性。这些波导的应用包括线性计算过程和使用线性结构的逻辑门仿真,以及其他场景。本文提出了一种6端口结的设计,该结在单端口无反射激励时表现出与其他三个端口相等的功率分裂。在研究这种结构时,提取了电信波长(约1550 nm)的散射矩阵。利用系统的线性以及散射矩阵来产生线性运算,例如考虑两个入射信号或来自不同端口的多个信号的信息路由。这些结果可以用来分析设计更大的网络,而不需要计算昂贵的试验和错误方法。
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引用次数: 0
Displacement and Vibration Measurements with Interferometers: Benchmark Configurations, Performance, and R&D Opportunities 位移和振动测量与干涉仪:基准配置,性能和研发机会
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-09-22 DOI: 10.1002/adpr.202500193
Silvano Donati

Many different approaches have been proposed or published in recent years on the measurement of small vibrations and/or large-amplitude displacements by interferometers, either traditional or self-mixing type. Most of them start from procuring a pair of orthogonal signals cos 2kΔs and sin 2kΔs, where k = 2π/λ and Δs is the variation of target distance, from which to proceed to calculate the measurand Δs with the atan of the ratio followed by an unfolding operation. These attempts are commented on, and it is shown that it is not really necessary to add phase modulators or other extra optical components nor to use elaborate signal processing to obtain the orthogonal pair, because simple hardware solutions readily supply, without the cosine and sine pair, a resolution close to the quantum limit together with excellent dynamic range, precision, linearity, and bandwidth. The examples reported in this article establish a benchmark of performances that must be referred to in developing new approaches that make sense, also considering that such performances have been offered by commercial instruments for several decades.

近年来,人们提出或发表了许多不同的方法来测量干涉仪的小振动和/或大振幅位移,无论是传统的还是自混合型的。它们大多从获取一对正交信号cos 2kΔs和sin 2kΔs开始,其中k = 2π/λ, Δs为目标距离的变化量,以此为基础计算测量值Δs与比值的tan,然后进行展开运算。对这些尝试进行了评论,并表明实际上不需要添加相位调制器或其他额外的光学元件,也不需要使用复杂的信号处理来获得正交对,因为简单的硬件解决方案很容易提供接近量子极限的分辨率,而不需要余弦和正弦对,同时具有出色的动态范围,精度,线性度和带宽。本文中报告的例子建立了一个性能基准,在开发有意义的新方法时必须参考,同时考虑到这种性能已经由商业乐器提供了几十年。
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引用次数: 0
High-Energy Femtosecond All-Fiber Laser Systems in 1.7–1.8 μm Using a Normal-Dispersion Tm-Doped Fiber 使用正色散tm掺杂光纤的1.7 ~ 1.8 μm高能飞秒全光纤激光器
IF 3.9 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-09-18 DOI: 10.1002/adpr.202500068
Shaoxiang Chen, Hongjie Chen, Raghuraman Sidharthan, Yuhao Chen, Dingyuan Tang, Seongwoo Yoo

A W-type normal dispersion thulium-doped fiber (NDTDF) is utilized to generate high average power, high-energy femtosecond pulses at 1.7 μm region for bio-imaging applications. Net normal dispersion cavity fiber lasers are used to generate positively chirped soliton pulses, which are subsequently amplified through the NDTDF. Because of the normal dispersion of the Tm-doped silica fiber, the amplified pulses are able to be compressed using a conventional telecommunication fiber such as SMF-28. Hence, an all-fiber ultrafast laser source is constructed in the 1.7 μm wavelength region for deep tissue imaging applications. This paper reports ≈230 nJ, with its corresponding average power as high as 1.74 W. Further adjustment of dispersion in the all-fiber configuration allows the main pulse duration to be compressed to ≈200 fs. Core size scalability of the proposed W-type NDTDF has also been investigated.

利用w型正色散掺铥光纤(NDTDF)在1.7 μm区域产生高平均功率、高能量飞秒脉冲,用于生物成像应用。净法向色散腔光纤激光器用于产生正啁啾孤子脉冲,该脉冲随后通过NDTDF被放大。由于tm掺杂二氧化硅光纤的正常色散,放大的脉冲可以使用传统的电信光纤(如SMF-28)进行压缩。因此,在1.7 μm波长区域构建了用于深层组织成像的全光纤超快激光源。本文报道了≈230 nJ,对应的平均功率高达1.74 W。进一步调整色散在全光纤配置允许主脉冲持续时间被压缩到约200fs。研究了所提出的w型NDTDF的芯尺寸可扩展性。
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引用次数: 0
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Advanced Photonics Research
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