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Recent Advances in Molecular Engineering for Viologen-Based Electrochromic Materials: A Mini-Review 基于病毒的电致变色材料分子工程的最新进展:微型综述
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-12 DOI: 10.1002/adpr.202400016
Bebin Ambrose, Murugan Krishnan, Kalaivanan Ramamurthy, Murugavel Kathiresan

Viologens, with their unique redox-active properties, have garnered increasing attention in the development of electrochromic devices. This review focuses on key strategies in molecular design, synthesis methodologies, and tailored functionalities that have propelled the field forward from 2019 to the present. The convergence of these approaches has led to the construction of viologen-based electrochromic materials with enhanced performance, stability, and responsiveness. The review not only examines the current state of the field but also explores promising outlooks and opportunities, including tailored applications, environmental sustainability, and integration with emerging technologies. The synergy between molecular engineering and viologen-based electrochromic materials holds significant promise, shaping the future of dynamic, responsive materials in diverse technological domains. This review serves as a valuable resource for researchers, offering insights into recent breakthroughs and inspiring further advancements in this rapidly evolving field.

病毒原具有独特的氧化还原活性特性,在电致变色设备的开发中日益受到关注。本综述重点介绍分子设计、合成方法和定制功能方面的关键策略,这些策略推动了该领域从 2019 年至今的发展。这些方法的汇聚使得基于紫胶的电致变色材料的性能、稳定性和响应性得到了增强。本综述不仅研究了该领域的现状,还探讨了前景广阔的前景和机遇,包括定制应用、环境可持续性以及与新兴技术的整合。分子工程与基于紫胶的电致变色材料之间的协同作用前景广阔,将在不同技术领域塑造动态响应材料的未来。这篇综述为研究人员提供了宝贵的资源,让他们深入了解最近取得的突破,并激励他们在这一快速发展的领域取得更大的进步。
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引用次数: 0
Broadband Diffractive Neural Networks Enabling Classification of Visible Wavelengths 可对可见光波长进行分类的宽带衍射神经网络
IF 3.7 Pub Date : 2024-06-12 DOI: 10.1002/adpr.202470016
Ying Zhi Cheong, Litty Thekkekara, Madhu Bhaskaran, Blanca del Rosal, Sharath Sriram

Diffractive Neural Networks

In article number 2300310, Ying Zhi Cheong, Blanca del Rosal, Sharath Sriram, and co-workers propose and demonstrate a microscale multi-layer diffractive neural network approach that classifies various wavelengths in the visible spectrum. This miniaturised classification approach, achieved through two-photon polymerization, has potential application in medical diagnosis to material science, enabling rapid detection of analytes based on the presence of optical extinction bands at specific wavelengths.

衍射神经网络 在编号为 2300310 的文章中,Ying Zhi Cheong、Blanca del Rosal、Sharath Sriram 及其合作者提出并展示了一种微型多层衍射神经网络方法,可对可见光谱中的各种波长进行分类。这种通过双光子聚合实现的微型分类方法可应用于医疗诊断和材料科学领域,根据特定波长的光学消光带的存在情况快速检测分析物。
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引用次数: 0
Progress on Coherent Perovskites Emitters: From Light-Emitting Diodes under High Current Density Operation to Laser Diodes 相干 Perovskites 发射器的研究进展:从高电流密度下的发光二极管到激光二极管
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-12 DOI: 10.1002/adpr.202400033
Gayoung Lee, Yejin Jun, Hyeonji Lee, Kwangdong Roh

Perovskites exhibit appealing optical and electrical properties, making them attractive candidates for efficient luminescent materials with low-cost and straightforward fabrication processes. Their versatility is highlighted by the ability to deposit perovskite thin films on various substrates, including silicon, glass, sapphire, and flexible substrates, enabling potential monolithic integration on silicon for applications such as photonic integrated circuits, high-speed communication. Extensive studies on perovskite light-emitting diodes have shown external quantum efficiencies exceeding 20% across a wide spectral range from deep blue to near-infrared, with chirality. Additionally, perovskite-based lasing action has been achieved under pulsed optical excitation and continuous-wave operation, as well as in functional diode structures. However, realizing electrically driven perovskite laser diodes for practical applications requires the injection of intense current densities. This review provides a comprehensive overview of the historical progress in perovskite lasers and light-emitting didoes, along with important design considerations essential for their development.

过氧化物具有诱人的光学和电学特性,使其成为具有低成本和直接制造工艺的高效发光材料的理想候选材料。它们的多功能性突出表现在能够在各种基底(包括硅、玻璃、蓝宝石和柔性基底)上沉积包晶体薄膜,从而有可能在硅上实现单片集成,用于光子集成电路和高速通信等应用。对包晶石发光二极管的广泛研究表明,在从深蓝到近红外的宽光谱范围内,其外部量子效率超过 20%,并具有手性。此外,在脉冲光激发、连续波操作以及功能二极管结构中,都实现了基于磷灰石的激光作用。然而,要在实际应用中实现电驱动包晶体激光二极管,需要注入高密度的电流。本综述全面概述了包晶体激光器和发光二极管的历史进程,以及对其发展至关重要的重要设计考虑因素。
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引用次数: 0
Pressure-Induced Successive Phase Transitions and Optical Properties in Lu2SiO5 Lu2SiO5 中压力诱导的连续相变和光学特性
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-02 DOI: 10.1002/adpr.202300319
Wenming Qi, Anwar Hushur, Lin He, Rabigul Tursun, Min Gao

Herein, lutecium silicate is used as a rock example to investigate its two high-pressure phases (7.4 GPa: HP-II and 25.3 GPa: HP-III) and lattice dynamics by in situ high-pressure Raman scattering up to 35.1 GPa. The evidence for a highly symmetrical insulator HP-III phase is obtained. Importantly, the high-pressure structure (metastable phases) after pressure quenching is also intercepted, indicating pressure-induced permanent densification. These findings provide Raman evidence for pressure-induced successive phase transitions of highly symmetric insulators intercepted in prototype Lu2SiO5 and physical insights to explain the self-regulation of rare earth-rich regions in facilitating highly effective global carbon cycling.

本文以硅酸镥岩为例,通过高达 35.1 GPa 的原位高压拉曼散射研究其两种高压相(7.4 GPa:HP-II 和 25.3 GPa:HP-III)和晶格动力学。结果证明存在高度对称的绝缘体 HP-III 相。重要的是,还截获了压力淬火后的高压结构(可转移相),表明了压力诱导的永久致密化。这些发现为在原型 Lu2SiO5 中截取高度对称绝缘体的压力诱导连续相变提供了拉曼证据,并为解释富稀土区域在促进高效全球碳循环方面的自我调节提供了物理见解。
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引用次数: 0
Ultrafast Terahertz Superconductor Van der Waals Metamaterial Photonic Switch 超快太赫兹超导体范德华超材料光子开关
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-02 DOI: 10.1002/adpr.202400045
Kaveh Delfanazari

The high-temperature layered superconductor (HTS) BSCCO is one of the key quantum material platforms in THz science and technology. Compact, stable, and reliable BSCCO THz photonic integrated circuit components can be developed to effectively and efficiently control and manipulate THz wave radiation, especially for future communication systems and network applications. Herein, the design, simulation, and modeling of ultrafast THz metamaterial photonic integrated circuits are reported on a few nanometer-thick HTS BSCCO van der Waals (vdWs), capable of the active modulation of phase with constant transmission coefficient over a narrow-frequency range. Meanwhile, the metamaterial circuit works as an amplitude modulator without significantly changing the phase in a different frequency band. Under the application of ultrashort optical pulses, the transient modulation dynamics of the THz metamaterial offer a fast-switching timescale of 50 ps. The dynamics of picosecond light–matter interaction, Cooper pairs breaking, photoinduced quasiparticles generation and recombination, phonon bottleneck effect, and emission and relaxation of bosons in BSCCO vdW metamaterial arrays are discussed for the potential application of multifunctional superconducting photonic integrated circuits in communication and quantum technologies.

高温层状超导体(HTS)BSCCO 是太赫兹科学与技术领域的关键量子材料平台之一。开发紧凑、稳定、可靠的 BSCCO 太赫兹光子集成电路元件,可有效控制和操纵太赫兹波辐射,尤其适用于未来的通信系统和网络应用。本文报告了超快太赫兹超材料光子集成电路的设计、仿真和建模,该集成电路基于几纳米厚的 HTS BSCCO 范德华(vdWs),能够在窄频率范围内以恒定的传输系数主动调制相位。同时,超材料电路可作为振幅调制器工作,而不会在不同频段显著改变相位。在超短光脉冲的作用下,太赫兹超材料的瞬态调制动力学具有 50 ps 的快速切换时间尺度。本文讨论了 BSCCO vdW 超材料阵列中皮秒光物质相互作用、库珀对断裂、光诱导的准粒子产生和重组、声子瓶颈效应以及玻色子的发射和弛豫等动力学问题,以探讨多功能超导光子集成电路在通信和量子技术中的潜在应用。
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引用次数: 0
Coherent and Incoherent Breathing Solitons in a Bidirectional Ultrafast Thulium Fiber Laser 双向超快铥光纤激光器中的相干和非相干呼吸孤子
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-02 DOI: 10.1002/adpr.202400049
Yi Zhou, Jiqiang Kang, Kenneth K. Y. Wong

Mode-locked lasers are prone to exhibit a wide range of dynamics, including the coherent dissipative soliton with high robustness or the possible emission of incoherent pulse bursts. Herein, it is proposed to expand the notion of dissipative breathing solitons to incoherent localized formation, which is illustrated experimentally by reporting original coherent and incoherent breathing solitons generated in a 2 μm bidirectional ultrafast fiber laser. A real-time spectral characterization of the breathing soliton dynamics with different coherence is provided, highlighting salient features of the self-organization. The switching between coherent breathing soliton and noise-like pulse is also experimentally demonstrated, corresponding to the multiple transient decoherence and coherence recovery. High behavior similarity exists in bidirectional solitons evolution owing to the common gain and loss modulation. Numerical simulations using a discrete laser model validate the experimental findings. This research generalizes previous observations of breathing solitons made in the coherent case and opens up new possibilities for generating breathers in various dissipative systems.

模式锁定激光器容易表现出多种动态,包括具有高鲁棒性的相干耗散孤子或可能发射的非相干脉冲串。本文提出将耗散呼吸孤子的概念扩展到非相干局部形成,并通过实验报告了在 2 μm 双向超快光纤激光器中产生的原始相干和非相干呼吸孤子。实验提供了不同相干性呼吸孤子动态的实时光谱特征,突出了自组织的显著特点。实验还证明了相干呼吸孤子和噪声脉冲之间的切换,这与多重瞬态退相干和相干恢复相对应。由于共同的增益和损耗调制,双向孤子演化的行为具有高度相似性。使用离散激光模型进行的数值模拟验证了实验结果。这项研究推广了之前在相干情况下观察到的呼吸孤子,为在各种耗散系统中产生呼吸开辟了新的可能性。
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引用次数: 0
Vortex-Beam Multiplexing Emitter Using Advanced Manufactured Leaky Cables 使用先进制造泄漏电缆的涡束复用发射器
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-05-26 DOI: 10.1002/adpr.202400001
Feiyang Deng, Kwai-Man Luk, Wenjian Sun, Ka Fai Chan

Although orbital angular momentum (OAM) is extensively explored and researched in various scientific domains, its practical application in wireless communications still faces numerous challenges. Notably, existing OAM beam generation technologies need to meet the diversified demands of modern wireless communication, such as miniaturization, cost-effectiveness, and system integration. Driven by the immense potential of OAM in communication systems, in this work, an innovative method based on leaky cables capable of simultaneously generating multiple vortex beams, overcoming a series of implementation issues associated with multiplexing emitters, is introduced. A design prototype is fabricated and tested, and the measurement results align closely with the simulations, validating the multifunctionality and practicality of the method. Moreover, the proposed strategy can seamlessly extend to optical frequencies using the concept of leaky fibers. In this method, not only efficient spatial utilization and excellent isolation are realized but also high cost-effectiveness is possessed. Compared to previous strategies, this technique may have an impact on simplifying the establishment of communication system platforms based on OAM multiplexing.

虽然轨道角动量(OAM)在各个科学领域都得到了广泛的探索和研究,但其在无线通信领域的实际应用仍面临诸多挑战。值得注意的是,现有的轨道角动量波束生成技术需要满足现代无线通信的多样化需求,如微型化、成本效益和系统集成。鉴于 OAM 在通信系统中的巨大潜力,本文介绍了一种基于泄漏电缆的创新方法,该方法能够同时产生多个涡旋波束,克服了与多路发射器相关的一系列实施问题。我们制作并测试了设计原型,测量结果与模拟结果非常吻合,验证了该方法的多功能性和实用性。此外,利用泄漏光纤的概念,所提出的策略可以无缝扩展到光学频率。在这种方法中,不仅实现了高效的空间利用和出色的隔离,还具有很高的成本效益。与之前的策略相比,该技术可能会对简化基于 OAM 复用的通信系统平台的建立产生影响。
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引用次数: 0
All-Bands-Flat Floquet Topological Photonic Insulators with Microring Lattices 具有微oring 晶格的全带平面浮凸拓扑光子绝缘体
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-05-26 DOI: 10.1002/adpr.202400023
Hanfa Song, Vien Van

Coupled microring lattices are versatile photonic systems that can be used to realize various topological phases of matter. In two-dimensional (2D) microring lattices, the periodic and unidirectional circulation of light in each microring gives rise to a time-like dimension, so that the lattice emulates a (2 + 1)D system with much richer topological behaviors than static 2D lattices. Accurate treatment of these systems requires a departure from the static tight-binding model of coupled resonators and take into account the periodic coupling sequence of light in the lattice network. This article provides an overview of the theory and design of (2 + 1)D microring lattices for realizing Floquet topological photonic insulators (TPIs). Particular focus is placed on the microring Lieb lattice with perfect couplings, which emulates an anomalous Floquet insulator with all flat bands. Such a system exhibits some unique properties, including wide edge mode continuum exceeding a Floquet–Brillouin zone, super-robustness to lattice disorder, Aharonov–Bohm (AB) caging and compact localized flat-band states that can be used to realize high-quality factor topological resonators. All-bands-flat Floquet–Lieb microring lattices provide a versatile platform for investigating topological physics as well as potential applications in realizing topologically-protected photonic devices.

耦合微晶格是一种多功能光子系统,可用于实现物质的各种拓扑相。在二维(2D)微晶格中,光在每个微晶格中的周期性单向循环产生了类时间维度,因此晶格模拟了一个(2 + 1)D 系统,其拓扑行为比静态的 2D 晶格丰富得多。要准确处理这些系统,就必须摆脱耦合谐振器的静态紧束模型,并考虑到晶格网络中光的周期性耦合序列。本文概述了用于实现 Floquet 拓扑光子绝缘体 (TPI) 的 (2 + 1)D 微菱晶格的理论和设计。文章特别强调了具有完美耦合的微oring Lieb 晶格,它模拟了具有所有平带的反常 Floquet 绝缘体。这种系统表现出一些独特的特性,包括超过弗洛克-布里渊区的宽边缘模式连续性、对晶格无序的超稳健性、阿哈诺夫-玻姆(AB)笼和紧凑的局部平带态,可用于实现高质量因子拓扑谐振器。全带扁平 Floquet-Lieb 微oring 晶格为研究拓扑物理以及实现拓扑保护光子器件的潜在应用提供了一个多功能平台。
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引用次数: 0
Miura Origami-Inspired Reconfigurable Phase Gradient Metasurface for Linearly and Circularly Polarized Differential Modulation 用于线性和圆极化差分调制的三浦折纸启发式可重构相位梯度元面
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-05-23 DOI: 10.1002/adpr.202400025
Zhibiao Zhu, Yongfeng Li, Jiafu Wang, Lixin Jiang, Zhe Qin, Lin Zheng, Hongya Chen, Wenjie Wang, Shaobo Qu

Miura origami's reconfigurable characteristic and structural asymmetry, combined with electromagnetic (EM) wave manipulation, crashed a unique spark. However, the complexity of the three-dimensional (3D) origami structure after folding makes it challenging to study the phase regulation mechanism. Here, we propose a reconfigurable phase gradient metasurface based on Miura origami and derive the underlying mechanism of phase modulation in detail under linearly and circularly polarized (LP and CP) incidence. We adopt the one-dimensional (1D) gradient design along the x direction to verify the idea. The phase calculation formulas are given under LP and CP incidence through the Jones matrix's derivation. The beam deflector angles corresponding to LP and CP waves are identical in the planar state. As the folding angle increases, the phase evolution rules corresponding to the LP and CP waves are discrepant, leading to differential beam steering. Finally, the origami sample is processed for verification, and the experimental data are consistent with the simulation and theoretically calculated values. We believe this work can help analyze the EM behavior of complex 3D origami structures and lay a foundation for designing a multifunctional EM origami metasurface.

三浦折纸的可重构特性和结构不对称性与电磁波操纵相结合,碰撞出独特的火花。然而,折叠后的三维(3D)折纸结构非常复杂,这给研究相位调节机制带来了挑战。在此,我们提出了一种基于三浦折纸的可重构相位梯度元表面,并详细推导了在线性和圆极化(LP 和 CP)入射条件下相位调制的基本机制。我们采用沿 x 方向的一维(1D)梯度设计来验证这一想法。通过琼斯矩阵的推导,我们给出了 LP 和 CP 入射条件下的相位计算公式。在平面状态下,LP 波和 CP 波对应的光束偏转角是相同的。随着折叠角的增大,LP 波和 CP 波对应的相位演化规则出现差异,从而导致不同的光束转向。最后,对折纸样品进行了验证,实验数据与模拟值和理论计算值一致。我们相信这项工作有助于分析复杂三维折纸结构的电磁行为,并为设计多功能电磁折纸元表面奠定基础。
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引用次数: 0
Robustness and Tunability of Symmetric-Protected Bound States in the Continuums and Quasi-Bound States in the Continuums in Terahertz Metasurfaces 太赫兹元表面中连续体中的对称保护束缚态和连续体中的准束缚态的稳健性和可调谐性
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-05-23 DOI: 10.1002/adpr.202400020
Jie Ji, Binbin Zhou, Peter Bøggild, Shihab Al-Daffaie, Peter Uhd Jepsen, Jaime Gomez Rivas

Symmetry-protected bound states in the continuum (BICs), emerging at the Γ0$left(Gammaright)_{0}$ point in the Brillouin zone of periodic lattices of scatters, are robust optical modes under modifications in the lattice if the C2 symmetry (two fold rotational symmetry) is preserved. In this study, the manipulation of these symmetry-protected BIC and quasi-BIC modes in a system comprising two metallic rods per unit cell by adjusting their lateral separation and displacement is focused on. With non-symmetric systems under 180° rotation, two distinct coupling mechanisms resulting from changes in the lateral separation are investigated: the coupling of two half-wavelength (λ/2) resonances and the coupling of two surface lattice resonances (SLRs). Notably, symmetric structures with minimal lateral separation cannot sustain BIC modes owing to the near-field coupling between the rods. However, when the lateral separation is sufficiently large, the existence of a BIC mode supported by an SLR remains robust even with positional shifts. Furthermore, increasing the lateral separation and the shift displacement between the rods in asymmetric systems induces a redshift and a blueshift in the quasi-BIC mode, respectively. This shift is attributed to the near-field coupling effect between two rods, enabling the tunability of the resonance frequency with a high-quality factor.

连续体中受对称保护的束缚态(BIC)出现在周期性散射晶格的布里渊区中的点上,如果 C2 对称性(两折旋转对称性)得以保留,那么这些束缚态在晶格改变的情况下是稳健的光学模式。在本研究中,重点研究了在一个由每个单元格中的两根金属棒组成的系统中,通过调整它们的横向分离和位移来操纵这些受对称保护的 BIC 和准 BIC 模式。在旋转 180° 的非对称系统中,研究了横向分离变化导致的两种不同耦合机制:两个半波长 (λ/2) 共振的耦合和两个表面晶格共振 (SLR) 的耦合。值得注意的是,由于棒之间的近场耦合,横向间隔最小的对称结构无法维持 BIC 模式。然而,当横向间距足够大时,由 SLR 支持的 BIC 模式即使在位置偏移的情况下也能保持稳定。此外,在不对称系统中,增加棒之间的横向间距和位移位移会分别引起准 BIC 模式的红移和蓝移。这种位移归因于两根棒之间的近场耦合效应,使共振频率的可调谐性达到了高质量系数。
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引用次数: 0
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Advanced Photonics Research
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