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Octave‐Spanning Second‐Harmonic Generation in Dispersion‐Engineered Lithium Niobate‐on‐Insulator Microwaveguide 弥散工程铌酸锂绝缘体微波导管中的倍频程二次谐波生成
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-07-10 DOI: 10.1002/adpr.202400051
Yongzhi Tang, Tingting Ding, Yuting Zhang, Wenjun Ding, Yiwen Huang, Jiayu Wang, Hao Li, Shijie Liu, Yuanlin Zheng, Xianfeng Chen
Broadband lasers, e.g., ultrashort lasers, optical supercontinuum, and frequency combs, are revolutionary coherent light sources, which enable a plethora of state‐of‐the‐art applications ranging from precision spectroscopy to optical clocks. However, the spectral broadening of these coherent light sources mainly relies on the third‐order nonlinearity () and is difficult to extend to the visible or shorter wavelength regime. Second‐order nonlinearity (), which is orders of magnitude larger than , becomes a powerful tool for the frequency translation if its broadband operation is well addressed. Herein, an octave‐spanning second‐harmonic generation scheme is experimentally demonstrated beyond an extremely large frequency range of 135 THz and high conversion efficiency of 1% for sub‐100 pJ for the near‐infrared picosecond supercontinuum in a fiber–waveguide–fiber configuration. The process relies on ultrabroadband birefringence phase matching in the dispersion‐engineered lithium niobate‐on‐insulator ridge microwaveguide. The mode area of microwaveguide well matches with single‐mode lens fiber, reducing coupling loss and ensuring easy packaging. The method provides a new approach to span the wavelength range of coherent light with ‐based wavelength translation for supercontinuum or frequency combs into the visible regime. The result would find applications in spectroscopy, astrophysics, atomic optics, optical synthesis, etc.
宽带激光器,如超短激光器、光学超连续激光器和频率梳,是革命性的相干光源,可实现从精密光谱学到光学时钟等大量最先进的应用。然而,这些相干光源的光谱增宽主要依赖于三阶非线性(),很难扩展到可见光或更短的波长范围。二阶非线性()比三阶非线性()大几个数量级,如果能很好地解决其宽带运行问题,二阶非线性()将成为频率转换的有力工具。在此,实验证明了一种倍频程跨二次谐波生成方案,其频率范围超过 135 太赫兹,在光纤波导-光纤配置中,近红外皮秒超连续的转换效率高达 1%,低于 100 pJ。该工艺依赖于色散工程铌酸锂-绝缘体脊微波导管中的超宽带双折射相位匹配。微波导管的模式区与单模透镜光纤匹配良好,从而降低了耦合损耗,并确保了封装的简易性。该方法为跨越相干光的波长范围提供了一种新方法。其结果将应用于光谱学、天体物理学、原子光学、光学合成等领域。
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引用次数: 0
Broadband Quantum Efficiency Enhancement of Al0.3InAsSb p–i–n Photodiodes with All-Dielectric Amorphous Germanium Metasurfaces 具有全介电非晶锗金属表面的 Al0.3InAsSb pi-n 光电二极管的宽带量子效率提升
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-07-10 DOI: 10.1002/adpr.202400090
Dongxia Wei, Bingtian Guo, Adam A. Dadey, J. Andrew McArthur, Junwu Bai, Seth R. Bank, Joe C. Campbell

Transparent amorphous germanium (a-Ge) has emerged as a promising material for engineering nanostructures and metasurfaces, offering significant potential for enhancing the performance of photonic devices in the short-wavelength infrared (SWIR) spectrum. Herein, the successful application of a-Ge metasurfaces with a truncated pyramid profile to enhance the external quantum efficiency (EQE) of a digital alloy Al0.3InAsSb p–i–n photodiode across a broad-wavelength range in the SWIR is presented. The experimental findings demonstrate a broadband enhancement in EQE. Two metasurface samples are designed to emphasize different-wavelength ranges. Notably, 51% improvement in EQE at 1550 nm and 125% enhancement at 2000 nm is achieved. Finite-difference time domain simulations show that the observed EQE improvement originates from the reduction of reflection and electromagnetic field enhancement. This study underscores the promising role of a-Ge metasurfaces in advancing the capabilities of SWIR photodetectors. It lays the groundwork for further exploration in optoelectronic device enhancements.

透明非晶锗(a-Ge)已成为一种前景广阔的工程纳米结构和元表面材料,为提高短波红外(SWIR)光谱中光子器件的性能提供了巨大潜力。本文介绍了成功应用具有截断金字塔轮廓的 a-Ge 元表面来提高数字合金 Al0.3InAsSb pi-n 光电二极管在 SWIR 宽波长范围内的外部量子效率 (EQE)。实验结果表明 EQE 具有宽带增强效果。设计了两个元表面样品来强调不同的波长范围。值得注意的是,在 1550 nm 波长处,EQE 提高了 51%,在 2000 nm 波长处,EQE 提高了 125%。有限差分时域模拟表明,所观察到的 EQE 改善源于反射的减少和电磁场的增强。这项研究强调了 a-Ge 元表面在提高 SWIR 光电探测器性能方面的重要作用。它为进一步探索光电器件的增强奠定了基础。
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引用次数: 0
Active Full‐Color Generation Based on a Liquid Crystal‐Integrated Plasmonic Metasurface 基于液晶集成等离子体元表面的有源全彩发生器
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-07-09 DOI: 10.1002/adpr.202300334
Dewang Huo, Guoqiang Li
Structural colors based on metasurfaces outperform traditional pigments and dyes in terms of nonfading, high spatial resolution, and high stability, usually incorporating active materials for tunability. Liquid crystals (LCs) are suitable for tunable structural color design due to their large birefringence and fast modulation by external stimuli. However, most LC‐integrated structural colors focus on tailoring the polarization angle of incident light to generate two colors and their mixing. Herein, a scheme of full‐color generation based on a plasmonic metasurface integrated with LCs utilizing the combination of the polarization angle rotation effect of the twisted‐nematic LCs and the refractive index modulation through the realignment of the LCs near the metasurface is demonstrated. Based on the proposed structural color method, full‐color generation of a record color gamut of 60.7% standard Red Green Blue region, equivalent to 43% National Television Standards Committee area, in the LC‐integrated metasurface, has been numerically realized by tuning the bias voltage of the LCs in reflection. The achieved color gamut is nearly 4 times wider than the previously reported result. The proposed active full‐color generation metasurface shows great potential in applications for low‐power reflective color display, anticounterfeiting, and optical encoding.
基于超表面的结构色彩在不褪色、高空间分辨率和高稳定性方面优于传统颜料和染料,通常还包含可调活性材料。液晶(LC)具有较大的双折射和快速受外部刺激调制的特性,因此适合用于可调结构色设计。然而,大多数集成了液晶的结构颜色都侧重于调整入射光的偏振角,以产生两种颜色及其混合。在此,我们展示了一种基于集成了 LC 的等离子体元表面的全色生成方案,该方案利用了扭曲向列 LC 的偏振角旋转效应和通过元表面附近 LC 的重新配置实现的折射率调制效应。基于所提出的结构色彩方法,通过在反射过程中调整 LC 的偏置电压,在 LC 集成的元表面上全彩生成了 60.7% 标准红绿蓝区域的创纪录色域,相当于 43% 的国家电视标准委员会区域。所实现的色域比之前报告的结果宽近 4 倍。所提出的有源全彩生成元表面在低功耗反射式彩色显示、防伪和光学编码等应用中显示出巨大的潜力。
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引用次数: 0
Silicon-Based 850 nm GaAs/GaAsP-Strained Quantum Well Lasers with Active Region Dislocation Blocking Layers 具有有源区位错阻挡层的硅基 850 nm GaAs/GaAsP 应变量子阱激光器
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-07-08 DOI: 10.1002/adpr.202470018
Jian Li, Chen Jiang, Hao Liu, Yang Zhang, Hao Zhai, Xin Wei, Qi Wang, Gang Wu, Chuanchuan Li, Xiaomin Ren

Quantum Well Lasers

Benefitting from the interaction of the GaAs/GaAsP strained quantum well and InAlAs active region dislocation blocking layer, in article number 2300348, Jian Li and co-workers show that the threading dislocation penetration to the quantum well region of the silicon-based quantum well lasers can be bended and blocked. By the introduction of this strain compensate stress control structure, the 850 nm room temperature continuous wave emitting silicon-based quantum well laser exhibits a 94.2 mW power output, a 715 Acm–2 threshold current density, and enhanced reliability.

量子阱激光器 得益于 GaAs/GaAsP 应变量子阱和 InAlAs 有源区位错阻挡层的相互作用,在文章编号 2300348 中,李健和合作者展示了可以弯曲和阻挡穿透到硅基量子阱激光器量子阱区的穿线位错。通过引入这种应变补偿应力控制结构,850 nm 室温连续波发射硅基量子阱激光器显示出 94.2 mW 的功率输出、715 Acm-2 的阈值电流密度和更高的可靠性。
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引用次数: 0
A Review: Active Tunable Terahertz Metamaterials 综述:有源可调谐太赫兹超材料
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-07-08 DOI: 10.1002/adpr.202470020
Jining Li, Jiyue Chen, Dexian Yan, Fei Fan, Kai Chen, Kai Zhong, Yuye Wang, Zhen Tian, Degang Xu

Active Tunable Terahertz Metamaterials

Metamaterials give terahertz technology a broader application prospect. Active control ability of terahertz metamaterials is highly valuable and captivating. In article number 2300351, Kai Chen, Degang Xu, and co-workers categorize four basic types of tunable terahertz metamaterials based on external stimuli. Mechanical modulation offers simple yet efficient modulation, while electrical and magnetic modulation provide convenient adjustment. Moreover, optical modulation focuses on incorporating various materials to high-speed control.

主动可调谐太赫兹超材料 超材料为太赫兹技术带来了更广阔的应用前景。太赫兹超材料的主动控制能力极具价值和魅力。在文章编号 2300351 中,陈凯、徐德刚及其合作者根据外部刺激将可调谐太赫兹超材料分为四种基本类型。机械调制提供了简单而高效的调制,而电调制和磁调制则提供了方便的调节。此外,光学调制侧重于结合各种材料进行高速控制。
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引用次数: 0
Key Factors in Achieving High Responsivity for Graphene-Based Terahertz Detection 实现石墨烯基太赫兹检测高响应度的关键因素
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-27 DOI: 10.1002/adpr.202300272
Long Xiao, Riccardo Degl’Innocenti, Zhiping Wang

Terahertz (THz) radiation is highly promising for various applications, from industrial inspections to medical diagnoses. Given the typically ultralow-level power of generated THz radiation, the achievement of high responsivity in THz detection stands as a critical imperative for its applications. Graphene-based detectors have become an attractive choice for THz detection due to the graphene unique 2D material structure, allowing a broad absorption spectrum and ultrafast response. Various plasmonic antenna arrays are also employed to couple with graphene, compensating for its modest optical absorption. However, the configuration of the plasmonic antenna arrays plays a crucial role in THz detection as it determines the graphene physical mechanisms of photodetection, directly impacting the final responsivity. Here, the key factors for achieving high responsivity are investigated and it is presented that reducing the gap size of the plasmonic antenna arrays to the nanoscale and implementing a series-connection configuration can result in a remarkable increase in responsivity, often by several orders of magnitude. Importantly, this approach effectively prevents short circuits and minimizes dark current, further enhancing the overall performance of the detection system.

从工业检测到医疗诊断,太赫兹(THz)辐射在各种应用领域都大有可为。由于产生的太赫兹辐射通常具有超低功率,因此在太赫兹检测中实现高响应率是其应用的关键所在。由于石墨烯独特的二维材料结构具有宽广的吸收光谱和超快的响应速度,因此基于石墨烯的探测器已成为太赫兹检测的一个极具吸引力的选择。各种等离子体天线阵列也被用来与石墨烯耦合,以补偿其适度的光学吸收。然而,质子天线阵列的配置在太赫兹探测中起着至关重要的作用,因为它决定了石墨烯光电探测的物理机制,直接影响最终的响应率。本文对实现高响应率的关键因素进行了研究,结果表明,将等离子天线阵列的间隙尺寸减小到纳米级并采用串联配置可显著提高响应率,通常可提高几个数量级。重要的是,这种方法能有效防止短路并将暗电流降至最低,从而进一步提高检测系统的整体性能。
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引用次数: 0
A Two-Stage Polymerization Strategy for Preparing Polymer-Network Liquid Crystals with Oxygen-Sensing Property 制备具有氧传感特性的聚合物网络液晶的两阶段聚合策略
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-27 DOI: 10.1002/adpr.202300340
Zongdai Liu, Zhibo Zhang, Yi Zhang, Dan Luo, Kun-Lin Yang

Polymer-network liquid crystal (PNLC) possesses both advantages of low-molecular-weight liquid crystal (LMWLC) and liquid crystal (LC) polymer. Herein, a two-stage polymerization strategy for the formation of unique PNLC with oxygen-sensing properties is reported. The reaction mixture consists of 6% diacrylate RM257, 93.5% LMWLC 4-cyano-4′-pentylbiphenyl (5CB), and 0.5% photoinitiator dimethoxy-2-phenylacetophenone (DMPA). In the first stage, the mixture is exposed to UV light for 2 min to form a primary polymer network, which is highly uniform with a planar orientation. However, some free radicals are trapped inside the LC due to the short UV exposure time. Subsequently, the trapped free radicals are released by heating the PNLC sample into an isotropic state. Under this condition, the free radicals can move freely and react with surrounding monomers to form a secondary polymer network, which is highly disordered and scatters light strongly. Because oxygen can deactivate free radicals trapped inside the PNLC, the phenomenon to detect oxygen and monitor the diffusion of oxygen through the PNLC is exploited. The PNLC-based oxygen sensor is potentially useful for the detection of oxygen and monitoring the exposure time to oxygen.

聚合物网络液晶(PNLC)兼具低分子量液晶(LMWLC)和液晶聚合物(LC)的优点。本文报告了一种两阶段聚合策略,用于形成具有氧传感特性的独特 PNLC。反应混合物由 6% 的二丙烯酸酯 RM257、93.5% 的 LMWLC 4-氰基-4′-戊基联苯(5CB)和 0.5% 的光引发剂二甲氧基-2-苯基苯乙酮(DMPA)组成。在第一阶段,将混合物暴露在紫外线下 2 分钟,以形成高度均匀且具有平面取向的初级聚合物网络。然而,由于紫外线照射时间较短,一些自由基被截留在 LC 内。随后,将 PNLC 样品加热至各向同性状态,被截留的自由基就会被释放出来。在这种情况下,自由基可以自由移动,并与周围的单体发生反应,形成高度无序且散射光强的二次聚合物网络。由于氧气可以使 PNLC 内的自由基失活,因此可以利用这一现象检测氧气并监测氧气在 PNLC 中的扩散。基于 PNLC 的氧气传感器可用于检测氧气和监测氧气暴露时间。
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引用次数: 0
Enhancement of Quantum Efficiency in Perovskite Solar Cells Through Whispering Gallery Modes from Titanium Oxide Micro-Resonators 通过氧化钛微谐振器的耳语画廊模式提高 Perovskite 太阳能电池的量子效率
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-27 DOI: 10.1002/adpr.202300339
Ayusmin Panda, Chandran Sudakar, Birabar Ranjit Kumar Nanda
<p>With the aid of 3D full-field finite difference time–domain simulations, model configurations for <span></span><math> <semantics> <mrow> <msub> <mrow> <mtext>CsPbI</mtext> </mrow> <mn>3</mn> </msub> </mrow> <annotation>$left(text{CsPbI}right)_{3}$</annotation> </semantics></math> thin-film solar cell devices that include periodically arranged <span></span><math> <semantics> <mrow> <msub> <mrow> <mtext>TiO</mtext> </mrow> <mn>2</mn> </msub> </mrow> <annotation>$left(text{TiO}right)_{2}$</annotation> </semantics></math> microspheres, exhibiting resonating whispering gallery modes (WGMs), are proposed. The <span></span><math> <semantics> <mrow> <msub> <mrow> <mtext>TiO</mtext> </mrow> <mn>2</mn> </msub> </mrow> <annotation>$left(text{TiO}right)_{2}$</annotation> </semantics></math> microspheres present, either immersed in perovskite or coated with perovskite layer, between the electron- and hole-transport layers show enhanced current-conversion efficiency. The presence of WGMs lead to enhancement in the absorption of <span></span><math> <semantics> <mrow> <msub> <mrow> <mtext>CsPbI</mtext> </mrow> <mn>3</mn> </msub> </mrow> <annotation>$left(text{CsPbI}right)_{3}$</annotation> </semantics></math> layer. The incoming electromagnetic wave couples with <span></span><math> <semantics> <mrow> <msub> <mrow> <mtext>TiO</mtext> </mrow> <mn>2</mn> </msub> </mrow> <annotation>$left(text{TiO}right)_{2}$</annotation> </semantics></math> microsphere and forms confined resonating modes. Different designs are examined for deciding the appropriate position of WGM exhibiting spheres with respect to thin-film perovskite solar cell (PSC) featuring back reflector and optimized antireflectance coating. Since the incoupling element is lossless, energy stored in microspheres is absorbed efficiently by the underlying active material. This directly contributes to the
借助三维全场有限差分时域模拟,我们提出了 CsPbI 3 $left(text{CsPbI}right)_{3}$ 薄膜太阳能电池器件的模型配置,其中包括周期性排列的 TiO 2 $left(text{TiO}right)_{2}$ 微球,这些微球表现出共振耳语廊模式 (WGM)。在电子传输层和空穴传输层之间的 TiO 2 $left(text{TiO}right)_{2}$微球,无论是浸没在包晶石中还是包覆在包晶石层上,都显示出更高的电流转换效率。WGM 的存在增强了 CsPbI 3 $left(text{CsPbI}right)_{3}$层的吸收。传入的电磁波与 TiO 2 微球耦合,形成封闭的共振模式。我们研究了不同的设计,以决定 WGM 显示球与具有背反射器和优化抗反射涂层的薄膜过氧化物太阳能电池(PSC)的适当位置。由于耦合元件是无损耗的,微球中储存的能量会被底层活性材料有效吸收。这直接提高了太阳能电池的电流密度。因此,在相同厚度的过氧化物层下,该装置的电流密度高达 23.62 mA cm-1,而平面太阳能电池装置的电流密度为 13.68 mA cm-1。这使得短路电流密度比尺寸相似的传统 PSCs 器件提高了 70% 以上。
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引用次数: 0
Terahertz Pseudo-Waveform-Selective Metasurface Absorber Based on a Square-Patch Structure Loaded with Linear Circuit Components 基于加载线性电路元件的方形贴片结构的太赫兹伪波形选择性元表面吸收器
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-27 DOI: 10.1002/adpr.202300303
Yongzhi Cheng, Rui Xing, Fu Chen, Hui Luo, Ashif Aminulloh Fathnan, Hiroki Wakatsuchi

In recent years, metasurfaces composed of lumped nonlinear circuits have been reported to exhibit the capability of detecting specific electromagnetic waves, even when the waves are of the same frequency, depending on their respective waveforms or, more precisely, their pulse widths. Herein, three types of metasurface absorbers (MSAs) are presented which are composed of a square-patch structure loaded with linear circuit components, including lumped resistors or resistors in parallel with capacitors/inductors, which can mimic the waveform-selective absorption behavior in the terahertz (THz) region. By judiciously selecting suitable values for the linear circuit components, these MSAs can achieve near-perfect absorption of incident continuous waves or longer pulses while exhibiting reduced absorption of short pulses at the same THz frequency. These linear circuit structures can be referred to as pseudo-waveform-selective MSAs because their waveform-selective absorption characteristics are primarily derived from the dispersion behavior of the resonator structures, as opposed to the frequency conversion commonly observed in nonlinear circuits. These outcomes and discoveries introduce an additional degree of freedom for waveform discrimination in the THz frequency range, potentially enabling a broader range of applications, including but not limited to detection, sensing, and wireless communication.

近年来,有报道称由叠加非线性电路组成的元表面具有探测特定电磁波的能力,即使这些电磁波的频率相同,这取决于它们各自的波形,或者更准确地说,取决于它们的脉冲宽度。本文介绍了三种类型的元表面吸收器(MSA),它们由加载线性电路元件的方形贴片结构组成,包括叠加电阻器或与电容器/电感器并联的电阻器,可模仿太赫兹(THz)区域的波形选择性吸收行为。通过明智地为线性电路元件选择合适的值,这些 MSA 可以实现对入射连续波或较长的脉冲近乎完美的吸收,同时在相同的太赫兹频率下表现出对短脉冲的吸收减弱。这些线性电路结构可称为伪波形选择 MSA,因为它们的波形选择吸收特性主要来自谐振器结构的色散行为,而非非线性电路中常见的频率转换。这些成果和发现为太赫兹频率范围内的波形分辨带来了额外的自由度,有可能实现更广泛的应用,包括但不限于探测、传感和无线通信。
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引用次数: 0
Silicon-Based 850 nm GaAs/GaAsP-Strained Quantum Well Lasers with Active Region Dislocation Blocking Layers 具有有源区位错阻挡层的硅基 850 nm GaAs/GaAsP 应变量子阱激光器
IF 3.7 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-19 DOI: 10.1002/adpr.202300348
Jian Li, Chen Jiang, Hao Liu, Yang Zhang, Hao Zhai, Xin Wei, Qi Wang, Gang Wu, Chuanchuan Li, Xiaomin Ren

A silicon-based room temperature (RT) continuous wave (CW) operation quantum well (QW) laser emitting at 850 nm is reported in this article. By applying the dislocation filter superlattice, the threading dislocation density of the GaAs pseudosubstrate on Si is reduced to 1.8 × 107 cm−2. The metal-organic chemical vapor deposition-grown laser structure with GaAs/GaAsP QW and InAlAs active region dislocation blocking layer are fabricated into broad-stripe Fabry–Perot laser diodes. A typical threshold current and threshold current density of 286 mA and 715 Acm−2 are obtained with 2 mm cavity length and 20 um stripe width samples. A 94.2 mW single-facet output power lasing around 854 nm and a 0.314 WA−1 slope efficiency is measured under RT CW operation. After a 10-min aging process, the tested laser can operate stably under continuous operation conditions at RT and the lifetime can be approximated using an exponential fitting curve, indicating a good life reliability of this QW laser.

本文报告了一种发射波长为 850 nm 的硅基室温(RT)连续波(CW)工作量子阱(QW)激光器。通过应用位错滤波器超晶格,硅基砷化镓伪基底的穿线位错密度降低到 1.8 × 107 cm-2。金属有机化学气相沉积生长的激光结构带有 GaAs/GaAsP QW 和 InAlAs 有源区位错阻挡层,被制作成宽条纹法布里-珀罗激光二极管。2 毫米腔长和 20 微米条纹宽度样品的典型阈值电流和阈值电流密度分别为 286 mA 和 715 Acm-2。在实时连续波工作条件下,测量到在 854 纳米附近有 94.2 mW 的单面输出功率和 0.314 WA-1 的斜率效率。经过 10 分钟的老化过程后,测试激光器可以在 RT 连续工作条件下稳定运行,其寿命可以用指数拟合曲线来近似估算,这表明这种 QW 激光器具有良好的寿命可靠性。
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引用次数: 0
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Advanced Photonics Research
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